Photoluminescence-tunable carbon dots from synergy effect of sulfur doping and water engineering
Multiple-color-emissive carbon dots (CDs) is one of the hotspots due to its potential in multi-fields. However, the exploring of efficient synthetic strategies and emission mechanisms still remain challenging. Herein, we report a facile solvothermal route to prepare CDs with tunable photoluminescenc...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Gao, Dong [verfasserIn] Zhang, Yusheng [verfasserIn] Liu, Amin [verfasserIn] Zhu, Yuda [verfasserIn] Chen, Suping [verfasserIn] Wei, Dan [verfasserIn] Sun, Jing [verfasserIn] Guo, Zhenzhen [verfasserIn] Fan, Hongsong [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2020 |
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| Schlagwörter: |
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| Übergeordnetes Werk: |
Enthalten in: The chemical engineering journal - Amsterdam : Elsevier, 1997, 388 |
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| Übergeordnetes Werk: |
volume:388 |
| DOI / URN: |
10.1016/j.cej.2020.124199 |
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| Katalog-ID: |
ELV004024567 |
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| 245 | 1 | 0 | |a Photoluminescence-tunable carbon dots from synergy effect of sulfur doping and water engineering |
| 264 | 1 | |c 2020 | |
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| 520 | |a Multiple-color-emissive carbon dots (CDs) is one of the hotspots due to its potential in multi-fields. However, the exploring of efficient synthetic strategies and emission mechanisms still remain challenging. Herein, we report a facile solvothermal route to prepare CDs with tunable photoluminescence (PL) from green to red via a novel PL-tuning strategy of sulfur doping and water engineering. By detailed characterizations and comparison, it is demonstrated that the S doping can significantly increase the content of graphitic nitrogen, resulting in the fluorescence shifting from green to yellow; on the other hand, water engineering is able to yield carboxyl group and enhance surface oxidation degree, which can further facilitate the PL shifting from yellow to red. Owning to multicolor emissions and S doping, the prepared PL-tunable CDs present versatility in various applications including fluorescent films, light-emitting diodes (LED), bioimaging probe and highly sensitive Fe3+ detector. | ||
| 650 | 4 | |a Carbon dots | |
| 650 | 4 | |a Tunable fluorescence | |
| 650 | 4 | |a Sulfur doping | |
| 650 | 4 | |a Water engineering | |
| 650 | 4 | |a Light-emitting diodes | |
| 650 | 4 | |a Intracellular Fe | |
| 700 | 1 | |a Zhang, Yusheng |e verfasserin |4 aut | |
| 700 | 1 | |a Liu, Amin |e verfasserin |4 aut | |
| 700 | 1 | |a Zhu, Yuda |e verfasserin |4 aut | |
| 700 | 1 | |a Chen, Suping |e verfasserin |4 aut | |
| 700 | 1 | |a Wei, Dan |e verfasserin |4 aut | |
| 700 | 1 | |a Sun, Jing |e verfasserin |4 aut | |
| 700 | 1 | |a Guo, Zhenzhen |e verfasserin |4 aut | |
| 700 | 1 | |a Fan, Hongsong |e verfasserin |0 (orcid)0000-0003-3812-9208 |4 aut | |
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10.1016/j.cej.2020.124199 doi (DE-627)ELV004024567 (ELSEVIER)S1385-8947(20)30190-X DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Gao, Dong verfasserin aut Photoluminescence-tunable carbon dots from synergy effect of sulfur doping and water engineering 2020 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Multiple-color-emissive carbon dots (CDs) is one of the hotspots due to its potential in multi-fields. However, the exploring of efficient synthetic strategies and emission mechanisms still remain challenging. Herein, we report a facile solvothermal route to prepare CDs with tunable photoluminescence (PL) from green to red via a novel PL-tuning strategy of sulfur doping and water engineering. By detailed characterizations and comparison, it is demonstrated that the S doping can significantly increase the content of graphitic nitrogen, resulting in the fluorescence shifting from green to yellow; on the other hand, water engineering is able to yield carboxyl group and enhance surface oxidation degree, which can further facilitate the PL shifting from yellow to red. Owning to multicolor emissions and S doping, the prepared PL-tunable CDs present versatility in various applications including fluorescent films, light-emitting diodes (LED), bioimaging probe and highly sensitive Fe3+ detector. Carbon dots Tunable fluorescence Sulfur doping Water engineering Light-emitting diodes Intracellular Fe Zhang, Yusheng verfasserin aut Liu, Amin verfasserin aut Zhu, Yuda verfasserin aut Chen, Suping verfasserin aut Wei, Dan verfasserin aut Sun, Jing verfasserin aut Guo, Zhenzhen verfasserin aut Fan, Hongsong verfasserin (orcid)0000-0003-3812-9208 aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 388 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:388 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 388 045F 660.05 |
| spelling |
