High-power lactate/O
As lactate is a useful biomarker for evaluating conditions of the body and also has a high theoretical energy density as a fuel, enzymatic biofuel cells (BFCs) that utilize lactate as a fuel have received considerable attention. In this study, we have developed a high-power lactate/O2 BFC that compr...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Shitanda, Isao [verfasserIn] Takamatsu, Kotaro [verfasserIn] Niiyama, Ayumu [verfasserIn] Mikawa, Tsutomu [verfasserIn] Hoshi, Yoshinao [verfasserIn] Itagaki, Masayuki [verfasserIn] Tsujimura, Seiya [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2019 |
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| Schlagwörter: |
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| Übergeordnetes Werk: |
Enthalten in: Journal of power sources - New York, NY [u.a.] : Elsevier, 1976, 436 |
|---|---|
| Übergeordnetes Werk: |
volume:436 |
| DOI / URN: |
10.1016/j.jpowsour.2019.226844 |
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| Katalog-ID: |
ELV002698137 |
|---|
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| 100 | 1 | |a Shitanda, Isao |e verfasserin |0 (orcid)0000-0001-9751-016X |4 aut | |
| 245 | 1 | 0 | |a High-power lactate/O |
| 264 | 1 | |c 2019 | |
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| 520 | |a As lactate is a useful biomarker for evaluating conditions of the body and also has a high theoretical energy density as a fuel, enzymatic biofuel cells (BFCs) that utilize lactate as a fuel have received considerable attention. In this study, we have developed a high-power lactate/O2 BFC that comprises composite electrodes made from carbon cloth as a current collector and MgO-templated porous carbon as an electroenzymatic reaction field and enzyme support. The bioanode contains lactate oxidase as an enzyme and 1-methoxy-5-methylphenazinium methylsulfate as a redox mediator. The biocathode contains bilirubin oxidase as an oxygen reduction electrocatalyst and 2,2′-azino-bis(3-ethylbenzothiazoline-6-sulfonic acid) as a mediator. To obtain an efficient gas diffusion biocathode, the hydrophobicity of the carbon cloth is modulated by modification with PTFE. The lactate/O2 BFC shows a maximum power density of 4.3 mW cm−2 at a lactate concentration of 300 mM. This high performance is promising for the development of BFCs for wearable applications. | ||
| 650 | 4 | |a Biofuel cell | |
| 650 | 4 | |a Lactate | |
| 650 | 4 | |a Water repellent | |
| 650 | 4 | |a Lactate oxidase | |
| 650 | 4 | |a Bilirubin oxidase | |
| 700 | 1 | |a Takamatsu, Kotaro |e verfasserin |4 aut | |
| 700 | 1 | |a Niiyama, Ayumu |e verfasserin |4 aut | |
| 700 | 1 | |a Mikawa, Tsutomu |e verfasserin |4 aut | |
| 700 | 1 | |a Hoshi, Yoshinao |e verfasserin |4 aut | |
| 700 | 1 | |a Itagaki, Masayuki |e verfasserin |4 aut | |
| 700 | 1 | |a Tsujimura, Seiya |e verfasserin |0 (orcid)0000-0001-9603-2418 |4 aut | |
| 773 | 0 | 8 | |i Enthalten in |t Journal of power sources |d New York, NY [u.a.] : Elsevier, 1976 |g 436 |h Online-Ressource |w (DE-627)302718923 |w (DE-600)1491915-1 |w (DE-576)259483958 |x 1873-2755 |7 nnns |
| 773 | 1 | 8 | |g volume:436 |
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10.1016/j.jpowsour.2019.226844 doi (DE-627)ELV002698137 (ELSEVIER)S0378-7753(19)30837-7 DE-627 ger DE-627 rda eng 620 DE-600 52.57 bkl 53.36 bkl Shitanda, Isao verfasserin (orcid)0000-0001-9751-016X aut High-power lactate/O 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier As lactate is a useful biomarker for evaluating conditions of the body and also has a high theoretical energy density as a fuel, enzymatic biofuel cells (BFCs) that utilize lactate as a fuel have received considerable attention. In this study, we have developed a high-power lactate/O2 BFC that comprises composite electrodes made from carbon cloth as a current collector and MgO-templated porous carbon as an electroenzymatic reaction field and enzyme support. The bioanode contains lactate oxidase as an enzyme and 1-methoxy-5-methylphenazinium methylsulfate as a redox mediator. The biocathode contains bilirubin oxidase as an oxygen reduction electrocatalyst and 2,2′-azino-bis(3-ethylbenzothiazoline-6-sulfonic acid) as a mediator. To obtain an efficient gas diffusion biocathode, the hydrophobicity of the carbon cloth is modulated by modification with PTFE. The lactate/O2 BFC shows a maximum power density of 4.3 mW cm−2 at a lactate