Preparation of size-controlled all-lignin based carbon nanospheres and their electrochemical performance in supercapacitor

Lignin, as the second most abundant biomass material in nature, is regarded as an ideal carbon precursor due to the presence of a larger amount of aromatic ring structural unit. Carbon nanospheres, as one of the vital members of carbon materials, are promising advanced materials for various areas. H...
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Autor*in:	Wang, Hang [verfasserIn] Xiong, Fuquan [verfasserIn] Yang, Jiamei [verfasserIn] Ma, Bole [verfasserIn] Qing, Yan [verfasserIn] Chu, Fuxiang [verfasserIn] Wu, Yiqiang [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2022

Schlagwörter:	Lignin Self-assembly Carbon nanospheres Supercapacitor

Übergeordnetes Werk:	Enthalten in: Industrial crops and products - New York, NY [u.a.] : Elsevier, 1992, 179
Übergeordnetes Werk:	volume:179

DOI / URN:	10.1016/j.indcrop.2022.114689

Katalog-ID:	ELV007527683

Internformat


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520			\|a Lignin, as the second most abundant biomass material in nature, is regarded as an ideal carbon precursor due to the presence of a larger amount of aromatic ring structural unit. Carbon nanospheres, as one of the vital members of carbon materials, are promising advanced materials for various areas. However, lignin-based carbon spheres suffered a complex fabrication process, high crosslinking between spheres, and non-adjustable micron size. Here, all-lignin based carbon nanospheres (LCNS) with tunable size and microstructure were prepared via self-assembly, stabilization treatment, and carbonization. Subsequently, their applications in supercapacitor electrode material were investigated. The results showed that the monodispersed, ordered, and regular carbon nanospheres could be constructed. The size of LCNS could be tuned ranging from 256 to 416 nm via changing the initial concentration of lignin between 0.5 and 2 mg mL−1. The as-prepared LCNS provided a specific surface area between 652 and 736 m2 g−1 through adjusting the size and microstructure. When the LCNS was assembled into the electrochemical capacitor, the LCNS electrode materials exhibited a high specific capacitance of 147 F g−1. Additionally, the LCNS-based symmetrical capacitor showed an ultralow characteristic relaxation time (0.86 s) and long cycle stability for 10,000 cycles. The capacitance properties could be regulated via reconciling the size of nanospheres and microstructure induced by carbonization temperature. The governable capacitance performance indicates that the as-prepared LCNS should be a promising candidate material for energy storage.
650		4	\|a Lignin
650		4	\|a Self-assembly
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700	1		\|a Xiong, Fuquan \|e verfasserin \|4 aut
700	1		\|a Yang, Jiamei \|e verfasserin \|4 aut
700	1		\|a Ma, Bole \|e verfasserin \|4 aut
700	1		\|a Qing, Yan \|e verfasserin \|4 aut
700	1		\|a Chu, Fuxiang \|e verfasserin \|4 aut
700	1		\|a Wu, Yiqiang \|e verfasserin \|4 aut
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Indexfelder

