MoS

Molybdenum disulfide (MoS2) nanosheet is an appealing material due to its various merits such as narrow bandgap, high photothermal conversion speed, and intrinsic sulfur-rich properties. Building up a MoS2-based smart material with all the merits combined has become a challenging topic. Herein, usin...
Ausführliche Beschreibung

Gespeichert in:

Autor*in:	Wei, Gumi [verfasserIn] Wei, Junjie [verfasserIn] Zhou, Jie [verfasserIn] Chen, Yonggui [verfasserIn] Wu, Dongbei [verfasserIn] Wang, Qigang [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2019

Schlagwörter:	Molybdenum disulfide Self-initiated hydrogel Ag Light-response Quick desorption Cyclic regeneration

Übergeordnetes Werk:	Enthalten in: The chemical engineering journal - Amsterdam : Elsevier, 1997, 382
Übergeordnetes Werk:	volume:382

DOI / URN:	10.1016/j.cej.2019.123018

Katalog-ID:	ELV00330339X

Internformat


LEADER	01000caa a22002652 4500
001	ELV00330339X
003	DE-627
005	20230524131647.0
007	cr uuu---uuuuu
008	230430s2019 xx \|\|\|\|\|o 00\| \|\|eng c
024	7		\|a 10.1016/j.cej.2019.123018 \|2 doi
035			\|a (DE-627)ELV00330339X
035			\|a (ELSEVIER)S1385-8947(19)32428-3
040			\|a DE-627 \|b ger \|c DE-627 \|e rda
041			\|a eng
082	0		\|a 660.05 \|q DE-101
082	0	4	\|a 660 \|q DE-101
082	0	4	\|a 660 \|q DE-600
084			\|a 58.10 \|2 bkl
100	1		\|a Wei, Gumi \|e verfasserin \|4 aut
245	1	0	\|a MoS
264		1	\|c 2019
336			\|a nicht spezifiziert \|b zzz \|2 rdacontent
337			\|a Computermedien \|b c \|2 rdamedia
338			\|a Online-Ressource \|b cr \|2 rdacarrier
520			\|a Molybdenum disulfide (MoS2) nanosheet is an appealing material due to its various merits such as narrow bandgap, high photothermal conversion speed, and intrinsic sulfur-rich properties. Building up a MoS2-based smart material with all the merits combined has become a challenging topic. Herein, using the monomer N-isopropylacrylamide (NIPAM), a MoS2 self-initiated hydrogel adsorbents was fabricated by manipulation of MoS2 nanosheets as a photoinitiator response to UV light. The hydrogel adsorbent presents a high selectivity to Ag+, and can be quickly recycled upon the photothermal effect induced by 808 nm near-infrared laser irradiation. The adsorption-desorption cycle can be repeated for at least 6 times without obvious decrease of the Ag+ adsorption capacity. The entropy change associated with the desorption process is −16.7 J·K−1·mol−1, which confirms a spontaneous NIR-induced Ag+ desorption. Our MoS2-based smart hydrogel proves to be energy-efficient, quick-regenerated material for Ag+ enrichment.
650		4	\|a Molybdenum disulfide
650		4	\|a Self-initiated hydrogel
