Electrochemical Zintl Cluster Bi

Bismuth, a promising attribute for sodium-ion batteries, which have been attracting significant attention owing to their advantages of high volumetric capacity and suitable operating potential. However, most traditional Bi-based materials are suffered from pulverization and fracture of the electrode...
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Gespeichert in:

Autor*in:	Li, Jiayang [verfasserIn] Fang, Susu [verfasserIn] Xu, Laiqiang [verfasserIn] Wang, Anni [verfasserIn] Zou, Kangyu [verfasserIn] Di, Andi [verfasserIn] Li, Fengrong [verfasserIn] Deng, Wentao [verfasserIn] Zou, Guoqiang [verfasserIn] Hou, Hongshuai [verfasserIn] Ji, Xiaobo [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2022

Schlagwörter:	Sodium-ion batteries Bi/GO composite Electrochemical method Anode materials Zintl clusters

Übergeordnetes Werk:	Enthalten in: Electrochimica acta - New York, NY [u.a.] : Elsevier, 1959, 413
Übergeordnetes Werk:	volume:413

DOI / URN:	10.1016/j.electacta.2022.140174

Katalog-ID:	ELV007610548

Internformat


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520			\|a Bismuth, a promising attribute for sodium-ion batteries, which have been attracting significant attention owing to their advantages of high volumetric capacity and suitable operating potential. However, most traditional Bi-based materials are suffered from pulverization and fracture of the electrodes caused by dramatic volume variation, consequently diminishing the cycle stability. Herein, in this work, bismuth embedded within graphene oxide matrices have been obtained by utilizing a novel and efficient electrochemical method. Through the strong reducing properties of Zintl clusters Bi2 2−, GO is partially reduced to generate reduced graphene oxide with better electrical conductivity. Simultaneously, Bi is strongly loaded on the GO through Bi-O-C bonding, which can form Bi2O2 2+ with excellent ionic conductivity. Moreover, the volume expansion of Bi during sodiation can be effectively buffered in the GO matrices. As a result, this Bi/GO composite exhibits excellent electrochemical performances in sodium-ion batteries (SIBs), including a high specific capacity of 258 mAh g−1 at 10 A g−1 and an excellent cycle stability with high retained capacity of 315 mAh g−1 after 500 cycles at 2 A g−1. This work paves the way to prepare designated promising electrode materials for high-performance SIBs, and thoroughly understands mechanism of electrochemical methods for preparing materials.
650		4	\|a Sodium-ion batteries
650		4	\|a Bi/GO composite
650		4	\|a Electrochemical method
650		4	\|a Anode materials
650		4	\|a Zintl clusters
700	1		\|a Fang, Susu \|e verfasserin \|4 aut
700	1		\|a Xu, Laiqiang \|e verfasserin \|4 aut
700	1		\|a Wang, Anni \|e verfasserin \|4 aut
700	1		\|a Zou, Kangyu \|e verfasserin \|4 aut
700	1		\|a Di, Andi \|e verfasserin \|0 (orcid)0000-0003-4527-2504 \|4 aut
700	1		\|a Li, Fengrong \|e verfasserin \|4 aut
700	1		\|a Deng, Wentao \|e verfasserin \|4 aut
700	1		\|a Zou, Guoqiang \|e verfasserin \|4 aut
700	1		\|a Hou, Hongshuai \|e verfasserin \|4 aut
700	1		\|a Ji, Xiaobo \|e verfasserin \|4 aut
773	0	8	\|i Enthalten in \|t Electrochimica acta \|d New York, NY [u.a.] : Elsevier, 1959 \|g 413 \|h Online-Ressource \|w (DE-627)300897561 \|w (DE-600)1483548-4 \|w (DE-576)094752451 \|x 1873-3859 \|7 nnns
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912			\|a GBV_ILN_2011
912			\|a GBV_ILN_2014
912			\|a GBV_ILN_2015
912			\|a GBV_ILN_2020
912			\|a GBV_ILN_2021
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912			\|a GBV_ILN_2027
912			\|a GBV_ILN_2034
912			\|a GBV_ILN_2038
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912			\|a GBV_ILN_2048
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912			\|a GBV_ILN_4333
912			\|a GBV_ILN_4334
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936	b	k	\|a 35.00 \|j Chemie: Allgemeines
951			\|a AR
952			\|d 413

