Fabrication of highly active Z-scheme Ag/g-C
The capacity of redox and the separation efficiency of electron-hole pairs are important indexes for evaluating the performance of photocatalyst. Herein, a novel Z-scheme Ag/g-C3N4-Ag-Ag3PO4 (1 1 0) photocatalyst is prepared by photo-assisted isoelectric point way. The prepared samples are character...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Li, Siyi [verfasserIn] Zhang, Meng [verfasserIn] Qu, Zhihui [verfasserIn] Cui, Xin [verfasserIn] Liu, Zhiyu [verfasserIn] Piao, Congcong [verfasserIn] Li, Shuguang [verfasserIn] Wang, Jun [verfasserIn] Song, Youtao [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2019 |
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| Schlagwörter: |
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| Übergeordnetes Werk: |
Enthalten in: The chemical engineering journal - Amsterdam : Elsevier, 1997, 382 |
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| Übergeordnetes Werk: |
volume:382 |
| DOI / URN: |
10.1016/j.cej.2019.122394 |
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| Katalog-ID: |
ELV003302644 |
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| 245 | 1 | 0 | |a Fabrication of highly active Z-scheme Ag/g-C |
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| 520 | |a The capacity of redox and the separation efficiency of electron-hole pairs are important indexes for evaluating the performance of photocatalyst. Herein, a novel Z-scheme Ag/g-C3N4-Ag-Ag3PO4 (1 1 0) photocatalyst is prepared by photo-assisted isoelectric point way. The prepared samples are characterized by XRD, SEM, TEM, EDS mappings, XPS, UV–vis, PL, TPR and EIS. The Z-scheme Ag/g-C3N4-Ag-Ag3PO4 (1 1 0) photocatalytic system exposes the Ag3PO4 (1 1 0) crystal plane with strong oxidizing ability and provides a large producing hydrogen reduction surface of g-C3N4 at the same time. Therefore, the photocatalytic degradation of levofloxacin (LEV) with simultaneous hydrogen production can be effectively achieved under visible light irradiation. Besides, the influence factors such as visible light irradiation time, sacrificial agents, Z-scheme Ag/g-C3N4-Ag-Ag3PO4 (1 1 0) photocatalyst dosage, initial pH and used times are studied systemically. Based on trapping tests and ESR analyzes, the mainly active species are confirmed in the photocatalytic degradation of LEV. Finally, the photocatalytic reaction mechanism on degradation of organic pollutants with simultaneous production hydrogen caused by Z-scheme Ag/g-C3N4-Ag-Ag3PO4 (1 1 0) photocatalyst is proposed. | ||
| 650 | 4 | |a Z-scheme Ag/g-C | |
| 650 | 4 | |a Ag | |
| 650 | 4 | |a Photo-assisted isoelectric point method | |
| 650 | 4 | |a Degradation of LEV | |
| 650 | 4 | |a Simultaneous hydrogen production | |
| 700 | 1 | |a Zhang, Meng |e verfasserin |4 aut | |
| 700 | 1 | |a Qu, Zhihui |e verfasserin |4 aut | |
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| 700 | 1 | |a Li, Shuguang |e verfasserin |4 aut | |
| 700 | 1 | |a Wang, Jun |e verfasserin |0 (orcid)0000-0002-3465-784X |4 aut | |
| 700 | 1 | |a Song, Youtao |e verfasserin |4 aut | |
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10.1016/j.cej.2019.122394 doi (DE-627)ELV003302644 (ELSEVIER)S1385-8947(19)31797-8 DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Li, Siyi verfasserin aut Fabrication of highly active Z-scheme Ag/g-C 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The capacity of redox and the separation efficiency of electron-hole pairs are important indexes for evaluating the performance of photocatalyst. Herein, a novel Z-scheme Ag/g-C3N4-Ag-Ag3PO4 (1 1 0) photocatalyst is prepared by photo-assisted isoelectric point way. The prepared samples are characterized by XRD, SEM, TEM, EDS mappings, XPS, UV–vis, PL, TPR and EIS. The Z-scheme