Enhancing the performance of hole-conductor free carbon-based perovskite solar cells through rutile-phase passivation of anatase TiO
Surface passivation of the electron transport layer in perovskite solar cells has been proven to be one crucial strategy to improve the power conversion efficiency. In this study, we introduce rutile phase titania shell to passivate anatase TiO2 scaffold, forming anataserutile mixed-phase TiO2 scaff...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Xiao, Yuqing [verfasserIn] Wang, Changlei [verfasserIn] Kondamareddy, Kiran Kumar [verfasserIn] Liu, Pei [verfasserIn] Qi, Fei [verfasserIn] Zhang, Huijie [verfasserIn] Guo, Shishang [verfasserIn] Zhao, Xing-Zhong [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2019 |
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| Schlagwörter: |
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| Übergeordnetes Werk: |
Enthalten in: Journal of power sources - New York, NY [u.a.] : Elsevier, 1976, 422, Seite 138-144 |
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| Übergeordnetes Werk: |
volume:422 ; pages:138-144 |
| DOI / URN: |
10.1016/j.jpowsour.2019.03.039 |
|---|
| Katalog-ID: |
ELV002021889 |
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| 245 | 1 | 0 | |a Enhancing the performance of hole-conductor free carbon-based perovskite solar cells through rutile-phase passivation of anatase TiO |
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| 520 | |a Surface passivation of the electron transport layer in perovskite solar cells has been proven to be one crucial strategy to improve the power conversion efficiency. In this study, we introduce rutile phase titania shell to passivate anatase TiO2 scaffold, forming anataserutile mixed-phase TiO2 scaffold in hole-conductor-free carbon based perovskite solar cells. Anatase@rutile mixed phase TiO2 films exhibit higher conductivity, faster charge extraction, lower trap density and suppressed charge recombination at the interface of TiO2/perovskite films in the modified devices as well, achieving a champion power conversion efficiency of 15.21% for carbon based perovskite solar cells. More importantly, benefiting from the stable and better ultraviolet light filtration properties of rutile phase TiO2, our devices exhibit excellent stability maintaining 92% of their initial efficiency after 200 days storage in ambient air, highlighting their merits as a potential competitor for future industrial photovoltaics. | ||
| 650 | 4 | |a Perovskite solar cells | |
| 650 | 4 | |a anatase@rutile mixed phase TiO | |
| 650 | 4 | |a Hole transport material free | |
| 650 | 4 | |a Surface passivation | |
| 650 | 4 | |a Long-term stability | |
| 700 | 1 | |a Wang, Changlei |e verfasserin |4 aut | |
| 700 | 1 | |a Kondamareddy, Kiran Kumar |e verfasserin |4 aut | |
| 700 | 1 | |a Liu, Pei |e verfasserin |4 aut | |
| 700 | 1 | |a Qi, Fei |e verfasserin |4 aut | |
| 700 | 1 | |a Zhang, Huijie |e verfasserin |4 aut | |
| 700 | 1 | |a Guo, Shishang |e verfasserin |0 (orcid)0000-0001-7210-4704 |4 aut | |
| 700 | 1 | |a Zhao, Xing-Zhong |e verfasserin |0 (orcid)0000-0002-4886-2342 |4 aut | |
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10.1016/j.jpowsour.2019.03.039 doi (DE-627)ELV002021889 (ELSEVIER)S0378-7753(19)30278-2 DE-627 ger DE-627 rda eng 620 DE-600 52.57 bkl 53.36 bkl Xiao, Yuqing verfasserin aut Enhancing the performance of hole-conductor free carbon-based perovskite solar cells through rutile-phase passivation of anatase TiO 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Surface passivation of the electron transport layer in perovskite solar cells has been proven to be one crucial strategy to improve the power conversion efficiency. In this study, we introduce rutile phase titania shell to passivate anatase TiO2 scaffold, forming anataserutile mixed-phase TiO2 scaffold in hole-conductor-free carbon based perovskite solar cells. Anatase@rutile mixed phase TiO2 films exhibit higher conductivity, faster charge extraction, lower trap density and suppressed charge recombination at the interface of TiO2/perovskite films in the modified devices as well, achieving a champion power conversion efficiency of 15.21% for carbon based perovskite solar cells. More importantly, benefiting from the stable and better ultraviolet light filtration properties of rutile phase TiO2, our devices exhibit excellent stability maintaining 92% of their initial efficiency after 200 days storage in ambient air, highlighting their merits as a potential competitor for future industrial