Construction of highly conductive network for improving electrochemical performance of lithium iron phosphate

High performance lithium iron phosphate (LFP) cathode materials were synthesized using amorphous carbon, carbon nanotubes (CNTs), and graphene (G) as conductive materials via sand milling and spray drying processes and followed by calcination. The structural characterizations indicated that CNTs and...
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Autor*in:	Cai, Yezheng [verfasserIn] Huang, Dequan [verfasserIn] Ma, Zhaoling [verfasserIn] Wang, Hongqiang [verfasserIn] Huang, Youguo [verfasserIn] Wu, Xianwen [verfasserIn] Li, Qingyu [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2019

Schlagwörter:	Lithium ion battery Cathode material Conductivity network Carbon nanotubes Graphene

Übergeordnetes Werk:	Enthalten in: Electrochimica acta - New York, NY [u.a.] : Elsevier, 1959, 305, Seite 563-570
Übergeordnetes Werk:	volume:305 ; pages:563-570

DOI / URN:	10.1016/j.electacta.2019.02.114

Katalog-ID:	ELV001997343

Internformat


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245	1	0	\|a Construction of highly conductive network for improving electrochemical performance of lithium iron phosphate
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520			\|a High performance lithium iron phosphate (LFP) cathode materials were synthesized using amorphous carbon, carbon nanotubes (CNTs), and graphene (G) as conductive materials via sand milling and spray drying processes and followed by calcination. The structural characterizations indicated that CNTs and G can well connected with LFP nanoparticles (NPs), which was coated with a thin layer of amorphous carbon, benefiting the construction of three-dimensional efficient conductive network. The electrochemical measurements confirmed that the introduction of CNTs and G can obviously decrease the charge transfer impedance of lithium ion battery and increase the discharge special capacity. The initial discharge special capacity increases in the order of LFP/C (150.3 mAh/g) < LFP/C/CNTs (155.7 mAh/g) < LFP/C/G (159.7 mAh/g) < LFP/C/G/CNTs (164.5 mAh/g) at 0.1 C. LFP/C/G/CNTs also exhibited considerable discharge special capacity (99.5 mAh/g) at high current of 5 C. Compared with LFP/C (248 Ω), LFP/C/G/CNTs (50 Ω) showed obviously decreased charge transfer impedance. Cycle performance test indicated that the specific capacity retention for LFP/C/G/CNTs was 99% after 200 cycles, displaying good cycle stability. The superior electrochemical performance of LFP/C/G/CNTs is attributed to the significantly synergistic effect of CNTs and G on decreasing charge transfer impedance by constructing highly three-dimensional conductive network. Besides, the effect of G to CNTs mass ratio and the calcination temperature on the electrochemical performance of LIBs were also discussed.
650		4	\|a Lithium ion battery
650		4	\|a Cathode material
650		4	\|a Conductivity network
650		4	\|a Carbon nanotubes
650		4	\|a Graphene
700	1		\|a Huang, Dequan \|e verfasserin \|4 aut
700	1		\|a Ma, Zhaoling \|e verfasserin \|4 aut
700	1		\|a Wang, Hongqiang \|e verfasserin \|4 aut
700	1		\|a Huang, Youguo \|e verfasserin \|4 aut
700	1		\|a Wu, Xianwen \|e verfasserin \|4 aut
700	1		\|a Li, Qingyu \|e verfasserin \|4 aut
773	0	8	\|i Enthalten in \|t Electrochimica acta \|d New York, NY [u.a.] : Elsevier, 1959 \|g 305, Seite 563-570 \|h Online-Ressource \|w (DE-627)300897561 \|w (DE-600)1483548-4 \|w (DE-576)094752451 \|x 1873-3859 \|7 nnns
773	1	8	\|g volume:305 \|g pages:563-570
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912			\|a GBV_ILN_31
912			\|a GBV_ILN_32
912			\|a GBV_ILN_40
912			\|a GBV_ILN_60
912			\|a GBV_ILN_62
912			\|a GBV_ILN_63
912			\|a GBV_ILN_65
912			\|a GBV_ILN_69
912			\|a GBV_ILN_70
912			\|a GBV_ILN_73
912			\|a GBV_ILN_74
912			\|a GBV_ILN_90
912			\|a GBV_ILN_95
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912			\|a GBV_ILN_105
912			\|a GBV_ILN_110
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912			\|a GBV_ILN_370
912			\|a GBV_ILN_602
912			\|a GBV_ILN_702
912			\|a GBV_ILN_2003
912			\|a GBV_ILN_2004
912			\|a GBV_ILN_2005
912			\|a GBV_ILN_2011
912			\|a GBV_ILN_2014
912			\|a GBV_ILN_2015
912			\|a GBV_ILN_2020
912			\|a GBV_ILN_2021
912			\|a GBV_ILN_2025
912			\|a GBV_ILN_2027
912			\|a GBV_ILN_2034
912			\|a GBV_ILN_2038
912			\|a GBV_ILN_2044
