Gold nanorods/g-C
Recently, broad spectrum (visible and near-infrared (NIR)) light utilization has aroused widespread attention in the research of photocatalysis. While g-C3N4, highly stable, cheap and easily synthesized, shows H2 evolution activity under visible light irradiation, it doesn’t perform under NIR light...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Tian, Huiyu [verfasserIn] Liu, Xiang [verfasserIn] Liang, Zhangqian [verfasserIn] Qiu, Pengyuan [verfasserIn] Qian, Xiu [verfasserIn] Cui, Hongzhi [verfasserIn] Tian, Jian [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2019 |
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| Schlagwörter: |
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| Übergeordnetes Werk: |
Enthalten in: Journal of colloid and interface science - Amsterdam [u.a.] : Elsevier, 1966, 557, Seite 700-708 |
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| Übergeordnetes Werk: |
volume:557 ; pages:700-708 |
| DOI / URN: |
10.1016/j.jcis.2019.09.075 |
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| Katalog-ID: |
ELV003044424 |
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| 520 | |a Recently, broad spectrum (visible and near-infrared (NIR)) light utilization has aroused widespread attention in the research of photocatalysis. While g-C3N4, highly stable, cheap and easily synthesized, shows H2 evolution activity under visible light irradiation, it doesn’t perform under NIR light irradiation. Here we report an Au nanorods (NRs)/g-C3N4 heterostructure with Au nanorods on g-C3N4’s surface. The most exciting feature of designed Au NRs/g-C3N4 heterostructures is that Au nanorods themselves are excited by visible and NIR light, which produce hot electrons and inject into g-C3N4. The photocatalytic H2 evolution rate of Au NRs/g-C3N4 heterostructures (350.6 μmol g−1 h−1) is nearly 4 times higher than that of g-C3N4 with Pt as cocatalyst (68.9 μmol g−1 h−1) under visible light illumination. The improved photocatalytic activity is ascribed to the increasing visible light-absorbing capacity of transverse surface plasmon resonance (TSPR) of Au nanorods and improved charge separation of Au NRs/g-C3N4 heterostructure. Even more important, Au NRs/g-C3N4 heterostructures achieve NIR photocatalytic H2 evolution performance (63.1 μmol g−1 h−1), owing to the longitudinal SPR (LSPR) effect of Au nanorods induced NIR light harvesting ability. | ||
| 650 | 4 | |a Photocatalytic H | |
| 650 | 4 | |a g-C | |
| 650 | 4 | |a Au nanorods | |
| 650 | 4 | |a Near-infrared | |
| 650 | 4 | |a Visible | |
| 700 | 1 | |a Liu, Xiang |e verfasserin |4 aut | |
| 700 | 1 | |a Liang, Zhangqian |e verfasserin |4 aut | |
| 700 | 1 | |a Qiu, Pengyuan |e verfasserin |4 aut | |
| 700 | 1 | |a Qian, Xiu |e verfasserin |4 aut | |
| 700 | 1 | |a Cui, Hongzhi |e verfasserin |0 (orcid)0000-0002-2212-0295 |4 aut | |
| 700 | 1 | |a Tian, Jian |e verfasserin |4 aut | |
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10.1016/j.jcis.2019.09.075 doi (DE-627)ELV003044424 (ELSEVIER)S0021-9797(19)31119-1 DE-627 ger DE-627 rda eng 540 DE-600 35.18 bkl Tian, Huiyu verfasserin aut Gold nanorods/g-C 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Recently, broad spectrum (visible and near-infrared (NIR)) light utilization has aroused widespread attention in the research of photocatalysis. While g-C3N4, highly stable, cheap and easily synthesized, shows H2 evolution activity under visible light irradiation, it doesn’t perform under NIR light irradiation. Here we report an Au nanorods (NRs)/g-C3N4 heterostructure with Au nanorods on g-C3N4’s surface. The most exciting feature of designed Au NRs/g-C3N4 heterostructures is that Au nanorods themselves are excited by visible and NIR light, which produce hot electrons and inject into g-C3N4. The