Major and trace elements in suspended matter of western Siberian rivers: First assessment across permafrost zones and landscape parameters of watersheds
In contrast to good understanding of chemical composition of the river suspended matter (RSM) of large rivers, small rivers remain strongly understudied, despite the fact that they can provide valuable information on mechanisms of RSM generation and transport depending on key environmental parameter...
Ausführliche Beschreibung
Autor*in: |
Krickov, Ivan V. [verfasserIn] Lim, Artem G. [verfasserIn] Manasypov, Rinat M. [verfasserIn] Loiko, Sergey V. [verfasserIn] Vorobyev, Sergey N. [verfasserIn] Shevchenko, Vladimir P. [verfasserIn] Dara, Olga M. [verfasserIn] Gordeev, Vyacheslav V. [verfasserIn] Pokrovsky, Oleg S. [verfasserIn] |
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Format: |
E-Artikel |
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Sprache: |
Englisch |
Erschienen: |
2019 |
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Schlagwörter: |
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Übergeordnetes Werk: |
Enthalten in: Geochimica et cosmochimica acta - New York, NY [u.a.] : Elsevier, 1950, 269, Seite 429-450 |
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Übergeordnetes Werk: |
volume:269 ; pages:429-450 |
DOI / URN: |
10.1016/j.gca.2019.11.005 |
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Katalog-ID: |
ELV003292096 |
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245 | 1 | 0 | |a Major and trace elements in suspended matter of western Siberian rivers: First assessment across permafrost zones and landscape parameters of watersheds |
264 | 1 | |c 2019 | |
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520 | |a In contrast to good understanding of chemical composition of the river suspended matter (RSM) of large rivers, small rivers remain strongly understudied, despite the fact that they can provide valuable information on mechanisms of RSM generation and transport depending on key environmental parameters of the watershed. This is especially true for permafrost-affected boreal and subarctic territories, subjected to strong modification due to permafrost thaw and landscape changes under climate warming. We selected Earth’s largest frozen peatland zone, the western Siberia Lowland (WSL) in order to test an impact of climate warming, permafrost thaw and landscape zone changes on riverine transport of particulate material from mainland to the Arctic Ocean. We sampled 33 small and medium size WSL rivers during spring flood, summer baseflow and autumn flood over a 1700 km gradient of climate and permafrost. Major and trace elements in particulate (>0.45 µm) and dissolved (<0.45 µm) fraction were analyzed. We hypothesize that future increase in active layer thickness and the change of dominant landscape from bogs and lakes to forest can be predicted via analyzing the actual pattern of RSM chemical composition across various permafrost zones and landscape parameters of WSL river watershed. We observed a minimum concentration of Li, Mg, Na, K, Rb, V, Cr, Zn, Cu, Co, Ni, Al, Ga, Y, REEs, Nb, W, Ti, Zr, Hf, Th and U in RSM collected from isolated and sporadic permafrost zones. Considering all seasons together, the presence of forest in the permafrost-bearing zone increased particulate concentrations of all alkalis and alkaline-earth elements, B, As, Nb, Mn, Co, Al, Ga, REEs, Ti, Zr, Hf, Th. This is consistent with element mobilization from mineral horizons that become available for interacting with soil fluids under forested regions. Lakes retained particulate alkaline-earths, Fe, Mn, Co, trivalent and tetravalent hydrolysates (TE3+, TE4+). The concentration of lithogenic low-soluble elements (TE3+, TE4+) in the RSM strongly increased with the river size (watershed area). | ||
650 | 4 | |a Trace metals | |
650 | 4 | |a Toxicant | |
650 | 4 | |a Micronutrient | |
650 | 4 | |a Season | |
650 | 4 | |a River suspended matter | |
650 | 4 | |a Permafrost | |
650 | 4 | |a Siberia | |
700 | 1 | |a Lim, Artem G. |e verfasserin |4 aut | |
700 | 1 | |a Manasypov, Rinat M. |e verfasserin |4 aut | |
700 | 1 | |a Loiko, Sergey V. |e verfasserin |4 aut | |
