Facile construction of N, P and O ternary self-doped hollow carbon microspheres with hierarchical porous structure for environmental applications

With the aim to develop novel adsorption materials for highly-efficient CO2 capture and organic dye removal, herein, N, P and O ternary self-doped hollow porous carbon microspheres (NPO-HPCSs) were fabricated via one-step direct carbonization of a single polymer precursor-crosslinked polyphosphazene...
Ausführliche Beschreibung

Gespeichert in:

Autor*in:	Fang, Xiaotong [verfasserIn] Wu, Pengchao [verfasserIn] Fu, Jianwei [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2021

Schlagwörter:	Hollow carbon microsphere Adsorption Doping Organic dye CO

Übergeordnetes Werk:	Enthalten in: Microporous and mesoporous materials - Amsterdam [u.a.] : Elsevier, 1998, 321
Übergeordnetes Werk:	volume:321

DOI / URN:	10.1016/j.micromeso.2021.111135

Katalog-ID:	ELV006041329

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520			\|a With the aim to develop novel adsorption materials for highly-efficient CO2 capture and organic dye removal, herein, N, P and O ternary self-doped hollow porous carbon microspheres (NPO-HPCSs) were fabricated via one-step direct carbonization of a single polymer precursor-crosslinked polyphosphazene. The morphology and microstructure of the NPO-HPCSs were characterized through TEM, SEM, XRD, XPS, FT-IR and N2 sorption test. The influences of initial dye concentration, solution pH, temperature and contact time on malachite green (MG) adsorption were systematically studied. Furthermore, three dynamic models coupled with four isotherm models were employed to coordinate the experimental data. Results show that the NPO-HPCSs own high specific surface area of up to 2153.46 m2 g−1, hierarchical pore structure and high heteroatom content. Meanwhile, the NPO-HPCSs delivered remarkably adsorption capacity towards MG (972 mg g−1 at 298 K), rapid adsorbing ratio (adsorption equilibrium time of 60 min), as well as excellent recycling stability. The outstanding adsorption performance of the NPO-HPCSs towards MG was attributed to the synergistic contribution of surface adsorption (electrostatic attraction, Lewis acid-base interaction and π-π stacking) and pore adsorption. Additionally, the NPO-HPCSs exhibited high CO2 capture capacities at atmospheric pressure: 2.84 mmol g−1 at 298 K and 4.83 mmol g−1 at 273 K, respectively.
650		4	\|a Hollow carbon microsphere
650		4	\|a Adsorption
650		4	\|a Doping
650		4	\|a Organic dye
650		4	\|a CO
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publishDate	2021
allfields	10.1016/j.micromeso.2021.111135 doi (DE-627)ELV006041329 (ELSEVIER)S1387-1811(21)00261-4 DE-627 ger DE-627 rda eng 530 DE-600 38.30 bkl 35.68 bkl 33.61 bkl 35.90 bkl 51.45 bkl Fang, Xiaotong verfasserin aut Facile construction of N, P and O ternary self-doped hollow carbon microspheres with hierarchical porous structure for environmental applications 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier With the aim to develop novel adsorption materials for highly-efficient CO2 capture and organic dye removal, herein, N, P and O ternary self-doped hollow porous carbon microspheres (NPO-HPCSs) were fabricated via one-step direct carbonization of a single polymer precursor-crosslinked polyphosphazene. The morphology and microstructure of the NPO-HPCSs were characterized through TEM, SEM, XRD, XPS, FT-IR and N2 sorption test. The influences of initial dye concentration, solution pH, temperature and contact time on malachite green (MG) adsorption were systematically studied. Furthermore, three dynamic models coupled with four isotherm models were employed to coordinate the experimental data. Results show that the NPO-HPCSs own high specific surface area of up to 2153.46 m2 g−1, hierarchical pore structure and high heteroatom content. Meanwhile, the NPO-HPCSs delivered remarkably adsorption capacity towards MG (972 mg g−1 at 298 K), rapid