Co-pyrolysis characteristics of camellia oleifera shell and coal in a TGA and a fixed-bed reactor

The pyrolysis characteristics of camellia oleifera shell (COS), coal and their mixture were investigated using a thermogravimetric analyzer (TGA) and fixed-bed reactor. The decomposition reactions and kinetic analyses of COS, coal and their mixture from using TGA were compared. The results showed th...
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Autor*in:	Zhang, Caixia [verfasserIn] Li, Shuqi [verfasserIn] Ouyang, Shaobo [verfasserIn] Tsang, Chi-Wing [verfasserIn] Xiong, Daolin [verfasserIn] Yang, Kai [verfasserIn] Zhou, Yuanfang [verfasserIn] Xiao, Yahui [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2021

Schlagwörter:	Camellia oleifera shell Coal Co-pyrolysis Synergistic effect Kinetic analysis

Übergeordnetes Werk:	Enthalten in: Journal of analytical and applied pyrolysis - New York, NY [u.a.] : Science Direct, 1979, 155
Übergeordnetes Werk:	volume:155

DOI / URN:	10.1016/j.jaap.2021.105035

Katalog-ID:	ELV005840961

Internformat


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024	7		\|a 10.1016/j.jaap.2021.105035 \|2 doi
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264		1	\|c 2021
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520			\|a The pyrolysis characteristics of camellia oleifera shell (COS), coal and their mixture were investigated using a thermogravimetric analyzer (TGA) and fixed-bed reactor. The decomposition reactions and kinetic analyses of COS, coal and their mixture from using TGA were compared. The results showed that during the pyrolysis process of COS and coal lonely, heat transfer hysteresis would occur with the increase of heating rates, and the synergistic effects during the co-pyrolysis of COS and coal could be enhanced by increasing the proportion of COS. In addition, from the results of kinetic analyses, in the range of 666∼750 °C, the activation energy (Ea) was gradually decreased with the increase of COS content, which was from about 59.7 kJ/mol to 12.7 kJ/mol. The effects of mixing ratio of COS to coal, pyrolysis temperature and heating rate on the pyrolysis process were further evaluated by using the fixed-bed reactor, and the optimal operating conditions were found (60% COS mixing ratio, 600 °C, and 10 °C/min) to obtain a higher yield of liquid around 30% and modifying the product composition. Gas products containing hydrogen, carbon-monoxide, carbon-dioxide and hydrocarbons were analyzed by gas chromatography (GC). Interestingly, the tar produced by co-pyrolysis of the blends was mainly composed of small molecule such as phenols, and there were basically no polycyclic aromatic hydrocarbons. For the fixed-bed reactor, the synergistic effects mainly impacted on the product composition, rather than the % distribution of the products.
650		4	\|a Camellia oleifera shell
650		4	\|a Coal
650		4	\|a Co-pyrolysis
650		4	\|a Synergistic effect
650		4	\|a Kinetic analysis
700	1		\|a Li, Shuqi \|e verfasserin \|4 aut
700	1		\|a Ouyang, Shaobo \|e verfasserin \|4 aut
700	1		\|a Tsang, Chi-Wing \|e verfasserin \|4 aut
700	1		\|a Xiong, Daolin \|e verfasserin \|4 aut
700	1		\|a Yang, Kai \|e verfasserin \|4 aut
700	1		\|a Zhou, Yuanfang \|e verfasserin \|4 aut
700	1		\|a Xiao, Yahui \|e verfasserin \|4 aut
773	0	8	\|i Enthalten in \|t Journal of analytical and applied pyrolysis \|d New York, NY [u.a.] : Science Direct, 1979 \|g 155 \|h Online-Ressource \|w (DE-627)301512841 \|w (DE-600)1484647-0 \|w (DE-576)259483877 \|x 0165-2370 \|7 nnns
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936	b	k	\|a 52.51 \|j Feuerungstechnik
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matchkey_str	article:01652370:2021----::oyoyicaatrsisfaelalieahladolnt
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publishDate	2021
