Improving the stability and scalability of all-inorganic inverted CsPbI

All-inorganic perovskite solar cells (PSCs) have potential to pass the stability international standard of IEC61215:2016 but cannot deliver high performance and stability due to the poor interface contact. In this paper, Sn-doped TiO2 (Ti1− x Sn...
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Autor*in:	Duan, Chenghao [verfasserIn] Wen, Qiaoyun [verfasserIn] Fan, Yan [verfasserIn] Li, Jiong [verfasserIn] Liu, Zidan [verfasserIn] Yan, Keyou [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2021

Schlagwörter:	All-inorganic perovskite Sn-doped TiO Ultrathin nanocrystal Stability Scalability

Übergeordnetes Werk:	Enthalten in: Journal of Energy Chemistry - Amsterdam [u.a.] : Elsevier, 2013, 68, Seite 176-183
Übergeordnetes Werk:	volume:68 ; pages:176-183

DOI / URN:	10.1016/j.jechem.2021.11.026

Katalog-ID:	ELV007636075

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520			\|a All-inorganic perovskite solar cells (PSCs) have potential to pass the stability international standard of IEC61215:2016 but cannot deliver high performance and stability due to the poor interface contact. In this paper, Sn-doped TiO2 (Ti1− x Sn x O2) ultrathin nanoparticles are prepared for electron transport layer (ETL) by solution process. The ultrathin Ti0.9Sn0.1O2 nanocrystals have greatly improved interface contact due to the facile film formation, good conductivity and high work function. The all-inorganic inverted NiO x /CsPbI2Br/Ti0.9Sn0.1O2 p-i-n device shows a power conversion efficiency (PCE) of 14.0%. We tested the heat stability, light stability and light-heat stability. After stored in 85 °C for 65 days, the inverted PSCs still retains 98% of initial efficiency. Under continuous standard one-sun illumination for 600 h, there is no efficiency decay, and under continuous illumination at 85 °C for 200 h, the device still retains 85% of initial efficiency. The 1.0 cm2 device of inverted structure shows a PCE of up to 11.2%. The ultrathin Ti1− x Sn x O2 is promising to improve the scalability and stability and thus increase the commercial prospect.
650		4	\|a All-inorganic perovskite
650		4	\|a Sn-doped TiO
650		4	\|a Ultrathin nanocrystal
650		4	\|a Stability
650		4	\|a Scalability
700	1		\|a Wen, Qiaoyun \|e verfasserin \|4 aut
700	1		\|a Fan, Yan \|e verfasserin \|4 aut
700	1		\|a Li, Jiong \|e verfasserin \|4 aut
700	1		\|a Liu, Zidan \|e verfasserin \|4 aut
700	1		\|a Yan, Keyou \|e verfasserin \|4 aut
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912			\|a GBV_ILN_90
912			\|a GBV_ILN_95
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912			\|a GBV_ILN_105
912			\|a GBV_ILN_110
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912			\|a GBV_ILN_224
912			\|a GBV_ILN_370
912			\|a GBV_ILN_602
912			\|a GBV_ILN_702
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912			\|a GBV_ILN_2003
912			\|a GBV_ILN_2004
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912			\|a GBV_ILN_2011
912			\|a GBV_ILN_2014
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912			\|a GBV_ILN_2020
912			\|a GBV_ILN_2021
912			\|a GBV_ILN_2025
912			\|a GBV_ILN_2026
912			\|a GBV_ILN_2027
912			\|a GBV_ILN_2034
912			\|a GBV_ILN_2038
912			\|a GBV_ILN_2044
912			\|a GBV_ILN_2048
912			\|a GBV_ILN_2049
912			\|a GBV_ILN_2050
912			\|a GBV_ILN_2055
912			\|a GBV_ILN_2056
912			\|a GBV_ILN_2059
912			\|a GBV_ILN_2061
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912			\|a GBV_ILN_4305
912			\|a GBV_ILN_4313
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912			\|a GBV_ILN_4324
912			\|a GBV_ILN_4325
912			\|a GBV_ILN_4326
912			\|a GBV_ILN_4333
912			\|a GBV_ILN_4334
912			\|a GBV_ILN_4335
912			\|a GBV_ILN_4338
912			\|a GBV_ILN_4393
951			\|a AR
952			\|d 68 \|h 176-183