Indexfelder

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matchkey_str	article:18733859:2022----::lcrceiaznl
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bklnumber	35.00
publishDate	2022
allfields	10.1016/j.electacta.2022.140174 doi (DE-627)ELV007610548 (ELSEVIER)S0013-4686(22)00346-2 DE-627 ger DE-627 rda eng 540 DE-600 35.00 bkl Li, Jiayang verfasserin aut Electrochemical Zintl Cluster Bi 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Bismuth, a promising attribute for sodium-ion batteries, which have been attracting significant attention owing to their advantages of high volumetric capacity and suitable operating potential. However, most traditional Bi-based materials are suffered from pulverization and fracture of the electrodes caused by dramatic volume variation, consequently diminishing the cycle stability. Herein, in this work, bismuth embedded within graphene oxide matrices have been obtained by utilizing a novel and efficient electrochemical method. Through the strong reducing properties of Zintl clusters Bi2 2−, GO is partially reduced to generate reduced graphene oxide with better electrical conductivity. Simultaneously, Bi is strongly loaded on the GO through Bi-O-C bonding, which can form Bi2O2 2+ with excellent ionic conductivity. Moreover, the volume expansion of Bi during sodiation can be effectively buffered in the GO matrices. As a result, this Bi/GO composite exhibits excellent electrochemical performances in sodium-ion batteries (SIBs), including a high specific capacity of 258 mAh g−1 at 10 A g−1 and an excellent cycle stability with high retained capacity of 315 mAh g−1 after 500 cycles at 2 A g−1. This work paves the way to prepare designated promising electrode materials for high-performance SIBs, and thoroughly understands mechanism of electrochemical methods for preparing materials. Sodium-ion batteries Bi/GO composite Electrochemical method Anode materials Zintl clusters Fang, Susu verfasserin aut Xu, Laiqiang verfasserin aut Wang, Anni verfasserin aut Zou, Kangyu verfasserin aut Di, Andi verfasserin (orcid)0000-0003-4527-2504 aut Li, Fengrong verfasserin aut Deng, Wentao verfasserin aut Zou, Guoqiang verfasserin aut Hou, Hongshuai verfasserin aut Ji, Xiaobo verfasserin aut Enthalten in Electrochimica acta New York, NY [u.a.] : Elsevier, 1959 413 Online-Ressource (DE-627)300897561 (DE-600)1483548-4 (DE-576)094752451 1873-3859 nnns volume:413 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.00 Chemie: Allgemeines AR 413
spelling	10.1016/j.electacta.2022.140174 doi (DE-627)ELV007610548 (ELSEVIER)S0013-4686(22)00346-2 DE-627 ger DE-627 rda eng 540 DE-600 35.00 bkl Li, Jiayang verfasserin aut Electrochemical Zintl Cluster Bi 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Bismuth, a promising attribute for sodium-ion batteries, which have been attracting significant attention owing to their advantages of high volumetric capacity and suitable operating potential. However, most traditional Bi-based materials are suffered from pulverization and fracture of the electrodes caused by dramatic volume variation, consequently diminishing the cycle stability. Herein, in this work, bismuth embedded within graphene oxide matrices have been obtained by utilizing a novel and efficient electrochemical method. Through the strong reducing properties of Zintl clusters Bi2 2−, GO is partially reduced to generate reduced graphene oxide with better electrical conductivity. Simultaneously, Bi is strongly loaded on the GO through Bi-O-C bonding, which can form Bi2O2 2+ with excellent ionic conductivity. Moreover, the volume expansion of Bi during sodiation can be effectively buffered in the GO matrices. As a result, this Bi/GO composite exhibits excellent electrochemical performances in sodium-ion batteries (SIBs), including a high specific capacity of 258 mAh g−1 at 10 A g−1 and an excellent cycle stability with high retained capacity of 315 mAh g−1 after 500 cycles at 2 A g−1. This work paves the way to prepare designated promising electrode materials for high-performance SIBs, and thoroughly understands mechanism of electrochemical methods for preparing materials. Sodium-ion batteries Bi/GO composite Electrochemical method Anode materials Zintl clusters Fang, Susu verfasserin aut Xu, Laiqiang verfasserin aut Wang, Anni verfasserin aut Zou, Kangyu verfasserin aut Di, Andi verfasserin (orcid)0000-0003-4527-2504 aut Li, Fengrong verfasserin aut Deng, Wentao verfasserin aut Zou, Guoqiang verfasserin aut Hou, Hongshuai verfasserin aut Ji, Xiaobo verfasserin aut Enthalten in Electrochimica acta New York, NY [u.a.] : Elsevier, 1959 413 Online-Ressource (DE-627)300897561 (DE-600)1483548-4 (DE-576)094752451 1873-3859 nnns volume:413 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.00 Chemie: Allgemeines AR 413
