Conformal dispersed cobalt nanoparticles in hollow carbon nanotube arrays for flexible Zn-air and Al-air batteries
The development of both flexible solid-state Zn-air and Al-air batteries are challenged by the efficient and stable air cathodes with high catalytic activities in both the oxygen reduction reaction (ORR) and the oxygen evolution reaction (OER). In this work, we report the rational design of hollow N...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Zhu, Chenyu [verfasserIn] Ma, Yuanyuan [verfasserIn] Zang, Wenjie [verfasserIn] Guan, Cao [verfasserIn] Liu, Ximeng [verfasserIn] Pennycook, Stephen J. [verfasserIn] Wang, John [verfasserIn] Huang, Wei [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2019 |
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| Schlagwörter: |
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| Übergeordnetes Werk: |
Enthalten in: The chemical engineering journal - Amsterdam : Elsevier, 1997, 369, Seite 988-995 |
|---|---|
| Übergeordnetes Werk: |
volume:369 ; pages:988-995 |
| DOI / URN: |
10.1016/j.cej.2019.03.147 |
|---|
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ELV002016966 |
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| 245 | 1 | 0 | |a Conformal dispersed cobalt nanoparticles in hollow carbon nanotube arrays for flexible Zn-air and Al-air batteries |
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| 520 | |a The development of both flexible solid-state Zn-air and Al-air batteries are challenged by the efficient and stable air cathodes with high catalytic activities in both the oxygen reduction reaction (ORR) and the oxygen evolution reaction (OER). In this work, we report the rational design of hollow N-doped carbon nanotube arrays embedded with confined Co nanoparticles (HCA-Co) through a facile solution-reaction and annealing process. Due to the unique integration of hollow carbon nanoarray with tiny cobalt nanoparticles, the obtained flexible HCA-Co electrode shows promising catalytic properties toward both ORR and OER that achieves a current density of 10 mA cm−2 at small overpotential of 290 mV in OER, and demonstrates an onset potential of 0.92 V in ORR. The HCA-Co can be applied as a binder-free air-cathode for flexible all-solid-state zinc-air batteries, which presents a relatively high open circuit potential (1.40 V) with better cycling stability than Pt/C based battery. The HCA-Co is also utilised as cathode for solid-state Al battery, which shows a high open circuit potential (1.966 V) with better mechanical flexibility than that of Pt/C-based battery. Such flexible electrode with excellent bifunctional catalytic properties hold great promise for the application in flexible electronics. | ||
| 650 | 4 | |a Hollow nanoarrays | |
| 650 | 4 | |a Metal-organic framework | |
| 650 | 4 | |a Bifunctional electrocatalyst | |
| 650 | 4 | |a Flexible Zn-air battery | |
| 650 | 4 | |a Flexible Al-air battery | |
| 700 | 1 | |a Ma, Yuanyuan |e verfasserin |4 aut | |
| 700 | 1 | |a Zang, Wenjie |e verfasserin |4 aut | |
| 700 | 1 | |a Guan, Cao |e verfasserin |4 aut | |
| 700 | 1 | |a Liu, Ximeng |e verfasserin |4 aut | |
| 700 | 1 | |a Pennycook, Stephen J. |e verfasserin |4 aut | |
| 700 | 1 | |a Wang, John |e verfasserin |4 aut | |
| 700 | 1 | |a Huang, Wei |e verfasserin |4 aut | |
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10.1016/j.cej.2019.03.147 doi (DE-627)ELV002016966 (ELSEVIER)S1385-8947(19)30611-4 DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Zhu, Chenyu verfasserin aut Conformal dispersed cobalt nanoparticles in hollow carbon nanotube arrays for flexible Zn-air and Al-air batteries 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The development of both flexible solid-state Zn-air and Al-air batteries are challenged by the efficient and stable air cathodes with high catalytic activities in both the oxygen reduction reaction (ORR) and the oxygen evolution reaction (OER). In this work, we report the rational design of hollow N-doped carbon nanotube arrays embedded with confined Co nanoparticles (HCA-Co) through a facile solution-reaction and annealing process. Due to the unique integration of hollow carbon nanoarray with tiny cobalt nanoparticles, the obtained flexible HCA-Co electrode shows promising catalytic properties toward both ORR and OER that achieves a current density of 10 mA cm−2 at small overpotential of 290 mV in OER, and demonstrates an onset potential of 0.92 V in ORR. The HCA-Co can be applied as a binder-free air-cathode for flexible all-solid-state zinc-air batteries, which presents a relatively high open circuit potential (1.40 V) with better cycling stability than Pt/C based battery. The HCA-Co is also utilised as cathode for solid-state Al battery, which shows a high open circuit potential (1.966 V) with better mechanical flexibility than that of Pt/C-based battery. Such flexible electrode with excellent bifunctional catalytic properties hold great promise for the application in flexible electronics. Hollow nanoarrays Metal-organic framework Bifunctional electrocatalyst Flexible Zn-air battery Flexible Al-air battery Ma, Yuanyuan verfasserin aut Zang, Wenjie verfasserin aut Guan, Cao verfasserin aut Liu, Ximeng verfasserin aut Pennycook, Stephen J. verfasserin aut Wang, John verfasserin aut Huang, Wei verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 369, Seite 988-995 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:369 pages:988-995 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 369 988-995 045F 660.05 |