Indexfelder

author_variant	c d cd q w qw y f yf j l jl z l zl k y ky
matchkey_str	article:2096885X:2021----::mrvntetbltadclbltoalnr
hierarchy_sort_str	2021
publishDate	2021
allfields	10.1016/j.jechem.2021.11.026 doi (DE-627)ELV007636075 (ELSEVIER)S2095-4956(21)00630-6 DE-627 ger DE-627 rda eng 540 DE-600 Duan, Chenghao verfasserin aut Improving the stability and scalability of all-inorganic inverted CsPbI 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier All-inorganic perovskite solar cells (PSCs) have potential to pass the stability international standard of IEC61215:2016 but cannot deliver high performance and stability due to the poor interface contact. In this paper, Sn-doped TiO2 (Ti1− x Sn x O2) ultrathin nanoparticles are prepared for electron transport layer (ETL) by solution process. The ultrathin Ti0.9Sn0.1O2 nanocrystals have greatly improved interface contact due to the facile film formation, good conductivity and high work function. The all-inorganic inverted NiO x /CsPbI2Br/Ti0.9Sn0.1O2 p-i-n device shows a power conversion efficiency (PCE) of 14.0%. We tested the heat stability, light stability and light-heat stability. After stored in 85 °C for 65 days, the inverted PSCs still retains 98% of initial efficiency. Under continuous standard one-sun illumination for 600 h, there is no efficiency decay, and under continuous illumination at 85 °C for 200 h, the device still retains 85% of initial efficiency. The 1.0 cm2 device of inverted structure shows a PCE of up to 11.2%. The ultrathin Ti1− x Sn x O2 is promising to improve the scalability and stability and thus increase the commercial prospect. All-inorganic perovskite Sn-doped TiO Ultrathin nanocrystal Stability Scalability Wen, Qiaoyun verfasserin aut Fan, Yan verfasserin aut Li, Jiong verfasserin aut Liu, Zidan verfasserin aut Yan, Keyou verfasserin aut Enthalten in Journal of Energy Chemistry Amsterdam [u.a.] : Elsevier, 2013 68, Seite 176-183 Online-Ressource (DE-627)745616399 (DE-600)2714311-9 (DE-576)382032861 2096-885X nnns volume:68 pages:176-183 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 AR 68 176-183
spelling	10.1016/j.jechem.2021.11.026 doi (DE-627)ELV007636075 (ELSEVIER)S2095-4956(21)00630-6 DE-627 ger DE-627 rda eng 540 DE-600 Duan, Chenghao verfasserin aut Improving the stability and scalability of all-inorganic inverted CsPbI 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier All-inorganic perovskite solar cells (PSCs) have potential to pass the stability international standard of IEC61215:2016 but cannot deliver high performance and stability due to the poor interface contact. In this paper, Sn-doped TiO2 (Ti1− x Sn x O2) ultrathin nanoparticles are prepared for electron transport layer (ETL) by solution process. The ultrathin Ti0.9Sn0.1O2 nanocrystals have greatly improved interface contact due to the facile film formation, good conductivity and high work function. The all-inorganic inverted NiO x /CsPbI2Br/Ti0.9Sn0.1O2 p-i-n device shows a power conversion efficiency (PCE) of 14.0%. We tested the heat stability, light stability and light-heat stability. After stored in 85 °C for 65 days, the inverted PSCs still retains 98% of initial efficiency. Under continuous standard one-sun illumination for 600 h, there is no efficiency decay, and under continuous illumination at 85 °C for 200 h, the device still retains 85% of initial efficiency. The 1.0 cm2 device of inverted structure shows a PCE of up to 11.2%. The ultrathin Ti1− x Sn x O2 is promising to improve the scalability and stability and thus increase the commercial prospect. All-inorganic perovskite Sn-doped TiO Ultrathin nanocrystal Stability Scalability Wen, Qiaoyun verfasserin aut Fan, Yan verfasserin aut Li, Jiong verfasserin aut Liu, Zidan verfasserin aut Yan, Keyou verfasserin aut Enthalten in Journal of Energy Chemistry Amsterdam [u.a.] : Elsevier, 2013 68, Seite 176-183 Online-Ressource (DE-627)745616399 (DE-600)2714311-9 (DE-576)382032861 2096-885X nnns volume:68 pages:176-183 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 AR 68 176-183
