Characterization of petroleum-based products in water samples by HS-MS

In forensic and environmental sciences, the identification of petroleum-based products is an important task to establish not only the origin of a given residue but also the hazard level or the appropriate cleanup procedure. A new strategy for the fingerprinting of petroleum-based products (PP) in wa...
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Gespeichert in:

Autor*in:	Ferreiro-González, Marta [verfasserIn] Aliaño-González, María José [verfasserIn] Barbero, Gerardo F. [verfasserIn] Palma, Miguel [verfasserIn] Barroso, Carmelo G. [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2018

Schlagwörter:	Petroleum-based products Fuel spills HS-MS Fingerprinting Characterization Chemometrics Water samples

Übergeordnetes Werk:	Enthalten in: Fuel - New York, NY [u.a.] : Elsevier, 1970, 222, Seite 506-512
Übergeordnetes Werk:	volume:222 ; pages:506-512

DOI / URN:	10.1016/j.fuel.2018.02.127

Katalog-ID:	ELV002040476

Internformat


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520			\|a In forensic and environmental sciences, the identification of petroleum-based products is an important task to establish not only the origin of a given residue but also the hazard level or the appropriate cleanup procedure. A new strategy for the fingerprinting of petroleum-based products (PP) in water samples (seawater and freshwater) for rapid and easy fuel spill identification has been developed. For this purpose, an HS-MS has been used in combination with chemometric tools such as linear discriminant analysis (LDA). A set of 70 samples from seven types of PPs (aromatic products, alcohols, normal alkanes, gasoline, diesel, lubricants and naphthenic-paraffinic products), all of which were added to water (seawater and freshwater), were analyzed. 100% of the samples were discriminated according to the type of petroleum-based products used regardless the nature of the water. Furthermore, a fingerprint was obtained for each petroleum product by plotting the m/z values selected by the LDA and this allowed the rapid identification of the petroleum products. The repeatability and intermediate precision were evaluated for both types of water samples and good values were obtained (RSD < 10%). The applicability of the method for the detection of lower proportions of PP was assessed and the same fingerprints were obtained for each PP, even when the volume was decreased down to 0.05%. The results demonstrate the potential of HS-MS in this field.
650		4	\|a Petroleum-based products
650		4	\|a Fuel spills
650		4	\|a HS-MS
650		4	\|a Fingerprinting
650		4	\|a Characterization
650		4	\|a Chemometrics
650		4	\|a Water samples
700	1		\|a Aliaño-González, María José \|e verfasserin \|4 aut
700	1		\|a Barbero, Gerardo F. \|e verfasserin \|4 aut
700	1		\|a Palma, Miguel \|e verfasserin \|0 (orcid)0000-0003-0870-403X \|4 aut
700	1		\|a Barroso, Carmelo G. \|e verfasserin \|4 aut
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912			\|a GBV_ILN_2056
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912			\|a GBV_ILN_4251
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912			\|a GBV_ILN_4323
912			\|a GBV_ILN_4324
912			\|a GBV_ILN_4326
912			\|a GBV_ILN_4333
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912			\|a GBV_ILN_4393
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publishDate	2018
allfields	10.1016/j.fuel.2018.02.127 doi (DE-627)ELV002040476 (ELSEVIER)S0016-2361(18)30310-7 DE-627 ger DE-627 rda eng 660 DE-600 58.21 bkl Ferreiro-González, Marta verfasserin aut Characterization of petroleum-based products in water samples by HS-MS 2018 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier In forensic and environmental sciences, the identification of petroleum-based products is an important task to establish not only the origin of a given residue but also the hazard level or the appropriate cleanup procedure. A new strategy for the fingerprinting of petroleum-based products (PP) in water samples (seawater and freshwater) for rapid and easy fuel spill identification has been developed. For this purpose, an HS-MS has been used in combination with chemometric tools such as linear discriminant analysis (LDA). A set of 70 samples from seven types of PPs (aromatic products, alcohols, normal alkanes, gasoline, diesel, lubricants and naphthenic-paraffinic products), all of which were added to water (seawater and freshwater), were analyzed. 