concentration of 300 mM. This high performance is promising for the development of BFCs for wearable applications. Biofuel cell Lactate Water repellent Lactate oxidase Bilirubin oxidase Takamatsu, Kotaro verfasserin aut Niiyama, Ayumu verfasserin aut Mikawa, Tsutomu verfasserin aut Hoshi, Yoshinao verfasserin aut Itagaki, Masayuki verfasserin aut Tsujimura, Seiya verfasserin (orcid)0000-0001-9603-2418 aut Enthalten in Journal of power sources New York, NY [u.a.] : Elsevier, 1976 436 Online-Ressource (DE-627)302718923 (DE-600)1491915-1 (DE-576)259483958 1873-2755 nnns volume:436 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 52.57 Energiespeicherung 53.36 Energiedirektumwandler elektrische Energiespeicher AR 436 |
| spelling |
10.1016/j.jpowsour.2019.226844 doi (DE-627)ELV002698137 (ELSEVIER)S0378-7753(19)30837-7 DE-627 ger DE-627 rda eng 620 DE-600 52.57 bkl 53.36 bkl Shitanda, Isao verfasserin (orcid)0000-0001-9751-016X aut High-power lactate/O 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier As lactate is a useful biomarker for evaluating conditions of the body and also has a high theoretical energy density as a fuel, enzymatic biofuel cells (BFCs) that utilize lactate as a fuel have received considerable attention. In this study, we have developed a high-power lactate/O2 BFC that comprises composite electrodes made from carbon cloth as a current collector and MgO-templated porous carbon as an electroenzymatic reaction field and enzyme support. The bioanode contains lactate oxidase as an enzyme and 1-methoxy-5-methylphenazinium methylsulfate as a redox mediator. The biocathode contains bilirubin oxidase as an oxygen reduction electrocatalyst and 2,2′-azino-bis(3-ethylbenzothiazoline-6-sulfonic acid) as a mediator. To obtain an efficient gas diffusion biocathode, the hydrophobicity of the carbon cloth is modulated by modification with PTFE. The lactate/O2 BFC shows a maximum power density of 4.3 mW cm−2 at a lactate concentration of 300 mM. This high performance is promising for the development of BFCs for wearable applications. Biofuel cell Lactate Water repellent Lactate oxidase Bilirubin oxidase Takamatsu, Kotaro verfasserin aut Niiyama, Ayumu verfasserin aut Mikawa, Tsutomu verfasserin aut Hoshi, Yoshinao verfasserin aut Itagaki, Masayuki verfasserin aut Tsujimura, Seiya verfasserin (orcid)0000-0001-9603-2418 aut Enthalten in Journal of power sources New York, NY [u.a.] : Elsevier, 1976 436 Online-Ressource (DE-627)302718923 (DE-600)1491915-1 (DE-576)259483958 1873-2755 nnns volume:436 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 52.57 Energiespeicherung 53.36 Energiedirektumwandler elektrische Energiespeicher AR 436 |
| allfields_unstemmed |
10.1016/j.jpowsour.2019.226844 doi (DE-627)ELV002698137 (ELSEVIER)S0378-7753(19)30837-7 DE-627 ger DE-627 rda eng 620 DE-600 52.57 bkl 53.36 bkl Shitanda, Isao verfasserin (orcid)0000-0001-9751-016X aut High-power lactate/O 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier As lactate is a useful biomarker for evaluating conditions of the body and also has a high theoretical energy density as a fuel, enzymatic biofuel cells (BFCs) that utilize lactate as a fuel have received considerable attention. In this study, we have developed a high-power lactate/O2 BFC that comprises composite electrodes made from carbon cloth as a current collector and MgO-templated porous carbon as an electroenzymatic reaction field and enzyme support. The bioanode contains lactate oxidase as an enzyme and 1-methoxy-5-methylphenazinium methylsulfate as a redox mediator. The biocathode contains bilirubin oxidase as an oxygen reduction electrocatalyst and 2,2′-azino-bis(3-ethylbenzothiazoline-6-sulfonic acid) as a mediator. To obtain an efficient gas diffusion biocathode, the hydrophobicity of the carbon cloth is modulated by modification with PTFE. The lactate/O2 BFC shows a maximum power density of 4.3 mW cm−2 at a lactate concentration of 300 mM. This high performance is promising for the development of BFCs for wearable applications. Biofuel cell Lactate Water repellent Lactate oxidase Bilirubin oxidase Takamatsu, Kotaro verfasserin aut Niiyama, Ayumu verfasserin aut Mikawa, Tsutomu verfasserin aut Hoshi, Yoshinao verfasserin aut Itagaki, Masayuki verfasserin aut Tsujimura, Seiya verfasserin (orcid)0000-0001-9603-2418 aut Enthalten in Journal of power sources New York, NY [u.a.] : Elsevier, 1976 436 Online-Ressource (DE-627)302718923 (DE-600)1491915-1 (DE-576)259483958 1873-2755 nnns volume:436 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 52.57 Energiespeicherung 53.36 Energiedirektumwandler elektrische Energiespeicher AR 436 |