Ag/g-C3N4-Ag-Ag3PO4 (1 1 0) photocatalytic system exposes the Ag3PO4 (1 1 0) crystal plane with strong oxidizing ability and provides a large producing hydrogen reduction surface of g-C3N4 at the same time. Therefore, the photocatalytic degradation of levofloxacin (LEV) with simultaneous hydrogen production can be effectively achieved under visible light irradiation. Besides, the influence factors such as visible light irradiation time, sacrificial agents, Z-scheme Ag/g-C3N4-Ag-Ag3PO4 (1 1 0) photocatalyst dosage, initial pH and used times are studied systemically. Based on trapping tests and ESR analyzes, the mainly active species are confirmed in the photocatalytic degradation of LEV. Finally, the photocatalytic reaction mechanism on degradation of organic pollutants with simultaneous production hydrogen caused by Z-scheme Ag/g-C3N4-Ag-Ag3PO4 (1 1 0) photocatalyst is proposed. Z-scheme Ag/g-C Ag Photo-assisted isoelectric point method Degradation of LEV Simultaneous hydrogen production Zhang, Meng verfasserin aut Qu, Zhihui verfasserin aut Cui, Xin verfasserin aut Liu, Zhiyu verfasserin aut Piao, Congcong verfasserin aut Li, Shuguang verfasserin aut Wang, Jun verfasserin (orcid)0000-0002-3465-784X aut Song, Youtao verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 382 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:382 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 382 045F 660.05 |
| spelling |
10.1016/j.cej.2019.122394 doi (DE-627)ELV003302644 (ELSEVIER)S1385-8947(19)31797-8 DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Li, Siyi verfasserin aut Fabrication of highly active Z-scheme Ag/g-C 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The capacity of redox and the separation efficiency of electron-hole pairs are important indexes for evaluating the performance of photocatalyst. Herein, a novel Z-scheme Ag/g-C3N4-Ag-Ag3PO4 (1 1 0) photocatalyst is prepared by photo-assisted isoelectric point way. The prepared samples are characterized by XRD, SEM, TEM, EDS mappings, XPS, UV–vis, PL, TPR and EIS. The Z-scheme Ag/g-C3N4-Ag-Ag3PO4 (1 1 0) photocatalytic system exposes the Ag3PO4 (1 1 0) crystal plane with strong oxidizing ability and provides a large producing hydrogen reduction surface of g-C3N4 at the same time. Therefore, the photocatalytic degradation of levofloxacin (LEV) with simultaneous hydrogen production can be effectively achieved under visible light irradiation. Besides, the influence factors such as visible light irradiation time, sacrificial agents, Z-scheme Ag/g-C3N4-Ag-Ag3PO4 (1 1 0) photocatalyst dosage, initial pH and used times are studied systemically. Based on trapping tests and ESR analyzes, the mainly active species are confirmed in the photocatalytic degradation of LEV. Finally, the photocatalytic reaction mechanism on degradation of organic pollutants with simultaneous production hydrogen caused by Z-scheme Ag/g-C3N4-Ag-Ag3PO4 (1 1 0) photocatalyst is proposed. Z-scheme Ag/g-C Ag Photo-assisted isoelectric point method Degradation of LEV Simultaneous hydrogen production Zhang, Meng verfasserin aut Qu, Zhihui verfasserin aut Cui, Xin verfasserin aut Liu, Zhiyu verfasserin aut Piao, Congcong verfasserin aut Li, Shuguang verfasserin aut Wang, Jun verfasserin (orcid)0000-0002-3465-784X aut Song, Youtao verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 382 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:382 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 382 045F 660.05 |
| allfields_unstemmed |
