Minimized external electric field on asymmetric monolayer maximizes charge separation for photocatalysis

Controlling charge flow direction is an effective strategy for carrier separation to improve photocatalytic performance. Herein, we create an external electric field (EEF) by chemically loading [Mo3S7]4+ clusters on the S-Zn side of asymmetric ZnIn2S4 (ZIS) monolayers to steer the charge flow. The E...
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Autor*in:	Yang, Weijie [verfasserIn] Wang, Xiao-Li [verfasserIn] Kong, Ningning [verfasserIn] Liu, Chengdong [verfasserIn] Sun, Peipei [verfasserIn] Wang, Zhiqiang [verfasserIn] Ding, Yayun [verfasserIn] Lin, Haiping [verfasserIn] Li, Dongsheng [verfasserIn] Wu, Tao [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2021

Schlagwörter:	External electric field Charged cluster Asymmetric monolayer Selective bond Charge separation

Übergeordnetes Werk:	Enthalten in: Applied catalysis / B - Amsterdam : Elsevier, 1992, 295
Übergeordnetes Werk:	volume:295

DOI / URN:	10.1016/j.apcatb.2021.120266

Katalog-ID:	ELV006039936

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245	1	0	\|a Minimized external electric field on asymmetric monolayer maximizes charge separation for photocatalysis
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520			\|a Controlling charge flow direction is an effective strategy for carrier separation to improve photocatalytic performance. Herein, we create an external electric field (EEF) by chemically loading [Mo3S7]4+ clusters on the S-Zn side of asymmetric ZnIn2S4 (ZIS) monolayers to steer the charge flow. The EEF that stems from the positively charged [Mo3S7]4+ clusters drives photogenerated electrons in the 2D monolayer to the S-Zn side, which are further transferred to the [Mo3S7]4+ clusters through the Mo–S bonds for photocatalytic hydrogen evolution (PHE). This structure exhibits an optimal PHE rate that is four times higher (6.44 mmol g−1 h−1) than that of ZIS (1.6 mmol g−1 h−1). Furthermore, the significance of the EEF for carrier separation was confirmed via density functional theory calculations based on charge density distribution. This special heterojunction provides a new strategy to accelerate the carrier separation in asymmetric 2D materials.
650		4	\|a External electric field
650		4	\|a Charged cluster
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650		4	\|a Selective bond
650		4	\|a Charge separation
700	1		\|a Wang, Xiao-Li \|e verfasserin \|4 aut
700	1		\|a Kong, Ningning \|e verfasserin \|4 aut
700	1		\|a Liu, Chengdong \|e verfasserin \|4 aut
700	1		\|a Sun, Peipei \|e verfasserin \|4 aut
700	1		\|a Wang, Zhiqiang \|e verfasserin \|4 aut
700	1		\|a Ding, Yayun \|e verfasserin \|4 aut
700	1		\|a Lin, Haiping \|e verfasserin \|4 aut
700	1		\|a Li, Dongsheng \|e verfasserin \|4 aut
700	1		\|a Wu, Tao \|e verfasserin \|0 (orcid)0000-0003-4443-1227 \|4 aut
773	0	8	\|i Enthalten in \|t Applied catalysis / B \|d Amsterdam : Elsevier, 1992 \|g 295 \|h Online-Ressource \|w (DE-627)320578658 \|w (DE-600)2017331-3 \|w (DE-576)095956344 \|x 0926-3373 \|7 nnns
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936	b	k	\|a 35.17 \|j Katalyse
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936	b	k	\|a 43.12 \|j Umweltchemie
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allfields	10.1016/j.apcatb.2021.120266 doi (DE-627)ELV006039936 (ELSEVIER)S0926-3373(21)00392-1 DE-627 ger DE-627 rda eng 540 DE-600 35.17 bkl 58.50 bkl 43.12 bkl Yang, Weijie verfasserin aut Minimized external electric field on asymmetric monolayer maximizes charge separation for photocatalysis 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Controlling charge flow direction is an effective strategy for carrier separation to improve photocatalytic performance. Herein, we create an external electric field (EEF) by chemically