allfields_unstemmed	10.1016/j.electacta.2022.140174 doi (DE-627)ELV007610548 (ELSEVIER)S0013-4686(22)00346-2 DE-627 ger DE-627 rda eng 540 DE-600 35.00 bkl Li, Jiayang verfasserin aut Electrochemical Zintl Cluster Bi 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Bismuth, a promising attribute for sodium-ion batteries, which have been attracting significant attention owing to their advantages of high volumetric capacity and suitable operating potential. However, most traditional Bi-based materials are suffered from pulverization and fracture of the electrodes caused by dramatic volume variation, consequently diminishing the cycle stability. Herein, in this work, bismuth embedded within graphene oxide matrices have been obtained by utilizing a novel and efficient electrochemical method. Through the strong reducing properties of Zintl clusters Bi2 2−, GO is partially reduced to generate reduced graphene oxide with better electrical conductivity. Simultaneously, Bi is strongly loaded on the GO through Bi-O-C bonding, which can form Bi2O2 2+ with excellent ionic conductivity. Moreover, the volume expansion of Bi during sodiation can be effectively buffered in the GO matrices. As a result, this Bi/GO composite exhibits excellent electrochemical performances in sodium-ion batteries (SIBs), including a high specific capacity of 258 mAh g−1 at 10 A g−1 and an excellent cycle stability with high retained capacity of 315 mAh g−1 after 500 cycles at 2 A g−1. This work paves the way to prepare designated promising electrode materials for high-performance SIBs, and thoroughly understands mechanism of electrochemical methods for preparing materials. Sodium-ion batteries Bi/GO composite Electrochemical method Anode materials Zintl clusters Fang, Susu verfasserin aut Xu, Laiqiang verfasserin aut Wang, Anni verfasserin aut Zou, Kangyu verfasserin aut Di, Andi verfasserin (orcid)0000-0003-4527-2504 aut Li, Fengrong verfasserin aut Deng, Wentao verfasserin aut Zou, Guoqiang verfasserin aut Hou, Hongshuai verfasserin aut Ji, Xiaobo verfasserin aut Enthalten in Electrochimica acta New York, NY [u.a.] : Elsevier, 1959 413 Online-Ressource (DE-627)300897561 (DE-600)1483548-4 (DE-576)094752451 1873-3859 nnns volume:413 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.00 Chemie: Allgemeines AR 413
allfieldsGer	10.1016/j.electacta.2022.140174 doi (DE-627)ELV007610548 (ELSEVIER)S0013-4686(22)00346-2 DE-627 ger DE-627 rda eng 540 DE-600 35.00 bkl Li, Jiayang verfasserin aut Electrochemical Zintl Cluster Bi 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Bismuth, a promising attribute for sodium-ion batteries, which have been attracting significant attention owing to their advantages of high volumetric capacity and suitable operating potential. However, most traditional Bi-based materials are suffered from pulverization and fracture of the electrodes caused by dramatic volume variation, consequently diminishing the cycle stability. Herein, in this work, bismuth embedded within graphene oxide matrices have been obtained by utilizing a novel and efficient electrochemical method. Through the strong reducing properties of Zintl clusters Bi2 2−, GO is partially reduced to generate reduced graphene oxide with better electrical conductivity. Simultaneously, Bi is strongly loaded on the GO through Bi-O-C bonding, which can form Bi2O2 2+ with excellent ionic conductivity. Moreover, the volume expansion of Bi during sodiation can be effectively buffered in the GO matrices. As a result, this Bi/GO composite exhibits excellent electrochemical performances in sodium-ion batteries (SIBs), including a high specific capacity of 258 mAh g−1 at 10 A g−1 and an excellent cycle stability with high retained capacity of 315 mAh g−1 after 500 cycles at 2 A g−1. This work paves the way to prepare designated promising electrode materials for high-performance SIBs, and thoroughly understands mechanism of electrochemical methods for preparing materials. Sodium-ion batteries Bi/GO composite Electrochemical method Anode materials Zintl clusters Fang, Susu verfasserin aut Xu, Laiqiang verfasserin aut Wang, Anni verfasserin aut Zou, Kangyu verfasserin aut Di, Andi verfasserin (orcid)0000-0003-4527-2504 aut Li, Fengrong verfasserin aut Deng, Wentao verfasserin aut Zou, Guoqiang verfasserin aut Hou, Hongshuai verfasserin aut Ji, Xiaobo verfasserin aut Enthalten in Electrochimica acta New York, NY [u.a.] : Elsevier, 1959 413 Online-Ressource (DE-627)300897561 (DE-600)1483548-4 (DE-576)094752451 1873-3859 nnns volume:413 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.00 Chemie: Allgemeines AR 413
