PVP-assisted synthesis of g–C

Carbon materials have attracted abundant attentions and been utilized widely as anodes in rechargeable Li+/Na+/K+ ions batteries. Regarding the various radius of alkali-metal-ions, reversible intercalation and deintercalation in interlayers of carbons requires different interplanar spacing. In this...
Ausführliche Beschreibung

Gespeichert in:

Autor*in:	Tang, Yihua [verfasserIn] Wang, Xiao [verfasserIn] Chen, Jingjing [verfasserIn] Wang, Xinxin [verfasserIn] Wang, Dajian [verfasserIn] Mao, Zhiyong [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2020

Schlagwörter:	N-doped graphene Graphitic carbon nitride Interplanar spacing Lithium ions batteries Sodium ions batteries

Übergeordnetes Werk:	Enthalten in: Carbon - Amsterdam [u.a.] : Elsevier Science, 1963, 174, Seite 98-109
Übergeordnetes Werk:	volume:174 ; pages:98-109

DOI / URN:	10.1016/j.carbon.2020.12.010

Katalog-ID:	ELV005552540

Internformat


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520			\|a Carbon materials have attracted abundant attentions and been utilized widely as anodes in rechargeable Li+/Na+/K+ ions batteries. Regarding the various radius of alkali-metal-ions, reversible intercalation and deintercalation in interlayers of carbons requires different interplanar spacing. In this work, N-doped graphene with tunable interplanar spacing is synthesized using graphitic carbon nitride (g-C3N4) as precursor with the assistance of polyvinylpyrrolidone (PVP). The obtained tunable interplanar spacing in the range from 0.34 nm to 0.45 nm with enlarged values is mainly ascribed to the high nitrogen doping levels (9.98–33.7 at. %), especially to the pyrrolic nitrogen. Serving as the anode materials in lithium ions batteries (LIBs) and sodium ions batteries (SIBs), promising specific capacities of 1236 mAh g−1 for LIBs and 300 mAh g−1 for SIBs at current density of 0.05 A g−1 and excellent cycling stability as well as acceptable rate capability are demonstrated for the resultant N-doped graphene. The influences of interplanar spacing on the electrochemical performances of LIBs and SIBs are investigated comparatively. This work outlines a facial route to synthesize N-doped graphene with tunable interplanar spacing, meeting the various requirements unitized as anodes in rechargeable Li+/Na+/K+ ions batteries.
650		4	\|a N-doped graphene
650		4	\|a Graphitic carbon nitride
650		4	\|a Interplanar spacing
650		4	\|a Lithium ions batteries