allfields_unstemmed	10.1016/j.jechem.2021.11.026 doi (DE-627)ELV007636075 (ELSEVIER)S2095-4956(21)00630-6 DE-627 ger DE-627 rda eng 540 DE-600 Duan, Chenghao verfasserin aut Improving the stability and scalability of all-inorganic inverted CsPbI 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier All-inorganic perovskite solar cells (PSCs) have potential to pass the stability international standard of IEC61215:2016 but cannot deliver high performance and stability due to the poor interface contact. In this paper, Sn-doped TiO2 (Ti1− x Sn x O2) ultrathin nanoparticles are prepared for electron transport layer (ETL) by solution process. The ultrathin Ti0.9Sn0.1O2 nanocrystals have greatly improved interface contact due to the facile film formation, good conductivity and high work function. The all-inorganic inverted NiO x /CsPbI2Br/Ti0.9Sn0.1O2 p-i-n device shows a power conversion efficiency (PCE) of 14.0%. We tested the heat stability, light stability and light-heat stability. After stored in 85 °C for 65 days, the inverted PSCs still retains 98% of initial efficiency. Under continuous standard one-sun illumination for 600 h, there is no efficiency decay, and under continuous illumination at 85 °C for 200 h, the device still retains 85% of initial efficiency. The 1.0 cm2 device of inverted structure shows a PCE of up to 11.2%. The ultrathin Ti1− x Sn x O2 is promising to improve the scalability and stability and thus increase the commercial prospect. All-inorganic perovskite Sn-doped TiO Ultrathin nanocrystal Stability Scalability Wen, Qiaoyun verfasserin aut Fan, Yan verfasserin aut Li, Jiong verfasserin aut Liu, Zidan verfasserin aut Yan, Keyou verfasserin aut Enthalten in Journal of Energy Chemistry Amsterdam [u.a.] : Elsevier, 2013 68, Seite 176-183 Online-Ressource (DE-627)745616399 (DE-600)2714311-9 (DE-576)382032861 2096-885X nnns volume:68 pages:176-183 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 AR 68 176-183
allfieldsGer	10.1016/j.jechem.2021.11.026 doi (DE-627)ELV007636075 (ELSEVIER)S2095-4956(21)00630-6 DE-627 ger DE-627 rda eng 540 DE-600 Duan, Chenghao verfasserin aut Improving the stability and scalability of all-inorganic inverted CsPbI 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier All-inorganic perovskite solar cells (PSCs) have potential to pass the stability international standard of IEC61215:2016 but cannot deliver high performance and stability due to the poor interface contact. In this paper, Sn-doped TiO2 (Ti1− x Sn x O2) ultrathin nanoparticles are prepared for electron transport layer (ETL) by solution process. The ultrathin Ti0.9Sn0.1O2 nanocrystals have greatly improved interface contact due to the facile film formation, good conductivity and high work function. The all-inorganic inverted NiO x /CsPbI2Br/Ti0.9Sn0.1O2 p-i-n device shows a power conversion efficiency (PCE) of 14.0%. We tested the heat stability, light stability and light-heat stability. After stored in 85 °C for 65 days, the inverted PSCs still retains 98% of initial efficiency. Under continuous standard one-sun illumination for 600 h, there is no efficiency decay, and under continuous illumination at 85 °C for 200 h, the device still retains 85% of initial efficiency. The 1.0 cm2 device of inverted structure shows a PCE of up to 11.2%. The ultrathin Ti1− x Sn x O2 is promising to improve the scalability and stability and thus increase the commercial prospect. All-inorganic perovskite Sn-doped TiO Ultrathin nanocrystal Stability Scalability Wen, Qiaoyun verfasserin aut Fan, Yan verfasserin aut Li, Jiong verfasserin aut Liu, Zidan verfasserin aut Yan, Keyou verfasserin aut Enthalten in Journal of Energy Chemistry Amsterdam [u.a.] : Elsevier, 2013 68, Seite 176-183 Online-Ressource (DE-627)745616399 (DE-600)2714311-9 (DE-576)382032861 2096-885X nnns volume:68 pages:176-183 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 AR 68 176-183
