Boron-speciation and aluminosilicate crystallization in alkali boroaluminosilicate glasses along the NaAl

The influences of boron on silicate glass dissolution behavior and crystallization have long been important in the nuclear waste glass and technical glass communities. Boron is a challenging component to model due to this ability to assume three- and four-fold coordinations with oxygen, as well as i...
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Autor*in:	Marcial, José [verfasserIn] Saleh, Muad [verfasserIn] Watson, Deborah [verfasserIn] Martin, Steve W. [verfasserIn] Crawford, Charles L. [verfasserIn] McCloy, John S. [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2019

Schlagwörter:	Boroaluminosilicate Glass structure EPSR NMR

Übergeordnetes Werk:	Enthalten in: Journal of non-crystalline solids - Amsterdam [u.a.] : Elsevier Science, 1968, 506, Seite 58-67
Übergeordnetes Werk:	volume:506 ; pages:58-67

DOI / URN:	10.1016/j.jnoncrysol.2019.01.001

Katalog-ID:	ELV001630288

Internformat


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245	1	0	\|a Boron-speciation and aluminosilicate crystallization in alkali boroaluminosilicate glasses along the NaAl
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520			\|a The influences of boron on silicate glass dissolution behavior and crystallization have long been important in the nuclear waste glass and technical glass communities. Boron is a challenging component to model due to this ability to assume three- and four-fold coordinations with oxygen, as well as its ability to form complex structural units with silicate tetrahedra. Furthermore, the low atomic mass limits the available characterization techniques. In the present work, recent literature findings on the compositional influence on boron speciation are implemented to interpret new data on alkali boroaluminosilicate glasses studied with 11B nuclear magnetic resonance (NMR), synchrotron X-ray scattering (s-XRS), and chemical durability measurements. The purpose of this study is to understand the influence of boron on the crystallization behavior of sodium and lithium aluminosilicate systems, NaAl1-xBxSiO4 and LiAl1-xBxSiO4, as applied to problems in nuclear waste vitrification. Comparisons are drawn between the alkali coordination number and crystallization behavior as a function of boron addition, as obtained through modeling of synchrotron X-ray total scattering using Empirical Potential Structural Refinement.
650		4	\|a Boroaluminosilicate
650		4	\|a Glass structure
650		4	\|a EPSR
650		4	\|a NMR
700	1		\|a Saleh, Muad \|e verfasserin \|4 aut
700	1		\|a Watson, Deborah \|e verfasserin \|4 aut
700	1		\|a Martin, Steve W. \|e verfasserin \|4 aut
700	1		\|a Crawford, Charles L. \|e verfasserin \|4 aut
700	1		\|a McCloy, John S. \|e verfasserin \|0 (orcid)0000-0001-7476-7771 \|4 aut
773	0	8	\|i Enthalten in \|t Journal of non-crystalline solids \|d Amsterdam [u.a.] : Elsevier Science, 1968 \|g 506, Seite 58-67 \|h Online-Ressource \|w (DE-627)306659808 \|w (DE-600)1500501-X \|w (DE-576)096806486 \|x 0022-3093 \|7 nnns
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936	b	k	\|a 51.45 \|j Werkstoffe mit besonderen Eigenschaften
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936	b	k	\|a 33.61 \|j Festkörperphysik
936	b	k	\|a 35.90 \|j Festkörperchemie
951			\|a AR
952			\|d 506 \|h 58-67

