Boron doped C

Compared to g-C3N4, g-C3N5 can harvest more visible light and prolong the lifetime of photogenerated carriers, and exhibited a more excellent NH3 yield under visible light. A new catalyst boron doping g-C3N5 (B-C3N5) was prepared by a simple one-step calcination for photocatalytic nitrogen fixation....
Ausführliche Beschreibung

Gespeichert in:

Autor*in:	Li, Kang [verfasserIn] Cai, Wei [verfasserIn] Zhang, Zhicheng [verfasserIn] Xie, Huifang [verfasserIn] Zhong, Qin [verfasserIn] Qu, Hongxia [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2022

Schlagwörter:	g-C B-doping Photocatalytic N

Übergeordnetes Werk:	Enthalten in: The chemical engineering journal - Amsterdam : Elsevier, 1997, 435
Übergeordnetes Werk:	volume:435

DOI / URN:	10.1016/j.cej.2022.135017

Katalog-ID:	ELV007483805

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allfields	10.1016/j.cej.2022.135017 doi (DE-627)ELV007483805 (ELSEVIER)S1385-8947(22)00523-X DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Li, Kang verfasserin aut Boron doped C 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Compared to g-C3N4, g-C3N5 can harvest more visible light and prolong the lifetime of photogenerated carriers, and exhibited a more excellent NH3 yield under visible light. A new catalyst boron doping g-C3N5 (B-C3N5) was prepared by a simple one-step calcination for photocatalytic nitrogen fixation. B-C3N5 achieved the NH3 yield up to 421.18 μmol h−1 g−1. Raman and ESR analysis reveal that the B tend to occupy the C vacancies in C3N5, which effectively improve the charge transfer capability and optimize band structure of B-C3N5. The B sites display perfect performance for N2 adsorption and activation to generate NH3. The intermediates of NRR process are identified by in-situ DRIFTS and a reaction mechanism is proposed to reveal the role of the B − O − H during the N2 adsorption, activation, and reduction process. g-C B-doping Photocatalytic N N Cai, Wei verfasserin aut Zhang, Zhicheng verfasserin aut Xie, Huifang verfasserin aut Zhong, Qin verfasserin aut Qu, Hongxia verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 435 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:435 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 435 045F 660.05
spelling	10.1016/j.cej.2022.135017 doi (DE-627)ELV007483805 (ELSEVIER)S1385-8947(22)00523-X DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Li, Kang verfasserin aut Boron doped C 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Compared to g-C3N4, g-C3N5 can harvest more visible light and prolong the lifetime of photogenerated carriers, and exhibited a more excellent NH3 yield under visible light. A new catalyst boron doping g-C3N5 (B-C3N5) was prepared by a simple one-step calcination for photocatalytic nitrogen fixation. B-C3N5 achieved the NH3 yield up to 421.18 μmol h−1 g−1. Raman and ESR analysis reveal that the B tend to occupy the C vacancies in C3N5, which effectively improve the charge transfer capability and optimize band structure of B-C3N5. The B sites display perfect performance for N2 adsorption and activation to generate NH3. The intermediates of NRR process are identified by in-situ DRIFTS and a reaction mechanism is proposed to reveal the role of the B − O − H during the N2 adsorption, activation, and reduction process. g-C B-doping Photocatalytic N N Cai, Wei verfasserin aut Zhang, Zhicheng verfasserin aut Xie, Huifang verfasserin aut Zhong, Qin verfasserin aut Qu, Hongxia verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 435 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:435 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 435 045F 660.05
allfields_unstemmed	10.1016/j.cej.2022.135017 doi (DE-627)ELV007483805 (ELSEVIER)S1385-8947(22)00523-X DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Li, Kang verfasserin aut Boron doped C 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Compared to g-C3N4, g-C3N5 can harvest more visible light and prolong the lifetime of photogenerated carriers, and exhibited a more excellent NH3 yield under visible light. A new catalyst boron doping g-C3N5 (B-C3N5) was prepared by a simple one-step calcination for photocatalytic nitrogen fixation. B-C3N5 achieved the NH3 yield up to 421.18 μmol h−1 g−1. Raman and ESR analysis reveal that the B tend to occupy the C vacancies in C3N5, which effectively improve the charge transfer capability and optimize band structure of B-C3N5. The B sites display perfect performance for N2 adsorption and activation to generate NH3. The intermediates of NRR process are identified by in-situ DRIFTS and a reaction mechanism is proposed to reveal the role of the B − O − H during the N2 adsorption, activation, and reduction process. g-C B-doping Photocatalytic N N Cai, Wei verfasserin aut Zhang, Zhicheng verfasserin aut Xie, Huifang verfasserin aut Zhong, Qin verfasserin aut Qu, Hongxia verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 435 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:435 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 435 045F 660.05
allfieldsGer	10.1016/j.cej.2022.135017 doi (DE-627)ELV007483805 (ELSEVIER)S1385-8947(22)00523-X DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Li, Kang verfasserin aut Boron doped C 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Compared to g-C3N4, g-C3N5 can harvest more visible light and prolong the lifetime of photogenerated carriers, and exhibited a more excellent NH3 yield under visible light. A new catalyst boron doping g-C3N5 (B-C3N5) was prepared by a simple one-step calcination for photocatalytic nitrogen fixation. B-C3N5 achieved the NH3 yield up to 421.18 μmol h−1 g−1. Raman and ESR analysis reveal that the B tend to occupy the C vacancies in C3N5, which effectively improve the charge transfer capability and optimize band structure of B-C3N5. The B sites display perfect performance for N2 adsorption and activation to generate NH3. The intermediates of NRR process are identified by in-situ DRIFTS and a reaction mechanism is proposed to reveal the role of the B − O − H during the N2 adsorption, activation, and reduction process. g-C B-doping Photocatalytic N N Cai, Wei verfasserin aut Zhang, Zhicheng verfasserin aut Xie, Huifang verfasserin aut Zhong, Qin verfasserin aut Qu, Hongxia verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 435 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:435 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 435 045F 660.05