allfieldsSound	10.1016/j.jechem.2021.11.026 doi (DE-627)ELV007636075 (ELSEVIER)S2095-4956(21)00630-6 DE-627 ger DE-627 rda eng 540 DE-600 Duan, Chenghao verfasserin aut Improving the stability and scalability of all-inorganic inverted CsPbI 2021 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier All-inorganic perovskite solar cells (PSCs) have potential to pass the stability international standard of IEC61215:2016 but cannot deliver high performance and stability due to the poor interface contact. In this paper, Sn-doped TiO2 (Ti1− x Sn x O2) ultrathin nanoparticles are prepared for electron transport layer (ETL) by solution process. The ultrathin Ti0.9Sn0.1O2 nanocrystals have greatly improved interface contact due to the facile film formation, good conductivity and high work function. The all-inorganic inverted NiO x /CsPbI2Br/Ti0.9Sn0.1O2 p-i-n device shows a power conversion efficiency (PCE) of 14.0%. We tested the heat stability, light stability and light-heat stability. After stored in 85 °C for 65 days, the inverted PSCs still retains 98% of initial efficiency. Under continuous standard one-sun illumination for 600 h, there is no efficiency decay, and under continuous illumination at 85 °C for 200 h, the device still retains 85% of initial efficiency. The 1.0 cm2 device of inverted structure shows a PCE of up to 11.2%. The ultrathin Ti1− x Sn x O2 is promising to improve the scalability and stability and thus increase the commercial prospect. All-inorganic perovskite Sn-doped TiO Ultrathin nanocrystal Stability Scalability Wen, Qiaoyun verfasserin aut Fan, Yan verfasserin aut Li, Jiong verfasserin aut Liu, Zidan verfasserin aut Yan, Keyou verfasserin aut Enthalten in Journal of Energy Chemistry Amsterdam [u.a.] : Elsevier, 2013 68, Seite 176-183 Online-Ressource (DE-627)745616399 (DE-600)2714311-9 (DE-576)382032861 2096-885X nnns volume:68 pages:176-183 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 AR 68 176-183
language	English
source	Enthalten in Journal of Energy Chemistry 68, Seite 176-183 volume:68 pages:176-183
sourceStr	Enthalten in Journal of Energy Chemistry 68, Seite 176-183 volume:68 pages:176-183
format_phy_str_mv	Article
institution	findex.gbv.de
topic_facet	All-inorganic perovskite Sn-doped TiO Ultrathin nanocrystal Stability Scalability
dewey-raw	540
isfreeaccess_bool	false
container_title	Journal of Energy Chemistry
authorswithroles_txt_mv	Duan, Chenghao @@aut@@ Wen, Qiaoyun @@aut@@ Fan, Yan @@aut@@ Li, Jiong @@aut@@ Liu, Zidan @@aut@@ Yan, Keyou @@aut@@
publishDateDaySort_date	2021-01-01T00:00:00Z
hierarchy_top_id	745616399
dewey-sort	3540
id	ELV007636075
language_de	englisch
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author	Duan, Chenghao
spellingShingle	Duan, Chenghao ddc 540 misc All-inorganic perovskite misc Sn-doped TiO misc Ultrathin nanocrystal misc Stability misc Scalability Improving the stability and scalability of all-inorganic inverted CsPbI
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topic_title	540 DE-600 Improving the stability and scalability of all-inorganic inverted CsPbI All-inorganic perovskite Sn-doped TiO Ultrathin nanocrystal Stability Scalability
topic	ddc 540 misc All-inorganic perovskite misc Sn-doped TiO misc Ultrathin nanocrystal misc Stability misc Scalability
topic_unstemmed	ddc 540 misc All-inorganic perovskite misc Sn-doped TiO misc Ultrathin nanocrystal misc Stability misc Scalability
topic_browse	ddc 540 misc All-inorganic perovskite misc Sn-doped TiO misc Ultrathin nanocrystal misc Stability misc Scalability
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title	Improving the stability and scalability of all-inorganic inverted CsPbI
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title_full	Improving the stability and scalability of all-inorganic inverted CsPbI
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author_browse	Duan, Chenghao Wen, Qiaoyun Fan, Yan Li, Jiong Liu, Zidan Yan, Keyou
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title_sort	improving the stability and scalability of all-inorganic inverted cspbi
title_auth	Improving the stability and scalability of all-inorganic inverted CsPbI