100% of the samples were discriminated according to the type of petroleum-based products used regardless the nature of the water. Furthermore, a fingerprint was obtained for each petroleum product by plotting the m/z values selected by the LDA and this allowed the rapid identification of the petroleum products. The repeatability and intermediate precision were evaluated for both types of water samples and good values were obtained (RSD < 10%). The applicability of the method for the detection of lower proportions of PP was assessed and the same fingerprints were obtained for each PP, even when the volume was decreased down to 0.05%. The results demonstrate the potential of HS-MS in this field. Petroleum-based products Fuel spills HS-MS Fingerprinting Characterization Chemometrics Water samples Aliaño-González, María José verfasserin aut Barbero, Gerardo F. verfasserin aut Palma, Miguel verfasserin (orcid)0000-0003-0870-403X aut Barroso, Carmelo G. verfasserin aut Enthalten in Fuel New York, NY [u.a.] : Elsevier, 1970 222, Seite 506-512 Online-Ressource (DE-627)300898584 (DE-600)1483656-7 (DE-576)09555176X 0016-2361 nnns volume:222 pages:506-512 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.21 Brennstoffe Kraftstoffe Explosivstoffe AR 222 506-512
spelling	10.1016/j.fuel.2018.02.127 doi (DE-627)ELV002040476 (ELSEVIER)S0016-2361(18)30310-7 DE-627 ger DE-627 rda eng 660 DE-600 58.21 bkl Ferreiro-González, Marta verfasserin aut Characterization of petroleum-based products in water samples by HS-MS 2018 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier In forensic and environmental sciences, the identification of petroleum-based products is an important task to establish not only the origin of a given residue but also the hazard level or the appropriate cleanup procedure. A new strategy for the fingerprinting of petroleum-based products (PP) in water samples (seawater and freshwater) for rapid and easy fuel spill identification has been developed. For this purpose, an HS-MS has been used in combination with chemometric tools such as linear discriminant analysis (LDA). A set of 70 samples from seven types of PPs (aromatic products, alcohols, normal alkanes, gasoline, diesel, lubricants and naphthenic-paraffinic products), all of which were added to water (seawater and freshwater), were analyzed. 100% of the samples were discriminated according to the type of petroleum-based products used regardless the nature of the water. Furthermore, a fingerprint was obtained for each petroleum product by plotting the m/z values selected by the LDA and this allowed the rapid identification of the petroleum products. The repeatability and intermediate precision were evaluated for both types of water samples and good values were obtained (RSD < 10%). The applicability of the method for the detection of lower proportions of PP was assessed and the same fingerprints were obtained for each PP, even when the volume was decreased down to 0.05%. The results demonstrate the potential of HS-MS in this field. Petroleum-based products Fuel spills HS-MS Fingerprinting Characterization Chemometrics Water samples Aliaño-González, María José verfasserin aut Barbero, Gerardo F. verfasserin aut Palma, Miguel verfasserin (orcid)0000-0003-0870-403X aut Barroso, Carmelo G. verfasserin aut Enthalten in Fuel New York, NY [u.a.] : Elsevier, 1970 222, Seite 506-512 Online-Ressource (DE-627)300898584 (DE-600)1483656-7 (DE-576)09555176X 0016-2361 nnns volume:222 pages:506-512 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.21 Brennstoffe Kraftstoffe Explosivstoffe AR 222 506-512
allfields_unstemmed	10.1016/j.fuel.2018.02.127 doi (DE-627)ELV002040476 (ELSEVIER)S0016-2361(18)30310-7 DE-627 ger DE-627 rda eng 660 DE-600 58.21 bkl Ferreiro-González, Marta verfasserin aut Characterization of petroleum-based products in water samples by HS-MS 2018 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier In forensic and environmental sciences, the identification of petroleum-based products is an important task to establish not only the origin of a given residue but also the hazard level or the appropriate cleanup procedure. A new strategy for the fingerprinting of petroleum-based products (PP) in water samples (seawater and freshwater) for rapid and easy fuel spill identification has been developed. For this purpose, an HS-MS has been used in combination with chemometric tools such as linear discriminant analysis (LDA). A set of 70 samples from seven types of PPs (aromatic products, alcohols, normal alkanes, gasoline, diesel, lubricants and naphthenic-paraffinic products), all of which were added to water (seawater and freshwater), were analyzed. 