The oxidation characteristics of furan derivatives and binary TPGME blends under engine relevant conditions

Furan and its derivatives have been receiving attention as next generation alternative fuels, related to advanced bio-oil production. However, the ignition quality of furans allows their use only as an additive to diesel fuel in CI engines, which potentially requires the continued use of a fossil-de...
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Gespeichert in:

Autor*in:	Wu, Shiliang [verfasserIn] Kang, Dongil [verfasserIn] Zhang, Huiyan [verfasserIn] Xiao, Rui [verfasserIn] Boehman, André L. [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2018

Schlagwörter:	Methylfuran Furfural TPGME Bio-fuel motored engine

Übergeordnetes Werk:	Enthalten in: Proceedings of the Combustion Institute - Combustion Institute ; ID: gnd/1004025-0, Amsterdam [u.a.] : Elsevier, 2000, 37, Seite 4635-4643
Übergeordnetes Werk:	volume:37 ; pages:4635-4643

DOI / URN:	10.1016/j.proci.2018.08.060

Katalog-ID:	ELV001527649

Internformat


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520			\|a Furan and its derivatives have been receiving attention as next generation alternative fuels, related to advanced bio-oil production. However, the ignition quality of furans allows their use only as an additive to diesel fuel in CI engines, which potentially requires the continued use of a fossil-derived base fuel. This study first adopts tri-propylene glycol mono-methyl ether (TPGME) as a substitute for diesel fuel with addition of furan and furan derivatives, including 2-methylfuran, 2,5-dimethylfuran, and furfural, thereby removing fossil-derived fuels from the mixture. With this motivation, gas-phase ignition characteristics of furans were investigated in a modified CFR motored engine, displaying an absence of low temperature heat release (LTHR), while n-heptane as a reference fuel shows a strong two-stage ignition characteristic under the same condition. The structural impact of furans is represented as global oxidation reactivities that are as follows: furan < 2-methylfuran < 2,5-dimethylfuran < furfural < n-heptane. The ranking of individual furans is supported by bond dissociation energies of each fuel's functional group substituent on the furan-ring. Ignition characteristics of TPGME display a strong low-temperature oxidation reactivity; however, its reactivity rapidly diminishes with increasing amounts of furan, shutting down low-temperature oxidation paths. The structural impact of furan and methyl-substituted furans on reactivity is significantly muted when blended with TPGME, as observed in a motored CFR engine and a constant volume spray combustion chamber.
650		4	\|a Methylfuran
650		4	\|a Furfural
650		4	\|a TPGME
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700	1		\|a Zhang, Huiyan \|e verfasserin \|4 aut
700	1		\|a Xiao, Rui \|e verfasserin \|4 aut
700	1		\|a Boehman, André L. \|e verfasserin \|0 (orcid)0000-0002-0965-9288 \|4 aut
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912			\|a GBV_ILN_2014
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912			\|a GBV_ILN_2021
912			\|a GBV_ILN_2025
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912			\|a GBV_ILN_2034
912			\|a GBV_ILN_2038
912			\|a GBV_ILN_2044
912			\|a GBV_ILN_2048
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912			\|a GBV_ILN_2050
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912			\|a GBV_ILN_2522
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912			\|a GBV_ILN_4046
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912			\|a GBV_ILN_4251
912			\|a GBV_ILN_4305
912			\|a GBV_ILN_4313
912			\|a GBV_ILN_4322
912			\|a GBV_ILN_4323
912			\|a GBV_ILN_4324
912			\|a GBV_ILN_4325
912			\|a GBV_ILN_4326
912			\|a GBV_ILN_4333
912			\|a GBV_ILN_4334
912			\|a GBV_ILN_4335
912			\|a GBV_ILN_4338
912			\|a GBV_ILN_4393
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author_variant	s w sw d k dk h z hz r x rx a l b al alb
matchkey_str	article:18732704:2018----::hoiainhrceitcofrneiaieadiaypmbedud
hierarchy_sort_str	2018
publishDate	2018
allfields	10.1016/j.proci.2018.08.060 doi (DE-627)ELV001527649 (ELSEVIER)S1540-7489(18)30604-7 DE-627 ger DE-627 rda eng 660 DE-600 Wu, Shiliang verfasserin (orcid)0000-0002-0196-1458 aut The oxidation characteristics of furan derivatives and binary TPGME blends under engine relevant conditions 2018 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Furan and its derivatives have been receiving attention as next generation alternative fuels, related to advanced bio-oil production. However, the ignition quality of furans allows their use only as an additive to diesel fuel in CI engines, which potentially requires the continued use of a fossil-derived base fuel. This study first adopts tri-propylene glycol mono-methyl ether (TPGME) as a substitute for diesel fuel with addition of furan and furan