A robust indium(III)−potassium(I) MOF with high CO
A heterometallic MOF, [NH2(Me)2]5[K3In8L8(H2O)6]·13DMA·12H2O (1), has been synthesized under solvothermal conditions by employing a pyridyl-decorated tetracarboxylate ligand, 2,2′-(pyridine-2,5-diyl)diterephthalic acid (H4L). Structural analysis demonstrates that 1 is a 3D microporous framework base...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Jiang, Tiantian [verfasserIn] Zhang, Bin [verfasserIn] Zhou, Huifang [verfasserIn] Wang, Weize [verfasserIn] Liu, Bo [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2020 |
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| Schlagwörter: |
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| Übergeordnetes Werk: |
Enthalten in: Journal of solid state chemistry - Orlando, Fla. : Academic Press, 1969, 292 |
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| Übergeordnetes Werk: |
volume:292 |
| DOI / URN: |
10.1016/j.jssc.2020.121726 |
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| Katalog-ID: |
ELV004908864 |
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| 024 | 7 | |a 10.1016/j.jssc.2020.121726 |2 doi | |
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| 245 | 1 | 0 | |a A robust indium(III)−potassium(I) MOF with high CO |
| 264 | 1 | |c 2020 | |
| 336 | |a nicht spezifiziert |b zzz |2 rdacontent | ||
| 337 | |a Computermedien |b c |2 rdamedia | ||
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| 520 | |a A heterometallic MOF, [NH2(Me)2]5[K3In8L8(H2O)6]·13DMA·12H2O (1), has been synthesized under solvothermal conditions by employing a pyridyl-decorated tetracarboxylate ligand, 2,2′-(pyridine-2,5-diyl)diterephthalic acid (H4L). Structural analysis demonstrates that 1 is a 3D microporous framework based on three kinds of inorganic secondary building units (SBUs), which shows an unprecedented 5-nodal (3,4,4,7,7)-connected topology. Especially, 1 possesses high chemical stability in pH = 2–13 aqueous solutions. The desolvated structure of 1 contains a highly polar pore system decorated with open metal sites, diethylammonium cations, and free pyridine atoms, leading to a high CO2/C2-hydrocarbons over CH4 separation performance. | ||
| 650 | 4 | |a Metal-organic framework | |
| 650 | 4 | |a Crystal structure | |
| 650 | 4 | |a Gas adsorption | |
| 650 | 4 | |a Separation | |
| 650 | 4 | |a Robust | |
| 700 | 1 | |a Zhang, Bin |e verfasserin |4 aut | |
| 700 | 1 | |a Zhou, Huifang |e verfasserin |4 aut | |
| 700 | 1 | |a Wang, Weize |e verfasserin |4 aut | |
| 700 | 1 | |a Liu, Bo |e verfasserin |4 aut | |
| 773 | 0 | 8 | |i Enthalten in |t Journal of solid state chemistry |d Orlando, Fla. : Academic Press, 1969 |g 292 |h Online-Ressource |w (DE-627)267328451 |w (DE-600)1469806-7 |w (DE-576)10337325X |7 nnns |
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2020 |
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35.90 |
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2020 |
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10.1016/j.jssc.2020.121726 doi (DE-627)ELV004908864 (ELSEVIER)S0022-4596(20)30556-9 DE-627 ger DE-627 rda eng 540 DE-600 35.90 bkl Jiang, Tiantian verfasserin aut A robust indium(III)−potassium(I) MOF with high CO 2020 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A heterometallic MOF, [NH2(Me)2]5[K3In8L8(H2O)6]·13DMA·12H2O (1), has been synthesized under solvothermal conditions by employing a pyridyl-decorated tetracarboxylate ligand, 2,2′-(pyridine-2,5-diyl)diterephthalic acid (H4L). Structural analysis demonstrates that 1 is a 3D microporous framework based on three kinds of inorganic secondary building units (SBUs), which shows an unprecedented 5-nodal (3,4,4,7,7)-connected topology. Especially, 1 possesses high chemical stability in pH = 2–13 aqueous solutions. The desolvated structure of 1 contains a highly polar pore system decorated with open metal sites, diethylammonium cations, and free pyridine atoms, leading to a high CO2/C2-hydrocarbons over CH4 separation performance. Metal-organic framework Crystal structure Gas adsorption Separation Robust Zhang, Bin verfasserin aut Zhou, Huifang verfasserin aut Wang, Weize verfasserin aut Liu, Bo verfasserin aut Enthalten in Journal of solid state chemistry Orlando, Fla. : Academic Press, 1969 292 Online-Ressource (DE-627)267328451 (DE-600)1469806-7 (DE-576)10337325X nnns volume:292 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.90 Festkörperchemie AR 292 |