adsorbing ratio (adsorption equilibrium time of 60 min), as well as excellent recycling stability. The outstanding adsorption performance of the NPO-HPCSs towards MG was attributed to the synergistic contribution of surface adsorption (electrostatic attraction, Lewis acid-base interaction and π-π stacking) and pore adsorption. Additionally, the NPO-HPCSs exhibited high CO2 capture capacities at atmospheric pressure: 2.84 mmol g−1 at 298 K and 4.83 mmol g−1 at 273 K, respectively. Hollow carbon microsphere Adsorption Doping Organic dye CO Wu, Pengchao verfasserin aut Fu, Jianwei verfasserin (orcid)0000-0002-2570-2610 aut Enthalten in Microporous and mesoporous materials Amsterdam [u.a.] : Elsevier, 1998 321 Online-Ressource (DE-627)318368277 (DE-600)2012505-7 (DE-576)09529998X 1387-1811 nnns volume:321 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 38.30 Mineralogie 35.68 Organische Verbindungen: Sonstiges 33.61 Festkörperphysik 35.90 Festkörperchemie 51.45 Werkstoffe mit besonderen Eigenschaften AR 321
spelling	10.1016/j.micromeso.2021.111135 doi (DE-627)ELV006041329 (ELSEVIER)S1387-1811(21)00261-4 DE-627 ger DE-627 rda eng 530 DE-600 38.30 bkl 35.68 bkl 33.61 bkl 35.90 bkl 51.45 bkl Fang, Xiaotong verfasserin aut Facile construction of N, P and O ternary self-doped hollow carbon microspheres with hierarchical porous structure for environmental applications 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier With the aim to develop novel adsorption materials for highly-efficient CO2 capture and organic dye removal, herein, N, P and O ternary self-doped hollow porous carbon microspheres (NPO-HPCSs) were fabricated via one-step direct carbonization of a single polymer precursor-crosslinked polyphosphazene. The morphology and microstructure of the NPO-HPCSs were characterized through TEM, SEM, XRD, XPS, FT-IR and N2 sorption test. The influences of initial dye concentration, solution pH, temperature and contact time on malachite green (MG) adsorption were systematically studied. Furthermore, three dynamic models coupled with four isotherm models were employed to coordinate the experimental data. Results show that the NPO-HPCSs own high specific surface area of up to 2153.46 m2 g−1, hierarchical pore structure and high heteroatom content. Meanwhile, the NPO-HPCSs delivered remarkably adsorption capacity towards MG (972 mg g−1 at 298 K), rapid adsorbing ratio (adsorption equilibrium time of 60 min), as well as excellent recycling stability. The outstanding adsorption performance of the NPO-HPCSs towards MG was attributed to the synergistic contribution of surface adsorption (electrostatic attraction, Lewis acid-base interaction and π-π stacking) and pore adsorption. Additionally, the NPO-HPCSs exhibited high CO2 capture capacities at atmospheric pressure: 2.84 mmol g−1 at 298 K and 4.83 mmol g−1 at 273 K, respectively. Hollow carbon microsphere Adsorption Doping Organic dye CO Wu, Pengchao verfasserin aut Fu, Jianwei verfasserin (orcid)0000-0002-2570-2610 aut Enthalten in Microporous and mesoporous materials Amsterdam [u.a.] : Elsevier, 1998 321 Online-Ressource (DE-627)318368277 (DE-600)2012505-7 (DE-576)09529998X 1387-1811 nnns volume:321 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 38.30 Mineralogie 35.68 Organische Verbindungen: Sonstiges 33.61 Festkörperphysik 35.90 Festkörperchemie 51.45 Werkstoffe mit besonderen Eigenschaften AR 321