650		4	\|a Ag
650		4	\|a Light-response
650		4	\|a Quick desorption
650		4	\|a Cyclic regeneration
700	1		\|a Wei, Junjie \|e verfasserin \|4 aut
700	1		\|a Zhou, Jie \|e verfasserin \|4 aut
700	1		\|a Chen, Yonggui \|e verfasserin \|0 (orcid)0000-0002-0078-2204 \|4 aut
700	1		\|a Wu, Dongbei \|e verfasserin \|4 aut
700	1		\|a Wang, Qigang \|e verfasserin \|0 (orcid)0000-0002-6571-2549 \|4 aut
773	0	8	\|i Enthalten in \|t The chemical engineering journal \|d Amsterdam : Elsevier, 1997 \|g 382 \|h Online-Ressource \|w (DE-627)320500322 \|w (DE-600)2012137-4 \|w (DE-576)098330152 \|x 1873-3212 \|7 nnns
773	1	8	\|g volume:382
912			\|a GBV_USEFLAG_U
912			\|a SYSFLAG_U
912			\|a GBV_ELV
912			\|a SSG-OLC-PHA
912			\|a GBV_ILN_20
912			\|a GBV_ILN_22
912			\|a GBV_ILN_23
912			\|a GBV_ILN_24
912			\|a GBV_ILN_31
912			\|a GBV_ILN_32
912			\|a GBV_ILN_40
912			\|a GBV_ILN_60
912			\|a GBV_ILN_62
912			\|a GBV_ILN_63
912			\|a GBV_ILN_65
912			\|a GBV_ILN_69
912			\|a GBV_ILN_70
912			\|a GBV_ILN_73
912			\|a GBV_ILN_74
912			\|a GBV_ILN_90
912			\|a GBV_ILN_95
912			\|a GBV_ILN_100
912			\|a GBV_ILN_105
912			\|a GBV_ILN_110
912			\|a GBV_ILN_150
912			\|a GBV_ILN_151
912			\|a GBV_ILN_224
912			\|a GBV_ILN_370
912			\|a GBV_ILN_602
912			\|a GBV_ILN_702
912			\|a GBV_ILN_2003
912			\|a GBV_ILN_2004
912			\|a GBV_ILN_2005
912			\|a GBV_ILN_2011
912			\|a GBV_ILN_2014
912			\|a GBV_ILN_2015
912			\|a GBV_ILN_2020
912			\|a GBV_ILN_2021
912			\|a GBV_ILN_2025
912			\|a GBV_ILN_2027
912			\|a GBV_ILN_2034
912			\|a GBV_ILN_2038
912			\|a GBV_ILN_2044
912			\|a GBV_ILN_2048
912			\|a GBV_ILN_2049
912			\|a GBV_ILN_2050
912			\|a GBV_ILN_2056
912			\|a GBV_ILN_2059
912			\|a GBV_ILN_2061
912			\|a GBV_ILN_2064
912			\|a GBV_ILN_2065
912			\|a GBV_ILN_2068
912			\|a GBV_ILN_2111
912			\|a GBV_ILN_2112
912			\|a GBV_ILN_2113
912			\|a GBV_ILN_2118
912			\|a GBV_ILN_2122
912			\|a GBV_ILN_2129
912			\|a GBV_ILN_2143
912			\|a GBV_ILN_2147
912			\|a GBV_ILN_2148
912			\|a GBV_ILN_2152
912			\|a GBV_ILN_2153
912			\|a GBV_ILN_2190
912			\|a GBV_ILN_2336
912			\|a GBV_ILN_2507
912			\|a GBV_ILN_2522
912			\|a GBV_ILN_4035
912			\|a GBV_ILN_4037
912			\|a GBV_ILN_4112
912			\|a GBV_ILN_4125
912			\|a GBV_ILN_4126
912			\|a GBV_ILN_4242
912			\|a GBV_ILN_4251
912			\|a GBV_ILN_4305
912			\|a GBV_ILN_4313
912			\|a GBV_ILN_4323
912			\|a GBV_ILN_4324
912			\|a GBV_ILN_4325
912			\|a GBV_ILN_4326
912			\|a GBV_ILN_4333
912			\|a GBV_ILN_4334
912			\|a GBV_ILN_4335
912			\|a GBV_ILN_4338
912			\|a GBV_ILN_4393
936	b	k	\|a 58.10 \|j Verfahrenstechnik: Allgemeines
951			\|a AR
952			\|d 382
953			\|2 045F \|a 660.05