author_variant	h w hw f x fx j y jy b m bm y q yq f c fc y w yw
matchkey_str	article:1872633X:2022----::rprtooszcnrlealinnaecronnshrsnterlcrceia
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publishDate	2022
allfields	10.1016/j.indcrop.2022.114689 doi (DE-627)ELV007527683 (ELSEVIER)S0926-6690(22)00172-8 DE-627 ger DE-627 rda eng 630 640 DE-600 48.30 bkl Wang, Hang verfasserin aut Preparation of size-controlled all-lignin based carbon nanospheres and their electrochemical performance in supercapacitor 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Lignin, as the second most abundant biomass material in nature, is regarded as an ideal carbon precursor due to the presence of a larger amount of aromatic ring structural unit. Carbon nanospheres, as one of the vital members of carbon materials, are promising advanced materials for various areas. However, lignin-based carbon spheres suffered a complex fabrication process, high crosslinking between spheres, and non-adjustable micron size. Here, all-lignin based carbon nanospheres (LCNS) with tunable size and microstructure were prepared via self-assembly, stabilization treatment, and carbonization. Subsequently, their applications in supercapacitor electrode material were investigated. The results showed that the monodispersed, ordered, and regular carbon nanospheres could be constructed. The size of LCNS could be tuned ranging from 256 to 416 nm via changing the initial concentration of lignin between 0.5 and 2 mg mL−1. The as-prepared LCNS provided a specific surface area between 652 and 736 m2 g−1 through adjusting the size and microstructure. When the LCNS was assembled into the electrochemical capacitor, the LCNS electrode materials exhibited a high specific capacitance of 147 F g−1. Additionally, the LCNS-based symmetrical capacitor showed an ultralow characteristic relaxation time (0.86 s) and long cycle stability for 10,000 cycles. The capacitance properties could be regulated via reconciling the size of nanospheres and microstructure induced by carbonization temperature. The governable capacitance performance indicates that the as-prepared LCNS should be a promising candidate material for energy storage. Lignin Self-assembly Carbon nanospheres Supercapacitor Xiong, Fuquan verfasserin aut Yang, Jiamei verfasserin aut Ma, Bole verfasserin aut Qing, Yan verfasserin aut Chu, Fuxiang verfasserin aut Wu, Yiqiang verfasserin aut Enthalten in Industrial crops and products New York, NY [u.a.] : Elsevier, 1992 179 Online-Ressource (DE-627)300894678 (DE-600)1483245-8 (DE-576)259270792 1872-633X nnns volume:179 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 48.30 Natürliche Ressourcen Land- und Forstwirtschaft AR 179
spelling	10.1016/j.indcrop.2022.114689 doi (DE-627)ELV007527683 (ELSEVIER)S0926-6690(22)00172-8 DE-627 ger DE-627 rda eng 630 640 DE-600 48.30 bkl Wang, Hang verfasserin aut Preparation of size-controlled all-lignin based carbon nanospheres and their electrochemical performance in supercapacitor 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Lignin, as the second most abundant biomass material in nature, is regarded as an ideal carbon precursor due to the presence of a larger amount of aromatic ring structural unit. Carbon nanospheres, as one of the vital members of carbon materials, are promising advanced materials for various areas. However, lignin-based carbon spheres suffered a complex fabrication process, high crosslinking between spheres, and non-adjustable micron size. Here, all-lignin based carbon nanospheres (LCNS) with tunable size and microstructure were prepared via self-assembly, stabilization treatment, and carbonization. Subsequently, their applications in supercapacitor electrode material were investigated. The results showed that the monodispersed, ordered, and regular carbon nanospheres could be constructed. The size of LCNS could be tuned ranging from 256 to 416 nm via changing the initial concentration of lignin between 0.5 and 2 mg mL−1. The as-prepared LCNS provided a specific surface area between 652 and 736 m2 g−1 through adjusting the size and microstructure. When the LCNS was assembled into the electrochemical capacitor, the LCNS electrode materials exhibited a high specific capacitance of 147 F g−1. Additionally, the LCNS-based symmetrical capacitor showed an ultralow characteristic relaxation time (0.86 s) and long cycle stability for 10,000 cycles. The capacitance properties could be regulated via reconciling the size of nanospheres and microstructure induced by carbonization temperature. The governable capacitance performance indicates that the as-prepared LCNS should be a promising candidate material for energy storage. Lignin Self-assembly Carbon nanospheres Supercapacitor Xiong, Fuquan verfasserin aut Yang, Jiamei verfasserin aut Ma, Bole verfasserin aut Qing, Yan verfasserin aut Chu, Fuxiang verfasserin aut Wu, Yiqiang verfasserin aut Enthalten in Industrial crops and products New York, NY [u.a.] : Elsevier, 1992 179 Online-Ressource (DE-627)300894678 (DE-600)1483245-8 (DE-576)259270792 1872-633X nnns volume:179 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 48.30 Natürliche Ressourcen Land- und Forstwirtschaft AR 179