100% of the samples were discriminated according to the type of petroleum-based products used regardless the nature of the water. Furthermore, a fingerprint was obtained for each petroleum product by plotting the m/z values selected by the LDA and this allowed the rapid identification of the petroleum products. The repeatability and intermediate precision were evaluated for both types of water samples and good values were obtained (RSD < 10%). The applicability of the method for the detection of lower proportions of PP was assessed and the same fingerprints were obtained for each PP, even when the volume was decreased down to 0.05%. The results demonstrate the potential of HS-MS in this field. Petroleum-based products Fuel spills HS-MS Fingerprinting Characterization Chemometrics Water samples Aliaño-González, María José verfasserin aut Barbero, Gerardo F. verfasserin aut Palma, Miguel verfasserin (orcid)0000-0003-0870-403X aut Barroso, Carmelo G. verfasserin aut Enthalten in Fuel New York, NY [u.a.] : Elsevier, 1970 222, Seite 506-512 Online-Ressource (DE-627)300898584 (DE-600)1483656-7 (DE-576)09555176X 0016-2361 nnns volume:222 pages:506-512 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.21 Brennstoffe Kraftstoffe Explosivstoffe AR 222 506-512
allfieldsGer	10.1016/j.fuel.2018.02.127 doi (DE-627)ELV002040476 (ELSEVIER)S0016-2361(18)30310-7 DE-627 ger DE-627 rda eng 660 DE-600 58.21 bkl Ferreiro-González, Marta verfasserin aut Characterization of petroleum-based products in water samples by HS-MS 2018 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier In forensic and environmental sciences, the identification of petroleum-based products is an important task to establish not only the origin of a given residue but also the hazard level or the appropriate cleanup procedure. A new strategy for the fingerprinting of petroleum-based products (PP) in water samples (seawater and freshwater) for rapid and easy fuel spill identification has been developed. For this purpose, an HS-MS has been used in combination with chemometric tools such as linear discriminant analysis (LDA). A set of 70 samples from seven types of PPs (aromatic products, alcohols, normal alkanes, gasoline, diesel, lubricants and naphthenic-paraffinic products), all of which were added to water (seawater and freshwater), were analyzed. 100% of the samples were discriminated according to the type of petroleum-based products used regardless the nature of the water. Furthermore, a fingerprint was obtained for each petroleum product by plotting the m/z values selected by the LDA and this allowed the rapid identification of the petroleum products. The repeatability and intermediate precision were evaluated for both types of water samples and good values were obtained (RSD < 10%). The applicability of the method for the detection of lower proportions of PP was assessed and the same fingerprints were obtained for each PP, even when the volume was decreased down to 0.05%. The results demonstrate the potential of HS-MS in this field. Petroleum-based products Fuel spills HS-MS Fingerprinting Characterization Chemometrics Water samples Aliaño-González, María José verfasserin aut Barbero, Gerardo F. verfasserin aut Palma, Miguel verfasserin (orcid)0000-0003-0870-403X aut Barroso, Carmelo G. verfasserin aut Enthalten in Fuel New York, NY [u.a.] : Elsevier, 1970 222, Seite 506-512 Online-Ressource (DE-627)300898584 (DE-600)1483656-7 (DE-576)09555176X 0016-2361 nnns volume:222 pages:506-512 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.21 Brennstoffe Kraftstoffe Explosivstoffe AR 222 506-512
