Self-floating biomass charcoal supported flower-like plasmon silver/carbon, nitrogen co-doped defective TiO
A self-floating biomass charcoal supported flower-like plasmon Ag/C, N co-doped defective TiO2 photocatalyst is fabricated by hydrothermal, calcination and photo-deposition strategies. Biomass charcoal, Ag nanoparticles, oxygen vacancy defects and C, N co-doping all favor to extend the photoresponse...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Wu, Chunxu [verfasserIn] Zhang, Jiaqi [verfasserIn] Fang, Bin [verfasserIn] Cui, Yongqian [verfasserIn] Xing, Zipeng [verfasserIn] Li, Zhenzi [verfasserIn] Zhou, Wei [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2021 |
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| Schlagwörter: |
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| Übergeordnetes Werk: |
Enthalten in: Journal of cleaner production - Amsterdam [u.a.] : Elsevier Science, 1993, 329 |
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| Übergeordnetes Werk: |
volume:329 |
| DOI / URN: |
10.1016/j.jclepro.2021.129723 |
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ELV00709115X |
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| 520 | |a A self-floating biomass charcoal supported flower-like plasmon Ag/C, N co-doped defective TiO2 photocatalyst is fabricated by hydrothermal, calcination and photo-deposition strategies. Biomass charcoal, Ag nanoparticles, oxygen vacancy defects and C, N co-doping all favor to extend the photoresponse to visible light region. The biomass charcoal plays the role of doping and floating supporter, which can make it float on surface of water and effectively improve the collection of sunlight. The resultant plasmon Ag/C, N co-doped defective TiO2 photocatalyst exhibits excellent visible-light-driven photocatalytic performance, in which the photocatalytic degradation ratio of 2,4-dichlorophenol and hydrogen evolution are up to 95% and 1269 μmol h−1 g−1, respectively, several times higher than that of pristine TiO2. It can be ascribed to the synergistic effect of surface plasmon resonance (SPR) effect of Ag nanoparticles, the efficient C, N co-doping and formation of oxygen vacancy defects promotes spatial charge separation and enhances visible light absorption. In addition, the long-term stability of this novel self-floating photocatalyst implies the potential practical applications. | ||
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| 650 | 4 | |a TiO | |
| 650 | 4 | |a Oxygen vacancy defect | |
| 650 | 4 | |a Surface plasmon resonance | |
| 700 | 1 | |a Zhang, Jiaqi |e verfasserin |4 aut | |
| 700 | 1 | |a Fang, Bin |e verfasserin |4 aut | |
| 700 | 1 | |a Cui, Yongqian |e verfasserin |4 aut | |
| 700 | 1 | |a Xing, Zipeng |e verfasserin |0 (orcid)0000-0002-9429-5780 |4 aut | |
| 700 | 1 | |a Li, Zhenzi |e verfasserin |4 aut | |
| 700 | 1 | |a Zhou, Wei |e verfasserin |4 aut | |
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10.1016/j.jclepro.2021.129723 doi (DE-627)ELV00709115X (ELSEVIER)S0959-6526(21)03900-7 DE-627 ger DE-627 rda eng 690 330 DE-600 43.35 bkl 85.35 bkl Wu, Chunxu verfasserin aut Self-floating biomass charcoal supported flower-like plasmon silver/carbon, nitrogen co-doped defective TiO 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A self-floating biomass charcoal supported flower-like plasmon Ag/C, N co-doped defective TiO2 photocatalyst is fabricated by hydrothermal, calcination and photo-deposition strategies. Biomass charcoal, Ag nanoparticles, oxygen vacancy defects and C, N co-doping all favor to extend the photoresponse to visible light region. The biomass charcoal plays the role of doping and floating supporter, which can make it float on surface of water and effectively improve the collection of sunlight. The resultant plasmon Ag/C, N co-doped defective TiO2 photocatalyst exhibits excellent visible-light-driven photocatalytic performance, in which the photocatalytic degradation ratio of 2,4-dichlorophenol and hydrogen evolution are up to 95% and 1269 μmol h−1 g−1, respectively, several times higher than that of pristine TiO2. It can be ascribed to the synergistic effect of surface plasmon resonance (SPR) effect of Ag nanoparticles, the efficient C, N co-doping and formation of oxygen vacancy defects promotes spatial charge separation and enhances visible light absorption. In addition, the long-term stability of this novel self-floating photocatalyst implies the potential practical applications. Photocatalysis Self-floating TiO Oxygen vacancy defect Surface plasmon resonance Zhang, Jiaqi verfasserin aut Fang, Bin verfasserin aut Cui, Yongqian verfasserin aut Xing, Zipeng verfasserin (orcid)0000-0002-9429-5780 aut Li, Zhenzi verfasserin aut Zhou, Wei verfasserin aut Enthalten in Journal of cleaner production Amsterdam [u.a.] : Elsevier Science, 1993 329 Online-Ressource (DE-627)324655878 (DE-600)2029338-0 (DE-576)252613988 0959-6526 nnns volume:329 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OPC-GGO GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 43.35 Umweltrichtlinien Umweltnormen 85.35 Fertigung AR 329 |