allfields	10.1016/j.jaap.2021.105035 doi (DE-627)ELV005840961 (ELSEVIER)S0165-2370(21)00021-8 DE-627 ger DE-627 rda eng 660 DE-600 52.51 bkl 35.24 bkl Zhang, Caixia verfasserin aut Co-pyrolysis characteristics of camellia oleifera shell and coal in a TGA and a fixed-bed reactor 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The pyrolysis characteristics of camellia oleifera shell (COS), coal and their mixture were investigated using a thermogravimetric analyzer (TGA) and fixed-bed reactor. The decomposition reactions and kinetic analyses of COS, coal and their mixture from using TGA were compared. The results showed that during the pyrolysis process of COS and coal lonely, heat transfer hysteresis would occur with the increase of heating rates, and the synergistic effects during the co-pyrolysis of COS and coal could be enhanced by increasing the proportion of COS. In addition, from the results of kinetic analyses, in the range of 666∼750 °C, the activation energy (Ea) was gradually decreased with the increase of COS content, which was from about 59.7 kJ/mol to 12.7 kJ/mol. The effects of mixing ratio of COS to coal, pyrolysis temperature and heating rate on the pyrolysis process were further evaluated by using the fixed-bed reactor, and the optimal operating conditions were found (60% COS mixing ratio, 600 °C, and 10 °C/min) to obtain a higher yield of liquid around 30% and modifying the product composition. Gas products containing hydrogen, carbon-monoxide, carbon-dioxide and hydrocarbons were analyzed by gas chromatography (GC). Interestingly, the tar produced by co-pyrolysis of the blends was mainly composed of small molecule such as phenols, and there were basically no polycyclic aromatic hydrocarbons. For the fixed-bed reactor, the synergistic effects mainly impacted on the product composition, rather than the % distribution of the products. Camellia oleifera shell Coal Co-pyrolysis Synergistic effect Kinetic analysis Li, Shuqi verfasserin aut Ouyang, Shaobo verfasserin aut Tsang, Chi-Wing verfasserin aut Xiong, Daolin verfasserin aut Yang, Kai verfasserin aut Zhou, Yuanfang verfasserin aut Xiao, Yahui verfasserin aut Enthalten in Journal of analytical and applied pyrolysis New York, NY [u.a.] : Science Direct, 1979 155 Online-Ressource (DE-627)301512841 (DE-600)1484647-0 (DE-576)259483877 0165-2370 nnns volume:155 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 52.51 Feuerungstechnik 35.24 Klassische analytische Chemie AR 155
spelling	10.1016/j.jaap.2021.105035 doi (DE-627)ELV005840961 (ELSEVIER)S0165-2370(21)00021-8 DE-627 ger DE-627 rda eng 660 DE-600 52.51 bkl 35.24 bkl Zhang, Caixia verfasserin aut Co-pyrolysis characteristics of camellia oleifera shell and coal in a TGA and a fixed-bed reactor 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The pyrolysis characteristics of camellia oleifera shell (COS), coal and their mixture were investigated using a thermogravimetric analyzer (TGA) and fixed-bed reactor. The decomposition reactions and kinetic analyses of COS, coal and their mixture from using TGA were compared. The results showed that during the pyrolysis process of COS and coal lonely, heat transfer hysteresis would occur with the increase of heating rates, and the synergistic effects during the co-pyrolysis of COS and coal could be enhanced by increasing the proportion of COS. In addition, from the results of kinetic analyses, in the range of 666∼750 °C, the activation energy (Ea) was gradually decreased with the increase of COS content, which was from about 59.7 kJ/mol to 12.7 kJ/mol. The effects of mixing ratio of COS to coal, pyrolysis temperature and heating rate on the pyrolysis process were further evaluated by using the fixed-bed reactor, and the optimal operating conditions were found (60% COS mixing ratio, 600 °C, and 10 °C/min) to obtain a higher yield of liquid around 30% and modifying the product composition. Gas products containing hydrogen, carbon-monoxide, carbon-dioxide and hydrocarbons were analyzed by gas chromatography (GC). Interestingly, the tar produced by co-pyrolysis of the blends was mainly composed of small molecule such as phenols, and there were basically no polycyclic aromatic hydrocarbons. For the fixed-bed reactor, the synergistic effects mainly impacted on the product composition, rather than the % distribution of the products. Camellia oleifera shell Coal Co-pyrolysis Synergistic effect Kinetic analysis Li, Shuqi verfasserin aut Ouyang, Shaobo verfasserin aut Tsang, Chi-Wing verfasserin aut Xiong, Daolin verfasserin aut Yang, Kai verfasserin aut Zhou, Yuanfang verfasserin aut Xiao, Yahui verfasserin aut Enthalten in Journal of analytical and applied pyrolysis New York, NY [u.a.] : Science Direct, 1979 155 Online-Ressource (DE-627)301512841 (DE-600)1484647-0 (DE-576)259483877 0165-2370 nnns volume:155 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 52.51 Feuerungstechnik 35.24 Klassische analytische Chemie AR 155
