Interfacial polarization triggered by glutamate accelerates dehydration of hydrated zinc ions for zinc-ion batteries
The huge activation energy barrier during the dehydration of hydrated zinc ions ([Zn(H2O)6]2+ → 6H2O + Zn2+) of aqueous zinc-ion batteries (ZIBs) has limited their capacity and hindered their development. Here, we report a novel and efficient method for accelerating the dehydration of hydrated zinc...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Jin, Yan Qi [verfasserIn] Chen, Hongzhan [verfasserIn] Peng, Linhui [verfasserIn] Chen, Zehai [verfasserIn] Cheng, Luo [verfasserIn] Song, Jidong [verfasserIn] Zhang, Hao [verfasserIn] Chen, Jian [verfasserIn] Xie, Fangyan [verfasserIn] Jin, Yanshuo [verfasserIn] Shi, Jifu [verfasserIn] Meng, Hui [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2020 |
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| Schlagwörter: |
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| Übergeordnetes Werk: |
Enthalten in: The chemical engineering journal - Amsterdam : Elsevier, 1997, 416 |
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| Übergeordnetes Werk: |
volume:416 |
| DOI / URN: |
10.1016/j.cej.2020.127704 |
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| Katalog-ID: |
ELV005919266 |
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| 245 | 1 | 0 | |a Interfacial polarization triggered by glutamate accelerates dehydration of hydrated zinc ions for zinc-ion batteries |
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| 520 | |a The huge activation energy barrier during the dehydration of hydrated zinc ions ([Zn(H2O)6]2+ → 6H2O + Zn2+) of aqueous zinc-ion batteries (ZIBs) has limited their capacity and hindered their development. Here, we report a novel and efficient method for accelerating the dehydration of hydrated zinc ions through interfacial polarization triggered by glutamate. Using MoS2 as a research model, the specific capacity of the MoS2 adsorbed by glutamate (Glu-MoS2) increased from 72 mAh g−1 to 182 mAh g−1, which is 2.5 times the original specific capacity. Different from changing the structure of materials, surface treatment also can significantly improve performance. In addition, there is a reversible phase conversion from the 2H phase to the 1 T phase during the charging and discharging process of Glu-MoS2, which plays an important role in optimizing the performance. The interfacial polarization caused by glutamate to reduce the activation energy of dehydration provides a new strategy to increase the capacity of ZIBs. | ||
| 650 | 4 | |a Zinc-ion battery | |
| 650 | 4 | |a Molybdenum disulfide | |
| 650 | 4 | |a Adsorption | |
| 650 | 4 | |a Interfacial polarization | |
| 650 | 4 | |a Dehydration | |
| 700 | 1 | |a Chen, Hongzhan |e verfasserin |4 aut | |
| 700 | 1 | |a Peng, Linhui |e verfasserin |4 aut | |
| 700 | 1 | |a Chen, Zehai |e verfasserin |4 aut | |
| 700 | 1 | |a Cheng, Luo |e verfasserin |4 aut | |
| 700 | 1 | |a Song, Jidong |e verfasserin |4 aut | |
| 700 | 1 | |a Zhang, Hao |e verfasserin |4 aut | |
| 700 | 1 | |a Chen, Jian |e verfasserin |4 aut | |
| 700 | 1 | |a Xie, Fangyan |e verfasserin |4 aut | |
| 700 | 1 | |a Jin, Yanshuo |e verfasserin |4 aut | |
| 700 | 1 | |a Shi, Jifu |e verfasserin |4 aut | |
| 700 | 1 | |a Meng, Hui |e verfasserin |4 aut | |
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10.1016/j.cej.2020.127704 doi (DE-627)ELV005919266 (ELSEVIER)S1385-8947(20)33826-2 DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Jin, Yan Qi verfasserin aut Interfacial polarization triggered by glutamate accelerates dehydration of hydrated zinc ions for zinc-ion batteries 2020 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The huge activation energy barrier during the dehydration of hydrated zinc ions ([Zn(H2O)6]2+ → 6H2O + Zn2+) of aqueous zinc-ion batteries (ZIBs) has limited their capacity and hindered their development. Here, we report a novel and efficient method for accelerating the dehydration of hydrated zinc ions through interfacial polarization triggered by glutamate. Using MoS2 as a research model, the specific capacity of the MoS2 adsorbed by glutamate (Glu-MoS2) increased from 72 mAh g−1 to 182 mAh g−1, which is 2.5 times the original specific capacity. Different from changing the structure of materials, surface treatment also can significantly improve performance. In addition, there is a reversible phase conversion from the 2H phase to the 1 T phase during the charging and discharging process of Glu-MoS2, which plays an important role in optimizing the performance. The interfacial