photocatalytic H2 evolution rate of Au NRs/g-C3N4 heterostructures (350.6 μmol g−1 h−1) is nearly 4 times higher than that of g-C3N4 with Pt as cocatalyst (68.9 μmol g−1 h−1) under visible light illumination. The improved photocatalytic activity is ascribed to the increasing visible light-absorbing capacity of transverse surface plasmon resonance (TSPR) of Au nanorods and improved charge separation of Au NRs/g-C3N4 heterostructure. Even more important, Au NRs/g-C3N4 heterostructures achieve NIR photocatalytic H2 evolution performance (63.1 μmol g−1 h−1), owing to the longitudinal SPR (LSPR) effect of Au nanorods induced NIR light harvesting ability. Photocatalytic H g-C Au nanorods Near-infrared Visible Liu, Xiang verfasserin aut Liang, Zhangqian verfasserin aut Qiu, Pengyuan verfasserin aut Qian, Xiu verfasserin aut Cui, Hongzhi verfasserin (orcid)0000-0002-2212-0295 aut Tian, Jian verfasserin aut Enthalten in Journal of colloid and interface science Amsterdam [u.a.] : Elsevier, 1966 557, Seite 700-708 Online-Ressource (DE-627)266891136 (DE-600)1469021-4 (DE-576)103373160 1095-7103 nnns volume:557 pages:700-708 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2411 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.18 Kolloidchemie Grenzflächenchemie AR 557 700-708 |
| spelling |
10.1016/j.jcis.2019.09.075 doi (DE-627)ELV003044424 (ELSEVIER)S0021-9797(19)31119-1 DE-627 ger DE-627 rda eng 540 DE-600 35.18 bkl Tian, Huiyu verfasserin aut Gold nanorods/g-C 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Recently, broad spectrum (visible and near-infrared (NIR)) light utilization has aroused widespread attention in the research of photocatalysis. While g-C3N4, highly stable, cheap and easily synthesized, shows H2 evolution activity under visible light irradiation, it doesn’t perform under NIR light irradiation. Here we report an Au nanorods (NRs)/g-C3N4 heterostructure with Au nanorods on g-C3N4’s surface. The most exciting feature of designed Au NRs/g-C3N4 heterostructures is that Au nanorods themselves are excited by visible and NIR light, which produce hot electrons and inject into g-C3N4. The photocatalytic H2 evolution rate of Au NRs/g-C3N4 heterostructures (350.6 μmol g−1 h−1) is nearly 4 times higher than that of g-C3N4 with Pt as cocatalyst (68.9 μmol g−1 h−1) under visible light illumination. The improved photocatalytic activity is ascribed to the increasing visible light-absorbing capacity of transverse surface plasmon resonance (TSPR) of Au nanorods and improved charge separation of Au NRs/g-C3N4 heterostructure. Even more important, Au NRs/g-C3N4 heterostructures achieve NIR photocatalytic H2 evolution performance (63.1 μmol g−1 h−1), owing to the longitudinal SPR (LSPR) effect of Au nanorods induced NIR light harvesting ability. Photocatalytic H g-C Au nanorods Near-infrared Visible Liu, Xiang verfasserin aut Liang, Zhangqian verfasserin aut Qiu, Pengyuan verfasserin aut Qian, Xiu verfasserin aut Cui, Hongzhi verfasserin (orcid)0000-0002-2212-0295 aut Tian, Jian verfasserin aut Enthalten in Journal of colloid and interface science Amsterdam [u.a.] : Elsevier, 1966 557, Seite 700-708 Online-Ressource (DE-627)266891136 (DE-600)1469021-4 (DE-576)103373160 1095-7103 nnns volume:557 pages:700-708 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2411 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.18 Kolloidchemie Grenzflächenchemie AR 557 700-708 |
| allfields_unstemmed |