loading [Mo3S7]4+ clusters on the S-Zn side of asymmetric ZnIn2S4 (ZIS) monolayers to steer the charge flow. The EEF that stems from the positively charged [Mo3S7]4+ clusters drives photogenerated electrons in the 2D monolayer to the S-Zn side, which are further transferred to the [Mo3S7]4+ clusters through the Mo–S bonds for photocatalytic hydrogen evolution (PHE). This structure exhibits an optimal PHE rate that is four times higher (6.44 mmol g−1 h−1) than that of ZIS (1.6 mmol g−1 h−1). Furthermore, the significance of the EEF for carrier separation was confirmed via density functional theory calculations based on charge density distribution. This special heterojunction provides a new strategy to accelerate the carrier separation in asymmetric 2D materials. External electric field Charged cluster Asymmetric monolayer Selective bond Charge separation Wang, Xiao-Li verfasserin aut Kong, Ningning verfasserin aut Liu, Chengdong verfasserin aut Sun, Peipei verfasserin aut Wang, Zhiqiang verfasserin aut Ding, Yayun verfasserin aut Lin, Haiping verfasserin aut Li, Dongsheng verfasserin aut Wu, Tao verfasserin (orcid)0000-0003-4443-1227 aut Enthalten in Applied catalysis / B Amsterdam : Elsevier, 1992 295 Online-Ressource (DE-627)320578658 (DE-600)2017331-3 (DE-576)095956344 0926-3373 nnns volume:295 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.17 Katalyse 58.50 Umwelttechnik: Allgemeines 43.12 Umweltchemie AR 295
spelling	10.1016/j.apcatb.2021.120266 doi (DE-627)ELV006039936 (ELSEVIER)S0926-3373(21)00392-1 DE-627 ger DE-627 rda eng 540 DE-600 35.17 bkl 58.50 bkl 43.12 bkl Yang, Weijie verfasserin aut Minimized external electric field on asymmetric monolayer maximizes charge separation for photocatalysis 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Controlling charge flow direction is an effective strategy for carrier separation to improve photocatalytic performance. Herein, we create an external electric field (EEF) by chemically loading [Mo3S7]4+ clusters on the S-Zn side of asymmetric ZnIn2S4 (ZIS) monolayers to steer the charge flow. The EEF that stems from the positively charged [Mo3S7]4+ clusters drives photogenerated electrons in the 2D monolayer to the S-Zn side, which are further transferred to the [Mo3S7]4+ clusters through the Mo–S bonds for photocatalytic hydrogen evolution (PHE). This structure exhibits an optimal PHE rate that is four times higher (6.44 mmol g−1 h−1) than that of ZIS (1.6 mmol g−1 h−1). Furthermore, the significance of the EEF for carrier separation was confirmed via density functional theory calculations based on charge density distribution. This special heterojunction provides a new strategy to accelerate the carrier separation in asymmetric 2D materials. External electric field Charged cluster Asymmetric monolayer Selective bond Charge separation Wang, Xiao-Li verfasserin aut Kong, Ningning verfasserin aut Liu, Chengdong verfasserin aut Sun, Peipei verfasserin aut Wang, Zhiqiang verfasserin aut Ding, Yayun verfasserin aut Lin, Haiping verfasserin aut Li, Dongsheng verfasserin aut Wu, Tao verfasserin (orcid)0000-0003-4443-1227 aut Enthalten in Applied catalysis / B Amsterdam : Elsevier, 1992 295 Online-Ressource (DE-627)320578658 (DE-600)2017331-3 (DE-576)095956344 0926-3373 nnns volume:295 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.17 Katalyse 58.50 Umwelttechnik: Allgemeines 43.12 Umweltchemie AR 295
