Boosted bisphenol A and Cr(VI) cleanup over Z-scheme WO

To develop a new efficient catalyst for contaminant removal and sustainable environment, series Z-scheme WO3/MIL-100(Fe) (MxWy) composites were easily prepared by ball-milling strategy, which were affirmed by various characterization techniques. All the as-prepared MxWy composites displayed superior...
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Autor*in:	Wang, Jia-Wei [verfasserIn] Qiu, Fu-Guo [verfasserIn] Wang, Peng [verfasserIn] Ge, Chengjun [verfasserIn] Wang, Chong-Chen [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2020

Schlagwörter:	MIL-100(Fe) WO Cr(VI) reduction Bisphenol A Z-Scheme

Übergeordnetes Werk:	Enthalten in: Journal of cleaner production - Amsterdam [u.a.] : Elsevier Science, 1993, 279
Übergeordnetes Werk:	volume:279

DOI / URN:	10.1016/j.jclepro.2020.123408

Katalog-ID:	ELV005073561

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allfields	10.1016/j.jclepro.2020.123408 doi (DE-627)ELV005073561 (ELSEVIER)S0959-6526(20)33453-3 DE-627 ger DE-627 rda eng 690 330 DE-600 43.35 bkl 85.35 bkl Wang, Jia-Wei verfasserin aut Boosted bisphenol A and Cr(VI) cleanup over Z-scheme WO 2020 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier To develop a new efficient catalyst for contaminant removal and sustainable environment, series Z-scheme WO3/MIL-100(Fe) (MxWy) composites were easily prepared by ball-milling strategy, which were affirmed by various characterization techniques. All the as-prepared MxWy composites displayed superior photocatalytic Cr(VI) reduction and photo-Fenton bisphenol A(BPA) degradation performances under LED visible light, in which the M80W120 could accomplish 100% Cr(VI) reduction via photocatalysis treatment within 60 min and 100% BPA degradation with the aid of photo-Fenton process in 20 min. The influences of different initial pH, co-existing foreign ions, low weight organic molecules and H2O2 dosage on photocatalytic/photo-Fenton performances were clarified. Moreover, M80W120 displayed outstanding stability and reusability during five successive cycling experiments on Cr(VI) sequestration and BPA degradation, respectively. Also, the possible degradation pathway of BPA degradation over M80W120 was clarified. Finally, a Z-scheme mechanism was put forward, which was further confirmed by active species capture, photo-deposition of PbO2 along with electron spin-resonance spectroscopy determination. The combination of MIL-100(Fe) and WO3 was confirmed to be an effective strategy for pollutant removal and cleaner production. MIL-100(Fe) WO Cr(VI) reduction Bisphenol A Z-Scheme Qiu, Fu-Guo verfasserin (orcid)0000-0002-6494-5746 aut Wang, Peng verfasserin aut Ge, Chengjun verfasserin aut Wang, Chong-Chen verfasserin aut Enthalten in Journal of cleaner production Amsterdam [u.a.] : Elsevier Science, 1993 279 Online-Ressource (DE-627)324655878 (DE-600)2029338-0 (DE-576)252613988 0959-6526 nnns volume:279 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OPC-GGO GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 43.35 Umweltrichtlinien Umweltnormen 85.35 Fertigung AR 279
spelling	10.1016/j.jclepro.2020.123408 doi (DE-627)ELV005073561 (ELSEVIER)S0959-6526(20)33453-3 DE-627 ger DE-627 rda eng 690 330 DE-600 43.35 bkl 85.35 bkl Wang, Jia-Wei verfasserin aut Boosted bisphenol A and Cr(VI) cleanup over Z-scheme WO 2020 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier To develop a new efficient catalyst for contaminant removal and sustainable environment, series Z-scheme WO3/MIL-100(Fe) (MxWy) composites were easily prepared by ball-milling strategy, which were affirmed by various characterization techniques. All the as-prepared MxWy composites displayed superior photocatalytic Cr(VI) reduction and photo-Fenton bisphenol A(BPA) degradation performances under LED visible light, in which the M80W120 could accomplish 100% Cr(VI) reduction via photocatalysis treatment within 60 min and 100% BPA degradation with the aid of photo-Fenton process in 20 min. The influences of different initial pH, co-existing foreign ions, low weight organic molecules and H2O2 dosage on photocatalytic/photo-Fenton performances were clarified. Moreover, M80W120 displayed outstanding stability and reusability during five successive cycling experiments on Cr(VI) sequestration and BPA degradation, respectively. Also, the possible degradation pathway of BPA degradation over M80W120 was clarified. Finally, a Z-scheme mechanism was put forward, which was further confirmed