Occurrence of the insecticide fipronil and its degradates in indoor dust from South, Central, and North China

No known data are available regarding the occurrence of fipronil (FP) in indoor dust in China, despite the fact that it is an emerging insecticide that is used extensively. In this study, FP and its derivatives (FPs), including fipronil sulfone (FP-SFO), fipronil sulfide, fipronil desulfinyl, and fi...
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Autor*in:	Shi, Lisha [verfasserIn] Jiang, Ying [verfasserIn] Wan, Yanjian [verfasserIn] Huang, Juan [verfasserIn] Meng, Qianqian [verfasserIn] He, Zhenyu [verfasserIn] Xu, Shunqing [verfasserIn] Xia, Wei [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2020

Schlagwörter:	Fipronil Degradates Insecticide contamination Indoor dust Temporal variation Spatial variation

Übergeordnetes Werk:	Enthalten in: The science of the total environment - Amsterdam [u.a.] : Elsevier Science, 1972, 741
Übergeordnetes Werk:	volume:741

DOI / URN:	10.1016/j.scitotenv.2020.140110

Katalog-ID:	ELV004565762

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520			\|a No known data are available regarding the occurrence of fipronil (FP) in indoor dust in China, despite the fact that it is an emerging insecticide that is used extensively. In this study, FP and its derivatives (FPs), including fipronil sulfone (FP-SFO), fipronil sulfide, fipronil desulfinyl, and fipronil amide, were determined in indoor dust samples (n = 436) collected from three different cities in China between 2016 and 2019, namely Shenzhen (February and September 2019), Wuhan (October 2016, October 2018, and August 2019), and Taiyuan (October 2016), located in south, central, and north China, respectively. FP and FP-SFO were the major target analytes detected in all dust samples, accounting for approximately 68.6–90.1% of the cumulative concentration of FPs (ΣFPs). The ΣFPs values for the dust samples ranged from not detected (ND) to 33.6 μg/g (median ± median absolute deviation [MAD]: 7.12 ± 6.44 ng/g), with a detection frequency of 95.6%. The median value of the ΣFPs of the dust samples collected from Shenzhen (22.6 ± 15.6 ng/g) was higher than that found in the dust samples collected in Taiyuan 2016 (1.87 ± 1.65 ng/g) and Wuhan (6.43 ± 5.62 ng/g). Significantly higher ΣFPs were observed in the dust samples collected in urban areas than in the rural areas of Taiyuan and Wuhan. Furthermore, an increasing trend of FP (from 2016 to 2018) in the rural areas of Wuhan, and a seasonal variation (summer > autumn) in FP, FP-SFO, and ΣFPs in the dust samples from urban areas of Wuhan were observed. The estimated daily intake of FPs via dust ingestion for people in Shenzhen was approximately 12 times higher than in Taiyuan based on the samples analyzed. This is the first study to describe the occurrence and spatiotemporal variations of FPs in indoor dust in China.
