Preparation of durable magnesium oxysulfate cement with the incorporation of mineral admixtures and sequestration of carbon dioxide
To reduce the consumption of energy and raw materials caused by the production of Portland cement and enhance the carbon dioxide sequestration of building materials, this paper aims to manufacture durable and green magnesium oxysulfate cement based on incorporating mineral admixtures (fly ash (FA) o...
Ausführliche Beschreibung
Autor*in: |
Li, Qiyan [verfasserIn] Su, Anshuang [verfasserIn] Gao, Xiaojian [verfasserIn] |
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Format: |
E-Artikel |
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Sprache: |
Englisch |
Erschienen: |
2021 |
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Schlagwörter: |
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Übergeordnetes Werk: |
Enthalten in: The science of the total environment - Amsterdam [u.a.] : Elsevier Science, 1972, 809 |
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Übergeordnetes Werk: |
volume:809 |
DOI / URN: |
10.1016/j.scitotenv.2021.152127 |
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Katalog-ID: |
ELV007258879 |
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245 | 1 | 0 | |a Preparation of durable magnesium oxysulfate cement with the incorporation of mineral admixtures and sequestration of carbon dioxide |
264 | 1 | |c 2021 | |
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520 | |a To reduce the consumption of energy and raw materials caused by the production of Portland cement and enhance the carbon dioxide sequestration of building materials, this paper aims to manufacture durable and green magnesium oxysulfate cement based on incorporating mineral admixtures (fly ash (FA) or ground granulated blast-furnace slag (GGBFS)) and CO2 curing treatment. Compressive strength, flexural strength, resistance to water and wetting-drying cycles of magnesium oxysulfate (MOS) were evaluated. Phase compositions and microstructures of typical samples were measured by X-ray diffraction (XRD), differential scanning calorimetry (DSC-TG), and scanning electron microscope (SEM) techniques. The results showed that mechanical strength and strength retention after wetting-drying treatment of MOS cement was increased by the sequestration of carbon dioxide. Both FA and GGBFS could improve the water resistance due to restrainting the phase conversion of MgO into Mg(OH)2. However, the addition of FA or GGBFS deteriorated the compressive strength of MOS cement samples after wetting-drying treatment, owing to the formation of more magnesium hydroxide crystals and decomposition of 5 Mg(OH)2·MgSO4·7H2O (5·1·7 phase). Furthermore, about 5% carbon dioxide can be captured by MOS cement paste during 24 h accelerated carbonation treatment. Therefore, the incorporation of mineral admixtures and sequestration of carbon dioxide was suggested as an effective method in manufacturing the highly durable and cleaner magnesium oxysulfate cement. | ||
650 | 4 | |a Magnesium oxysulfate cement | |
650 | 4 | |a Sequestration of CO | |
650 | 4 | |a Durable | |
650 | 4 | |a Compressive strength | |
650 | 4 | |a Water resistance | |
700 | 1 | |a Su, Anshuang |e verfasserin |4 aut | |
700 | 1 | |a Gao, Xiaojian |e verfasserin |4 aut | |
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allfields |
10.1016/j.scitotenv.2021.152127 doi (DE-627)ELV007258879 (ELSEVIER)S0048-9697(21)07203-X DE-627 ger DE-627 rda eng 333.7 610 DE-600 43.12 bkl 43.13 bkl 44.13 bkl Li, Qiyan verfasserin aut Preparation of durable magnesium oxysulfate cement with the incorporation of mineral admixtures and sequestration of carbon dioxide 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier To reduce the consumption of energy and raw materials caused by the production of Portland cement and enhance the carbon dioxide sequestration of building materials, this paper aims to manufacture durable and green magnesium oxysulfate cement based on incorporating mineral admixtures (fly ash (FA) or ground granulated blast-furnace slag (GGBFS)) and CO2 curing treatment. Compressive strength, flexural strength, resistance to water and wetting-drying cycles of magnesium oxysulfate (MOS) were evaluated. Phase compositions and microstructures of typical samples were measured by X-ray diffraction (XRD), differential scanning calorimetry (DSC-TG), and