polarization caused by glutamate to reduce the activation energy of dehydration provides a new strategy to increase the capacity of ZIBs. Zinc-ion battery Molybdenum disulfide Adsorption Interfacial polarization Dehydration Chen, Hongzhan verfasserin aut Peng, Linhui verfasserin aut Chen, Zehai verfasserin aut Cheng, Luo verfasserin aut Song, Jidong verfasserin aut Zhang, Hao verfasserin aut Chen, Jian verfasserin aut Xie, Fangyan verfasserin aut Jin, Yanshuo verfasserin aut Shi, Jifu verfasserin aut Meng, Hui verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 416 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:416 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 416 045F 660.05 |
| spelling |
10.1016/j.cej.2020.127704 doi (DE-627)ELV005919266 (ELSEVIER)S1385-8947(20)33826-2 DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Jin, Yan Qi verfasserin aut Interfacial polarization triggered by glutamate accelerates dehydration of hydrated zinc ions for zinc-ion batteries 2020 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The huge activation energy barrier during the dehydration of hydrated zinc ions ([Zn(H2O)6]2+ → 6H2O + Zn2+) of aqueous zinc-ion batteries (ZIBs) has limited their capacity and hindered their development. Here, we report a novel and efficient method for accelerating the dehydration of hydrated zinc ions through interfacial polarization triggered by glutamate. Using MoS2 as a research model, the specific capacity of the MoS2 adsorbed by glutamate (Glu-MoS2) increased from 72 mAh g−1 to 182 mAh g−1, which is 2.5 times the original specific capacity. Different from changing the structure of materials, surface treatment also can significantly improve performance. In addition, there is a reversible phase conversion from the 2H phase to the 1 T phase during the charging and discharging process of Glu-MoS2, which plays an important role in optimizing the performance. The interfacial polarization caused by glutamate to reduce the activation energy of dehydration provides a new strategy to increase the capacity of ZIBs. Zinc-ion battery Molybdenum disulfide Adsorption Interfacial polarization Dehydration Chen, Hongzhan verfasserin aut Peng, Linhui verfasserin aut Chen, Zehai verfasserin aut Cheng, Luo verfasserin aut Song, Jidong verfasserin aut Zhang, Hao verfasserin aut Chen, Jian verfasserin aut Xie, Fangyan verfasserin aut Jin, Yanshuo verfasserin aut Shi, Jifu verfasserin aut Meng, Hui verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 416 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:416 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 416 045F 660.05 |
| allfields_unstemmed |
10.1016/j.cej.2020.127704 doi (DE-627)ELV005919266 (ELSEVIER)S1385-8947(20)33826-2 DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Jin, Yan Qi verfasserin aut Interfacial polarization triggered by glutamate accelerates dehydration of hydrated zinc ions for zinc-ion batteries 2020 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The huge activation energy barrier during the dehydration of hydrated zinc ions ([Zn(H2O)6]2+ → 6H2O + Zn2+) of aqueous zinc-ion batteries (ZIBs) has limited their capacity and hindered their development. Here, we report a novel and efficient method for accelerating the dehydration of hydrated zinc ions through interfacial polarization triggered by glutamate. Using MoS2 as a research model, the specific capacity of the MoS2 adsorbed by glutamate (Glu-MoS2) increased from 72 mAh g−1 to 182 mAh g−1, which is 2.5 times the original specific capacity. Different from changing the structure of materials, surface treatment also can significantly improve performance. In addition, there is a reversible phase conversion from the 2H phase to the 1 T phase during the charging and discharging process of Glu-MoS2, which plays an important role in optimizing the performance. The interfacial polarization caused by glutamate to reduce the activation energy of dehydration provides a new strategy to increase the capacity of ZIBs. Zinc-ion battery Molybdenum disulfide Adsorption Interfacial polarization Dehydration Chen, Hongzhan verfasserin aut Peng, Linhui verfasserin aut Chen, Zehai verfasserin aut Cheng, Luo verfasserin aut Song, Jidong verfasserin aut Zhang, Hao verfasserin aut Chen, Jian verfasserin aut Xie, Fangyan verfasserin aut Jin, Yanshuo verfasserin aut Shi, Jifu verfasserin aut Meng, Hui verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 416 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:416 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 416 045F 660.05 |