derivatives, including 2-methylfuran, 2,5-dimethylfuran, and furfural, thereby removing fossil-derived fuels from the mixture. With this motivation, gas-phase ignition characteristics of furans were investigated in a modified CFR motored engine, displaying an absence of low temperature heat release (LTHR), while n-heptane as a reference fuel shows a strong two-stage ignition characteristic under the same condition. The structural impact of furans is represented as global oxidation reactivities that are as follows: furan < 2-methylfuran < 2,5-dimethylfuran < furfural < n-heptane. The ranking of individual furans is supported by bond dissociation energies of each fuel's functional group substituent on the furan-ring. Ignition characteristics of TPGME display a strong low-temperature oxidation reactivity; however, its reactivity rapidly diminishes with increasing amounts of furan, shutting down low-temperature oxidation paths. The structural impact of furan and methyl-substituted furans on reactivity is significantly muted when blended with TPGME, as observed in a motored CFR engine and a constant volume spray combustion chamber. Methylfuran Furfural TPGME Bio-fuel motored engine Kang, Dongil verfasserin aut Zhang, Huiyan verfasserin aut Xiao, Rui verfasserin aut Boehman, André L. verfasserin (orcid)0000-0002-0965-9288 aut Enthalten in Combustion Institute ; ID: gnd/1004025-0 Proceedings of the Combustion Institute Amsterdam [u.a.] : Elsevier, 2000 37, Seite 4635-4643 Online-Ressource (DE-627)495741140 (DE-600)2197968-6 (DE-576)259486582 1873-2704 nnns volume:37 pages:4635-4643 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 AR 37 4635-4643
spelling	10.1016/j.proci.2018.08.060 doi (DE-627)ELV001527649 (ELSEVIER)S1540-7489(18)30604-7 DE-627 ger DE-627 rda eng 660 DE-600 Wu, Shiliang verfasserin (orcid)0000-0002-0196-1458 aut The oxidation characteristics of furan derivatives and binary TPGME blends under engine relevant conditions 2018 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Furan and its derivatives have been receiving attention as next generation alternative fuels, related to advanced bio-oil production. However, the ignition quality of furans allows their use only as an additive to diesel fuel in CI engines, which potentially requires the continued use of a fossil-derived base fuel. This study first adopts tri-propylene glycol mono-methyl ether (TPGME) as a substitute for diesel fuel with addition of furan and furan derivatives, including 2-methylfuran, 2,5-dimethylfuran, and furfural, thereby removing fossil-derived fuels from the mixture. With this motivation, gas-phase ignition characteristics of furans were investigated in a modified CFR motored engine, displaying an absence of low temperature heat release (LTHR), while n-heptane as a reference fuel shows a strong two-stage ignition characteristic under the same condition. The structural impact of furans is represented as global oxidation reactivities that are as follows: furan < 2-methylfuran < 2,5-dimethylfuran < furfural < n-heptane. The ranking of individual furans is supported by bond dissociation energies of each fuel's functional group substituent on the furan-ring. Ignition characteristics of TPGME display a strong low-temperature oxidation reactivity; however, its reactivity rapidly diminishes with increasing amounts of furan, shutting down low-temperature oxidation paths. The structural impact of furan and methyl-substituted furans on reactivity is significantly muted when blended with TPGME, as observed in a motored CFR engine and a constant volume spray combustion chamber. Methylfuran Furfural TPGME Bio-fuel motored engine Kang, Dongil verfasserin aut Zhang, Huiyan verfasserin aut Xiao, Rui verfasserin aut Boehman, André L. verfasserin (orcid)0000-0002-0965-9288 aut Enthalten in Combustion Institute ; ID: gnd/1004025-0 Proceedings of the Combustion Institute Amsterdam [u.a.] : Elsevier, 2000 37, Seite 4635-4643 Online-Ressource (DE-627)495741140 (DE-600)2197968-6 (DE-576)259486582 1873-2704 nnns volume:37 pages:4635-4643 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 AR 37 4635-4643
allfields_unstemmed	10.1016/j.proci.2018.08.060 doi (DE-627)ELV001527649 (ELSEVIER)S1540-7489(18)30604-7 DE-627 ger DE-627 rda eng 660 DE-600 Wu, Shiliang verfasserin (orcid)0000-0002-0196-1458 aut The oxidation characteristics of furan derivatives and binary TPGME blends under engine relevant conditions 2018 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Furan and its derivatives have been receiving attention as next generation alternative fuels, related to advanced bio-oil production. However, the ignition quality of furans allows their use only as an additive to diesel fuel in CI engines, which potentially requires the continued use of a fossil-derived base fuel. This study first adopts tri-propylene glycol mono-methyl ether (TPGME) as a substitute for diesel fuel with