allfields_unstemmed	10.1016/j.micromeso.2021.111135 doi (DE-627)ELV006041329 (ELSEVIER)S1387-1811(21)00261-4 DE-627 ger DE-627 rda eng 530 DE-600 38.30 bkl 35.68 bkl 33.61 bkl 35.90 bkl 51.45 bkl Fang, Xiaotong verfasserin aut Facile construction of N, P and O ternary self-doped hollow carbon microspheres with hierarchical porous structure for environmental applications 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier With the aim to develop novel adsorption materials for highly-efficient CO2 capture and organic dye removal, herein, N, P and O ternary self-doped hollow porous carbon microspheres (NPO-HPCSs) were fabricated via one-step direct carbonization of a single polymer precursor-crosslinked polyphosphazene. The morphology and microstructure of the NPO-HPCSs were characterized through TEM, SEM, XRD, XPS, FT-IR and N2 sorption test. The influences of initial dye concentration, solution pH, temperature and contact time on malachite green (MG) adsorption were systematically studied. Furthermore, three dynamic models coupled with four isotherm models were employed to coordinate the experimental data. Results show that the NPO-HPCSs own high specific surface area of up to 2153.46 m2 g−1, hierarchical pore structure and high heteroatom content. Meanwhile, the NPO-HPCSs delivered remarkably adsorption capacity towards MG (972 mg g−1 at 298 K), rapid adsorbing ratio (adsorption equilibrium time of 60 min), as well as excellent recycling stability. The outstanding adsorption performance of the NPO-HPCSs towards MG was attributed to the synergistic contribution of surface adsorption (electrostatic attraction, Lewis acid-base interaction and π-π stacking) and pore adsorption. Additionally, the NPO-HPCSs exhibited high CO2 capture capacities at atmospheric pressure: 2.84 mmol g−1 at 298 K and 4.83 mmol g−1 at 273 K, respectively. Hollow carbon microsphere Adsorption Doping Organic dye CO Wu, Pengchao verfasserin aut Fu, Jianwei verfasserin (orcid)0000-0002-2570-2610 aut Enthalten in Microporous and mesoporous materials Amsterdam [u.a.] : Elsevier, 1998 321 Online-Ressource (DE-627)318368277 (DE-600)2012505-7 (DE-576)09529998X 1387-1811 nnns volume:321 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 38.30 Mineralogie 35.68 Organische Verbindungen: Sonstiges 33.61 Festkörperphysik 35.90 Festkörperchemie 51.45 Werkstoffe mit besonderen Eigenschaften AR 321
allfieldsGer	10.1016/j.micromeso.2021.111135 doi (DE-627)ELV006041329 (ELSEVIER)S1387-1811(21)00261-4 DE-627 ger DE-627 rda eng 530 DE-600 38.30 bkl 35.68 bkl 33.61 bkl 35.90 bkl 51.45 bkl Fang, Xiaotong verfasserin aut Facile construction of N, P and O ternary self-doped hollow carbon microspheres with hierarchical porous structure for environmental applications 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier With the aim to develop novel adsorption materials for highly-efficient CO2 capture and organic dye removal, herein, N, P and O ternary self-doped hollow porous carbon microspheres (NPO-HPCSs) were fabricated via one-step direct carbonization of a single polymer precursor-crosslinked polyphosphazene. The morphology and microstructure of the NPO-HPCSs were characterized through TEM, SEM, XRD, XPS, FT-IR and N2 sorption test. The influences of initial dye concentration, solution pH, temperature and contact time on malachite green (MG) adsorption were systematically studied. Furthermore, three dynamic models coupled with four isotherm models were employed to coordinate the experimental data. Results show that the NPO-HPCSs own high specific surface area of up to 2153.46 m2 g−1, hierarchical pore structure and high heteroatom content. Meanwhile, the NPO-HPCSs delivered remarkably adsorption capacity towards MG (972 mg g−1 at 298 K), rapid adsorbing ratio (adsorption equilibrium time of 60 min), as well as excellent recycling stability. The outstanding adsorption performance of the NPO-HPCSs towards MG was attributed to the synergistic contribution of surface adsorption (electrostatic attraction, Lewis acid-base interaction and π-π stacking) and pore adsorption. Additionally, the NPO-HPCSs exhibited high CO2 capture capacities at atmospheric pressure: 2.84 mmol g−1 at 298 K and 4.83 mmol g−1 at 273 K, respectively. Hollow carbon microsphere Adsorption Doping Organic dye CO Wu, Pengchao verfasserin aut Fu, Jianwei verfasserin (orcid)0000-0002-2570-2610 aut Enthalten in Microporous and mesoporous materials Amsterdam [u.a.] : Elsevier, 1998 321 Online-Ressource (DE-627)318368277 (DE-600)2012505-7 (DE-576)09529998X 1387-1811 nnns volume:321 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 38.30 Mineralogie 35.68 Organische Verbindungen: Sonstiges 33.61 Festkörperphysik 35.90 Festkörperchemie 51.45 Werkstoffe mit besonderen Eigenschaften AR 321
