Tailoring the pore structure modified with functional groups for superior CO

In this work, the ultra-uniform amidated nitrogen (N)-doped carbon sphere (ANG-Cs) adsorbent with different pore sizes and modified by kinds of functional groups was developed for efficient carbon dioxide (CO2) adsorption, simultaneously obtaining the excellent selectivity of CO2/N2 from the simulat...
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Autor*in:	An, Xuefei [verfasserIn] Zhao, Kun [verfasserIn] Zhang, Weiping [verfasserIn] Yang, Jiahan [verfasserIn] Liao, Yujie [verfasserIn] Wang, Lemeng [verfasserIn] Fu, Dong [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2021

Schlagwörter:	Surface modification and Pore structure CO Water resistance and chemical stability Ultra-low emission flue gas

Übergeordnetes Werk:	Enthalten in: Fuel - New York, NY [u.a.] : Elsevier, 1970, 309
Übergeordnetes Werk:	volume:309

DOI / URN:	10.1016/j.fuel.2021.122175

Katalog-ID:	ELV006914829

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520			\|a In this work, the ultra-uniform amidated nitrogen (N)-doped carbon sphere (ANG-Cs) adsorbent with different pore sizes and modified by kinds of functional groups was developed for efficient carbon dioxide (CO2) adsorption, simultaneously obtaining the excellent selectivity of CO2/N2 from the simulated ultra-low emission flue gas. We fabricated the uniformly monodispersed glucose-based carbon microspheres via a creative ethanol-assisted hydrothermal method, and also systematically explored and discussed the relationship between porous structures functional alkaline-containing N-groups and CO2 adsorption capacity. Impressively, the pore size distribution arranged from micro- to mesoporous region along with large surface area of 1217 m2/g, that is benefit for the adsorption of small acid gas like CO2. Moreover, the adsorption capacity of the optimized ANG-Cs reached 4.89 mmol/g under 298 K and 1 bar, and the predictable adsorption selectivity of pure CO2/N2 was as high as 43 in the simulated ultra-low emission flue gas. More importantly, when compared with some advanced MOF-based adsorbents, ANG-Cs not only owns similar CO2 adsorption performance, but also keeps higher water resistance, chemical stability and lower cost. Therefore, this promising ANG-Cs with green synthesis for the controllable CO2 adsorption and separation pushes the progress in industry application of ultra-low emission gas.
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700	1		\|a Wang, Lemeng \|e verfasserin \|4 aut
700	1		\|a Fu, Dong \|e verfasserin \|4 aut
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publishDate	2021
allfields	10.1016/j.fuel.2021.122175 doi (DE-627)ELV006914829 (ELSEVIER)S0016-2361(21)02051-2 DE-627 ger DE-627 rda eng 660 DE-600 58.21 bkl An, Xuefei verfasserin aut Tailoring the pore structure modified with functional groups for superior CO 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier In this work, the ultra-uniform amidated nitrogen (N)-doped carbon sphere (ANG-Cs) adsorbent with different pore sizes and modified by kinds of functional groups was developed for efficient carbon dioxide (CO2) adsorption, simultaneously obtaining the excellent selectivity of CO2/N2 from the simulated ultra-low emission flue gas. We fabricated the uniformly monodispersed glucose-based carbon microspheres via a creative ethanol-assisted hydrothermal method, and also systematically explored and discussed the relationship between porous structures functional alkaline-containing N-groups and CO2 adsorption capacity. Impressively, the pore size distribution arranged from micro- to mesoporous region along with large surface area of 1217 m2/g, that is benefit for the adsorption of small acid gas like CO2. Moreover, the adsorption capacity of the optimized ANG-Cs reached 4.89 mmol/g under 298 K and 1 bar, and the predictable adsorption selectivity of pure CO2/N2 was as high as 43 in the simulated ultra-low emission flue gas. More importantly, when compared with some advanced MOF-based adsorbents, ANG-Cs not only owns similar CO2 adsorption performance, but also keeps higher water resistance, chemical stability and lower cost. Therefore, this promising ANG-Cs with green synthesis for the controllable CO2 adsorption and separation pushes the progress in industry application of ultra-low emission gas. Surface modification and Pore structure CO CO Water resistance and chemical stability Ultra-low emission flue gas Zhao, Kun verfasserin aut Zhang, Weiping verfasserin aut Yang, Jiahan verfasserin aut Liao, Yujie verfasserin aut Wang, Lemeng verfasserin aut Fu, Dong verfasserin aut Enthalten in Fuel New York, NY [u.a.] : Elsevier, 1970 309 Online-Ressource (DE-627)300898584 (DE-600)1483656-7 (DE-576)09555176X 0016-2361 nnns volume:309 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.21 Brennstoffe Kraftstoffe Explosivstoffe AR 309