650		4	\|a Fipronil
650		4	\|a Degradates
650		4	\|a Insecticide contamination
650		4	\|a Indoor dust
650		4	\|a Temporal variation
650		4	\|a Spatial variation
700	1		\|a Jiang, Ying \|e verfasserin \|4 aut
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700	1		\|a Meng, Qianqian \|e verfasserin \|4 aut
700	1		\|a He, Zhenyu \|e verfasserin \|4 aut
700	1		\|a Xu, Shunqing \|e verfasserin \|4 aut
700	1		\|a Xia, Wei \|e verfasserin \|4 aut
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936	b	k	\|a 43.12 \|j Umweltchemie
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Indexfelder

author_variant	l s ls y j yj y w yw j h jh q m qm z h zh s x sx w x wx
matchkey_str	article:18791026:2020----::curnefhisciieirnlniserdtsnnorutrm
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publishDate	2020
allfields	10.1016/j.scitotenv.2020.140110 doi (DE-627)ELV004565762 (ELSEVIER)S0048-9697(20)33631-7 DE-627 ger DE-627 rda eng 333.7 610 DE-600 43.12 bkl 43.13 bkl 44.13 bkl Shi, Lisha verfasserin aut Occurrence of the insecticide fipronil and its degradates in indoor dust from South, Central, and North China 2020 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier No known data are available regarding the occurrence of fipronil (FP) in indoor dust in China, despite the fact that it is an emerging insecticide that is used extensively. In this study, FP and its derivatives (FPs), including fipronil sulfone (FP-SFO), fipronil sulfide, fipronil desulfinyl, and fipronil amide, were determined in indoor dust samples (n = 436) collected from three different cities in China between 2016 and 2019, namely Shenzhen (February and September 2019), Wuhan (October 2016, October 2018, and August 2019), and Taiyuan (October 2016), located in south, central, and north China, respectively. FP and FP-SFO were the major target analytes detected in all dust samples, accounting for approximately 68.6–90.1% of the cumulative concentration of FPs (ΣFPs). The ΣFPs values for the dust samples ranged from not detected (ND) to 33.6 μg/g (median ± median absolute deviation [MAD]: 7.12 ± 6.44 ng/g), with a detection frequency of 95.6%. The median value of the ΣFPs of the dust samples collected from Shenzhen (22.6 ± 15.6 ng/g) was higher than that found in the dust samples collected in Taiyuan 2016 (1.87 ± 1.65 ng/g) and Wuhan (6.43 ± 5.62 ng/g). Significantly higher ΣFPs were observed in the dust samples collected in urban areas than in the rural areas of Taiyuan and Wuhan. Furthermore, an increasing trend of FP (from 2016 to 2018) in the rural areas of Wuhan, and a seasonal variation (summer > autumn) in FP, FP-SFO, and ΣFPs in the dust samples from urban areas of Wuhan were observed. The estimated daily intake of FPs via dust ingestion for people in Shenzhen was approximately 12 times higher than in Taiyuan based on the samples analyzed. This is the first study to describe the occurrence and spatiotemporal variations of FPs in indoor dust in China. Fipronil Degradates Insecticide contamination Indoor dust Temporal variation Spatial variation Jiang, Ying verfasserin aut Wan, Yanjian verfasserin aut Huang, Juan verfasserin aut Meng, Qianqian verfasserin aut He, Zhenyu verfasserin aut Xu, Shunqing verfasserin aut Xia, Wei verfasserin aut Enthalten in The science of the total environment Amsterdam [u.a.] : Elsevier Science, 1972 741 Online-Ressource (DE-627)306591456 (DE-600)1498726-0 (DE-576)081953178 1879-1026 nnns volume:741 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA SSG-OPC-GGO GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 43.12 Umweltchemie 43.13 Umwelttoxikologie 44.13 Medizinische Ökologie AR 741