allfieldsSound	10.1016/j.electacta.2022.140174 doi (DE-627)ELV007610548 (ELSEVIER)S0013-4686(22)00346-2 DE-627 ger DE-627 rda eng 540 DE-600 35.00 bkl Li, Jiayang verfasserin aut Electrochemical Zintl Cluster Bi 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Bismuth, a promising attribute for sodium-ion batteries, which have been attracting significant attention owing to their advantages of high volumetric capacity and suitable operating potential. However, most traditional Bi-based materials are suffered from pulverization and fracture of the electrodes caused by dramatic volume variation, consequently diminishing the cycle stability. Herein, in this work, bismuth embedded within graphene oxide matrices have been obtained by utilizing a novel and efficient electrochemical method. Through the strong reducing properties of Zintl clusters Bi2 2−, GO is partially reduced to generate reduced graphene oxide with better electrical conductivity. Simultaneously, Bi is strongly loaded on the GO through Bi-O-C bonding, which can form Bi2O2 2+ with excellent ionic conductivity. Moreover, the volume expansion of Bi during sodiation can be effectively buffered in the GO matrices. As a result, this Bi/GO composite exhibits excellent electrochemical performances in sodium-ion batteries (SIBs), including a high specific capacity of 258 mAh g−1 at 10 A g−1 and an excellent cycle stability with high retained capacity of 315 mAh g−1 after 500 cycles at 2 A g−1. This work paves the way to prepare designated promising electrode materials for high-performance SIBs, and thoroughly understands mechanism of electrochemical methods for preparing materials. Sodium-ion batteries Bi/GO composite Electrochemical method Anode materials Zintl clusters Fang, Susu verfasserin aut Xu, Laiqiang verfasserin aut Wang, Anni verfasserin aut Zou, Kangyu verfasserin aut Di, Andi verfasserin (orcid)0000-0003-4527-2504 aut Li, Fengrong verfasserin aut Deng, Wentao verfasserin aut Zou, Guoqiang verfasserin aut Hou, Hongshuai verfasserin aut Ji, Xiaobo verfasserin aut Enthalten in Electrochimica acta New York, NY [u.a.] : Elsevier, 1959 413 Online-Ressource (DE-627)300897561 (DE-600)1483548-4 (DE-576)094752451 1873-3859 nnns volume:413 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.00 Chemie: Allgemeines AR 413
language	English
source	Enthalten in Electrochimica acta 413 volume:413
sourceStr	Enthalten in Electrochimica acta 413 volume:413
format_phy_str_mv	Article
bklname	Chemie: Allgemeines
institution	findex.gbv.de
topic_facet	Sodium-ion batteries Bi/GO composite Electrochemical method Anode materials Zintl clusters
dewey-raw	540
isfreeaccess_bool	false
container_title	Electrochimica acta
authorswithroles_txt_mv	Li, Jiayang @@aut@@ Fang, Susu @@aut@@ Xu, Laiqiang @@aut@@ Wang, Anni @@aut@@ Zou, Kangyu @@aut@@ Di, Andi @@aut@@ Li, Fengrong @@aut@@ Deng, Wentao @@aut@@ Zou, Guoqiang @@aut@@ Hou, Hongshuai @@aut@@ Ji, Xiaobo @@aut@@
publishDateDaySort_date	2022-01-01T00:00:00Z
hierarchy_top_id	300897561
dewey-sort	3540
id	ELV007610548
language_de	englisch
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author	Li, Jiayang
spellingShingle	Li, Jiayang ddc 540 bkl 35.00 misc Sodium-ion batteries misc Bi/GO composite misc Electrochemical method misc Anode materials misc Zintl clusters Electrochemical Zintl Cluster Bi
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topic_title	540 DE-600 35.00 bkl Electrochemical Zintl Cluster Bi Sodium-ion batteries Bi/GO composite Electrochemical method Anode materials Zintl clusters
topic	ddc 540 bkl 35.00 misc Sodium-ion batteries misc Bi/GO composite misc Electrochemical method misc Anode materials misc Zintl clusters
topic_unstemmed	ddc 540 bkl 35.00 misc Sodium-ion batteries misc Bi/GO composite misc Electrochemical method misc Anode materials misc Zintl clusters
topic_browse	ddc 540 bkl 35.00 misc Sodium-ion batteries misc Bi/GO composite misc Electrochemical method misc Anode materials misc Zintl clusters
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title	Electrochemical Zintl Cluster Bi
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title_full	Electrochemical Zintl Cluster Bi
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author_browse	Li, Jiayang Fang, Susu Xu, Laiqiang Wang, Anni Zou, Kangyu Di, Andi Li, Fengrong Deng, Wentao Zou, Guoqiang Hou, Hongshuai Ji, Xiaobo
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title_sort	electrochemical zintl cluster bi
title_auth	Electrochemical Zintl Cluster Bi