Indexfelder

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bklnumber	51.45 51.60 33.61 35.90
publishDate	2019
allfields	10.1016/j.jnoncrysol.2019.01.001 doi (DE-627)ELV001630288 (ELSEVIER)S0022-3093(19)30002-X DE-627 ger DE-627 rda eng 660 670 DE-600 51.45 bkl 51.60 bkl 33.61 bkl 35.90 bkl Marcial, José verfasserin (orcid)0000-0001-6156-5310 aut Boron-speciation and aluminosilicate crystallization in alkali boroaluminosilicate glasses along the NaAl 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The influences of boron on silicate glass dissolution behavior and crystallization have long been important in the nuclear waste glass and technical glass communities. Boron is a challenging component to model due to this ability to assume three- and four-fold coordinations with oxygen, as well as its ability to form complex structural units with silicate tetrahedra. Furthermore, the low atomic mass limits the available characterization techniques. In the present work, recent literature findings on the compositional influence on boron speciation are implemented to interpret new data on alkali boroaluminosilicate glasses studied with 11B nuclear magnetic resonance (NMR), synchrotron X-ray scattering (s-XRS), and chemical durability measurements. The purpose of this study is to understand the influence of boron on the crystallization behavior of sodium and lithium aluminosilicate systems, NaAl1-xBxSiO4 and LiAl1-xBxSiO4, as applied to problems in nuclear waste vitrification. Comparisons are drawn between the alkali coordination number and crystallization behavior as a function of boron addition, as obtained through modeling of synchrotron X-ray total scattering using Empirical Potential Structural Refinement. Boroaluminosilicate Glass structure EPSR NMR Saleh, Muad verfasserin aut Watson, Deborah verfasserin aut Martin, Steve W. verfasserin aut Crawford, Charles L. verfasserin aut McCloy, John S. verfasserin (orcid)0000-0001-7476-7771 aut Enthalten in Journal of non-crystalline solids Amsterdam [u.a.] : Elsevier Science, 1968 506, Seite 58-67 Online-Ressource (DE-627)306659808 (DE-600)1500501-X (DE-576)096806486 0022-3093 nnns volume:506 pages:58-67 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2008 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 51.45 Werkstoffe mit besonderen Eigenschaften 51.60 Keramische Werkstoffe Hartstoffe Werkstoffkunde 33.61 Festkörperphysik 35.90 Festkörperchemie AR 506 58-67
spelling	10.1016/j.jnoncrysol.2019.01.001 doi (DE-627)ELV001630288 (ELSEVIER)S0022-3093(19)30002-X DE-627 ger DE-627 rda eng 660 670 DE-600 51.45 bkl 51.60 bkl 33.61 bkl 35.90 bkl Marcial, José verfasserin (orcid)0000-0001-6156-5310 aut Boron-speciation and aluminosilicate crystallization in alkali boroaluminosilicate glasses along the NaAl 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The influences of boron on silicate glass dissolution behavior and crystallization have long been important in the nuclear waste glass and technical glass communities. Boron is a challenging component to model due to this ability to assume three- and four-fold coordinations with oxygen, as well as its ability to form complex structural units with silicate tetrahedra. Furthermore, the low atomic mass limits the available characterization techniques. In the present work, recent literature findings on the compositional influence on boron speciation are implemented to interpret new data on alkali boroaluminosilicate glasses studied with 11B nuclear magnetic resonance (NMR), synchrotron X-ray scattering (s-XRS), and chemical durability measurements. The purpose of this study is to understand the influence of boron on the crystallization behavior of sodium and lithium aluminosilicate systems, NaAl1-xBxSiO4 and LiAl1-xBxSiO4, as applied to problems in nuclear waste vitrification. Comparisons are drawn between the alkali coordination number and crystallization behavior as a function of boron addition, as obtained through modeling of synchrotron X-ray total scattering using Empirical Potential Structural Refinement. Boroaluminosilicate Glass structure EPSR NMR Saleh, Muad verfasserin aut Watson, Deborah verfasserin aut Martin, Steve W. verfasserin aut Crawford, Charles L. verfasserin aut McCloy, John S. verfasserin (orcid)0000-0001-7476-7771 aut Enthalten in Journal of non-crystalline solids Amsterdam [u.a.] : Elsevier Science, 1968 506, Seite 58-67 Online-Ressource (DE-627)306659808 (DE-600)1500501-X (DE-576)096806486 0022-3093 nnns volume:506 pages:58-67 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2008 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 51.45 Werkstoffe mit besonderen Eigenschaften 51.60 Keramische Werkstoffe Hartstoffe Werkstoffkunde 33.61 Festkörperphysik 35.90 Festkörperchemie AR 506 58-67