by active species capture, photo-deposition of PbO2 along with electron spin-resonance spectroscopy determination. The combination of MIL-100(Fe) and WO3 was confirmed to be an effective strategy for pollutant removal and cleaner production. MIL-100(Fe) WO Cr(VI) reduction Bisphenol A Z-Scheme Qiu, Fu-Guo verfasserin (orcid)0000-0002-6494-5746 aut Wang, Peng verfasserin aut Ge, Chengjun verfasserin aut Wang, Chong-Chen verfasserin aut Enthalten in Journal of cleaner production Amsterdam [u.a.] : Elsevier Science, 1993 279 Online-Ressource (DE-627)324655878 (DE-600)2029338-0 (DE-576)252613988 0959-6526 nnns volume:279 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OPC-GGO GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 43.35 Umweltrichtlinien Umweltnormen 85.35 Fertigung AR 279
allfields_unstemmed	10.1016/j.jclepro.2020.123408 doi (DE-627)ELV005073561 (ELSEVIER)S0959-6526(20)33453-3 DE-627 ger DE-627 rda eng 690 330 DE-600 43.35 bkl 85.35 bkl Wang, Jia-Wei verfasserin aut Boosted bisphenol A and Cr(VI) cleanup over Z-scheme WO 2020 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier To develop a new efficient catalyst for contaminant removal and sustainable environment, series Z-scheme WO3/MIL-100(Fe) (MxWy) composites were easily prepared by ball-milling strategy, which were affirmed by various characterization techniques. All the as-prepared MxWy composites displayed superior photocatalytic Cr(VI) reduction and photo-Fenton bisphenol A(BPA) degradation performances under LED visible light, in which the M80W120 could accomplish 100% Cr(VI) reduction via photocatalysis treatment within 60 min and 100% BPA degradation with the aid of photo-Fenton process in 20 min. The influences of different initial pH, co-existing foreign ions, low weight organic molecules and H2O2 dosage on photocatalytic/photo-Fenton performances were clarified. Moreover, M80W120 displayed outstanding stability and reusability during five successive cycling experiments on Cr(VI) sequestration and BPA degradation, respectively. Also, the possible degradation pathway of BPA degradation over M80W120 was clarified. Finally, a Z-scheme mechanism was put forward, which was further confirmed by active species capture, photo-deposition of PbO2 along with electron spin-resonance spectroscopy determination. The combination of MIL-100(Fe) and WO3 was confirmed to be an effective strategy for pollutant removal and cleaner production. MIL-100(Fe) WO Cr(VI) reduction Bisphenol A Z-Scheme Qiu, Fu-Guo verfasserin (orcid)0000-0002-6494-5746 aut Wang, Peng verfasserin aut Ge, Chengjun verfasserin aut Wang, Chong-Chen verfasserin aut Enthalten in Journal of cleaner production Amsterdam [u.a.] : Elsevier Science, 1993 279 Online-Ressource (DE-627)324655878 (DE-600)2029338-0 (DE-576)252613988 0959-6526 nnns volume:279 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OPC-GGO GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 43.35 Umweltrichtlinien Umweltnormen 85.35 Fertigung AR 279
allfieldsGer	10.1016/j.jclepro.2020.123408 doi (DE-627)ELV005073561 (ELSEVIER)S0959-6526(20)33453-3 DE-627 ger DE-627 rda eng 690 330 DE-600 43.35 bkl 85.35 bkl Wang, Jia-Wei verfasserin aut Boosted bisphenol A and Cr(VI) cleanup over Z-scheme WO 2020 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier To develop a new efficient catalyst for contaminant removal and sustainable environment, series Z-scheme WO3/MIL-100(Fe) (MxWy) composites were easily prepared by ball-milling strategy, which were affirmed by various characterization techniques. All the as-prepared MxWy composites displayed superior photocatalytic Cr(VI) reduction and photo-Fenton bisphenol A(BPA) degradation performances under LED visible light, in which the M80W120 could accomplish 100% Cr(VI) reduction via photocatalysis treatment within 60 min and 100% BPA degradation with the aid of photo-Fenton process in 20 min. The influences of different initial pH, co-existing foreign ions, low weight organic molecules and H2O2 dosage on photocatalytic/photo-Fenton performances were clarified. Moreover, M80W120 displayed outstanding stability and reusability during five successive cycling experiments on Cr(VI) sequestration and BPA degradation, respectively. Also, the possible degradation pathway of BPA degradation over M80W120 was clarified. Finally, a Z-scheme mechanism was put forward, which was further confirmed by active species capture, photo-deposition of PbO2 along with electron spin-resonance spectroscopy determination. The combination of MIL-100(Fe) and WO3 was confirmed to be an effective strategy for pollutant removal and cleaner production. MIL-100(Fe) WO Cr(VI) reduction Bisphenol A Z-Scheme Qiu, Fu-Guo verfasserin (orcid)0000-0002-6494-5746 aut Wang, Peng verfasserin aut Ge, Chengjun verfasserin aut Wang, Chong-Chen verfasserin aut Enthalten in Journal of cleaner production Amsterdam [u.a.] : Elsevier Science, 1993 279 Online-Ressource (DE-627)324655878 (DE-600)2029338-0 (DE-576)252613988 0959-6526 nnns volume:279 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OPC-GGO GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 43.35 Umweltrichtlinien Umweltnormen 85.35 Fertigung AR 279
