Silica nanoparticles doped with a benzo[
A reusable colorimetric and phosphorescent probe for continuous detection of bisulfite and Hg2+/Cu2+ in water has been rationally designed by silica nanoparticles doped with a new iridium(III) complex. In the presence of HSO3 −, it demonstrated intensively enhanced phosphorescence as w...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Li, Xianghong [verfasserIn] Zeng, Rongqing [verfasserIn] Xie, Chaoyi [verfasserIn] Tang, Dingguo [verfasserIn] Li, Qin [verfasserIn] Zhang, Bingguang [verfasserIn] Huang, Tao [verfasserIn] |
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| Format: |
E-Artikel |
|---|---|
| Sprache: |
Englisch |
| Erschienen: |
2019 |
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| Schlagwörter: |
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| Übergeordnetes Werk: |
Enthalten in: Dyes and pigments - Amsterdam [u.a.] : Elsevier Science, 1980, 165, Seite 128-136 |
|---|---|
| Übergeordnetes Werk: |
volume:165 ; pages:128-136 |
| DOI / URN: |
10.1016/j.dyepig.2019.02.018 |
|---|
| Katalog-ID: |
ELV001962906 |
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| 245 | 1 | 0 | |a Silica nanoparticles doped with a benzo[ |
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| 520 | |a A reusable colorimetric and phosphorescent probe for continuous detection of bisulfite and Hg2+/Cu2+ in water has been rationally designed by silica nanoparticles doped with a new iridium(III) complex. In the presence of HSO3 −, it demonstrated intensively enhanced phosphorescence as well as instantaneous solution color change from dark-green to light-yellow. However, it is interesting that the enhanced phosphorescence caused by bisulfite can be subsequently quenched by Hg2+ or Cu2+, and then be re-enhanced by the further addition of bisulfite. Moreover, a good linearity was observed between phosphorescent intensities of the probe and concentrations of HSO3 −, Hg2+ and Cu2+ with satisfactory detection limits of 0.80, 0.77 and 0.85 μM, respectively. It should be noted that this off-on-off phosphorescent process can be circled for several times by adding bisulfite and Hg2+ or Cu2+ alternately. As a result, the newly designed probe can be repeatedly used for detection of HSO3 −, Hg2+ and Cu2+ at low detection limits, which would be more efficient and less expensive than a one-to-one analysis method. | ||
| 650 | 4 | |a Silica nanoparticles | |
| 650 | 4 | |a Reusable probe | |
| 650 | 4 | |a Iridium(III) complex | |
| 650 | 4 | |a Hg | |
| 650 | 4 | |a HSO | |
| 650 | 4 | |a Phosphorescence | |
| 700 | 1 | |a Zeng, Rongqing |e verfasserin |4 aut | |
| 700 | 1 | |a Xie, Chaoyi |e verfasserin |4 aut | |
| 700 | 1 | |a Tang, Dingguo |e verfasserin |4 aut | |
| 700 | 1 | |a Li, Qin |e verfasserin |4 aut | |
| 700 | 1 | |a Zhang, Bingguang |e verfasserin |4 aut | |
| 700 | 1 | |a Huang, Tao |e verfasserin |4 aut | |
| 773 | 0 | 8 | |i Enthalten in |t Dyes and pigments |d Amsterdam [u.a.] : Elsevier Science, 1980 |g 165, Seite 128-136 |h Online-Ressource |w (DE-627)306658755 |w (DE-600)1500382-6 |w (DE-576)116550910 |x 0143-7208 |7 nnns |
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| 936 | b | k | |a 58.26 |j Technologie der Farben und Lacke |
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10.1016/j.dyepig.2019.02.018 doi (DE-627)ELV001962906 (ELSEVIER)S0143-7208(18)32346-5 DE-627 ger DE-627 rda eng 660 DE-600 58.26 bkl Li, Xianghong verfasserin aut Silica nanoparticles doped with a benzo[ 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A reusable colorimetric and phosphorescent probe for continuous detection of bisulfite and Hg2+/Cu2+ in water has been rationally designed by silica nanoparticles doped with a new iridium(III) complex. In the presence of HSO3 −, it demonstrated intensively enhanced phosphorescence as well as instantaneous solution color change from dark-green to light-yellow. However, it is interesting that the enhanced phosphorescence caused by bisulfite can be subsequently quenched by Hg2+ or Cu2+, and then be re-enhanced by the further addition of bisulfite. Moreover, a good linearity was observed between phosphorescent intensities of the probe and concentrations