Fabrication of celluloseMg(OH)
The utilization of renewable biomass cellulose in treating pollution of heavy metal ions (HMIs) is one of overarching and appealing strategies, because it simultaneously satisfies sustainable development and resolves ever-increasing environmental issue. In this regard, the composite celluloseMg(OH)2...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Zhao, Nian-Dan [verfasserIn] Wang, Yan [verfasserIn] Zou, Xiao-Hang [verfasserIn] Yin, Wei-Ming [verfasserIn] Wang, Xin-Yu [verfasserIn] Guo, Yuan-Ru [verfasserIn] Pan, Qing-Jiang [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2021 |
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| Schlagwörter: |
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| Übergeordnetes Werk: |
Enthalten in: The chemical engineering journal - Amsterdam : Elsevier, 1997, 426 |
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| Übergeordnetes Werk: |
volume:426 |
| DOI / URN: |
10.1016/j.cej.2021.130812 |
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| Katalog-ID: |
ELV006874495 |
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| 245 | 1 | 0 | |a Fabrication of celluloseMg(OH) |
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| 520 | |a The utilization of renewable biomass cellulose in treating pollution of heavy metal ions (HMIs) is one of overarching and appealing strategies, because it simultaneously satisfies sustainable development and resolves ever-increasing environmental issue. In this regard, the composite celluloseMg(OH)2 was prepared via a facile method and explored for its use as water treatment agent. It is demonstrated that the smaller and thinner hexagonal Mg(OH)2 flakes are constructed onto the cellulose substrate by self-assembling; two components are chemically coupled via hydrogen bonds and Mg-Oc (cellulose oxygen) dative bonds; what’s more, the coupling of cellulose with Mg(OH)2 (101) facet is much more preferential than with (001) facet. The resultant composite material shows remarkable HMI removal performance: large capacities of 734.9, 595.8 and 1473.1 mg g−1 for Cd2+, Cu2+ and Pb2+, respectively. Further assisted by good shaping property of the cellulose substrate, the composite is capable of being made into filter, which practically separates HMIs and purifies wastewater with high removal efficiency (99.99%) for Cd2+ even after operating for 110 days and potable water can be obtained. The mechanism is delineated with removal models and characterizations of HMI-recovered products. | ||
| 650 | 4 | |a Cellulose@Mg(OH) | |
| 650 | 4 | |a Interfacial coupling | |
| 650 | 4 | |a HMI pollution remediation | |
| 650 | 4 | |a Removal mechanism | |
| 650 | 4 | |a DFT calculation | |
| 700 | 1 | |a Wang, Yan |e verfasserin |4 aut | |
| 700 | 1 | |a Zou, Xiao-Hang |e verfasserin |4 aut | |
| 700 | 1 | |a Yin, Wei-Ming |e verfasserin |0 (orcid)0000-0001-8481-9678 |4 aut | |
| 700 | 1 | |a Wang, Xin-Yu |e verfasserin |4 aut | |
| 700 | 1 | |a Guo, Yuan-Ru |e verfasserin |4 aut | |
| 700 | 1 | |a Pan, Qing-Jiang |e verfasserin |0 (orcid)0000-0003-2763-6976 |4 aut | |
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10.1016/j.cej.2021.130812 doi (DE-627)ELV006874495 (ELSEVIER)S1385-8947(21)02397-4 DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Zhao, Nian-Dan verfasserin aut Fabrication of celluloseMg(OH) 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The utilization of renewable biomass cellulose in treating pollution of heavy metal ions (HMIs) is one of overarching and appealing strategies, because it simultaneously satisfies sustainable development and resolves ever-increasing environmental issue. In this regard, the composite celluloseMg(OH)2 was prepared via a facile method and explored for its use as water treatment agent. It is demonstrated that the smaller and thinner hexagonal Mg(OH)2 flakes are constructed onto the cellulose substrate by self-assembling; two components are chemically coupled via hydrogen bonds and Mg-Oc (cellulose oxygen) dative bonds; what’s more, the coupling of cellulose with Mg(OH)2 (101) facet is much more preferential than with (001) facet. The resultant composite material shows remarkable HMI removal performance: large capacities of 734.9, 595.8 and 1473.1 mg g−1 for Cd2+, Cu2+ and Pb2+, respectively. Further assisted by good shaping property of the cellulose substrate, the composite is capable of being made into filter, which practically separates HMIs and purifies wastewater with high removal efficiency (99.99%) for