700 | 1 | |a Vorobyev, Sergey N. |e verfasserin |4 aut | |
700 | 1 | |a Shevchenko, Vladimir P. |e verfasserin |4 aut | |
700 | 1 | |a Dara, Olga M. |e verfasserin |4 aut | |
700 | 1 | |a Gordeev, Vyacheslav V. |e verfasserin |4 aut | |
700 | 1 | |a Pokrovsky, Oleg S. |e verfasserin |4 aut | |
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10.1016/j.gca.2019.11.005 doi (DE-627)ELV003292096 (ELSEVIER)S0016-7037(19)30703-3 DE-627 ger DE-627 rda eng 550 DE-600 38.32 bkl 39.29 bkl Krickov, Ivan V. verfasserin aut Major and trace elements in suspended matter of western Siberian rivers: First assessment across permafrost zones and landscape parameters of watersheds 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier In contrast to good understanding of chemical composition of the river suspended matter (RSM) of large rivers, small rivers remain strongly understudied, despite the fact that they can provide valuable information on mechanisms of RSM generation and transport depending on key environmental parameters of the watershed. This is especially true for permafrost-affected boreal and subarctic territories, subjected to strong modification due to permafrost thaw and landscape changes under climate warming. We selected Earth’s largest frozen peatland zone, the western Siberia Lowland (WSL) in order to test an impact of climate warming, permafrost thaw and landscape zone changes on riverine transport of particulate material from mainland to the Arctic Ocean. We sampled 33 small and medium size WSL rivers during spring flood, summer baseflow and autumn flood over a 1700 km gradient of climate and permafrost. Major and trace elements in particulate (>0.45 µm) and dissolved (<0.45 µm) fraction were analyzed. We hypothesize that future increase in active layer thickness and the change of dominant landscape from bogs and lakes to forest can be predicted via analyzing the actual pattern of RSM chemical composition across various permafrost zones and landscape parameters of WSL river watershed. We observed a minimum concentration of Li, Mg, Na, K, Rb, V, Cr, Zn, Cu, Co, Ni, Al, Ga, Y, REEs, Nb, W, Ti, Zr, Hf, Th and U in RSM collected from isolated and sporadic permafrost zones. Considering all seasons together, the presence of forest in the permafrost-bearing zone increased particulate concentrations of all alkalis and alkaline-earth elements, B, As, Nb, Mn, Co, Al, Ga, REEs, Ti, Zr, Hf, Th. This is consistent with element mobilization from mineral horizons that become available for interacting with soil fluids under forested regions. Lakes retained particulate alkaline-earths, Fe, Mn, Co, trivalent and tetravalent hydrolysates (TE3+, TE4+). The concentration of lithogenic low-soluble elements (TE3+, TE4+) in the RSM strongly increased with the river size (watershed area). Trace metals Toxicant Micronutrient Season River suspended matter Permafrost Siberia Lim, Artem G. verfasserin aut Manasypov, Rinat M. verfasserin aut Loiko, Sergey V. verfasserin aut Vorobyev, Sergey N. verfasserin aut Shevchenko, Vladimir P. verfasserin aut Dara, Olga M. verfasserin aut Gordeev, Vyacheslav V. verfasserin aut Pokrovsky, Oleg S. verfasserin aut Enthalten in Geochimica et cosmochimica acta New York, NY [u.a.] : Elsevier, 1950 269, Seite 429-450 Online-Ressource (DE-627)300898797 (DE-600)1483679-8 (DE-576)120883465 0016-7037 nnns volume:269 pages:429-450 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OPC-GGO SSG-OPC-AST GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 38.32 Geochemie 39.29 Theoretische Astronomie: Sonstiges AR 269 429-450 |
spelling |
