Enhanced particulate Hg export at the permafrost boundary, western Siberia
Arctic permafrost soils contain large amounts of organic carbon and the pollutant mercury (Hg). Arctic warming and associated changes in hydrology, biogeochemistry and ecology risk mobilizing soil Hg to rivers and to the Arctic Ocean, yet little is known about the quantity, timing and mechanisms inv...
Ausführliche Beschreibung
Autor*in: |
Lim, Artem G. [verfasserIn] Sonke, Jeroen E. [verfasserIn] Krickov, Ivan V. [verfasserIn] Manasypov, Rinat M. [verfasserIn] Loiko, Sergey V. [verfasserIn] Pokrovsky, Oleg S. [verfasserIn] |
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Format: |
E-Artikel |
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Sprache: |
Englisch |
Erschienen: |
2019 |
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Schlagwörter: |
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Übergeordnetes Werk: |
Enthalten in: Environmental pollution - Amsterdam [u.a.] : Elsevier Science, 1970, 254 |
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Übergeordnetes Werk: |
volume:254 |
DOI / URN: |
10.1016/j.envpol.2019.113083 |
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Katalog-ID: |
ELV002892014 |
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520 | |a Arctic permafrost soils contain large amounts of organic carbon and the pollutant mercury (Hg). Arctic warming and associated changes in hydrology, biogeochemistry and ecology risk mobilizing soil Hg to rivers and to the Arctic Ocean, yet little is known about the quantity, timing and mechanisms involved. Here we investigate seasonal particulate Hg (PHg) and organic carbon (POC) export in 32 small and medium rivers across a 1700 km latitudinal permafrost transect of the western Siberian Lowland. The PHg concentrations in suspended matter increased with decreasing watershed size. This underlines the significance of POC-rich small streams and wetlands in PHg export from watersheds. Maximum PHg concentrations and export fluxes were located in rivers at the beginning of permafrost zone (sporadic permafrost). We suggest this reflects enhanced Hg mobilization at the permafrost boundary, due to maximal depth of the thawed peat layer. Both the thickness of the active (unfrozen) peat layer and PHg run-off progressively move to the north during the summer and fall seasons, thus leading to maximal PHg export at the sporadic to discontinuous permafrost zone. The discharge-weighed PHg:POC ratio in western Siberian rivers (2.7 ± 0.5 μg Hg: g C) extrapolated to the whole Ob River basin yields a PHg flux of 1.5 ± 0.3 Mg y−1, consistent with previous estimates. For current climate warming and permafrost thaw scenarios in western Siberia, we predict that a northward shift of permafrost boundaries and increase of active layer depth may enhance the PHg export by small rivers to the Arctic Ocean by a factor of two over the next 10–50 years. | ||
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700 | 1 | |a Sonke, Jeroen E. |e verfasserin |4 aut | |
700 | 1 | |a Krickov, Ivan V. |e verfasserin |4 aut | |
700 | 1 | |a Manasypov, Rinat M. |e verfasserin |4 aut | |
700 | 1 | |a Loiko, Sergey V. |e verfasserin |4 aut | |
700 | 1 | |a Pokrovsky, Oleg S. |e verfasserin |4 aut | |
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10.1016/j.envpol.2019.113083 doi (DE-627)ELV002892014 (ELSEVIER)S0269-7491(19)32132-3 DE-627 ger DE-627 rda eng 333.7 570 690 DE-600 BIODIV DE-30 fid 48.00 bkl Lim, Artem G. verfasserin aut Enhanced particulate Hg export at the permafrost boundary, western Siberia 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Arctic permafrost soils contain large amounts of organic carbon and the pollutant mercury (Hg). Arctic warming and associated changes in hydrology, biogeochemistry and ecology risk mobilizing soil Hg to rivers and to the Arctic Ocean, yet little is known about the quantity, timing and mechanisms involved. Here we investigate seasonal particulate Hg (PHg) and organic carbon (POC) export in 32 small and medium rivers across a 1700 km latitudinal permafrost transect of the western Siberian Lowland. The PHg concentrations in suspended matter increased with decreasing watershed size. This underlines the significance of POC-rich small streams and wetlands in PHg export from watersheds. Maximum PHg concentrations and export fluxes were located in rivers at the beginning of permafrost zone (sporadic permafrost). We suggest this reflects enhanced Hg mobilization at the permafrost boundary, due to maximal