Indexfelder

author_variant	g w gw j w jw j z jz y c yc d w dw q w qw
matchkey_str	article:18733212:2019----::
hierarchy_sort_str	2019
bklnumber	58.10
publishDate	2019
allfields	10.1016/j.cej.2019.123018 doi (DE-627)ELV00330339X (ELSEVIER)S1385-8947(19)32428-3 DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Wei, Gumi verfasserin aut MoS 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Molybdenum disulfide (MoS2) nanosheet is an appealing material due to its various merits such as narrow bandgap, high photothermal conversion speed, and intrinsic sulfur-rich properties. Building up a MoS2-based smart material with all the merits combined has become a challenging topic. Herein, using the monomer N-isopropylacrylamide (NIPAM), a MoS2 self-initiated hydrogel adsorbents was fabricated by manipulation of MoS2 nanosheets as a photoinitiator response to UV light. The hydrogel adsorbent presents a high selectivity to Ag+, and can be quickly recycled upon the photothermal effect induced by 808 nm near-infrared laser irradiation. The adsorption-desorption cycle can be repeated for at least 6 times without obvious decrease of the Ag+ adsorption capacity. The entropy change associated with the desorption process is −16.7 J·K−1·mol−1, which confirms a spontaneous NIR-induced Ag+ desorption. Our MoS2-based smart hydrogel proves to be energy-efficient, quick-regenerated material for Ag+ enrichment. Molybdenum disulfide Self-initiated hydrogel Ag Light-response Quick desorption Cyclic regeneration Wei, Junjie verfasserin aut Zhou, Jie verfasserin aut Chen, Yonggui verfasserin (orcid)0000-0002-0078-2204 aut Wu, Dongbei verfasserin aut Wang, Qigang verfasserin (orcid)0000-0002-6571-2549 aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 382 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:382 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 382 045F 660.05
spelling	10.1016/j.cej.2019.123018 doi (DE-627)ELV00330339X (ELSEVIER)S1385-8947(19)32428-3 DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Wei, Gumi verfasserin aut MoS 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Molybdenum disulfide (MoS2) nanosheet is an appealing material due to its various merits such as narrow bandgap, high photothermal conversion speed, and intrinsic sulfur-rich properties. Building up a MoS2-based smart material with all the merits combined has become a challenging topic. Herein, using the monomer N-isopropylacrylamide (NIPAM), a MoS2 self-initiated hydrogel adsorbents was fabricated by manipulation of MoS2 nanosheets as a photoinitiator response to UV light. The hydrogel adsorbent presents a high selectivity to Ag+, and can be quickly recycled upon the photothermal effect induced by 808 nm near-infrared laser irradiation. The adsorption-desorption cycle can be repeated for at least 6 times without obvious decrease of the Ag+ adsorption capacity. The entropy change associated with the desorption process is −16.7 J·K−1·mol−1, which confirms a spontaneous NIR-induced Ag+ desorption. Our MoS2-based smart hydrogel proves to be energy-efficient, quick-regenerated material for Ag+ enrichment. Molybdenum disulfide Self-initiated hydrogel Ag Light-response Quick desorption Cyclic regeneration Wei, Junjie verfasserin aut Zhou, Jie verfasserin aut Chen, Yonggui verfasserin (orcid)0000-0002-0078-2204 aut Wu, Dongbei verfasserin aut Wang, Qigang verfasserin (orcid)0000-0002-6571-2549 aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 382 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:382 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 382 045F 660.05
allfields_unstemmed	10.1016/j.cej.2019.123018 doi (DE-627)ELV00330339X (ELSEVIER)S1385-8947(19)32428-3 DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Wei, Gumi verfasserin aut MoS 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Molybdenum disulfide (MoS2) nanosheet is an appealing material due to its various merits such as narrow bandgap, high photothermal conversion speed, and intrinsic sulfur-rich properties. Building up a MoS2-based smart material with all the merits combined has become a challenging topic. Herein, using the monomer N-isopropylacrylamide (NIPAM), a MoS2 self-initiated hydrogel adsorbents was fabricated by manipulation of MoS2 nanosheets as a photoinitiator response to UV light. The hydrogel adsorbent presents a high selectivity to Ag+, and can be quickly recycled upon the photothermal effect induced by 808 nm near-infrared laser irradiation. The adsorption-desorption cycle can be repeated for at least 6 times without obvious decrease of the Ag+ adsorption capacity. The entropy change associated with the desorption process is −16.7 J·K−1·mol−1, which confirms a spontaneous NIR-induced Ag+ desorption. Our MoS2-based smart hydrogel proves to be energy-efficient, quick-regenerated material for Ag+ enrichment. Molybdenum disulfide Self-initiated hydrogel Ag Light-response Quick desorption Cyclic regeneration Wei, Junjie verfasserin aut Zhou, Jie verfasserin aut Chen, Yonggui verfasserin (orcid)0000-0002-0078-2204 aut Wu, Dongbei verfasserin aut Wang, Qigang verfasserin (orcid)0000-0002-6571-2549 aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 382 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:382 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 382 045F 660.05