10.1016/j.gca.2019.11.005 doi (DE-627)ELV003292096 (ELSEVIER)S0016-7037(19)30703-3 DE-627 ger DE-627 rda eng 550 DE-600 38.32 bkl 39.29 bkl Krickov, Ivan V. verfasserin aut Major and trace elements in suspended matter of western Siberian rivers: First assessment across permafrost zones and landscape parameters of watersheds 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier In contrast to good understanding of chemical composition of the river suspended matter (RSM) of large rivers, small rivers remain strongly understudied, despite the fact that they can provide valuable information on mechanisms of RSM generation and transport depending on key environmental parameters of the watershed. This is especially true for permafrost-affected boreal and subarctic territories, subjected to strong modification due to permafrost thaw and landscape changes under climate warming. We selected Earth’s largest frozen peatland zone, the western Siberia Lowland (WSL) in order to test an impact of climate warming, permafrost thaw and landscape zone changes on riverine transport of particulate material from mainland to the Arctic Ocean. We sampled 33 small and medium size WSL rivers during spring flood, summer baseflow and autumn flood over a 1700 km gradient of climate and permafrost. Major and trace elements in particulate (>0.45 µm) and dissolved (<0.45 µm) fraction were analyzed. We hypothesize that future increase in active layer thickness and the change of dominant landscape from bogs and lakes to forest can be predicted via analyzing the actual pattern of RSM chemical composition across various permafrost zones and landscape parameters of WSL river watershed. We observed a minimum concentration of Li, Mg, Na, K, Rb, V, Cr, Zn, Cu, Co, Ni, Al, Ga, Y, REEs, Nb, W, Ti, Zr, Hf, Th and U in RSM collected from isolated and sporadic permafrost zones. Considering all seasons together, the presence of forest in the permafrost-bearing zone increased particulate concentrations of all alkalis and alkaline-earth elements, B, As, Nb, Mn, Co, Al, Ga, REEs, Ti, Zr, Hf, Th. This is consistent with element mobilization from mineral horizons that become available for interacting with soil fluids under forested regions. Lakes retained particulate alkaline-earths, Fe, Mn, Co, trivalent and tetravalent hydrolysates (TE3+, TE4+). The concentration of lithogenic low-soluble elements (TE3+, TE4+) in the RSM strongly increased with the river size (watershed area). Trace metals Toxicant Micronutrient Season River suspended matter Permafrost Siberia Lim, Artem G. verfasserin aut Manasypov, Rinat M. verfasserin aut Loiko, Sergey V. verfasserin aut Vorobyev, Sergey N. verfasserin aut Shevchenko, Vladimir P. verfasserin aut Dara, Olga M. verfasserin aut Gordeev, Vyacheslav V. verfasserin aut Pokrovsky, Oleg S. verfasserin aut Enthalten in Geochimica et cosmochimica acta New York, NY [u.a.] : Elsevier, 1950 269, Seite 429-450 Online-Ressource (DE-627)300898797 (DE-600)1483679-8 (DE-576)120883465 0016-7037 nnns volume:269 pages:429-450 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OPC-GGO SSG-OPC-AST GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 38.32 Geochemie 39.29 Theoretische Astronomie: Sonstiges AR 269 429-450 |
allfields_unstemmed |
10.1016/j.gca.2019.11.005 doi (DE-627)ELV003292096 (ELSEVIER)S0016-7037(19)30703-3 DE-627 ger DE-627 rda eng 550 DE-600 38.32 bkl 39.29 bkl Krickov, Ivan V. verfasserin aut Major and trace elements in suspended matter of western Siberian rivers: First assessment across permafrost zones and landscape parameters of watersheds 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier In contrast to good understanding of chemical composition of the river suspended matter (RSM) of large rivers, small rivers remain strongly understudied, despite the fact that they can provide valuable information on mechanisms of RSM generation and transport depending on key environmental parameters of the watershed. This is especially true for permafrost-affected boreal and subarctic territories, subjected to strong modification due to permafrost thaw and landscape changes under climate warming. We selected Earth’s largest frozen peatland zone, the western Siberia Lowland (WSL) in order to test an impact of climate warming, permafrost thaw and landscape zone changes on riverine transport of particulate material from mainland to the Arctic Ocean. We sampled 33 small and medium size WSL rivers during spring flood, summer baseflow and autumn flood over a 1700 km gradient of climate and permafrost. Major and trace elements in particulate (>0.45 µm) and dissolved (<0.45 µm) fraction were analyzed. We hypothesize that future increase in active layer thickness and the change of dominant landscape from bogs and lakes to forest can be predicted via analyzing the