Three-dimensional ordered phosphotungstic acid/TiO

A series of phosphotungstic acid (HPW)/TiO2 materials with three-dimensional continuous and ordered macroporous structure, ranging from 130 nm to 300 nm in size, are synthesized by colloidal crystal templates and used as catalysts for oxidative desulfurization (ODS) of model oil. The structure and p...
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Gespeichert in:

Autor*in:	Yue, Du [verfasserIn] Lei, Jiaheng [verfasserIn] Peng, Yang [verfasserIn] Li, Junsheng [verfasserIn] Du, Xiaodi [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2018

Schlagwörter:	3DOM structure Phosphotungstic acid Oxidative desulfurization

Übergeordnetes Werk:	Enthalten in: Fuel - New York, NY [u.a.] : Elsevier, 1970, 226, Seite 148-155
Übergeordnetes Werk:	volume:226 ; pages:148-155

DOI / URN:	10.1016/j.fuel.2018.03.106

Katalog-ID:	ELV001327801

Internformat


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024	7		\|a 10.1016/j.fuel.2018.03.106 \|2 doi
035			\|a (DE-627)ELV001327801
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245	1	0	\|a Three-dimensional ordered phosphotungstic acid/TiO
264		1	\|c 2018
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337			\|a Computermedien \|b c \|2 rdamedia
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520			\|a A series of phosphotungstic acid (HPW)/TiO2 materials with three-dimensional continuous and ordered macroporous structure, ranging from 130 nm to 300 nm in size, are synthesized by colloidal crystal templates and used as catalysts for oxidative desulfurization (ODS) of model oil. The structure and properties of 3DOM HPW/TiO2 catalysts are characterized by powder X-ray diffraction (XRD), scanning electron microscope (SEM), transmission electron microscopy (TEM), N2 adsorption–desorption isotherms, inductively coupled plasma-optical emission spectrophotometer (ICP) and fourier transform infrared spectra (FT-IR). Characterization results demonstrate that all the HPW/TiO2 samples possess a large BET surface area and three-dimensional ordered macroporous structure with Keggin-type HPW dispersed homogeneously in TiO2 framework. 3DOM HPW/TiO2 with an average pore diameter around 250 nm presents the highest catalytic activity for dibenzothiophene (DBT), which can be attributed to the combination of its large enough macropores allowing for efficient mass transport and its high surface area enabling sufficient exposure of catalytic active sites. Furthermore, the catalyst is recovered and reused for seven runs with no obviously decrease in catalytic activity.
650		4	\|a 3DOM structure
650		4	\|a Phosphotungstic acid
650		4	\|a Oxidative desulfurization
700	1		\|a Lei, Jiaheng \|e verfasserin \|4 aut
700	1		\|a Peng, Yang \|e verfasserin \|4 aut
700	1		\|a Li, Junsheng \|e verfasserin \|4 aut
700	1		\|a Du, Xiaodi \|e verfasserin \|4 aut
773	0	8	\|i Enthalten in \|t Fuel \|d New York, NY [u.a.] : Elsevier, 1970 \|g 226, Seite 148-155 \|h Online-Ressource \|w (DE-627)300898584 \|w (DE-600)1483656-7 \|w (DE-576)09555176X \|x 0016-2361 \|7 nnns
773	1	8	\|g volume:226 \|g pages:148-155
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912			\|a GBV_ILN_24
912			\|a GBV_ILN_31
912			\|a GBV_ILN_32
912			\|a GBV_ILN_40
912			\|a GBV_ILN_60
912			\|a GBV_ILN_62
912			\|a GBV_ILN_63
912			\|a GBV_ILN_65
912			\|a GBV_ILN_69
912			\|a GBV_ILN_70
912			\|a GBV_ILN_73
912			\|a GBV_ILN_74
912			\|a GBV_ILN_90
912			\|a GBV_ILN_95
912			\|a GBV_ILN_100
912			\|a GBV_ILN_105
912			\|a GBV_ILN_110
912			\|a GBV_ILN_150
912			\|a GBV_ILN_151
912			\|a GBV_ILN_224
912			\|a GBV_ILN_370
912			\|a GBV_ILN_602
912			\|a GBV_ILN_702
912			\|a GBV_ILN_2003
912			\|a GBV_ILN_2004
912			\|a GBV_ILN_2005
912			\|a GBV_ILN_2006
912			\|a GBV_ILN_2008
912			\|a GBV_ILN_2010
912			\|a GBV_ILN_2011
912			\|a GBV_ILN_2014
912			\|a GBV_ILN_2015
912			\|a GBV_ILN_2020
912			\|a GBV_ILN_2021
912			\|a GBV_ILN_2025
912			\|a GBV_ILN_2027
912			\|a GBV_ILN_2034
912			\|a GBV_ILN_2038
912			\|a GBV_ILN_2044
912			\|a GBV_ILN_2048
912			\|a GBV_ILN_2049
912			\|a GBV_ILN_2050
912			\|a GBV_ILN_2056
912			\|a GBV_ILN_2059
912			\|a GBV_ILN_2061
912			\|a GBV_ILN_2064
912			\|a GBV_ILN_2065
912			\|a GBV_ILN_2068
912			\|a GBV_ILN_2088
912			\|a GBV_ILN_2111
912			\|a GBV_ILN_2112
912			\|a GBV_ILN_2113
912			\|a GBV_ILN_2118
912			\|a GBV_ILN_2122
912			\|a GBV_ILN_2129
912			\|a GBV_ILN_2143
912			\|a GBV_ILN_2147
912			\|a GBV_ILN_2148
912			\|a GBV_ILN_2152
912			\|a GBV_ILN_2153
912			\|a GBV_ILN_2190
912			\|a GBV_ILN_2336
912			\|a GBV_ILN_2470
912			\|a GBV_ILN_2507
912			\|a GBV_ILN_2522
912			\|a GBV_ILN_4035
912			\|a GBV_ILN_4037
912			\|a GBV_ILN_4046
912			\|a GBV_ILN_4112
912			\|a GBV_ILN_4125
912			\|a GBV_ILN_4126
912			\|a GBV_ILN_4242
912			\|a GBV_ILN_4251
912			\|a GBV_ILN_4305
912			\|a GBV_ILN_4313
912			\|a GBV_ILN_4322
912			\|a GBV_ILN_4323
912			\|a GBV_ILN_4324
912			\|a GBV_ILN_4326
912			\|a GBV_ILN_4333
912			\|a GBV_ILN_4334
912			\|a GBV_ILN_4335
912			\|a GBV_ILN_4338
912			\|a GBV_ILN_4393
936	b	k	\|a 58.21 \|j Brennstoffe \|j Kraftstoffe \|j Explosivstoffe
951			\|a AR
952			\|d 226 \|h 148-155