scanning electron microscope (SEM) techniques. The results showed that mechanical strength and strength retention after wetting-drying treatment of MOS cement was increased by the sequestration of carbon dioxide. Both FA and GGBFS could improve the water resistance due to restrainting the phase conversion of MgO into Mg(OH)2. However, the addition of FA or GGBFS deteriorated the compressive strength of MOS cement samples after wetting-drying treatment, owing to the formation of more magnesium hydroxide crystals and decomposition of 5 Mg(OH)2·MgSO4·7H2O (5·1·7 phase). Furthermore, about 5% carbon dioxide can be captured by MOS cement paste during 24 h accelerated carbonation treatment. Therefore, the incorporation of mineral admixtures and sequestration of carbon dioxide was suggested as an effective method in manufacturing the highly durable and cleaner magnesium oxysulfate cement. Magnesium oxysulfate cement Sequestration of CO Durable Compressive strength Water resistance Su, Anshuang verfasserin aut Gao, Xiaojian verfasserin aut Enthalten in The science of the total environment Amsterdam [u.a.] : Elsevier Science, 1972 809 Online-Ressource (DE-627)306591456 (DE-600)1498726-0 (DE-576)081953178 1879-1026 nnns volume:809 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA SSG-OPC-GGO GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 43.12 Umweltchemie 43.13 Umwelttoxikologie 44.13 Medizinische Ökologie AR 809 |
spelling |
10.1016/j.scitotenv.2021.152127 doi (DE-627)ELV007258879 (ELSEVIER)S0048-9697(21)07203-X DE-627 ger DE-627 rda eng 333.7 610 DE-600 43.12 bkl 43.13 bkl 44.13 bkl Li, Qiyan verfasserin aut Preparation of durable magnesium oxysulfate cement with the incorporation of mineral admixtures and sequestration of carbon dioxide 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier To reduce the consumption of energy and raw materials caused by the production of Portland cement and enhance the carbon dioxide sequestration of building materials, this paper aims to manufacture durable and green magnesium oxysulfate cement based on incorporating mineral admixtures (fly ash (FA) or ground granulated blast-furnace slag (GGBFS)) and CO2 curing treatment. Compressive strength, flexural strength, resistance to water and wetting-drying cycles of magnesium oxysulfate (MOS) were evaluated. Phase compositions and microstructures of typical samples were measured by X-ray diffraction (XRD), differential scanning calorimetry (DSC-TG), and scanning electron microscope (SEM) techniques. The results showed that mechanical strength and strength retention after wetting-drying treatment of MOS cement was increased by the sequestration of carbon dioxide. Both FA and GGBFS could improve the water resistance due to restrainting the phase conversion of MgO into Mg(OH)2. However, the addition of FA or GGBFS deteriorated the compressive strength of MOS cement samples after wetting-drying treatment, owing to the formation of more magnesium hydroxide crystals and decomposition of 5 Mg(OH)2·MgSO4·7H2O (5·1·7 phase). Furthermore, about 5% carbon dioxide can be captured by MOS cement paste during 24 h accelerated carbonation treatment. Therefore, the incorporation of mineral admixtures and sequestration of carbon dioxide was suggested as an effective method in manufacturing the highly durable and cleaner magnesium oxysulfate cement. Magnesium oxysulfate cement Sequestration of CO Durable Compressive strength Water resistance Su, Anshuang verfasserin aut Gao, Xiaojian verfasserin aut Enthalten in The science of the total environment Amsterdam [u.a.] : Elsevier Science, 1972 809 Online-Ressource (DE-627)306591456 (DE-600)1498726-0 (DE-576)081953178 1879-1026 nnns volume:809 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA SSG-OPC-GGO GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 43.12 Umweltchemie 43.13 Umwelttoxikologie 44.13 Medizinische Ökologie AR 809 |
allfields_unstemmed |