addition of furan and furan derivatives, including 2-methylfuran, 2,5-dimethylfuran, and furfural, thereby removing fossil-derived fuels from the mixture. With this motivation, gas-phase ignition characteristics of furans were investigated in a modified CFR motored engine, displaying an absence of low temperature heat release (LTHR), while n-heptane as a reference fuel shows a strong two-stage ignition characteristic under the same condition. The structural impact of furans is represented as global oxidation reactivities that are as follows: furan < 2-methylfuran < 2,5-dimethylfuran < furfural < n-heptane. The ranking of individual furans is supported by bond dissociation energies of each fuel's functional group substituent on the furan-ring. Ignition characteristics of TPGME display a strong low-temperature oxidation reactivity; however, its reactivity rapidly diminishes with increasing amounts of furan, shutting down low-temperature oxidation paths. The structural impact of furan and methyl-substituted furans on reactivity is significantly muted when blended with TPGME, as observed in a motored CFR engine and a constant volume spray combustion chamber. Methylfuran Furfural TPGME Bio-fuel motored engine Kang, Dongil verfasserin aut Zhang, Huiyan verfasserin aut Xiao, Rui verfasserin aut Boehman, André L. verfasserin (orcid)0000-0002-0965-9288 aut Enthalten in Combustion Institute ; ID: gnd/1004025-0 Proceedings of the Combustion Institute Amsterdam [u.a.] : Elsevier, 2000 37, Seite 4635-4643 Online-Ressource (DE-627)495741140 (DE-600)2197968-6 (DE-576)259486582 1873-2704 nnns volume:37 pages:4635-4643 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 AR 37 4635-4643
allfieldsGer	10.1016/j.proci.2018.08.060 doi (DE-627)ELV001527649 (ELSEVIER)S1540-7489(18)30604-7 DE-627 ger DE-627 rda eng 660 DE-600 Wu, Shiliang verfasserin (orcid)0000-0002-0196-1458 aut The oxidation characteristics of furan derivatives and binary TPGME blends under engine relevant conditions 2018 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Furan and its derivatives have been receiving attention as next generation alternative fuels, related to advanced bio-oil production. However, the ignition quality of furans allows their use only as an additive to diesel fuel in CI engines, which potentially requires the continued use of a fossil-derived base fuel. This study first adopts tri-propylene glycol mono-methyl ether (TPGME) as a substitute for diesel fuel with addition of furan and furan derivatives, including 2-methylfuran, 2,5-dimethylfuran, and furfural, thereby removing fossil-derived fuels from the mixture. With this motivation, gas-phase ignition characteristics of furans were investigated in a modified CFR motored engine, displaying an absence of low temperature heat release (LTHR), while n-heptane as a reference fuel shows a strong two-stage ignition characteristic under the same condition. The structural impact of furans is represented as global oxidation reactivities that are as follows: furan < 2-methylfuran < 2,5-dimethylfuran < furfural < n-heptane. The ranking of individual furans is supported by bond dissociation energies of each fuel's functional group substituent on the furan-ring. Ignition characteristics of TPGME display a strong low-temperature oxidation reactivity; however, its reactivity rapidly diminishes with increasing amounts of furan, shutting down low-temperature oxidation paths. The structural impact of furan and methyl-substituted furans on reactivity is significantly muted when blended with TPGME, as observed in a motored CFR engine and a constant volume spray combustion chamber. Methylfuran Furfural TPGME Bio-fuel motored engine Kang, Dongil verfasserin aut Zhang, Huiyan verfasserin aut Xiao, Rui verfasserin aut Boehman, André L. verfasserin (orcid)0000-0002-0965-9288 aut Enthalten in Combustion Institute ; ID: gnd/1004025-0 Proceedings of the Combustion Institute Amsterdam [u.a.] : Elsevier, 2000 37, Seite 4635-4643 Online-Ressource (DE-627)495741140 (DE-600)2197968-6 (DE-576)259486582 1873-2704 nnns volume:37 pages:4635-4643 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 AR 37 4635-4643
allfieldsSound	10.1016/j.proci.2018.08.060 doi (DE-627)ELV001527649 (ELSEVIER)S1540-7489(18)30604-7 DE-627 ger DE-627 rda eng 660 DE-600 Wu, Shiliang verfasserin (orcid)0000-0002-0196-1458 aut The oxidation characteristics of furan derivatives and binary TPGME blends under engine relevant conditions 2018 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Furan and its derivatives have been receiving attention as next generation alternative fuels, related to advanced bio-oil production. However, the ignition quality of furans allows their use only as an additive to diesel fuel in CI engines, which potentially requires the continued use of a fossil-derived base fuel. This study first adopts tri-propylene glycol mono-methyl ether (TPGME) as a