| spelling |
10.1016/j.jclepro.2021.129723 doi (DE-627)ELV00709115X (ELSEVIER)S0959-6526(21)03900-7 DE-627 ger DE-627 rda eng 690 330 DE-600 43.35 bkl 85.35 bkl Wu, Chunxu verfasserin aut Self-floating biomass charcoal supported flower-like plasmon silver/carbon, nitrogen co-doped defective TiO 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A self-floating biomass charcoal supported flower-like plasmon Ag/C, N co-doped defective TiO2 photocatalyst is fabricated by hydrothermal, calcination and photo-deposition strategies. Biomass charcoal, Ag nanoparticles, oxygen vacancy defects and C, N co-doping all favor to extend the photoresponse to visible light region. The biomass charcoal plays the role of doping and floating supporter, which can make it float on surface of water and effectively improve the collection of sunlight. The resultant plasmon Ag/C, N co-doped defective TiO2 photocatalyst exhibits excellent visible-light-driven photocatalytic performance, in which the photocatalytic degradation ratio of 2,4-dichlorophenol and hydrogen evolution are up to 95% and 1269 μmol h−1 g−1, respectively, several times higher than that of pristine TiO2. It can be ascribed to the synergistic effect of surface plasmon resonance (SPR) effect of Ag nanoparticles, the efficient C, N co-doping and formation of oxygen vacancy defects promotes spatial charge separation and enhances visible light absorption. In addition, the long-term stability of this novel self-floating photocatalyst implies the potential practical applications. Photocatalysis Self-floating TiO Oxygen vacancy defect Surface plasmon resonance Zhang, Jiaqi verfasserin aut Fang, Bin verfasserin aut Cui, Yongqian verfasserin aut Xing, Zipeng verfasserin (orcid)0000-0002-9429-5780 aut Li, Zhenzi verfasserin aut Zhou, Wei verfasserin aut Enthalten in Journal of cleaner production Amsterdam [u.a.] : Elsevier Science, 1993 329 Online-Ressource (DE-627)324655878 (DE-600)2029338-0 (DE-576)252613988 0959-6526 nnns volume:329 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OPC-GGO GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 43.35 Umweltrichtlinien Umweltnormen 85.35 Fertigung AR 329 |
| allfields_unstemmed |
10.1016/j.jclepro.2021.129723 doi (DE-627)ELV00709115X (ELSEVIER)S0959-6526(21)03900-7 DE-627 ger DE-627 rda eng 690 330 DE-600 43.35 bkl 85.35 bkl Wu, Chunxu verfasserin aut Self-floating biomass charcoal supported flower-like plasmon silver/carbon, nitrogen co-doped defective TiO 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A self-floating biomass charcoal supported flower-like plasmon Ag/C, N co-doped defective TiO2 photocatalyst is fabricated by hydrothermal, calcination and photo-deposition strategies. Biomass charcoal, Ag nanoparticles, oxygen vacancy defects and C, N co-doping all favor to extend the photoresponse to visible light region. The biomass charcoal plays the role of doping and floating supporter, which can make it float on surface of water and effectively improve the collection of sunlight. The resultant plasmon Ag/C, N co-doped defective TiO2 photocatalyst exhibits excellent visible-light-driven photocatalytic performance, in which the photocatalytic degradation ratio of 2,4-dichlorophenol and hydrogen evolution are up to 95% and 1269 μmol h−1 g−1, respectively, several times higher than that of pristine TiO2. It can be ascribed to the synergistic effect of surface plasmon resonance (SPR) effect of Ag nanoparticles, the efficient C, N co-doping and formation of oxygen vacancy defects promotes spatial charge separation and enhances visible light absorption. In addition, the long-term stability of this novel self-floating photocatalyst implies the potential practical applications. Photocatalysis Self-floating TiO Oxygen vacancy defect Surface plasmon resonance Zhang, Jiaqi verfasserin aut Fang, Bin verfasserin aut Cui, Yongqian verfasserin aut Xing, Zipeng verfasserin (orcid)0000-0002-9429-5780 aut Li, Zhenzi verfasserin aut Zhou, Wei verfasserin aut Enthalten in Journal of cleaner production Amsterdam [u.a.] : Elsevier Science, 1993 329 Online-Ressource (DE-627)324655878 (DE-600)2029338-0 (DE-576)252613988 0959-6526 nnns volume:329 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OPC-GGO GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 43.35 Umweltrichtlinien Umweltnormen 85.35 Fertigung AR 329 |