10.1016/j.scitotenv.2021.152127 doi (DE-627)ELV007258879 (ELSEVIER)S0048-9697(21)07203-X DE-627 ger DE-627 rda eng 333.7 610 DE-600 43.12 bkl 43.13 bkl 44.13 bkl Li, Qiyan verfasserin aut Preparation of durable magnesium oxysulfate cement with the incorporation of mineral admixtures and sequestration of carbon dioxide 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier To reduce the consumption of energy and raw materials caused by the production of Portland cement and enhance the carbon dioxide sequestration of building materials, this paper aims to manufacture durable and green magnesium oxysulfate cement based on incorporating mineral admixtures (fly ash (FA) or ground granulated blast-furnace slag (GGBFS)) and CO2 curing treatment. Compressive strength, flexural strength, resistance to water and wetting-drying cycles of magnesium oxysulfate (MOS) were evaluated. Phase compositions and microstructures of typical samples were measured by X-ray diffraction (XRD), differential scanning calorimetry (DSC-TG), and scanning electron microscope (SEM) techniques. The results showed that mechanical strength and strength retention after wetting-drying treatment of MOS cement was increased by the sequestration of carbon dioxide. Both FA and GGBFS could improve the water resistance due to restrainting the phase conversion of MgO into Mg(OH)2. However, the addition of FA or GGBFS deteriorated the compressive strength of MOS cement samples after wetting-drying treatment, owing to the formation of more magnesium hydroxide crystals and decomposition of 5 Mg(OH)2·MgSO4·7H2O (5·1·7 phase). Furthermore, about 5% carbon dioxide can be captured by MOS cement paste during 24 h accelerated carbonation treatment. Therefore, the incorporation of mineral admixtures and sequestration of carbon dioxide was suggested as an effective method in manufacturing the highly durable and cleaner magnesium oxysulfate cement. Magnesium oxysulfate cement Sequestration of CO Durable Compressive strength Water resistance Su, Anshuang verfasserin aut Gao, Xiaojian verfasserin aut Enthalten in The science of the total environment Amsterdam [u.a.] : Elsevier Science, 1972 809 Online-Ressource (DE-627)306591456 (DE-600)1498726-0 (DE-576)081953178 1879-1026 nnns volume:809 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA SSG-OPC-GGO GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 43.12 Umweltchemie 43.13 Umwelttoxikologie 44.13 Medizinische Ökologie AR 809 |
allfieldsGer |
10.1016/j.scitotenv.2021.152127 doi (DE-627)ELV007258879 (ELSEVIER)S0048-9697(21)07203-X DE-627 ger DE-627 rda eng 333.7 610 DE-600 43.12 bkl 43.13 bkl 44.13 bkl Li, Qiyan verfasserin aut Preparation of durable magnesium oxysulfate cement with the incorporation of mineral admixtures and sequestration of carbon dioxide 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier To reduce the consumption of energy and raw materials caused by the production of Portland cement and enhance the carbon dioxide sequestration of building materials, this paper aims to manufacture durable and green magnesium oxysulfate cement based on incorporating mineral admixtures (fly ash (FA) or ground granulated blast-furnace slag (GGBFS)) and CO2 curing treatment. Compressive strength, flexural strength, resistance to water and wetting-drying cycles of magnesium oxysulfate (MOS) were evaluated. Phase compositions and microstructures of typical samples were measured by X-ray diffraction (XRD), differential scanning calorimetry (DSC-TG), and scanning electron microscope (SEM) techniques. The results showed that mechanical strength and strength retention after wetting-drying treatment of MOS cement was increased by the sequestration of carbon dioxide. Both FA and GGBFS could improve the water resistance due to restrainting the phase conversion of MgO into Mg(OH)2. However, the addition of FA or GGBFS deteriorated the compressive strength of MOS cement samples after wetting-drying treatment, owing to the formation of more magnesium hydroxide crystals and decomposition of 5 Mg(OH)2·MgSO4·7H2O (5·1·7 phase). Furthermore, about 5% carbon dioxide can be captured by MOS cement paste during 24 h accelerated carbonation treatment. Therefore, the incorporation of mineral admixtures and sequestration of carbon dioxide was suggested as an effective method in manufacturing the highly durable and cleaner magnesium oxysulfate cement. Magnesium oxysulfate cement Sequestration of CO Durable Compressive strength Water resistance Su, Anshuang verfasserin aut Gao, Xiaojian verfasserin aut Enthalten in The science of the total environment Amsterdam [u.a.] : Elsevier Science, 1972 809 Online-Ressource (DE-627)306591456 (DE-600)1498726-0 (DE-576)081953178 1879-1026 nnns volume:809 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA SSG-OPC-GGO GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 43.12 Umweltchemie 43.13 Umwelttoxikologie 44.13 Medizinische Ökologie AR 809 |