spelling	10.1016/j.scitotenv.2020.140110 doi (DE-627)ELV004565762 (ELSEVIER)S0048-9697(20)33631-7 DE-627 ger DE-627 rda eng 333.7 610 DE-600 43.12 bkl 43.13 bkl 44.13 bkl Shi, Lisha verfasserin aut Occurrence of the insecticide fipronil and its degradates in indoor dust from South, Central, and North China 2020 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier No known data are available regarding the occurrence of fipronil (FP) in indoor dust in China, despite the fact that it is an emerging insecticide that is used extensively. In this study, FP and its derivatives (FPs), including fipronil sulfone (FP-SFO), fipronil sulfide, fipronil desulfinyl, and fipronil amide, were determined in indoor dust samples (n = 436) collected from three different cities in China between 2016 and 2019, namely Shenzhen (February and September 2019), Wuhan (October 2016, October 2018, and August 2019), and Taiyuan (October 2016), located in south, central, and north China, respectively. FP and FP-SFO were the major target analytes detected in all dust samples, accounting for approximately 68.6–90.1% of the cumulative concentration of FPs (ΣFPs). The ΣFPs values for the dust samples ranged from not detected (ND) to 33.6 μg/g (median ± median absolute deviation [MAD]: 7.12 ± 6.44 ng/g), with a detection frequency of 95.6%. The median value of the ΣFPs of the dust samples collected from Shenzhen (22.6 ± 15.6 ng/g) was higher than that found in the dust samples collected in Taiyuan 2016 (1.87 ± 1.65 ng/g) and Wuhan (6.43 ± 5.62 ng/g). Significantly higher ΣFPs were observed in the dust samples collected in urban areas than in the rural areas of Taiyuan and Wuhan. Furthermore, an increasing trend of FP (from 2016 to 2018) in the rural areas of Wuhan, and a seasonal variation (summer > autumn) in FP, FP-SFO, and ΣFPs in the dust samples from urban areas of Wuhan were observed. The estimated daily intake of FPs via dust ingestion for people in Shenzhen was approximately 12 times higher than in Taiyuan based on the samples analyzed. This is the first study to describe the occurrence and spatiotemporal variations of FPs in indoor dust in China. Fipronil Degradates Insecticide contamination Indoor dust Temporal variation Spatial variation Jiang, Ying verfasserin aut Wan, Yanjian verfasserin aut Huang, Juan verfasserin aut Meng, Qianqian verfasserin aut He, Zhenyu verfasserin aut Xu, Shunqing verfasserin aut Xia, Wei verfasserin aut Enthalten in The science of the total environment Amsterdam [u.a.] : Elsevier Science, 1972 741 Online-Ressource (DE-627)306591456 (DE-600)1498726-0 (DE-576)081953178 1879-1026 nnns volume:741 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA SSG-OPC-GGO GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 43.12 Umweltchemie 43.13 Umwelttoxikologie 44.13 Medizinische Ökologie AR 741
allfields_unstemmed	10.1016/j.scitotenv.2020.140110 doi (DE-627)ELV004565762 (ELSEVIER)S0048-9697(20)33631-7 DE-627 ger DE-627 rda eng 333.7 610 DE-600 43.12 bkl 43.13 bkl 44.13 bkl Shi, Lisha verfasserin aut Occurrence of the insecticide fipronil and its degradates in indoor dust from South, Central, and North China 2020 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier No known data are available regarding the occurrence of fipronil (FP) in indoor dust in China, despite the fact that it is an emerging insecticide that is used extensively. In this study, FP and its derivatives (FPs), including fipronil sulfone (FP-SFO), fipronil sulfide, fipronil desulfinyl, and fipronil amide, were determined in indoor dust samples (n = 436) collected from three different cities in China between 2016 and 2019, namely Shenzhen (February and September 2019), Wuhan (October 2016, October 2018, and August 2019), and Taiyuan (October 2016), located in south, central, and north China, respectively. FP and FP-SFO were the major target analytes detected in all dust samples, accounting for approximately 68.6–90.1% of the cumulative concentration of FPs (ΣFPs). The ΣFPs values for the dust samples ranged from not detected (ND) to 33.6 μg/g (median ± median absolute deviation [MAD]: 7.12 ± 6.44 ng/g), with a detection frequency of 95.6%. The median value of the ΣFPs of the dust samples collected from Shenzhen (22.6 ± 15.6 ng/g) was higher than that found in the dust samples collected in Taiyuan 2016 (1.87 ± 1.65 ng/g) and Wuhan (6.43 ± 5.62 ng/g). Significantly higher ΣFPs were observed in the dust samples collected in urban areas than in the rural areas of Taiyuan and Wuhan. Furthermore, an increasing trend of FP (from 2016 to 2018) in the rural areas of Wuhan, and a seasonal variation (summer > autumn) in FP, FP-SFO, and ΣFPs in the dust samples from urban areas of Wuhan were observed. The estimated daily intake of FPs via dust ingestion for people in Shenzhen was approximately 12 times higher than in Taiyuan based on the samples analyzed. This is the first study to describe the occurrence and spatiotemporal variations of FPs in indoor dust in China. Fipronil Degradates Insecticide contamination Indoor dust Temporal variation Spatial variation Jiang, Ying verfasserin aut Wan, Yanjian verfasserin aut Huang, Juan verfasserin aut Meng, Qianqian verfasserin aut He, Zhenyu verfasserin aut Xu, Shunqing verfasserin aut Xia, Wei verfasserin aut Enthalten in The science of the total environment Amsterdam [u.a.] : Elsevier Science, 1972 741 Online-Ressource (DE-627)306591456 (DE-600)1498726-0 (DE-576)081953178 1879-1026 nnns volume:741 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA SSG-OPC-GGO GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 43.12 Umweltchemie 43.13 Umwelttoxikologie 44.13 Medizinische Ökologie AR 741
allfieldsGer	10.1016/j.scitotenv.2020.140110 doi (DE-627)ELV004565762 (ELSEVIER)S0048-9697(20)33631-7 DE-627 ger DE-627 rda eng 333.7 610 DE-600 43.12 bkl 43.13 bkl 44.13 bkl Shi, Lisha verfasserin aut Occurrence of the insecticide fipronil and its degradates in indoor dust from South, Central, and North China 2020 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier No known data are available regarding the occurrence of fipronil (FP) in indoor dust in China, despite the fact that it is an emerging insecticide that is used extensively. In this study, FP and its derivatives (FPs), including fipronil sulfone (FP-SFO), fipronil sulfide, fipronil desulfinyl, and fipronil amide, were determined in indoor dust samples (n = 436) collected from three different cities in China between 2016 and 2019, namely Shenzhen (February and September 2019), Wuhan (October 2016, October 2018, and August 2019), and Taiyuan (October 2016), located in south, central, and north China, respectively. FP and FP-SFO were the major target analytes detected in all dust samples, accounting for approximately 68.6–90.1% of the cumulative concentration of FPs (ΣFPs). The ΣFPs values for the dust samples ranged from not detected (ND) to 33.6 μg/g (median ± median absolute deviation [MAD]: 7.12 ± 6.44 ng/g), with a detection frequency of 95.6%. The median value of the ΣFPs of the dust samples collected from Shenzhen (22.6 ± 15.6 ng/g) was higher than that found in the dust samples collected in Taiyuan 2016 (1.87 ± 1.65 ng/g) and Wuhan (6.43 ± 5.62 ng/g). Significantly higher ΣFPs were observed in the dust samples collected in urban areas than in the rural areas of Taiyuan and Wuhan. Furthermore, an increasing trend of FP (from 2016 to 2018) in the rural areas of Wuhan, and a seasonal variation (summer > autumn) in FP, FP-SFO, and ΣFPs in the dust samples from urban areas of Wuhan were observed. The estimated daily intake of FPs via dust ingestion for people in Shenzhen was approximately 12 times higher than in Taiyuan based on the samples analyzed. This is the first study to describe the occurrence and spatiotemporal variations of FPs in indoor dust in China. Fipronil Degradates Insecticide contamination Indoor dust Temporal