allfields_unstemmed	10.1016/j.jaap.2021.105035 doi (DE-627)ELV005840961 (ELSEVIER)S0165-2370(21)00021-8 DE-627 ger DE-627 rda eng 660 DE-600 52.51 bkl 35.24 bkl Zhang, Caixia verfasserin aut Co-pyrolysis characteristics of camellia oleifera shell and coal in a TGA and a fixed-bed reactor 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The pyrolysis characteristics of camellia oleifera shell (COS), coal and their mixture were investigated using a thermogravimetric analyzer (TGA) and fixed-bed reactor. The decomposition reactions and kinetic analyses of COS, coal and their mixture from using TGA were compared. The results showed that during the pyrolysis process of COS and coal lonely, heat transfer hysteresis would occur with the increase of heating rates, and the synergistic effects during the co-pyrolysis of COS and coal could be enhanced by increasing the proportion of COS. In addition, from the results of kinetic analyses, in the range of 666∼750 °C, the activation energy (Ea) was gradually decreased with the increase of COS content, which was from about 59.7 kJ/mol to 12.7 kJ/mol. The effects of mixing ratio of COS to coal, pyrolysis temperature and heating rate on the pyrolysis process were further evaluated by using the fixed-bed reactor, and the optimal operating conditions were found (60% COS mixing ratio, 600 °C, and 10 °C/min) to obtain a higher yield of liquid around 30% and modifying the product composition. Gas products containing hydrogen, carbon-monoxide, carbon-dioxide and hydrocarbons were analyzed by gas chromatography (GC). Interestingly, the tar produced by co-pyrolysis of the blends was mainly composed of small molecule such as phenols, and there were basically no polycyclic aromatic hydrocarbons. For the fixed-bed reactor, the synergistic effects mainly impacted on the product composition, rather than the % distribution of the products. Camellia oleifera shell Coal Co-pyrolysis Synergistic effect Kinetic analysis Li, Shuqi verfasserin aut Ouyang, Shaobo verfasserin aut Tsang, Chi-Wing verfasserin aut Xiong, Daolin verfasserin aut Yang, Kai verfasserin aut Zhou, Yuanfang verfasserin aut Xiao, Yahui verfasserin aut Enthalten in Journal of analytical and applied pyrolysis New York, NY [u.a.] : Science Direct, 1979 155 Online-Ressource (DE-627)301512841 (DE-600)1484647-0 (DE-576)259483877 0165-2370 nnns volume:155 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 52.51 Feuerungstechnik 35.24 Klassische analytische Chemie AR 155
allfieldsGer	10.1016/j.jaap.2021.105035 doi (DE-627)ELV005840961 (ELSEVIER)S0165-2370(21)00021-8 DE-627 ger DE-627 rda eng 660 DE-600 52.51 bkl 35.24 bkl Zhang, Caixia verfasserin aut Co-pyrolysis characteristics of camellia oleifera shell and coal in a TGA and a fixed-bed reactor 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The pyrolysis characteristics of camellia oleifera shell (COS), coal and their mixture were investigated using a thermogravimetric analyzer (TGA) and fixed-bed reactor. The decomposition reactions and kinetic analyses of COS, coal and their mixture from using TGA were compared. The results showed that during the pyrolysis process of COS and coal lonely, heat transfer hysteresis would occur with the increase of heating rates, and the synergistic effects during the co-pyrolysis of COS and coal could be enhanced by increasing the proportion of COS. In addition, from the results of kinetic analyses, in the range of 666∼750 °C, the activation energy (Ea) was gradually decreased with the increase of COS content, which was from about 59.7 kJ/mol to 12.7 kJ/mol. The effects of mixing ratio of COS to coal, pyrolysis temperature and heating rate on the pyrolysis process were further evaluated by using the fixed-bed reactor, and the optimal