actual pattern of RSM chemical composition across various permafrost zones and landscape parameters of WSL river watershed. We observed a minimum concentration of Li, Mg, Na, K, Rb, V, Cr, Zn, Cu, Co, Ni, Al, Ga, Y, REEs, Nb, W, Ti, Zr, Hf, Th and U in RSM collected from isolated and sporadic permafrost zones. Considering all seasons together, the presence of forest in the permafrost-bearing zone increased particulate concentrations of all alkalis and alkaline-earth elements, B, As, Nb, Mn, Co, Al, Ga, REEs, Ti, Zr, Hf, Th. This is consistent with element mobilization from mineral horizons that become available for interacting with soil fluids under forested regions. Lakes retained particulate alkaline-earths, Fe, Mn, Co, trivalent and tetravalent hydrolysates (TE3+, TE4+). The concentration of lithogenic low-soluble elements (TE3+, TE4+) in the RSM strongly increased with the river size (watershed area). Trace metals Toxicant Micronutrient Season River suspended matter Permafrost Siberia Lim, Artem G. verfasserin aut Manasypov, Rinat M. verfasserin aut Loiko, Sergey V. verfasserin aut Vorobyev, Sergey N. verfasserin aut Shevchenko, Vladimir P. verfasserin aut Dara, Olga M. verfasserin aut Gordeev, Vyacheslav V. verfasserin aut Pokrovsky, Oleg S. verfasserin aut Enthalten in Geochimica et cosmochimica acta New York, NY [u.a.] : Elsevier, 1950 269, Seite 429-450 Online-Ressource (DE-627)300898797 (DE-600)1483679-8 (DE-576)120883465 0016-7037 nnns volume:269 pages:429-450 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OPC-GGO SSG-OPC-AST GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 38.32 Geochemie 39.29 Theoretische Astronomie: Sonstiges AR 269 429-450 |
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10.1016/j.gca.2019.11.005 doi (DE-627)ELV003292096 (ELSEVIER)S0016-7037(19)30703-3 DE-627 ger DE-627 rda eng 550 DE-600 38.32 bkl 39.29 bkl Krickov, Ivan V. verfasserin aut Major and trace elements in suspended matter of western Siberian rivers: First assessment across permafrost zones and landscape parameters of watersheds 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier In contrast to good understanding of chemical composition of the river suspended matter (RSM) of large rivers, small rivers remain strongly understudied, despite the fact that they can provide valuable information on mechanisms of RSM generation and transport depending on key environmental parameters of the watershed. This is especially true for permafrost-affected boreal and subarctic territories, subjected to strong modification due to permafrost thaw and landscape changes under climate warming. We selected Earth’s largest frozen peatland zone, the western Siberia Lowland (WSL) in order to test an impact of climate warming, permafrost thaw and landscape zone changes on riverine transport of particulate material from mainland to the Arctic Ocean. We sampled 33 small and medium size WSL rivers during spring flood, summer baseflow and autumn flood over a 1700 km gradient of climate and permafrost. Major and trace elements in particulate (>0.45 µm) and dissolved (<0.45 µm) fraction were analyzed. We hypothesize that future increase in active layer thickness and the change of dominant landscape from bogs and lakes to forest can be predicted via analyzing the actual pattern of RSM chemical composition across various permafrost zones and landscape parameters of WSL river watershed. We observed a minimum concentration of Li, Mg, Na, K, Rb, V, Cr, Zn, Cu, Co, Ni, Al, Ga, Y, REEs, Nb, W, Ti, Zr, Hf, Th and U in RSM collected from isolated and sporadic permafrost zones. Considering all seasons together, the presence of forest in the permafrost-bearing zone increased particulate concentrations of all alkalis and alkaline-earth elements, B, As, Nb, Mn, Co, Al, Ga, REEs, Ti, Zr, Hf, Th. This is consistent with element mobilization from mineral horizons that become available for interacting with soil fluids under forested regions. Lakes retained particulate alkaline-earths, Fe, Mn, Co, trivalent and tetravalent hydrolysates (TE3+, TE4+). The concentration of lithogenic low-soluble elements (TE3+, TE4+) in the RSM strongly increased with the river size (watershed