photovoltaics. Perovskite solar cells anatase@rutile mixed phase TiO Hole transport material free Surface passivation Long-term stability Wang, Changlei verfasserin aut Kondamareddy, Kiran Kumar verfasserin aut Liu, Pei verfasserin aut Qi, Fei verfasserin aut Zhang, Huijie verfasserin aut Guo, Shishang verfasserin (orcid)0000-0001-7210-4704 aut Zhao, Xing-Zhong verfasserin (orcid)0000-0002-4886-2342 aut Enthalten in Journal of power sources New York, NY [u.a.] : Elsevier, 1976 422, Seite 138-144 Online-Ressource (DE-627)302718923 (DE-600)1491915-1 (DE-576)259483958 1873-2755 nnns volume:422 pages:138-144 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 52.57 Energiespeicherung 53.36 Energiedirektumwandler elektrische Energiespeicher AR 422 138-144 |
| spelling |
10.1016/j.jpowsour.2019.03.039 doi (DE-627)ELV002021889 (ELSEVIER)S0378-7753(19)30278-2 DE-627 ger DE-627 rda eng 620 DE-600 52.57 bkl 53.36 bkl Xiao, Yuqing verfasserin aut Enhancing the performance of hole-conductor free carbon-based perovskite solar cells through rutile-phase passivation of anatase TiO 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Surface passivation of the electron transport layer in perovskite solar cells has been proven to be one crucial strategy to improve the power conversion efficiency. In this study, we introduce rutile phase titania shell to passivate anatase TiO2 scaffold, forming anataserutile mixed-phase TiO2 scaffold in hole-conductor-free carbon based perovskite solar cells. Anatase@rutile mixed phase TiO2 films exhibit higher conductivity, faster charge extraction, lower trap density and suppressed charge recombination at the interface of TiO2/perovskite films in the modified devices as well, achieving a champion power conversion efficiency of 15.21% for carbon based perovskite solar cells. More importantly, benefiting from the stable and better ultraviolet light filtration properties of rutile phase TiO2, our devices exhibit excellent stability maintaining 92% of their initial efficiency after 200 days storage in ambient air, highlighting their merits as a potential competitor for future industrial photovoltaics. Perovskite solar cells anatase@rutile mixed phase TiO Hole transport material free Surface passivation Long-term stability Wang, Changlei verfasserin aut Kondamareddy, Kiran Kumar verfasserin aut Liu, Pei verfasserin aut Qi, Fei verfasserin aut Zhang, Huijie verfasserin aut Guo, Shishang verfasserin (orcid)0000-0001-7210-4704 aut Zhao, Xing-Zhong verfasserin (orcid)0000-0002-4886-2342 aut Enthalten in Journal of power sources New York, NY [u.a.] : Elsevier, 1976 422, Seite 138-144 Online-Ressource (DE-627)302718923 (DE-600)1491915-1 (DE-576)259483958 1873-2755 nnns volume:422 pages:138-144 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 52.57 Energiespeicherung 53.36 Energiedirektumwandler elektrische Energiespeicher AR 422 138-144 |
| allfields_unstemmed |
10.1016/j.jpowsour.2019.03.039 doi (DE-627)ELV002021889 (ELSEVIER)S0378-7753(19)30278-2 DE-627 ger DE-627 rda eng 620 DE-600 52.57 bkl 53.36 bkl Xiao, Yuqing verfasserin aut Enhancing the performance of hole-conductor free carbon-based perovskite solar cells through rutile-phase passivation of anatase TiO 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Surface passivation of the electron transport layer in perovskite solar cells has been proven to be one crucial strategy to improve the power conversion efficiency. In this study, we introduce rutile phase titania shell to passivate anatase TiO2 scaffold, forming anataserutile mixed-phase TiO2 scaffold in hole-conductor-free carbon based perovskite solar cells. Anatase@rutile mixed phase TiO2 films exhibit higher conductivity, faster charge extraction, lower trap density and suppressed charge recombination at the interface of TiO2/perovskite films in the modified devices as well, achieving a champion power conversion efficiency of 15.21% for carbon based perovskite solar cells. More importantly, benefiting from the stable and better ultraviolet light filtration properties of rutile phase TiO2, our devices exhibit excellent stability maintaining 92% of their initial efficiency after 200 days storage in ambient air, highlighting their merits as a potential competitor for future industrial photovoltaics. Perovskite solar cells anatase@rutile mixed phase TiO Hole transport material free Surface passivation Long-term stability Wang, Changlei verfasserin aut Kondamareddy, Kiran Kumar verfasserin aut Liu, Pei verfasserin aut Qi, Fei verfasserin aut Zhang, Huijie verfasserin aut Guo, Shishang verfasserin (orcid)0000-0001-7210-4704 aut Zhao, Xing-Zhong verfasserin (orcid)0000-0002-4886-2342 aut Enthalten in Journal of power sources New York, NY [u.a.] : Elsevier, 1976 422, Seite 138-144 Online-Ressource (DE-627)302718923 (DE-600)1491915-1 (DE-576)259483958 1873-2755 nnns volume:422 pages:138-144 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 52.57 Energiespeicherung 53.36 Energiedirektumwandler elektrische Energiespeicher AR 422 138-144 |