allfields_unstemmed	10.1016/j.apcatb.2021.120266 doi (DE-627)ELV006039936 (ELSEVIER)S0926-3373(21)00392-1 DE-627 ger DE-627 rda eng 540 DE-600 35.17 bkl 58.50 bkl 43.12 bkl Yang, Weijie verfasserin aut Minimized external electric field on asymmetric monolayer maximizes charge separation for photocatalysis 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Controlling charge flow direction is an effective strategy for carrier separation to improve photocatalytic performance. Herein, we create an external electric field (EEF) by chemically loading [Mo3S7]4+ clusters on the S-Zn side of asymmetric ZnIn2S4 (ZIS) monolayers to steer the charge flow. The EEF that stems from the positively charged [Mo3S7]4+ clusters drives photogenerated electrons in the 2D monolayer to the S-Zn side, which are further transferred to the [Mo3S7]4+ clusters through the Mo–S bonds for photocatalytic hydrogen evolution (PHE). This structure exhibits an optimal PHE rate that is four times higher (6.44 mmol g−1 h−1) than that of ZIS (1.6 mmol g−1 h−1). Furthermore, the significance of the EEF for carrier separation was confirmed via density functional theory calculations based on charge density distribution. This special heterojunction provides a new strategy to accelerate the carrier separation in asymmetric 2D materials. External electric field Charged cluster Asymmetric monolayer Selective bond Charge separation Wang, Xiao-Li verfasserin aut Kong, Ningning verfasserin aut Liu, Chengdong verfasserin aut Sun, Peipei verfasserin aut Wang, Zhiqiang verfasserin aut Ding, Yayun verfasserin aut Lin, Haiping verfasserin aut Li, Dongsheng verfasserin aut Wu, Tao verfasserin (orcid)0000-0003-4443-1227 aut Enthalten in Applied catalysis / B Amsterdam : Elsevier, 1992 295 Online-Ressource (DE-627)320578658 (DE-600)2017331-3 (DE-576)095956344 0926-3373 nnns volume:295 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.17 Katalyse 58.50 Umwelttechnik: Allgemeines 43.12 Umweltchemie AR 295
allfieldsGer	10.1016/j.apcatb.2021.120266 doi (DE-627)ELV006039936 (ELSEVIER)S0926-3373(21)00392-1 DE-627 ger DE-627 rda eng 540 DE-600 35.17 bkl 58.50 bkl 43.12 bkl Yang, Weijie verfasserin aut Minimized external electric field on asymmetric monolayer maximizes charge separation for photocatalysis 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Controlling charge flow direction is an effective strategy for carrier separation to improve photocatalytic performance. Herein, we create an external electric field (EEF) by chemically loading [Mo3S7]4+ clusters on the S-Zn side of asymmetric ZnIn2S4 (ZIS) monolayers to steer the charge flow. The EEF that stems from the positively charged [Mo3S7]4+ clusters drives photogenerated electrons in the 2D monolayer to the S-Zn side, which are further transferred to the [Mo3S7]4+ clusters through the Mo–S bonds for photocatalytic hydrogen evolution (PHE). This structure exhibits an optimal PHE rate that is four times higher (6.44 mmol g−1 h−1) than that of ZIS (1.6 mmol g−1 h−1). Furthermore, the significance of the EEF for carrier separation was confirmed via density functional theory calculations based on charge density distribution. This special heterojunction provides a new strategy to accelerate the carrier separation in asymmetric 2D materials. External electric field Charged cluster Asymmetric monolayer Selective bond Charge separation Wang, Xiao-Li verfasserin aut Kong, Ningning verfasserin aut Liu, Chengdong verfasserin aut Sun, Peipei verfasserin aut Wang, Zhiqiang verfasserin aut Ding, Yayun verfasserin aut Lin, Haiping verfasserin aut Li, Dongsheng verfasserin aut Wu, Tao verfasserin (orcid)0000-0003-4443-1227 aut Enthalten in Applied catalysis / B Amsterdam : Elsevier, 1992 295 Online-Ressource (DE-627)320578658 (DE-600)2017331-3 (DE-576)095956344 0926-3373 nnns volume:295 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.17 Katalyse 58.50 Umwelttechnik: Allgemeines 43.12 Umweltchemie AR 295