area). Trace metals Toxicant Micronutrient Season River suspended matter Permafrost Siberia Lim, Artem G. verfasserin aut Manasypov, Rinat M. verfasserin aut Loiko, Sergey V. verfasserin aut Vorobyev, Sergey N. verfasserin aut Shevchenko, Vladimir P. verfasserin aut Dara, Olga M. verfasserin aut Gordeev, Vyacheslav V. verfasserin aut Pokrovsky, Oleg S. verfasserin aut Enthalten in Geochimica et cosmochimica acta New York, NY [u.a.] : Elsevier, 1950 269, Seite 429-450 Online-Ressource (DE-627)300898797 (DE-600)1483679-8 (DE-576)120883465 0016-7037 nnns volume:269 pages:429-450 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OPC-GGO SSG-OPC-AST GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 38.32 Geochemie 39.29 Theoretische Astronomie: Sonstiges AR 269 429-450 |
allfieldsSound |
10.1016/j.gca.2019.11.005 doi (DE-627)ELV003292096 (ELSEVIER)S0016-7037(19)30703-3 DE-627 ger DE-627 rda eng 550 DE-600 38.32 bkl 39.29 bkl Krickov, Ivan V. verfasserin aut Major and trace elements in suspended matter of western Siberian rivers: First assessment across permafrost zones and landscape parameters of watersheds 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier In contrast to good understanding of chemical composition of the river suspended matter (RSM) of large rivers, small rivers remain strongly understudied, despite the fact that they can provide valuable information on mechanisms of RSM generation and transport depending on key environmental parameters of the watershed. This is especially true for permafrost-affected boreal and subarctic territories, subjected to strong modification due to permafrost thaw and landscape changes under climate warming. We selected Earth’s largest frozen peatland zone, the western Siberia Lowland (WSL) in order to test an impact of climate warming, permafrost thaw and landscape zone changes on riverine transport of particulate material from mainland to the Arctic Ocean. We sampled 33 small and medium size WSL rivers during spring flood, summer baseflow and autumn flood over a 1700 km gradient of climate and permafrost. Major and trace elements in particulate (>0.45 µm) and dissolved (<0.45 µm) fraction were analyzed. We hypothesize that future increase in active layer thickness and the change of dominant landscape from bogs and lakes to forest can be predicted via analyzing the actual pattern of RSM chemical composition across various permafrost zones and landscape parameters of WSL river watershed. We observed a minimum concentration of Li, Mg, Na, K, Rb, V, Cr, Zn, Cu, Co, Ni, Al, Ga, Y, REEs, Nb, W, Ti, Zr, Hf, Th and U in RSM collected from isolated and sporadic permafrost zones. Considering all seasons together, the presence of forest in the permafrost-bearing zone increased particulate concentrations of all alkalis and alkaline-earth elements, B, As, Nb, Mn, Co, Al, Ga, REEs, Ti, Zr, Hf, Th. This is consistent with element mobilization from mineral horizons that become available for interacting with soil fluids under forested regions. Lakes retained particulate alkaline-earths, Fe, Mn, Co, trivalent and tetravalent hydrolysates (TE3+, TE4+). The concentration of lithogenic low-soluble elements (TE3+, TE4+) in the RSM strongly increased with the river size (watershed area). Trace metals Toxicant Micronutrient Season River suspended matter Permafrost Siberia Lim, Artem G. verfasserin aut Manasypov, Rinat M. verfasserin aut Loiko, Sergey V. verfasserin aut Vorobyev, Sergey N. verfasserin aut Shevchenko, Vladimir P. verfasserin aut Dara, Olga M. verfasserin aut Gordeev, Vyacheslav V. verfasserin aut Pokrovsky, Oleg S. verfasserin aut Enthalten in Geochimica et cosmochimica acta New York, NY [u.a.] : Elsevier, 1950 269, Seite 429-450 Online-Ressource (DE-627)300898797 (DE-600)1483679-8 (DE-576)120883465 0016-7037 nnns volume:269 pages:429-450 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OPC-GGO SSG-OPC-AST GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 38.32 Geochemie 39.29 Theoretische Astronomie: Sonstiges AR 269 429-450 |
language |
English |
source |
Enthalten in Geochimica et cosmochimica acta 269, Seite 429-450 volume:269 pages:429-450 |