Cd2+ even after operating for 110 days and potable water can be obtained. The mechanism is delineated with removal models and characterizations of HMI-recovered products. Cellulose@Mg(OH) Interfacial coupling HMI pollution remediation Removal mechanism DFT calculation Wang, Yan verfasserin aut Zou, Xiao-Hang verfasserin aut Yin, Wei-Ming verfasserin (orcid)0000-0001-8481-9678 aut Wang, Xin-Yu verfasserin aut Guo, Yuan-Ru verfasserin aut Pan, Qing-Jiang verfasserin (orcid)0000-0003-2763-6976 aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 426 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:426 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 426 045F 660.05 |
| spelling |
10.1016/j.cej.2021.130812 doi (DE-627)ELV006874495 (ELSEVIER)S1385-8947(21)02397-4 DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Zhao, Nian-Dan verfasserin aut Fabrication of celluloseMg(OH) 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The utilization of renewable biomass cellulose in treating pollution of heavy metal ions (HMIs) is one of overarching and appealing strategies, because it simultaneously satisfies sustainable development and resolves ever-increasing environmental issue. In this regard, the composite celluloseMg(OH)2 was prepared via a facile method and explored for its use as water treatment agent. It is demonstrated that the smaller and thinner hexagonal Mg(OH)2 flakes are constructed onto the cellulose substrate by self-assembling; two components are chemically coupled via hydrogen bonds and Mg-Oc (cellulose oxygen) dative bonds; what’s more, the coupling of cellulose with Mg(OH)2 (101) facet is much more preferential than with (001) facet. The resultant composite material shows remarkable HMI removal performance: large capacities of 734.9, 595.8 and 1473.1 mg g−1 for Cd2+, Cu2+ and Pb2+, respectively. Further assisted by good shaping property of the cellulose substrate, the composite is capable of being made into filter, which practically separates HMIs and purifies wastewater with high removal efficiency (99.99%) for Cd2+ even after operating for 110 days and potable water can be obtained. The mechanism is delineated with removal models and characterizations of HMI-recovered products. Cellulose@Mg(OH) Interfacial coupling HMI pollution remediation Removal mechanism DFT calculation Wang, Yan verfasserin aut Zou, Xiao-Hang verfasserin aut Yin, Wei-Ming verfasserin (orcid)0000-0001-8481-9678 aut Wang, Xin-Yu verfasserin aut Guo, Yuan-Ru verfasserin aut Pan, Qing-Jiang verfasserin (orcid)0000-0003-2763-6976 aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 426 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:426 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 426 045F 660.05 |
| allfields_unstemmed |
10.1016/j.cej.2021.130812 doi (DE-627)ELV006874495 (ELSEVIER)S1385-8947(21)02397-4 DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Zhao, Nian-Dan verfasserin aut Fabrication of celluloseMg(OH) 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The utilization of renewable biomass cellulose in treating pollution of heavy metal ions (HMIs) is one of overarching and appealing strategies, because it simultaneously satisfies sustainable development and resolves ever-increasing environmental issue. In this regard, the composite celluloseMg(OH)2 was prepared via a facile method and explored for its use as water treatment agent. It is demonstrated that the smaller and thinner hexagonal Mg(OH)2 flakes are constructed onto the cellulose substrate by self-assembling; two components are chemically coupled via hydrogen bonds and Mg-Oc (cellulose oxygen) dative bonds; what’s more, the coupling of cellulose with Mg(OH)2 (101) facet is much more preferential than with (001) facet. The resultant composite material shows remarkable HMI removal performance: large capacities of 734.9, 595.8 and 1473.1 mg g−1 for Cd2+, Cu2+ and Pb2+, respectively. Further assisted by good shaping property of the cellulose substrate, the composite is capable of being made into filter, which practically separates HMIs and purifies wastewater with high removal efficiency (99.99%) for Cd2+ even after operating for 110 days and potable water can be obtained. The mechanism is delineated with removal models and characterizations of HMI-recovered products. Cellulose@Mg(OH) Interfacial coupling HMI pollution remediation Removal mechanism DFT calculation Wang, Yan verfasserin aut Zou, Xiao-Hang verfasserin aut Yin, Wei-Ming verfasserin (orcid)0000-0001-8481-9678 aut Wang, Xin-Yu verfasserin aut Guo, Yuan-Ru verfasserin aut Pan, Qing-Jiang verfasserin (orcid)0000-0003-2763-6976 aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 426 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:426 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 426 045F 660.05 |