650		4	\|a Sodium ions batteries
700	1		\|a Wang, Xiao \|e verfasserin \|4 aut
700	1		\|a Chen, Jingjing \|e verfasserin \|4 aut
700	1		\|a Wang, Xinxin \|e verfasserin \|4 aut
700	1		\|a Wang, Dajian \|e verfasserin \|4 aut
700	1		\|a Mao, Zhiyong \|e verfasserin \|0 (orcid)0000-0003-0125-3408 \|4 aut
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912			\|a GBV_ILN_23
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912			\|a GBV_ILN_31
912			\|a GBV_ILN_32
912			\|a GBV_ILN_40
912			\|a GBV_ILN_60
912			\|a GBV_ILN_62
912			\|a GBV_ILN_63
912			\|a GBV_ILN_65
912			\|a GBV_ILN_69
912			\|a GBV_ILN_70
912			\|a GBV_ILN_73
912			\|a GBV_ILN_74
912			\|a GBV_ILN_90
912			\|a GBV_ILN_95
912			\|a GBV_ILN_100
912			\|a GBV_ILN_101
912			\|a GBV_ILN_105
912			\|a GBV_ILN_110
912			\|a GBV_ILN_150
912			\|a GBV_ILN_151
912			\|a GBV_ILN_224
912			\|a GBV_ILN_370
912			\|a GBV_ILN_602
912			\|a GBV_ILN_702
912			\|a GBV_ILN_2003
912			\|a GBV_ILN_2004
912			\|a GBV_ILN_2005
912			\|a GBV_ILN_2006
912			\|a GBV_ILN_2008
912			\|a GBV_ILN_2011
912			\|a GBV_ILN_2014
912			\|a GBV_ILN_2015
912			\|a GBV_ILN_2020
912			\|a GBV_ILN_2021
912			\|a GBV_ILN_2025
912			\|a GBV_ILN_2027
912			\|a GBV_ILN_2034
912			\|a GBV_ILN_2038
912			\|a GBV_ILN_2044
912			\|a GBV_ILN_2048
912			\|a GBV_ILN_2049
912			\|a GBV_ILN_2050
912			\|a GBV_ILN_2056
912			\|a GBV_ILN_2059
912			\|a GBV_ILN_2061
912			\|a GBV_ILN_2064
912			\|a GBV_ILN_2065
912			\|a GBV_ILN_2068
912			\|a GBV_ILN_2088
912			\|a GBV_ILN_2111
912			\|a GBV_ILN_2112
912			\|a GBV_ILN_2113
912			\|a GBV_ILN_2118
912			\|a GBV_ILN_2122
912			\|a GBV_ILN_2129
912			\|a GBV_ILN_2143
912			\|a GBV_ILN_2147
912			\|a GBV_ILN_2148
912			\|a GBV_ILN_2152
912			\|a GBV_ILN_2153
912			\|a GBV_ILN_2190
912			\|a GBV_ILN_2336
912			\|a GBV_ILN_2470
912			\|a GBV_ILN_2507
912			\|a GBV_ILN_2522
912			\|a GBV_ILN_4035
912			\|a GBV_ILN_4037
912			\|a GBV_ILN_4046
912			\|a GBV_ILN_4112
912			\|a GBV_ILN_4125
912			\|a GBV_ILN_4126
912			\|a GBV_ILN_4242
912			\|a GBV_ILN_4251
912			\|a GBV_ILN_4305
912			\|a GBV_ILN_4313
912			\|a GBV_ILN_4322
912			\|a GBV_ILN_4323
912			\|a GBV_ILN_4324
912			\|a GBV_ILN_4326
912			\|a GBV_ILN_4333
912			\|a GBV_ILN_4334
912			\|a GBV_ILN_4335
912			\|a GBV_ILN_4338
912			\|a GBV_ILN_4393
936	b	k	\|a 51.79 \|j Sonstige Werkstoffe
936	b	k	\|a 35.48 \|j Sonstige anorganische Elemente und ihre Verbindungen
951			\|a AR
952			\|d 174 \|h 98-109