Indexfelder

author_variant	d y dy j l jl y p yp j l jl x d xd
matchkey_str	article:00162361:2018----::hedmninlreepopou
hierarchy_sort_str	2018
bklnumber	58.21
publishDate	2018
allfields	10.1016/j.fuel.2018.03.106 doi (DE-627)ELV001327801 (ELSEVIER)S0016-2361(18)30514-3 DE-627 ger DE-627 rda eng 660 DE-600 58.21 bkl Yue, Du verfasserin aut Three-dimensional ordered phosphotungstic acid/TiO 2018 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A series of phosphotungstic acid (HPW)/TiO2 materials with three-dimensional continuous and ordered macroporous structure, ranging from 130 nm to 300 nm in size, are synthesized by colloidal crystal templates and used as catalysts for oxidative desulfurization (ODS) of model oil. The structure and properties of 3DOM HPW/TiO2 catalysts are characterized by powder X-ray diffraction (XRD), scanning electron microscope (SEM), transmission electron microscopy (TEM), N2 adsorption–desorption isotherms, inductively coupled plasma-optical emission spectrophotometer (ICP) and fourier transform infrared spectra (FT-IR). Characterization results demonstrate that all the HPW/TiO2 samples possess a large BET surface area and three-dimensional ordered macroporous structure with Keggin-type HPW dispersed homogeneously in TiO2 framework. 3DOM HPW/TiO2 with an average pore diameter around 250 nm presents the highest catalytic activity for dibenzothiophene (DBT), which can be attributed to the combination of its large enough macropores allowing for efficient mass transport and its high surface area enabling sufficient exposure of catalytic active sites. Furthermore, the catalyst is recovered and reused for seven runs with no obviously decrease in catalytic activity. 3DOM structure Phosphotungstic acid Oxidative desulfurization Lei, Jiaheng verfasserin aut Peng, Yang verfasserin aut Li, Junsheng verfasserin aut Du, Xiaodi verfasserin aut Enthalten in Fuel New York, NY [u.a.] : Elsevier, 1970 226, Seite 148-155 Online-Ressource (DE-627)300898584 (DE-600)1483656-7 (DE-576)09555176X 0016-2361 nnns volume:226 pages:148-155 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.21 Brennstoffe Kraftstoffe Explosivstoffe AR 226 148-155
spelling	10.1016/j.fuel.2018.03.106 doi (DE-627)ELV001327801 (ELSEVIER)S0016-2361(18)30514-3 DE-627 ger DE-627 rda eng 660 DE-600 58.21 bkl Yue, Du verfasserin aut Three-dimensional ordered phosphotungstic acid/TiO 2018 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A series of phosphotungstic acid (HPW)/TiO2 materials with three-dimensional continuous and ordered macroporous structure, ranging from 130 nm to 300 nm in size, are synthesized by colloidal crystal templates and used as catalysts for oxidative desulfurization (ODS) of model oil. The structure and properties of 3DOM HPW/TiO2 catalysts are characterized by powder X-ray diffraction (XRD), scanning electron microscope (SEM), transmission electron microscopy (TEM), N2 adsorption–desorption isotherms, inductively coupled plasma-optical emission spectrophotometer (ICP) and fourier transform infrared spectra (FT-IR). Characterization results demonstrate that all the HPW/TiO2 samples possess a large BET surface area and three-dimensional ordered macroporous structure with Keggin-type HPW dispersed homogeneously in TiO2 framework. 3DOM HPW/TiO2 with an average pore diameter around 250 nm presents the highest catalytic activity for dibenzothiophene (DBT), which can be attributed to the combination of its large enough macropores allowing for efficient mass transport and its high surface area enabling sufficient exposure of catalytic active sites. Furthermore, the catalyst is recovered and reused for seven runs with no obviously decrease in catalytic activity. 3DOM structure Phosphotungstic acid Oxidative desulfurization Lei, Jiaheng verfasserin aut Peng, Yang verfasserin aut Li, Junsheng verfasserin aut Du, Xiaodi verfasserin aut Enthalten in Fuel New York, NY [u.a.] : Elsevier, 1970 226, Seite 148-155 Online-Ressource (DE-627)300898584 (DE-600)1483656-7 (DE-576)09555176X 0016-2361 nnns volume:226 pages:148-155 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.21 Brennstoffe Kraftstoffe Explosivstoffe AR 226 148-155