of HSO3 −, Hg2+ and Cu2+ with satisfactory detection limits of 0.80, 0.77 and 0.85 μM, respectively. It should be noted that this off-on-off phosphorescent process can be circled for several times by adding bisulfite and Hg2+ or Cu2+ alternately. As a result, the newly designed probe can be repeatedly used for detection of HSO3 −, Hg2+ and Cu2+ at low detection limits, which would be more efficient and less expensive than a one-to-one analysis method. Silica nanoparticles Reusable probe Iridium(III) complex Hg HSO Phosphorescence Zeng, Rongqing verfasserin aut Xie, Chaoyi verfasserin aut Tang, Dingguo verfasserin aut Li, Qin verfasserin aut Zhang, Bingguang verfasserin aut Huang, Tao verfasserin aut Enthalten in Dyes and pigments Amsterdam [u.a.] : Elsevier Science, 1980 165, Seite 128-136 Online-Ressource (DE-627)306658755 (DE-600)1500382-6 (DE-576)116550910 0143-7208 nnns volume:165 pages:128-136 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.26 Technologie der Farben und Lacke AR 165 128-136 |
| spelling |
10.1016/j.dyepig.2019.02.018 doi (DE-627)ELV001962906 (ELSEVIER)S0143-7208(18)32346-5 DE-627 ger DE-627 rda eng 660 DE-600 58.26 bkl Li, Xianghong verfasserin aut Silica nanoparticles doped with a benzo[ 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A reusable colorimetric and phosphorescent probe for continuous detection of bisulfite and Hg2+/Cu2+ in water has been rationally designed by silica nanoparticles doped with a new iridium(III) complex. In the presence of HSO3 −, it demonstrated intensively enhanced phosphorescence as well as instantaneous solution color change from dark-green to light-yellow. However, it is interesting that the enhanced phosphorescence caused by bisulfite can be subsequently quenched by Hg2+ or Cu2+, and then be re-enhanced by the further addition of bisulfite. Moreover, a good linearity was observed between phosphorescent intensities of the probe and concentrations of HSO3 −, Hg2+ and Cu2+ with satisfactory detection limits of 0.80, 0.77 and 0.85 μM, respectively. It should be noted that this off-on-off phosphorescent process can be circled for several times by adding bisulfite and Hg2+ or Cu2+ alternately. As a result, the newly designed probe can be repeatedly used for detection of HSO3 −, Hg2+ and Cu2+ at low detection limits, which would be more efficient and less expensive than a one-to-one analysis method. Silica nanoparticles Reusable probe Iridium(III) complex Hg HSO Phosphorescence Zeng, Rongqing verfasserin aut Xie, Chaoyi verfasserin aut Tang, Dingguo verfasserin aut Li, Qin verfasserin aut Zhang, Bingguang verfasserin aut Huang, Tao verfasserin aut Enthalten in Dyes and pigments Amsterdam [u.a.] : Elsevier Science, 1980 165, Seite 128-136 Online-Ressource (DE-627)306658755 (DE-600)1500382-6 (DE-576)116550910 0143-7208 nnns volume:165 pages:128-136 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.26 Technologie der Farben und Lacke AR 165 128-136 |
| allfields_unstemmed |
10.1016/j.dyepig.2019.02.018 doi (DE-627)ELV001962906 (ELSEVIER)S0143-7208(18)32346-5 DE-627 ger DE-627 rda eng 660 DE-600 58.26 bkl Li, Xianghong verfasserin aut Silica nanoparticles doped with a benzo[ 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A reusable colorimetric and phosphorescent probe for continuous detection of bisulfite and Hg2+/Cu2+ in water has been rationally designed by silica nanoparticles doped with a new iridium(III) complex. In the presence of HSO3 −, it demonstrated intensively enhanced phosphorescence as well as instantaneous solution color change from dark-green to light-yellow. However, it is interesting that the enhanced phosphorescence caused by bisulfite can be subsequently quenched by Hg2+ or Cu2+, and then be re-enhanced by the further addition of bisulfite. Moreover, a good linearity was observed between phosphorescent intensities of the probe and concentrations of HSO3 −, Hg2+ and Cu2+ with satisfactory detection limits of 0.80, 0.77 and 0.85 μM, respectively. It should be noted that this off-on-off phosphorescent process can be circled for several times by adding bisulfite and Hg2+ or Cu2+ alternately. As a result, the newly designed probe can be repeatedly used for detection