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10.1016/j.scitotenv.2021.152127 doi (DE-627)ELV007258879 (ELSEVIER)S0048-9697(21)07203-X DE-627 ger DE-627 rda eng 333.7 610 DE-600 43.12 bkl 43.13 bkl 44.13 bkl Li, Qiyan verfasserin aut Preparation of durable magnesium oxysulfate cement with the incorporation of mineral admixtures and sequestration of carbon dioxide 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier To reduce the consumption of energy and raw materials caused by the production of Portland cement and enhance the carbon dioxide sequestration of building materials, this paper aims to manufacture durable and green magnesium oxysulfate cement based on incorporating mineral admixtures (fly ash (FA) or ground granulated blast-furnace slag (GGBFS)) and CO2 curing treatment. Compressive strength, flexural strength, resistance to water and wetting-drying cycles of magnesium oxysulfate (MOS) were evaluated. Phase compositions and microstructures of typical samples were measured by X-ray diffraction (XRD), differential scanning calorimetry (DSC-TG), and scanning electron microscope (SEM) techniques. The results showed that mechanical strength and strength retention after wetting-drying treatment of MOS cement was increased by the sequestration of carbon dioxide. Both FA and GGBFS could improve the water resistance due to restrainting the phase conversion of MgO into Mg(OH)2. However, the addition of FA or GGBFS deteriorated the compressive strength of MOS cement samples after wetting-drying treatment, owing to the formation of more magnesium hydroxide crystals and decomposition of 5 Mg(OH)2·MgSO4·7H2O (5·1·7 phase). Furthermore, about 5% carbon dioxide can be captured by MOS cement paste during 24 h accelerated carbonation treatment. Therefore, the incorporation of mineral admixtures and sequestration of carbon dioxide was suggested as an effective method in manufacturing the highly durable and cleaner magnesium oxysulfate cement. Magnesium oxysulfate cement Sequestration of CO Durable Compressive strength Water resistance Su, Anshuang verfasserin aut Gao, Xiaojian verfasserin aut Enthalten in The science of the total environment Amsterdam [u.a.] : Elsevier Science, 1972 809 Online-Ressource (DE-627)306591456 (DE-600)1498726-0 (DE-576)081953178 1879-1026 nnns volume:809 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA SSG-OPC-GGO GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 43.12 Umweltchemie 43.13 Umwelttoxikologie 44.13 Medizinische Ökologie AR 809 |
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333.7 610 DE-600 43.12 bkl 43.13 bkl 44.13 bkl Preparation of durable magnesium oxysulfate cement with the incorporation of mineral admixtures and sequestration of carbon dioxide Magnesium oxysulfate cement Sequestration of CO Durable Compressive strength Water resistance |
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Preparation of durable magnesium oxysulfate cement with the incorporation of mineral admixtures and sequestration of carbon dioxide |
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Preparation of durable magnesium oxysulfate cement with the incorporation of mineral admixtures and sequestration of carbon dioxide |
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Li, Qiyan |
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Li, Qiyan Su, Anshuang Gao, Xiaojian |
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10.1016/j.scitotenv.2021.152127 |
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preparation of durable magnesium oxysulfate cement with the incorporation of mineral admixtures and sequestration of carbon dioxide |
title_auth |
Preparation of durable magnesium oxysulfate cement with the incorporation of mineral admixtures and sequestration of carbon dioxide |
abstract |