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10.1016/j.cej.2019.03.147 doi (DE-627)ELV002016966 (ELSEVIER)S1385-8947(19)30611-4 DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Zhu, Chenyu verfasserin aut Conformal dispersed cobalt nanoparticles in hollow carbon nanotube arrays for flexible Zn-air and Al-air batteries 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The development of both flexible solid-state Zn-air and Al-air batteries are challenged by the efficient and stable air cathodes with high catalytic activities in both the oxygen reduction reaction (ORR) and the oxygen evolution reaction (OER). In this work, we report the rational design of hollow N-doped carbon nanotube arrays embedded with confined Co nanoparticles (HCA-Co) through a facile solution-reaction and annealing process. Due to the unique integration of hollow carbon nanoarray with tiny cobalt nanoparticles, the obtained flexible HCA-Co electrode shows promising catalytic properties toward both ORR and OER that achieves a current density of 10 mA cm−2 at small overpotential of 290 mV in OER, and demonstrates an onset potential of 0.92 V in ORR. The HCA-Co can be applied as a binder-free air-cathode for flexible all-solid-state zinc-air batteries, which presents a relatively high open circuit potential (1.40 V) with better cycling stability than Pt/C based battery. The HCA-Co is also utilised as cathode for solid-state Al battery, which shows a high open circuit potential (1.966 V) with better mechanical flexibility than that of Pt/C-based battery. Such flexible electrode with excellent bifunctional catalytic properties hold great promise for the application in flexible electronics. Hollow nanoarrays Metal-organic framework Bifunctional electrocatalyst Flexible Zn-air battery Flexible Al-air battery Ma, Yuanyuan verfasserin aut Zang, Wenjie verfasserin aut Guan, Cao verfasserin aut Liu, Ximeng verfasserin aut Pennycook, Stephen J. verfasserin aut Wang, John verfasserin aut Huang, Wei verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 369, Seite 988-995 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:369 pages:988-995 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 369 988-995 045F 660.05 |
| allfields_unstemmed |
10.1016/j.cej.2019.03.147 doi (DE-627)ELV002016966 (ELSEVIER)S1385-8947(19)30611-4 DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Zhu, Chenyu verfasserin aut Conformal dispersed cobalt nanoparticles in hollow carbon nanotube arrays for flexible Zn-air and Al-air batteries 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The development of both flexible solid-state Zn-air and Al-air batteries are challenged by the efficient and stable air cathodes with high catalytic activities in both the oxygen reduction reaction (ORR) and the oxygen evolution reaction (OER). In this work, we report the rational design of hollow N-doped carbon nanotube arrays embedded with confined Co nanoparticles (HCA-Co) through a facile solution-reaction and annealing process. Due to the unique integration of hollow carbon nanoarray with tiny cobalt nanoparticles, the obtained flexible HCA-Co electrode shows promising catalytic properties toward both ORR and OER that achieves a current density of 10 mA cm−2 at small overpotential of 290 mV in OER, and demonstrates an onset potential of 0.92 V in ORR. The HCA-Co can be applied as a binder-free air-cathode for flexible all-solid-state zinc-air batteries, which presents a relatively high open circuit potential (1.40 V) with better cycling stability than Pt/C based battery. The HCA-Co is also utilised as cathode for solid-state Al battery, which shows a high open circuit potential (1.966 V) with better mechanical flexibility than that of Pt/C-based battery. Such flexible electrode with excellent bifunctional catalytic properties hold great promise for the application in flexible electronics. Hollow nanoarrays Metal-organic framework Bifunctional electrocatalyst Flexible Zn-air battery Flexible Al-air battery Ma, Yuanyuan verfasserin aut Zang, Wenjie verfasserin aut Guan, Cao verfasserin aut Liu, Ximeng verfasserin aut Pennycook, Stephen J. verfasserin aut Wang, John verfasserin aut Huang, Wei verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 369, Seite 988-995 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:369 pages:988-995 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 369 988-995 045F 660.05 |