allfieldsSound	10.1016/j.apcatb.2021.120266 doi (DE-627)ELV006039936 (ELSEVIER)S0926-3373(21)00392-1 DE-627 ger DE-627 rda eng 540 DE-600 35.17 bkl 58.50 bkl 43.12 bkl Yang, Weijie verfasserin aut Minimized external electric field on asymmetric monolayer maximizes charge separation for photocatalysis 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Controlling charge flow direction is an effective strategy for carrier separation to improve photocatalytic performance. Herein, we create an external electric field (EEF) by chemically loading [Mo3S7]4+ clusters on the S-Zn side of asymmetric ZnIn2S4 (ZIS) monolayers to steer the charge flow. The EEF that stems from the positively charged [Mo3S7]4+ clusters drives photogenerated electrons in the 2D monolayer to the S-Zn side, which are further transferred to the [Mo3S7]4+ clusters through the Mo–S bonds for photocatalytic hydrogen evolution (PHE). This structure exhibits an optimal PHE rate that is four times higher (6.44 mmol g−1 h−1) than that of ZIS (1.6 mmol g−1 h−1). Furthermore, the significance of the EEF for carrier separation was confirmed via density functional theory calculations based on charge density distribution. This special heterojunction provides a new strategy to accelerate the carrier separation in asymmetric 2D materials. External electric field Charged cluster Asymmetric monolayer Selective bond Charge separation Wang, Xiao-Li verfasserin aut Kong, Ningning verfasserin aut Liu, Chengdong verfasserin aut Sun, Peipei verfasserin aut Wang, Zhiqiang verfasserin aut Ding, Yayun verfasserin aut Lin, Haiping verfasserin aut Li, Dongsheng verfasserin aut Wu, Tao verfasserin (orcid)0000-0003-4443-1227 aut Enthalten in Applied catalysis / B Amsterdam : Elsevier, 1992 295 Online-Ressource (DE-627)320578658 (DE-600)2017331-3 (DE-576)095956344 0926-3373 nnns volume:295 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.17 Katalyse 58.50 Umwelttechnik: Allgemeines 43.12 Umweltchemie AR 295
language	English
source	Enthalten in Applied catalysis / B 295 volume:295
sourceStr	Enthalten in Applied catalysis / B 295 volume:295
format_phy_str_mv	Article
bklname	Katalyse Umwelttechnik: Allgemeines Umweltchemie
institution	findex.gbv.de
topic_facet	External electric field Charged cluster Asymmetric monolayer Selective bond Charge separation
dewey-raw	540
isfreeaccess_bool	false
container_title	Applied catalysis / B
authorswithroles_txt_mv	Yang, Weijie @@aut@@ Wang, Xiao-Li @@aut@@ Kong, Ningning @@aut@@ Liu, Chengdong @@aut@@ Sun, Peipei @@aut@@ Wang, Zhiqiang @@aut@@ Ding, Yayun @@aut@@ Lin, Haiping @@aut@@ Li, Dongsheng @@aut@@ Wu, Tao @@aut@@
publishDateDaySort_date	2021-01-01T00:00:00Z
hierarchy_top_id	320578658
dewey-sort	3540
id	ELV006039936
language_de	englisch
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author	Yang, Weijie
spellingShingle	Yang, Weijie ddc 540 bkl 35.17 bkl 58.50 bkl 43.12 misc External electric field misc Charged cluster misc Asymmetric monolayer misc Selective bond misc Charge separation Minimized external electric field on asymmetric monolayer maximizes charge separation for photocatalysis
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topic_title	540 DE-600 35.17 bkl 58.50 bkl 43.12 bkl Minimized external electric field on asymmetric monolayer maximizes charge separation for photocatalysis External electric field Charged cluster Asymmetric monolayer Selective bond Charge separation
topic	ddc 540 bkl 35.17 bkl 58.50 bkl 43.12 misc External electric field misc Charged cluster misc Asymmetric monolayer misc Selective bond misc Charge separation
topic_unstemmed	ddc 540 bkl 35.17 bkl 58.50 bkl 43.12 misc External electric field misc Charged cluster misc Asymmetric monolayer misc Selective bond misc Charge separation
topic_browse	ddc 540 bkl 35.17 bkl 58.50 bkl 43.12 misc External electric field misc Charged cluster misc Asymmetric monolayer misc Selective bond misc Charge separation
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title	Minimized external electric field on asymmetric monolayer maximizes charge separation for photocatalysis
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title_full	Minimized external electric field on asymmetric monolayer maximizes charge separation for photocatalysis