10.1016/j.cej.2020.124199 doi (DE-627)ELV004024567 (ELSEVIER)S1385-8947(20)30190-X DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Gao, Dong verfasserin aut Photoluminescence-tunable carbon dots from synergy effect of sulfur doping and water engineering 2020 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Multiple-color-emissive carbon dots (CDs) is one of the hotspots due to its potential in multi-fields. However, the exploring of efficient synthetic strategies and emission mechanisms still remain challenging. Herein, we report a facile solvothermal route to prepare CDs with tunable photoluminescence (PL) from green to red via a novel PL-tuning strategy of sulfur doping and water engineering. By detailed characterizations and comparison, it is demonstrated that the S doping can significantly increase the content of graphitic nitrogen, resulting in the fluorescence shifting from green to yellow; on the other hand, water engineering is able to yield carboxyl group and enhance surface oxidation degree, which can further facilitate the PL shifting from yellow to red. Owning to multicolor emissions and S doping, the prepared PL-tunable CDs present versatility in various applications including fluorescent films, light-emitting diodes (LED), bioimaging probe and highly sensitive Fe3+ detector. Carbon dots Tunable fluorescence Sulfur doping Water engineering Light-emitting diodes Intracellular Fe Zhang, Yusheng verfasserin aut Liu, Amin verfasserin aut Zhu, Yuda verfasserin aut Chen, Suping verfasserin aut Wei, Dan verfasserin aut Sun, Jing verfasserin aut Guo, Zhenzhen verfasserin aut Fan, Hongsong verfasserin (orcid)0000-0003-3812-9208 aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 388 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:388 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 388 045F 660.05 |
| allfields_unstemmed |
10.1016/j.cej.2020.124199 doi (DE-627)ELV004024567 (ELSEVIER)S1385-8947(20)30190-X DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Gao, Dong verfasserin aut Photoluminescence-tunable carbon dots from synergy effect of sulfur doping and water engineering 2020 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Multiple-color-emissive carbon dots (CDs) is one of the hotspots due to its potential in multi-fields. However, the exploring of efficient synthetic strategies and emission mechanisms still remain challenging. Herein, we report a facile solvothermal route to prepare CDs with tunable photoluminescence (PL) from green to red via a novel PL-tuning strategy of sulfur doping and water engineering. By detailed characterizations and comparison, it is demonstrated that the S doping can significantly increase the content of graphitic nitrogen, resulting in the fluorescence shifting from green to yellow; on the other hand, water engineering is able to yield carboxyl group and enhance surface oxidation degree, which can further facilitate the PL shifting from yellow to red. Owning to multicolor emissions and S doping, the prepared PL-tunable CDs present versatility in various applications including fluorescent films, light-emitting diodes (LED), bioimaging probe and highly sensitive Fe3+ detector. Carbon dots Tunable fluorescence Sulfur doping Water engineering Light-emitting diodes Intracellular Fe Zhang, Yusheng verfasserin aut Liu, Amin verfasserin aut Zhu, Yuda verfasserin aut Chen, Suping verfasserin aut Wei, Dan verfasserin aut Sun, Jing verfasserin aut Guo, Zhenzhen verfasserin aut Fan, Hongsong verfasserin (orcid)0000-0003-3812-9208 aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 388 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:388 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 388 045F 660.05 |
| allfieldsGer |
10.1016/j.cej.2020.124199 doi (DE-627)ELV004024567 (ELSEVIER)S1385-8947(20)30190-X DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Gao, Dong verfasserin aut Photoluminescence-tunable carbon dots from synergy effect of sulfur doping and water engineering 2020 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Multiple-color-emissive carbon dots (CDs) is one of the hotspots due to its potential in multi-fields. However, the exploring of efficient synthetic strategies and emission mechanisms still remain challenging. Herein, we report a facile solvothermal route to prepare CDs with tunable photoluminescence (PL) from green to red via a novel PL-tuning strategy of sulfur doping and water engineering. By detailed characterizations and comparison, it is demonstrated that the S doping can significantly increase the content of graphitic nitrogen, resulting in the fluorescence shifting from green to yellow; on the other hand, water engineering is able to yield carboxyl group and enhance surface oxidation degree, which can further facilitate the PL shifting from yellow to red. Owning to multicolor emissions and S doping, the prepared PL-tunable CDs present versatility in various applications including fluorescent films, light-emitting diodes (LED), bioimaging probe and highly sensitive Fe3+ detector. Carbon dots Tunable fluorescence Sulfur doping Water engineering Light-emitting diodes Intracellular Fe Zhang, Yusheng verfasserin aut Liu, Amin verfasserin aut Zhu, Yuda verfasserin aut Chen, Suping verfasserin aut Wei, Dan verfasserin aut Sun, Jing verfasserin aut Guo, Zhenzhen verfasserin aut Fan, Hongsong verfasserin (orcid)0000-0003-3812-9208 aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 388 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:388 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 388 045F 660.05 |