spelling	10.1016/j.fuel.2021.122175 doi (DE-627)ELV006914829 (ELSEVIER)S0016-2361(21)02051-2 DE-627 ger DE-627 rda eng 660 DE-600 58.21 bkl An, Xuefei verfasserin aut Tailoring the pore structure modified with functional groups for superior CO 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier In this work, the ultra-uniform amidated nitrogen (N)-doped carbon sphere (ANG-Cs) adsorbent with different pore sizes and modified by kinds of functional groups was developed for efficient carbon dioxide (CO2) adsorption, simultaneously obtaining the excellent selectivity of CO2/N2 from the simulated ultra-low emission flue gas. We fabricated the uniformly monodispersed glucose-based carbon microspheres via a creative ethanol-assisted hydrothermal method, and also systematically explored and discussed the relationship between porous structures functional alkaline-containing N-groups and CO2 adsorption capacity. Impressively, the pore size distribution arranged from micro- to mesoporous region along with large surface area of 1217 m2/g, that is benefit for the adsorption of small acid gas like CO2. Moreover, the adsorption capacity of the optimized ANG-Cs reached 4.89 mmol/g under 298 K and 1 bar, and the predictable adsorption selectivity of pure CO2/N2 was as high as 43 in the simulated ultra-low emission flue gas. More importantly, when compared with some advanced MOF-based adsorbents, ANG-Cs not only owns similar CO2 adsorption performance, but also keeps higher water resistance, chemical stability and lower cost. Therefore, this promising ANG-Cs with green synthesis for the controllable CO2 adsorption and separation pushes the progress in industry application of ultra-low emission gas. Surface modification and Pore structure CO CO Water resistance and chemical stability Ultra-low emission flue gas Zhao, Kun verfasserin aut Zhang, Weiping verfasserin aut Yang, Jiahan verfasserin aut Liao, Yujie verfasserin aut Wang, Lemeng verfasserin aut Fu, Dong verfasserin aut Enthalten in Fuel New York, NY [u.a.] : Elsevier, 1970 309 Online-Ressource (DE-627)300898584 (DE-600)1483656-7 (DE-576)09555176X 0016-2361 nnns volume:309 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.21 Brennstoffe Kraftstoffe Explosivstoffe AR 309
allfields_unstemmed	10.1016/j.fuel.2021.122175 doi (DE-627)ELV006914829 (ELSEVIER)S0016-2361(21)02051-2 DE-627 ger DE-627 rda eng 660 DE-600 58.21 bkl An, Xuefei verfasserin aut Tailoring the pore structure modified with functional groups for superior CO 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier In this work, the ultra-uniform amidated nitrogen (N)-doped carbon sphere (ANG-Cs) adsorbent with different pore sizes and modified by kinds of functional groups was developed for efficient carbon dioxide (CO2) adsorption, simultaneously obtaining the excellent selectivity of CO2/N2 from the simulated ultra-low emission flue gas. We fabricated the uniformly monodispersed glucose-based carbon microspheres via a creative ethanol-assisted hydrothermal method, and also systematically explored and discussed the relationship between porous structures functional alkaline-containing N-groups and CO2 adsorption capacity. Impressively, the pore size distribution arranged from micro- to mesoporous region along with large surface area of 1217 m2/g, that is benefit for the adsorption of small acid gas like CO2. Moreover, the adsorption capacity of the optimized ANG-Cs reached 4.89 mmol/g under 298 K and 1 bar, and the predictable adsorption selectivity of pure CO2/N2 was as high as 43 in the simulated ultra-low emission flue gas. More importantly, when compared with some advanced MOF-based adsorbents, ANG-Cs not only owns similar CO2 adsorption performance, but also keeps higher water resistance, chemical stability and lower cost. Therefore, this promising ANG-Cs with green synthesis for the controllable CO2 adsorption and separation pushes the progress in industry application of ultra-low emission gas. Surface modification and Pore structure CO CO Water resistance and chemical stability Ultra-low emission flue gas Zhao, Kun verfasserin aut Zhang, Weiping verfasserin aut Yang, Jiahan verfasserin aut Liao, Yujie verfasserin aut Wang, Lemeng verfasserin aut Fu, Dong verfasserin aut Enthalten in Fuel New York, NY [u.a.] : Elsevier, 1970 309 Online-Ressource (DE-627)300898584 (DE-600)1483656-7 (DE-576)09555176X 0016-2361 nnns volume:309 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.21 Brennstoffe Kraftstoffe Explosivstoffe AR 309