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Enthalten in Geochimica et cosmochimica acta 269, Seite 429-450 volume:269 pages:429-450 |
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Trace metals Toxicant Micronutrient Season River suspended matter Permafrost Siberia |
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container_title |
Geochimica et cosmochimica acta |
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Krickov, Ivan V. @@aut@@ Lim, Artem G. @@aut@@ Manasypov, Rinat M. @@aut@@ Loiko, Sergey V. @@aut@@ Vorobyev, Sergey N. @@aut@@ Shevchenko, Vladimir P. @@aut@@ Dara, Olga M. @@aut@@ Gordeev, Vyacheslav V. @@aut@@ Pokrovsky, Oleg S. @@aut@@ |
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2019-01-01T00:00:00Z |
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Krickov, Ivan V. |
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Krickov, Ivan V. ddc 550 bkl 38.32 bkl 39.29 misc Trace metals misc Toxicant misc Micronutrient misc Season misc River suspended matter misc Permafrost misc Siberia Major and trace elements in suspended matter of western Siberian rivers: First assessment across permafrost zones and landscape parameters of watersheds |
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550 DE-600 38.32 bkl 39.29 bkl Major and trace elements in suspended matter of western Siberian rivers: First assessment across permafrost zones and landscape parameters of watersheds Trace metals Toxicant Micronutrient Season River suspended matter Permafrost Siberia |
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ddc 550 bkl 38.32 bkl 39.29 misc Trace metals misc Toxicant misc Micronutrient misc Season misc River suspended matter misc Permafrost misc Siberia |
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Major and trace elements in suspended matter of western Siberian rivers: First assessment across permafrost zones and landscape parameters of watersheds |
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Major and trace elements in suspended matter of western Siberian rivers: First assessment across permafrost zones and landscape parameters of watersheds |
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Geochimica et cosmochimica acta |
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Krickov, Ivan V. Lim, Artem G. Manasypov, Rinat M. Loiko, Sergey V. Vorobyev, Sergey N. Shevchenko, Vladimir P. Dara, Olga M. Gordeev, Vyacheslav V. Pokrovsky, Oleg S. |
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major and trace elements in suspended matter of western siberian rivers: first assessment across permafrost zones and landscape parameters of watersheds |
title_auth |
Major and trace elements in suspended matter of western Siberian rivers: First assessment across permafrost zones and landscape parameters of watersheds |
abstract |
In contrast to good understanding of chemical composition of the river suspended matter (RSM) of large rivers, small rivers remain strongly understudied, despite the fact that they can provide valuable information on mechanisms of RSM generation and transport depending on key environmental parameters of the watershed. This is especially true for permafrost-affected boreal and subarctic territories, subjected to strong modification due to permafrost thaw and landscape changes under climate warming. We selected Earth’s largest frozen peatland zone, the western Siberia Lowland (WSL) in order to test an impact of climate warming, permafrost thaw and landscape zone changes on riverine transport of particulate material from mainland to the Arctic Ocean. We sampled 33 small and medium size WSL rivers during spring flood, summer baseflow and autumn flood over a 1700 km gradient of climate and permafrost. Major and trace elements in particulate (>0.45 µm) and dissolved (<0.45 µm) fraction were analyzed. We hypothesize that future increase in active layer thickness and the change of dominant landscape from bogs and lakes to forest can be predicted via analyzing the actual pattern of RSM chemical composition across various permafrost zones and landscape parameters of WSL river watershed. We observed a minimum concentration of Li, Mg, Na, K, Rb, V, Cr, Zn, Cu, Co, Ni, Al, Ga, Y, REEs, Nb, W, Ti, Zr, Hf, Th and U