912			\|a GBV_ILN_2048
912			\|a GBV_ILN_2049
912			\|a GBV_ILN_2050
912			\|a GBV_ILN_2056
912			\|a GBV_ILN_2059
912			\|a GBV_ILN_2061
912			\|a GBV_ILN_2064
912			\|a GBV_ILN_2065
912			\|a GBV_ILN_2068
912			\|a GBV_ILN_2111
912			\|a GBV_ILN_2112
912			\|a GBV_ILN_2113
912			\|a GBV_ILN_2118
912			\|a GBV_ILN_2122
912			\|a GBV_ILN_2129
912			\|a GBV_ILN_2143
912			\|a GBV_ILN_2147
912			\|a GBV_ILN_2148
912			\|a GBV_ILN_2152
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912			\|a GBV_ILN_2507
912			\|a GBV_ILN_2522
912			\|a GBV_ILN_4035
912			\|a GBV_ILN_4037
912			\|a GBV_ILN_4112
912			\|a GBV_ILN_4125
912			\|a GBV_ILN_4126
912			\|a GBV_ILN_4242
912			\|a GBV_ILN_4251
912			\|a GBV_ILN_4305
912			\|a GBV_ILN_4313
912			\|a GBV_ILN_4323
912			\|a GBV_ILN_4324
912			\|a GBV_ILN_4326
912			\|a GBV_ILN_4333
912			\|a GBV_ILN_4334
912			\|a GBV_ILN_4335
912			\|a GBV_ILN_4338
912			\|a GBV_ILN_4393
936	b	k	\|a 35.00 \|j Chemie: Allgemeines
951			\|a AR
952			\|d 305 \|h 563-570

Indexfelder

author_variant	y c yc d h dh z m zm h w hw y h yh x w xw q l ql
matchkey_str	article:18733859:2019----::osrcinfihyodcieewrfrmrvneetohmclefra
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publishDate	2019
allfields	10.1016/j.electacta.2019.02.114 doi (DE-627)ELV001997343 (ELSEVIER)S0013-4686(19)30384-6 DE-627 ger DE-627 rda eng 540 DE-600 35.00 bkl Cai, Yezheng verfasserin aut Construction of highly conductive network for improving electrochemical performance of lithium iron phosphate 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier High performance lithium iron phosphate (LFP) cathode materials were synthesized using amorphous carbon, carbon nanotubes (CNTs), and graphene (G) as conductive materials via sand milling and spray drying processes and followed by calcination. The structural characterizations indicated that CNTs and G can well connected with LFP nanoparticles (NPs), which was coated with a thin layer of amorphous carbon, benefiting the construction of three-dimensional efficient conductive network. The electrochemical measurements confirmed that the introduction of CNTs and G can obviously decrease the charge transfer impedance of lithium ion battery and increase the discharge special capacity. The initial discharge special capacity increases in the order of LFP/C (150.3 mAh/g) < LFP/C/CNTs (155.7 mAh/g) < LFP/C/G (159.7 mAh/g) < LFP/C/G/CNTs (164.5 mAh/g) at 0.1 C. LFP/C/G/CNTs also exhibited considerable discharge special capacity (99.5 mAh/g) at high current of 5 C. Compared with LFP/C (248 Ω), LFP/C/G/CNTs (50 Ω) showed obviously decreased charge transfer impedance. Cycle performance test indicated that the specific capacity retention for LFP/C/G/CNTs was 99% after 200 cycles, displaying good cycle stability. The superior electrochemical performance of LFP/C/G/CNTs is attributed to the significantly synergistic effect of CNTs and G on decreasing charge transfer impedance by constructing highly three-dimensional conductive network. Besides, the effect of G to CNTs mass ratio and the calcination temperature on the electrochemical performance of LIBs were also discussed. Lithium ion battery Cathode material Conductivity network Carbon nanotubes Graphene Huang, Dequan verfasserin aut Ma, Zhaoling verfasserin aut Wang, Hongqiang verfasserin aut Huang, Youguo verfasserin aut Wu, Xianwen verfasserin aut Li, Qingyu verfasserin aut Enthalten in Electrochimica acta New York, NY [u.a.] : Elsevier, 1959 305, Seite 563-570 Online-Ressource (DE-627)300897561 (DE-600)1483548-4 (DE-576)094752451 1873-3859 nnns volume:305 pages:563-570 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.00 Chemie: Allgemeines AR 305 563-570
spelling	10.1016/j.electacta.2019.02.114 doi (DE-627)ELV001997343 (ELSEVIER)S0013-4686(19)30384-6 DE-627 ger DE-627 rda eng 540 DE-600 35.00 bkl Cai, Yezheng verfasserin aut Construction of highly conductive network for improving electrochemical performance of lithium iron phosphate 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier High performance lithium iron phosphate (LFP) cathode materials were synthesized using amorphous carbon, carbon nanotubes (CNTs), and graphene (G) as conductive materials via sand milling and spray drying processes and followed by calcination. The structural characterizations indicated that CNTs and G can well connected with LFP nanoparticles (NPs), which was