Indexfelder

author_variant	y t yt x w xw j c jc x w xw d w dw z m zm
matchkey_str	article:00086223:2020----::vassesnhs
hierarchy_sort_str	2020
bklnumber	51.79 35.48
publishDate	2020
allfields	10.1016/j.carbon.2020.12.010 doi (DE-627)ELV005552540 (ELSEVIER)S0008-6223(20)31187-8 DE-627 ger DE-627 rda eng 540 DE-600 51.79 bkl 35.48 bkl Tang, Yihua verfasserin aut PVP-assisted synthesis of g–C 2020 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Carbon materials have attracted abundant attentions and been utilized widely as anodes in rechargeable Li+/Na+/K+ ions batteries. Regarding the various radius of alkali-metal-ions, reversible intercalation and deintercalation in interlayers of carbons requires different interplanar spacing. In this work, N-doped graphene with tunable interplanar spacing is synthesized using graphitic carbon nitride (g-C3N4) as precursor with the assistance of polyvinylpyrrolidone (PVP). The obtained tunable interplanar spacing in the range from 0.34 nm to 0.45 nm with enlarged values is mainly ascribed to the high nitrogen doping levels (9.98–33.7 at. %), especially to the pyrrolic nitrogen. Serving as the anode materials in lithium ions batteries (LIBs) and sodium ions batteries (SIBs), promising specific capacities of 1236 mAh g−1 for LIBs and 300 mAh g−1 for SIBs at current density of 0.05 A g−1 and excellent cycling stability as well as acceptable rate capability are demonstrated for the resultant N-doped graphene. The influences of interplanar spacing on the electrochemical performances of LIBs and SIBs are investigated comparatively. This work outlines a facial route to synthesize N-doped graphene with tunable interplanar spacing, meeting the various requirements unitized as anodes in rechargeable Li+/Na+/K+ ions batteries. N-doped graphene Graphitic carbon nitride Interplanar spacing Lithium ions batteries Sodium ions batteries Wang, Xiao verfasserin aut Chen, Jingjing verfasserin aut Wang, Xinxin verfasserin aut Wang, Dajian verfasserin aut Mao, Zhiyong verfasserin (orcid)0000-0003-0125-3408 aut Enthalten in Carbon Amsterdam [u.a.] : Elsevier Science, 1963 174, Seite 98-109 Online-Ressource (DE-627)320522164 (DE-600)2014715-6 (DE-576)103484280 0008-6223 nnns volume:174 pages:98-109 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 51.79 Sonstige Werkstoffe 35.48 Sonstige anorganische Elemente und ihre Verbindungen AR 174 98-109
spelling	10.1016/j.carbon.2020.12.010 doi (DE-627)ELV005552540 (ELSEVIER)S0008-6223(20)31187-8 DE-627 ger DE-627 rda eng 540 DE-600 51.79 bkl 35.48 bkl Tang, Yihua verfasserin aut PVP-assisted synthesis of g–C 2020 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Carbon materials have attracted abundant attentions and been utilized widely as anodes in rechargeable Li+/Na+/K+ ions batteries. Regarding the various radius of alkali-metal-ions, reversible intercalation and deintercalation in interlayers of carbons requires different interplanar spacing. In this work, N-doped graphene with tunable interplanar spacing is synthesized using graphitic carbon nitride (g-C3N4) as precursor with the assistance of polyvinylpyrrolidone (PVP). The obtained tunable interplanar spacing in the range from 0.34 nm to 0.45 nm with enlarged values is mainly ascribed to the high nitrogen doping levels (9.98–33.7 at. %), especially to the pyrrolic nitrogen. Serving as the anode materials in lithium ions batteries (LIBs) and sodium ions batteries (SIBs), promising specific capacities of 1236 mAh g−1 for LIBs and 300 mAh g−1 for SIBs at current density of 0.05 A g−1 and excellent cycling stability as well as acceptable rate capability are demonstrated for the resultant N-doped graphene. The influences of interplanar spacing on the electrochemical performances of LIBs and SIBs are investigated comparatively. This work outlines a facial route to synthesize N-doped graphene with tunable interplanar spacing, meeting the various requirements unitized as anodes in rechargeable Li+/Na+/K+ ions batteries. N-doped graphene Graphitic carbon nitride Interplanar spacing Lithium ions batteries Sodium ions batteries Wang, Xiao verfasserin aut Chen, Jingjing verfasserin aut Wang, Xinxin verfasserin aut Wang, Dajian verfasserin aut Mao, Zhiyong verfasserin (orcid)0000-0003-0125-3408 aut Enthalten in Carbon Amsterdam [u.a.] : Elsevier Science, 1963 174, Seite 98-109 Online-Ressource (DE-627)320522164 (DE-600)2014715-6 (DE-576)103484280 0008-6223 nnns volume:174 pages:98-109 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 51.79 Sonstige Werkstoffe 35.48 Sonstige anorganische Elemente und ihre Verbindungen AR 174 98-109