allfieldsSound	10.1016/j.fuel.2018.02.127 doi (DE-627)ELV002040476 (ELSEVIER)S0016-2361(18)30310-7 DE-627 ger DE-627 rda eng 660 DE-600 58.21 bkl Ferreiro-González, Marta verfasserin aut Characterization of petroleum-based products in water samples by HS-MS 2018 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier In forensic and environmental sciences, the identification of petroleum-based products is an important task to establish not only the origin of a given residue but also the hazard level or the appropriate cleanup procedure. A new strategy for the fingerprinting of petroleum-based products (PP) in water samples (seawater and freshwater) for rapid and easy fuel spill identification has been developed. For this purpose, an HS-MS has been used in combination with chemometric tools such as linear discriminant analysis (LDA). A set of 70 samples from seven types of PPs (aromatic products, alcohols, normal alkanes, gasoline, diesel, lubricants and naphthenic-paraffinic products), all of which were added to water (seawater and freshwater), were analyzed. 100% of the samples were discriminated according to the type of petroleum-based products used regardless the nature of the water. Furthermore, a fingerprint was obtained for each petroleum product by plotting the m/z values selected by the LDA and this allowed the rapid identification of the petroleum products. The repeatability and intermediate precision were evaluated for both types of water samples and good values were obtained (RSD < 10%). The applicability of the method for the detection of lower proportions of PP was assessed and the same fingerprints were obtained for each PP, even when the volume was decreased down to 0.05%. The results demonstrate the potential of HS-MS in this field. Petroleum-based products Fuel spills HS-MS Fingerprinting Characterization Chemometrics Water samples Aliaño-González, María José verfasserin aut Barbero, Gerardo F. verfasserin aut Palma, Miguel verfasserin (orcid)0000-0003-0870-403X aut Barroso, Carmelo G. verfasserin aut Enthalten in Fuel New York, NY [u.a.] : Elsevier, 1970 222, Seite 506-512 Online-Ressource (DE-627)300898584 (DE-600)1483656-7 (DE-576)09555176X 0016-2361 nnns volume:222 pages:506-512 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.21 Brennstoffe Kraftstoffe Explosivstoffe AR 222 506-512
language	English
source	Enthalten in Fuel 222, Seite 506-512 volume:222 pages:506-512
sourceStr	Enthalten in Fuel 222, Seite 506-512 volume:222 pages:506-512
format_phy_str_mv	Article
bklname	Brennstoffe Kraftstoffe Explosivstoffe
institution	findex.gbv.de
topic_facet	Petroleum-based products Fuel spills HS-MS Fingerprinting Characterization Chemometrics Water samples
dewey-raw	660
isfreeaccess_bool	false
container_title	Fuel
authorswithroles_txt_mv	Ferreiro-González, Marta @@aut@@ Aliaño-González, María José @@aut@@ Barbero, Gerardo F. @@aut@@ Palma, Miguel @@aut@@ Barroso, Carmelo G. @@aut@@
publishDateDaySort_date	2018-01-01T00:00:00Z
hierarchy_top_id	300898584
dewey-sort	3660
id	ELV002040476
language_de	englisch
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author	Ferreiro-González, Marta
spellingShingle	Ferreiro-González, Marta ddc 660 bkl 58.21 misc Petroleum-based products misc Fuel spills misc HS-MS misc Fingerprinting misc Characterization misc Chemometrics misc Water samples Characterization of petroleum-based products in water samples by HS-MS
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topic_title	660 DE-600 58.21 bkl Characterization of petroleum-based products in water samples by HS-MS Petroleum-based products Fuel spills HS-MS Fingerprinting Characterization Chemometrics Water samples
topic	ddc 660 bkl 58.21 misc Petroleum-based products misc Fuel spills misc HS-MS misc Fingerprinting misc Characterization misc Chemometrics misc Water samples
topic_unstemmed	ddc 660 bkl 58.21 misc Petroleum-based products misc Fuel spills misc HS-MS misc Fingerprinting misc Characterization misc Chemometrics misc Water samples
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title	Characterization of petroleum-based products in water samples by HS-MS
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title_full	Characterization of petroleum-based products in water samples by HS-MS
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author_browse	Ferreiro-González, Marta Aliaño-González, María José Barbero, Gerardo F. Palma, Miguel Barroso, Carmelo G.
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title_sort	characterization of petroleum-based products in water samples by hs-ms
title_auth	Characterization of petroleum-based products in water samples by HS-MS
