A novel UiO-66/PSF-composite membrane for the rejection of multiple antibiotics: Numerical simulation and experiment verification

UiO-66 nanoparticles were fabricated and applied to the support layer of a novel, thin-film nanocomposite membrane for treatment of wastewater containing antibiotics. The incorporation of the UiO-66 particle structure improved the stability and permeability of the membrane. When the membrane with 0....
Ausführliche Beschreibung

Gespeichert in:

Autor*in:	Mu, Tianwei [verfasserIn] Zhang, Yueyang [verfasserIn] Shi, Wei [verfasserIn] Chen, Gang [verfasserIn] Liu, Yanbiao [verfasserIn] Huang, Manhong [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2020

Schlagwörter:	Forward osmosis Electrospinning nanofiber Metal-organic frameworks Antibiotic wastewater Multiple solutes forward-osmosis model

Übergeordnetes Werk:	Enthalten in: Chemosphere - Amsterdam [u.a.] : Elsevier Science, 1972, 269
Übergeordnetes Werk:	volume:269

DOI / URN:	10.1016/j.chemosphere.2020.128686

Katalog-ID:	ELV005561892

Internformat


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245	1	0	\|a A novel UiO-66/PSF-composite membrane for the rejection of multiple antibiotics: Numerical simulation and experiment verification
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520			\|a UiO-66 nanoparticles were fabricated and applied to the support layer of a novel, thin-film nanocomposite membrane for treatment of wastewater containing antibiotics. The incorporation of the UiO-66 particle structure improved the stability and permeability of the membrane. When the membrane with 0.5 wt% of UiO-66 particles was used to treat antibiotic wastewater by a forward-osmosis process, the water flux reached 50.78 LMH (L·m−2·h−1), an increase of 46% compared with the membrane without UiO-66 particles. The rejections of six types of antibiotics improved to over 99.94%. Even trimethoprims rejection rate enhanced to 100% because antibiotics exposed on the surface of the UiO-66 nanoparticles. The forward osmosis model could explain the mechanism of permeation, and predict water flux and rejection. Thus, a novel mathematical model with Gaussian pore distribution and different potential functions was proposed to process multiple-solute transportation and rejection on the charged surface of the membrane. The rejection of six antibiotics was predicted by the iteration algorithm, and the errors of water flux, salt flux, and rejection rates were less than 1.3 LMH, 0.2 gMH (g·m−2 h−1), and 1.7% between the predictions and the experiments, respectively. The accuracy of the proposed model was higher than the model published before. Therefore, the experimental results and the theoretical model provide a significant insight into the synthesis thin-film composite membranes and application of water purification.
650		4	\|a Forward osmosis
650		4	\|a Electrospinning nanofiber
650		4	\|a Metal-organic frameworks
650		4	\|a Antibiotic wastewater
650		4	\|a Multiple solutes forward-osmosis model
700	1		\|a Zhang, Yueyang \|e verfasserin \|4 aut
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700	1		\|a Liu, Yanbiao \|e verfasserin \|4 aut
700	1		\|a Huang, Manhong \|e verfasserin \|4 aut
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936	b	k	\|a 43.00 \|j Umweltforschung \|j Umweltschutz: Allgemeines
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Indexfelder