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10.1016/j.cej.2020.124199 doi (DE-627)ELV004024567 (ELSEVIER)S1385-8947(20)30190-X DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Gao, Dong verfasserin aut Photoluminescence-tunable carbon dots from synergy effect of sulfur doping and water engineering 2020 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Multiple-color-emissive carbon dots (CDs) is one of the hotspots due to its potential in multi-fields. However, the exploring of efficient synthetic strategies and emission mechanisms still remain challenging. Herein, we report a facile solvothermal route to prepare CDs with tunable photoluminescence (PL) from green to red via a novel PL-tuning strategy of sulfur doping and water engineering. By detailed characterizations and comparison, it is demonstrated that the S doping can significantly increase the content of graphitic nitrogen, resulting in the fluorescence shifting from green to yellow; on the other hand, water engineering is able to yield carboxyl group and enhance surface oxidation degree, which can further facilitate the PL shifting from yellow to red. Owning to multicolor emissions and S doping, the prepared PL-tunable CDs present versatility in various applications including fluorescent films, light-emitting diodes (LED), bioimaging probe and highly sensitive Fe3+ detector. Carbon dots Tunable fluorescence Sulfur doping Water engineering Light-emitting diodes Intracellular Fe Zhang, Yusheng verfasserin aut Liu, Amin verfasserin aut Zhu, Yuda verfasserin aut Chen, Suping verfasserin aut Wei, Dan verfasserin aut Sun, Jing verfasserin aut Guo, Zhenzhen verfasserin aut Fan, Hongsong verfasserin (orcid)0000-0003-3812-9208 aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 388 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:388 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 388 045F 660.05 |
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660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Photoluminescence-tunable carbon dots from synergy effect of sulfur doping and water engineering Carbon dots Tunable fluorescence Sulfur doping Water engineering Light-emitting diodes Intracellular Fe |
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Photoluminescence-tunable carbon dots from synergy effect of sulfur doping and water engineering |
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Photoluminescence-tunable carbon dots from synergy effect of sulfur doping and water engineering |
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Gao, Dong Zhang, Yusheng Liu, Amin Zhu, Yuda Chen, Suping Wei, Dan Sun, Jing Guo, Zhenzhen Fan, Hongsong |
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photoluminescence-tunable carbon dots from synergy effect of sulfur doping and water engineering |
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Photoluminescence-tunable carbon dots from synergy effect of sulfur doping and water engineering |
| abstract |
Multiple-color-emissive carbon dots (CDs) is one of the hotspots due to its potential in multi-fields. However, the exploring of efficient synthetic strategies and emission mechanisms still remain challenging. Herein, we report a facile solvothermal route to prepare CDs with tunable photoluminescence (PL) from green to red via a novel PL-tuning strategy of sulfur doping and water engineering. By detailed characterizations and comparison, it is demonstrated that the S doping can significantly increase the content of graphitic nitrogen, resulting in the fluorescence shifting from green to yellow; on the other hand, water engineering is able to yield carboxyl group and enhance surface oxidation degree, which can further facilitate the PL shifting from yellow to red. Owning to multicolor emissions and S doping, the prepared PL-tunable CDs present versatility in various applications including fluorescent films, light-emitting diodes (LED), bioimaging probe and highly sensitive Fe3+ detector. |
| abstractGer |
Multiple-color-emissive carbon dots (CDs) is one of the hotspots due to its potential in multi-fields. However, the exploring of efficient synthetic strategies and emission mechanisms still remain challenging. Herein, we report a facile solvothermal route to prepare CDs with tunable photoluminescence (PL) from green to red via a novel PL-tuning strategy of sulfur doping and water engineering. By detailed characterizations and comparison, it is demonstrated that the S doping can significantly increase the content of graphitic nitrogen, resulting in the fluorescence shifting from green to yellow; on the other hand, water engineering is able to yield carboxyl group and enhance surface oxidation degree, which can further facilitate the PL shifting from yellow to red. Owning to multicolor emissions and S doping, the prepared PL-tunable CDs present versatility in various applications including fluorescent films, light-emitting diodes (LED), bioimaging probe and highly sensitive Fe3+ detector. |
| abstract_unstemmed |
Multiple-color-emissive carbon dots (CDs) is one of the hotspots due to its potential in multi-fields. However, the exploring of efficient synthetic strategies and emission mechanisms still remain challenging. Herein, we report a facile solvothermal route to prepare CDs with tunable photoluminescence (PL) from green to red via a novel PL-tuning strategy of sulfur doping and water engineering. By detailed characterizations and comparison, it is demonstrated that the S doping can significantly increase the content of graphitic nitrogen, resulting in the fluorescence shifting from green to yellow; on the other hand, water engineering is able to yield carboxyl group and enhance surface oxidation degree, which can further facilitate the PL shifting from yellow to red. Owning to multicolor emissions and S doping, the prepared PL-tunable CDs present versatility in various applications including fluorescent films, light-emitting diodes (LED), bioimaging probe and highly sensitive Fe3+ detector. |
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