allfields_unstemmed	10.1016/j.carbon.2020.12.010 doi (DE-627)ELV005552540 (ELSEVIER)S0008-6223(20)31187-8 DE-627 ger DE-627 rda eng 540 DE-600 51.79 bkl 35.48 bkl Tang, Yihua verfasserin aut PVP-assisted synthesis of g–C 2020 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Carbon materials have attracted abundant attentions and been utilized widely as anodes in rechargeable Li+/Na+/K+ ions batteries. Regarding the various radius of alkali-metal-ions, reversible intercalation and deintercalation in interlayers of carbons requires different interplanar spacing. In this work, N-doped graphene with tunable interplanar spacing is synthesized using graphitic carbon nitride (g-C3N4) as precursor with the assistance of polyvinylpyrrolidone (PVP). The obtained tunable interplanar spacing in the range from 0.34 nm to 0.45 nm with enlarged values is mainly ascribed to the high nitrogen doping levels (9.98–33.7 at. %), especially to the pyrrolic nitrogen. Serving as the anode materials in lithium ions batteries (LIBs) and sodium ions batteries (SIBs), promising specific capacities of 1236 mAh g−1 for LIBs and 300 mAh g−1 for SIBs at current density of 0.05 A g−1 and excellent cycling stability as well as acceptable rate capability are demonstrated for the resultant N-doped graphene. The influences of interplanar spacing on the electrochemical performances of LIBs and SIBs are investigated comparatively. This work outlines a facial route to synthesize N-doped graphene with tunable interplanar spacing, meeting the various requirements unitized as anodes in rechargeable Li+/Na+/K+ ions batteries. N-doped graphene Graphitic carbon nitride Interplanar spacing Lithium ions batteries Sodium ions batteries Wang, Xiao verfasserin aut Chen, Jingjing verfasserin aut Wang, Xinxin verfasserin aut Wang, Dajian verfasserin aut Mao, Zhiyong verfasserin (orcid)0000-0003-0125-3408 aut Enthalten in Carbon Amsterdam [u.a.] : Elsevier Science, 1963 174, Seite 98-109 Online-Ressource (DE-627)320522164 (DE-600)2014715-6 (DE-576)103484280 0008-6223 nnns volume:174 pages:98-109 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 51.79 Sonstige Werkstoffe 35.48 Sonstige anorganische Elemente und ihre Verbindungen AR 174 98-109
allfieldsGer	10.1016/j.carbon.2020.12.010 doi (DE-627)ELV005552540 (ELSEVIER)S0008-6223(20)31187-8 DE-627 ger DE-627 rda eng 540 DE-600 51.79 bkl 35.48 bkl Tang, Yihua verfasserin aut PVP-assisted synthesis of g–C 2020 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Carbon materials have attracted abundant attentions and been utilized widely as anodes in rechargeable Li+/Na+/K+ ions batteries. Regarding the various radius of alkali-metal-ions, reversible intercalation and deintercalation in interlayers of carbons requires different interplanar spacing. In this work, N-doped graphene with tunable interplanar spacing is synthesized using graphitic carbon nitride (g-C3N4) as precursor with the assistance of polyvinylpyrrolidone (PVP). The obtained tunable interplanar spacing in the range from 0.34 nm to 0.45 nm with enlarged values is mainly ascribed to the high nitrogen doping levels (9.98–33.7 at. %), especially to the pyrrolic nitrogen. Serving as the anode materials in lithium ions batteries (LIBs) and sodium ions batteries (SIBs), promising specific capacities of 1236 mAh g−1 for LIBs and 300 mAh g−1 for SIBs at current density of 0.05 A g−1 and excellent cycling stability as well as acceptable rate capability are demonstrated for the resultant N-doped graphene. The influences of interplanar spacing on the electrochemical performances of LIBs and SIBs are investigated comparatively. This work outlines a facial route to synthesize N-doped graphene with tunable interplanar spacing, meeting the various requirements unitized as anodes in rechargeable Li+/Na+/K+ ions batteries. N-doped graphene Graphitic carbon nitride Interplanar spacing Lithium ions batteries Sodium ions batteries Wang, Xiao verfasserin aut Chen, Jingjing verfasserin aut Wang, Xinxin verfasserin aut Wang, Dajian verfasserin aut Mao, Zhiyong verfasserin (orcid)0000-0003-0125-3408 aut Enthalten in Carbon Amsterdam [u.a.] : Elsevier Science, 1963 174, Seite 98-109 Online-Ressource (DE-627)320522164 (DE-600)2014715-6 (DE-576)103484280 0008-6223 nnns volume:174 pages:98-109 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 51.79 Sonstige Werkstoffe 35.48 Sonstige anorganische Elemente und ihre Verbindungen AR 174 98-109