allfields_unstemmed	10.1016/j.indcrop.2022.114689 doi (DE-627)ELV007527683 (ELSEVIER)S0926-6690(22)00172-8 DE-627 ger DE-627 rda eng 630 640 DE-600 48.30 bkl Wang, Hang verfasserin aut Preparation of size-controlled all-lignin based carbon nanospheres and their electrochemical performance in supercapacitor 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Lignin, as the second most abundant biomass material in nature, is regarded as an ideal carbon precursor due to the presence of a larger amount of aromatic ring structural unit. Carbon nanospheres, as one of the vital members of carbon materials, are promising advanced materials for various areas. However, lignin-based carbon spheres suffered a complex fabrication process, high crosslinking between spheres, and non-adjustable micron size. Here, all-lignin based carbon nanospheres (LCNS) with tunable size and microstructure were prepared via self-assembly, stabilization treatment, and carbonization. Subsequently, their applications in supercapacitor electrode material were investigated. The results showed that the monodispersed, ordered, and regular carbon nanospheres could be constructed. The size of LCNS could be tuned ranging from 256 to 416 nm via changing the initial concentration of lignin between 0.5 and 2 mg mL−1. The as-prepared LCNS provided a specific surface area between 652 and 736 m2 g−1 through adjusting the size and microstructure. When the LCNS was assembled into the electrochemical capacitor, the LCNS electrode materials exhibited a high specific capacitance of 147 F g−1. Additionally, the LCNS-based symmetrical capacitor showed an ultralow characteristic relaxation time (0.86 s) and long cycle stability for 10,000 cycles. The capacitance properties could be regulated via reconciling the size of nanospheres and microstructure induced by carbonization temperature. The governable capacitance performance indicates that the as-prepared LCNS should be a promising candidate material for energy storage. Lignin Self-assembly Carbon nanospheres Supercapacitor Xiong, Fuquan verfasserin aut Yang, Jiamei verfasserin aut Ma, Bole verfasserin aut Qing, Yan verfasserin aut Chu, Fuxiang verfasserin aut Wu, Yiqiang verfasserin aut Enthalten in Industrial crops and products New York, NY [u.a.] : Elsevier, 1992 179 Online-Ressource (DE-627)300894678 (DE-600)1483245-8 (DE-576)259270792 1872-633X nnns volume:179 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 48.30 Natürliche Ressourcen Land- und Forstwirtschaft AR 179
allfieldsGer	10.1016/j.indcrop.2022.114689 doi (DE-627)ELV007527683 (ELSEVIER)S0926-6690(22)00172-8 DE-627 ger DE-627 rda eng 630 640 DE-600 48.30 bkl Wang, Hang verfasserin aut Preparation of size-controlled all-lignin based carbon nanospheres and their electrochemical performance in supercapacitor 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Lignin, as the second most abundant biomass material in nature, is regarded as an ideal carbon precursor due to the presence of a larger amount of aromatic ring structural unit. Carbon nanospheres, as one of the vital members of carbon materials, are promising advanced materials for various areas. However, lignin-based carbon spheres suffered a complex fabrication process, high crosslinking between spheres, and non-adjustable micron size. Here, all-lignin based carbon nanospheres (LCNS) with tunable size and microstructure were prepared via self-assembly, stabilization treatment, and carbonization. Subsequently, their applications in supercapacitor electrode material were investigated. The results showed that the monodispersed, ordered, and regular carbon nanospheres could be constructed. The size of LCNS could be tuned ranging from 256 to 416 nm via changing the initial concentration of lignin between 0.5 and 2 mg mL−1. The as-prepared LCNS provided a specific surface area between 652 and 736 m2 g−1 through adjusting the size and microstructure. When the LCNS was assembled into the electrochemical capacitor, the LCNS electrode materials exhibited a high specific capacitance of 147 F g−1. Additionally, the LCNS-based symmetrical capacitor showed an ultralow characteristic relaxation time (0.86 s) and long cycle stability for 10,000 cycles. The capacitance properties could be regulated via reconciling the size of nanospheres and microstructure induced by carbonization temperature. The governable capacitance performance indicates that the as-prepared LCNS should be a promising candidate material for energy storage. Lignin Self-assembly Carbon nanospheres Supercapacitor Xiong, Fuquan verfasserin aut Yang, Jiamei verfasserin aut Ma, Bole verfasserin aut Qing, Yan verfasserin aut Chu, Fuxiang verfasserin aut Wu, Yiqiang verfasserin aut Enthalten in Industrial crops and products New York, NY [u.a.] : Elsevier, 1992 179 Online-Ressource (DE-627)300894678 (DE-600)1483245-8 (DE-576)259270792 1872-633X nnns volume:179 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 48.30 Natürliche Ressourcen Land- und Forstwirtschaft AR 179