10.1016/j.jcis.2019.09.075 doi (DE-627)ELV003044424 (ELSEVIER)S0021-9797(19)31119-1 DE-627 ger DE-627 rda eng 540 DE-600 35.18 bkl Tian, Huiyu verfasserin aut Gold nanorods/g-C 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Recently, broad spectrum (visible and near-infrared (NIR)) light utilization has aroused widespread attention in the research of photocatalysis. While g-C3N4, highly stable, cheap and easily synthesized, shows H2 evolution activity under visible light irradiation, it doesn’t perform under NIR light irradiation. Here we report an Au nanorods (NRs)/g-C3N4 heterostructure with Au nanorods on g-C3N4’s surface. The most exciting feature of designed Au NRs/g-C3N4 heterostructures is that Au nanorods themselves are excited by visible and NIR light, which produce hot electrons and inject into g-C3N4. The photocatalytic H2 evolution rate of Au NRs/g-C3N4 heterostructures (350.6 μmol g−1 h−1) is nearly 4 times higher than that of g-C3N4 with Pt as cocatalyst (68.9 μmol g−1 h−1) under visible light illumination. The improved photocatalytic activity is ascribed to the increasing visible light-absorbing capacity of transverse surface plasmon resonance (TSPR) of Au nanorods and improved charge separation of Au NRs/g-C3N4 heterostructure. Even more important, Au NRs/g-C3N4 heterostructures achieve NIR photocatalytic H2 evolution performance (63.1 μmol g−1 h−1), owing to the longitudinal SPR (LSPR) effect of Au nanorods induced NIR light harvesting ability. Photocatalytic H g-C Au nanorods Near-infrared Visible Liu, Xiang verfasserin aut Liang, Zhangqian verfasserin aut Qiu, Pengyuan verfasserin aut Qian, Xiu verfasserin aut Cui, Hongzhi verfasserin (orcid)0000-0002-2212-0295 aut Tian, Jian verfasserin aut Enthalten in Journal of colloid and interface science Amsterdam [u.a.] : Elsevier, 1966 557, Seite 700-708 Online-Ressource (DE-627)266891136 (DE-600)1469021-4 (DE-576)103373160 1095-7103 nnns volume:557 pages:700-708 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2411 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.18 Kolloidchemie Grenzflächenchemie AR 557 700-708 |
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10.1016/j.jcis.2019.09.075 doi (DE-627)ELV003044424 (ELSEVIER)S0021-9797(19)31119-1 DE-627 ger DE-627 rda eng 540 DE-600 35.18 bkl Tian, Huiyu verfasserin aut Gold nanorods/g-C 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Recently, broad spectrum (visible and near-infrared (NIR)) light utilization has aroused widespread attention in the research of photocatalysis. While g-C3N4, highly stable, cheap and easily synthesized, shows H2 evolution activity under visible light irradiation, it doesn’t perform under NIR light irradiation. Here we report an Au nanorods (NRs)/g-C3N4 heterostructure with Au nanorods on g-C3N4’s surface. The most exciting feature of designed Au NRs/g-C3N4 heterostructures is that Au nanorods themselves are excited by visible and NIR light, which produce hot electrons and inject into g-C3N4. The photocatalytic H2 evolution rate of Au NRs/g-C3N4 heterostructures (350.6 μmol g−1 h−1) is nearly 4 times higher than that of g-C3N4 with Pt as cocatalyst (68.9 μmol g−1 h−1) under visible light illumination. The improved photocatalytic activity is ascribed to the increasing visible light-absorbing capacity of transverse surface plasmon resonance (TSPR) of Au nanorods and improved charge separation of Au NRs/g-C3N4 heterostructure. Even more important, Au NRs/g-C3N4 heterostructures achieve NIR photocatalytic H2 evolution performance (63.1 μmol g−1 h−1), owing to the longitudinal SPR (LSPR) effect of Au nanorods induced NIR light harvesting ability. Photocatalytic H g-C Au nanorods Near-infrared Visible Liu, Xiang verfasserin aut Liang, Zhangqian verfasserin aut Qiu, Pengyuan verfasserin aut Qian, Xiu verfasserin aut Cui, Hongzhi verfasserin (orcid)0000-0002-2212-0295 aut Tian, Jian verfasserin aut Enthalten in Journal of colloid and interface science Amsterdam [u.a.] : Elsevier, 1966 557, Seite 700-708 Online-Ressource (DE-627)266891136 (DE-600)1469021-4 (DE-576)103373160 1095-7103 nnns volume:557 pages:700-708 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2411 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.18 Kolloidchemie Grenzflächenchemie AR 557 700-708 |