allfieldsSound	10.1016/j.micromeso.2021.111135 doi (DE-627)ELV006041329 (ELSEVIER)S1387-1811(21)00261-4 DE-627 ger DE-627 rda eng 530 DE-600 38.30 bkl 35.68 bkl 33.61 bkl 35.90 bkl 51.45 bkl Fang, Xiaotong verfasserin aut Facile construction of N, P and O ternary self-doped hollow carbon microspheres with hierarchical porous structure for environmental applications 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier With the aim to develop novel adsorption materials for highly-efficient CO2 capture and organic dye removal, herein, N, P and O ternary self-doped hollow porous carbon microspheres (NPO-HPCSs) were fabricated via one-step direct carbonization of a single polymer precursor-crosslinked polyphosphazene. The morphology and microstructure of the NPO-HPCSs were characterized through TEM, SEM, XRD, XPS, FT-IR and N2 sorption test. The influences of initial dye concentration, solution pH, temperature and contact time on malachite green (MG) adsorption were systematically studied. Furthermore, three dynamic models coupled with four isotherm models were employed to coordinate the experimental data. Results show that the NPO-HPCSs own high specific surface area of up to 2153.46 m2 g−1, hierarchical pore structure and high heteroatom content. Meanwhile, the NPO-HPCSs delivered remarkably adsorption capacity towards MG (972 mg g−1 at 298 K), rapid adsorbing ratio (adsorption equilibrium time of 60 min), as well as excellent recycling stability. The outstanding adsorption performance of the NPO-HPCSs towards MG was attributed to the synergistic contribution of surface adsorption (electrostatic attraction, Lewis acid-base interaction and π-π stacking) and pore adsorption. Additionally, the NPO-HPCSs exhibited high CO2 capture capacities at atmospheric pressure: 2.84 mmol g−1 at 298 K and 4.83 mmol g−1 at 273 K, respectively. Hollow carbon microsphere Adsorption Doping Organic dye CO Wu, Pengchao verfasserin aut Fu, Jianwei verfasserin (orcid)0000-0002-2570-2610 aut Enthalten in Microporous and mesoporous materials Amsterdam [u.a.] : Elsevier, 1998 321 Online-Ressource (DE-627)318368277 (DE-600)2012505-7 (DE-576)09529998X 1387-1811 nnns volume:321 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 38.30 Mineralogie 35.68 Organische Verbindungen: Sonstiges 33.61 Festkörperphysik 35.90 Festkörperchemie 51.45 Werkstoffe mit besonderen Eigenschaften AR 321
language	English
source	Enthalten in Microporous and mesoporous materials 321 volume:321
sourceStr	Enthalten in Microporous and mesoporous materials 321 volume:321
format_phy_str_mv	Article
bklname	Mineralogie Organische Verbindungen: Sonstiges Festkörperphysik Festkörperchemie Werkstoffe mit besonderen Eigenschaften
institution	findex.gbv.de
topic_facet	Hollow carbon microsphere Adsorption Doping Organic dye CO
dewey-raw	530
isfreeaccess_bool	false
container_title	Microporous and mesoporous materials
authorswithroles_txt_mv	Fang, Xiaotong @@aut@@ Wu, Pengchao @@aut@@ Fu, Jianwei @@aut@@
publishDateDaySort_date	2021-01-01T00:00:00Z
hierarchy_top_id	318368277
dewey-sort	3530
id	ELV006041329
language_de	englisch
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The morphology and microstructure of the NPO-HPCSs were characterized through TEM, SEM, XRD, XPS, FT-IR and N2 sorption test. The influences of initial dye concentration, solution pH, temperature and contact time on malachite green (MG) adsorption were systematically studied. Furthermore, three dynamic models coupled with four isotherm models were employed to coordinate the experimental data. Results show that the NPO-HPCSs own high specific surface area of up to 2153.46 m2 g−1, hierarchical pore structure and high heteroatom content. Meanwhile, the NPO-HPCSs delivered remarkably adsorption capacity towards MG (972 mg g−1 at 298 K), rapid adsorbing ratio (adsorption equilibrium time of 60 min), as well as excellent recycling stability. The outstanding adsorption performance of the NPO-HPCSs towards MG was attributed to the synergistic contribution of surface adsorption (electrostatic attraction, Lewis acid-base interaction and π-π stacking) and pore adsorption. 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author	Fang, Xiaotong