of HSO3 −, Hg2+ and Cu2+ at low detection limits, which would be more efficient and less expensive than a one-to-one analysis method. Silica nanoparticles Reusable probe Iridium(III) complex Hg HSO Phosphorescence Zeng, Rongqing verfasserin aut Xie, Chaoyi verfasserin aut Tang, Dingguo verfasserin aut Li, Qin verfasserin aut Zhang, Bingguang verfasserin aut Huang, Tao verfasserin aut Enthalten in Dyes and pigments Amsterdam [u.a.] : Elsevier Science, 1980 165, Seite 128-136 Online-Ressource (DE-627)306658755 (DE-600)1500382-6 (DE-576)116550910 0143-7208 nnns volume:165 pages:128-136 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.26 Technologie der Farben und Lacke AR 165 128-136 |
| allfieldsGer |
10.1016/j.dyepig.2019.02.018 doi (DE-627)ELV001962906 (ELSEVIER)S0143-7208(18)32346-5 DE-627 ger DE-627 rda eng 660 DE-600 58.26 bkl Li, Xianghong verfasserin aut Silica nanoparticles doped with a benzo[ 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A reusable colorimetric and phosphorescent probe for continuous detection of bisulfite and Hg2+/Cu2+ in water has been rationally designed by silica nanoparticles doped with a new iridium(III) complex. In the presence of HSO3 −, it demonstrated intensively enhanced phosphorescence as well as instantaneous solution color change from dark-green to light-yellow. However, it is interesting that the enhanced phosphorescence caused by bisulfite can be subsequently quenched by Hg2+ or Cu2+, and then be re-enhanced by the further addition of bisulfite. Moreover, a good linearity was observed between phosphorescent intensities of the probe and concentrations of HSO3 −, Hg2+ and Cu2+ with satisfactory detection limits of 0.80, 0.77 and 0.85 μM, respectively. It should be noted that this off-on-off phosphorescent process can be circled for several times by adding bisulfite and Hg2+ or Cu2+ alternately. As a result, the newly designed probe can be repeatedly used for detection of HSO3 −, Hg2+ and Cu2+ at low detection limits, which would be more efficient and less expensive than a one-to-one analysis method. Silica nanoparticles Reusable probe Iridium(III) complex Hg HSO Phosphorescence Zeng, Rongqing verfasserin aut Xie, Chaoyi verfasserin aut Tang, Dingguo verfasserin aut Li, Qin verfasserin aut Zhang, Bingguang verfasserin aut Huang, Tao verfasserin aut Enthalten in Dyes and pigments Amsterdam [u.a.] : Elsevier Science, 1980 165, Seite 128-136 Online-Ressource (DE-627)306658755 (DE-600)1500382-6 (DE-576)116550910 0143-7208 nnns volume:165 pages:128-136 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.26 Technologie der Farben und Lacke AR 165 128-136 |
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10.1016/j.dyepig.2019.02.018 doi (DE-627)ELV001962906 (ELSEVIER)S0143-7208(18)32346-5 DE-627 ger DE-627 rda eng 660 DE-600 58.26 bkl Li, Xianghong verfasserin aut Silica nanoparticles doped with a benzo[ 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A reusable colorimetric and phosphorescent probe for continuous detection of bisulfite and Hg2+/Cu2+ in water has been rationally designed by silica nanoparticles doped with a new iridium(III) complex. In the presence of HSO3 −, it demonstrated intensively enhanced phosphorescence as well as instantaneous solution color change from dark-green to light-yellow. However, it is interesting that the enhanced phosphorescence caused by bisulfite can be subsequently quenched by Hg2+ or Cu2+, and then be re-enhanced by the further addition of bisulfite. Moreover, a good linearity was observed between phosphorescent intensities of the probe and concentrations of HSO3 −, Hg2+ and Cu2+ with satisfactory detection limits of 0.80, 0.77 and 0.85 μM, respectively. It should be noted that this off-on-off phosphorescent process can be circled for several times by adding bisulfite and Hg2+ or Cu2+ alternately. As a result, the newly designed probe can be repeatedly used for detection of HSO3 −, Hg2+ and Cu2+ at low detection limits, which would be more efficient and less expensive than a one-to-one analysis method. Silica nanoparticles Reusable probe Iridium(III) complex Hg HSO Phosphorescence Zeng, Rongqing verfasserin aut Xie, Chaoyi verfasserin aut Tang, Dingguo verfasserin aut Li, Qin verfasserin aut Zhang, Bingguang verfasserin aut Huang, Tao verfasserin aut Enthalten in Dyes and pigments Amsterdam [u.a.] : Elsevier Science, 1980 165, Seite 128-136 Online-Ressource (DE-627)306658755 (DE-600)1500382-6 (DE-576)116550910 0143-7208 nnns volume:165 pages:128-136 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.26 Technologie der Farben und Lacke AR 165 128-136 |