| allfieldsGer |
10.1016/j.cej.2021.130812 doi (DE-627)ELV006874495 (ELSEVIER)S1385-8947(21)02397-4 DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Zhao, Nian-Dan verfasserin aut Fabrication of celluloseMg(OH) 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The utilization of renewable biomass cellulose in treating pollution of heavy metal ions (HMIs) is one of overarching and appealing strategies, because it simultaneously satisfies sustainable development and resolves ever-increasing environmental issue. In this regard, the composite celluloseMg(OH)2 was prepared via a facile method and explored for its use as water treatment agent. It is demonstrated that the smaller and thinner hexagonal Mg(OH)2 flakes are constructed onto the cellulose substrate by self-assembling; two components are chemically coupled via hydrogen bonds and Mg-Oc (cellulose oxygen) dative bonds; what’s more, the coupling of cellulose with Mg(OH)2 (101) facet is much more preferential than with (001) facet. The resultant composite material shows remarkable HMI removal performance: large capacities of 734.9, 595.8 and 1473.1 mg g−1 for Cd2+, Cu2+ and Pb2+, respectively. Further assisted by good shaping property of the cellulose substrate, the composite is capable of being made into filter, which practically separates HMIs and purifies wastewater with high removal efficiency (99.99%) for Cd2+ even after operating for 110 days and potable water can be obtained. The mechanism is delineated with removal models and characterizations of HMI-recovered products. Cellulose@Mg(OH) Interfacial coupling HMI pollution remediation Removal mechanism DFT calculation Wang, Yan verfasserin aut Zou, Xiao-Hang verfasserin aut Yin, Wei-Ming verfasserin (orcid)0000-0001-8481-9678 aut Wang, Xin-Yu verfasserin aut Guo, Yuan-Ru verfasserin aut Pan, Qing-Jiang verfasserin (orcid)0000-0003-2763-6976 aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 426 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:426 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 426 045F 660.05 |
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10.1016/j.cej.2021.130812 doi (DE-627)ELV006874495 (ELSEVIER)S1385-8947(21)02397-4 DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Zhao, Nian-Dan verfasserin aut Fabrication of celluloseMg(OH) 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The utilization of renewable biomass cellulose in treating pollution of heavy metal ions (HMIs) is one of overarching and appealing strategies, because it simultaneously satisfies sustainable development and resolves ever-increasing environmental issue. In this regard, the composite celluloseMg(OH)2 was prepared via a facile method and explored for its use as water treatment agent. It is demonstrated that the smaller and thinner hexagonal Mg(OH)2 flakes are constructed onto the cellulose substrate by self-assembling; two components are chemically coupled via hydrogen bonds and Mg-Oc (cellulose oxygen) dative bonds; what’s more, the coupling of cellulose with Mg(OH)2 (101) facet is much more preferential than with (001) facet. The resultant composite material shows remarkable HMI removal performance: large capacities of 734.9, 595.8 and 1473.1 mg g−1 for Cd2+, Cu2+ and Pb2+, respectively. Further assisted by good shaping property of the cellulose substrate, the composite is capable of being made into filter, which practically separates HMIs and purifies wastewater with high removal efficiency (99.99%) for Cd2+ even after operating for 110 days and potable water can be obtained. The mechanism is delineated with removal models and characterizations of HMI-recovered products. Cellulose@Mg(OH) Interfacial coupling HMI pollution remediation Removal mechanism DFT calculation Wang, Yan verfasserin aut Zou, Xiao-Hang verfasserin aut Yin, Wei-Ming verfasserin (orcid)0000-0001-8481-9678 aut Wang, Xin-Yu verfasserin aut Guo, Yuan-Ru verfasserin aut Pan, Qing-Jiang verfasserin (orcid)0000-0003-2763-6976 aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 426 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:426 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 426 045F 660.05 |