10.1016/j.cej.2019.122394 doi (DE-627)ELV003302644 (ELSEVIER)S1385-8947(19)31797-8 DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Li, Siyi verfasserin aut Fabrication of highly active Z-scheme Ag/g-C 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The capacity of redox and the separation efficiency of electron-hole pairs are important indexes for evaluating the performance of photocatalyst. Herein, a novel Z-scheme Ag/g-C3N4-Ag-Ag3PO4 (1 1 0) photocatalyst is prepared by photo-assisted isoelectric point way. The prepared samples are characterized by XRD, SEM, TEM, EDS mappings, XPS, UV–vis, PL, TPR and EIS. The Z-scheme Ag/g-C3N4-Ag-Ag3PO4 (1 1 0) photocatalytic system exposes the Ag3PO4 (1 1 0) crystal plane with strong oxidizing ability and provides a large producing hydrogen reduction surface of g-C3N4 at the same time. Therefore, the photocatalytic degradation of levofloxacin (LEV) with simultaneous hydrogen production can be effectively achieved under visible light irradiation. Besides, the influence factors such as visible light irradiation time, sacrificial agents, Z-scheme Ag/g-C3N4-Ag-Ag3PO4 (1 1 0) photocatalyst dosage, initial pH and used times are studied systemically. Based on trapping tests and ESR analyzes, the mainly active species are confirmed in the photocatalytic degradation of LEV. Finally, the photocatalytic reaction mechanism on degradation of organic pollutants with simultaneous production hydrogen caused by Z-scheme Ag/g-C3N4-Ag-Ag3PO4 (1 1 0) photocatalyst is proposed. Z-scheme Ag/g-C Ag Photo-assisted isoelectric point method Degradation of LEV Simultaneous hydrogen production Zhang, Meng verfasserin aut Qu, Zhihui verfasserin aut Cui, Xin verfasserin aut Liu, Zhiyu verfasserin aut Piao, Congcong verfasserin aut Li, Shuguang verfasserin aut Wang, Jun verfasserin (orcid)0000-0002-3465-784X aut Song, Youtao verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 382 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:382 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 382 045F 660.05 |
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10.1016/j.cej.2019.122394 doi (DE-627)ELV003302644 (ELSEVIER)S1385-8947(19)31797-8 DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Li, Siyi verfasserin aut Fabrication of highly active Z-scheme Ag/g-C 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The capacity of redox and the separation efficiency of electron-hole pairs are important indexes for evaluating the performance of photocatalyst. Herein, a novel Z-scheme Ag/g-C3N4-Ag-Ag3PO4 (1 1 0) photocatalyst is prepared by photo-assisted isoelectric point way. The prepared samples are characterized by XRD, SEM, TEM, EDS mappings, XPS, UV–vis, PL, TPR and EIS. The Z-scheme Ag/g-C3N4-Ag-Ag3PO4 (1 1 0) photocatalytic system exposes the Ag3PO4 (1 1 0) crystal plane with strong oxidizing ability and provides a large producing hydrogen reduction surface of g-C3N4 at the same time. Therefore, the photocatalytic degradation of levofloxacin (LEV) with simultaneous hydrogen production can be effectively achieved under visible light irradiation. Besides, the influence factors such as visible light irradiation time, sacrificial agents, Z-scheme Ag/g-C3N4-Ag-Ag3PO4 (1 1 0) photocatalyst dosage, initial pH and used times are studied systemically. Based on trapping tests and ESR analyzes, the mainly active species are confirmed in the photocatalytic degradation of LEV. Finally, the photocatalytic reaction mechanism on degradation of organic pollutants with simultaneous production hydrogen caused by Z-scheme Ag/g-C3N4-Ag-Ag3PO4 (1 1 0) photocatalyst is proposed. Z-scheme Ag/g-C Ag Photo-assisted isoelectric point method Degradation of LEV Simultaneous hydrogen production Zhang, Meng verfasserin aut Qu, Zhihui verfasserin aut Cui, Xin verfasserin aut Liu, Zhiyu verfasserin aut Piao, Congcong verfasserin aut Li, Shuguang verfasserin aut Wang, Jun verfasserin (orcid)0000-0002-3465-784X aut Song, Youtao verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 382 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:382 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 382 045F 660.05 |