abstract	In forensic and environmental sciences, the identification of petroleum-based products is an important task to establish not only the origin of a given residue but also the hazard level or the appropriate cleanup procedure. A new strategy for the fingerprinting of petroleum-based products (PP) in water samples (seawater and freshwater) for rapid and easy fuel spill identification has been developed. For this purpose, an HS-MS has been used in combination with chemometric tools such as linear discriminant analysis (LDA). A set of 70 samples from seven types of PPs (aromatic products, alcohols, normal alkanes, gasoline, diesel, lubricants and naphthenic-paraffinic products), all of which were added to water (seawater and freshwater), were analyzed. 100% of the samples were discriminated according to the type of petroleum-based products used regardless the nature of the water. Furthermore, a fingerprint was obtained for each petroleum product by plotting the m/z values selected by the LDA and this allowed the rapid identification of the petroleum products. The repeatability and intermediate precision were evaluated for both types of water samples and good values were obtained (RSD < 10%). The applicability of the method for the detection of lower proportions of PP was assessed and the same fingerprints were obtained for each PP, even when the volume was decreased down to 0.05%. The results demonstrate the potential of HS-MS in this field.
abstractGer	In forensic and environmental sciences, the identification of petroleum-based products is an important task to establish not only the origin of a given residue but also the hazard level or the appropriate cleanup procedure. A new strategy for the fingerprinting of petroleum-based products (PP) in water samples (seawater and freshwater) for rapid and easy fuel spill identification has been developed. For this purpose, an HS-MS has been used in combination with chemometric tools such as linear discriminant analysis (LDA). A set of 70 samples from seven types of PPs (aromatic products, alcohols, normal alkanes, gasoline, diesel, lubricants and naphthenic-paraffinic products), all of which were added to water (seawater and freshwater), were analyzed. 100% of the samples were discriminated according to the type of petroleum-based products used regardless the nature of the water. Furthermore, a fingerprint was obtained for each petroleum product by plotting the m/z values selected by the LDA and this allowed the rapid identification of the petroleum products. The repeatability and intermediate precision were evaluated for both types of water samples and good values were obtained (RSD < 10%). The applicability of the method for the detection of lower proportions of PP was assessed and the same fingerprints were obtained for each PP, even when the volume was decreased down to 0.05%. The results demonstrate the potential of HS-MS in this field.
abstract_unstemmed	In forensic and environmental sciences, the identification of petroleum-based products is an important task to establish not only the origin of a given residue but also the hazard level or the appropriate cleanup procedure. A new strategy for the fingerprinting of petroleum-based products (PP) in water samples (seawater and freshwater) for rapid and easy fuel spill identification has been developed. For this purpose, an HS-MS has been used in combination with chemometric tools such as linear discriminant analysis (LDA). A set of 70 samples from seven types of PPs (aromatic products, alcohols, normal alkanes, gasoline, diesel, lubricants and naphthenic-paraffinic products), all of which were added to water (seawater and freshwater), were analyzed. 100% of the samples were discriminated according to the type of petroleum-based products used regardless the nature of the water. Furthermore, a fingerprint was obtained for each petroleum product by plotting the m/z values selected by the LDA and this allowed the rapid identification of the petroleum products. The repeatability and intermediate precision were evaluated for both types of water samples and good values were obtained (RSD < 10%). The applicability of the method for the detection of lower proportions of PP was assessed and the same fingerprints were obtained for each PP, even when the volume was decreased down to 0.05%. The results demonstrate the potential of HS-MS in this field.
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title_short	Characterization of petroleum-based products in water samples by HS-MS
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author2	Aliaño-González, María José Barbero, Gerardo F. Palma, Miguel Barroso, Carmelo G.
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up_date	2024-07-06T23:24:55.579Z
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Characterization of petroleum-based products in water samples by HS-MS

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