Facet engineering of WO

Hydrogen generation via photoelectrochemical (PEC) technology is one of the most ideal strategies for providing sustainable fuel, in particular, from abundant natural resource (such as seawater). Herein, we demonstrate facet-controlled WO3 array decorated with reasonable distribution of dual-cocatal...
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Autor*in:	Liu, Jingchao [verfasserIn] Xu, Si-Min [verfasserIn] Li, Yanfei [verfasserIn] Zhang, Ruikang [verfasserIn] Shao, Mingfei [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2019

Schlagwörter:	Photoelectrochemical hydrogen generation Natural seawater WO Facet engineering Dual-cocatalysts

Übergeordnetes Werk:	Enthalten in: Applied catalysis / B - Amsterdam : Elsevier, 1992, 264
Übergeordnetes Werk:	volume:264

DOI / URN:	10.1016/j.apcatb.2019.118540

Katalog-ID:	ELV003525619

Internformat


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520			\|a Hydrogen generation via photoelectrochemical (PEC) technology is one of the most ideal strategies for providing sustainable fuel, in particular, from abundant natural resource (such as seawater). Herein, we demonstrate facet-controlled WO3 array decorated with reasonable distribution of dual-cocatalysts, which shows highly efficient and stable PEC H2 generation from natural seawater. The experimental and theoretical results illustrate that photo-generated electrons and holes accumulate directionally on different crystal facets of WO3 to achieve effective spatial separation, owing to the divergent energy levels of each crystal facet. Moreover, the charge utilization is further enhanced by selective modification of Ag nanoparticles and ZnFe-layered double hydroxide on different crystal facets reasonably, getting an average PEC H2 production of 38.18 μmol h−1 from natural seawater with excellent stability. This work opens up a new facet engineering pathway for the fabrication of novel photoelectrodes, which have potential applications in the fields of solar energy conversion and storage.
650		4	\|a Photoelectrochemical hydrogen generation
650		4	\|a Natural seawater
650		4	\|a WO
650		4	\|a Facet engineering
650		4	\|a Dual-cocatalysts
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700	1		\|a Zhang, Ruikang \|e verfasserin \|4 aut
700	1		\|a Shao, Mingfei \|e verfasserin \|0 (orcid)0000-0002-6461-623X \|4 aut
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author_variant	j l jl s m x smx y l yl r z rz m s ms
matchkey_str	article:09263373:2019----::aeegnei
hierarchy_sort_str	2019
bklnumber	35.17 58.50 43.12
publishDate	2019
allfields	10.1016/j.apcatb.2019.118540 doi (DE-627)ELV003525619 (ELSEVIER)S0926-3373(19)31286-X DE-627 ger DE-627 rda eng 540 DE-600 35.17 bkl 58.50 bkl 43.12 bkl Liu, Jingchao verfasserin aut Facet engineering of WO 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Hydrogen generation via photoelectrochemical (PEC) technology is one of the most ideal strategies for providing sustainable fuel, in particular, from abundant natural resource (such as seawater). Herein, we demonstrate facet-controlled WO3 array decorated with reasonable distribution of dual-cocatalysts, which shows highly efficient and stable PEC H2 generation from natural seawater. The experimental and theoretical results illustrate that photo-generated electrons and holes accumulate directionally on different crystal facets of WO3 to achieve effective spatial separation, owing to the divergent energy levels of each crystal facet. Moreover, the charge utilization is further enhanced by selective modification of Ag nanoparticles and ZnFe-layered double hydroxide on different crystal facets reasonably, getting an average PEC H2 production of 38.18 μmol h−1 from natural seawater with excellent stability. This work opens up a new facet engineering pathway for the fabrication of novel photoelectrodes, which have potential applications in the fields of solar energy conversion and storage. Photoelectrochemical hydrogen generation Natural seawater WO Facet engineering Dual-cocatalysts Xu, Si-Min verfasserin aut Li, Yanfei verfasserin aut Zhang, Ruikang verfasserin aut Shao, Mingfei verfasserin (orcid)0000-0002-6461-623X aut Enthalten in Applied catalysis / B Amsterdam : Elsevier, 1992 264 Online-Ressource (DE-627)320578658 (DE-600)2017331-3 (DE-576)095956344 0926-3373 nnns volume:264 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.17 Katalyse 58.50 Umwelttechnik: Allgemeines 43.12 Umweltchemie AR 264