in RSM collected from isolated and sporadic permafrost zones. Considering all seasons together, the presence of forest in the permafrost-bearing zone increased particulate concentrations of all alkalis and alkaline-earth elements, B, As, Nb, Mn, Co, Al, Ga, REEs, Ti, Zr, Hf, Th. This is consistent with element mobilization from mineral horizons that become available for interacting with soil fluids under forested regions. Lakes retained particulate alkaline-earths, Fe, Mn, Co, trivalent and tetravalent hydrolysates (TE3+, TE4+). The concentration of lithogenic low-soluble elements (TE3+, TE4+) in the RSM strongly increased with the river size (watershed area). |
abstractGer |
In contrast to good understanding of chemical composition of the river suspended matter (RSM) of large rivers, small rivers remain strongly understudied, despite the fact that they can provide valuable information on mechanisms of RSM generation and transport depending on key environmental parameters of the watershed. This is especially true for permafrost-affected boreal and subarctic territories, subjected to strong modification due to permafrost thaw and landscape changes under climate warming. We selected Earth’s largest frozen peatland zone, the western Siberia Lowland (WSL) in order to test an impact of climate warming, permafrost thaw and landscape zone changes on riverine transport of particulate material from mainland to the Arctic Ocean. We sampled 33 small and medium size WSL rivers during spring flood, summer baseflow and autumn flood over a 1700 km gradient of climate and permafrost. Major and trace elements in particulate (>0.45 µm) and dissolved (<0.45 µm) fraction were analyzed. We hypothesize that future increase in active layer thickness and the change of dominant landscape from bogs and lakes to forest can be predicted via analyzing the actual pattern of RSM chemical composition across various permafrost zones and landscape parameters of WSL river watershed. We observed a minimum concentration of Li, Mg, Na, K, Rb, V, Cr, Zn, Cu, Co, Ni, Al, Ga, Y, REEs, Nb, W, Ti, Zr, Hf, Th and U in RSM collected from isolated and sporadic permafrost zones. Considering all seasons together, the presence of forest in the permafrost-bearing zone increased particulate concentrations of all alkalis and alkaline-earth elements, B, As, Nb, Mn, Co, Al, Ga, REEs, Ti, Zr, Hf, Th. This is consistent with element mobilization from mineral horizons that become available for interacting with soil fluids under forested regions. Lakes retained particulate alkaline-earths, Fe, Mn, Co, trivalent and tetravalent hydrolysates (TE3+, TE4+). The concentration of lithogenic low-soluble elements (TE3+, TE4+) in the RSM strongly increased with the river size (watershed area). |
abstract_unstemmed |
In contrast to good understanding of chemical composition of the river suspended matter (RSM) of large rivers, small rivers remain strongly understudied, despite the fact that they can provide valuable information on mechanisms of RSM generation and transport depending on key environmental parameters of the watershed. This is especially true for permafrost-affected boreal and subarctic territories, subjected to strong modification due to permafrost thaw and landscape changes under climate warming. We selected Earth’s largest frozen peatland zone, the western Siberia Lowland (WSL) in order to test an impact of climate warming, permafrost thaw and landscape zone changes on riverine transport of particulate material from mainland to the Arctic Ocean. We sampled 33 small and medium size WSL rivers during spring flood, summer baseflow and autumn flood over a 1700 km gradient of climate and permafrost. Major and trace elements in particulate (>0.45 µm) and dissolved (<0.45 µm) fraction were analyzed. We hypothesize that future increase in active layer thickness and the change of dominant landscape from bogs and lakes to forest can be predicted via analyzing the actual pattern of RSM chemical composition across various permafrost zones and landscape parameters of WSL river watershed. We observed a minimum concentration of Li, Mg, Na, K, Rb, V, Cr, Zn, Cu, Co, Ni, Al, Ga, Y, REEs, Nb, W, Ti, Zr, Hf, Th and