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10.1016/j.jpowsour.2019.03.039 doi (DE-627)ELV002021889 (ELSEVIER)S0378-7753(19)30278-2 DE-627 ger DE-627 rda eng 620 DE-600 52.57 bkl 53.36 bkl Xiao, Yuqing verfasserin aut Enhancing the performance of hole-conductor free carbon-based perovskite solar cells through rutile-phase passivation of anatase TiO 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Surface passivation of the electron transport layer in perovskite solar cells has been proven to be one crucial strategy to improve the power conversion efficiency. In this study, we introduce rutile phase titania shell to passivate anatase TiO2 scaffold, forming anataserutile mixed-phase TiO2 scaffold in hole-conductor-free carbon based perovskite solar cells. Anatase@rutile mixed phase TiO2 films exhibit higher conductivity, faster charge extraction, lower trap density and suppressed charge recombination at the interface of TiO2/perovskite films in the modified devices as well, achieving a champion power conversion efficiency of 15.21% for carbon based perovskite solar cells. More importantly, benefiting from the stable and better ultraviolet light filtration properties of rutile phase TiO2, our devices exhibit excellent stability maintaining 92% of their initial efficiency after 200 days storage in ambient air, highlighting their merits as a potential competitor for future industrial photovoltaics. Perovskite solar cells anatase@rutile mixed phase TiO Hole transport material free Surface passivation Long-term stability Wang, Changlei verfasserin aut Kondamareddy, Kiran Kumar verfasserin aut Liu, Pei verfasserin aut Qi, Fei verfasserin aut Zhang, Huijie verfasserin aut Guo, Shishang verfasserin (orcid)0000-0001-7210-4704 aut Zhao, Xing-Zhong verfasserin (orcid)0000-0002-4886-2342 aut Enthalten in Journal of power sources New York, NY [u.a.] : Elsevier, 1976 422, Seite 138-144 Online-Ressource (DE-627)302718923 (DE-600)1491915-1 (DE-576)259483958 1873-2755 nnns volume:422 pages:138-144 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 52.57 Energiespeicherung 53.36 Energiedirektumwandler elektrische Energiespeicher AR 422 138-144 |
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10.1016/j.jpowsour.2019.03.039 doi (DE-627)ELV002021889 (ELSEVIER)S0378-7753(19)30278-2 DE-627 ger DE-627 rda eng 620 DE-600 52.57 bkl 53.36 bkl Xiao, Yuqing verfasserin aut Enhancing the performance of hole-conductor free carbon-based perovskite solar cells through rutile-phase passivation of anatase TiO 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Surface passivation of the electron transport layer in perovskite solar cells has been proven to be one crucial strategy to improve the power conversion efficiency. In this study, we introduce rutile phase titania shell to passivate anatase TiO2 scaffold, forming anataserutile mixed-phase TiO2 scaffold in hole-conductor-free carbon based perovskite solar cells. Anatase@rutile mixed phase TiO2 films exhibit higher conductivity, faster charge extraction, lower trap density and suppressed charge recombination at the interface of TiO2/perovskite films in the modified devices as well, achieving a champion power conversion efficiency of 15.21% for carbon based perovskite solar cells. More importantly, benefiting from the stable and better ultraviolet light filtration properties of rutile phase TiO2, our devices exhibit excellent stability maintaining 92% of their initial efficiency after 200 days storage in ambient air, highlighting their merits as a potential competitor for future industrial photovoltaics. Perovskite solar cells anatase@rutile mixed phase TiO Hole transport material free Surface passivation Long-term stability Wang, Changlei verfasserin aut Kondamareddy, Kiran Kumar verfasserin aut Liu, Pei verfasserin aut Qi, Fei verfasserin aut Zhang, Huijie verfasserin aut Guo, Shishang verfasserin (orcid)0000-0001-7210-4704 aut Zhao, Xing-Zhong verfasserin (orcid)0000-0002-4886-2342 aut Enthalten in Journal of power sources New York, NY [u.a.] : Elsevier, 1976 422, Seite 138-144 Online-Ressource (DE-627)302718923 (DE-600)1491915-1 (DE-576)259483958 1873-2755 nnns volume:422 pages:138-144 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 52.57 Energiespeicherung 53.36 Energiedirektumwandler elektrische Energiespeicher AR 422 138-144 |