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publishDate	2020
allfields	10.1016/j.chemosphere.2020.128686 doi (DE-627)ELV005561892 (ELSEVIER)S0045-6535(20)32884-8 DE-627 ger DE-627 rda eng 333.7 DE-600 43.00 bkl Mu, Tianwei verfasserin aut A novel UiO-66/PSF-composite membrane for the rejection of multiple antibiotics: Numerical simulation and experiment verification 2020 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier UiO-66 nanoparticles were fabricated and applied to the support layer of a novel, thin-film nanocomposite membrane for treatment of wastewater containing antibiotics. The incorporation of the UiO-66 particle structure improved the stability and permeability of the membrane. When the membrane with 0.5 wt% of UiO-66 particles was used to treat antibiotic wastewater by a forward-osmosis process, the water flux reached 50.78 LMH (L·m−2·h−1), an increase of 46% compared with the membrane without UiO-66 particles. The rejections of six types of antibiotics improved to over 99.94%. Even trimethoprims rejection rate enhanced to 100% because antibiotics exposed on the surface of the UiO-66 nanoparticles. The forward osmosis model could explain the mechanism of permeation, and predict water flux and rejection. Thus, a novel mathematical model with Gaussian pore distribution and different potential functions was proposed to process multiple-solute transportation and rejection on the charged surface of the membrane. The rejection of six antibiotics was predicted by the iteration algorithm, and the errors of water flux, salt flux, and rejection rates were less than 1.3 LMH, 0.2 gMH (g·m−2 h−1), and 1.7% between the predictions and the experiments, respectively. The accuracy of the proposed model was higher than the model published before. Therefore, the experimental results and the theoretical model provide a significant insight into the synthesis thin-film composite membranes and application of water purification. Forward osmosis Electrospinning nanofiber Metal-organic frameworks Antibiotic wastewater Multiple solutes forward-osmosis model Zhang, Yueyang verfasserin aut Shi, Wei verfasserin aut Chen, Gang verfasserin aut Liu, Yanbiao verfasserin aut Huang, Manhong verfasserin aut Enthalten in Chemosphere Amsterdam [u.a.] : Elsevier Science, 1972 269 Online-Ressource (DE-627)306354217 (DE-600)1496851-4 (DE-576)081952961 1879-1298 nnns volume:269 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA SSG-OPC-GGO GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 43.00 Umweltforschung Umweltschutz: Allgemeines AR 269
spelling	10.1016/j.chemosphere.2020.128686 doi (DE-627)ELV005561892 (ELSEVIER)S0045-6535(20)32884-8 DE-627 ger DE-627 rda eng 333.7 DE-600 43.00 bkl Mu, Tianwei verfasserin aut A novel UiO-66/PSF-composite membrane for the rejection of multiple antibiotics: Numerical simulation and experiment verification 2020 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier UiO-66 nanoparticles were fabricated and applied to the support layer of a novel, thin-film nanocomposite membrane for treatment of wastewater containing antibiotics. The incorporation of the UiO-66 particle structure improved the stability and permeability of the membrane. When the membrane with 0.5 wt% of UiO-66 particles was used to treat antibiotic wastewater by a forward-osmosis process, the water flux reached 50.78 LMH (L·m−2·h−1), an increase of 46% compared with the membrane without UiO-66 particles. The rejections of six types of antibiotics improved to over 99.94%. Even trimethoprims rejection rate enhanced to 100% because antibiotics exposed on the surface of the UiO-66 nanoparticles. The forward osmosis model could explain the mechanism of permeation, and predict water flux and rejection. Thus, a novel mathematical model with Gaussian pore distribution and different potential functions was proposed to process multiple-solute transportation and rejection on the charged surface of the membrane. The rejection of six antibiotics was predicted by the iteration algorithm, and the errors of water flux, salt flux, and rejection rates were less than 1.3 LMH, 0.2 gMH (g·m−2 h−1), and 1.7% between the predictions and the experiments, respectively. The accuracy of the proposed model was higher than the model published before. Therefore, the experimental results and the theoretical model provide a significant insight into the synthesis thin-film composite membranes and application of water purification. Forward osmosis Electrospinning nanofiber Metal-organic frameworks Antibiotic wastewater Multiple solutes forward-osmosis model Zhang, Yueyang verfasserin aut Shi, Wei verfasserin aut Chen, Gang verfasserin aut Liu, Yanbiao verfasserin aut Huang, Manhong verfasserin aut Enthalten in Chemosphere Amsterdam [u.a.] : Elsevier Science, 1972 269 Online-Ressource (DE-627)306354217 (DE-600)1496851-4 (DE-576)081952961 1879-1298 nnns volume:269 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA SSG-OPC-GGO GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 43.00 Umweltforschung Umweltschutz: Allgemeines AR 269