allfields_unstemmed	10.1016/j.fuel.2018.03.106 doi (DE-627)ELV001327801 (ELSEVIER)S0016-2361(18)30514-3 DE-627 ger DE-627 rda eng 660 DE-600 58.21 bkl Yue, Du verfasserin aut Three-dimensional ordered phosphotungstic acid/TiO 2018 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A series of phosphotungstic acid (HPW)/TiO2 materials with three-dimensional continuous and ordered macroporous structure, ranging from 130 nm to 300 nm in size, are synthesized by colloidal crystal templates and used as catalysts for oxidative desulfurization (ODS) of model oil. The structure and properties of 3DOM HPW/TiO2 catalysts are characterized by powder X-ray diffraction (XRD), scanning electron microscope (SEM), transmission electron microscopy (TEM), N2 adsorption–desorption isotherms, inductively coupled plasma-optical emission spectrophotometer (ICP) and fourier transform infrared spectra (FT-IR). Characterization results demonstrate that all the HPW/TiO2 samples possess a large BET surface area and three-dimensional ordered macroporous structure with Keggin-type HPW dispersed homogeneously in TiO2 framework. 3DOM HPW/TiO2 with an average pore diameter around 250 nm presents the highest catalytic activity for dibenzothiophene (DBT), which can be attributed to the combination of its large enough macropores allowing for efficient mass transport and its high surface area enabling sufficient exposure of catalytic active sites. Furthermore, the catalyst is recovered and reused for seven runs with no obviously decrease in catalytic activity. 3DOM structure Phosphotungstic acid Oxidative desulfurization Lei, Jiaheng verfasserin aut Peng, Yang verfasserin aut Li, Junsheng verfasserin aut Du, Xiaodi verfasserin aut Enthalten in Fuel New York, NY [u.a.] : Elsevier, 1970 226, Seite 148-155 Online-Ressource (DE-627)300898584 (DE-600)1483656-7 (DE-576)09555176X 0016-2361 nnns volume:226 pages:148-155 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.21 Brennstoffe Kraftstoffe Explosivstoffe AR 226 148-155
allfieldsGer	10.1016/j.fuel.2018.03.106 doi (DE-627)ELV001327801 (ELSEVIER)S0016-2361(18)30514-3 DE-627 ger DE-627 rda eng 660 DE-600 58.21 bkl Yue, Du verfasserin aut Three-dimensional ordered phosphotungstic acid/TiO 2018 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A series of phosphotungstic acid (HPW)/TiO2 materials with three-dimensional continuous and ordered macroporous structure, ranging from 130 nm to 300 nm in size, are synthesized by colloidal crystal templates and used as catalysts for oxidative desulfurization (ODS) of model oil. The structure and properties of 3DOM HPW/TiO2 catalysts are characterized by powder X-ray diffraction (XRD), scanning electron microscope (SEM), transmission electron microscopy (TEM), N2 adsorption–desorption isotherms, inductively coupled plasma-optical emission spectrophotometer (ICP) and fourier transform infrared spectra (FT-IR). Characterization results demonstrate that all the HPW/TiO2 samples possess a large BET surface area and three-dimensional ordered macroporous structure with Keggin-type HPW dispersed homogeneously in TiO2 framework. 3DOM HPW/TiO2 with an average pore diameter around 250 nm presents the highest catalytic activity for dibenzothiophene (DBT), which can be attributed to the combination of its large enough macropores allowing for efficient mass transport and its high surface area enabling sufficient exposure of catalytic active sites. Furthermore, the catalyst is recovered and reused for seven runs with no obviously decrease in catalytic activity. 3DOM structure Phosphotungstic acid Oxidative desulfurization Lei, Jiaheng verfasserin aut Peng, Yang verfasserin aut Li, Junsheng verfasserin aut Du, Xiaodi verfasserin aut Enthalten in Fuel New York, NY [u.a.] : Elsevier, 1970 226, Seite 148-155 Online-Ressource (DE-627)300898584 (DE-600)1483656-7 (DE-576)09555176X 0016-2361 nnns volume:226 pages:148-155 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.21 Brennstoffe Kraftstoffe Explosivstoffe AR 226 148-155