allfieldsGer	10.1016/j.cej.2019.123018 doi (DE-627)ELV00330339X (ELSEVIER)S1385-8947(19)32428-3 DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Wei, Gumi verfasserin aut MoS 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Molybdenum disulfide (MoS2) nanosheet is an appealing material due to its various merits such as narrow bandgap, high photothermal conversion speed, and intrinsic sulfur-rich properties. Building up a MoS2-based smart material with all the merits combined has become a challenging topic. Herein, using the monomer N-isopropylacrylamide (NIPAM), a MoS2 self-initiated hydrogel adsorbents was fabricated by manipulation of MoS2 nanosheets as a photoinitiator response to UV light. The hydrogel adsorbent presents a high selectivity to Ag+, and can be quickly recycled upon the photothermal effect induced by 808 nm near-infrared laser irradiation. The adsorption-desorption cycle can be repeated for at least 6 times without obvious decrease of the Ag+ adsorption capacity. The entropy change associated with the desorption process is −16.7 J·K−1·mol−1, which confirms a spontaneous NIR-induced Ag+ desorption. Our MoS2-based smart hydrogel proves to be energy-efficient, quick-regenerated material for Ag+ enrichment. Molybdenum disulfide Self-initiated hydrogel Ag Light-response Quick desorption Cyclic regeneration Wei, Junjie verfasserin aut Zhou, Jie verfasserin aut Chen, Yonggui verfasserin (orcid)0000-0002-0078-2204 aut Wu, Dongbei verfasserin aut Wang, Qigang verfasserin (orcid)0000-0002-6571-2549 aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 382 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:382 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 382 045F 660.05
allfieldsSound	10.1016/j.cej.2019.123018 doi (DE-627)ELV00330339X (ELSEVIER)S1385-8947(19)32428-3 DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Wei, Gumi verfasserin aut MoS 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Molybdenum disulfide (MoS2) nanosheet is an appealing material due to its various merits such as narrow bandgap, high photothermal conversion speed, and intrinsic sulfur-rich properties. Building up a MoS2-based smart material with all the merits combined has become a challenging topic. Herein, using the monomer N-isopropylacrylamide (NIPAM), a MoS2 self-initiated hydrogel adsorbents was fabricated by manipulation of MoS2 nanosheets as a photoinitiator response to UV light. The hydrogel adsorbent presents a high selectivity to Ag+, and can be quickly recycled upon the photothermal effect induced by 808 nm near-infrared laser irradiation. The adsorption-desorption cycle can be repeated for at least 6 times without obvious decrease of the Ag+ adsorption capacity. The entropy change associated with the desorption process is −16.7 J·K−1·mol−1, which confirms a spontaneous NIR-induced Ag+ desorption. Our MoS2-based smart hydrogel proves to be energy-efficient, quick-regenerated material for Ag+ enrichment. Molybdenum disulfide Self-initiated hydrogel Ag Light-response Quick desorption Cyclic regeneration Wei, Junjie verfasserin aut Zhou, Jie verfasserin aut Chen, Yonggui verfasserin (orcid)0000-0002-0078-2204 aut Wu, Dongbei verfasserin aut Wang, Qigang verfasserin (orcid)0000-0002-6571-2549 aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 382 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:382 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 382 045F 660.05
language	English
source	Enthalten in The chemical engineering journal 382 volume:382
sourceStr	Enthalten in The chemical engineering journal 382 volume:382
format_phy_str_mv	Article
bklname	Verfahrenstechnik: Allgemeines
institution	findex.gbv.de
topic_facet	Molybdenum disulfide Self-initiated hydrogel Ag Light-response Quick desorption Cyclic regeneration
dewey-raw	660.05
isfreeaccess_bool	false
container_title	The chemical engineering journal
authorswithroles_txt_mv	Wei, Gumi @@aut@@ Wei, Junjie @@aut@@ Zhou, Jie @@aut@@ Chen, Yonggui @@aut@@ Wu, Dongbei @@aut@@ Wang, Qigang @@aut@@
publishDateDaySort_date	2019-01-01T00:00:00Z
hierarchy_top_id	320500322
dewey-sort	3660.05
id	ELV00330339X
language_de	englisch
fullrecord	<?xml version="1.0" encoding="UTF-8"?><collection xmlns="http://www.loc.gov/MARC21/slim"><record><leader>01000caa a22002652 4500</leader><controlfield tag="001">ELV00330339X</controlfield><controlfield tag="003">DE-627</controlfield><controlfield tag="005">20230524131647.0</controlfield><controlfield tag="007">cr uuu---uuuuu</controlfield><controlfield tag="008">230430s2019 xx \|\|\|\|\|o 00\| \|\|eng c</controlfield><datafield tag="024" ind1="7" ind2=" "><subfield code="a">10.1016/j.cej.2019.123018</subfield><subfield code="2">doi</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(DE-627)ELV00330339X</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(ELSEVIER)S1385-8947(19)32428-3</subfield></datafield><datafield tag="040" ind1=" " ind2=" "><subfield code="a">DE-627</subfield><subfield code="b">ger</subfield><subfield code="c">DE-627</subfield><subfield code="e">rda</subfield></datafield><datafield tag="041" ind1=" " ind2=" "><subfield code="a">eng</subfield></datafield><datafield tag="082" ind1="0" ind2=" "><subfield code="a">660.05</subfield><subfield code="q">DE-101</subfield></datafield><datafield tag="082" ind1="0" ind2="4"><subfield code="a">660</subfield><subfield code="q">DE-101</subfield></datafield><datafield tag="082" ind1="0" ind2="4"><subfield code="a">660</subfield><subfield code="q">DE-600</subfield></datafield><datafield tag="084" ind1=" " ind2=" "><subfield code="a">58.10</subfield><subfield code="2">bkl</subfield></datafield><datafield tag="100" ind1="1" ind2=" "><subfield code="a">Wei, Gumi</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="245" ind1="1" ind2="0"><subfield code="a">MoS</subfield></datafield><datafield tag="264" ind1=" " ind2="1"><subfield code="c">2019</subfield></datafield><datafield tag="336" ind1=" " ind2=" "><subfield code="a">nicht spezifiziert</subfield><subfield code="b">zzz</subfield><subfield code="2">rdacontent</subfield></datafield><datafield tag="337" ind1=" " ind2=" "><subfield code="a">Computermedien</subfield><subfield code="b">c</subfield><subfield code="2">rdamedia</subfield></datafield><datafield tag="338" ind1=" " ind2=" "><subfield code="a">Online-Ressource</subfield><subfield code="b">cr</subfield><subfield code="2">rdacarrier</subfield></datafield><datafield tag="520" ind1=" " ind2=" "><subfield code="a">Molybdenum disulfide (MoS2) nanosheet is an appealing material due to its various merits such as narrow bandgap, high photothermal conversion speed, and intrinsic sulfur-rich properties. Building up a MoS2-based smart material with all the merits combined has become a challenging topic. Herein, using the monomer N-isopropylacrylamide (NIPAM), a MoS2 self-initiated hydrogel adsorbents was fabricated by manipulation of MoS2 nanosheets as a photoinitiator response to UV light. The hydrogel adsorbent presents a high selectivity to Ag+, and can be quickly recycled upon the photothermal effect induced by 808 nm near-infrared laser irradiation. The adsorption-desorption cycle can be repeated for at least 6 times without obvious decrease of the Ag+ adsorption capacity. The entropy change associated with the desorption process is −16.7 J·K−1·mol−1, which confirms a spontaneous NIR-induced Ag+ desorption. Our MoS2-based smart hydrogel proves to be energy-efficient, quick-regenerated material for Ag+ enrichment.