allfieldsSound	10.1016/j.cej.2022.135017 doi (DE-627)ELV007483805 (ELSEVIER)S1385-8947(22)00523-X DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Li, Kang verfasserin aut Boron doped C 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Compared to g-C3N4, g-C3N5 can harvest more visible light and prolong the lifetime of photogenerated carriers, and exhibited a more excellent NH3 yield under visible light. A new catalyst boron doping g-C3N5 (B-C3N5) was prepared by a simple one-step calcination for photocatalytic nitrogen fixation. B-C3N5 achieved the NH3 yield up to 421.18 μmol h−1 g−1. Raman and ESR analysis reveal that the B tend to occupy the C vacancies in C3N5, which effectively improve the charge transfer capability and optimize band structure of B-C3N5. The B sites display perfect performance for N2 adsorption and activation to generate NH3. The intermediates of NRR process are identified by in-situ DRIFTS and a reaction mechanism is proposed to reveal the role of the B − O − H during the N2 adsorption, activation, and reduction process. g-C B-doping Photocatalytic N N Cai, Wei verfasserin aut Zhang, Zhicheng verfasserin aut Xie, Huifang verfasserin aut Zhong, Qin verfasserin aut Qu, Hongxia verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 435 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:435 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 435 045F 660.05
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authorswithroles_txt_mv	Li, Kang @@aut@@ Cai, Wei @@aut@@ Zhang, Zhicheng @@aut@@ Xie, Huifang @@aut@@ Zhong, Qin @@aut@@ Qu, Hongxia @@aut@@
publishDateDaySort_date	2022-01-01T00:00:00Z
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id	ELV007483805
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author	Li, Kang
spellingShingle	Li, Kang ddc 660.05 ddc 660 bkl 58.10 misc g-C misc B-doping misc Photocatalytic misc N Boron doped C
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title	Boron doped C
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title_full	Boron doped C
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title_sort	boron doped c
title_auth	Boron doped C
abstract	Compared to g-C3N4, g-C3N5 can harvest more visible light and prolong the lifetime of photogenerated carriers, and exhibited a more excellent NH3 yield under visible light. A new catalyst boron doping g-C3N5 (B-C3N5) was prepared by a simple one-step calcination for photocatalytic nitrogen fixation. B-C3N5 achieved the NH3 yield up to 421.18 μmol h−1 g−1. Raman and ESR analysis reveal that the B tend to occupy the C vacancies in C3N5, which effectively improve the charge transfer capability and optimize band structure of B-C3N5. The B sites display perfect performance for N2 adsorption and activation to generate NH3. The intermediates of NRR process are identified by in-situ DRIFTS and a reaction mechanism is proposed to reveal the role of the B − O − H during the N2 adsorption, activation, and reduction process.
abstractGer	Compared to g-C3N4, g-C3N5 can harvest more visible light and prolong the lifetime of photogenerated carriers, and exhibited a more excellent NH3 yield under visible light. A new catalyst boron doping g-C3N5 (B-C3N5) was prepared by a simple one-step calcination for photocatalytic nitrogen fixation. B-C3N5 achieved the NH3 yield up to 421.18 μmol h−1 g−1. Raman and ESR analysis reveal that the B tend to occupy the C vacancies in C3N5, which effectively improve the charge transfer capability and optimize band structure of B-C3N5. The B sites display perfect performance for N2 adsorption and activation to generate NH3. The intermediates of NRR process are identified by in-situ DRIFTS and a reaction mechanism is proposed to reveal the role of the B − O − H during the N2 adsorption, activation, and reduction process.
abstract_unstemmed	Compared to g-C3N4, g-C3N5 can harvest more visible light and prolong the lifetime of photogenerated carriers, and exhibited a more excellent NH3 yield under visible light. A new catalyst boron doping g-C3N5 (B-C3N5) was prepared by a simple one-step calcination for photocatalytic nitrogen fixation. B-C3N5 achieved the NH3 yield up to 421.18 μmol h−1 g−1. Raman and ESR analysis reveal that the B tend to occupy the C vacancies in C3N5, which effectively improve the charge transfer capability and optimize band structure of B-C3N5. The B sites display perfect performance for N2 adsorption and activation to generate NH3. The intermediates of NRR process are identified by in-situ DRIFTS and a reaction mechanism is proposed to reveal the role of the B − O − H during the N2 adsorption, activation, and reduction process.
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title_short	Boron doped C
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author2	Cai, Wei Zhang, Zhicheng Xie, Huifang Zhong, Qin Qu, Hongxia
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doi_str	10.1016/j.cej.2022.135017
up_date	2024-07-07T00:53:51.465Z
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Boron doped C

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