To reduce the consumption of energy and raw materials caused by the production of Portland cement and enhance the carbon dioxide sequestration of building materials, this paper aims to manufacture durable and green magnesium oxysulfate cement based on incorporating mineral admixtures (fly ash (FA) or ground granulated blast-furnace slag (GGBFS)) and CO2 curing treatment. Compressive strength, flexural strength, resistance to water and wetting-drying cycles of magnesium oxysulfate (MOS) were evaluated. Phase compositions and microstructures of typical samples were measured by X-ray diffraction (XRD), differential scanning calorimetry (DSC-TG), and scanning electron microscope (SEM) techniques. The results showed that mechanical strength and strength retention after wetting-drying treatment of MOS cement was increased by the sequestration of carbon dioxide. Both FA and GGBFS could improve the water resistance due to restrainting the phase conversion of MgO into Mg(OH)2. However, the addition of FA or GGBFS deteriorated the compressive strength of MOS cement samples after wetting-drying treatment, owing to the formation of more magnesium hydroxide crystals and decomposition of 5 Mg(OH)2·MgSO4·7H2O (5·1·7 phase). Furthermore, about 5% carbon dioxide can be captured by MOS cement paste during 24 h accelerated carbonation treatment. Therefore, the incorporation of mineral admixtures and sequestration of carbon dioxide was suggested as an effective method in manufacturing the highly durable and cleaner magnesium oxysulfate cement. |
abstractGer |
To reduce the consumption of energy and raw materials caused by the production of Portland cement and enhance the carbon dioxide sequestration of building materials, this paper aims to manufacture durable and green magnesium oxysulfate cement based on incorporating mineral admixtures (fly ash (FA) or ground granulated blast-furnace slag (GGBFS)) and CO2 curing treatment. Compressive strength, flexural strength, resistance to water and wetting-drying cycles of magnesium oxysulfate (MOS) were evaluated. Phase compositions and microstructures of typical samples were measured by X-ray diffraction (XRD), differential scanning calorimetry (DSC-TG), and scanning electron microscope (SEM) techniques. The results showed that mechanical strength and strength retention after wetting-drying treatment of MOS cement was increased by the sequestration of carbon dioxide. Both FA and GGBFS could improve the water resistance due to restrainting the phase conversion of MgO into Mg(OH)2. However, the addition of FA or GGBFS deteriorated the compressive strength of MOS cement samples after wetting-drying treatment, owing to the formation of more magnesium hydroxide crystals and decomposition of 5 Mg(OH)2·MgSO4·7H2O (5·1·7 phase). Furthermore, about 5% carbon dioxide can be captured by MOS cement paste during 24 h accelerated carbonation treatment. Therefore, the incorporation of mineral admixtures and sequestration of carbon dioxide was suggested as an effective method in manufacturing the highly durable and cleaner magnesium oxysulfate cement. |
abstract_unstemmed |
To reduce the consumption of energy and raw materials caused by the production of Portland cement and enhance the carbon dioxide sequestration of building materials, this paper aims to manufacture durable and green magnesium oxysulfate cement based on incorporating mineral admixtures (fly ash (FA) or ground granulated blast-furnace slag (GGBFS)) and CO2 curing treatment. Compressive strength, flexural strength, resistance to water and wetting-drying cycles of magnesium oxysulfate (MOS) were evaluated. Phase compositions and microstructures of typical samples were measured by X-ray diffraction (XRD), differential scanning calorimetry (DSC-TG), and scanning electron microscope (SEM) techniques. The results showed that mechanical strength and strength retention after wetting-drying treatment of MOS cement was increased by the sequestration of carbon dioxide. Both FA and GGBFS could improve the water resistance due to restrainting the phase conversion of MgO into Mg(OH)2. However, the addition of FA or GGBFS deteriorated the compressive strength of MOS cement samples after wetting-drying treatment, owing to the formation of more magnesium hydroxide crystals and decomposition of 5 Mg(OH)2·MgSO4·7H2O (5·1·7 phase). Furthermore, about 5% carbon dioxide can be captured by MOS cement paste during 24 h accelerated carbonation treatment. Therefore, the incorporation of mineral admixtures and sequestration of carbon dioxide was suggested as an effective method in manufacturing the highly durable and cleaner magnesium oxysulfate cement. |
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Preparation of durable magnesium oxysulfate cement with the incorporation of mineral admixtures and sequestration of carbon dioxide |
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