allfields_unstemmed	10.1016/j.jnoncrysol.2019.01.001 doi (DE-627)ELV001630288 (ELSEVIER)S0022-3093(19)30002-X DE-627 ger DE-627 rda eng 660 670 DE-600 51.45 bkl 51.60 bkl 33.61 bkl 35.90 bkl Marcial, José verfasserin (orcid)0000-0001-6156-5310 aut Boron-speciation and aluminosilicate crystallization in alkali boroaluminosilicate glasses along the NaAl 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The influences of boron on silicate glass dissolution behavior and crystallization have long been important in the nuclear waste glass and technical glass communities. Boron is a challenging component to model due to this ability to assume three- and four-fold coordinations with oxygen, as well as its ability to form complex structural units with silicate tetrahedra. Furthermore, the low atomic mass limits the available characterization techniques. In the present work, recent literature findings on the compositional influence on boron speciation are implemented to interpret new data on alkali boroaluminosilicate glasses studied with 11B nuclear magnetic resonance (NMR), synchrotron X-ray scattering (s-XRS), and chemical durability measurements. The purpose of this study is to understand the influence of boron on the crystallization behavior of sodium and lithium aluminosilicate systems, NaAl1-xBxSiO4 and LiAl1-xBxSiO4, as applied to problems in nuclear waste vitrification. Comparisons are drawn between the alkali coordination number and crystallization behavior as a function of boron addition, as obtained through modeling of synchrotron X-ray total scattering using Empirical Potential Structural Refinement. Boroaluminosilicate Glass structure EPSR NMR Saleh, Muad verfasserin aut Watson, Deborah verfasserin aut Martin, Steve W. verfasserin aut Crawford, Charles L. verfasserin aut McCloy, John S. verfasserin (orcid)0000-0001-7476-7771 aut Enthalten in Journal of non-crystalline solids Amsterdam [u.a.] : Elsevier Science, 1968 506, Seite 58-67 Online-Ressource (DE-627)306659808 (DE-600)1500501-X (DE-576)096806486 0022-3093 nnns volume:506 pages:58-67 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2008 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 51.45 Werkstoffe mit besonderen Eigenschaften 51.60 Keramische Werkstoffe Hartstoffe Werkstoffkunde 33.61 Festkörperphysik 35.90 Festkörperchemie AR 506 58-67
allfieldsGer	10.1016/j.jnoncrysol.2019.01.001 doi (DE-627)ELV001630288 (ELSEVIER)S0022-3093(19)30002-X DE-627 ger DE-627 rda eng 660 670 DE-600 51.45 bkl 51.60 bkl 33.61 bkl 35.90 bkl Marcial, José verfasserin (orcid)0000-0001-6156-5310 aut Boron-speciation and aluminosilicate crystallization in alkali boroaluminosilicate glasses along the NaAl 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The influences of boron on silicate glass dissolution behavior and crystallization have long been important in the nuclear waste glass and technical glass communities. Boron is a challenging component to model due to this ability to assume three- and four-fold coordinations with oxygen, as well as its ability to form complex structural units with silicate tetrahedra. Furthermore, the low atomic mass limits the available characterization techniques. In the present work, recent literature findings on the compositional influence on boron speciation are implemented to interpret new data on alkali boroaluminosilicate glasses studied with 11B nuclear magnetic resonance (NMR), synchrotron X-ray scattering (s-XRS), and chemical durability measurements. The purpose of this study is to understand the influence of boron on the crystallization behavior of sodium and lithium aluminosilicate systems, NaAl1-xBxSiO4 and LiAl1-xBxSiO4, as applied to problems in nuclear waste vitrification. Comparisons are drawn between the alkali coordination number and crystallization behavior as a function of boron addition, as obtained through modeling of synchrotron X-ray total scattering using Empirical Potential Structural Refinement. Boroaluminosilicate Glass structure EPSR NMR Saleh, Muad verfasserin aut Watson, Deborah verfasserin aut Martin, Steve W. verfasserin aut Crawford, Charles L. verfasserin aut McCloy, John S. verfasserin (orcid)0000-0001-7476-7771 aut Enthalten in Journal of non-crystalline solids Amsterdam [u.a.] : Elsevier Science, 1968 506, Seite 58-67 Online-Ressource (DE-627)306659808 (DE-600)1500501-X (DE-576)096806486 0022-3093 nnns volume:506 pages:58-67 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2008 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 51.45 Werkstoffe mit besonderen Eigenschaften 51.60 Keramische Werkstoffe Hartstoffe Werkstoffkunde 33.61 Festkörperphysik 35.90 Festkörperchemie AR 506 58-67