</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Molybdenum disulfide</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Self-initiated hydrogel</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Ag</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Light-response</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Quick desorption</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Cyclic regeneration</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Wei, Junjie</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Zhou, Jie</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Chen, Yonggui</subfield><subfield code="e">verfasserin</subfield><subfield code="0">(orcid)0000-0002-0078-2204</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Wu, Dongbei</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Wang, Qigang</subfield><subfield code="e">verfasserin</subfield><subfield code="0">(orcid)0000-0002-6571-2549</subfield><subfield code="4">aut</subfield></datafield><datafield tag="773" ind1="0" ind2="8"><subfield code="i">Enthalten in</subfield><subfield code="t">The chemical engineering journal</subfield><subfield code="d">Amsterdam : Elsevier, 1997</subfield><subfield code="g">382</subfield><subfield code="h">Online-Ressource</subfield><subfield code="w">(DE-627)320500322</subfield><subfield code="w">(DE-600)2012137-4</subfield><subfield code="w">(DE-576)098330152</subfield><subfield code="x">1873-3212</subfield><subfield code="7">nnns</subfield></datafield><datafield tag="773" ind1="1" ind2="8"><subfield code="g">volume:382</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_USEFLAG_U</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">SYSFLAG_U</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ELV</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">SSG-OLC-PHA</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_20</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_22</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_23</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_24</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_31</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_32</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_40</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_60</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_62</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_63</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_65</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_69</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_70</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_73</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_74</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_90</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_95</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_100</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_105</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_110</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_150</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_151</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_224</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_370</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_602</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_702</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2003</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2004</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2005</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2011</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2014</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2015</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2020</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2021</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2025</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2027</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2034</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2038</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2044</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2048</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2049</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2050</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2056</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2059</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2061</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2064</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2065</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2068</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2111</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2112</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2113</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2118</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2122</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2129</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2143</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2147</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2148</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2152</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2153</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2190</