variation Spatial variation Jiang, Ying verfasserin aut Wan, Yanjian verfasserin aut Huang, Juan verfasserin aut Meng, Qianqian verfasserin aut He, Zhenyu verfasserin aut Xu, Shunqing verfasserin aut Xia, Wei verfasserin aut Enthalten in The science of the total environment Amsterdam [u.a.] : Elsevier Science, 1972 741 Online-Ressource (DE-627)306591456 (DE-600)1498726-0 (DE-576)081953178 1879-1026 nnns volume:741 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA SSG-OPC-GGO GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 43.12 Umweltchemie 43.13 Umwelttoxikologie 44.13 Medizinische Ökologie AR 741
allfieldsSound	10.1016/j.scitotenv.2020.140110 doi (DE-627)ELV004565762 (ELSEVIER)S0048-9697(20)33631-7 DE-627 ger DE-627 rda eng 333.7 610 DE-600 43.12 bkl 43.13 bkl 44.13 bkl Shi, Lisha verfasserin aut Occurrence of the insecticide fipronil and its degradates in indoor dust from South, Central, and North China 2020 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier No known data are available regarding the occurrence of fipronil (FP) in indoor dust in China, despite the fact that it is an emerging insecticide that is used extensively. In this study, FP and its derivatives (FPs), including fipronil sulfone (FP-SFO), fipronil sulfide, fipronil desulfinyl, and fipronil amide, were determined in indoor dust samples (n = 436) collected from three different cities in China between 2016 and 2019, namely Shenzhen (February and September 2019), Wuhan (October 2016, October 2018, and August 2019), and Taiyuan (October 2016), located in south, central, and north China, respectively. FP and FP-SFO were the major target analytes detected in all dust samples, accounting for approximately 68.6–90.1% of the cumulative concentration of FPs (ΣFPs). The ΣFPs values for the dust samples ranged from not detected (ND) to 33.6 μg/g (median ± median absolute deviation [MAD]: 7.12 ± 6.44 ng/g), with a detection frequency of 95.6%. The median value of the ΣFPs of the dust samples collected from Shenzhen (22.6 ± 15.6 ng/g) was higher than that found in the dust samples collected in Taiyuan 2016 (1.87 ± 1.65 ng/g) and Wuhan (6.43 ± 5.62 ng/g). Significantly higher ΣFPs were observed in the dust samples collected in urban areas than in the rural areas of Taiyuan and Wuhan. Furthermore, an increasing trend of FP (from 2016 to 2018) in the rural areas of Wuhan, and a seasonal variation (summer > autumn) in FP, FP-SFO, and ΣFPs in the dust samples from urban areas of Wuhan were observed. The estimated daily intake of FPs via dust ingestion for people in Shenzhen was approximately 12 times higher than in Taiyuan based on the samples analyzed. This is the first study to describe the occurrence and spatiotemporal variations of FPs in indoor dust in China. Fipronil Degradates Insecticide contamination Indoor dust Temporal variation Spatial variation Jiang, Ying verfasserin aut Wan, Yanjian verfasserin aut Huang, Juan verfasserin aut Meng, Qianqian verfasserin aut He, Zhenyu verfasserin aut Xu, Shunqing verfasserin aut Xia, Wei verfasserin aut Enthalten in The science of the total environment Amsterdam [u.a.] : Elsevier Science, 1972 741 Online-Ressource (DE-627)306591456 (DE-600)1498726-0 (DE-576)081953178 1879-1026 nnns volume:741 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA SSG-OPC-GGO GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 43.12 Umweltchemie 43.13 Umwelttoxikologie 44.13 Medizinische Ökologie AR 741
language	English
source	Enthalten in The science of the total environment 741 volume:741
sourceStr	Enthalten in The science of the total environment 741 volume:741
format_phy_str_mv	Article
bklname	Umweltchemie Umwelttoxikologie Medizinische Ökologie
institution	findex.gbv.de
topic_facet	Fipronil Degradates Insecticide contamination Indoor dust Temporal variation Spatial variation
dewey-raw	333.7