allfieldsSound	10.1016/j.indcrop.2022.114689 doi (DE-627)ELV007527683 (ELSEVIER)S0926-6690(22)00172-8 DE-627 ger DE-627 rda eng 630 640 DE-600 48.30 bkl Wang, Hang verfasserin aut Preparation of size-controlled all-lignin based carbon nanospheres and their electrochemical performance in supercapacitor 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Lignin, as the second most abundant biomass material in nature, is regarded as an ideal carbon precursor due to the presence of a larger amount of aromatic ring structural unit. Carbon nanospheres, as one of the vital members of carbon materials, are promising advanced materials for various areas. However, lignin-based carbon spheres suffered a complex fabrication process, high crosslinking between spheres, and non-adjustable micron size. Here, all-lignin based carbon nanospheres (LCNS) with tunable size and microstructure were prepared via self-assembly, stabilization treatment, and carbonization. Subsequently, their applications in supercapacitor electrode material were investigated. The results showed that the monodispersed, ordered, and regular carbon nanospheres could be constructed. The size of LCNS could be tuned ranging from 256 to 416 nm via changing the initial concentration of lignin between 0.5 and 2 mg mL−1. The as-prepared LCNS provided a specific surface area between 652 and 736 m2 g−1 through adjusting the size and microstructure. When the LCNS was assembled into the electrochemical capacitor, the LCNS electrode materials exhibited a high specific capacitance of 147 F g−1. Additionally, the LCNS-based symmetrical capacitor showed an ultralow characteristic relaxation time (0.86 s) and long cycle stability for 10,000 cycles. The capacitance properties could be regulated via reconciling the size of nanospheres and microstructure induced by carbonization temperature. The governable capacitance performance indicates that the as-prepared LCNS should be a promising candidate material for energy storage. Lignin Self-assembly Carbon nanospheres Supercapacitor Xiong, Fuquan verfasserin aut Yang, Jiamei verfasserin aut Ma, Bole verfasserin aut Qing, Yan verfasserin aut Chu, Fuxiang verfasserin aut Wu, Yiqiang verfasserin aut Enthalten in Industrial crops and products New York, NY [u.a.] : Elsevier, 1992 179 Online-Ressource (DE-627)300894678 (DE-600)1483245-8 (DE-576)259270792 1872-633X nnns volume:179 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 48.30 Natürliche Ressourcen Land- und Forstwirtschaft AR 179
language	English
source	Enthalten in Industrial crops and products 179 volume:179
sourceStr	Enthalten in Industrial crops and products 179 volume:179
format_phy_str_mv	Article
bklname	Natürliche Ressourcen
institution	findex.gbv.de
topic_facet	Lignin Self-assembly Carbon nanospheres Supercapacitor
dewey-raw	630
isfreeaccess_bool	false
container_title	Industrial crops and products
authorswithroles_txt_mv	Wang, Hang @@aut@@ Xiong, Fuquan @@aut@@ Yang, Jiamei @@aut@@ Ma, Bole @@aut@@ Qing, Yan @@aut@@ Chu, Fuxiang @@aut@@ Wu, Yiqiang @@aut@@
publishDateDaySort_date	2022-01-01T00:00:00Z
hierarchy_top_id	300894678
dewey-sort	3630
id	ELV007527683
language_de	englisch
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author	Wang, Hang
spellingShingle	Wang, Hang ddc 630 bkl 48.30 misc Lignin misc Self-assembly misc Carbon nanospheres misc Supercapacitor Preparation of size-controlled all-lignin based carbon nanospheres and their electrochemical performance in supercapacitor
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topic_title	630 640 DE-600 48.30 bkl Preparation of size-controlled all-lignin based carbon nanospheres and their electrochemical performance in supercapacitor Lignin Self-assembly Carbon nanospheres Supercapacitor
topic	ddc 630 bkl 48.30 misc Lignin misc Self-assembly misc Carbon nanospheres misc Supercapacitor
topic_unstemmed	ddc 630 bkl 48.30 misc Lignin misc Self-assembly misc Carbon nanospheres misc Supercapacitor
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title	Preparation of size-controlled all-lignin based carbon nanospheres and their electrochemical performance in supercapacitor
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title_full	Preparation of size-controlled all-lignin based carbon nanospheres and their electrochemical performance in supercapacitor
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author_browse	Wang, Hang Xiong, Fuquan Yang, Jiamei Ma, Bole Qing, Yan Chu, Fuxiang Wu, Yiqiang
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author-letter	Wang, Hang
doi_str_mv	10.1016/j.indcrop.2022.114689
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title_sort	preparation of size-controlled all-lignin based carbon nanospheres and their electrochemical performance in supercapacitor
title_auth	Preparation of size-controlled all-lignin based carbon nanospheres and their electrochemical performance in supercapacitor
