Bismuth-antimony alloy nanoparticles encapsulated in 3D carbon framework: Synergistic effect for enhancing interfacial potassium storage
Bismuth-antimony (BiSb) alloy combines the low volume expansion of Bi with the high theoretical capacity of Sb and very suitable for application for energy storage. However, the low reversible capacity and poor conductivity of BiSb are still a challenge for promoting their potassium (K) storage prop...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Wu, Qingzhao [verfasserIn] Chen, Bochao [verfasserIn] Xie, Haonan [verfasserIn] Bai, Xiangren [verfasserIn] Liang, Ming [verfasserIn] Wu, Zhiyi [verfasserIn] Jin, Xiaoying [verfasserIn] He, Chunnian [verfasserIn] Zhao, Naiqin [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2021 |
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| Schlagwörter: |
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| Übergeordnetes Werk: |
Enthalten in: The chemical engineering journal - Amsterdam : Elsevier, 1997, 430 |
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| Übergeordnetes Werk: |
volume:430 |
| DOI / URN: |
10.1016/j.cej.2021.132906 |
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| Katalog-ID: |
ELV007129785 |
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| 245 | 1 | 0 | |a Bismuth-antimony alloy nanoparticles encapsulated in 3D carbon framework: Synergistic effect for enhancing interfacial potassium storage |
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| 520 | |a Bismuth-antimony (BiSb) alloy combines the low volume expansion of Bi with the high theoretical capacity of Sb and very suitable for application for energy storage. However, the low reversible capacity and poor conductivity of BiSb are still a challenge for promoting their potassium (K) storage properties. Herein, the homogeneous BiSb nanoconfined in three-dimensional (3D) carbon framework were synthesized by NaCl-template assisted method. In the as-constructed architecture, the nano-sized BiSb alloy particles not only shorten the electronic transport route, but also offer adequate K-storage active sites by virtue of the interface between binary alloy and graphene-like coating layers, which were theoretically validated by the density functional theory simulations. Furthermore, the carbon structure can effectively alleviate the internal stress of BiSb during the charging and discharging processes due to the robust integrated structure, i.e. graphene-like layer coated BiSb that embedded into 3D carbon architecture. As a result, the composite electrode exhibits a stable cycling of 303.5 mA h g−1 after 1000 cycles at 500 mA g−1, and a high-rate performance of 246.8 mA h g−1 at 2 A g−1. This work indicates that the enhancement of interfacial K-storage through biphasic synergistic effect will serve as a reference for the development of other energy storage materials. | ||
| 650 | 4 | |a BiSb alloy | |
| 650 | 4 | |a 3D structure | |
| 650 | 4 | |a Synergy effect | |
| 650 | 4 | |a Interface | |
| 650 | 4 | |a Potassium-ion batteries | |
| 700 | 1 | |a Chen, Bochao |e verfasserin |4 aut | |
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| 700 | 1 | |a Liang, Ming |e verfasserin |4 aut | |
| 700 | 1 | |a Wu, Zhiyi |e verfasserin |4 aut | |
| 700 | 1 | |a Jin, Xiaoying |e verfasserin |4 aut | |
| 700 | 1 | |a He, Chunnian |e verfasserin |4 aut | |
| 700 | 1 | |a Zhao, Naiqin |e verfasserin |4 aut | |
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10.1016/j.cej.2021.132906 doi (DE-627)ELV007129785 (ELSEVIER)S1385-8947(21)04481-8 DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Wu, Qingzhao verfasserin aut Bismuth-antimony alloy nanoparticles encapsulated in 3D carbon framework: Synergistic effect for enhancing interfacial potassium storage 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Bismuth-antimony (BiSb) alloy combines the low volume expansion of Bi with the high theoretical capacity of Sb and very suitable for application for energy storage. However, the low reversible capacity and poor conductivity of BiSb are still a challenge for promoting their potassium (K) storage properties. Herein, the homogeneous BiSb nanoconfined in three-dimensional (3D) carbon framework were synthesized by NaCl-template assisted method. In the as-constructed architecture, the nano-sized BiSb alloy particles not only shorten the electronic transport route, but also offer adequate K-storage active sites by virtue of the interface between binary alloy and graphene-like coating layers, which were theoretically validated by the density functional theory simulations. Furthermore, the carbon structure can effectively alleviate the internal stress of BiSb during the charging and discharging processes due to the robust integrated structure, i.e. graphene-like layer coated BiSb that embedded into 3D carbon architecture. As a result, the composite electrode exhibits a stable cycling of 303.5 mA h g−1 after 1000 cycles at 500 mA g−1, and a high-rate performance of 246.8 mA h g−1 at 2 A g−1. This work indicates that the enhancement of interfacial K-storage through biphasic synergistic effect will serve as a reference for the development of other energy storage materials. BiSb alloy 3D structure Synergy effect Interface Potassium-ion batteries Chen, Bochao verfasserin aut Xie, Haonan verfasserin aut Bai, Xiangren verfasserin aut Liang, Ming verfasserin aut Wu, Zhiyi verfasserin aut Jin, Xiaoying verfasserin aut He, Chunnian verfasserin aut Zhao, Naiqin verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 430 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:430 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 430 045F 660.05 |