allfieldsSound	10.1016/j.fuel.2018.03.106 doi (DE-627)ELV001327801 (ELSEVIER)S0016-2361(18)30514-3 DE-627 ger DE-627 rda eng 660 DE-600 58.21 bkl Yue, Du verfasserin aut Three-dimensional ordered phosphotungstic acid/TiO 2018 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A series of phosphotungstic acid (HPW)/TiO2 materials with three-dimensional continuous and ordered macroporous structure, ranging from 130 nm to 300 nm in size, are synthesized by colloidal crystal templates and used as catalysts for oxidative desulfurization (ODS) of model oil. The structure and properties of 3DOM HPW/TiO2 catalysts are characterized by powder X-ray diffraction (XRD), scanning electron microscope (SEM), transmission electron microscopy (TEM), N2 adsorption–desorption isotherms, inductively coupled plasma-optical emission spectrophotometer (ICP) and fourier transform infrared spectra (FT-IR). Characterization results demonstrate that all the HPW/TiO2 samples possess a large BET surface area and three-dimensional ordered macroporous structure with Keggin-type HPW dispersed homogeneously in TiO2 framework. 3DOM HPW/TiO2 with an average pore diameter around 250 nm presents the highest catalytic activity for dibenzothiophene (DBT), which can be attributed to the combination of its large enough macropores allowing for efficient mass transport and its high surface area enabling sufficient exposure of catalytic active sites. Furthermore, the catalyst is recovered and reused for seven runs with no obviously decrease in catalytic activity. 3DOM structure Phosphotungstic acid Oxidative desulfurization Lei, Jiaheng verfasserin aut Peng, Yang verfasserin aut Li, Junsheng verfasserin aut Du, Xiaodi verfasserin aut Enthalten in Fuel New York, NY [u.a.] : Elsevier, 1970 226, Seite 148-155 Online-Ressource (DE-627)300898584 (DE-600)1483656-7 (DE-576)09555176X 0016-2361 nnns volume:226 pages:148-155 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.21 Brennstoffe Kraftstoffe Explosivstoffe AR 226 148-155
language	English
source	Enthalten in Fuel 226, Seite 148-155 volume:226 pages:148-155
sourceStr	Enthalten in Fuel 226, Seite 148-155 volume:226 pages:148-155
format_phy_str_mv	Article
bklname	Brennstoffe Kraftstoffe Explosivstoffe
institution	findex.gbv.de
topic_facet	3DOM structure Phosphotungstic acid Oxidative desulfurization
dewey-raw	660
isfreeaccess_bool	false
container_title	Fuel
authorswithroles_txt_mv	Yue, Du @@aut@@ Lei, Jiaheng @@aut@@ Peng, Yang @@aut@@ Li, Junsheng @@aut@@ Du, Xiaodi @@aut@@
publishDateDaySort_date	2018-01-01T00:00:00Z
hierarchy_top_id	300898584
dewey-sort	3660
id	ELV001327801
language_de	englisch
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author	Yue, Du
spellingShingle	Yue, Du ddc 660 bkl 58.21 misc 3DOM structure misc Phosphotungstic acid misc Oxidative desulfurization Three-dimensional ordered phosphotungstic acid/TiO
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topic_title	660 DE-600 58.21 bkl Three-dimensional ordered phosphotungstic acid/TiO 3DOM structure Phosphotungstic acid Oxidative desulfurization
topic	ddc 660 bkl 58.21 misc 3DOM structure misc Phosphotungstic acid misc Oxidative desulfurization
topic_unstemmed	ddc 660 bkl 58.21 misc 3DOM structure misc Phosphotungstic acid misc Oxidative desulfurization
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title	Three-dimensional ordered phosphotungstic acid/TiO
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title_full	Three-dimensional ordered phosphotungstic acid/TiO
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title_sort	three-dimensional ordered phosphotungstic acid/tio
title_auth	Three-dimensional ordered phosphotungstic acid/TiO