coated with a thin layer of amorphous carbon, benefiting the construction of three-dimensional efficient conductive network. The electrochemical measurements confirmed that the introduction of CNTs and G can obviously decrease the charge transfer impedance of lithium ion battery and increase the discharge special capacity. The initial discharge special capacity increases in the order of LFP/C (150.3 mAh/g) < LFP/C/CNTs (155.7 mAh/g) < LFP/C/G (159.7 mAh/g) < LFP/C/G/CNTs (164.5 mAh/g) at 0.1 C. LFP/C/G/CNTs also exhibited considerable discharge special capacity (99.5 mAh/g) at high current of 5 C. Compared with LFP/C (248 Ω), LFP/C/G/CNTs (50 Ω) showed obviously decreased charge transfer impedance. Cycle performance test indicated that the specific capacity retention for LFP/C/G/CNTs was 99% after 200 cycles, displaying good cycle stability. The superior electrochemical performance of LFP/C/G/CNTs is attributed to the significantly synergistic effect of CNTs and G on decreasing charge transfer impedance by constructing highly three-dimensional conductive network. Besides, the effect of G to CNTs mass ratio and the calcination temperature on the electrochemical performance of LIBs were also discussed. Lithium ion battery Cathode material Conductivity network Carbon nanotubes Graphene Huang, Dequan verfasserin aut Ma, Zhaoling verfasserin aut Wang, Hongqiang verfasserin aut Huang, Youguo verfasserin aut Wu, Xianwen verfasserin aut Li, Qingyu verfasserin aut Enthalten in Electrochimica acta New York, NY [u.a.] : Elsevier, 1959 305, Seite 563-570 Online-Ressource (DE-627)300897561 (DE-600)1483548-4 (DE-576)094752451 1873-3859 nnns volume:305 pages:563-570 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.00 Chemie: Allgemeines AR 305 563-570
allfields_unstemmed	10.1016/j.electacta.2019.02.114 doi (DE-627)ELV001997343 (ELSEVIER)S0013-4686(19)30384-6 DE-627 ger DE-627 rda eng 540 DE-600 35.00 bkl Cai, Yezheng verfasserin aut Construction of highly conductive network for improving electrochemical performance of lithium iron phosphate 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier High performance lithium iron phosphate (LFP) cathode materials were synthesized using amorphous carbon, carbon nanotubes (CNTs), and graphene (G) as conductive materials via sand milling and spray drying processes and followed by calcination. The structural characterizations indicated that CNTs and G can well connected with LFP nanoparticles (NPs), which was coated with a thin layer of amorphous carbon, benefiting the construction of three-dimensional efficient conductive network. The electrochemical measurements confirmed that the introduction of CNTs and G can obviously decrease the charge transfer impedance of lithium ion battery and increase the discharge special capacity. The initial discharge special capacity increases in the order of LFP/C (150.3 mAh/g) < LFP/C/CNTs (155.7 mAh/g) < LFP/C/G (159.7 mAh/g) < LFP/C/G/CNTs (164.5 mAh/g) at 0.1 C. LFP/C/G/CNTs also exhibited considerable discharge special capacity (99.5 mAh/g) at high current of 5 C. Compared with LFP/C (248 Ω), LFP/C/G/CNTs (50 Ω) showed obviously decreased charge transfer impedance. Cycle performance test indicated that the specific capacity retention for LFP/C/G/CNTs was 99% after 200 cycles, displaying good cycle stability. The superior electrochemical performance of LFP/C/G/CNTs is attributed to the significantly synergistic effect of CNTs and G on decreasing charge transfer impedance by constructing highly three-dimensional conductive network. Besides, the effect of G to CNTs mass ratio and the calcination temperature on the electrochemical performance of LIBs were also discussed. Lithium ion battery Cathode material Conductivity network Carbon nanotubes Graphene Huang, Dequan verfasserin aut Ma, Zhaoling verfasserin aut Wang, Hongqiang verfasserin aut Huang, Youguo verfasserin aut Wu, Xianwen verfasserin aut Li, Qingyu verfasserin aut Enthalten in Electrochimica acta New York, NY [u.a.] : Elsevier, 1959 305, Seite 563-570 Online-Ressource (DE-627)300897561 (DE-600)1483548-4 (DE-576)094752451 1873-3859 nnns volume:305 pages:563-570 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.00 Chemie: Allgemeines AR 305 563-570