isfreeaccess_bool	false
container_title	The science of the total environment
authorswithroles_txt_mv	Shi, Lisha @@aut@@ Jiang, Ying @@aut@@ Wan, Yanjian @@aut@@ Huang, Juan @@aut@@ Meng, Qianqian @@aut@@ He, Zhenyu @@aut@@ Xu, Shunqing @@aut@@ Xia, Wei @@aut@@
publishDateDaySort_date	2020-01-01T00:00:00Z
hierarchy_top_id	306591456
dewey-sort	3333.7
id	ELV004565762
language_de	englisch
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author	Shi, Lisha
spellingShingle	Shi, Lisha ddc 333.7 bkl 43.12 bkl 43.13 bkl 44.13 misc Fipronil misc Degradates misc Insecticide contamination misc Indoor dust misc Temporal variation misc Spatial variation Occurrence of the insecticide fipronil and its degradates in indoor dust from South, Central, and North China
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topic_title	333.7 610 DE-600 43.12 bkl 43.13 bkl 44.13 bkl Occurrence of the insecticide fipronil and its degradates in indoor dust from South, Central, and North China Fipronil Degradates Insecticide contamination Indoor dust Temporal variation Spatial variation
topic	ddc 333.7 bkl 43.12 bkl 43.13 bkl 44.13 misc Fipronil misc Degradates misc Insecticide contamination misc Indoor dust misc Temporal variation misc Spatial variation
topic_unstemmed	ddc 333.7 bkl 43.12 bkl 43.13 bkl 44.13 misc Fipronil misc Degradates misc Insecticide contamination misc Indoor dust misc Temporal variation misc Spatial variation
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title	Occurrence of the insecticide fipronil and its degradates in indoor dust from South, Central, and North China
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title_full	Occurrence of the insecticide fipronil and its degradates in indoor dust from South, Central, and North China
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title_sort	occurrence of the insecticide fipronil and its degradates in indoor dust from south, central, and north china
title_auth	Occurrence of the insecticide fipronil and its degradates in indoor dust from South, Central, and North China
abstract	No known data are available regarding the occurrence of fipronil (FP) in indoor dust in China, despite the fact that it is an emerging insecticide that is used extensively. In this study, FP and its derivatives (FPs), including fipronil sulfone (FP-SFO), fipronil sulfide, fipronil desulfinyl, and fipronil amide, were determined in indoor dust samples (n = 436) collected from three different cities in China between 2016 and 2019, namely Shenzhen (February and September 2019), Wuhan (October 2016, October 2018, and August 2019), and Taiyuan (October 2016), located in south, central, and north China, respectively. FP and FP-SFO were the major target analytes detected in all dust samples, accounting for approximately 68.6–90.1% of the cumulative concentration of FPs (ΣFPs). The ΣFPs values for the dust samples ranged from not detected (ND) to 33.6 μg/g (median ± median absolute deviation [MAD]: 7.12 ± 6.44 ng/g), with a detection frequency of 95.6%. The median value of the ΣFPs of the dust samples collected from Shenzhen (22.6 ± 15.6 ng/g) was higher than that found in the dust samples collected in Taiyuan 2016 (1.87 ± 1.65 ng/g) and Wuhan (6.43 ± 5.62 ng/g). Significantly higher ΣFPs were observed in the dust samples collected in urban areas than in the rural areas of Taiyuan and Wuhan. Furthermore, an increasing trend of FP (from 2016 to 2018) in the rural areas of Wuhan, and a seasonal variation (summer > autumn) in FP, FP-SFO, and ΣFPs in the dust samples from urban areas of Wuhan were observed. The estimated daily intake of FPs via dust ingestion for people in Shenzhen was approximately 12 times higher than in Taiyuan based on the samples analyzed. This is the first study to describe the occurrence and spatiotemporal variations of FPs in indoor dust in China.