allfieldsSound	10.1016/j.jnoncrysol.2019.01.001 doi (DE-627)ELV001630288 (ELSEVIER)S0022-3093(19)30002-X DE-627 ger DE-627 rda eng 660 670 DE-600 51.45 bkl 51.60 bkl 33.61 bkl 35.90 bkl Marcial, José verfasserin (orcid)0000-0001-6156-5310 aut Boron-speciation and aluminosilicate crystallization in alkali boroaluminosilicate glasses along the NaAl 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The influences of boron on silicate glass dissolution behavior and crystallization have long been important in the nuclear waste glass and technical glass communities. Boron is a challenging component to model due to this ability to assume three- and four-fold coordinations with oxygen, as well as its ability to form complex structural units with silicate tetrahedra. Furthermore, the low atomic mass limits the available characterization techniques. In the present work, recent literature findings on the compositional influence on boron speciation are implemented to interpret new data on alkali boroaluminosilicate glasses studied with 11B nuclear magnetic resonance (NMR), synchrotron X-ray scattering (s-XRS), and chemical durability measurements. The purpose of this study is to understand the influence of boron on the crystallization behavior of sodium and lithium aluminosilicate systems, NaAl1-xBxSiO4 and LiAl1-xBxSiO4, as applied to problems in nuclear waste vitrification. Comparisons are drawn between the alkali coordination number and crystallization behavior as a function of boron addition, as obtained through modeling of synchrotron X-ray total scattering using Empirical Potential Structural Refinement. Boroaluminosilicate Glass structure EPSR NMR Saleh, Muad verfasserin aut Watson, Deborah verfasserin aut Martin, Steve W. verfasserin aut Crawford, Charles L. verfasserin aut McCloy, John S. verfasserin (orcid)0000-0001-7476-7771 aut Enthalten in Journal of non-crystalline solids Amsterdam [u.a.] : Elsevier Science, 1968 506, Seite 58-67 Online-Ressource (DE-627)306659808 (DE-600)1500501-X (DE-576)096806486 0022-3093 nnns volume:506 pages:58-67 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2008 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 51.45 Werkstoffe mit besonderen Eigenschaften 51.60 Keramische Werkstoffe Hartstoffe Werkstoffkunde 33.61 Festkörperphysik 35.90 Festkörperchemie AR 506 58-67
language	English
source	Enthalten in Journal of non-crystalline solids 506, Seite 58-67 volume:506 pages:58-67
sourceStr	Enthalten in Journal of non-crystalline solids 506, Seite 58-67 volume:506 pages:58-67
format_phy_str_mv	Article
bklname	Werkstoffe mit besonderen Eigenschaften Keramische Werkstoffe Hartstoffe Festkörperphysik Festkörperchemie
institution	findex.gbv.de
topic_facet	Boroaluminosilicate Glass structure EPSR NMR
dewey-raw	660
isfreeaccess_bool	false
container_title	Journal of non-crystalline solids
authorswithroles_txt_mv	Marcial, José @@aut@@ Saleh, Muad @@aut@@ Watson, Deborah @@aut@@ Martin, Steve W. @@aut@@ Crawford, Charles L. @@aut@@ McCloy, John S. @@aut@@
publishDateDaySort_date	2019-01-01T00:00:00Z
hierarchy_top_id	306659808
dewey-sort	3660
id	ELV001630288
language_de	englisch
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author	Marcial, José
spellingShingle	Marcial, José ddc 660 bkl 51.45 bkl 51.60 bkl 33.61 bkl 35.90 misc Boroaluminosilicate misc Glass structure misc EPSR misc NMR Boron-speciation and aluminosilicate crystallization in alkali boroaluminosilicate glasses along the NaAl
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topic_title	660 670 DE-600 51.45 bkl 51.60 bkl 33.61 bkl 35.90 bkl Boron-speciation and aluminosilicate crystallization in alkali boroaluminosilicate glasses along the NaAl Boroaluminosilicate Glass structure EPSR NMR
topic	ddc 660 bkl 51.45 bkl 51.60 bkl 33.61 bkl 35.90 misc Boroaluminosilicate misc Glass structure misc EPSR misc NMR
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title	Boron-speciation and aluminosilicate crystallization in alkali boroaluminosilicate glasses along the NaAl
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title_full	Boron-speciation and aluminosilicate crystallization in alkali boroaluminosilicate glasses along the NaAl