allfields_unstemmed	10.1016/j.chemosphere.2020.128686 doi (DE-627)ELV005561892 (ELSEVIER)S0045-6535(20)32884-8 DE-627 ger DE-627 rda eng 333.7 DE-600 43.00 bkl Mu, Tianwei verfasserin aut A novel UiO-66/PSF-composite membrane for the rejection of multiple antibiotics: Numerical simulation and experiment verification 2020 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier UiO-66 nanoparticles were fabricated and applied to the support layer of a novel, thin-film nanocomposite membrane for treatment of wastewater containing antibiotics. The incorporation of the UiO-66 particle structure improved the stability and permeability of the membrane. When the membrane with 0.5 wt% of UiO-66 particles was used to treat antibiotic wastewater by a forward-osmosis process, the water flux reached 50.78 LMH (L·m−2·h−1), an increase of 46% compared with the membrane without UiO-66 particles. The rejections of six types of antibiotics improved to over 99.94%. Even trimethoprims rejection rate enhanced to 100% because antibiotics exposed on the surface of the UiO-66 nanoparticles. The forward osmosis model could explain the mechanism of permeation, and predict water flux and rejection. Thus, a novel mathematical model with Gaussian pore distribution and different potential functions was proposed to process multiple-solute transportation and rejection on the charged surface of the membrane. The rejection of six antibiotics was predicted by the iteration algorithm, and the errors of water flux, salt flux, and rejection rates were less than 1.3 LMH, 0.2 gMH (g·m−2 h−1), and 1.7% between the predictions and the experiments, respectively. The accuracy of the proposed model was higher than the model published before. Therefore, the experimental results and the theoretical model provide a significant insight into the synthesis thin-film composite membranes and application of water purification. Forward osmosis Electrospinning nanofiber Metal-organic frameworks Antibiotic wastewater Multiple solutes forward-osmosis model Zhang, Yueyang verfasserin aut Shi, Wei verfasserin aut Chen, Gang verfasserin aut Liu, Yanbiao verfasserin aut Huang, Manhong verfasserin aut Enthalten in Chemosphere Amsterdam [u.a.] : Elsevier Science, 1972 269 Online-Ressource (DE-627)306354217 (DE-600)1496851-4 (DE-576)081952961 1879-1298 nnns volume:269 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA SSG-OPC-GGO GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 43.00 Umweltforschung Umweltschutz: Allgemeines AR 269
allfieldsGer	10.1016/j.chemosphere.2020.128686 doi (DE-627)ELV005561892 (ELSEVIER)S0045-6535(20)32884-8 DE-627 ger DE-627 rda eng 333.7 DE-600 43.00 bkl Mu, Tianwei verfasserin aut A novel UiO-66/PSF-composite membrane for the rejection of multiple antibiotics: Numerical simulation and experiment verification 2020 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier UiO-66 nanoparticles were fabricated and applied to the support layer of a novel, thin-film nanocomposite membrane for treatment of wastewater containing antibiotics. The incorporation of the UiO-66 particle structure improved the stability and permeability of the membrane. When the membrane with 0.5 wt% of UiO-66 particles was used to treat antibiotic wastewater by a forward-osmosis process, the water flux reached 50.78 LMH (L·m−2·h−1), an increase of 46% compared with the membrane without UiO-66 particles. The rejections of six types of antibiotics improved to over 99.94%. Even trimethoprims rejection rate enhanced to 100% because antibiotics exposed on the surface of the UiO-66 nanoparticles. The forward osmosis model could explain the mechanism of permeation, and predict water flux and rejection. Thus, a novel mathematical model with Gaussian pore distribution and different potential functions was proposed to process multiple-solute transportation and rejection on the charged surface of the membrane. The rejection of six antibiotics was predicted by the iteration algorithm, and the errors of water flux, salt flux, and rejection rates were less than 1.3 LMH, 0.2 gMH (g·m−2 h−1), and 1.7% between the predictions and the experiments, respectively. The accuracy of the proposed model was higher than the model published before. Therefore, the experimental results and the theoretical model provide a significant insight into the synthesis thin-film composite membranes and application of water purification. Forward osmosis Electrospinning nanofiber Metal-organic frameworks Antibiotic wastewater Multiple solutes forward-osmosis model Zhang, Yueyang verfasserin aut Shi, Wei verfasserin aut Chen, Gang verfasserin aut Liu, Yanbiao verfasserin aut Huang, Manhong verfasserin aut Enthalten in Chemosphere Amsterdam [u.a.] : Elsevier Science, 1972 269 Online-Ressource (DE-627)306354217 (DE-600)1496851-4 (DE-576)081952961 1879-1298 nnns volume:269 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA SSG-OPC-GGO GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 43.00 Umweltforschung Umweltschutz: Allgemeines AR 269