abstract	Lignin, as the second most abundant biomass material in nature, is regarded as an ideal carbon precursor due to the presence of a larger amount of aromatic ring structural unit. Carbon nanospheres, as one of the vital members of carbon materials, are promising advanced materials for various areas. However, lignin-based carbon spheres suffered a complex fabrication process, high crosslinking between spheres, and non-adjustable micron size. Here, all-lignin based carbon nanospheres (LCNS) with tunable size and microstructure were prepared via self-assembly, stabilization treatment, and carbonization. Subsequently, their applications in supercapacitor electrode material were investigated. The results showed that the monodispersed, ordered, and regular carbon nanospheres could be constructed. The size of LCNS could be tuned ranging from 256 to 416 nm via changing the initial concentration of lignin between 0.5 and 2 mg mL−1. The as-prepared LCNS provided a specific surface area between 652 and 736 m2 g−1 through adjusting the size and microstructure. When the LCNS was assembled into the electrochemical capacitor, the LCNS electrode materials exhibited a high specific capacitance of 147 F g−1. Additionally, the LCNS-based symmetrical capacitor showed an ultralow characteristic relaxation time (0.86 s) and long cycle stability for 10,000 cycles. The capacitance properties could be regulated via reconciling the size of nanospheres and microstructure induced by carbonization temperature. The governable capacitance performance indicates that the as-prepared LCNS should be a promising candidate material for energy storage.
abstractGer	Lignin, as the second most abundant biomass material in nature, is regarded as an ideal carbon precursor due to the presence of a larger amount of aromatic ring structural unit. Carbon nanospheres, as one of the vital members of carbon materials, are promising advanced materials for various areas. However, lignin-based carbon spheres suffered a complex fabrication process, high crosslinking between spheres, and non-adjustable micron size. Here, all-lignin based carbon nanospheres (LCNS) with tunable size and microstructure were prepared via self-assembly, stabilization treatment, and carbonization. Subsequently, their applications in supercapacitor electrode material were investigated. The results showed that the monodispersed, ordered, and regular carbon nanospheres could be constructed. The size of LCNS could be tuned ranging from 256 to 416 nm via changing the initial concentration of lignin between 0.5 and 2 mg mL−1. The as-prepared LCNS provided a specific surface area between 652 and 736 m2 g−1 through adjusting the size and microstructure. When the LCNS was assembled into the electrochemical capacitor, the LCNS electrode materials exhibited a high specific capacitance of 147 F g−1. Additionally, the LCNS-based symmetrical capacitor showed an ultralow characteristic relaxation time (0.86 s) and long cycle stability for 10,000 cycles. The capacitance properties could be regulated via reconciling the size of nanospheres and microstructure induced by carbonization temperature. The governable capacitance performance indicates that the as-prepared LCNS should be a promising candidate material for energy storage.
abstract_unstemmed	Lignin, as the second most abundant biomass material in nature, is regarded as an ideal carbon precursor due to the presence of a larger amount of aromatic ring structural unit. Carbon nanospheres, as one of the vital members of carbon materials, are promising advanced materials for various areas. However, lignin-based carbon spheres suffered a complex fabrication process, high crosslinking between spheres, and non-adjustable micron size. Here, all-lignin based carbon nanospheres (LCNS) with tunable size and microstructure were prepared via self-assembly, stabilization treatment, and carbonization. Subsequently, their applications in supercapacitor electrode material were investigated. The results showed that the monodispersed, ordered, and regular carbon nanospheres could be constructed. The size of LCNS could be tuned ranging from 256 to 416 nm via changing the initial concentration of lignin between 0.5 and 2 mg mL−1. The as-prepared LCNS provided a specific surface area between 652 and 736 m2 g−1 through adjusting the size and microstructure. When the LCNS was assembled into the electrochemical capacitor, the LCNS electrode materials exhibited a high specific capacitance of 147 F g−1. Additionally, the LCNS-based symmetrical capacitor showed an ultralow characteristic relaxation time (0.86 s) and long cycle stability for 10,000 cycles. The capacitance properties could be regulated via reconciling the size of nanospheres and microstructure induced by carbonization temperature. The governable capacitance performance indicates that the as-prepared LCNS should be a promising candidate material for energy storage.
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title_short	Preparation of size-controlled all-lignin based carbon nanospheres and their electrochemical performance in supercapacitor
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author2	Xiong, Fuquan Yang, Jiamei Ma, Bole Qing, Yan Chu, Fuxiang Wu, Yiqiang
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doi_str	10.1016/j.indcrop.2022.114689
up_date	2024-07-06T16:34:20.591Z
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Preparation of size-controlled all-lignin based carbon nanospheres and their electrochemical performance in supercapacitor

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