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660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Fabrication of celluloseMg(OH) Cellulose@Mg(OH) Interfacial coupling HMI pollution remediation Removal mechanism DFT calculation |
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Zhao, Nian-Dan Wang, Yan Zou, Xiao-Hang Yin, Wei-Ming Wang, Xin-Yu Guo, Yuan-Ru Pan, Qing-Jiang |
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fabrication of cellulosemg(oh) |
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Fabrication of celluloseMg(OH) |
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The utilization of renewable biomass cellulose in treating pollution of heavy metal ions (HMIs) is one of overarching and appealing strategies, because it simultaneously satisfies sustainable development and resolves ever-increasing environmental issue. In this regard, the composite celluloseMg(OH)2 was prepared via a facile method and explored for its use as water treatment agent. It is demonstrated that the smaller and thinner hexagonal Mg(OH)2 flakes are constructed onto the cellulose substrate by self-assembling; two components are chemically coupled via hydrogen bonds and Mg-Oc (cellulose oxygen) dative bonds; what’s more, the coupling of cellulose with Mg(OH)2 (101) facet is much more preferential than with (001) facet. The resultant composite material shows remarkable HMI removal performance: large capacities of 734.9, 595.8 and 1473.1 mg g−1 for Cd2+, Cu2+ and Pb2+, respectively. Further assisted by good shaping property of the cellulose substrate, the composite is capable of being made into filter, which practically separates HMIs and purifies wastewater with high removal efficiency (99.99%) for Cd2+ even after operating for 110 days and potable water can be obtained. The mechanism is delineated with removal models and characterizations of HMI-recovered products. |
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The utilization of renewable biomass cellulose in treating pollution of heavy metal ions (HMIs) is one of overarching and appealing strategies, because it simultaneously satisfies sustainable development and resolves ever-increasing environmental issue. In this regard, the composite celluloseMg(OH)2 was prepared via a facile method and explored for its use as water treatment agent. It is demonstrated that the smaller and thinner hexagonal Mg(OH)2 flakes are constructed onto the cellulose substrate by self-assembling; two components are chemically coupled via hydrogen bonds and Mg-Oc (cellulose oxygen) dative bonds; what’s more, the coupling of cellulose with Mg(OH)2 (101) facet is much more preferential than with (001) facet. The resultant composite material shows remarkable HMI removal performance: large capacities of 734.9, 595.8 and 1473.1 mg g−1 for Cd2+, Cu2+ and Pb2+, respectively. Further assisted by good shaping property of the cellulose substrate, the composite is capable of being made into filter, which practically separates HMIs and purifies wastewater with high removal efficiency (99.99%) for Cd2+ even after operating for 110 days and potable water can be obtained. The mechanism is delineated with removal models and characterizations of HMI-recovered products. |
| abstract_unstemmed |
The utilization of renewable biomass cellulose in treating pollution of heavy metal ions (HMIs) is one of overarching and appealing strategies, because it simultaneously satisfies sustainable development and resolves ever-increasing environmental issue. In this regard, the composite celluloseMg(OH)2 was prepared via a facile method and explored for its use as water treatment agent. It is demonstrated that the smaller and thinner hexagonal Mg(OH)2 flakes are constructed onto the cellulose substrate by self-assembling; two components are chemically coupled via hydrogen bonds and Mg-Oc (cellulose oxygen) dative bonds; what’s more, the coupling of cellulose with Mg(OH)2 (101) facet is much more preferential than with (001) facet. The resultant composite material shows remarkable HMI removal performance: large capacities of 734.9, 595.8 and 1473.1 mg g−1 for Cd2+, Cu2+ and Pb2+, respectively. Further assisted by good shaping property of the cellulose substrate, the composite is capable of being made into filter, which practically separates HMIs and purifies wastewater with high removal efficiency (99.99%) for Cd2+ even after operating for 110 days and potable water can be obtained. The mechanism is delineated with removal models and characterizations of HMI-recovered products. |
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