depth of the thawed peat layer. Both the thickness of the active (unfrozen) peat layer and PHg run-off progressively move to the north during the summer and fall seasons, thus leading to maximal PHg export at the sporadic to discontinuous permafrost zone. The discharge-weighed PHg:POC ratio in western Siberian rivers (2.7 ± 0.5 μg Hg: g C) extrapolated to the whole Ob River basin yields a PHg flux of 1.5 ± 0.3 Mg y−1, consistent with previous estimates. For current climate warming and permafrost thaw scenarios in western Siberia, we predict that a northward shift of permafrost boundaries and increase of active layer depth may enhance the PHg export by small rivers to the Arctic Ocean by a factor of two over the next 10–50 years. Particulate Suspended Landscape Bog Lake Forest Thaw Siberia Sonke, Jeroen E. verfasserin aut Krickov, Ivan V. verfasserin aut Manasypov, Rinat M. verfasserin aut Loiko, Sergey V. verfasserin aut Pokrovsky, Oleg S. verfasserin aut Enthalten in Environmental pollution Amsterdam [u.a.] : Elsevier Science, 1970 254 Online-Ressource (DE-627)320507750 (DE-600)2013037-5 (DE-576)094752591 1873-6424 nnns volume:254 GBV_USEFLAG_U SYSFLAG_U GBV_ELV FID-BIODIV SSG-OLC-PHA SSG-OPC-FOR GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 48.00 Land- und Forstwirtschaft: Allgemeines AR 254 |
spelling |
10.1016/j.envpol.2019.113083 doi (DE-627)ELV002892014 (ELSEVIER)S0269-7491(19)32132-3 DE-627 ger DE-627 rda eng 333.7 570 690 DE-600 BIODIV DE-30 fid 48.00 bkl Lim, Artem G. verfasserin aut Enhanced particulate Hg export at the permafrost boundary, western Siberia 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Arctic permafrost soils contain large amounts of organic carbon and the pollutant mercury (Hg). Arctic warming and associated changes in hydrology, biogeochemistry and ecology risk mobilizing soil Hg to rivers and to the Arctic Ocean, yet little is known about the quantity, timing and mechanisms involved. Here we investigate seasonal particulate Hg (PHg) and organic carbon (POC) export in 32 small and medium rivers across a 1700 km latitudinal permafrost transect of the western Siberian Lowland. The PHg concentrations in suspended matter increased with decreasing watershed size. This underlines the significance of POC-rich small streams and wetlands in PHg export from watersheds. Maximum PHg concentrations and export fluxes were located in rivers at the beginning of permafrost zone (sporadic permafrost). We suggest this reflects enhanced Hg mobilization at the permafrost boundary, due to maximal depth of the thawed peat layer. Both the thickness of the active (unfrozen) peat layer and PHg run-off progressively move to the north during the summer and fall seasons, thus leading to maximal PHg export at the sporadic to discontinuous permafrost zone. The discharge-weighed PHg:POC ratio in western Siberian rivers (2.7 ± 0.5 μg Hg: g C) extrapolated to the whole Ob River basin yields a PHg flux of 1.5 ± 0.3 Mg y−1, consistent with previous estimates. For current climate warming and permafrost thaw scenarios in western Siberia, we predict that a northward shift of permafrost boundaries and increase of active layer depth may enhance the PHg export by small rivers to the Arctic Ocean by a factor of two over the next 10–50 years. Particulate Suspended Landscape Bog Lake Forest Thaw Siberia Sonke, Jeroen E. verfasserin aut Krickov, Ivan V. verfasserin aut Manasypov, Rinat M. verfasserin aut Loiko, Sergey V. verfasserin aut Pokrovsky, Oleg S. verfasserin aut Enthalten in Environmental pollution Amsterdam [u.a.] : Elsevier Science, 1970 254 Online-Ressource (DE-627)320507750 (DE-600)2013037-5 (DE-576)094752591 1873-6424 nnns volume:254 GBV_USEFLAG_U SYSFLAG_U GBV_ELV FID-BIODIV SSG-OLC-PHA SSG-OPC-FOR GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 48.00 Land- und Forstwirtschaft: Allgemeines AR 254 |
allfields_unstemmed |