| spelling |
10.1016/j.cej.2021.132906 doi (DE-627)ELV007129785 (ELSEVIER)S1385-8947(21)04481-8 DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Wu, Qingzhao verfasserin aut Bismuth-antimony alloy nanoparticles encapsulated in 3D carbon framework: Synergistic effect for enhancing interfacial potassium storage 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Bismuth-antimony (BiSb) alloy combines the low volume expansion of Bi with the high theoretical capacity of Sb and very suitable for application for energy storage. However, the low reversible capacity and poor conductivity of BiSb are still a challenge for promoting their potassium (K) storage properties. Herein, the homogeneous BiSb nanoconfined in three-dimensional (3D) carbon framework were synthesized by NaCl-template assisted method. In the as-constructed architecture, the nano-sized BiSb alloy particles not only shorten the electronic transport route, but also offer adequate K-storage active sites by virtue of the interface between binary alloy and graphene-like coating layers, which were theoretically validated by the density functional theory simulations. Furthermore, the carbon structure can effectively alleviate the internal stress of BiSb during the charging and discharging processes due to the robust integrated structure, i.e. graphene-like layer coated BiSb that embedded into 3D carbon architecture. As a result, the composite electrode exhibits a stable cycling of 303.5 mA h g−1 after 1000 cycles at 500 mA g−1, and a high-rate performance of 246.8 mA h g−1 at 2 A g−1. This work indicates that the enhancement of interfacial K-storage through biphasic synergistic effect will serve as a reference for the development of other energy storage materials. BiSb alloy 3D structure Synergy effect Interface Potassium-ion batteries Chen, Bochao verfasserin aut Xie, Haonan verfasserin aut Bai, Xiangren verfasserin aut Liang, Ming verfasserin aut Wu, Zhiyi verfasserin aut Jin, Xiaoying verfasserin aut He, Chunnian verfasserin aut Zhao, Naiqin verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 430 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:430 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 430 045F 660.05 |
| allfields_unstemmed |
10.1016/j.cej.2021.132906 doi (DE-627)ELV007129785 (ELSEVIER)S1385-8947(21)04481-8 DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Wu, Qingzhao verfasserin aut Bismuth-antimony alloy nanoparticles encapsulated in 3D carbon framework: Synergistic effect for enhancing interfacial potassium storage 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Bismuth-antimony (BiSb) alloy combines the low volume expansion of Bi with the high theoretical capacity of Sb and very suitable for application for energy storage. However, the low reversible capacity and poor conductivity of BiSb are still a challenge for promoting their potassium (K) storage properties. Herein, the homogeneous BiSb nanoconfined in three-dimensional (3D) carbon framework were synthesized by NaCl-template assisted method. In the as-constructed architecture, the nano-sized BiSb alloy particles not only shorten the electronic transport route, but also offer adequate K-storage active sites by virtue of the interface between binary alloy and graphene-like coating layers, which were theoretically validated by the density functional theory simulations. Furthermore, the carbon structure can effectively alleviate the internal stress of BiSb during the charging and discharging processes due to the robust integrated structure, i.e. graphene-like layer coated BiSb that embedded into 3D carbon architecture. As a result, the composite electrode exhibits a stable cycling of 303.5 mA h g−1 after 1000 cycles at 500 mA g−1, and a high-rate performance of 246.8 mA h g−1 at 2 A g−1. This work indicates that the enhancement of interfacial K-storage through biphasic synergistic effect will serve as a reference for the development of other energy storage materials. BiSb alloy 3D structure Synergy effect Interface Potassium-ion batteries Chen, Bochao verfasserin aut Xie, Haonan verfasserin aut Bai, Xiangren verfasserin aut Liang, Ming verfasserin aut Wu, Zhiyi verfasserin aut Jin, Xiaoying verfasserin aut He, Chunnian verfasserin aut Zhao, Naiqin verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 430 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:430 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 430 045F 660.05 |