allfieldsSound	10.1016/j.jclepro.2020.123408 doi (DE-627)ELV005073561 (ELSEVIER)S0959-6526(20)33453-3 DE-627 ger DE-627 rda eng 690 330 DE-600 43.35 bkl 85.35 bkl Wang, Jia-Wei verfasserin aut Boosted bisphenol A and Cr(VI) cleanup over Z-scheme WO 2020 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier To develop a new efficient catalyst for contaminant removal and sustainable environment, series Z-scheme WO3/MIL-100(Fe) (MxWy) composites were easily prepared by ball-milling strategy, which were affirmed by various characterization techniques. All the as-prepared MxWy composites displayed superior photocatalytic Cr(VI) reduction and photo-Fenton bisphenol A(BPA) degradation performances under LED visible light, in which the M80W120 could accomplish 100% Cr(VI) reduction via photocatalysis treatment within 60 min and 100% BPA degradation with the aid of photo-Fenton process in 20 min. The influences of different initial pH, co-existing foreign ions, low weight organic molecules and H2O2 dosage on photocatalytic/photo-Fenton performances were clarified. Moreover, M80W120 displayed outstanding stability and reusability during five successive cycling experiments on Cr(VI) sequestration and BPA degradation, respectively. Also, the possible degradation pathway of BPA degradation over M80W120 was clarified. Finally, a Z-scheme mechanism was put forward, which was further confirmed by active species capture, photo-deposition of PbO2 along with electron spin-resonance spectroscopy determination. The combination of MIL-100(Fe) and WO3 was confirmed to be an effective strategy for pollutant removal and cleaner production. MIL-100(Fe) WO Cr(VI) reduction Bisphenol A Z-Scheme Qiu, Fu-Guo verfasserin (orcid)0000-0002-6494-5746 aut Wang, Peng verfasserin aut Ge, Chengjun verfasserin aut Wang, Chong-Chen verfasserin aut Enthalten in Journal of cleaner production Amsterdam [u.a.] : Elsevier Science, 1993 279 Online-Ressource (DE-627)324655878 (DE-600)2029338-0 (DE-576)252613988 0959-6526 nnns volume:279 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OPC-GGO GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 43.35 Umweltrichtlinien Umweltnormen 85.35 Fertigung AR 279
language	English
source	Enthalten in Journal of cleaner production 279 volume:279
sourceStr	Enthalten in Journal of cleaner production 279 volume:279
format_phy_str_mv	Article
bklname	Umweltrichtlinien Umweltnormen Fertigung
institution	findex.gbv.de
topic_facet	MIL-100(Fe) WO Cr(VI) reduction Bisphenol A Z-Scheme
dewey-raw	690
isfreeaccess_bool	false
container_title	Journal of cleaner production
authorswithroles_txt_mv	Wang, Jia-Wei @@aut@@ Qiu, Fu-Guo @@aut@@ Wang, Peng @@aut@@ Ge, Chengjun @@aut@@ Wang, Chong-Chen @@aut@@
publishDateDaySort_date	2020-01-01T00:00:00Z
hierarchy_top_id	324655878
dewey-sort	3690
id	ELV005073561
language_de	englisch
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author	Wang, Jia-Wei
spellingShingle	Wang, Jia-Wei ddc 690 bkl 43.35 bkl 85.35 misc MIL-100(Fe) misc WO misc Cr(VI) reduction misc Bisphenol A misc Z-Scheme Boosted bisphenol A and Cr(VI) cleanup over Z-scheme WO
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topic_title	690 330 DE-600 43.35 bkl 85.35 bkl Boosted bisphenol A and Cr(VI) cleanup over Z-scheme WO MIL-100(Fe) WO Cr(VI) reduction Bisphenol A Z-Scheme
topic	ddc 690 bkl 43.35 bkl 85.35 misc MIL-100(Fe) misc WO misc Cr(VI) reduction misc Bisphenol A misc Z-Scheme
topic_unstemmed	ddc 690 bkl 43.35 bkl 85.35 misc MIL-100(Fe) misc WO misc Cr(VI) reduction misc Bisphenol A misc Z-Scheme
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title	Boosted bisphenol A and Cr(VI) cleanup over Z-scheme WO
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title_full	Boosted bisphenol A and Cr(VI) cleanup over Z-scheme WO
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title_sort	boosted bisphenol a and cr(vi) cleanup over z-scheme wo