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660 DE-600 58.26 bkl Silica nanoparticles doped with a benzo[ Silica nanoparticles Reusable probe Iridium(III) complex Hg HSO Phosphorescence |
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silica nanoparticles doped with a benzo[ |
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A reusable colorimetric and phosphorescent probe for continuous detection of bisulfite and Hg2+/Cu2+ in water has been rationally designed by silica nanoparticles doped with a new iridium(III) complex. In the presence of HSO3 −, it demonstrated intensively enhanced phosphorescence as well as instantaneous solution color change from dark-green to light-yellow. However, it is interesting that the enhanced phosphorescence caused by bisulfite can be subsequently quenched by Hg2+ or Cu2+, and then be re-enhanced by the further addition of bisulfite. Moreover, a good linearity was observed between phosphorescent intensities of the probe and concentrations of HSO3 −, Hg2+ and Cu2+ with satisfactory detection limits of 0.80, 0.77 and 0.85 μM, respectively. It should be noted that this off-on-off phosphorescent process can be circled for several times by adding bisulfite and Hg2+ or Cu2+ alternately. As a result, the newly designed probe can be repeatedly used for detection of HSO3 −, Hg2+ and Cu2+ at low detection limits, which would be more efficient and less expensive than a one-to-one analysis method. |
| abstractGer |
A reusable colorimetric and phosphorescent probe for continuous detection of bisulfite and Hg2+/Cu2+ in water has been rationally designed by silica nanoparticles doped with a new iridium(III) complex. In the presence of HSO3 −, it demonstrated intensively enhanced phosphorescence as well as instantaneous solution color change from dark-green to light-yellow. However, it is interesting that the enhanced phosphorescence caused by bisulfite can be subsequently quenched by Hg2+ or Cu2+, and then be re-enhanced by the further addition of bisulfite. Moreover, a good linearity was observed between phosphorescent intensities of the probe and concentrations of HSO3 −, Hg2+ and Cu2+ with satisfactory detection limits of 0.80, 0.77 and 0.85 μM, respectively. It should be noted that this off-on-off phosphorescent process can be circled for several times by adding bisulfite and Hg2+ or Cu2+ alternately. As a result, the newly designed probe can be repeatedly used for detection of HSO3 −, Hg2+ and Cu2+ at low detection limits, which would be more efficient and less expensive than a one-to-one analysis method. |
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A reusable colorimetric and phosphorescent probe for continuous detection of bisulfite and Hg2+/Cu2+ in water has been rationally designed by silica nanoparticles doped with a new iridium(III) complex. In the presence of HSO3 −, it demonstrated intensively enhanced phosphorescence as well as instantaneous solution color change from dark-green to light-yellow. However, it is interesting that the enhanced phosphorescence caused by bisulfite can be subsequently quenched by Hg2+ or Cu2+, and then be re-enhanced by the further addition of bisulfite. Moreover, a good linearity was observed between phosphorescent intensities of the probe and concentrations of HSO3 −, Hg2+ and Cu2+ with satisfactory detection limits of 0.80, 0.77 and 0.85 μM, respectively. It should be noted that this off-on-off phosphorescent process can be circled for several times by adding bisulfite and Hg2+ or Cu2+ alternately. As a result, the newly designed probe can be repeatedly used for detection of HSO3 −, Hg2+ and Cu2+ at low detection limits, which would be more efficient and less expensive than a one-to-one analysis method. |
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