spelling	10.1016/j.apcatb.2019.118540 doi (DE-627)ELV003525619 (ELSEVIER)S0926-3373(19)31286-X DE-627 ger DE-627 rda eng 540 DE-600 35.17 bkl 58.50 bkl 43.12 bkl Liu, Jingchao verfasserin aut Facet engineering of WO 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Hydrogen generation via photoelectrochemical (PEC) technology is one of the most ideal strategies for providing sustainable fuel, in particular, from abundant natural resource (such as seawater). Herein, we demonstrate facet-controlled WO3 array decorated with reasonable distribution of dual-cocatalysts, which shows highly efficient and stable PEC H2 generation from natural seawater. The experimental and theoretical results illustrate that photo-generated electrons and holes accumulate directionally on different crystal facets of WO3 to achieve effective spatial separation, owing to the divergent energy levels of each crystal facet. Moreover, the charge utilization is further enhanced by selective modification of Ag nanoparticles and ZnFe-layered double hydroxide on different crystal facets reasonably, getting an average PEC H2 production of 38.18 μmol h−1 from natural seawater with excellent stability. This work opens up a new facet engineering pathway for the fabrication of novel photoelectrodes, which have potential applications in the fields of solar energy conversion and storage. Photoelectrochemical hydrogen generation Natural seawater WO Facet engineering Dual-cocatalysts Xu, Si-Min verfasserin aut Li, Yanfei verfasserin aut Zhang, Ruikang verfasserin aut Shao, Mingfei verfasserin (orcid)0000-0002-6461-623X aut Enthalten in Applied catalysis / B Amsterdam : Elsevier, 1992 264 Online-Ressource (DE-627)320578658 (DE-600)2017331-3 (DE-576)095956344 0926-3373 nnns volume:264 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.17 Katalyse 58.50 Umwelttechnik: Allgemeines 43.12 Umweltchemie AR 264
allfields_unstemmed	10.1016/j.apcatb.2019.118540 doi (DE-627)ELV003525619 (ELSEVIER)S0926-3373(19)31286-X DE-627 ger DE-627 rda eng 540 DE-600 35.17 bkl 58.50 bkl 43.12 bkl Liu, Jingchao verfasserin aut Facet engineering of WO 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Hydrogen generation via photoelectrochemical (PEC) technology is one of the most ideal strategies for providing sustainable fuel, in particular, from abundant natural resource (such as seawater). Herein, we demonstrate facet-controlled WO3 array decorated with reasonable distribution of dual-cocatalysts, which shows highly efficient and stable PEC H2 generation from natural seawater. The experimental and theoretical results illustrate that photo-generated electrons and holes accumulate directionally on different crystal facets of WO3 to achieve effective spatial separation, owing to the divergent energy levels of each crystal facet. Moreover, the charge utilization is further enhanced by selective modification of Ag nanoparticles and ZnFe-layered double hydroxide on different crystal facets reasonably, getting an average PEC H2 production of 38.18 μmol h−1 from natural seawater with excellent stability. This work opens up a new facet engineering pathway for the fabrication of novel photoelectrodes, which have potential applications in the fields of solar energy conversion and storage. Photoelectrochemical hydrogen generation Natural seawater WO Facet engineering Dual-cocatalysts Xu, Si-Min verfasserin aut Li, Yanfei verfasserin aut Zhang, Ruikang verfasserin aut Shao, Mingfei verfasserin (orcid)0000-0002-6461-623X aut Enthalten in Applied catalysis / B Amsterdam : Elsevier, 1992 264 Online-Ressource (DE-627)320578658 (DE-600)2017331-3 (DE-576)095956344 0926-3373 nnns volume:264 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.17 Katalyse 58.50 Umwelttechnik: Allgemeines 43.12 Umweltchemie AR 264