10.1016/j.envpol.2019.113083 doi (DE-627)ELV002892014 (ELSEVIER)S0269-7491(19)32132-3 DE-627 ger DE-627 rda eng 333.7 570 690 DE-600 BIODIV DE-30 fid 48.00 bkl Lim, Artem G. verfasserin aut Enhanced particulate Hg export at the permafrost boundary, western Siberia 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Arctic permafrost soils contain large amounts of organic carbon and the pollutant mercury (Hg). Arctic warming and associated changes in hydrology, biogeochemistry and ecology risk mobilizing soil Hg to rivers and to the Arctic Ocean, yet little is known about the quantity, timing and mechanisms involved. Here we investigate seasonal particulate Hg (PHg) and organic carbon (POC) export in 32 small and medium rivers across a 1700 km latitudinal permafrost transect of the western Siberian Lowland. The PHg concentrations in suspended matter increased with decreasing watershed size. This underlines the significance of POC-rich small streams and wetlands in PHg export from watersheds. Maximum PHg concentrations and export fluxes were located in rivers at the beginning of permafrost zone (sporadic permafrost). We suggest this reflects enhanced Hg mobilization at the permafrost boundary, due to maximal depth of the thawed peat layer. Both the thickness of the active (unfrozen) peat layer and PHg run-off progressively move to the north during the summer and fall seasons, thus leading to maximal PHg export at the sporadic to discontinuous permafrost zone. The discharge-weighed PHg:POC ratio in western Siberian rivers (2.7 ± 0.5 μg Hg: g C) extrapolated to the whole Ob River basin yields a PHg flux of 1.5 ± 0.3 Mg y−1, consistent with previous estimates. For current climate warming and permafrost thaw scenarios in western Siberia, we predict that a northward shift of permafrost boundaries and increase of active layer depth may enhance the PHg export by small rivers to the Arctic Ocean by a factor of two over the next 10–50 years. Particulate Suspended Landscape Bog Lake Forest Thaw Siberia Sonke, Jeroen E. verfasserin aut Krickov, Ivan V. verfasserin aut Manasypov, Rinat M. verfasserin aut Loiko, Sergey V. verfasserin aut Pokrovsky, Oleg S. verfasserin aut Enthalten in Environmental pollution Amsterdam [u.a.] : Elsevier Science, 1970 254 Online-Ressource (DE-627)320507750 (DE-600)2013037-5 (DE-576)094752591 1873-6424 nnns volume:254 GBV_USEFLAG_U SYSFLAG_U GBV_ELV FID-BIODIV SSG-OLC-PHA SSG-OPC-FOR GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 48.00 Land- und Forstwirtschaft: Allgemeines AR 254 |
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10.1016/j.envpol.2019.113083 doi (DE-627)ELV002892014 (ELSEVIER)S0269-7491(19)32132-3 DE-627 ger DE-627 rda eng 333.7 570 690 DE-600 BIODIV DE-30 fid 48.00 bkl Lim, Artem G. verfasserin aut Enhanced particulate Hg export at the permafrost boundary, western Siberia 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Arctic permafrost soils contain large amounts of organic carbon and the pollutant mercury (Hg). Arctic warming and associated changes in hydrology, biogeochemistry and ecology risk mobilizing soil Hg to rivers and to the Arctic Ocean, yet little is known about the quantity, timing and mechanisms involved. Here we investigate seasonal particulate Hg (PHg) and organic carbon (POC) export in 32 small and medium rivers across a 1700 km latitudinal permafrost transect of the western Siberian Lowland. The PHg concentrations in suspended matter increased with decreasing watershed size. This underlines the significance of POC-rich small streams and wetlands in PHg export from watersheds. Maximum PHg concentrations and export fluxes were located in rivers at the beginning of permafrost zone (sporadic permafrost). We suggest this reflects enhanced Hg mobilization at the permafrost boundary, due to maximal depth of the thawed peat layer. Both the thickness of the active (unfrozen) peat layer and PHg run-off progressively move to the north during the summer and fall seasons, thus leading to maximal PHg export at the sporadic to discontinuous permafrost zone. The discharge-weighed PHg:POC ratio in western Siberian rivers (2.7 ± 0.5 μg Hg: g C) extrapolated to the whole Ob River basin yields a PHg flux of 1.5 ± 0.3 Mg y−1, consistent with previous estimates. For current climate warming and permafrost thaw scenarios in western Siberia, we predict that a northward shift of permafrost boundaries and increase of active layer depth may enhance the PHg export by small rivers to the Arctic Ocean by a factor of two over the next 10–50 years. Particulate Suspended Landscape Bog Lake Forest Thaw Siberia Sonke, Jeroen E. verfasserin aut Krickov, Ivan V. verfasserin aut Manasypov, Rinat M. verfasserin aut Loiko, Sergey V. verfasserin aut Pokrovsky, Oleg S. verfasserin aut Enthalten in Environmental pollution Amsterdam [u.a.] : Elsevier Science, 1970 254 Online-Ressource (DE-627)320507750 (DE-600)2013037-5 (DE-576)094752591 1873-6424 nnns volume:254 GBV_USEFLAG_U SYSFLAG_U GBV_ELV FID-BIODIV SSG-OLC-PHA SSG-OPC-FOR GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 48.00 Land- und Forstwirtschaft: Allgemeines AR 254 |