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10.1016/j.cej.2019.03.147 doi (DE-627)ELV002016966 (ELSEVIER)S1385-8947(19)30611-4 DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Zhu, Chenyu verfasserin aut Conformal dispersed cobalt nanoparticles in hollow carbon nanotube arrays for flexible Zn-air and Al-air batteries 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The development of both flexible solid-state Zn-air and Al-air batteries are challenged by the efficient and stable air cathodes with high catalytic activities in both the oxygen reduction reaction (ORR) and the oxygen evolution reaction (OER). In this work, we report the rational design of hollow N-doped carbon nanotube arrays embedded with confined Co nanoparticles (HCA-Co) through a facile solution-reaction and annealing process. Due to the unique integration of hollow carbon nanoarray with tiny cobalt nanoparticles, the obtained flexible HCA-Co electrode shows promising catalytic properties toward both ORR and OER that achieves a current density of 10 mA cm−2 at small overpotential of 290 mV in OER, and demonstrates an onset potential of 0.92 V in ORR. The HCA-Co can be applied as a binder-free air-cathode for flexible all-solid-state zinc-air batteries, which presents a relatively high open circuit potential (1.40 V) with better cycling stability than Pt/C based battery. The HCA-Co is also utilised as cathode for solid-state Al battery, which shows a high open circuit potential (1.966 V) with better mechanical flexibility than that of Pt/C-based battery. Such flexible electrode with excellent bifunctional catalytic properties hold great promise for the application in flexible electronics. Hollow nanoarrays Metal-organic framework Bifunctional electrocatalyst Flexible Zn-air battery Flexible Al-air battery Ma, Yuanyuan verfasserin aut Zang, Wenjie verfasserin aut Guan, Cao verfasserin aut Liu, Ximeng verfasserin aut Pennycook, Stephen J. verfasserin aut Wang, John verfasserin aut Huang, Wei verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 369, Seite 988-995 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:369 pages:988-995 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 369 988-995 045F 660.05 |
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10.1016/j.cej.2019.03.147 doi (DE-627)ELV002016966 (ELSEVIER)S1385-8947(19)30611-4 DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Zhu, Chenyu verfasserin aut Conformal dispersed cobalt nanoparticles in hollow carbon nanotube arrays for flexible Zn-air and Al-air batteries 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The development of both flexible solid-state Zn-air and Al-air batteries are challenged by the efficient and stable air cathodes with high catalytic activities in both the oxygen reduction reaction (ORR) and the oxygen evolution reaction (OER). In this work, we report the rational design of hollow N-doped carbon nanotube arrays embedded with confined Co nanoparticles (HCA-Co) through a facile solution-reaction and annealing process. Due to the unique integration of hollow carbon nanoarray with tiny cobalt nanoparticles, the obtained flexible HCA-Co electrode shows promising catalytic properties toward both ORR and OER that achieves a current density of 10 mA cm−2 at small overpotential of 290 mV in OER, and demonstrates an onset potential of 0.92 V in ORR. The HCA-Co can be applied as a binder-free air-cathode for flexible all-solid-state zinc-air batteries, which presents a relatively high open circuit potential (1.40 V) with better cycling stability than Pt/C based battery. The HCA-Co is also utilised as cathode for solid-state Al battery, which shows a high open circuit potential (1.966 V) with better mechanical flexibility than that of Pt/C-based battery. Such flexible electrode with excellent bifunctional catalytic properties hold great promise for the application in flexible electronics. Hollow nanoarrays Metal-organic framework Bifunctional electrocatalyst Flexible Zn-air battery Flexible Al-air battery Ma, Yuanyuan verfasserin aut Zang, Wenjie verfasserin aut Guan, Cao verfasserin aut Liu, Ximeng verfasserin aut Pennycook, Stephen J. verfasserin aut Wang, John verfasserin aut Huang, Wei verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 369, Seite 988-995 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:369 pages:988-995 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 369 988-995 045F 660.05 |
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660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Conformal dispersed cobalt nanoparticles in hollow carbon nanotube arrays for flexible Zn-air and Al-air batteries Hollow nanoarrays Metal-organic framework Bifunctional electrocatalyst Flexible Zn-air battery Flexible Al-air battery |