operating conditions were found (60% COS mixing ratio, 600 °C, and 10 °C/min) to obtain a higher yield of liquid around 30% and modifying the product composition. Gas products containing hydrogen, carbon-monoxide, carbon-dioxide and hydrocarbons were analyzed by gas chromatography (GC). Interestingly, the tar produced by co-pyrolysis of the blends was mainly composed of small molecule such as phenols, and there were basically no polycyclic aromatic hydrocarbons. For the fixed-bed reactor, the synergistic effects mainly impacted on the product composition, rather than the % distribution of the products. Camellia oleifera shell Coal Co-pyrolysis Synergistic effect Kinetic analysis Li, Shuqi verfasserin aut Ouyang, Shaobo verfasserin aut Tsang, Chi-Wing verfasserin aut Xiong, Daolin verfasserin aut Yang, Kai verfasserin aut Zhou, Yuanfang verfasserin aut Xiao, Yahui verfasserin aut Enthalten in Journal of analytical and applied pyrolysis New York, NY [u.a.] : Science Direct, 1979 155 Online-Ressource (DE-627)301512841 (DE-600)1484647-0 (DE-576)259483877 0165-2370 nnns volume:155 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 52.51 Feuerungstechnik 35.24 Klassische analytische Chemie AR 155
allfieldsSound	10.1016/j.jaap.2021.105035 doi (DE-627)ELV005840961 (ELSEVIER)S0165-2370(21)00021-8 DE-627 ger DE-627 rda eng 660 DE-600 52.51 bkl 35.24 bkl Zhang, Caixia verfasserin aut Co-pyrolysis characteristics of camellia oleifera shell and coal in a TGA and a fixed-bed reactor 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The pyrolysis characteristics of camellia oleifera shell (COS), coal and their mixture were investigated using a thermogravimetric analyzer (TGA) and fixed-bed reactor. The decomposition reactions and kinetic analyses of COS, coal and their mixture from using TGA were compared. The results showed that during the pyrolysis process of COS and coal lonely, heat transfer hysteresis would occur with the increase of heating rates, and the synergistic effects during the co-pyrolysis of COS and coal could be enhanced by increasing the proportion of COS. In addition, from the results of kinetic analyses, in the range of 666∼750 °C, the activation energy (Ea) was gradually decreased with the increase of COS content, which was from about 59.7 kJ/mol to 12.7 kJ/mol. The effects of mixing ratio of COS to coal, pyrolysis temperature and heating rate on the pyrolysis process were further evaluated by using the fixed-bed reactor, and the optimal operating conditions were found (60% COS mixing ratio, 600 °C, and 10 °C/min) to obtain a higher yield of liquid around 30% and modifying the product composition. Gas products containing hydrogen, carbon-monoxide, carbon-dioxide and hydrocarbons were analyzed by gas chromatography (GC). Interestingly, the tar produced by co-pyrolysis of the blends was mainly composed of small molecule such as phenols, and there were basically no polycyclic aromatic hydrocarbons. For the fixed-bed reactor, the synergistic effects mainly impacted on the product composition, rather than the % distribution of the products. Camellia oleifera shell Coal Co-pyrolysis Synergistic effect Kinetic analysis Li, Shuqi verfasserin aut Ouyang, Shaobo verfasserin aut Tsang, Chi-Wing verfasserin aut Xiong, Daolin verfasserin aut Yang, Kai verfasserin aut Zhou, Yuanfang verfasserin aut Xiao, Yahui verfasserin aut Enthalten in Journal of analytical and applied pyrolysis New York, NY [u.a.] : Science Direct, 1979 155 Online-Ressource (DE-627)301512841 (DE-600)1484647-0 (DE-576)259483877 0165-2370 nnns volume:155 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 52.51 Feuerungstechnik 35.24 Klassische analytische Chemie AR 155
language	English
source	Enthalten in Journal of analytical and applied pyrolysis 155 volume:155
sourceStr	Enthalten in Journal of analytical and applied pyrolysis 155 volume:155
format_phy_str_mv	Article
bklname	Feuerungstechnik Klassische analytische Chemie
institution	findex.gbv.de
topic_facet	Camellia oleifera shell Coal Co-pyrolysis Synergistic effect Kinetic analysis
dewey-raw	660
isfreeaccess_bool	false
container_title	Journal of analytical and applied pyrolysis