| spelling |
10.1016/j.jssc.2020.121726 doi (DE-627)ELV004908864 (ELSEVIER)S0022-4596(20)30556-9 DE-627 ger DE-627 rda eng 540 DE-600 35.90 bkl Jiang, Tiantian verfasserin aut A robust indium(III)−potassium(I) MOF with high CO 2020 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A heterometallic MOF, [NH2(Me)2]5[K3In8L8(H2O)6]·13DMA·12H2O (1), has been synthesized under solvothermal conditions by employing a pyridyl-decorated tetracarboxylate ligand, 2,2′-(pyridine-2,5-diyl)diterephthalic acid (H4L). Structural analysis demonstrates that 1 is a 3D microporous framework based on three kinds of inorganic secondary building units (SBUs), which shows an unprecedented 5-nodal (3,4,4,7,7)-connected topology. Especially, 1 possesses high chemical stability in pH = 2–13 aqueous solutions. The desolvated structure of 1 contains a highly polar pore system decorated with open metal sites, diethylammonium cations, and free pyridine atoms, leading to a high CO2/C2-hydrocarbons over CH4 separation performance. Metal-organic framework Crystal structure Gas adsorption Separation Robust Zhang, Bin verfasserin aut Zhou, Huifang verfasserin aut Wang, Weize verfasserin aut Liu, Bo verfasserin aut Enthalten in Journal of solid state chemistry Orlando, Fla. : Academic Press, 1969 292 Online-Ressource (DE-627)267328451 (DE-600)1469806-7 (DE-576)10337325X nnns volume:292 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.90 Festkörperchemie AR 292 |
| allfields_unstemmed |
10.1016/j.jssc.2020.121726 doi (DE-627)ELV004908864 (ELSEVIER)S0022-4596(20)30556-9 DE-627 ger DE-627 rda eng 540 DE-600 35.90 bkl Jiang, Tiantian verfasserin aut A robust indium(III)−potassium(I) MOF with high CO 2020 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A heterometallic MOF, [NH2(Me)2]5[K3In8L8(H2O)6]·13DMA·12H2O (1), has been synthesized under solvothermal conditions by employing a pyridyl-decorated tetracarboxylate ligand, 2,2′-(pyridine-2,5-diyl)diterephthalic acid (H4L). Structural analysis demonstrates that 1 is a 3D microporous framework based on three kinds of inorganic secondary building units (SBUs), which shows an unprecedented 5-nodal (3,4,4,7,7)-connected topology. Especially, 1 possesses high chemical stability in pH = 2–13 aqueous solutions. The desolvated structure of 1 contains a highly polar pore system decorated with open metal sites, diethylammonium cations, and free pyridine atoms, leading to a high CO2/C2-hydrocarbons over CH4 separation performance. Metal-organic framework Crystal structure Gas adsorption Separation Robust Zhang, Bin verfasserin aut Zhou, Huifang verfasserin aut Wang, Weize verfasserin aut Liu, Bo verfasserin aut Enthalten in Journal of solid state chemistry Orlando, Fla. : Academic Press, 1969 292 Online-Ressource (DE-627)267328451 (DE-600)1469806-7 (DE-576)10337325X nnns volume:292 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.90 Festkörperchemie AR 292 |
| allfieldsGer |