allfieldsGer	10.1016/j.fuel.2021.122175 doi (DE-627)ELV006914829 (ELSEVIER)S0016-2361(21)02051-2 DE-627 ger DE-627 rda eng 660 DE-600 58.21 bkl An, Xuefei verfasserin aut Tailoring the pore structure modified with functional groups for superior CO 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier In this work, the ultra-uniform amidated nitrogen (N)-doped carbon sphere (ANG-Cs) adsorbent with different pore sizes and modified by kinds of functional groups was developed for efficient carbon dioxide (CO2) adsorption, simultaneously obtaining the excellent selectivity of CO2/N2 from the simulated ultra-low emission flue gas. We fabricated the uniformly monodispersed glucose-based carbon microspheres via a creative ethanol-assisted hydrothermal method, and also systematically explored and discussed the relationship between porous structures functional alkaline-containing N-groups and CO2 adsorption capacity. Impressively, the pore size distribution arranged from micro- to mesoporous region along with large surface area of 1217 m2/g, that is benefit for the adsorption of small acid gas like CO2. Moreover, the adsorption capacity of the optimized ANG-Cs reached 4.89 mmol/g under 298 K and 1 bar, and the predictable adsorption selectivity of pure CO2/N2 was as high as 43 in the simulated ultra-low emission flue gas. More importantly, when compared with some advanced MOF-based adsorbents, ANG-Cs not only owns similar CO2 adsorption performance, but also keeps higher water resistance, chemical stability and lower cost. Therefore, this promising ANG-Cs with green synthesis for the controllable CO2 adsorption and separation pushes the progress in industry application of ultra-low emission gas. Surface modification and Pore structure CO CO Water resistance and chemical stability Ultra-low emission flue gas Zhao, Kun verfasserin aut Zhang, Weiping verfasserin aut Yang, Jiahan verfasserin aut Liao, Yujie verfasserin aut Wang, Lemeng verfasserin aut Fu, Dong verfasserin aut Enthalten in Fuel New York, NY [u.a.] : Elsevier, 1970 309 Online-Ressource (DE-627)300898584 (DE-600)1483656-7 (DE-576)09555176X 0016-2361 nnns volume:309 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.21 Brennstoffe Kraftstoffe Explosivstoffe AR 309
allfieldsSound	10.1016/j.fuel.2021.122175 doi (DE-627)ELV006914829 (ELSEVIER)S0016-2361(21)02051-2 DE-627 ger DE-627 rda eng 660 DE-600 58.21 bkl An, Xuefei verfasserin aut Tailoring the pore structure modified with functional groups for superior CO 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier In this work, the ultra-uniform amidated nitrogen (N)-doped carbon sphere (ANG-Cs) adsorbent with different pore sizes and modified by kinds of functional groups was developed for efficient carbon dioxide (CO2) adsorption, simultaneously obtaining the excellent selectivity of CO2/N2 from the simulated ultra-low emission flue gas. We fabricated the uniformly monodispersed glucose-based carbon microspheres via a creative ethanol-assisted hydrothermal method, and also systematically explored and discussed the relationship between porous structures functional alkaline-containing N-groups and CO2 adsorption capacity. Impressively, the pore size distribution arranged from micro- to mesoporous region along with large surface area of 1217 m2/g, that is benefit for the adsorption of small acid gas like CO2. Moreover, the adsorption capacity of the optimized ANG-Cs reached 4.89 mmol/g under 298 K and 1 bar, and the predictable adsorption selectivity of pure CO2/N2 was as high as 43 in the simulated ultra-low emission flue gas. More importantly, when compared with some advanced MOF-based adsorbents, ANG-Cs not only owns similar CO2 adsorption performance, but also keeps higher water resistance, chemical stability and lower cost. Therefore, this promising ANG-Cs with green synthesis for the controllable CO2 adsorption and separation pushes the progress in industry application of ultra-low emission gas. Surface modification and Pore structure CO CO Water resistance and chemical stability Ultra-low emission flue gas Zhao, Kun verfasserin aut Zhang, Weiping verfasserin aut Yang, Jiahan verfasserin aut Liao, Yujie verfasserin aut Wang, Lemeng verfasserin aut Fu, Dong verfasserin aut Enthalten in Fuel New York, NY [u.a.] : Elsevier, 1970 309 Online-Ressource (DE-627)300898584 (DE-600)1483656-7 (DE-576)09555176X 0016-2361 nnns volume:309 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.21 Brennstoffe Kraftstoffe Explosivstoffe AR 309