authorswithroles_txt_mv	Zhang, Caixia @@aut@@ Li, Shuqi @@aut@@ Ouyang, Shaobo @@aut@@ Tsang, Chi-Wing @@aut@@ Xiong, Daolin @@aut@@ Yang, Kai @@aut@@ Zhou, Yuanfang @@aut@@ Xiao, Yahui @@aut@@
publishDateDaySort_date	2021-01-01T00:00:00Z
hierarchy_top_id	301512841
dewey-sort	3660
id	ELV005840961
language_de	englisch
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Gas products containing hydrogen, carbon-monoxide, carbon-dioxide and hydrocarbons were analyzed by gas chromatography (GC). Interestingly, the tar produced by co-pyrolysis of the blends was mainly composed of small molecule such as phenols, and there were basically no polycyclic aromatic hydrocarbons. 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author	Zhang, Caixia
spellingShingle	Zhang, Caixia ddc 660 bkl 52.51 bkl 35.24 misc Camellia oleifera shell misc Coal misc Co-pyrolysis misc Synergistic effect misc Kinetic analysis Co-pyrolysis characteristics of camellia oleifera shell and coal in a TGA and a fixed-bed reactor
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topic_title	660 DE-600 52.51 bkl 35.24 bkl Co-pyrolysis characteristics of camellia oleifera shell and coal in a TGA and a fixed-bed reactor Camellia oleifera shell Coal Co-pyrolysis Synergistic effect Kinetic analysis
topic	ddc 660 bkl 52.51 bkl 35.24 misc Camellia oleifera shell misc Coal misc Co-pyrolysis misc Synergistic effect misc Kinetic analysis
topic_unstemmed	ddc 660 bkl 52.51 bkl 35.24 misc Camellia oleifera shell misc Coal misc Co-pyrolysis misc Synergistic effect misc Kinetic analysis
topic_browse	ddc 660 bkl 52.51 bkl 35.24 misc Camellia oleifera shell misc Coal misc Co-pyrolysis misc Synergistic effect misc Kinetic analysis
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title	Co-pyrolysis characteristics of camellia oleifera shell and coal in a TGA and a fixed-bed reactor
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title_full	Co-pyrolysis characteristics of camellia oleifera shell and coal in a TGA and a fixed-bed reactor
author_sort	Zhang, Caixia
journal	Journal of analytical and applied pyrolysis
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author_browse	Zhang, Caixia Li, Shuqi Ouyang, Shaobo Tsang, Chi-Wing Xiong, Daolin Yang, Kai Zhou, Yuanfang Xiao, Yahui
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author-letter	Zhang, Caixia
doi_str_mv	10.1016/j.jaap.2021.105035
dewey-full	660
author2-role	verfasserin
title_sort	co-pyrolysis characteristics of camellia oleifera shell and coal in a tga and a fixed-bed reactor
title_auth	Co-pyrolysis characteristics of camellia oleifera shell and coal in a TGA and a fixed-bed reactor
abstract	The pyrolysis characteristics of camellia oleifera shell (COS), coal and their mixture were investigated using a thermogravimetric analyzer (TGA) and fixed-bed reactor. The decomposition reactions and kinetic analyses of COS, coal and their mixture from using TGA were compared. The results showed that during the pyrolysis process of COS and coal lonely, heat transfer hysteresis would occur with the increase of heating rates, and the synergistic effects during the co-pyrolysis of COS and coal could be enhanced by increasing the proportion of COS. In addition, from the results of kinetic analyses, in the range of 666∼750 °C, the activation energy (Ea) was gradually decreased with the increase of COS content, which was from about 59.7 kJ/mol to 12.7 kJ/mol. The effects of mixing ratio of COS to coal, pyrolysis temperature and heating rate on the pyrolysis process were further evaluated by using the fixed-bed reactor, and the optimal operating conditions were found (60% COS mixing ratio, 600 °C, and 10 °C/min) to obtain a higher yield of liquid around 30% and modifying the product composition. Gas products containing hydrogen, carbon-monoxide, carbon-dioxide and hydrocarbons were analyzed by gas chromatography (GC). Interestingly, the tar produced by co-pyrolysis of the blends was mainly composed of small molecule such as phenols, and there were basically no polycyclic aromatic hydrocarbons. For the fixed-bed reactor, the synergistic effects mainly impacted on the product composition, rather than the % distribution of the products.