allfieldsGer	10.1016/j.electacta.2019.02.114 doi (DE-627)ELV001997343 (ELSEVIER)S0013-4686(19)30384-6 DE-627 ger DE-627 rda eng 540 DE-600 35.00 bkl Cai, Yezheng verfasserin aut Construction of highly conductive network for improving electrochemical performance of lithium iron phosphate 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier High performance lithium iron phosphate (LFP) cathode materials were synthesized using amorphous carbon, carbon nanotubes (CNTs), and graphene (G) as conductive materials via sand milling and spray drying processes and followed by calcination. The structural characterizations indicated that CNTs and G can well connected with LFP nanoparticles (NPs), which was coated with a thin layer of amorphous carbon, benefiting the construction of three-dimensional efficient conductive network. The electrochemical measurements confirmed that the introduction of CNTs and G can obviously decrease the charge transfer impedance of lithium ion battery and increase the discharge special capacity. The initial discharge special capacity increases in the order of LFP/C (150.3 mAh/g) < LFP/C/CNTs (155.7 mAh/g) < LFP/C/G (159.7 mAh/g) < LFP/C/G/CNTs (164.5 mAh/g) at 0.1 C. LFP/C/G/CNTs also exhibited considerable discharge special capacity (99.5 mAh/g) at high current of 5 C. Compared with LFP/C (248 Ω), LFP/C/G/CNTs (50 Ω) showed obviously decreased charge transfer impedance. Cycle performance test indicated that the specific capacity retention for LFP/C/G/CNTs was 99% after 200 cycles, displaying good cycle stability. The superior electrochemical performance of LFP/C/G/CNTs is attributed to the significantly synergistic effect of CNTs and G on decreasing charge transfer impedance by constructing highly three-dimensional conductive network. Besides, the effect of G to CNTs mass ratio and the calcination temperature on the electrochemical performance of LIBs were also discussed. Lithium ion battery Cathode material Conductivity network Carbon nanotubes Graphene Huang, Dequan verfasserin aut Ma, Zhaoling verfasserin aut Wang, Hongqiang verfasserin aut Huang, Youguo verfasserin aut Wu, Xianwen verfasserin aut Li, Qingyu verfasserin aut Enthalten in Electrochimica acta New York, NY [u.a.] : Elsevier, 1959 305, Seite 563-570 Online-Ressource (DE-627)300897561 (DE-600)1483548-4 (DE-576)094752451 1873-3859 nnns volume:305 pages:563-570 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.00 Chemie: Allgemeines AR 305 563-570
allfieldsSound	10.1016/j.electacta.2019.02.114 doi (DE-627)ELV001997343 (ELSEVIER)S0013-4686(19)30384-6 DE-627 ger DE-627 rda eng 540 DE-600 35.00 bkl Cai, Yezheng verfasserin aut Construction of highly conductive network for improving electrochemical performance of lithium iron phosphate 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier High performance lithium iron phosphate (LFP) cathode materials were synthesized using amorphous carbon, carbon nanotubes (CNTs), and graphene (G) as conductive materials via sand milling and spray drying processes and followed by calcination. The structural characterizations indicated that CNTs and G can well connected with LFP nanoparticles (NPs), which was coated with a thin layer of amorphous carbon, benefiting the construction of three-dimensional efficient conductive network. The electrochemical measurements confirmed that the introduction of CNTs and G can obviously decrease the charge transfer impedance of lithium ion battery and increase the discharge special capacity. The initial discharge special capacity increases in the order of LFP/C (150.3 mAh/g) < LFP/C/CNTs (155.7 mAh/g) < LFP/C/G (159.7 mAh/g) < LFP/C/G/CNTs (164.5 mAh/g) at 0.1 C. LFP/C/G/CNTs also exhibited considerable discharge special capacity (99.5 mAh/g) at high current of 5 C. Compared with LFP/C (248 Ω), LFP/C/G/CNTs (50 Ω) showed obviously decreased charge transfer impedance. Cycle performance test indicated that the specific capacity retention for LFP/C/G/CNTs was 99% after 200 cycles, displaying good cycle stability. The superior electrochemical performance of LFP/C/G/CNTs is attributed to the significantly synergistic effect of CNTs and G on decreasing charge transfer impedance by constructing highly three-dimensional conductive network. Besides, the effect of G to CNTs mass ratio and the calcination temperature on the electrochemical performance of LIBs were also discussed. Lithium ion battery Cathode material Conductivity network Carbon nanotubes Graphene Huang, Dequan verfasserin aut Ma, Zhaoling verfasserin aut Wang, Hongqiang verfasserin aut Huang, Youguo verfasserin aut Wu, Xianwen verfasserin aut Li, Qingyu verfasserin aut Enthalten in Electrochimica acta New York, NY [u.a.] : Elsevier, 1959 305, Seite 563-570 Online-Ressource (DE-627)300897561 (DE-600)1483548-4 (DE-576)094752451 1873-3859 nnns volume:305 pages:563-570 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.00 Chemie: Allgemeines AR 305 563-570