| allfieldsGer |
10.1016/j.jclepro.2021.129723 doi (DE-627)ELV00709115X (ELSEVIER)S0959-6526(21)03900-7 DE-627 ger DE-627 rda eng 690 330 DE-600 43.35 bkl 85.35 bkl Wu, Chunxu verfasserin aut Self-floating biomass charcoal supported flower-like plasmon silver/carbon, nitrogen co-doped defective TiO 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A self-floating biomass charcoal supported flower-like plasmon Ag/C, N co-doped defective TiO2 photocatalyst is fabricated by hydrothermal, calcination and photo-deposition strategies. Biomass charcoal, Ag nanoparticles, oxygen vacancy defects and C, N co-doping all favor to extend the photoresponse to visible light region. The biomass charcoal plays the role of doping and floating supporter, which can make it float on surface of water and effectively improve the collection of sunlight. The resultant plasmon Ag/C, N co-doped defective TiO2 photocatalyst exhibits excellent visible-light-driven photocatalytic performance, in which the photocatalytic degradation ratio of 2,4-dichlorophenol and hydrogen evolution are up to 95% and 1269 μmol h−1 g−1, respectively, several times higher than that of pristine TiO2. It can be ascribed to the synergistic effect of surface plasmon resonance (SPR) effect of Ag nanoparticles, the efficient C, N co-doping and formation of oxygen vacancy defects promotes spatial charge separation and enhances visible light absorption. In addition, the long-term stability of this novel self-floating photocatalyst implies the potential practical applications. Photocatalysis Self-floating TiO Oxygen vacancy defect Surface plasmon resonance Zhang, Jiaqi verfasserin aut Fang, Bin verfasserin aut Cui, Yongqian verfasserin aut Xing, Zipeng verfasserin (orcid)0000-0002-9429-5780 aut Li, Zhenzi verfasserin aut Zhou, Wei verfasserin aut Enthalten in Journal of cleaner production Amsterdam [u.a.] : Elsevier Science, 1993 329 Online-Ressource (DE-627)324655878 (DE-600)2029338-0 (DE-576)252613988 0959-6526 nnns volume:329 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OPC-GGO GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 43.35 Umweltrichtlinien Umweltnormen 85.35 Fertigung AR 329 |
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10.1016/j.jclepro.2021.129723 doi (DE-627)ELV00709115X (ELSEVIER)S0959-6526(21)03900-7 DE-627 ger DE-627 rda eng 690 330 DE-600 43.35 bkl 85.35 bkl Wu, Chunxu verfasserin aut Self-floating biomass charcoal supported flower-like plasmon silver/carbon, nitrogen co-doped defective TiO 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier A self-floating biomass charcoal supported flower-like plasmon Ag/C, N co-doped defective TiO2 photocatalyst is fabricated by hydrothermal, calcination and photo-deposition strategies. Biomass charcoal, Ag nanoparticles, oxygen vacancy defects and C, N co-doping all favor to extend the photoresponse to visible light region. The biomass charcoal plays the role of doping and floating supporter, which can make it float on surface of water and effectively improve the collection of sunlight. The resultant plasmon Ag/C, N co-doped defective TiO2 photocatalyst exhibits excellent visible-light-driven photocatalytic performance, in which the photocatalytic degradation ratio of 2,4-dichlorophenol and hydrogen evolution are up to 95% and 1269 μmol h−1 g−1, respectively, several times higher than that of pristine TiO2. It can be ascribed to the synergistic effect of surface plasmon resonance (SPR) effect of Ag nanoparticles, the efficient C, N co-doping and formation of oxygen vacancy defects promotes spatial charge separation and enhances visible light absorption. In addition, the long-term stability of this novel self-floating photocatalyst implies the potential practical applications. Photocatalysis Self-floating TiO Oxygen vacancy defect Surface plasmon resonance Zhang, Jiaqi verfasserin aut Fang, Bin verfasserin aut Cui, Yongqian verfasserin aut Xing, Zipeng verfasserin (orcid)0000-0002-9429-5780 aut Li, Zhenzi verfasserin aut Zhou, Wei verfasserin aut Enthalten in Journal of cleaner production Amsterdam [u.a.] : Elsevier Science, 1993 329 Online-Ressource (DE-627)324655878 (DE-600)2029338-0 (DE-576)252613988 0959-6526 nnns volume:329 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OPC-GGO GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 43.35 Umweltrichtlinien Umweltnormen 85.35 Fertigung AR 329 |