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Conformal dispersed cobalt nanoparticles in hollow carbon nanotube arrays for flexible Zn-air and Al-air batteries |
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Zhu, Chenyu Ma, Yuanyuan Zang, Wenjie Guan, Cao Liu, Ximeng Pennycook, Stephen J. Wang, John Huang, Wei |
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conformal dispersed cobalt nanoparticles in hollow carbon nanotube arrays for flexible zn-air and al-air batteries |
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Conformal dispersed cobalt nanoparticles in hollow carbon nanotube arrays for flexible Zn-air and Al-air batteries |
| abstract |
The development of both flexible solid-state Zn-air and Al-air batteries are challenged by the efficient and stable air cathodes with high catalytic activities in both the oxygen reduction reaction (ORR) and the oxygen evolution reaction (OER). In this work, we report the rational design of hollow N-doped carbon nanotube arrays embedded with confined Co nanoparticles (HCA-Co) through a facile solution-reaction and annealing process. Due to the unique integration of hollow carbon nanoarray with tiny cobalt nanoparticles, the obtained flexible HCA-Co electrode shows promising catalytic properties toward both ORR and OER that achieves a current density of 10 mA cm−2 at small overpotential of 290 mV in OER, and demonstrates an onset potential of 0.92 V in ORR. The HCA-Co can be applied as a binder-free air-cathode for flexible all-solid-state zinc-air batteries, which presents a relatively high open circuit potential (1.40 V) with better cycling stability than Pt/C based battery. The HCA-Co is also utilised as cathode for solid-state Al battery, which shows a high open circuit potential (1.966 V) with better mechanical flexibility than that of Pt/C-based battery. Such flexible electrode with excellent bifunctional catalytic properties hold great promise for the application in flexible electronics. |
| abstractGer |
The development of both flexible solid-state Zn-air and Al-air batteries are challenged by the efficient and stable air cathodes with high catalytic activities in both the oxygen reduction reaction (ORR) and the oxygen evolution reaction (OER). In this work, we report the rational design of hollow N-doped carbon nanotube arrays embedded with confined Co nanoparticles (HCA-Co) through a facile solution-reaction and annealing process. Due to the unique integration of hollow carbon nanoarray with tiny cobalt nanoparticles, the obtained flexible HCA-Co electrode shows promising catalytic properties toward both ORR and OER that achieves a current density of 10 mA cm−2 at small overpotential of 290 mV in OER, and demonstrates an onset potential of 0.92 V in ORR. The HCA-Co can be applied as a binder-free air-cathode for flexible all-solid-state zinc-air batteries, which presents a relatively high open circuit potential (1.40 V) with better cycling stability than Pt/C based battery. The HCA-Co is also utilised as cathode for solid-state Al battery, which shows a high open circuit potential (1.966 V) with better mechanical flexibility than that of Pt/C-based battery. Such flexible electrode with excellent bifunctional catalytic properties hold great promise for the application in flexible electronics. |
| abstract_unstemmed |
The development of both flexible solid-state Zn-air and Al-air batteries are challenged by the efficient and stable air cathodes with high catalytic activities in both the oxygen reduction reaction (ORR) and the oxygen evolution reaction (OER). In this work, we report the rational design of hollow N-doped carbon nanotube arrays embedded with confined Co nanoparticles (HCA-Co) through a facile solution-reaction and annealing process. Due to the unique integration of hollow carbon nanoarray with tiny cobalt nanoparticles, the obtained flexible HCA-Co electrode shows promising catalytic properties toward both ORR and OER that achieves a current density of 10 mA cm−2 at small overpotential of 290 mV in OER, and demonstrates an onset potential of 0.92 V in ORR. The HCA-Co can be applied as a binder-free air-cathode for flexible all-solid-state zinc-air batteries, which presents a relatively high open circuit potential (1.40 V) with better cycling stability than Pt/C based battery. The HCA-Co is also utilised as cathode for solid-state Al battery, which shows a high open circuit potential (1.966 V) with better mechanical flexibility than that of Pt/C-based battery. Such flexible electrode with excellent bifunctional catalytic properties hold great promise for the application in flexible electronics. |
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Conformal dispersed cobalt nanoparticles in hollow carbon nanotube arrays for flexible Zn-air and Al-air batteries |
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Ma, Yuanyuan Zang, Wenjie Guan, Cao Liu, Ximeng Pennycook, Stephen J. Wang, John Huang, Wei |
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