language	English
source	Enthalten in Electrochimica acta 305, Seite 563-570 volume:305 pages:563-570
sourceStr	Enthalten in Electrochimica acta 305, Seite 563-570 volume:305 pages:563-570
format_phy_str_mv	Article
bklname	Chemie: Allgemeines
institution	findex.gbv.de
topic_facet	Lithium ion battery Cathode material Conductivity network Carbon nanotubes Graphene
dewey-raw	540
isfreeaccess_bool	false
container_title	Electrochimica acta
authorswithroles_txt_mv	Cai, Yezheng @@aut@@ Huang, Dequan @@aut@@ Ma, Zhaoling @@aut@@ Wang, Hongqiang @@aut@@ Huang, Youguo @@aut@@ Wu, Xianwen @@aut@@ Li, Qingyu @@aut@@
publishDateDaySort_date	2019-01-01T00:00:00Z
hierarchy_top_id	300897561
dewey-sort	3540
id	ELV001997343
language_de	englisch
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author	Cai, Yezheng
spellingShingle	Cai, Yezheng ddc 540 bkl 35.00 misc Lithium ion battery misc Cathode material misc Conductivity network misc Carbon nanotubes misc Graphene Construction of highly conductive network for improving electrochemical performance of lithium iron phosphate
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topic_title	540 DE-600 35.00 bkl Construction of highly conductive network for improving electrochemical performance of lithium iron phosphate Lithium ion battery Cathode material Conductivity network Carbon nanotubes Graphene
topic	ddc 540 bkl 35.00 misc Lithium ion battery misc Cathode material misc Conductivity network misc Carbon nanotubes misc Graphene
topic_unstemmed	ddc 540 bkl 35.00 misc Lithium ion battery misc Cathode material misc Conductivity network misc Carbon nanotubes misc Graphene
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title	Construction of highly conductive network for improving electrochemical performance of lithium iron phosphate
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title_full	Construction of highly conductive network for improving electrochemical performance of lithium iron phosphate
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author_browse	Cai, Yezheng Huang, Dequan Ma, Zhaoling Wang, Hongqiang Huang, Youguo Wu, Xianwen Li, Qingyu
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title_sort	construction of highly conductive network for improving electrochemical performance of lithium iron phosphate
title_auth	Construction of highly conductive network for improving electrochemical performance of lithium iron phosphate
abstract	High performance lithium iron phosphate (LFP) cathode materials were synthesized using amorphous carbon, carbon nanotubes (CNTs), and graphene (G) as conductive materials via sand milling and spray drying processes and followed by calcination. The structural characterizations indicated that CNTs and G can well connected with LFP nanoparticles (NPs), which was coated with a thin layer of amorphous carbon, benefiting the construction of three-dimensional efficient conductive network. The electrochemical measurements confirmed that the introduction of CNTs and G can obviously decrease the charge transfer impedance of lithium ion battery and increase the discharge special capacity. The initial discharge special capacity increases in the order of LFP/C (150.3 mAh/g) < LFP/C/CNTs (155.7 mAh/g) < LFP/C/G (159.7 mAh/g) < LFP/C/G/CNTs (164.5 mAh/g) at 0.1 C. LFP/C/G/CNTs also exhibited considerable discharge special capacity (99.5 mAh/g) at high current of 5 C. Compared with LFP/C (248 Ω), LFP/C/G/CNTs (50 Ω) showed obviously decreased charge transfer impedance. Cycle performance test indicated that the specific capacity retention for LFP/C/G/CNTs was 99% after 200 cycles, displaying good cycle stability. The superior electrochemical performance of LFP/C/G/CNTs is attributed to the significantly synergistic effect of CNTs and G on decreasing charge transfer impedance by constructing highly three-dimensional conductive network. Besides, the effect of G to CNTs mass ratio and the calcination temperature on the electrochemical performance of LIBs were also discussed.