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10.1016/j.cej.2020.127704 doi (DE-627)ELV005919266 (ELSEVIER)S1385-8947(20)33826-2 DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Jin, Yan Qi verfasserin aut Interfacial polarization triggered by glutamate accelerates dehydration of hydrated zinc ions for zinc-ion batteries 2020 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The huge activation energy barrier during the dehydration of hydrated zinc ions ([Zn(H2O)6]2+ → 6H2O + Zn2+) of aqueous zinc-ion batteries (ZIBs) has limited their capacity and hindered their development. Here, we report a novel and efficient method for accelerating the dehydration of hydrated zinc ions through interfacial polarization triggered by glutamate. Using MoS2 as a research model, the specific capacity of the MoS2 adsorbed by glutamate (Glu-MoS2) increased from 72 mAh g−1 to 182 mAh g−1, which is 2.5 times the original specific capacity. Different from changing the structure of materials, surface treatment also can significantly improve performance. In addition, there is a reversible phase conversion from the 2H phase to the 1 T phase during the charging and discharging process of Glu-MoS2, which plays an important role in optimizing the performance. The interfacial polarization caused by glutamate to reduce the activation energy of dehydration provides a new strategy to increase the capacity of ZIBs. Zinc-ion battery Molybdenum disulfide Adsorption Interfacial polarization Dehydration Chen, Hongzhan verfasserin aut Peng, Linhui verfasserin aut Chen, Zehai verfasserin aut Cheng, Luo verfasserin aut Song, Jidong verfasserin aut Zhang, Hao verfasserin aut Chen, Jian verfasserin aut Xie, Fangyan verfasserin aut Jin, Yanshuo verfasserin aut Shi, Jifu verfasserin aut Meng, Hui verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 416 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:416 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 416 045F 660.05 |
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10.1016/j.cej.2020.127704 doi (DE-627)ELV005919266 (ELSEVIER)S1385-8947(20)33826-2 DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Jin, Yan Qi verfasserin aut Interfacial polarization triggered by glutamate accelerates dehydration of hydrated zinc ions for zinc-ion batteries 2020 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The huge activation energy barrier during the dehydration of hydrated zinc ions ([Zn(H2O)6]2+ → 6H2O + Zn2+) of aqueous zinc-ion batteries (ZIBs) has limited their capacity and hindered their development. Here, we report a novel and efficient method for accelerating the dehydration of hydrated zinc ions through interfacial polarization triggered by glutamate. Using MoS2 as a research model, the specific capacity of the MoS2 adsorbed by glutamate (Glu-MoS2) increased from 72 mAh g−1 to 182 mAh g−1, which is 2.5 times the original specific capacity. Different from changing the structure of materials, surface treatment also can significantly improve performance. In addition, there is a reversible phase conversion from the 2H phase to the 1 T phase during the charging and discharging process of Glu-MoS2, which plays an important role in optimizing the performance. The interfacial polarization caused by glutamate to reduce the activation energy of dehydration provides a new strategy to increase the capacity of ZIBs. Zinc-ion battery Molybdenum disulfide Adsorption Interfacial polarization Dehydration Chen, Hongzhan verfasserin aut Peng, Linhui verfasserin aut Chen, Zehai verfasserin aut Cheng, Luo verfasserin aut Song, Jidong verfasserin aut Zhang, Hao verfasserin aut Chen, Jian verfasserin aut Xie, Fangyan verfasserin aut Jin, Yanshuo verfasserin aut Shi, Jifu verfasserin aut Meng, Hui verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 416 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:416 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 416 045F 660.05 |
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Jin, Yan Qi @@aut@@ Chen, Hongzhan @@aut@@ Peng, Linhui @@aut@@ Chen, Zehai @@aut@@ Cheng, Luo @@aut@@ Song, Jidong @@aut@@ Zhang, Hao @@aut@@ Chen, Jian @@aut@@ Xie, Fangyan @@aut@@ Jin, Yanshuo @@aut@@ Shi, Jifu @@aut@@ Meng, Hui @@aut@@ |
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Jin, Yan Qi |
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Jin, Yan Qi ddc 660.05 ddc 660 bkl 58.10 misc Zinc-ion battery misc Molybdenum disulfide misc Adsorption misc Interfacial polarization misc Dehydration Interfacial polarization triggered by glutamate accelerates dehydration of hydrated zinc ions for zinc-ion batteries |