abstractGer	The pyrolysis characteristics of camellia oleifera shell (COS), coal and their mixture were investigated using a thermogravimetric analyzer (TGA) and fixed-bed reactor. The decomposition reactions and kinetic analyses of COS, coal and their mixture from using TGA were compared. The results showed that during the pyrolysis process of COS and coal lonely, heat transfer hysteresis would occur with the increase of heating rates, and the synergistic effects during the co-pyrolysis of COS and coal could be enhanced by increasing the proportion of COS. In addition, from the results of kinetic analyses, in the range of 666∼750 °C, the activation energy (Ea) was gradually decreased with the increase of COS content, which was from about 59.7 kJ/mol to 12.7 kJ/mol. The effects of mixing ratio of COS to coal, pyrolysis temperature and heating rate on the pyrolysis process were further evaluated by using the fixed-bed reactor, and the optimal operating conditions were found (60% COS mixing ratio, 600 °C, and 10 °C/min) to obtain a higher yield of liquid around 30% and modifying the product composition. Gas products containing hydrogen, carbon-monoxide, carbon-dioxide and hydrocarbons were analyzed by gas chromatography (GC). Interestingly, the tar produced by co-pyrolysis of the blends was mainly composed of small molecule such as phenols, and there were basically no polycyclic aromatic hydrocarbons. For the fixed-bed reactor, the synergistic effects mainly impacted on the product composition, rather than the % distribution of the products.
abstract_unstemmed	The pyrolysis characteristics of camellia oleifera shell (COS), coal and their mixture were investigated using a thermogravimetric analyzer (TGA) and fixed-bed reactor. The decomposition reactions and kinetic analyses of COS, coal and their mixture from using TGA were compared. The results showed that during the pyrolysis process of COS and coal lonely, heat transfer hysteresis would occur with the increase of heating rates, and the synergistic effects during the co-pyrolysis of COS and coal could be enhanced by increasing the proportion of COS. In addition, from the results of kinetic analyses, in the range of 666∼750 °C, the activation energy (Ea) was gradually decreased with the increase of COS content, which was from about 59.7 kJ/mol to 12.7 kJ/mol. The effects of mixing ratio of COS to coal, pyrolysis temperature and heating rate on the pyrolysis process were further evaluated by using the fixed-bed reactor, and the optimal operating conditions were found (60% COS mixing ratio, 600 °C, and 10 °C/min) to obtain a higher yield of liquid around 30% and modifying the product composition. Gas products containing hydrogen, carbon-monoxide, carbon-dioxide and hydrocarbons were analyzed by gas chromatography (GC). Interestingly, the tar produced by co-pyrolysis of the blends was mainly composed of small molecule such as phenols, and there were basically no polycyclic aromatic hydrocarbons. For the fixed-bed reactor, the synergistic effects mainly impacted on the product composition, rather than the % distribution of the products.
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title_short	Co-pyrolysis characteristics of camellia oleifera shell and coal in a TGA and a fixed-bed reactor
remote_bool	true
author2	Li, Shuqi Ouyang, Shaobo Tsang, Chi-Wing Xiong, Daolin Yang, Kai Zhou, Yuanfang Xiao, Yahui
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doi_str	10.1016/j.jaap.2021.105035
up_date	2024-07-06T19:20:48.311Z
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Co-pyrolysis characteristics of camellia oleifera shell and coal in a TGA and a fixed-bed reactor

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