allfieldsSound	10.1016/j.chemosphere.2020.128686 doi (DE-627)ELV005561892 (ELSEVIER)S0045-6535(20)32884-8 DE-627 ger DE-627 rda eng 333.7 DE-600 43.00 bkl Mu, Tianwei verfasserin aut A novel UiO-66/PSF-composite membrane for the rejection of multiple antibiotics: Numerical simulation and experiment verification 2020 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier UiO-66 nanoparticles were fabricated and applied to the support layer of a novel, thin-film nanocomposite membrane for treatment of wastewater containing antibiotics. The incorporation of the UiO-66 particle structure improved the stability and permeability of the membrane. When the membrane with 0.5 wt% of UiO-66 particles was used to treat antibiotic wastewater by a forward-osmosis process, the water flux reached 50.78 LMH (L·m−2·h−1), an increase of 46% compared with the membrane without UiO-66 particles. The rejections of six types of antibiotics improved to over 99.94%. Even trimethoprims rejection rate enhanced to 100% because antibiotics exposed on the surface of the UiO-66 nanoparticles. The forward osmosis model could explain the mechanism of permeation, and predict water flux and rejection. Thus, a novel mathematical model with Gaussian pore distribution and different potential functions was proposed to process multiple-solute transportation and rejection on the charged surface of the membrane. The rejection of six antibiotics was predicted by the iteration algorithm, and the errors of water flux, salt flux, and rejection rates were less than 1.3 LMH, 0.2 gMH (g·m−2 h−1), and 1.7% between the predictions and the experiments, respectively. The accuracy of the proposed model was higher than the model published before. Therefore, the experimental results and the theoretical model provide a significant insight into the synthesis thin-film composite membranes and application of water purification. Forward osmosis Electrospinning nanofiber Metal-organic frameworks Antibiotic wastewater Multiple solutes forward-osmosis model Zhang, Yueyang verfasserin aut Shi, Wei verfasserin aut Chen, Gang verfasserin aut Liu, Yanbiao verfasserin aut Huang, Manhong verfasserin aut Enthalten in Chemosphere Amsterdam [u.a.] : Elsevier Science, 1972 269 Online-Ressource (DE-627)306354217 (DE-600)1496851-4 (DE-576)081952961 1879-1298 nnns volume:269 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA SSG-OPC-GGO GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 43.00 Umweltforschung Umweltschutz: Allgemeines AR 269
language	English
source	Enthalten in Chemosphere 269 volume:269
sourceStr	Enthalten in Chemosphere 269 volume:269
format_phy_str_mv	Article
bklname	Umweltforschung Umweltschutz: Allgemeines
institution	findex.gbv.de
topic_facet	Forward osmosis Electrospinning nanofiber Metal-organic frameworks Antibiotic wastewater Multiple solutes forward-osmosis model
dewey-raw	333.7
isfreeaccess_bool	false
container_title	Chemosphere
authorswithroles_txt_mv	Mu, Tianwei @@aut@@ Zhang, Yueyang @@aut@@ Shi, Wei @@aut@@ Chen, Gang @@aut@@ Liu, Yanbiao @@aut@@ Huang, Manhong @@aut@@
publishDateDaySort_date	2020-01-01T00:00:00Z
hierarchy_top_id	306354217
dewey-sort	3333.7
id	ELV005561892
language_de	englisch
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author	Mu, Tianwei
spellingShingle	Mu, Tianwei ddc 333.7 bkl 43.00 misc Forward osmosis misc Electrospinning nanofiber misc Metal-organic frameworks misc Antibiotic wastewater misc Multiple solutes forward-osmosis model A novel UiO-66/PSF-composite membrane for the rejection of multiple antibiotics: Numerical simulation and experiment verification
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topic_title	333.7 DE-600 43.00 bkl A novel UiO-66/PSF-composite membrane for the rejection of multiple antibiotics: Numerical simulation and experiment verification Forward osmosis Electrospinning nanofiber Metal-organic frameworks Antibiotic wastewater Multiple solutes forward-osmosis model
topic	ddc 333.7 bkl 43.00 misc Forward osmosis misc Electrospinning nanofiber misc Metal-organic frameworks misc Antibiotic wastewater misc Multiple solutes forward-osmosis model
topic_unstemmed	ddc 333.7 bkl 43.00 misc Forward osmosis misc Electrospinning nanofiber misc Metal-organic frameworks misc Antibiotic wastewater misc Multiple solutes forward-osmosis model
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title	A novel UiO-66/PSF-composite membrane for the rejection of multiple antibiotics: Numerical simulation and experiment verification
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title_full	A novel UiO-66/PSF-composite membrane for the rejection of multiple antibiotics: Numerical simulation and experiment verification
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author_browse	Mu, Tianwei Zhang, Yueyang Shi, Wei Chen, Gang Liu, Yanbiao Huang, Manhong
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title_sort	a novel uio-66/psf-composite membrane for the rejection of multiple antibiotics: numerical simulation and experiment verification
title_auth	A novel UiO-66/PSF-composite membrane for the rejection of multiple antibiotics: Numerical simulation and experiment verification