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Xiao, Yuqing @@aut@@ Wang, Changlei @@aut@@ Kondamareddy, Kiran Kumar @@aut@@ Liu, Pei @@aut@@ Qi, Fei @@aut@@ Zhang, Huijie @@aut@@ Guo, Shishang @@aut@@ Zhao, Xing-Zhong @@aut@@ |
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620 DE-600 52.57 bkl 53.36 bkl Enhancing the performance of hole-conductor free carbon-based perovskite solar cells through rutile-phase passivation of anatase TiO Perovskite solar cells anatase@rutile mixed phase TiO Hole transport material free Surface passivation Long-term stability |
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enhancing the performance of hole-conductor free carbon-based perovskite solar cells through rutile-phase passivation of anatase tio |
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Enhancing the performance of hole-conductor free carbon-based perovskite solar cells through rutile-phase passivation of anatase TiO |
| abstract |
Surface passivation of the electron transport layer in perovskite solar cells has been proven to be one crucial strategy to improve the power conversion efficiency. In this study, we introduce rutile phase titania shell to passivate anatase TiO2 scaffold, forming anataserutile mixed-phase TiO2 scaffold in hole-conductor-free carbon based perovskite solar cells. Anatase@rutile mixed phase TiO2 films exhibit higher conductivity, faster charge extraction, lower trap density and suppressed charge recombination at the interface of TiO2/perovskite films in the modified devices as well, achieving a champion power conversion efficiency of 15.21% for carbon based perovskite solar cells. More importantly, benefiting from the stable and better ultraviolet light filtration properties of rutile phase TiO2, our devices exhibit excellent stability maintaining 92% of their initial efficiency after 200 days storage in ambient air, highlighting their merits as a potential competitor for future industrial photovoltaics. |
| abstractGer |
Surface passivation of the electron transport layer in perovskite solar cells has been proven to be one crucial strategy to improve the power conversion efficiency. In this study, we introduce rutile phase titania shell to passivate anatase TiO2 scaffold, forming anataserutile mixed-phase TiO2 scaffold in hole-conductor-free carbon based perovskite solar cells. Anatase@rutile mixed phase TiO2 films exhibit higher conductivity, faster charge extraction, lower trap density and suppressed charge recombination at the interface of TiO2/perovskite films in the modified devices as well, achieving a champion power conversion efficiency of 15.21% for carbon based perovskite solar cells. More importantly, benefiting from the stable and better ultraviolet light filtration properties of rutile phase TiO2, our devices exhibit excellent stability maintaining 92% of their initial efficiency after 200 days storage in ambient air, highlighting their merits as a potential competitor for future industrial photovoltaics. |
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Surface passivation of the electron transport layer in perovskite solar cells has been proven to be one crucial strategy to improve the power conversion efficiency. In this study, we introduce rutile phase titania shell to passivate anatase TiO2 scaffold, forming anataserutile mixed-phase TiO2 scaffold in hole-conductor-free carbon based perovskite solar cells. Anatase@rutile mixed phase TiO2 films exhibit higher conductivity, faster charge extraction, lower trap density and suppressed charge recombination at the interface of TiO2/perovskite films in the modified devices as well, achieving a champion power conversion efficiency of 15.21% for carbon based perovskite solar cells. More importantly, benefiting from the stable and better ultraviolet light filtration properties of rutile phase TiO2, our devices exhibit excellent stability maintaining 92% of their initial efficiency after 200 days storage in ambient air, highlighting their merits as a potential competitor for future industrial photovoltaics. |
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Enhancing the performance of hole-conductor free carbon-based perovskite solar cells through rutile-phase passivation of anatase TiO |
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| score |
7.400161 |