language	English
source	Enthalten in Fuel 309 volume:309
sourceStr	Enthalten in Fuel 309 volume:309
format_phy_str_mv	Article
bklname	Brennstoffe Kraftstoffe Explosivstoffe
institution	findex.gbv.de
topic_facet	Surface modification and Pore structure CO Water resistance and chemical stability Ultra-low emission flue gas
dewey-raw	660
isfreeaccess_bool	false
container_title	Fuel
authorswithroles_txt_mv	An, Xuefei @@aut@@ Zhao, Kun @@aut@@ Zhang, Weiping @@aut@@ Yang, Jiahan @@aut@@ Liao, Yujie @@aut@@ Wang, Lemeng @@aut@@ Fu, Dong @@aut@@
publishDateDaySort_date	2021-01-01T00:00:00Z
hierarchy_top_id	300898584
dewey-sort	3660
id	ELV006914829
language_de	englisch
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author	An, Xuefei
spellingShingle	An, Xuefei ddc 660 bkl 58.21 misc Surface modification and Pore structure misc CO misc Water resistance and chemical stability misc Ultra-low emission flue gas Tailoring the pore structure modified with functional groups for superior CO
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topic_title	660 DE-600 58.21 bkl Tailoring the pore structure modified with functional groups for superior CO Surface modification and Pore structure CO Water resistance and chemical stability Ultra-low emission flue gas
topic	ddc 660 bkl 58.21 misc Surface modification and Pore structure misc CO misc Water resistance and chemical stability misc Ultra-low emission flue gas
topic_unstemmed	ddc 660 bkl 58.21 misc Surface modification and Pore structure misc CO misc Water resistance and chemical stability misc Ultra-low emission flue gas
topic_browse	ddc 660 bkl 58.21 misc Surface modification and Pore structure misc CO misc Water resistance and chemical stability misc Ultra-low emission flue gas
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title	Tailoring the pore structure modified with functional groups for superior CO
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title_full	Tailoring the pore structure modified with functional groups for superior CO
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author_browse	An, Xuefei Zhao, Kun Zhang, Weiping Yang, Jiahan Liao, Yujie Wang, Lemeng Fu, Dong
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doi_str_mv	10.1016/j.fuel.2021.122175
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title_sort	tailoring the pore structure modified with functional groups for superior co
title_auth	Tailoring the pore structure modified with functional groups for superior CO
abstract	In this work, the ultra-uniform amidated nitrogen (N)-doped carbon sphere (ANG-Cs) adsorbent with different pore sizes and modified by kinds of functional groups was developed for efficient carbon dioxide (CO2) adsorption, simultaneously obtaining the excellent selectivity of CO2/N2 from the simulated ultra-low emission flue gas. We fabricated the uniformly monodispersed glucose-based carbon microspheres via a creative ethanol-assisted hydrothermal method, and also systematically explored and discussed the relationship between porous structures functional alkaline-containing N-groups and CO2 adsorption capacity. Impressively, the pore size distribution arranged from micro- to mesoporous region along with large surface area of 1217 m2/g, that is benefit for the adsorption of small acid gas like CO2. Moreover, the adsorption capacity of the optimized ANG-Cs reached 4.89 mmol/g under 298 K and 1 bar, and the predictable adsorption selectivity of pure CO2/N2 was as high as 43 in the simulated ultra-low emission flue gas. More importantly, when compared with some advanced MOF-based adsorbents, ANG-Cs not only owns similar CO2 adsorption performance, but also keeps higher water resistance, chemical stability and lower cost. Therefore, this promising ANG-Cs with green synthesis for the controllable CO2 adsorption and separation pushes the progress in industry application of ultra-low emission gas.