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10.1016/j.envpol.2019.113083 doi (DE-627)ELV002892014 (ELSEVIER)S0269-7491(19)32132-3 DE-627 ger DE-627 rda eng 333.7 570 690 DE-600 BIODIV DE-30 fid 48.00 bkl Lim, Artem G. verfasserin aut Enhanced particulate Hg export at the permafrost boundary, western Siberia 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Arctic permafrost soils contain large amounts of organic carbon and the pollutant mercury (Hg). Arctic warming and associated changes in hydrology, biogeochemistry and ecology risk mobilizing soil Hg to rivers and to the Arctic Ocean, yet little is known about the quantity, timing and mechanisms involved. Here we investigate seasonal particulate Hg (PHg) and organic carbon (POC) export in 32 small and medium rivers across a 1700 km latitudinal permafrost transect of the western Siberian Lowland. The PHg concentrations in suspended matter increased with decreasing watershed size. This underlines the significance of POC-rich small streams and wetlands in PHg export from watersheds. Maximum PHg concentrations and export fluxes were located in rivers at the beginning of permafrost zone (sporadic permafrost). We suggest this reflects enhanced Hg mobilization at the permafrost boundary, due to maximal depth of the thawed peat layer. Both the thickness of the active (unfrozen) peat layer and PHg run-off progressively move to the north during the summer and fall seasons, thus leading to maximal PHg export at the sporadic to discontinuous permafrost zone. The discharge-weighed PHg:POC ratio in western Siberian rivers (2.7 ± 0.5 μg Hg: g C) extrapolated to the whole Ob River basin yields a PHg flux of 1.5 ± 0.3 Mg y−1, consistent with previous estimates. For current climate warming and permafrost thaw scenarios in western Siberia, we predict that a northward shift of permafrost boundaries and increase of active layer depth may enhance the PHg export by small rivers to the Arctic Ocean by a factor of two over the next 10–50 years. Particulate Suspended Landscape Bog Lake Forest Thaw Siberia Sonke, Jeroen E. verfasserin aut Krickov, Ivan V. verfasserin aut Manasypov, Rinat M. verfasserin aut Loiko, Sergey V. verfasserin aut Pokrovsky, Oleg S. verfasserin aut Enthalten in Environmental pollution Amsterdam [u.a.] : Elsevier Science, 1970 254 Online-Ressource (DE-627)320507750 (DE-600)2013037-5 (DE-576)094752591 1873-6424 nnns volume:254 GBV_USEFLAG_U SYSFLAG_U GBV_ELV FID-BIODIV SSG-OLC-PHA SSG-OPC-FOR GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 48.00 Land- und Forstwirtschaft: Allgemeines AR 254 |
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Lim, Artem G. @@aut@@ Sonke, Jeroen E. @@aut@@ Krickov, Ivan V. @@aut@@ Manasypov, Rinat M. @@aut@@ Loiko, Sergey V. @@aut@@ Pokrovsky, Oleg S. @@aut@@ |
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Lim, Artem G. ddc 333.7 fid BIODIV bkl 48.00 misc Particulate misc Suspended misc Landscape misc Bog misc Lake misc Forest misc Thaw misc Siberia Enhanced particulate Hg export at the permafrost boundary, western Siberia |
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333.7 570 690 DE-600 BIODIV DE-30 fid 48.00 bkl Enhanced particulate Hg export at the permafrost boundary, western Siberia Particulate Suspended Landscape Bog Lake Forest Thaw Siberia |
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Enhanced particulate Hg export at the permafrost boundary, western Siberia |
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Enhanced particulate Hg export at the permafrost boundary, western Siberia |
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Lim, Artem G. Sonke, Jeroen E. Krickov, Ivan V. Manasypov, Rinat M. Loiko, Sergey V. Pokrovsky, Oleg S. |
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enhanced particulate hg export at the permafrost boundary, western siberia |
title_auth |
Enhanced particulate Hg export at the permafrost boundary, western Siberia |
abstract |