abstractGer	No known data are available regarding the occurrence of fipronil (FP) in indoor dust in China, despite the fact that it is an emerging insecticide that is used extensively. In this study, FP and its derivatives (FPs), including fipronil sulfone (FP-SFO), fipronil sulfide, fipronil desulfinyl, and fipronil amide, were determined in indoor dust samples (n = 436) collected from three different cities in China between 2016 and 2019, namely Shenzhen (February and September 2019), Wuhan (October 2016, October 2018, and August 2019), and Taiyuan (October 2016), located in south, central, and north China, respectively. FP and FP-SFO were the major target analytes detected in all dust samples, accounting for approximately 68.6–90.1% of the cumulative concentration of FPs (ΣFPs). The ΣFPs values for the dust samples ranged from not detected (ND) to 33.6 μg/g (median ± median absolute deviation [MAD]: 7.12 ± 6.44 ng/g), with a detection frequency of 95.6%. The median value of the ΣFPs of the dust samples collected from Shenzhen (22.6 ± 15.6 ng/g) was higher than that found in the dust samples collected in Taiyuan 2016 (1.87 ± 1.65 ng/g) and Wuhan (6.43 ± 5.62 ng/g). Significantly higher ΣFPs were observed in the dust samples collected in urban areas than in the rural areas of Taiyuan and Wuhan. Furthermore, an increasing trend of FP (from 2016 to 2018) in the rural areas of Wuhan, and a seasonal variation (summer > autumn) in FP, FP-SFO, and ΣFPs in the dust samples from urban areas of Wuhan were observed. The estimated daily intake of FPs via dust ingestion for people in Shenzhen was approximately 12 times higher than in Taiyuan based on the samples analyzed. This is the first study to describe the occurrence and spatiotemporal variations of FPs in indoor dust in China.
abstract_unstemmed	No known data are available regarding the occurrence of fipronil (FP) in indoor dust in China, despite the fact that it is an emerging insecticide that is used extensively. In this study, FP and its derivatives (FPs), including fipronil sulfone (FP-SFO), fipronil sulfide, fipronil desulfinyl, and fipronil amide, were determined in indoor dust samples (n = 436) collected from three different cities in China between 2016 and 2019, namely Shenzhen (February and September 2019), Wuhan (October 2016, October 2018, and August 2019), and Taiyuan (October 2016), located in south, central, and north China, respectively. FP and FP-SFO were the major target analytes detected in all dust samples, accounting for approximately 68.6–90.1% of the cumulative concentration of FPs (ΣFPs). The ΣFPs values for the dust samples ranged from not detected (ND) to 33.6 μg/g (median ± median absolute deviation [MAD]: 7.12 ± 6.44 ng/g), with a detection frequency of 95.6%. The median value of the ΣFPs of the dust samples collected from Shenzhen (22.6 ± 15.6 ng/g) was higher than that found in the dust samples collected in Taiyuan 2016 (1.87 ± 1.65 ng/g) and Wuhan (6.43 ± 5.62 ng/g). Significantly higher ΣFPs were observed in the dust samples collected in urban areas than in the rural areas of Taiyuan and Wuhan. Furthermore, an increasing trend of FP (from 2016 to 2018) in the rural areas of Wuhan, and a seasonal variation (summer > autumn) in FP, FP-SFO, and ΣFPs in the dust samples from urban areas of Wuhan were observed. The estimated daily intake of FPs via dust ingestion for people in Shenzhen was approximately 12 times higher than in Taiyuan based on the samples analyzed. This is the first study to describe the occurrence and spatiotemporal variations of FPs in indoor dust in China.