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title_sort	minimized external electric field on asymmetric monolayer maximizes charge separation for photocatalysis
title_auth	Minimized external electric field on asymmetric monolayer maximizes charge separation for photocatalysis
abstract	Controlling charge flow direction is an effective strategy for carrier separation to improve photocatalytic performance. Herein, we create an external electric field (EEF) by chemically loading [Mo3S7]4+ clusters on the S-Zn side of asymmetric ZnIn2S4 (ZIS) monolayers to steer the charge flow. The EEF that stems from the positively charged [Mo3S7]4+ clusters drives photogenerated electrons in the 2D monolayer to the S-Zn side, which are further transferred to the [Mo3S7]4+ clusters through the Mo–S bonds for photocatalytic hydrogen evolution (PHE). This structure exhibits an optimal PHE rate that is four times higher (6.44 mmol g−1 h−1) than that of ZIS (1.6 mmol g−1 h−1). Furthermore, the significance of the EEF for carrier separation was confirmed via density functional theory calculations based on charge density distribution. This special heterojunction provides a new strategy to accelerate the carrier separation in asymmetric 2D materials.
abstractGer	Controlling charge flow direction is an effective strategy for carrier separation to improve photocatalytic performance. Herein, we create an external electric field (EEF) by chemically loading [Mo3S7]4+ clusters on the S-Zn side of asymmetric ZnIn2S4 (ZIS) monolayers to steer the charge flow. The EEF that stems from the positively charged [Mo3S7]4+ clusters drives photogenerated electrons in the 2D monolayer to the S-Zn side, which are further transferred to the [Mo3S7]4+ clusters through the Mo–S bonds for photocatalytic hydrogen evolution (PHE). This structure exhibits an optimal PHE rate that is four times higher (6.44 mmol g−1 h−1) than that of ZIS (1.6 mmol g−1 h−1). Furthermore, the significance of the EEF for carrier separation was confirmed via density functional theory calculations based on charge density distribution. This special heterojunction provides a new strategy to accelerate the carrier separation in asymmetric 2D materials.
abstract_unstemmed	Controlling charge flow direction is an effective strategy for carrier separation to improve photocatalytic performance. Herein, we create an external electric field (EEF) by chemically loading [Mo3S7]4+ clusters on the S-Zn side of asymmetric ZnIn2S4 (ZIS) monolayers to steer the charge flow. The EEF that stems from the positively charged [Mo3S7]4+ clusters drives photogenerated electrons in the 2D monolayer to the S-Zn side, which are further transferred to the [Mo3S7]4+ clusters through the Mo–S bonds for photocatalytic hydrogen evolution (PHE). This structure exhibits an optimal PHE rate that is four times higher (6.44 mmol g−1 h−1) than that of ZIS (1.6 mmol g−1 h−1). Furthermore, the significance of the EEF for carrier separation was confirmed via density functional theory calculations based on charge density distribution. This special heterojunction provides a new strategy to accelerate the carrier separation in asymmetric 2D materials.
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title_short	Minimized external electric field on asymmetric monolayer maximizes charge separation for photocatalysis
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author2	Wang, Xiao-Li Kong, Ningning Liu, Chengdong Sun, Peipei Wang, Zhiqiang Ding, Yayun Lin, Haiping Li, Dongsheng Wu, Tao
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up_date	2024-07-06T20:01:04.498Z
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Minimized external electric field on asymmetric monolayer maximizes charge separation for photocatalysis

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