spellingShingle	Fang, Xiaotong ddc 530 bkl 38.30 bkl 35.68 bkl 33.61 bkl 35.90 bkl 51.45 misc Hollow carbon microsphere misc Adsorption misc Doping misc Organic dye misc CO Facile construction of N, P and O ternary self-doped hollow carbon microspheres with hierarchical porous structure for environmental applications
authorStr	Fang, Xiaotong
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topic_title	530 DE-600 38.30 bkl 35.68 bkl 33.61 bkl 35.90 bkl 51.45 bkl Facile construction of N, P and O ternary self-doped hollow carbon microspheres with hierarchical porous structure for environmental applications Hollow carbon microsphere Adsorption Doping Organic dye CO
topic	ddc 530 bkl 38.30 bkl 35.68 bkl 33.61 bkl 35.90 bkl 51.45 misc Hollow carbon microsphere misc Adsorption misc Doping misc Organic dye misc CO
topic_unstemmed	ddc 530 bkl 38.30 bkl 35.68 bkl 33.61 bkl 35.90 bkl 51.45 misc Hollow carbon microsphere misc Adsorption misc Doping misc Organic dye misc CO
topic_browse	ddc 530 bkl 38.30 bkl 35.68 bkl 33.61 bkl 35.90 bkl 51.45 misc Hollow carbon microsphere misc Adsorption misc Doping misc Organic dye misc CO
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title	Facile construction of N, P and O ternary self-doped hollow carbon microspheres with hierarchical porous structure for environmental applications
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title_full	Facile construction of N, P and O ternary self-doped hollow carbon microspheres with hierarchical porous structure for environmental applications
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author_browse	Fang, Xiaotong Wu, Pengchao Fu, Jianwei
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title_sort	facile construction of n, p and o ternary self-doped hollow carbon microspheres with hierarchical porous structure for environmental applications
title_auth	Facile construction of N, P and O ternary self-doped hollow carbon microspheres with hierarchical porous structure for environmental applications
abstract	With the aim to develop novel adsorption materials for highly-efficient CO2 capture and organic dye removal, herein, N, P and O ternary self-doped hollow porous carbon microspheres (NPO-HPCSs) were fabricated via one-step direct carbonization of a single polymer precursor-crosslinked polyphosphazene. The morphology and microstructure of the NPO-HPCSs were characterized through TEM, SEM, XRD, XPS, FT-IR and N2 sorption test. The influences of initial dye concentration, solution pH, temperature and contact time on malachite green (MG) adsorption were systematically studied. Furthermore, three dynamic models coupled with four isotherm models were employed to coordinate the experimental data. Results show that the NPO-HPCSs own high specific surface area of up to 2153.46 m2 g−1, hierarchical pore structure and high heteroatom content. Meanwhile, the NPO-HPCSs delivered remarkably adsorption capacity towards MG (972 mg g−1 at 298 K), rapid adsorbing ratio (adsorption equilibrium time of 60 min), as well as excellent recycling stability. The outstanding adsorption performance of the NPO-HPCSs towards MG was attributed to the synergistic contribution of surface adsorption (electrostatic attraction, Lewis acid-base interaction and π-π stacking) and pore adsorption. Additionally, the NPO-HPCSs exhibited high CO2 capture capacities at atmospheric pressure: 2.84 mmol g−1 at 298 K and 4.83 mmol g−1 at 273 K, respectively.