allfieldsSound	10.1016/j.carbon.2020.12.010 doi (DE-627)ELV005552540 (ELSEVIER)S0008-6223(20)31187-8 DE-627 ger DE-627 rda eng 540 DE-600 51.79 bkl 35.48 bkl Tang, Yihua verfasserin aut PVP-assisted synthesis of g–C 2020 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Carbon materials have attracted abundant attentions and been utilized widely as anodes in rechargeable Li+/Na+/K+ ions batteries. Regarding the various radius of alkali-metal-ions, reversible intercalation and deintercalation in interlayers of carbons requires different interplanar spacing. In this work, N-doped graphene with tunable interplanar spacing is synthesized using graphitic carbon nitride (g-C3N4) as precursor with the assistance of polyvinylpyrrolidone (PVP). The obtained tunable interplanar spacing in the range from 0.34 nm to 0.45 nm with enlarged values is mainly ascribed to the high nitrogen doping levels (9.98–33.7 at. %), especially to the pyrrolic nitrogen. Serving as the anode materials in lithium ions batteries (LIBs) and sodium ions batteries (SIBs), promising specific capacities of 1236 mAh g−1 for LIBs and 300 mAh g−1 for SIBs at current density of 0.05 A g−1 and excellent cycling stability as well as acceptable rate capability are demonstrated for the resultant N-doped graphene. The influences of interplanar spacing on the electrochemical performances of LIBs and SIBs are investigated comparatively. This work outlines a facial route to synthesize N-doped graphene with tunable interplanar spacing, meeting the various requirements unitized as anodes in rechargeable Li+/Na+/K+ ions batteries. N-doped graphene Graphitic carbon nitride Interplanar spacing Lithium ions batteries Sodium ions batteries Wang, Xiao verfasserin aut Chen, Jingjing verfasserin aut Wang, Xinxin verfasserin aut Wang, Dajian verfasserin aut Mao, Zhiyong verfasserin (orcid)0000-0003-0125-3408 aut Enthalten in Carbon Amsterdam [u.a.] : Elsevier Science, 1963 174, Seite 98-109 Online-Ressource (DE-627)320522164 (DE-600)2014715-6 (DE-576)103484280 0008-6223 nnns volume:174 pages:98-109 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 51.79 Sonstige Werkstoffe 35.48 Sonstige anorganische Elemente und ihre Verbindungen AR 174 98-109
language	English
source	Enthalten in Carbon 174, Seite 98-109 volume:174 pages:98-109
sourceStr	Enthalten in Carbon 174, Seite 98-109 volume:174 pages:98-109
format_phy_str_mv	Article
bklname	Sonstige Werkstoffe Sonstige anorganische Elemente und ihre Verbindungen
institution	findex.gbv.de
topic_facet	N-doped graphene Graphitic carbon nitride Interplanar spacing Lithium ions batteries Sodium ions batteries
dewey-raw	540
isfreeaccess_bool	false
container_title	Carbon
authorswithroles_txt_mv	Tang, Yihua @@aut@@ Wang, Xiao @@aut@@ Chen, Jingjing @@aut@@ Wang, Xinxin @@aut@@ Wang, Dajian @@aut@@ Mao, Zhiyong @@aut@@
publishDateDaySort_date	2020-01-01T00:00:00Z
hierarchy_top_id	320522164
dewey-sort	3540
id	ELV005552540
language_de	englisch
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author	Tang, Yihua
spellingShingle	Tang, Yihua ddc 540 bkl 51.79 bkl 35.48 misc N-doped graphene misc Graphitic carbon nitride misc Interplanar spacing misc Lithium ions batteries misc Sodium ions batteries PVP-assisted synthesis of g–C
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topic_title	540 DE-600 51.79 bkl 35.48 bkl PVP-assisted synthesis of g–C N-doped graphene Graphitic carbon nitride Interplanar spacing Lithium ions batteries Sodium ions batteries
topic	ddc 540 bkl 51.79 bkl 35.48 misc N-doped graphene misc Graphitic carbon nitride misc Interplanar spacing misc Lithium ions batteries misc Sodium ions batteries
topic_unstemmed	ddc 540 bkl 51.79 bkl 35.48 misc N-doped graphene misc Graphitic carbon nitride misc Interplanar spacing misc Lithium ions batteries misc Sodium ions batteries
topic_browse	ddc 540 bkl 51.79 bkl 35.48 misc N-doped graphene misc Graphitic carbon nitride misc Interplanar spacing misc Lithium ions batteries misc Sodium ions batteries
format_facet	Elektronische Aufsätze Aufsätze Elektronische Ressource
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title	PVP-assisted synthesis of g–C
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title_full	PVP-assisted synthesis of g–C
author_sort	Tang, Yihua
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author_browse	Tang, Yihua Wang, Xiao Chen, Jingjing Wang, Xinxin Wang, Dajian Mao, Zhiyong
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author-letter	Tang, Yihua
doi_str_mv	10.1016/j.carbon.2020.12.010
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title_sort	pvp-assisted synthesis of g–c