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10.1016/j.cej.2019.122394 doi (DE-627)ELV003302644 (ELSEVIER)S1385-8947(19)31797-8 DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Li, Siyi verfasserin aut Fabrication of highly active Z-scheme Ag/g-C 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The capacity of redox and the separation efficiency of electron-hole pairs are important indexes for evaluating the performance of photocatalyst. Herein, a novel Z-scheme Ag/g-C3N4-Ag-Ag3PO4 (1 1 0) photocatalyst is prepared by photo-assisted isoelectric point way. The prepared samples are characterized by XRD, SEM, TEM, EDS mappings, XPS, UV–vis, PL, TPR and EIS. The Z-scheme Ag/g-C3N4-Ag-Ag3PO4 (1 1 0) photocatalytic system exposes the Ag3PO4 (1 1 0) crystal plane with strong oxidizing ability and provides a large producing hydrogen reduction surface of g-C3N4 at the same time. Therefore, the photocatalytic degradation of levofloxacin (LEV) with simultaneous hydrogen production can be effectively achieved under visible light irradiation. Besides, the influence factors such as visible light irradiation time, sacrificial agents, Z-scheme Ag/g-C3N4-Ag-Ag3PO4 (1 1 0) photocatalyst dosage, initial pH and used times are studied systemically. Based on trapping tests and ESR analyzes, the mainly active species are confirmed in the photocatalytic degradation of LEV. Finally, the photocatalytic reaction mechanism on degradation of organic pollutants with simultaneous production hydrogen caused by Z-scheme Ag/g-C3N4-Ag-Ag3PO4 (1 1 0) photocatalyst is proposed. Z-scheme Ag/g-C Ag Photo-assisted isoelectric point method Degradation of LEV Simultaneous hydrogen production Zhang, Meng verfasserin aut Qu, Zhihui verfasserin aut Cui, Xin verfasserin aut Liu, Zhiyu verfasserin aut Piao, Congcong verfasserin aut Li, Shuguang verfasserin aut Wang, Jun verfasserin (orcid)0000-0002-3465-784X aut Song, Youtao verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 382 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:382 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 382 045F 660.05 |
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Li, Siyi @@aut@@ Zhang, Meng @@aut@@ Qu, Zhihui @@aut@@ Cui, Xin @@aut@@ Liu, Zhiyu @@aut@@ Piao, Congcong @@aut@@ Li, Shuguang @@aut@@ Wang, Jun @@aut@@ Song, Youtao @@aut@@ |
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Li, Siyi |
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660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Fabrication of highly active Z-scheme Ag/g-C Z-scheme Ag/g-C Ag Photo-assisted isoelectric point method Degradation of LEV Simultaneous hydrogen production |
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ddc 660.05 ddc 660 bkl 58.10 misc Z-scheme Ag/g-C misc Ag misc Photo-assisted isoelectric point method misc Degradation of LEV misc Simultaneous hydrogen production |
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ddc 660.05 ddc 660 bkl 58.10 misc Z-scheme Ag/g-C misc Ag misc Photo-assisted isoelectric point method misc Degradation of LEV misc Simultaneous hydrogen production |
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Fabrication of highly active Z-scheme Ag/g-C |
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Li, Siyi Zhang, Meng Qu, Zhihui Cui, Xin Liu, Zhiyu Piao, Congcong Li, Shuguang Wang, Jun Song, Youtao |
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fabrication of highly active z-scheme ag/g-c |
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Fabrication of highly active Z-scheme Ag/g-C |
| abstract |