abstractGer	High performance lithium iron phosphate (LFP) cathode materials were synthesized using amorphous carbon, carbon nanotubes (CNTs), and graphene (G) as conductive materials via sand milling and spray drying processes and followed by calcination. The structural characterizations indicated that CNTs and G can well connected with LFP nanoparticles (NPs), which was coated with a thin layer of amorphous carbon, benefiting the construction of three-dimensional efficient conductive network. The electrochemical measurements confirmed that the introduction of CNTs and G can obviously decrease the charge transfer impedance of lithium ion battery and increase the discharge special capacity. The initial discharge special capacity increases in the order of LFP/C (150.3 mAh/g) < LFP/C/CNTs (155.7 mAh/g) < LFP/C/G (159.7 mAh/g) < LFP/C/G/CNTs (164.5 mAh/g) at 0.1 C. LFP/C/G/CNTs also exhibited considerable discharge special capacity (99.5 mAh/g) at high current of 5 C. Compared with LFP/C (248 Ω), LFP/C/G/CNTs (50 Ω) showed obviously decreased charge transfer impedance. Cycle performance test indicated that the specific capacity retention for LFP/C/G/CNTs was 99% after 200 cycles, displaying good cycle stability. The superior electrochemical performance of LFP/C/G/CNTs is attributed to the significantly synergistic effect of CNTs and G on decreasing charge transfer impedance by constructing highly three-dimensional conductive network. Besides, the effect of G to CNTs mass ratio and the calcination temperature on the electrochemical performance of LIBs were also discussed.
abstract_unstemmed	High performance lithium iron phosphate (LFP) cathode materials were synthesized using amorphous carbon, carbon nanotubes (CNTs), and graphene (G) as conductive materials via sand milling and spray drying processes and followed by calcination. The structural characterizations indicated that CNTs and G can well connected with LFP nanoparticles (NPs), which was coated with a thin layer of amorphous carbon, benefiting the construction of three-dimensional efficient conductive network. The electrochemical measurements confirmed that the introduction of CNTs and G can obviously decrease the charge transfer impedance of lithium ion battery and increase the discharge special capacity. The initial discharge special capacity increases in the order of LFP/C (150.3 mAh/g) < LFP/C/CNTs (155.7 mAh/g) < LFP/C/G (159.7 mAh/g) < LFP/C/G/CNTs (164.5 mAh/g) at 0.1 C. LFP/C/G/CNTs also exhibited considerable discharge special capacity (99.5 mAh/g) at high current of 5 C. Compared with LFP/C (248 Ω), LFP/C/G/CNTs (50 Ω) showed obviously decreased charge transfer impedance. Cycle performance test indicated that the specific capacity retention for LFP/C/G/CNTs was 99% after 200 cycles, displaying good cycle stability. The superior electrochemical performance of LFP/C/G/CNTs is attributed to the significantly synergistic effect of CNTs and G on decreasing charge transfer impedance by constructing highly three-dimensional conductive network. Besides, the effect of G to CNTs mass ratio and the calcination temperature on the electrochemical performance of LIBs were also discussed.
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title_short	Construction of highly conductive network for improving electrochemical performance of lithium iron phosphate
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author2	Huang, Dequan Ma, Zhaoling Wang, Hongqiang Huang, Youguo Wu, Xianwen Li, Qingyu
author2Str	Huang, Dequan Ma, Zhaoling Wang, Hongqiang Huang, Youguo Wu, Xianwen Li, Qingyu
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doi_str	10.1016/j.electacta.2019.02.114
up_date	2024-07-06T23:16:43.991Z
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Construction of highly conductive network for improving electrochemical performance of lithium iron phosphate

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