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660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Interfacial polarization triggered by glutamate accelerates dehydration of hydrated zinc ions for zinc-ion batteries Zinc-ion battery Molybdenum disulfide Adsorption Interfacial polarization Dehydration |
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Interfacial polarization triggered by glutamate accelerates dehydration of hydrated zinc ions for zinc-ion batteries |
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Jin, Yan Qi Chen, Hongzhan Peng, Linhui Chen, Zehai Cheng, Luo Song, Jidong Zhang, Hao Chen, Jian Xie, Fangyan Jin, Yanshuo Shi, Jifu Meng, Hui |
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interfacial polarization triggered by glutamate accelerates dehydration of hydrated zinc ions for zinc-ion batteries |
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Interfacial polarization triggered by glutamate accelerates dehydration of hydrated zinc ions for zinc-ion batteries |
| abstract |
The huge activation energy barrier during the dehydration of hydrated zinc ions ([Zn(H2O)6]2+ → 6H2O + Zn2+) of aqueous zinc-ion batteries (ZIBs) has limited their capacity and hindered their development. Here, we report a novel and efficient method for accelerating the dehydration of hydrated zinc ions through interfacial polarization triggered by glutamate. Using MoS2 as a research model, the specific capacity of the MoS2 adsorbed by glutamate (Glu-MoS2) increased from 72 mAh g−1 to 182 mAh g−1, which is 2.5 times the original specific capacity. Different from changing the structure of materials, surface treatment also can significantly improve performance. In addition, there is a reversible phase conversion from the 2H phase to the 1 T phase during the charging and discharging process of Glu-MoS2, which plays an important role in optimizing the performance. The interfacial polarization caused by glutamate to reduce the activation energy of dehydration provides a new strategy to increase the capacity of ZIBs. |
| abstractGer |
The huge activation energy barrier during the dehydration of hydrated zinc ions ([Zn(H2O)6]2+ → 6H2O + Zn2+) of aqueous zinc-ion batteries (ZIBs) has limited their capacity and hindered their development. Here, we report a novel and efficient method for accelerating the dehydration of hydrated zinc ions through interfacial polarization triggered by glutamate. Using MoS2 as a research model, the specific capacity of the MoS2 adsorbed by glutamate (Glu-MoS2) increased from 72 mAh g−1 to 182 mAh g−1, which is 2.5 times the original specific capacity. Different from changing the structure of materials, surface treatment also can significantly improve performance. In addition, there is a reversible phase conversion from the 2H phase to the 1 T phase during the charging and discharging process of Glu-MoS2, which plays an important role in optimizing the performance. The interfacial polarization caused by glutamate to reduce the activation energy of dehydration provides a new strategy to increase the capacity of ZIBs. |
| abstract_unstemmed |
The huge activation energy barrier during the dehydration of hydrated zinc ions ([Zn(H2O)6]2+ → 6H2O + Zn2+) of aqueous zinc-ion batteries (ZIBs) has limited their capacity and hindered their development. Here, we report a novel and efficient method for accelerating the dehydration of hydrated zinc ions through interfacial polarization triggered by glutamate. Using MoS2 as a research model, the specific capacity of the MoS2 adsorbed by glutamate (Glu-MoS2) increased from 72 mAh g−1 to 182 mAh g−1, which is 2.5 times the original specific capacity. Different from changing the structure of materials, surface treatment also can significantly improve performance. In addition, there is a reversible phase conversion from the 2H phase to the 1 T phase during the charging and discharging process of Glu-MoS2, which plays an important role in optimizing the performance. The interfacial polarization caused by glutamate to reduce the activation energy of dehydration provides a new strategy to increase the capacity of ZIBs. |
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Interfacial polarization triggered by glutamate accelerates dehydration of hydrated zinc ions for zinc-ion batteries |
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Chen, Hongzhan Peng, Linhui Chen, Zehai Cheng, Luo Song, Jidong Zhang, Hao Chen, Jian Xie, Fangyan Jin, Yanshuo Shi, Jifu Meng, Hui |
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