substitute for diesel fuel with addition of furan and furan derivatives, including 2-methylfuran, 2,5-dimethylfuran, and furfural, thereby removing fossil-derived fuels from the mixture. With this motivation, gas-phase ignition characteristics of furans were investigated in a modified CFR motored engine, displaying an absence of low temperature heat release (LTHR), while n-heptane as a reference fuel shows a strong two-stage ignition characteristic under the same condition. The structural impact of furans is represented as global oxidation reactivities that are as follows: furan < 2-methylfuran < 2,5-dimethylfuran < furfural < n-heptane. The ranking of individual furans is supported by bond dissociation energies of each fuel's functional group substituent on the furan-ring. Ignition characteristics of TPGME display a strong low-temperature oxidation reactivity; however, its reactivity rapidly diminishes with increasing amounts of furan, shutting down low-temperature oxidation paths. The structural impact of furan and methyl-substituted furans on reactivity is significantly muted when blended with TPGME, as observed in a motored CFR engine and a constant volume spray combustion chamber. Methylfuran Furfural TPGME Bio-fuel motored engine Kang, Dongil verfasserin aut Zhang, Huiyan verfasserin aut Xiao, Rui verfasserin aut Boehman, André L. verfasserin (orcid)0000-0002-0965-9288 aut Enthalten in Combustion Institute ; ID: gnd/1004025-0 Proceedings of the Combustion Institute Amsterdam [u.a.] : Elsevier, 2000 37, Seite 4635-4643 Online-Ressource (DE-627)495741140 (DE-600)2197968-6 (DE-576)259486582 1873-2704 nnns volume:37 pages:4635-4643 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 AR 37 4635-4643
language	English
source	Enthalten in Proceedings of the Combustion Institute 37, Seite 4635-4643 volume:37 pages:4635-4643
sourceStr	Enthalten in Proceedings of the Combustion Institute 37, Seite 4635-4643 volume:37 pages:4635-4643
format_phy_str_mv	Article
institution	findex.gbv.de
topic_facet	Methylfuran Furfural TPGME Bio-fuel motored engine
dewey-raw	660
isfreeaccess_bool	false
container_title	Proceedings of the Combustion Institute
authorswithroles_txt_mv	Wu, Shiliang @@aut@@ Kang, Dongil @@aut@@ Zhang, Huiyan @@aut@@ Xiao, Rui @@aut@@ Boehman, André L. @@aut@@
publishDateDaySort_date	2018-01-01T00:00:00Z
hierarchy_top_id	495741140
dewey-sort	3660
id	ELV001527649
language_de	englisch
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The ranking of individual furans is supported by bond dissociation energies of each fuel's functional group substituent on the furan-ring. Ignition characteristics of TPGME display a strong low-temperature oxidation reactivity; however, its reactivity rapidly diminishes with increasing amounts of furan, shutting down low-temperature oxidation paths. 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author	Wu, Shiliang
spellingShingle	Wu, Shiliang ddc 660 misc Methylfuran misc Furfural misc TPGME misc Bio-fuel misc motored engine The oxidation characteristics of furan derivatives and binary TPGME blends under engine relevant conditions
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topic_title	660 DE-600 The oxidation characteristics of furan derivatives and binary TPGME blends under engine relevant conditions Methylfuran Furfural TPGME Bio-fuel motored engine
topic	ddc 660 misc Methylfuran misc Furfural misc TPGME misc Bio-fuel misc motored engine
topic_unstemmed	ddc 660 misc Methylfuran misc Furfural misc TPGME misc Bio-fuel misc motored engine
topic_browse	ddc 660 misc Methylfuran misc Furfural misc TPGME misc Bio-fuel misc motored engine
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title	The oxidation characteristics of furan derivatives and binary TPGME blends under engine relevant conditions
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title_full	The oxidation characteristics of furan derivatives and binary TPGME blends under engine relevant conditions
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author_browse	Wu, Shiliang Kang, Dongil Zhang, Huiyan Xiao, Rui Boehman, André L.
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title_sort	the oxidation characteristics of furan derivatives and binary tpgme blends under engine relevant conditions
title_auth	The oxidation characteristics of furan derivatives and binary TPGME blends under engine relevant conditions