title_auth	Boosted bisphenol A and Cr(VI) cleanup over Z-scheme WO
abstract	To develop a new efficient catalyst for contaminant removal and sustainable environment, series Z-scheme WO3/MIL-100(Fe) (MxWy) composites were easily prepared by ball-milling strategy, which were affirmed by various characterization techniques. All the as-prepared MxWy composites displayed superior photocatalytic Cr(VI) reduction and photo-Fenton bisphenol A(BPA) degradation performances under LED visible light, in which the M80W120 could accomplish 100% Cr(VI) reduction via photocatalysis treatment within 60 min and 100% BPA degradation with the aid of photo-Fenton process in 20 min. The influences of different initial pH, co-existing foreign ions, low weight organic molecules and H2O2 dosage on photocatalytic/photo-Fenton performances were clarified. Moreover, M80W120 displayed outstanding stability and reusability during five successive cycling experiments on Cr(VI) sequestration and BPA degradation, respectively. Also, the possible degradation pathway of BPA degradation over M80W120 was clarified. Finally, a Z-scheme mechanism was put forward, which was further confirmed by active species capture, photo-deposition of PbO2 along with electron spin-resonance spectroscopy determination. The combination of MIL-100(Fe) and WO3 was confirmed to be an effective strategy for pollutant removal and cleaner production.
abstractGer	To develop a new efficient catalyst for contaminant removal and sustainable environment, series Z-scheme WO3/MIL-100(Fe) (MxWy) composites were easily prepared by ball-milling strategy, which were affirmed by various characterization techniques. All the as-prepared MxWy composites displayed superior photocatalytic Cr(VI) reduction and photo-Fenton bisphenol A(BPA) degradation performances under LED visible light, in which the M80W120 could accomplish 100% Cr(VI) reduction via photocatalysis treatment within 60 min and 100% BPA degradation with the aid of photo-Fenton process in 20 min. The influences of different initial pH, co-existing foreign ions, low weight organic molecules and H2O2 dosage on photocatalytic/photo-Fenton performances were clarified. Moreover, M80W120 displayed outstanding stability and reusability during five successive cycling experiments on Cr(VI) sequestration and BPA degradation, respectively. Also, the possible degradation pathway of BPA degradation over M80W120 was clarified. Finally, a Z-scheme mechanism was put forward, which was further confirmed by active species capture, photo-deposition of PbO2 along with electron spin-resonance spectroscopy determination. The combination of MIL-100(Fe) and WO3 was confirmed to be an effective strategy for pollutant removal and cleaner production.
abstract_unstemmed	To develop a new efficient catalyst for contaminant removal and sustainable environment, series Z-scheme WO3/MIL-100(Fe) (MxWy) composites were easily prepared by ball-milling strategy, which were affirmed by various characterization techniques. All the as-prepared MxWy composites displayed superior photocatalytic Cr(VI) reduction and photo-Fenton bisphenol A(BPA) degradation performances under LED visible light, in which the M80W120 could accomplish 100% Cr(VI) reduction via photocatalysis treatment within 60 min and 100% BPA degradation with the aid of photo-Fenton process in 20 min. The influences of different initial pH, co-existing foreign ions, low weight organic molecules and H2O2 dosage on photocatalytic/photo-Fenton performances were clarified. Moreover, M80W120 displayed outstanding stability and reusability during five successive cycling experiments on Cr(VI) sequestration and BPA degradation, respectively. Also, the possible degradation pathway of BPA degradation over M80W120 was clarified. Finally, a Z-scheme mechanism was put forward, which was further confirmed by active species capture, photo-deposition of PbO2 along with electron spin-resonance spectroscopy determination. The combination of MIL-100(Fe) and WO3 was confirmed to be an effective strategy for pollutant removal and cleaner production.
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title_short	Boosted bisphenol A and Cr(VI) cleanup over Z-scheme WO
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author2	Qiu, Fu-Guo Wang, Peng Ge, Chengjun Wang, Chong-Chen
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up_date	2024-07-06T16:43:49.546Z
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