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10.1016/j.jcis.2019.09.075 doi (DE-627)ELV003044424 (ELSEVIER)S0021-9797(19)31119-1 DE-627 ger DE-627 rda eng 540 DE-600 35.18 bkl Tian, Huiyu verfasserin aut Gold nanorods/g-C 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Recently, broad spectrum (visible and near-infrared (NIR)) light utilization has aroused widespread attention in the research of photocatalysis. While g-C3N4, highly stable, cheap and easily synthesized, shows H2 evolution activity under visible light irradiation, it doesn’t perform under NIR light irradiation. Here we report an Au nanorods (NRs)/g-C3N4 heterostructure with Au nanorods on g-C3N4’s surface. The most exciting feature of designed Au NRs/g-C3N4 heterostructures is that Au nanorods themselves are excited by visible and NIR light, which produce hot electrons and inject into g-C3N4. The photocatalytic H2 evolution rate of Au NRs/g-C3N4 heterostructures (350.6 μmol g−1 h−1) is nearly 4 times higher than that of g-C3N4 with Pt as cocatalyst (68.9 μmol g−1 h−1) under visible light illumination. The improved photocatalytic activity is ascribed to the increasing visible light-absorbing capacity of transverse surface plasmon resonance (TSPR) of Au nanorods and improved charge separation of Au NRs/g-C3N4 heterostructure. Even more important, Au NRs/g-C3N4 heterostructures achieve NIR photocatalytic H2 evolution performance (63.1 μmol g−1 h−1), owing to the longitudinal SPR (LSPR) effect of Au nanorods induced NIR light harvesting ability. Photocatalytic H g-C Au nanorods Near-infrared Visible Liu, Xiang verfasserin aut Liang, Zhangqian verfasserin aut Qiu, Pengyuan verfasserin aut Qian, Xiu verfasserin aut Cui, Hongzhi verfasserin (orcid)0000-0002-2212-0295 aut Tian, Jian verfasserin aut Enthalten in Journal of colloid and interface science Amsterdam [u.a.] : Elsevier, 1966 557, Seite 700-708 Online-Ressource (DE-627)266891136 (DE-600)1469021-4 (DE-576)103373160 1095-7103 nnns volume:557 pages:700-708 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2411 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.18 Kolloidchemie Grenzflächenchemie AR 557 700-708 |
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Enthalten in Journal of colloid and interface science 557, Seite 700-708 volume:557 pages:700-708 |
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Photocatalytic H g-C Au nanorods Near-infrared Visible |
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Tian, Huiyu @@aut@@ Liu, Xiang @@aut@@ Liang, Zhangqian @@aut@@ Qiu, Pengyuan @@aut@@ Qian, Xiu @@aut@@ Cui, Hongzhi @@aut@@ Tian, Jian @@aut@@ |
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2019-01-01T00:00:00Z |
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Tian, Huiyu |
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Tian, Huiyu ddc 540 bkl 35.18 misc Photocatalytic H misc g-C misc Au nanorods misc Near-infrared misc Visible Gold nanorods/g-C |
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540 DE-600 35.18 bkl Gold nanorods/g-C Photocatalytic H g-C Au nanorods Near-infrared Visible |
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ddc 540 bkl 35.18 misc Photocatalytic H misc g-C misc Au nanorods misc Near-infrared misc Visible |
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ddc 540 bkl 35.18 misc Photocatalytic H misc g-C misc Au nanorods misc Near-infrared misc Visible |
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Tian, Huiyu Liu, Xiang Liang, Zhangqian Qiu, Pengyuan Qian, Xiu Cui, Hongzhi Tian, Jian |