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2336</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2507</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2522</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_4035</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_4037</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_4112</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_4125</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_4126</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_4242</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_4251</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_4305</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_4313</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_4323</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_4324</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_4325</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_4326</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_4333</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_4334</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_4335</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_4338</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_4393</subfield></datafield><datafield tag="936" ind1="b" ind2="k"><subfield code="a">58.10</subfield><subfield code="j">Verfahrenstechnik: Allgemeines</subfield></datafield><datafield tag="951" ind1=" " ind2=" "><subfield code="a">AR</subfield></datafield><datafield tag="952" ind1=" " ind2=" "><subfield code="d">382</subfield></datafield><datafield tag="953" ind1=" " ind2=" "><subfield code="2">045F</subfield><subfield code="a">660.05</subfield></datafield></record></collection>
author	Wei, Gumi
spellingShingle	Wei, Gumi ddc 660.05 ddc 660 bkl 58.10 misc Molybdenum disulfide misc Self-initiated hydrogel misc Ag misc Light-response misc Quick desorption misc Cyclic regeneration MoS
authorStr	Wei, Gumi
ppnlink_with_tag_str_mv	@@773@@(DE-627)320500322
format	electronic Article
dewey-ones	660 - Chemical engineering
delete_txt_mv	keep
author_role	aut aut aut aut aut aut
collection	elsevier
remote_str	true
illustrated	Not Illustrated
issn	1873-3212
topic_title	660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl MoS Molybdenum disulfide Self-initiated hydrogel Ag Light-response Quick desorption Cyclic regeneration
topic	ddc 660.05 ddc 660 bkl 58.10 misc Molybdenum disulfide misc Self-initiated hydrogel misc Ag misc Light-response misc Quick desorption misc Cyclic regeneration
topic_unstemmed	ddc 660.05 ddc 660 bkl 58.10 misc Molybdenum disulfide misc Self-initiated hydrogel misc Ag misc Light-response misc Quick desorption misc Cyclic regeneration
topic_browse	ddc 660.05 ddc 660 bkl 58.10 misc Molybdenum disulfide misc Self-initiated hydrogel misc Ag misc Light-response misc Quick desorption misc Cyclic regeneration
format_facet	Elektronische Aufsätze Aufsätze Elektronische Ressource
format_main_str_mv	Text Zeitschrift/Artikel
carriertype_str_mv	cr
hierarchy_parent_title	The chemical engineering journal
hierarchy_parent_id	320500322
dewey-tens	660 - Chemical engineering
hierarchy_top_title	The chemical engineering journal
isfreeaccess_txt	false
familylinks_str_mv	(DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152
title	MoS
ctrlnum	(DE-627)ELV00330339X (ELSEVIER)S1385-8947(19)32428-3
title_full	MoS
author_sort	Wei, Gumi
journal	The chemical engineering journal
journalStr	The chemical engineering journal
lang_code	eng
isOA_bool	false
dewey-hundreds	600 - Technology
recordtype	marc
publishDateSort	2019
contenttype_str_mv	zzz
author_browse	Wei, Gumi Wei, Junjie Zhou, Jie Chen, Yonggui Wu, Dongbei Wang, Qigang
container_volume	382
class	660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl
format_se	Elektronische Aufsätze
author-letter	Wei, Gumi
doi_str_mv	10.1016/j.cej.2019.123018
normlink	(ORCID)0000-0002-0078-2204 (ORCID)0000-0002-6571-2549
normlink_prefix_str_mv	(orcid)0000-0002-0078-2204 (orcid)0000-0002-6571-2549
dewey-full	660.05 660
author2-role	verfasserin
title_sort	mos
title_auth	MoS
abstract	Molybdenum disulfide (MoS2) nanosheet is an appealing material due to its various merits such as narrow bandgap, high photothermal conversion speed, and intrinsic sulfur-rich properties. Building up a MoS2-based smart material with all the merits combined has become a challenging topic. Herein, using the monomer N-isopropylacrylamide (NIPAM), a MoS2 self-initiated hydrogel adsorbents was fabricated by manipulation of MoS2 nanosheets as a photoinitiator response to UV light. The hydrogel adsorbent presents a high selectivity to Ag+, and can be quickly recycled upon the photothermal effect induced by 808 nm near-infrared laser irradiation. The adsorption-desorption cycle can be repeated for at least 6 times without obvious decrease of the Ag+ adsorption capacity. The entropy change associated with the desorption process is −16.7 J·K−1·mol−1, which confirms a spontaneous NIR-induced Ag+ desorption. Our MoS2-based smart hydrogel proves to be energy-efficient, quick-regenerated material for Ag+ enrichment.
abstractGer	Molybdenum disulfide (MoS2) nanosheet is an appealing material due to its various merits such as narrow bandgap, high photothermal conversion speed, and intrinsic sulfur-rich properties. Building up a MoS2-based smart material with all the merits combined has become a challenging topic. Herein, using the monomer N-isopropylacrylamide (NIPAM), a MoS2 self-initiated hydrogel adsorbents was fabricated by manipulation of MoS2 nanosheets as a photoinitiator response to UV light. The hydrogel adsorbent presents a high selectivity to Ag+, and can be quickly recycled upon the photothermal effect induced by 808 nm near-infrared laser irradiation. The adsorption-desorption cycle can be repeated for at least 6 times without obvious decrease of the Ag+ adsorption capacity. The entropy change associated with the desorption process is −16.7 J·K−1·mol−1, which confirms a spontaneous NIR-induced Ag+ desorption. Our MoS2-based smart hydrogel proves to be energy-efficient, quick-regenerated material for Ag+ enrichment.