abstract	Furan and its derivatives have been receiving attention as next generation alternative fuels, related to advanced bio-oil production. However, the ignition quality of furans allows their use only as an additive to diesel fuel in CI engines, which potentially requires the continued use of a fossil-derived base fuel. This study first adopts tri-propylene glycol mono-methyl ether (TPGME) as a substitute for diesel fuel with addition of furan and furan derivatives, including 2-methylfuran, 2,5-dimethylfuran, and furfural, thereby removing fossil-derived fuels from the mixture. With this motivation, gas-phase ignition characteristics of furans were investigated in a modified CFR motored engine, displaying an absence of low temperature heat release (LTHR), while n-heptane as a reference fuel shows a strong two-stage ignition characteristic under the same condition. The structural impact of furans is represented as global oxidation reactivities that are as follows: furan < 2-methylfuran < 2,5-dimethylfuran < furfural < n-heptane. The ranking of individual furans is supported by bond dissociation energies of each fuel's functional group substituent on the furan-ring. Ignition characteristics of TPGME display a strong low-temperature oxidation reactivity; however, its reactivity rapidly diminishes with increasing amounts of furan, shutting down low-temperature oxidation paths. The structural impact of furan and methyl-substituted furans on reactivity is significantly muted when blended with TPGME, as observed in a motored CFR engine and a constant volume spray combustion chamber.
abstractGer	Furan and its derivatives have been receiving attention as next generation alternative fuels, related to advanced bio-oil production. However, the ignition quality of furans allows their use only as an additive to diesel fuel in CI engines, which potentially requires the continued use of a fossil-derived base fuel. This study first adopts tri-propylene glycol mono-methyl ether (TPGME) as a substitute for diesel fuel with addition of furan and furan derivatives, including 2-methylfuran, 2,5-dimethylfuran, and furfural, thereby removing fossil-derived fuels from the mixture. With this motivation, gas-phase ignition characteristics of furans were investigated in a modified CFR motored engine, displaying an absence of low temperature heat release (LTHR), while n-heptane as a reference fuel shows a strong two-stage ignition characteristic under the same condition. The structural impact of furans is represented as global oxidation reactivities that are as follows: furan < 2-methylfuran < 2,5-dimethylfuran < furfural < n-heptane. The ranking of individual furans is supported by bond dissociation energies of each fuel's functional group substituent on the furan-ring. Ignition characteristics of TPGME display a strong low-temperature oxidation reactivity; however, its reactivity rapidly diminishes with increasing amounts of furan, shutting down low-temperature oxidation paths. The structural impact of furan and methyl-substituted furans on reactivity is significantly muted when blended with TPGME, as observed in a motored CFR engine and a constant volume spray combustion chamber.
abstract_unstemmed	Furan and its derivatives have been receiving attention as next generation alternative fuels, related to advanced bio-oil production. However, the ignition quality of furans allows their use only as an additive to diesel fuel in CI engines, which potentially requires the continued use of a fossil-derived base fuel. This study first adopts tri-propylene glycol mono-methyl ether (TPGME) as a substitute for diesel fuel with addition of furan and furan derivatives, including 2-methylfuran, 2,5-dimethylfuran, and furfural, thereby removing fossil-derived fuels from the mixture. With this motivation, gas-phase ignition characteristics of furans were investigated in a modified CFR motored engine, displaying an absence of low temperature heat release (LTHR), while n-heptane as a reference fuel shows a strong two-stage ignition characteristic under the same condition. The structural impact of furans is represented as global oxidation reactivities that are as follows: furan < 2-methylfuran < 2,5-dimethylfuran < furfural < n-heptane. The ranking of individual furans is supported by bond dissociation energies of each fuel's functional group substituent on the furan-ring. Ignition characteristics of TPGME display a strong low-temperature oxidation reactivity; however, its reactivity rapidly diminishes with increasing amounts of furan, shutting down low-temperature oxidation paths. The structural impact of furan and methyl-substituted furans on reactivity is significantly muted when blended with TPGME, as observed in a motored CFR engine and a constant volume spray combustion chamber.
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title_short	The oxidation characteristics of furan derivatives and binary TPGME blends under engine relevant conditions
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author2	Kang, Dongil Zhang, Huiyan Xiao, Rui Boehman, André L.
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doi_str	10.1016/j.proci.2018.08.060
up_date	2024-07-06T21:40:45.403Z
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The oxidation characteristics of furan derivatives and binary TPGME blends under engine relevant conditions

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