allfieldsGer	10.1016/j.apcatb.2019.118540 doi (DE-627)ELV003525619 (ELSEVIER)S0926-3373(19)31286-X DE-627 ger DE-627 rda eng 540 DE-600 35.17 bkl 58.50 bkl 43.12 bkl Liu, Jingchao verfasserin aut Facet engineering of WO 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Hydrogen generation via photoelectrochemical (PEC) technology is one of the most ideal strategies for providing sustainable fuel, in particular, from abundant natural resource (such as seawater). Herein, we demonstrate facet-controlled WO3 array decorated with reasonable distribution of dual-cocatalysts, which shows highly efficient and stable PEC H2 generation from natural seawater. The experimental and theoretical results illustrate that photo-generated electrons and holes accumulate directionally on different crystal facets of WO3 to achieve effective spatial separation, owing to the divergent energy levels of each crystal facet. Moreover, the charge utilization is further enhanced by selective modification of Ag nanoparticles and ZnFe-layered double hydroxide on different crystal facets reasonably, getting an average PEC H2 production of 38.18 μmol h−1 from natural seawater with excellent stability. This work opens up a new facet engineering pathway for the fabrication of novel photoelectrodes, which have potential applications in the fields of solar energy conversion and storage. Photoelectrochemical hydrogen generation Natural seawater WO Facet engineering Dual-cocatalysts Xu, Si-Min verfasserin aut Li, Yanfei verfasserin aut Zhang, Ruikang verfasserin aut Shao, Mingfei verfasserin (orcid)0000-0002-6461-623X aut Enthalten in Applied catalysis / B Amsterdam : Elsevier, 1992 264 Online-Ressource (DE-627)320578658 (DE-600)2017331-3 (DE-576)095956344 0926-3373 nnns volume:264 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.17 Katalyse 58.50 Umwelttechnik: Allgemeines 43.12 Umweltchemie AR 264
allfieldsSound	10.1016/j.apcatb.2019.118540 doi (DE-627)ELV003525619 (ELSEVIER)S0926-3373(19)31286-X DE-627 ger DE-627 rda eng 540 DE-600 35.17 bkl 58.50 bkl 43.12 bkl Liu, Jingchao verfasserin aut Facet engineering of WO 2019 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Hydrogen generation via photoelectrochemical (PEC) technology is one of the most ideal strategies for providing sustainable fuel, in particular, from abundant natural resource (such as seawater). Herein, we demonstrate facet-controlled WO3 array decorated with reasonable distribution of dual-cocatalysts, which shows highly efficient and stable PEC H2 generation from natural seawater. The experimental and theoretical results illustrate that photo-generated electrons and holes accumulate directionally on different crystal facets of WO3 to achieve effective spatial separation, owing to the divergent energy levels of each crystal facet. Moreover, the charge utilization is further enhanced by selective modification of Ag nanoparticles and ZnFe-layered double hydroxide on different crystal facets reasonably, getting an average PEC H2 production of 38.18 μmol h−1 from natural seawater with excellent stability. This work opens up a new facet engineering pathway for the fabrication of novel photoelectrodes, which have potential applications in the fields of solar energy conversion and storage. Photoelectrochemical hydrogen generation Natural seawater WO Facet engineering Dual-cocatalysts Xu, Si-Min verfasserin aut Li, Yanfei verfasserin aut Zhang, Ruikang verfasserin aut Shao, Mingfei verfasserin (orcid)0000-0002-6461-623X aut Enthalten in Applied catalysis / B Amsterdam : Elsevier, 1992 264 Online-Ressource (DE-627)320578658 (DE-600)2017331-3 (DE-576)095956344 0926-3373 nnns volume:264 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.17 Katalyse 58.50 Umwelttechnik: Allgemeines 43.12 Umweltchemie AR 264
language	English
source	Enthalten in Applied catalysis / B 264 volume:264
sourceStr	Enthalten in Applied catalysis / B 264 volume:264
format_phy_str_mv	Article
bklname	Katalyse Umwelttechnik: Allgemeines Umweltchemie
institution	findex.gbv.de
topic_facet	Photoelectrochemical hydrogen generation Natural seawater WO Facet engineering Dual-cocatalysts
dewey-raw	540
isfreeaccess_bool	false
container_title	Applied catalysis / B
authorswithroles_txt_mv	Liu, Jingchao @@aut@@ Xu, Si-Min @@aut@@ Li, Yanfei @@aut@@ Zhang, Ruikang @@aut@@ Shao, Mingfei @@aut@@
publishDateDaySort_date	2019-01-01T00:00:00Z
hierarchy_top_id	320578658
dewey-sort	3540
id	ELV003525619
language_de	englisch
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author	Liu, Jingchao
spellingShingle	Liu, Jingchao ddc 540 bkl 35.17 bkl 58.50 bkl 43.12 misc Photoelectrochemical hydrogen generation misc Natural seawater misc WO misc Facet engineering misc Dual-cocatalysts Facet engineering of WO