abstractGer	With the aim to develop novel adsorption materials for highly-efficient CO2 capture and organic dye removal, herein, N, P and O ternary self-doped hollow porous carbon microspheres (NPO-HPCSs) were fabricated via one-step direct carbonization of a single polymer precursor-crosslinked polyphosphazene. The morphology and microstructure of the NPO-HPCSs were characterized through TEM, SEM, XRD, XPS, FT-IR and N2 sorption test. The influences of initial dye concentration, solution pH, temperature and contact time on malachite green (MG) adsorption were systematically studied. Furthermore, three dynamic models coupled with four isotherm models were employed to coordinate the experimental data. Results show that the NPO-HPCSs own high specific surface area of up to 2153.46 m2 g−1, hierarchical pore structure and high heteroatom content. Meanwhile, the NPO-HPCSs delivered remarkably adsorption capacity towards MG (972 mg g−1 at 298 K), rapid adsorbing ratio (adsorption equilibrium time of 60 min), as well as excellent recycling stability. The outstanding adsorption performance of the NPO-HPCSs towards MG was attributed to the synergistic contribution of surface adsorption (electrostatic attraction, Lewis acid-base interaction and π-π stacking) and pore adsorption. Additionally, the NPO-HPCSs exhibited high CO2 capture capacities at atmospheric pressure: 2.84 mmol g−1 at 298 K and 4.83 mmol g−1 at 273 K, respectively.
abstract_unstemmed	With the aim to develop novel adsorption materials for highly-efficient CO2 capture and organic dye removal, herein, N, P and O ternary self-doped hollow porous carbon microspheres (NPO-HPCSs) were fabricated via one-step direct carbonization of a single polymer precursor-crosslinked polyphosphazene. The morphology and microstructure of the NPO-HPCSs were characterized through TEM, SEM, XRD, XPS, FT-IR and N2 sorption test. The influences of initial dye concentration, solution pH, temperature and contact time on malachite green (MG) adsorption were systematically studied. Furthermore, three dynamic models coupled with four isotherm models were employed to coordinate the experimental data. Results show that the NPO-HPCSs own high specific surface area of up to 2153.46 m2 g−1, hierarchical pore structure and high heteroatom content. Meanwhile, the NPO-HPCSs delivered remarkably adsorption capacity towards MG (972 mg g−1 at 298 K), rapid adsorbing ratio (adsorption equilibrium time of 60 min), as well as excellent recycling stability. The outstanding adsorption performance of the NPO-HPCSs towards MG was attributed to the synergistic contribution of surface adsorption (electrostatic attraction, Lewis acid-base interaction and π-π stacking) and pore adsorption. Additionally, the NPO-HPCSs exhibited high CO2 capture capacities at atmospheric pressure: 2.84 mmol g−1 at 298 K and 4.83 mmol g−1 at 273 K, respectively.
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title_short	Facile construction of N, P and O ternary self-doped hollow carbon microspheres with hierarchical porous structure for environmental applications
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up_date	2024-07-06T20:01:22.310Z
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Facile construction of N, P and O ternary self-doped hollow carbon microspheres with hierarchical porous structure for environmental applications

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