abstract	A series of phosphotungstic acid (HPW)/TiO2 materials with three-dimensional continuous and ordered macroporous structure, ranging from 130 nm to 300 nm in size, are synthesized by colloidal crystal templates and used as catalysts for oxidative desulfurization (ODS) of model oil. The structure and properties of 3DOM HPW/TiO2 catalysts are characterized by powder X-ray diffraction (XRD), scanning electron microscope (SEM), transmission electron microscopy (TEM), N2 adsorption–desorption isotherms, inductively coupled plasma-optical emission spectrophotometer (ICP) and fourier transform infrared spectra (FT-IR). Characterization results demonstrate that all the HPW/TiO2 samples possess a large BET surface area and three-dimensional ordered macroporous structure with Keggin-type HPW dispersed homogeneously in TiO2 framework. 3DOM HPW/TiO2 with an average pore diameter around 250 nm presents the highest catalytic activity for dibenzothiophene (DBT), which can be attributed to the combination of its large enough macropores allowing for efficient mass transport and its high surface area enabling sufficient exposure of catalytic active sites. Furthermore, the catalyst is recovered and reused for seven runs with no obviously decrease in catalytic activity.
abstractGer	A series of phosphotungstic acid (HPW)/TiO2 materials with three-dimensional continuous and ordered macroporous structure, ranging from 130 nm to 300 nm in size, are synthesized by colloidal crystal templates and used as catalysts for oxidative desulfurization (ODS) of model oil. The structure and properties of 3DOM HPW/TiO2 catalysts are characterized by powder X-ray diffraction (XRD), scanning electron microscope (SEM), transmission electron microscopy (TEM), N2 adsorption–desorption isotherms, inductively coupled plasma-optical emission spectrophotometer (ICP) and fourier transform infrared spectra (FT-IR). Characterization results demonstrate that all the HPW/TiO2 samples possess a large BET surface area and three-dimensional ordered macroporous structure with Keggin-type HPW dispersed homogeneously in TiO2 framework. 3DOM HPW/TiO2 with an average pore diameter around 250 nm presents the highest catalytic activity for dibenzothiophene (DBT), which can be attributed to the combination of its large enough macropores allowing for efficient mass transport and its high surface area enabling sufficient exposure of catalytic active sites. Furthermore, the catalyst is recovered and reused for seven runs with no obviously decrease in catalytic activity.
abstract_unstemmed	A series of phosphotungstic acid (HPW)/TiO2 materials with three-dimensional continuous and ordered macroporous structure, ranging from 130 nm to 300 nm in size, are synthesized by colloidal crystal templates and used as catalysts for oxidative desulfurization (ODS) of model oil. The structure and properties of 3DOM HPW/TiO2 catalysts are characterized by powder X-ray diffraction (XRD), scanning electron microscope (SEM), transmission electron microscopy (TEM), N2 adsorption–desorption isotherms, inductively coupled plasma-optical emission spectrophotometer (ICP) and fourier transform infrared spectra (FT-IR). Characterization results demonstrate that all the HPW/TiO2 samples possess a large BET surface area and three-dimensional ordered macroporous structure with Keggin-type HPW dispersed homogeneously in TiO2 framework. 3DOM HPW/TiO2 with an average pore diameter around 250 nm presents the highest catalytic activity for dibenzothiophene (DBT), which can be attributed to the combination of its large enough macropores allowing for efficient mass transport and its high surface area enabling sufficient exposure of catalytic active sites. Furthermore, the catalyst is recovered and reused for seven runs with no obviously decrease in catalytic activity.
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title_short	Three-dimensional ordered phosphotungstic acid/TiO
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up_date	2024-07-06T20:59:52.446Z
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score	7.4009056

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Three-dimensional ordered phosphotungstic acid/TiO

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Vorhandene Bände

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