The capacity of redox and the separation efficiency of electron-hole pairs are important indexes for evaluating the performance of photocatalyst. Herein, a novel Z-scheme Ag/g-C3N4-Ag-Ag3PO4 (1 1 0) photocatalyst is prepared by photo-assisted isoelectric point way. The prepared samples are characterized by XRD, SEM, TEM, EDS mappings, XPS, UV–vis, PL, TPR and EIS. The Z-scheme Ag/g-C3N4-Ag-Ag3PO4 (1 1 0) photocatalytic system exposes the Ag3PO4 (1 1 0) crystal plane with strong oxidizing ability and provides a large producing hydrogen reduction surface of g-C3N4 at the same time. Therefore, the photocatalytic degradation of levofloxacin (LEV) with simultaneous hydrogen production can be effectively achieved under visible light irradiation. Besides, the influence factors such as visible light irradiation time, sacrificial agents, Z-scheme Ag/g-C3N4-Ag-Ag3PO4 (1 1 0) photocatalyst dosage, initial pH and used times are studied systemically. Based on trapping tests and ESR analyzes, the mainly active species are confirmed in the photocatalytic degradation of LEV. Finally, the photocatalytic reaction mechanism on degradation of organic pollutants with simultaneous production hydrogen caused by Z-scheme Ag/g-C3N4-Ag-Ag3PO4 (1 1 0) photocatalyst is proposed. |
| abstractGer |
The capacity of redox and the separation efficiency of electron-hole pairs are important indexes for evaluating the performance of photocatalyst. Herein, a novel Z-scheme Ag/g-C3N4-Ag-Ag3PO4 (1 1 0) photocatalyst is prepared by photo-assisted isoelectric point way. The prepared samples are characterized by XRD, SEM, TEM, EDS mappings, XPS, UV–vis, PL, TPR and EIS. The Z-scheme Ag/g-C3N4-Ag-Ag3PO4 (1 1 0) photocatalytic system exposes the Ag3PO4 (1 1 0) crystal plane with strong oxidizing ability and provides a large producing hydrogen reduction surface of g-C3N4 at the same time. Therefore, the photocatalytic degradation of levofloxacin (LEV) with simultaneous hydrogen production can be effectively achieved under visible light irradiation. Besides, the influence factors such as visible light irradiation time, sacrificial agents, Z-scheme Ag/g-C3N4-Ag-Ag3PO4 (1 1 0) photocatalyst dosage, initial pH and used times are studied systemically. Based on trapping tests and ESR analyzes, the mainly active species are confirmed in the photocatalytic degradation of LEV. Finally, the photocatalytic reaction mechanism on degradation of organic pollutants with simultaneous production hydrogen caused by Z-scheme Ag/g-C3N4-Ag-Ag3PO4 (1 1 0) photocatalyst is proposed. |
| abstract_unstemmed |
The capacity of redox and the separation efficiency of electron-hole pairs are important indexes for evaluating the performance of photocatalyst. Herein, a novel Z-scheme Ag/g-C3N4-Ag-Ag3PO4 (1 1 0) photocatalyst is prepared by photo-assisted isoelectric point way. The prepared samples are characterized by XRD, SEM, TEM, EDS mappings, XPS, UV–vis, PL, TPR and EIS. The Z-scheme Ag/g-C3N4-Ag-Ag3PO4 (1 1 0) photocatalytic system exposes the Ag3PO4 (1 1 0) crystal plane with strong oxidizing ability and provides a large producing hydrogen reduction surface of g-C3N4 at the same time. Therefore, the photocatalytic degradation of levofloxacin (LEV) with simultaneous hydrogen production can be effectively achieved under visible light irradiation. Besides, the influence factors such as visible light irradiation time, sacrificial agents, Z-scheme Ag/g-C3N4-Ag-Ag3PO4 (1 1 0) photocatalyst dosage, initial pH and used times are studied systemically. Based on trapping tests and ESR analyzes, the mainly active species are confirmed in the photocatalytic degradation of LEV. Finally, the photocatalytic reaction mechanism on degradation of organic pollutants with simultaneous production hydrogen caused by Z-scheme Ag/g-C3N4-Ag-Ag3PO4 (1 1 0) photocatalyst is proposed. |
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Fabrication of highly active Z-scheme Ag/g-C |
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| score |
7.401634 |