abstract	Bismuth, a promising attribute for sodium-ion batteries, which have been attracting significant attention owing to their advantages of high volumetric capacity and suitable operating potential. However, most traditional Bi-based materials are suffered from pulverization and fracture of the electrodes caused by dramatic volume variation, consequently diminishing the cycle stability. Herein, in this work, bismuth embedded within graphene oxide matrices have been obtained by utilizing a novel and efficient electrochemical method. Through the strong reducing properties of Zintl clusters Bi2 2−, GO is partially reduced to generate reduced graphene oxide with better electrical conductivity. Simultaneously, Bi is strongly loaded on the GO through Bi-O-C bonding, which can form Bi2O2 2+ with excellent ionic conductivity. Moreover, the volume expansion of Bi during sodiation can be effectively buffered in the GO matrices. As a result, this Bi/GO composite exhibits excellent electrochemical performances in sodium-ion batteries (SIBs), including a high specific capacity of 258 mAh g−1 at 10 A g−1 and an excellent cycle stability with high retained capacity of 315 mAh g−1 after 500 cycles at 2 A g−1. This work paves the way to prepare designated promising electrode materials for high-performance SIBs, and thoroughly understands mechanism of electrochemical methods for preparing materials.
abstractGer	Bismuth, a promising attribute for sodium-ion batteries, which have been attracting significant attention owing to their advantages of high volumetric capacity and suitable operating potential. However, most traditional Bi-based materials are suffered from pulverization and fracture of the electrodes caused by dramatic volume variation, consequently diminishing the cycle stability. Herein, in this work, bismuth embedded within graphene oxide matrices have been obtained by utilizing a novel and efficient electrochemical method. Through the strong reducing properties of Zintl clusters Bi2 2−, GO is partially reduced to generate reduced graphene oxide with better electrical conductivity. Simultaneously, Bi is strongly loaded on the GO through Bi-O-C bonding, which can form Bi2O2 2+ with excellent ionic conductivity. Moreover, the volume expansion of Bi during sodiation can be effectively buffered in the GO matrices. As a result, this Bi/GO composite exhibits excellent electrochemical performances in sodium-ion batteries (SIBs), including a high specific capacity of 258 mAh g−1 at 10 A g−1 and an excellent cycle stability with high retained capacity of 315 mAh g−1 after 500 cycles at 2 A g−1. This work paves the way to prepare designated promising electrode materials for high-performance SIBs, and thoroughly understands mechanism of electrochemical methods for preparing materials.
abstract_unstemmed	Bismuth, a promising attribute for sodium-ion batteries, which have been attracting significant attention owing to their advantages of high volumetric capacity and suitable operating potential. However, most traditional Bi-based materials are suffered from pulverization and fracture of the electrodes caused by dramatic volume variation, consequently diminishing the cycle stability. Herein, in this work, bismuth embedded within graphene oxide matrices have been obtained by utilizing a novel and efficient electrochemical method. Through the strong reducing properties of Zintl clusters Bi2 2−, GO is partially reduced to generate reduced graphene oxide with better electrical conductivity. Simultaneously, Bi is strongly loaded on the GO through Bi-O-C bonding, which can form Bi2O2 2+ with excellent ionic conductivity. Moreover, the volume expansion of Bi during sodiation can be effectively buffered in the GO matrices. As a result, this Bi/GO composite exhibits excellent electrochemical performances in sodium-ion batteries (SIBs), including a high specific capacity of 258 mAh g−1 at 10 A g−1 and an excellent cycle stability with high retained capacity of 315 mAh g−1 after 500 cycles at 2 A g−1. This work paves the way to prepare designated promising electrode materials for high-performance SIBs, and thoroughly understands mechanism of electrochemical methods for preparing materials.
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title_short	Electrochemical Zintl Cluster Bi
remote_bool	true
author2	Fang, Susu Xu, Laiqiang Wang, Anni Zou, Kangyu Di, Andi Li, Fengrong Deng, Wentao Zou, Guoqiang Hou, Hongshuai Ji, Xiaobo
author2Str	Fang, Susu Xu, Laiqiang Wang, Anni Zou, Kangyu Di, Andi Li, Fengrong Deng, Wentao Zou, Guoqiang Hou, Hongshuai Ji, Xiaobo
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up_date	2024-07-06T16:51:25.334Z
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