10.1016/j.jssc.2020.121726 doi (DE-627)ELV004908864 (ELSEVIER)S0022-4596(20)30556-9 DE-627 ger DE-627 rda eng 540 DE-600 35.90 bkl Jiang, Tiantian verfasserin aut A robust indium(III)−potassium(I) MOF with high CO 2020 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A heterometallic MOF, [NH2(Me)2]5[K3In8L8(H2O)6]·13DMA·12H2O (1), has been synthesized under solvothermal conditions by employing a pyridyl-decorated tetracarboxylate ligand, 2,2′-(pyridine-2,5-diyl)diterephthalic acid (H4L). Structural analysis demonstrates that 1 is a 3D microporous framework based on three kinds of inorganic secondary building units (SBUs), which shows an unprecedented 5-nodal (3,4,4,7,7)-connected topology. Especially, 1 possesses high chemical stability in pH = 2–13 aqueous solutions. The desolvated structure of 1 contains a highly polar pore system decorated with open metal sites, diethylammonium cations, and free pyridine atoms, leading to a high CO2/C2-hydrocarbons over CH4 separation performance. Metal-organic framework Crystal structure Gas adsorption Separation Robust Zhang, Bin verfasserin aut Zhou, Huifang verfasserin aut Wang, Weize verfasserin aut Liu, Bo verfasserin aut Enthalten in Journal of solid state chemistry Orlando, Fla. : Academic Press, 1969 292 Online-Ressource (DE-627)267328451 (DE-600)1469806-7 (DE-576)10337325X nnns volume:292 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.90 Festkörperchemie AR 292 |
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a robust indium(iii)−potassium(i) mof with high co |
| title_auth |
A robust indium(III)−potassium(I) MOF with high CO |
| abstract |
A heterometallic MOF, [NH2(Me)2]5[K3In8L8(H2O)6]·13DMA·12H2O (1), has been synthesized under solvothermal conditions by employing a pyridyl-decorated tetracarboxylate ligand, 2,2′-(pyridine-2,5-diyl)diterephthalic acid (H4L). Structural analysis demonstrates that 1 is a 3D microporous framework based on three kinds of inorganic secondary building units (SBUs), which shows an unprecedented 5-nodal (3,4,4,7,7)-connected topology. Especially, 1 possesses high chemical stability in pH = 2–13 aqueous solutions. The desolvated structure of 1 contains a highly polar pore system decorated with open metal sites, diethylammonium cations, and free pyridine atoms, leading to a high CO2/C2-hydrocarbons over CH4 separation performance. |
| abstractGer |
A heterometallic MOF, [NH2(Me)2]5[K3In8L8(H2O)6]·13DMA·12H2O (1), has been synthesized under solvothermal conditions by employing a pyridyl-decorated tetracarboxylate ligand, 2,2′-(pyridine-2,5-diyl)diterephthalic acid (H4L). Structural analysis demonstrates that 1 is a 3D microporous framework based on three kinds of inorganic secondary building units (SBUs), which shows an unprecedented 5-nodal (3,4,4,7,7)-connected topology. Especially, 1 possesses high chemical stability in pH = 2–13 aqueous solutions. The desolvated structure of 1 contains a highly polar pore system decorated with open metal sites, diethylammonium cations, and free pyridine atoms, leading to a high CO2/C2-hydrocarbons over CH4 separation performance. |
| abstract_unstemmed |
A heterometallic MOF, [NH2(Me)2]5[K3In8L8(H2O)6]·13DMA·12H2O (1), has been synthesized under solvothermal conditions by employing a pyridyl-decorated tetracarboxylate ligand, 2,2′-(pyridine-2,5-diyl)diterephthalic acid (H4L). Structural analysis demonstrates that 1 is a 3D microporous framework based on three kinds of inorganic secondary building units (SBUs), which shows an unprecedented 5-nodal (3,4,4,7,7)-connected topology. Especially, 1 possesses high chemical stability in pH = 2–13 aqueous solutions. The desolvated structure of 1 contains a highly polar pore system decorated with open metal sites, diethylammonium cations, and free pyridine atoms, leading to a high CO2/C2-hydrocarbons over CH4 separation performance. |
| collection_details |
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| title_short |
A robust indium(III)−potassium(I) MOF with high CO |
| remote_bool |
true |
| author2 |
Zhang, Bin Zhou, Huifang Wang, Weize Liu, Bo |
| author2Str |
Zhang, Bin Zhou, Huifang Wang, Weize Liu, Bo |
| ppnlink |
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| mediatype_str_mv |
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| doi_str |
10.1016/j.jssc.2020.121726 |
| up_date |
2024-07-07T00:32:44.904Z |
| _version_ |
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