abstract_unstemmed	Molybdenum disulfide (MoS2) nanosheet is an appealing material due to its various merits such as narrow bandgap, high photothermal conversion speed, and intrinsic sulfur-rich properties. Building up a MoS2-based smart material with all the merits combined has become a challenging topic. Herein, using the monomer N-isopropylacrylamide (NIPAM), a MoS2 self-initiated hydrogel adsorbents was fabricated by manipulation of MoS2 nanosheets as a photoinitiator response to UV light. The hydrogel adsorbent presents a high selectivity to Ag+, and can be quickly recycled upon the photothermal effect induced by 808 nm near-infrared laser irradiation. The adsorption-desorption cycle can be repeated for at least 6 times without obvious decrease of the Ag+ adsorption capacity. The entropy change associated with the desorption process is −16.7 J·K−1·mol−1, which confirms a spontaneous NIR-induced Ag+ desorption. Our MoS2-based smart hydrogel proves to be energy-efficient, quick-regenerated material for Ag+ enrichment.
collection_details	GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393
title_short	MoS
remote_bool	true
author2	Wei, Junjie Zhou, Jie Chen, Yonggui Wu, Dongbei Wang, Qigang
author2Str	Wei, Junjie Zhou, Jie Chen, Yonggui Wu, Dongbei Wang, Qigang
ppnlink	320500322
mediatype_str_mv	c
isOA_txt	false
hochschulschrift_bool	false
doi_str	10.1016/j.cej.2019.123018
up_date	2024-07-06T19:10:28.329Z
_version_	1803857982475206656
fullrecord_marcxml	<?xml version="1.0" encoding="UTF-8"?><collection xmlns="http://www.loc.gov/MARC21/slim"><record><leader>01000caa a22002652 4500</leader><controlfield tag="001">ELV00330339X</controlfield><controlfield tag="003">DE-627</controlfield><controlfield tag="005">20230524131647.0</controlfield><controlfield tag="007">cr uuu---uuuuu</controlfield><controlfield tag="008">230430s2019 xx \|\|\|\|\|o 00\| \|\|eng c</controlfield><datafield tag="024" ind1="7" ind2=" "><subfield code="a">10.1016/j.cej.2019.123018</subfield><subfield code="2">doi</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(DE-627)ELV00330339X</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(ELSEVIER)S1385-8947(19)32428-3</subfield></datafield><datafield tag="040" ind1=" " ind2=" "><subfield code="a">DE-627</subfield><subfield code="b">ger</subfield><subfield code="c">DE-627</subfield><subfield code="e">rda</subfield></datafield><datafield tag="041" ind1=" " ind2=" "><subfield code="a">eng</subfield></datafield><datafield tag="082" ind1="0" ind2=" "><subfield code="a">660.05</subfield><subfield code="q">DE-101</subfield></datafield><datafield tag="082" ind1="0" ind2="4"><subfield code="a">660</subfield><subfield code="q">DE-101</subfield></datafield><datafield tag="082" ind1="0" ind2="4"><subfield code="a">660</subfield><subfield code="q">DE-600</subfield></datafield><datafield tag="084" ind1=" " ind2=" "><subfield code="a">58.10</subfield><subfield code="2">bkl</subfield></datafield><datafield tag="100" ind1="1" ind2=" "><subfield code="a">Wei, Gumi</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="245" ind1="1" ind2="0"><subfield code="a">MoS</subfield></datafield><datafield tag="264" ind1=" " ind2="1"><subfield code="c">2019</subfield></datafield><datafield tag="336" ind1=" " ind2=" "><subfield code="a">nicht spezifiziert</subfield><subfield code="b">zzz</subfield><subfield code="2">rdacontent</subfield></datafield><datafield tag="337" ind1=" " ind2=" "><subfield code="a">Computermedien</subfield><subfield code="b">c</subfield><subfield code="2">rdamedia</subfield></datafield><datafield tag="338" ind1=" " ind2=" "><subfield code="a">Online-Ressource</subfield><subfield code="b">cr</subfield><subfield code="2">rdacarrier</subfield></datafield><datafield tag="520" ind1=" " ind2=" "><subfield code="a">Molybdenum disulfide (MoS2) nanosheet is an appealing material due to its various merits such as narrow bandgap, high photothermal conversion speed, and intrinsic sulfur-rich properties. Building up a MoS2-based smart material with all the merits combined has become a challenging topic. Herein, using the monomer N-isopropylacrylamide (NIPAM), a MoS2 self-initiated hydrogel adsorbents was fabricated by manipulation of MoS2 nanosheets as a photoinitiator response to UV light. The hydrogel adsorbent presents a high selectivity to Ag+, and can be quickly recycled upon the photothermal effect induced by 808 nm near-infrared laser irradiation. The adsorption-desorption cycle can be repeated for at least 6 times without obvious decrease of the Ag+ adsorption capacity. The entropy change associated with the desorption process is −16.7 J·K−1·mol−1, which confirms a spontaneous NIR-induced Ag+ desorption. Our MoS2-based smart hydrogel proves to be energy-efficient, quick-regenerated material for Ag+ enrichment.</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Molybdenum disulfide</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Self-initiated hydrogel</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Ag</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Light-response</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Quick desorption</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Cyclic regeneration</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Wei, Junjie</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Zhou, Jie</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Chen, Yonggui</subfield><subfield code="e">verfasserin</subfield><subfield code="0">(orcid)0000-0002-0078-2204</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Wu, Dongbei</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Wang, Qigang</subfield><subfield code="e">verfasserin</subfield><subfield code="0">(orcid)0000-0002-6571-2549</subfield><subfield code="4">aut</subfield></datafield><datafield tag="773" ind1="0" ind2="8"><subfield code="i">Enthalten in</subfield><subfield code="t">The chemical engineering journal</subfield><subfield code="d">Amsterdam : Elsevier, 1997</subfield><subfield