| allfieldsGer |
10.1016/j.jpowsour.2019.226844 doi (DE-627)ELV002698137 (ELSEVIER)S0378-7753(19)30837-7 DE-627 ger DE-627 rda eng 620 DE-600 52.57 bkl 53.36 bkl Shitanda, Isao verfasserin (orcid)0000-0001-9751-016X aut High-power lactate/O 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier As lactate is a useful biomarker for evaluating conditions of the body and also has a high theoretical energy density as a fuel, enzymatic biofuel cells (BFCs) that utilize lactate as a fuel have received considerable attention. In this study, we have developed a high-power lactate/O2 BFC that comprises composite electrodes made from carbon cloth as a current collector and MgO-templated porous carbon as an electroenzymatic reaction field and enzyme support. The bioanode contains lactate oxidase as an enzyme and 1-methoxy-5-methylphenazinium methylsulfate as a redox mediator. The biocathode contains bilirubin oxidase as an oxygen reduction electrocatalyst and 2,2′-azino-bis(3-ethylbenzothiazoline-6-sulfonic acid) as a mediator. To obtain an efficient gas diffusion biocathode, the hydrophobicity of the carbon cloth is modulated by modification with PTFE. The lactate/O2 BFC shows a maximum power density of 4.3 mW cm−2 at a lactate concentration of 300 mM. This high performance is promising for the development of BFCs for wearable applications. Biofuel cell Lactate Water repellent Lactate oxidase Bilirubin oxidase Takamatsu, Kotaro verfasserin aut Niiyama, Ayumu verfasserin aut Mikawa, Tsutomu verfasserin aut Hoshi, Yoshinao verfasserin aut Itagaki, Masayuki verfasserin aut Tsujimura, Seiya verfasserin (orcid)0000-0001-9603-2418 aut Enthalten in Journal of power sources New York, NY [u.a.] : Elsevier, 1976 436 Online-Ressource (DE-627)302718923 (DE-600)1491915-1 (DE-576)259483958 1873-2755 nnns volume:436 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 52.57 Energiespeicherung 53.36 Energiedirektumwandler elektrische Energiespeicher AR 436 |
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10.1016/j.jpowsour.2019.226844 doi (DE-627)ELV002698137 (ELSEVIER)S0378-7753(19)30837-7 DE-627 ger DE-627 rda eng 620 DE-600 52.57 bkl 53.36 bkl Shitanda, Isao verfasserin (orcid)0000-0001-9751-016X aut High-power lactate/O 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier As lactate is a useful biomarker for evaluating conditions of the body and also has a high theoretical energy density as a fuel, enzymatic biofuel cells (BFCs) that utilize lactate as a fuel have received considerable attention. In this study, we have developed a high-power lactate/O2 BFC that comprises composite electrodes made from carbon cloth as a current collector and MgO-templated porous carbon as an electroenzymatic reaction field and enzyme support. The bioanode contains lactate oxidase as an enzyme and 1-methoxy-5-methylphenazinium methylsulfate as a redox mediator. The biocathode contains bilirubin oxidase as an oxygen reduction electrocatalyst and 2,2′-azino-bis(3-ethylbenzothiazoline-6-sulfonic acid) as a mediator. To obtain an efficient gas diffusion biocathode, the hydrophobicity of the carbon cloth is modulated by modification with PTFE. The lactate/O2 BFC shows a maximum power density of 4.3 mW cm−2 at a lactate concentration of 300 mM. This high performance is promising for the development of BFCs for wearable applications. Biofuel cell Lactate Water repellent Lactate oxidase Bilirubin oxidase Takamatsu, Kotaro verfasserin aut Niiyama, Ayumu verfasserin aut Mikawa, Tsutomu verfasserin aut Hoshi, Yoshinao verfasserin aut Itagaki, Masayuki verfasserin aut Tsujimura, Seiya verfasserin (orcid)0000-0001-9603-2418 aut Enthalten in Journal of power sources New York, NY [u.a.] : Elsevier, 1976 436 Online-Ressource (DE-627)302718923 (DE-600)1491915-1 (DE-576)259483958 1873-2755 nnns volume:436 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 52.57 Energiespeicherung 53.36 Energiedirektumwandler elektrische Energiespeicher AR 436 |
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Biofuel cell Lactate Water repellent Lactate oxidase Bilirubin oxidase |
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Shitanda, Isao @@aut@@ Takamatsu, Kotaro @@aut@@ Niiyama, Ayumu @@aut@@ Mikawa, Tsutomu @@aut@@ Hoshi, Yoshinao @@aut@@ Itagaki, Masayuki @@aut@@ Tsujimura, Seiya @@aut@@ |