abstract	UiO-66 nanoparticles were fabricated and applied to the support layer of a novel, thin-film nanocomposite membrane for treatment of wastewater containing antibiotics. The incorporation of the UiO-66 particle structure improved the stability and permeability of the membrane. When the membrane with 0.5 wt% of UiO-66 particles was used to treat antibiotic wastewater by a forward-osmosis process, the water flux reached 50.78 LMH (L·m−2·h−1), an increase of 46% compared with the membrane without UiO-66 particles. The rejections of six types of antibiotics improved to over 99.94%. Even trimethoprims rejection rate enhanced to 100% because antibiotics exposed on the surface of the UiO-66 nanoparticles. The forward osmosis model could explain the mechanism of permeation, and predict water flux and rejection. Thus, a novel mathematical model with Gaussian pore distribution and different potential functions was proposed to process multiple-solute transportation and rejection on the charged surface of the membrane. The rejection of six antibiotics was predicted by the iteration algorithm, and the errors of water flux, salt flux, and rejection rates were less than 1.3 LMH, 0.2 gMH (g·m−2 h−1), and 1.7% between the predictions and the experiments, respectively. The accuracy of the proposed model was higher than the model published before. Therefore, the experimental results and the theoretical model provide a significant insight into the synthesis thin-film composite membranes and application of water purification.
abstractGer	UiO-66 nanoparticles were fabricated and applied to the support layer of a novel, thin-film nanocomposite membrane for treatment of wastewater containing antibiotics. The incorporation of the UiO-66 particle structure improved the stability and permeability of the membrane. When the membrane with 0.5 wt% of UiO-66 particles was used to treat antibiotic wastewater by a forward-osmosis process, the water flux reached 50.78 LMH (L·m−2·h−1), an increase of 46% compared with the membrane without UiO-66 particles. The rejections of six types of antibiotics improved to over 99.94%. Even trimethoprims rejection rate enhanced to 100% because antibiotics exposed on the surface of the UiO-66 nanoparticles. The forward osmosis model could explain the mechanism of permeation, and predict water flux and rejection. Thus, a novel mathematical model with Gaussian pore distribution and different potential functions was proposed to process multiple-solute transportation and rejection on the charged surface of the membrane. The rejection of six antibiotics was predicted by the iteration algorithm, and the errors of water flux, salt flux, and rejection rates were less than 1.3 LMH, 0.2 gMH (g·m−2 h−1), and 1.7% between the predictions and the experiments, respectively. The accuracy of the proposed model was higher than the model published before. Therefore, the experimental results and the theoretical model provide a significant insight into the synthesis thin-film composite membranes and application of water purification.
abstract_unstemmed	UiO-66 nanoparticles were fabricated and applied to the support layer of a novel, thin-film nanocomposite membrane for treatment of wastewater containing antibiotics. The incorporation of the UiO-66 particle structure improved the stability and permeability of the membrane. When the membrane with 0.5 wt% of UiO-66 particles was used to treat antibiotic wastewater by a forward-osmosis process, the water flux reached 50.78 LMH (L·m−2·h−1), an increase of 46% compared with the membrane without UiO-66 particles. The rejections of six types of antibiotics improved to over 99.94%. Even trimethoprims rejection rate enhanced to 100% because antibiotics exposed on the surface of the UiO-66 nanoparticles. The forward osmosis model could explain the mechanism of permeation, and predict water flux and rejection. Thus, a novel mathematical model with Gaussian pore distribution and different potential functions was proposed to process multiple-solute transportation and rejection on the charged surface of the membrane. The rejection of six antibiotics was predicted by the iteration algorithm, and the errors of water flux, salt flux, and rejection rates were less than 1.3 LMH, 0.2 gMH (g·m−2 h−1), and 1.7% between the predictions and the experiments, respectively. The accuracy of the proposed model was higher than the model published before. Therefore, the experimental results and the theoretical model provide a significant insight into the synthesis thin-film composite membranes and application of water purification.
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title_short	A novel UiO-66/PSF-composite membrane for the rejection of multiple antibiotics: Numerical simulation and experiment verification
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author2	Zhang, Yueyang Shi, Wei Chen, Gang Liu, Yanbiao Huang, Manhong
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up_date	2024-07-06T18:23:26.753Z
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A novel UiO-66/PSF-composite membrane for the rejection of multiple antibiotics: Numerical simulation and experiment verification

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