code="g">382</subfield><subfield code="h">Online-Ressource</subfield><subfield code="w">(DE-627)320500322</subfield><subfield code="w">(DE-600)2012137-4</subfield><subfield code="w">(DE-576)098330152</subfield><subfield code="x">1873-3212</subfield><subfield code="7">nnns</subfield></datafield><datafield tag="773" ind1="1" ind2="8"><subfield code="g">volume:382</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_USEFLAG_U</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">SYSFLAG_U</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ELV</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">SSG-OLC-PHA</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_20</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_22</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_23</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_24</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_31</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_32</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_40</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_60</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_62</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_63</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_65</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_69</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_70</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_73</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_74</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_90</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_95</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_100</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_105</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_110</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_150</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_151</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_224</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_370</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_602</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_702</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2003</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2004</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2005</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2011</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2014</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2015</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2020</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2021</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2025</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2027</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2034</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2038</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2044</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2048</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2049</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2050</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2056</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2059</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2061</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2064</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2065</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2068</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2111</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2112</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2113</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2118</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2122</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2129</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2143</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2147</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2148</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2152</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2153</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2190</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2336</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2507</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_2522</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_4035</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_4037</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_4112</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_4125</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_4126</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_4242</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_4251</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_4305</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_4313</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_4323</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_4324</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_4325</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_4326</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_4333</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_4334</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_4335</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_4338</subfield></datafield><datafield tag="912" ind1=" " ind2=" "><subfield code="a">GBV_ILN_4393</subfield></datafield><datafield tag="936" ind1="b" ind2="k"><subfield code="a">58.10</subfield><subfield code="j">Verfahrenstechnik: Allgemeines</subfield></datafield><datafield tag="951" ind1=" " ind2=" "><subfield code="a">AR</subfield></datafield><datafield tag="952" ind1=" " ind2=" "><subfield code="d">382</subfield></datafield><datafield tag="953" ind1=" " ind2=" "><subfield code="2">045F</subfield><subfield code="a">660.05</subfield></datafield></record></collection>
score	7.40121

Nicht das Richtige dabei?

Schreiben Sie uns!

MoS

Nicht das Richtige dabei?

Zugang & Verfügbarkeit

Vorhandene Bände

Nicht das Richtige dabei?