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Self-floating biomass charcoal supported flower-like plasmon silver/carbon, nitrogen co-doped defective TiO |
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Self-floating biomass charcoal supported flower-like plasmon silver/carbon, nitrogen co-doped defective TiO |
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Wu, Chunxu Zhang, Jiaqi Fang, Bin Cui, Yongqian Xing, Zipeng Li, Zhenzi Zhou, Wei |
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self-floating biomass charcoal supported flower-like plasmon silver/carbon, nitrogen co-doped defective tio |
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Self-floating biomass charcoal supported flower-like plasmon silver/carbon, nitrogen co-doped defective TiO |
| abstract |
A self-floating biomass charcoal supported flower-like plasmon Ag/C, N co-doped defective TiO2 photocatalyst is fabricated by hydrothermal, calcination and photo-deposition strategies. Biomass charcoal, Ag nanoparticles, oxygen vacancy defects and C, N co-doping all favor to extend the photoresponse to visible light region. The biomass charcoal plays the role of doping and floating supporter, which can make it float on surface of water and effectively improve the collection of sunlight. The resultant plasmon Ag/C, N co-doped defective TiO2 photocatalyst exhibits excellent visible-light-driven photocatalytic performance, in which the photocatalytic degradation ratio of 2,4-dichlorophenol and hydrogen evolution are up to 95% and 1269 μmol h−1 g−1, respectively, several times higher than that of pristine TiO2. It can be ascribed to the synergistic effect of surface plasmon resonance (SPR) effect of Ag nanoparticles, the efficient C, N co-doping and formation of oxygen vacancy defects promotes spatial charge separation and enhances visible light absorption. In addition, the long-term stability of this novel self-floating photocatalyst implies the potential practical applications. |
| abstractGer |
A self-floating biomass charcoal supported flower-like plasmon Ag/C, N co-doped defective TiO2 photocatalyst is fabricated by hydrothermal, calcination and photo-deposition strategies. Biomass charcoal, Ag nanoparticles, oxygen vacancy defects and C, N co-doping all favor to extend the photoresponse to visible light region. The biomass charcoal plays the role of doping and floating supporter, which can make it float on surface of water and effectively improve the collection of sunlight. The resultant plasmon Ag/C, N co-doped defective TiO2 photocatalyst exhibits excellent visible-light-driven photocatalytic performance, in which the photocatalytic degradation ratio of 2,4-dichlorophenol and hydrogen evolution are up to 95% and 1269 μmol h−1 g−1, respectively, several times higher than that of pristine TiO2. It can be ascribed to the synergistic effect of surface plasmon resonance (SPR) effect of Ag nanoparticles, the efficient C, N co-doping and formation of oxygen vacancy defects promotes spatial charge separation and enhances visible light absorption. In addition, the long-term stability of this novel self-floating photocatalyst implies the potential practical applications. |
| abstract_unstemmed |
A self-floating biomass charcoal supported flower-like plasmon Ag/C, N co-doped defective TiO2 photocatalyst is fabricated by hydrothermal, calcination and photo-deposition strategies. Biomass charcoal, Ag nanoparticles, oxygen vacancy defects and C, N co-doping all favor to extend the photoresponse to visible light region. The biomass charcoal plays the role of doping and floating supporter, which can make it float on surface of water and effectively improve the collection of sunlight. The resultant plasmon Ag/C, N co-doped defective TiO2 photocatalyst exhibits excellent visible-light-driven photocatalytic performance, in which the photocatalytic degradation ratio of 2,4-dichlorophenol and hydrogen evolution are up to 95% and 1269 μmol h−1 g−1, respectively, several times higher than that of pristine TiO2. It can be ascribed to the synergistic effect of surface plasmon resonance (SPR) effect of Ag nanoparticles, the efficient C, N co-doping and formation of oxygen vacancy defects promotes spatial charge separation and enhances visible light absorption. In addition, the long-term stability of this novel self-floating photocatalyst implies the potential practical applications. |
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Self-floating biomass charcoal supported flower-like plasmon silver/carbon, nitrogen co-doped defective TiO |
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