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title_sort	boron-speciation and aluminosilicate crystallization in alkali boroaluminosilicate glasses along the naal
title_auth	Boron-speciation and aluminosilicate crystallization in alkali boroaluminosilicate glasses along the NaAl
abstract	The influences of boron on silicate glass dissolution behavior and crystallization have long been important in the nuclear waste glass and technical glass communities. Boron is a challenging component to model due to this ability to assume three- and four-fold coordinations with oxygen, as well as its ability to form complex structural units with silicate tetrahedra. Furthermore, the low atomic mass limits the available characterization techniques. In the present work, recent literature findings on the compositional influence on boron speciation are implemented to interpret new data on alkali boroaluminosilicate glasses studied with 11B nuclear magnetic resonance (NMR), synchrotron X-ray scattering (s-XRS), and chemical durability measurements. The purpose of this study is to understand the influence of boron on the crystallization behavior of sodium and lithium aluminosilicate systems, NaAl1-xBxSiO4 and LiAl1-xBxSiO4, as applied to problems in nuclear waste vitrification. Comparisons are drawn between the alkali coordination number and crystallization behavior as a function of boron addition, as obtained through modeling of synchrotron X-ray total scattering using Empirical Potential Structural Refinement.
abstractGer	The influences of boron on silicate glass dissolution behavior and crystallization have long been important in the nuclear waste glass and technical glass communities. Boron is a challenging component to model due to this ability to assume three- and four-fold coordinations with oxygen, as well as its ability to form complex structural units with silicate tetrahedra. Furthermore, the low atomic mass limits the available characterization techniques. In the present work, recent literature findings on the compositional influence on boron speciation are implemented to interpret new data on alkali boroaluminosilicate glasses studied with 11B nuclear magnetic resonance (NMR), synchrotron X-ray scattering (s-XRS), and chemical durability measurements. The purpose of this study is to understand the influence of boron on the crystallization behavior of sodium and lithium aluminosilicate systems, NaAl1-xBxSiO4 and LiAl1-xBxSiO4, as applied to problems in nuclear waste vitrification. Comparisons are drawn between the alkali coordination number and crystallization behavior as a function of boron addition, as obtained through modeling of synchrotron X-ray total scattering using Empirical Potential Structural Refinement.
abstract_unstemmed	The influences of boron on silicate glass dissolution behavior and crystallization have long been important in the nuclear waste glass and technical glass communities. Boron is a challenging component to model due to this ability to assume three- and four-fold coordinations with oxygen, as well as its ability to form complex structural units with silicate tetrahedra. Furthermore, the low atomic mass limits the available characterization techniques. In the present work, recent literature findings on the compositional influence on boron speciation are implemented to interpret new data on alkali boroaluminosilicate glasses studied with 11B nuclear magnetic resonance (NMR), synchrotron X-ray scattering (s-XRS), and chemical durability measurements. The purpose of this study is to understand the influence of boron on the crystallization behavior of sodium and lithium aluminosilicate systems, NaAl1-xBxSiO4 and LiAl1-xBxSiO4, as applied to problems in nuclear waste vitrification. Comparisons are drawn between the alkali coordination number and crystallization behavior as a function of boron addition, as obtained through modeling of synchrotron X-ray total scattering using Empirical Potential Structural Refinement.
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title_short	Boron-speciation and aluminosilicate crystallization in alkali boroaluminosilicate glasses along the NaAl
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up_date	2024-07-06T22:02:01.435Z
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Boron-speciation and aluminosilicate crystallization in alkali boroaluminosilicate glasses along the NaAl

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