U in RSM collected from isolated and sporadic permafrost zones. Considering all seasons together, the presence of forest in the permafrost-bearing zone increased particulate concentrations of all alkalis and alkaline-earth elements, B, As, Nb, Mn, Co, Al, Ga, REEs, Ti, Zr, Hf, Th. This is consistent with element mobilization from mineral horizons that become available for interacting with soil fluids under forested regions. Lakes retained particulate alkaline-earths, Fe, Mn, Co, trivalent and tetravalent hydrolysates (TE3+, TE4+). The concentration of lithogenic low-soluble elements (TE3+, TE4+) in the RSM strongly increased with the river size (watershed area). |
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title_short |
Major and trace elements in suspended matter of western Siberian rivers: First assessment across permafrost zones and landscape parameters of watersheds |
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Lim, Artem G. Manasypov, Rinat M. Loiko, Sergey V. Vorobyev, Sergey N. Shevchenko, Vladimir P. Dara, Olga M. Gordeev, Vyacheslav V. Pokrovsky, Oleg S. |
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Lim, Artem G. Manasypov, Rinat M. Loiko, Sergey V. Vorobyev, Sergey N. Shevchenko, Vladimir P. Dara, Olga M. Gordeev, Vyacheslav V. Pokrovsky, Oleg S. |
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This is especially true for permafrost-affected boreal and subarctic territories, subjected to strong modification due to permafrost thaw and landscape changes under climate warming. We selected Earth’s largest frozen peatland zone, the western Siberia Lowland (WSL) in order to test an impact of climate warming, permafrost thaw and landscape zone changes on riverine transport of particulate material from mainland to the Arctic Ocean. We sampled 33 small and medium size WSL rivers during spring flood, summer baseflow and autumn flood over a 1700 km gradient of climate and permafrost. Major and trace elements in particulate (>0.45 µm) and dissolved (<0.45 µm) fraction were analyzed. We hypothesize that future increase in active layer thickness and the change of dominant landscape from bogs and lakes to forest can be predicted via analyzing the actual pattern of RSM chemical composition across various permafrost zones and landscape parameters of WSL river watershed. We observed a minimum concentration of Li, Mg, Na, K, Rb, V, Cr, Zn, Cu, Co, Ni, Al, Ga, Y, REEs, Nb, W, Ti, Zr, Hf, Th and U in RSM collected from isolated and sporadic permafrost zones. Considering all seasons together, the presence of forest in the permafrost-bearing zone increased particulate concentrations of all alkalis and alkaline-earth elements, B, As, Nb, Mn, Co, Al, Ga, REEs, Ti, Zr, Hf, Th. This is consistent with element mobilization from mineral horizons that become available for interacting with soil fluids under forested regions. Lakes retained particulate alkaline-earths, Fe, Mn, Co, trivalent and tetravalent hydrolysates (TE3+, TE4+). The concentration of lithogenic low-soluble elements (TE3+, TE4+) in the RSM strongly increased with the river size (watershed area).</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Trace metals</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Toxicant</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Micronutrient</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Season</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">River suspended matter</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Permafrost</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Siberia</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Lim, Artem G.</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Manasypov, Rinat M.</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Loiko, Sergey V.</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Vorobyev, Sergey N.</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Shevchenko, Vladimir P.</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Dara, Olga M.</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Gordeev, Vyacheslav V.</subfield><subfield code="e">verfasserin</subfield><subfield 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