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topic_title	540 DE-600 35.17 bkl 58.50 bkl 43.12 bkl Facet engineering of WO Photoelectrochemical hydrogen generation Natural seawater WO Facet engineering Dual-cocatalysts
topic	ddc 540 bkl 35.17 bkl 58.50 bkl 43.12 misc Photoelectrochemical hydrogen generation misc Natural seawater misc WO misc Facet engineering misc Dual-cocatalysts
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title	Facet engineering of WO
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title_full	Facet engineering of WO
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title_sort	facet engineering of wo
title_auth	Facet engineering of WO
abstract	Hydrogen generation via photoelectrochemical (PEC) technology is one of the most ideal strategies for providing sustainable fuel, in particular, from abundant natural resource (such as seawater). Herein, we demonstrate facet-controlled WO3 array decorated with reasonable distribution of dual-cocatalysts, which shows highly efficient and stable PEC H2 generation from natural seawater. The experimental and theoretical results illustrate that photo-generated electrons and holes accumulate directionally on different crystal facets of WO3 to achieve effective spatial separation, owing to the divergent energy levels of each crystal facet. Moreover, the charge utilization is further enhanced by selective modification of Ag nanoparticles and ZnFe-layered double hydroxide on different crystal facets reasonably, getting an average PEC H2 production of 38.18 μmol h−1 from natural seawater with excellent stability. This work opens up a new facet engineering pathway for the fabrication of novel photoelectrodes, which have potential applications in the fields of solar energy conversion and storage.
abstractGer	Hydrogen generation via photoelectrochemical (PEC) technology is one of the most ideal strategies for providing sustainable fuel, in particular, from abundant natural resource (such as seawater). Herein, we demonstrate facet-controlled WO3 array decorated with reasonable distribution of dual-cocatalysts, which shows highly efficient and stable PEC H2 generation from natural seawater. The experimental and theoretical results illustrate that photo-generated electrons and holes accumulate directionally on different crystal facets of WO3 to achieve effective spatial separation, owing to the divergent energy levels of each crystal facet. Moreover, the charge utilization is further enhanced by selective modification of Ag nanoparticles and ZnFe-layered double hydroxide on different crystal facets reasonably, getting an average PEC H2 production of 38.18 μmol h−1 from natural seawater with excellent stability. This work opens up a new facet engineering pathway for the fabrication of novel photoelectrodes, which have potential applications in the fields of solar energy conversion and storage.
abstract_unstemmed	Hydrogen generation via photoelectrochemical (PEC) technology is one of the most ideal strategies for providing sustainable fuel, in particular, from abundant natural resource (such as seawater). Herein, we demonstrate facet-controlled WO3 array decorated with reasonable distribution of dual-cocatalysts, which shows highly efficient and stable PEC H2 generation from natural seawater. The experimental and theoretical results illustrate that photo-generated electrons and holes accumulate directionally on different crystal facets of WO3 to achieve effective spatial separation, owing to the divergent energy levels of each crystal facet. Moreover, the charge utilization is further enhanced by selective modification of Ag nanoparticles and ZnFe-layered double hydroxide on different crystal facets reasonably, getting an average PEC H2 production of 38.18 μmol h−1 from natural seawater with excellent stability. This work opens up a new facet engineering pathway for the fabrication of novel photoelectrodes, which have potential applications in the fields of solar energy conversion and storage.
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title_short	Facet engineering of WO
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up_date	2024-07-06T19:55:05.516Z
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Facet engineering of WO

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