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10.1016/j.cej.2021.132906 doi (DE-627)ELV007129785 (ELSEVIER)S1385-8947(21)04481-8 DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Wu, Qingzhao verfasserin aut Bismuth-antimony alloy nanoparticles encapsulated in 3D carbon framework: Synergistic effect for enhancing interfacial potassium storage 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Bismuth-antimony (BiSb) alloy combines the low volume expansion of Bi with the high theoretical capacity of Sb and very suitable for application for energy storage. However, the low reversible capacity and poor conductivity of BiSb are still a challenge for promoting their potassium (K) storage properties. Herein, the homogeneous BiSb nanoconfined in three-dimensional (3D) carbon framework were synthesized by NaCl-template assisted method. In the as-constructed architecture, the nano-sized BiSb alloy particles not only shorten the electronic transport route, but also offer adequate K-storage active sites by virtue of the interface between binary alloy and graphene-like coating layers, which were theoretically validated by the density functional theory simulations. Furthermore, the carbon structure can effectively alleviate the internal stress of BiSb during the charging and discharging processes due to the robust integrated structure, i.e. graphene-like layer coated BiSb that embedded into 3D carbon architecture. As a result, the composite electrode exhibits a stable cycling of 303.5 mA h g−1 after 1000 cycles at 500 mA g−1, and a high-rate performance of 246.8 mA h g−1 at 2 A g−1. This work indicates that the enhancement of interfacial K-storage through biphasic synergistic effect will serve as a reference for the development of other energy storage materials. BiSb alloy 3D structure Synergy effect Interface Potassium-ion batteries Chen, Bochao verfasserin aut Xie, Haonan verfasserin aut Bai, Xiangren verfasserin aut Liang, Ming verfasserin aut Wu, Zhiyi verfasserin aut Jin, Xiaoying verfasserin aut He, Chunnian verfasserin aut Zhao, Naiqin verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 430 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:430 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 430 045F 660.05 |
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10.1016/j.cej.2021.132906 doi (DE-627)ELV007129785 (ELSEVIER)S1385-8947(21)04481-8 DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Wu, Qingzhao verfasserin aut Bismuth-antimony alloy nanoparticles encapsulated in 3D carbon framework: Synergistic effect for enhancing interfacial potassium storage 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Bismuth-antimony (BiSb) alloy combines the low volume expansion of Bi with the high theoretical capacity of Sb and very suitable for application for energy storage. However, the low reversible capacity and poor conductivity of BiSb are still a challenge for promoting their potassium (K) storage properties. Herein, the homogeneous BiSb nanoconfined in three-dimensional (3D) carbon framework were synthesized by NaCl-template assisted method. In the as-constructed architecture, the nano-sized BiSb alloy particles not only shorten the electronic transport route, but also offer adequate K-storage active sites by virtue of the interface between binary alloy and graphene-like coating layers, which were theoretically validated by the density functional theory simulations. Furthermore, the carbon structure can effectively alleviate the internal stress of BiSb during the charging and discharging processes due to the robust integrated structure, i.e. graphene-like layer coated BiSb that embedded into 3D carbon architecture. As a result, the composite electrode exhibits a stable cycling of 303.5 mA h g−1 after 1000 cycles at 500 mA g−1, and a high-rate performance of 246.8 mA h g−1 at 2 A g−1. This work indicates that the enhancement of interfacial K-storage through biphasic synergistic effect will serve as a reference for the development of other energy storage materials. BiSb alloy 3D structure Synergy effect Interface Potassium-ion batteries Chen, Bochao verfasserin aut Xie, Haonan verfasserin aut Bai, Xiangren verfasserin aut Liang, Ming verfasserin aut Wu, Zhiyi verfasserin aut Jin, Xiaoying verfasserin aut He, Chunnian verfasserin aut Zhao, Naiqin verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 430 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:430 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 430 045F 660.05 |
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Wu, Qingzhao |
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Wu, Qingzhao ddc 660.05 ddc 660 bkl 58.10 misc BiSb alloy misc 3D structure misc Synergy effect misc Interface misc Potassium-ion batteries Bismuth-antimony alloy nanoparticles encapsulated in 3D carbon framework: Synergistic effect for enhancing interfacial potassium storage |
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660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Bismuth-antimony alloy nanoparticles encapsulated in 3D carbon framework: Synergistic effect for enhancing interfacial potassium storage BiSb alloy 3D structure Synergy effect Interface Potassium-ion batteries |
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Bismuth-antimony alloy nanoparticles encapsulated in 3D carbon framework: Synergistic effect for enhancing interfacial potassium storage |