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title_short	Occurrence of the insecticide fipronil and its degradates in indoor dust from South, Central, and North China
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author2	Jiang, Ying Wan, Yanjian Huang, Juan Meng, Qianqian He, Zhenyu Xu, Shunqing Xia, Wei
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up_date	2024-07-06T23:25:20.899Z
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fullrecord_marcxml	<?xml version="1.0" encoding="UTF-8"?><collection xmlns="http://www.loc.gov/MARC21/slim"><record><leader>01000caa a22002652 4500</leader><controlfield tag="001">ELV004565762</controlfield><controlfield tag="003">DE-627</controlfield><controlfield tag="005">20230524140457.0</controlfield><controlfield tag="007">cr uuu---uuuuu</controlfield><controlfield tag="008">230502s2020 xx \|\|\|\|\|o 00\| \|\|eng c</controlfield><datafield tag="024" ind1="7" ind2=" "><subfield code="a">10.1016/j.scitotenv.2020.140110</subfield><subfield code="2">doi</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(DE-627)ELV004565762</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(ELSEVIER)S0048-9697(20)33631-7</subfield></datafield><datafield tag="040" ind1=" " ind2=" "><subfield code="a">DE-627</subfield><subfield code="b">ger</subfield><subfield code="c">DE-627</subfield><subfield code="e">rda</subfield></datafield><datafield tag="041" ind1=" " ind2=" "><subfield code="a">eng</subfield></datafield><datafield tag="082" ind1="0" ind2="4"><subfield code="a">333.7</subfield><subfield code="a">610</subfield><subfield code="q">DE-600</subfield></datafield><datafield tag="084" ind1=" " ind2=" "><subfield code="a">43.12</subfield><subfield code="2">bkl</subfield></datafield><datafield tag="084" ind1=" " ind2=" "><subfield code="a">43.13</subfield><subfield code="2">bkl</subfield></datafield><datafield tag="084" ind1=" " ind2=" "><subfield code="a">44.13</subfield><subfield code="2">bkl</subfield></datafield><datafield tag="100" ind1="1" ind2=" "><subfield code="a">Shi, Lisha</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="245" ind1="1" ind2="0"><subfield code="a">Occurrence of the insecticide fipronil and its degradates in indoor dust from South, Central, and North China</subfield></datafield><datafield tag="264" ind1=" " ind2="1"><subfield code="c">2020</subfield></datafield><datafield tag="336" ind1=" " ind2=" "><subfield code="a">nicht spezifiziert</subfield><subfield code="b">zzz</subfield><subfield code="2">rdacontent</subfield></datafield><datafield tag="337" ind1=" " ind2=" "><subfield code="a">Computermedien</subfield><subfield code="b">c</subfield><subfield code="2">rdamedia</subfield></datafield><datafield tag="338" ind1=" " ind2=" "><subfield code="a">Online-Ressource</subfield><subfield code="b">cr</subfield><subfield code="2">rdacarrier</subfield></datafield><datafield tag="520" ind1=" " ind2=" "><subfield code="a">No known data are available regarding the occurrence of fipronil (FP) in indoor dust in China, despite the fact that it is an emerging insecticide that is used extensively. In this study, FP and its derivatives (FPs), including fipronil sulfone (FP-SFO), fipronil sulfide, fipronil desulfinyl, and fipronil amide, were determined in indoor dust samples (n = 436) collected from three different cities in China between 2016 and 2019, namely Shenzhen (February and September 2019), Wuhan (October 2016, October 2018, and August 2019), and Taiyuan (October 2016), located in south, central, and north China, respectively. FP and FP-SFO were the major target analytes detected in all dust samples, accounting for approximately 68.6–90.1% of the cumulative concentration of FPs (ΣFPs). The ΣFPs values for the dust samples ranged from not detected (ND) to 33.6 μg/g (median ± median absolute deviation [MAD]: 7.12 ± 6.44 ng/g), with a detection frequency of 95.6%. The median value of the ΣFPs of the dust samples collected from Shenzhen (22.6 ± 15.6 ng/g) was higher than that found in the dust samples collected in Taiyuan 2016 (1.87 ± 1.65 ng/g) and Wuhan (6.43 ± 5.62 ng/g). Significantly higher ΣFPs were observed in the dust samples collected in urban areas than in the rural areas of Taiyuan and Wuhan. Furthermore, an increasing trend of FP (from 2016 to 2018) in the rural areas of Wuhan, and a seasonal variation (summer > autumn) in FP, FP-SFO, and ΣFPs in the dust samples from urban areas of Wuhan were observed. The estimated daily intake of FPs via dust ingestion for people in Shenzhen was approximately 12 times higher than in Taiyuan based on the samples analyzed. 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Occurrence of the insecticide fipronil and its degradates in indoor dust from South, Central, and North China

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