abstractGer	In this work, the ultra-uniform amidated nitrogen (N)-doped carbon sphere (ANG-Cs) adsorbent with different pore sizes and modified by kinds of functional groups was developed for efficient carbon dioxide (CO2) adsorption, simultaneously obtaining the excellent selectivity of CO2/N2 from the simulated ultra-low emission flue gas. We fabricated the uniformly monodispersed glucose-based carbon microspheres via a creative ethanol-assisted hydrothermal method, and also systematically explored and discussed the relationship between porous structures functional alkaline-containing N-groups and CO2 adsorption capacity. Impressively, the pore size distribution arranged from micro- to mesoporous region along with large surface area of 1217 m2/g, that is benefit for the adsorption of small acid gas like CO2. Moreover, the adsorption capacity of the optimized ANG-Cs reached 4.89 mmol/g under 298 K and 1 bar, and the predictable adsorption selectivity of pure CO2/N2 was as high as 43 in the simulated ultra-low emission flue gas. More importantly, when compared with some advanced MOF-based adsorbents, ANG-Cs not only owns similar CO2 adsorption performance, but also keeps higher water resistance, chemical stability and lower cost. Therefore, this promising ANG-Cs with green synthesis for the controllable CO2 adsorption and separation pushes the progress in industry application of ultra-low emission gas.
abstract_unstemmed	In this work, the ultra-uniform amidated nitrogen (N)-doped carbon sphere (ANG-Cs) adsorbent with different pore sizes and modified by kinds of functional groups was developed for efficient carbon dioxide (CO2) adsorption, simultaneously obtaining the excellent selectivity of CO2/N2 from the simulated ultra-low emission flue gas. We fabricated the uniformly monodispersed glucose-based carbon microspheres via a creative ethanol-assisted hydrothermal method, and also systematically explored and discussed the relationship between porous structures functional alkaline-containing N-groups and CO2 adsorption capacity. Impressively, the pore size distribution arranged from micro- to mesoporous region along with large surface area of 1217 m2/g, that is benefit for the adsorption of small acid gas like CO2. Moreover, the adsorption capacity of the optimized ANG-Cs reached 4.89 mmol/g under 298 K and 1 bar, and the predictable adsorption selectivity of pure CO2/N2 was as high as 43 in the simulated ultra-low emission flue gas. More importantly, when compared with some advanced MOF-based adsorbents, ANG-Cs not only owns similar CO2 adsorption performance, but also keeps higher water resistance, chemical stability and lower cost. Therefore, this promising ANG-Cs with green synthesis for the controllable CO2 adsorption and separation pushes the progress in industry application of ultra-low emission gas.
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title_short	Tailoring the pore structure modified with functional groups for superior CO
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author2	Zhao, Kun Zhang, Weiping Yang, Jiahan Liao, Yujie Wang, Lemeng Fu, Dong
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doi_str	10.1016/j.fuel.2021.122175
up_date	2024-07-06T22:59:11.322Z
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score	7.400613

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Tailoring the pore structure modified with functional groups for superior CO

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