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Bismuth-antimony alloy nanoparticles encapsulated in 3D carbon framework: Synergistic effect for enhancing interfacial potassium storage |
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Wu, Qingzhao Chen, Bochao Xie, Haonan Bai, Xiangren Liang, Ming Wu, Zhiyi Jin, Xiaoying He, Chunnian Zhao, Naiqin |
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bismuth-antimony alloy nanoparticles encapsulated in 3d carbon framework: synergistic effect for enhancing interfacial potassium storage |
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Bismuth-antimony alloy nanoparticles encapsulated in 3D carbon framework: Synergistic effect for enhancing interfacial potassium storage |
| abstract |
Bismuth-antimony (BiSb) alloy combines the low volume expansion of Bi with the high theoretical capacity of Sb and very suitable for application for energy storage. However, the low reversible capacity and poor conductivity of BiSb are still a challenge for promoting their potassium (K) storage properties. Herein, the homogeneous BiSb nanoconfined in three-dimensional (3D) carbon framework were synthesized by NaCl-template assisted method. In the as-constructed architecture, the nano-sized BiSb alloy particles not only shorten the electronic transport route, but also offer adequate K-storage active sites by virtue of the interface between binary alloy and graphene-like coating layers, which were theoretically validated by the density functional theory simulations. Furthermore, the carbon structure can effectively alleviate the internal stress of BiSb during the charging and discharging processes due to the robust integrated structure, i.e. graphene-like layer coated BiSb that embedded into 3D carbon architecture. As a result, the composite electrode exhibits a stable cycling of 303.5 mA h g−1 after 1000 cycles at 500 mA g−1, and a high-rate performance of 246.8 mA h g−1 at 2 A g−1. This work indicates that the enhancement of interfacial K-storage through biphasic synergistic effect will serve as a reference for the development of other energy storage materials. |
| abstractGer |
Bismuth-antimony (BiSb) alloy combines the low volume expansion of Bi with the high theoretical capacity of Sb and very suitable for application for energy storage. However, the low reversible capacity and poor conductivity of BiSb are still a challenge for promoting their potassium (K) storage properties. Herein, the homogeneous BiSb nanoconfined in three-dimensional (3D) carbon framework were synthesized by NaCl-template assisted method. In the as-constructed architecture, the nano-sized BiSb alloy particles not only shorten the electronic transport route, but also offer adequate K-storage active sites by virtue of the interface between binary alloy and graphene-like coating layers, which were theoretically validated by the density functional theory simulations. Furthermore, the carbon structure can effectively alleviate the internal stress of BiSb during the charging and discharging processes due to the robust integrated structure, i.e. graphene-like layer coated BiSb that embedded into 3D carbon architecture. As a result, the composite electrode exhibits a stable cycling of 303.5 mA h g−1 after 1000 cycles at 500 mA g−1, and a high-rate performance of 246.8 mA h g−1 at 2 A g−1. This work indicates that the enhancement of interfacial K-storage through biphasic synergistic effect will serve as a reference for the development of other energy storage materials. |
| abstract_unstemmed |
Bismuth-antimony (BiSb) alloy combines the low volume expansion of Bi with the high theoretical capacity of Sb and very suitable for application for energy storage. However, the low reversible capacity and poor conductivity of BiSb are still a challenge for promoting their potassium (K) storage properties. Herein, the homogeneous BiSb nanoconfined in three-dimensional (3D) carbon framework were synthesized by NaCl-template assisted method. In the as-constructed architecture, the nano-sized BiSb alloy particles not only shorten the electronic transport route, but also offer adequate K-storage active sites by virtue of the interface between binary alloy and graphene-like coating layers, which were theoretically validated by the density functional theory simulations. Furthermore, the carbon structure can effectively alleviate the internal stress of BiSb during the charging and discharging processes due to the robust integrated structure, i.e. graphene-like layer coated BiSb that embedded into 3D carbon architecture. As a result, the composite electrode exhibits a stable cycling of 303.5 mA h g−1 after 1000 cycles at 500 mA g−1, and a high-rate performance of 246.8 mA h g−1 at 2 A g−1. This work indicates that the enhancement of interfacial K-storage through biphasic synergistic effect will serve as a reference for the development of other energy storage materials. |
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Bismuth-antimony alloy nanoparticles encapsulated in 3D carbon framework: Synergistic effect for enhancing interfacial potassium storage |
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