abstract	All-inorganic perovskite solar cells (PSCs) have potential to pass the stability international standard of IEC61215:2016 but cannot deliver high performance and stability due to the poor interface contact. In this paper, Sn-doped TiO2 (Ti1− x Sn x O2) ultrathin nanoparticles are prepared for electron transport layer (ETL) by solution process. The ultrathin Ti0.9Sn0.1O2 nanocrystals have greatly improved interface contact due to the facile film formation, good conductivity and high work function. The all-inorganic inverted NiO x /CsPbI2Br/Ti0.9Sn0.1O2 p-i-n device shows a power conversion efficiency (PCE) of 14.0%. We tested the heat stability, light stability and light-heat stability. After stored in 85 °C for 65 days, the inverted PSCs still retains 98% of initial efficiency. Under continuous standard one-sun illumination for 600 h, there is no efficiency decay, and under continuous illumination at 85 °C for 200 h, the device still retains 85% of initial efficiency. The 1.0 cm2 device of inverted structure shows a PCE of up to 11.2%. The ultrathin Ti1− x Sn x O2 is promising to improve the scalability and stability and thus increase the commercial prospect.
abstractGer	All-inorganic perovskite solar cells (PSCs) have potential to pass the stability international standard of IEC61215:2016 but cannot deliver high performance and stability due to the poor interface contact. In this paper, Sn-doped TiO2 (Ti1− x Sn x O2) ultrathin nanoparticles are prepared for electron transport layer (ETL) by solution process. The ultrathin Ti0.9Sn0.1O2 nanocrystals have greatly improved interface contact due to the facile film formation, good conductivity and high work function. The all-inorganic inverted NiO x /CsPbI2Br/Ti0.9Sn0.1O2 p-i-n device shows a power conversion efficiency (PCE) of 14.0%. We tested the heat stability, light stability and light-heat stability. After stored in 85 °C for 65 days, the inverted PSCs still retains 98% of initial efficiency. Under continuous standard one-sun illumination for 600 h, there is no efficiency decay, and under continuous illumination at 85 °C for 200 h, the device still retains 85% of initial efficiency. The 1.0 cm2 device of inverted structure shows a PCE of up to 11.2%. The ultrathin Ti1− x Sn x O2 is promising to improve the scalability and stability and thus increase the commercial prospect.
abstract_unstemmed	All-inorganic perovskite solar cells (PSCs) have potential to pass the stability international standard of IEC61215:2016 but cannot deliver high performance and stability due to the poor interface contact. In this paper, Sn-doped TiO2 (Ti1− x Sn x O2) ultrathin nanoparticles are prepared for electron transport layer (ETL) by solution process. The ultrathin Ti0.9Sn0.1O2 nanocrystals have greatly improved interface contact due to the facile film formation, good conductivity and high work function. The all-inorganic inverted NiO x /CsPbI2Br/Ti0.9Sn0.1O2 p-i-n device shows a power conversion efficiency (PCE) of 14.0%. We tested the heat stability, light stability and light-heat stability. After stored in 85 °C for 65 days, the inverted PSCs still retains 98% of initial efficiency. Under continuous standard one-sun illumination for 600 h, there is no efficiency decay, and under continuous illumination at 85 °C for 200 h, the device still retains 85% of initial efficiency. The 1.0 cm2 device of inverted structure shows a PCE of up to 11.2%. The ultrathin Ti1− x Sn x O2 is promising to improve the scalability and stability and thus increase the commercial prospect.
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title_short	Improving the stability and scalability of all-inorganic inverted CsPbI
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author2	Wen, Qiaoyun Fan, Yan Li, Jiong Liu, Zidan Yan, Keyou
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doi_str	10.1016/j.jechem.2021.11.026
up_date	2024-07-06T16:56:51.241Z
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Improving the stability and scalability of all-inorganic inverted CsPbI

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