title_auth	PVP-assisted synthesis of g–C
abstract	Carbon materials have attracted abundant attentions and been utilized widely as anodes in rechargeable Li+/Na+/K+ ions batteries. Regarding the various radius of alkali-metal-ions, reversible intercalation and deintercalation in interlayers of carbons requires different interplanar spacing. In this work, N-doped graphene with tunable interplanar spacing is synthesized using graphitic carbon nitride (g-C3N4) as precursor with the assistance of polyvinylpyrrolidone (PVP). The obtained tunable interplanar spacing in the range from 0.34 nm to 0.45 nm with enlarged values is mainly ascribed to the high nitrogen doping levels (9.98–33.7 at. %), especially to the pyrrolic nitrogen. Serving as the anode materials in lithium ions batteries (LIBs) and sodium ions batteries (SIBs), promising specific capacities of 1236 mAh g−1 for LIBs and 300 mAh g−1 for SIBs at current density of 0.05 A g−1 and excellent cycling stability as well as acceptable rate capability are demonstrated for the resultant N-doped graphene. The influences of interplanar spacing on the electrochemical performances of LIBs and SIBs are investigated comparatively. This work outlines a facial route to synthesize N-doped graphene with tunable interplanar spacing, meeting the various requirements unitized as anodes in rechargeable Li+/Na+/K+ ions batteries.
abstractGer	Carbon materials have attracted abundant attentions and been utilized widely as anodes in rechargeable Li+/Na+/K+ ions batteries. Regarding the various radius of alkali-metal-ions, reversible intercalation and deintercalation in interlayers of carbons requires different interplanar spacing. In this work, N-doped graphene with tunable interplanar spacing is synthesized using graphitic carbon nitride (g-C3N4) as precursor with the assistance of polyvinylpyrrolidone (PVP). The obtained tunable interplanar spacing in the range from 0.34 nm to 0.45 nm with enlarged values is mainly ascribed to the high nitrogen doping levels (9.98–33.7 at. %), especially to the pyrrolic nitrogen. Serving as the anode materials in lithium ions batteries (LIBs) and sodium ions batteries (SIBs), promising specific capacities of 1236 mAh g−1 for LIBs and 300 mAh g−1 for SIBs at current density of 0.05 A g−1 and excellent cycling stability as well as acceptable rate capability are demonstrated for the resultant N-doped graphene. The influences of interplanar spacing on the electrochemical performances of LIBs and SIBs are investigated comparatively. This work outlines a facial route to synthesize N-doped graphene with tunable interplanar spacing, meeting the various requirements unitized as anodes in rechargeable Li+/Na+/K+ ions batteries.
abstract_unstemmed	Carbon materials have attracted abundant attentions and been utilized widely as anodes in rechargeable Li+/Na+/K+ ions batteries. Regarding the various radius of alkali-metal-ions, reversible intercalation and deintercalation in interlayers of carbons requires different interplanar spacing. In this work, N-doped graphene with tunable interplanar spacing is synthesized using graphitic carbon nitride (g-C3N4) as precursor with the assistance of polyvinylpyrrolidone (PVP). The obtained tunable interplanar spacing in the range from 0.34 nm to 0.45 nm with enlarged values is mainly ascribed to the high nitrogen doping levels (9.98–33.7 at. %), especially to the pyrrolic nitrogen. Serving as the anode materials in lithium ions batteries (LIBs) and sodium ions batteries (SIBs), promising specific capacities of 1236 mAh g−1 for LIBs and 300 mAh g−1 for SIBs at current density of 0.05 A g−1 and excellent cycling stability as well as acceptable rate capability are demonstrated for the resultant N-doped graphene. The influences of interplanar spacing on the electrochemical performances of LIBs and SIBs are investigated comparatively. This work outlines a facial route to synthesize N-doped graphene with tunable interplanar spacing, meeting the various requirements unitized as anodes in rechargeable Li+/Na+/K+ ions batteries.
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title_short	PVP-assisted synthesis of g–C
remote_bool	true
author2	Wang, Xiao Chen, Jingjing Wang, Xinxin Wang, Dajian Mao, Zhiyong
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doi_str	10.1016/j.carbon.2020.12.010
up_date	2024-07-06T18:21:26.534Z
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score	7.4002113

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PVP-assisted synthesis of g–C

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