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Recently, broad spectrum (visible and near-infrared (NIR)) light utilization has aroused widespread attention in the research of photocatalysis. While g-C3N4, highly stable, cheap and easily synthesized, shows H2 evolution activity under visible light irradiation, it doesn’t perform under NIR light irradiation. Here we report an Au nanorods (NRs)/g-C3N4 heterostructure with Au nanorods on g-C3N4’s surface. The most exciting feature of designed Au NRs/g-C3N4 heterostructures is that Au nanorods themselves are excited by visible and NIR light, which produce hot electrons and inject into g-C3N4. The photocatalytic H2 evolution rate of Au NRs/g-C3N4 heterostructures (350.6 μmol g−1 h−1) is nearly 4 times higher than that of g-C3N4 with Pt as cocatalyst (68.9 μmol g−1 h−1) under visible light illumination. The improved photocatalytic activity is ascribed to the increasing visible light-absorbing capacity of transverse surface plasmon resonance (TSPR) of Au nanorods and improved charge separation of Au NRs/g-C3N4 heterostructure. Even more important, Au NRs/g-C3N4 heterostructures achieve NIR photocatalytic H2 evolution performance (63.1 μmol g−1 h−1), owing to the longitudinal SPR (LSPR) effect of Au nanorods induced NIR light harvesting ability. |
| abstractGer |
Recently, broad spectrum (visible and near-infrared (NIR)) light utilization has aroused widespread attention in the research of photocatalysis. While g-C3N4, highly stable, cheap and easily synthesized, shows H2 evolution activity under visible light irradiation, it doesn’t perform under NIR light irradiation. Here we report an Au nanorods (NRs)/g-C3N4 heterostructure with Au nanorods on g-C3N4’s surface. The most exciting feature of designed Au NRs/g-C3N4 heterostructures is that Au nanorods themselves are excited by visible and NIR light, which produce hot electrons and inject into g-C3N4. The photocatalytic H2 evolution rate of Au NRs/g-C3N4 heterostructures (350.6 μmol g−1 h−1) is nearly 4 times higher than that of g-C3N4 with Pt as cocatalyst (68.9 μmol g−1 h−1) under visible light illumination. The improved photocatalytic activity is ascribed to the increasing visible light-absorbing capacity of transverse surface plasmon resonance (TSPR) of Au nanorods and improved charge separation of Au NRs/g-C3N4 heterostructure. Even more important, Au NRs/g-C3N4 heterostructures achieve NIR photocatalytic H2 evolution performance (63.1 μmol g−1 h−1), owing to the longitudinal SPR (LSPR) effect of Au nanorods induced NIR light harvesting ability. |
| abstract_unstemmed |
Recently, broad spectrum (visible and near-infrared (NIR)) light utilization has aroused widespread attention in the research of photocatalysis. While g-C3N4, highly stable, cheap and easily synthesized, shows H2 evolution activity under visible light irradiation, it doesn’t perform under NIR light irradiation. Here we report an Au nanorods (NRs)/g-C3N4 heterostructure with Au nanorods on g-C3N4’s surface. The most exciting feature of designed Au NRs/g-C3N4 heterostructures is that Au nanorods themselves are excited by visible and NIR light, which produce hot electrons and inject into g-C3N4. The photocatalytic H2 evolution rate of Au NRs/g-C3N4 heterostructures (350.6 μmol g−1 h−1) is nearly 4 times higher than that of g-C3N4 with Pt as cocatalyst (68.9 μmol g−1 h−1) under visible light illumination. The improved photocatalytic activity is ascribed to the increasing visible light-absorbing capacity of transverse surface plasmon resonance (TSPR) of Au nanorods and improved charge separation of Au NRs/g-C3N4 heterostructure. Even more important, Au NRs/g-C3N4 heterostructures achieve NIR photocatalytic H2 evolution performance (63.1 μmol g−1 h−1), owing to the longitudinal SPR (LSPR) effect of Au nanorods induced NIR light harvesting ability. |
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