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2019-01-01T00:00:00Z |
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620 DE-600 52.57 bkl 53.36 bkl High-power lactate/O Biofuel cell Lactate Water repellent Lactate oxidase Bilirubin oxidase |
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ddc 620 bkl 52.57 bkl 53.36 misc Biofuel cell misc Lactate misc Water repellent misc Lactate oxidase misc Bilirubin oxidase |
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Shitanda, Isao Takamatsu, Kotaro Niiyama, Ayumu Mikawa, Tsutomu Hoshi, Yoshinao Itagaki, Masayuki Tsujimura, Seiya |
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10.1016/j.jpowsour.2019.226844 |
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high-power lactate/o |
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High-power lactate/O |
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As lactate is a useful biomarker for evaluating conditions of the body and also has a high theoretical energy density as a fuel, enzymatic biofuel cells (BFCs) that utilize lactate as a fuel have received considerable attention. In this study, we have developed a high-power lactate/O2 BFC that comprises composite electrodes made from carbon cloth as a current collector and MgO-templated porous carbon as an electroenzymatic reaction field and enzyme support. The bioanode contains lactate oxidase as an enzyme and 1-methoxy-5-methylphenazinium methylsulfate as a redox mediator. The biocathode contains bilirubin oxidase as an oxygen reduction electrocatalyst and 2,2′-azino-bis(3-ethylbenzothiazoline-6-sulfonic acid) as a mediator. To obtain an efficient gas diffusion biocathode, the hydrophobicity of the carbon cloth is modulated by modification with PTFE. The lactate/O2 BFC shows a maximum power density of 4.3 mW cm−2 at a lactate concentration of 300 mM. This high performance is promising for the development of BFCs for wearable applications. |
| abstractGer |
As lactate is a useful biomarker for evaluating conditions of the body and also has a high theoretical energy density as a fuel, enzymatic biofuel cells (BFCs) that utilize lactate as a fuel have received considerable attention. In this study, we have developed a high-power lactate/O2 BFC that comprises composite electrodes made from carbon cloth as a current collector and MgO-templated porous carbon as an electroenzymatic reaction field and enzyme support. The bioanode contains lactate oxidase as an enzyme and 1-methoxy-5-methylphenazinium methylsulfate as a redox mediator. The biocathode contains bilirubin oxidase as an oxygen reduction electrocatalyst and 2,2′-azino-bis(3-ethylbenzothiazoline-6-sulfonic acid) as a mediator. To obtain an efficient gas diffusion biocathode, the hydrophobicity of the carbon cloth is modulated by modification with PTFE. The lactate/O2 BFC shows a maximum power density of 4.3 mW cm−2 at a lactate concentration of 300 mM. This high performance is promising for the development of BFCs for wearable applications. |
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As lactate is a useful biomarker for evaluating conditions of the body and also has a high theoretical energy density as a fuel, enzymatic biofuel cells (BFCs) that utilize lactate as a fuel have received considerable attention. In this study, we have developed a high-power lactate/O2 BFC that comprises composite electrodes made from carbon cloth as a current collector and MgO-templated porous carbon as an electroenzymatic reaction field and enzyme support. The bioanode contains lactate oxidase as an enzyme and 1-methoxy-5-methylphenazinium methylsulfate as a redox mediator. The biocathode contains bilirubin oxidase as an oxygen reduction electrocatalyst and 2,2′-azino-bis(3-ethylbenzothiazoline-6-sulfonic acid) as a mediator. To obtain an efficient gas diffusion biocathode, the hydrophobicity of the carbon cloth is modulated by modification with PTFE. The lactate/O2 BFC shows a maximum power density of 4.3 mW cm−2 at a lactate concentration of 300 mM. This high performance is promising for the development of BFCs for wearable applications. |
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Takamatsu, Kotaro Niiyama, Ayumu Mikawa, Tsutomu Hoshi, Yoshinao Itagaki, Masayuki Tsujimura, Seiya |
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