Arctic permafrost soils contain large amounts of organic carbon and the pollutant mercury (Hg). Arctic warming and associated changes in hydrology, biogeochemistry and ecology risk mobilizing soil Hg to rivers and to the Arctic Ocean, yet little is known about the quantity, timing and mechanisms involved. Here we investigate seasonal particulate Hg (PHg) and organic carbon (POC) export in 32 small and medium rivers across a 1700 km latitudinal permafrost transect of the western Siberian Lowland. The PHg concentrations in suspended matter increased with decreasing watershed size. This underlines the significance of POC-rich small streams and wetlands in PHg export from watersheds. Maximum PHg concentrations and export fluxes were located in rivers at the beginning of permafrost zone (sporadic permafrost). We suggest this reflects enhanced Hg mobilization at the permafrost boundary, due to maximal depth of the thawed peat layer. Both the thickness of the active (unfrozen) peat layer and PHg run-off progressively move to the north during the summer and fall seasons, thus leading to maximal PHg export at the sporadic to discontinuous permafrost zone. The discharge-weighed PHg:POC ratio in western Siberian rivers (2.7 ± 0.5 μg Hg: g C) extrapolated to the whole Ob River basin yields a PHg flux of 1.5 ± 0.3 Mg y−1, consistent with previous estimates. For current climate warming and permafrost thaw scenarios in western Siberia, we predict that a northward shift of permafrost boundaries and increase of active layer depth may enhance the PHg export by small rivers to the Arctic Ocean by a factor of two over the next 10–50 years. |
abstractGer |
Arctic permafrost soils contain large amounts of organic carbon and the pollutant mercury (Hg). Arctic warming and associated changes in hydrology, biogeochemistry and ecology risk mobilizing soil Hg to rivers and to the Arctic Ocean, yet little is known about the quantity, timing and mechanisms involved. Here we investigate seasonal particulate Hg (PHg) and organic carbon (POC) export in 32 small and medium rivers across a 1700 km latitudinal permafrost transect of the western Siberian Lowland. The PHg concentrations in suspended matter increased with decreasing watershed size. This underlines the significance of POC-rich small streams and wetlands in PHg export from watersheds. Maximum PHg concentrations and export fluxes were located in rivers at the beginning of permafrost zone (sporadic permafrost). We suggest this reflects enhanced Hg mobilization at the permafrost boundary, due to maximal depth of the thawed peat layer. Both the thickness of the active (unfrozen) peat layer and PHg run-off progressively move to the north during the summer and fall seasons, thus leading to maximal PHg export at the sporadic to discontinuous permafrost zone. The discharge-weighed PHg:POC ratio in western Siberian rivers (2.7 ± 0.5 μg Hg: g C) extrapolated to the whole Ob River basin yields a PHg flux of 1.5 ± 0.3 Mg y−1, consistent with previous estimates. For current climate warming and permafrost thaw scenarios in western Siberia, we predict that a northward shift of permafrost boundaries and increase of active layer depth may enhance the PHg export by small rivers to the Arctic Ocean by a factor of two over the next 10–50 years. |
abstract_unstemmed |
Arctic permafrost soils contain large amounts of organic carbon and the pollutant mercury (Hg). Arctic warming and associated changes in hydrology, biogeochemistry and ecology risk mobilizing soil Hg to rivers and to the Arctic Ocean, yet little is known about the quantity, timing and mechanisms involved. Here we investigate seasonal particulate Hg (PHg) and organic carbon (POC) export in 32 small and medium rivers across a 1700 km latitudinal permafrost transect of the western Siberian Lowland. The PHg concentrations in suspended matter increased with decreasing watershed size. This underlines the significance of POC-rich small streams and wetlands in PHg export from watersheds. Maximum PHg concentrations and export fluxes were located in rivers at the beginning of permafrost zone (sporadic permafrost). We suggest this reflects enhanced Hg mobilization at the permafrost boundary, due to maximal depth of the thawed peat layer. Both the thickness of the active (unfrozen) peat layer and PHg run-off progressively move to the north during the summer and fall seasons, thus leading to maximal PHg export at the sporadic to discontinuous permafrost zone. The discharge-weighed PHg:POC ratio in western Siberian rivers (2.7 ± 0.5 μg Hg: g C) extrapolated to the whole Ob River basin yields a PHg flux of 1.5 ± 0.3 Mg y−1, consistent with previous estimates. For current climate warming and permafrost thaw scenarios in western Siberia, we predict that a northward shift of permafrost boundaries and increase of active layer depth may enhance the PHg export by small rivers to the Arctic Ocean by a factor of two over the next 10–50 years. |
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title_short |
Enhanced particulate Hg export at the permafrost boundary, western Siberia |
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score |
7.399989 |