One-pot synthesis of m-Bi

Developing efficient photocatalysts is critical for degradation of organic pollutants. Herein, a highly efficient heterojunction photocatalyst (m-Bi2O4/Bi2O4−x/BiOCl) was synthesized by a hydrothermal method. Through changing the added volume of concentrated HCl acid, the ternary composite based on...
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Autor*in:	Liu, Miaomiao [verfasserIn] Liu, Gang [verfasserIn] Liu, Xinmei [verfasserIn] Wang, Xiaoyi [verfasserIn] Chen, YunLong [verfasserIn] Yang, Wenlong [verfasserIn] Gao, Chunpeng [verfasserIn] Wang, Guanxiang [verfasserIn] Teng, Zhengchun [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2022

Schlagwörter:	Bi Ternary heterojunction Photocatalytic activity Organic pollutant

Übergeordnetes Werk:	Enthalten in: Colloids and surfaces / A - Amsterdam [u.a.] : Elsevier Science, 1993, 643
Übergeordnetes Werk:	volume:643

DOI / URN:	10.1016/j.colsurfa.2022.128772

Katalog-ID:	ELV00766236X

Internformat


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520			\|a Developing efficient photocatalysts is critical for degradation of organic pollutants. Herein, a highly efficient heterojunction photocatalyst (m-Bi2O4/Bi2O4−x/BiOCl) was synthesized by a hydrothermal method. Through changing the added volume of concentrated HCl acid, the ternary composite based on BiOCl nanosheets matrix on which the m-Bi2O4 micro-rods and the Bi2O4−x nanospheres are firmly attached. The prepared m-Bi2O4/Bi2O4−x/BiOCl showed a favorable degradation rate and mineralization ability towards Bisphenol A (BPA) and Ciprofloxacin (CIP) under visible light irradiation, which degraded 98.3% of BPA in 30 min, 82.3% of CIP in 80 min, and the rate constants were around 30.16 and 2.82 times higher than that of pure BiOCl, respectively. This enhanced photocatalytic activity of m-Bi2O4/Bi2O4−x/BiOCl composite can be originated from the improved light adsorption range and the synergistic effect of type-II and the Z-scheme charge transfer on the interfaces of m-Bi2O4, Bi2O4−x and BiOCl, which then lead to an accelerated separation and migration of photo-generated carriers. Meanwhile, the photoluminescence (PL) test and photoelectrochemistry (PEC) test provided strong evidence for the construction of the heterojunction. Moreover, the repeatability of m-Bi2O4/Bi2O4−x/BiOCl heterojunction photocatalyst was also investigated, and it still remained 90% photocatalytic activity after four successive cycles. This work proposed a possible photocatalytic pathway for m-Bi2O4/Bi2O4−x/BiOCl, which would open up a new avenue for water environment treatment utilizing ternary photocatalysts.
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700	1		\|a Gao, Chunpeng \|e verfasserin \|4 aut
700	1		\|a Wang, Guanxiang \|e verfasserin \|4 aut
700	1		\|a Teng, Zhengchun \|e verfasserin \|4 aut
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Indexfelder

author_variant	m l ml g l gl x l xl x w xw y c yc w y wy c g cg g w gw z t zt
matchkey_str	article:18734359:2022----::nptytei
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publishDate	2022
allfields	10.1016/j.colsurfa.2022.128772 doi (DE-627)ELV00766236X (ELSEVIER)S0927-7757(22)00527-1 DE-627 ger DE-627 rda eng 540 DE-600 35.18 bkl 33.68 bkl 52.78 bkl 58.20 bkl Liu, Miaomiao verfasserin aut One-pot synthesis of m-Bi 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Developing efficient photocatalysts is critical for degradation of organic pollutants. Herein, a highly efficient heterojunction photocatalyst (m-Bi2O4/Bi2O4−x/BiOCl) was synthesized by a hydrothermal method. Through changing the added volume of concentrated HCl acid, the ternary composite based on BiOCl nanosheets matrix on which the m-Bi2O4 micro-rods and the Bi2O4−x nanospheres are firmly attached. The prepared m-Bi2O4/Bi2O4−x/BiOCl showed a favorable degradation rate and mineralization ability towards Bisphenol A (BPA) and Ciprofloxacin (CIP) under visible light irradiation, which degraded 98.3% of BPA in 30 min, 82.3% of CIP in 80 min, and the rate constants were around 30.16 and 2.82 times higher than that of pure BiOCl, respectively. This enhanced photocatalytic activity of m-Bi2O4/Bi2O4−x/BiOCl composite can be originated from the improved light adsorption range and the synergistic effect of type-II and the Z-scheme charge transfer on the interfaces of m-Bi2O4, Bi2O4−x and BiOCl, which then lead to an accelerated separation and migration of photo-generated carriers. Meanwhile, the photoluminescence (PL) test and photoelectrochemistry (PEC) test provided strong evidence for the construction of the heterojunction. Moreover, the repeatability of m-Bi2O4/Bi2O4−x/BiOCl heterojunction photocatalyst was also investigated, and it still remained 90% photocatalytic activity after four successive cycles. This work proposed a possible photocatalytic pathway for m-Bi2O4/Bi2O4−x/BiOCl, which would open up a new avenue for water environment treatment utilizing ternary photocatalysts. Bi Ternary heterojunction Photocatalytic activity Organic pollutant Liu, Gang verfasserin aut Liu, Xinmei verfasserin aut Wang, Xiaoyi verfasserin aut Chen, YunLong verfasserin aut Yang, Wenlong verfasserin aut Gao, Chunpeng verfasserin aut Wang, Guanxiang verfasserin aut Teng, Zhengchun verfasserin aut Enthalten in Colloids and surfaces / A Amsterdam [u.a.] : Elsevier Science, 1993 643 Online-Ressource (DE-627)306659956 (DE-600)1500517-3 (DE-576)098614843 1873-4359 nnns volume:643 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2411 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.18 Kolloidchemie Grenzflächenchemie 33.68 Oberflächen Dünne Schichten Grenzflächen Physik 52.78 Oberflächentechnik Wärmebehandlung 58.20 Chemische Technologien: Allgemeines AR 643
spelling	10.1016/j.colsurfa.2022.128772 doi (DE-627)ELV00766236X (ELSEVIER)S0927-7757(22)00527-1 DE-627 ger DE-627 rda eng 540 DE-600 35.18 bkl 33.68 bkl 52.78 bkl 58.20 bkl Liu, Miaomiao verfasserin aut One-pot synthesis of m-Bi 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Developing efficient photocatalysts is critical for degradation of organic pollutants. Herein, a highly efficient heterojunction photocatalyst (m-Bi2O4/Bi2O4−x/BiOCl) was synthesized by a hydrothermal method. Through changing the added volume of concentrated HCl acid, the ternary composite based on BiOCl nanosheets matrix on which the m-Bi2O4 micro-rods and the Bi2O4−x nanospheres are firmly attached. The prepared m-Bi2O4/Bi2O4−x/BiOCl showed a favorable degradation rate and mineralization ability towards Bisphenol A (BPA) and Ciprofloxacin (CIP) under visible light irradiation, which degraded 98.3% of BPA in 30 min, 82.3% of CIP in 80 min, and the rate constants were around 30.16 and 2.82 times higher than that of pure BiOCl, respectively. This enhanced photocatalytic activity of m-Bi2O4/Bi2O4−x/BiOCl composite can be originated from the improved light adsorption range and the synergistic effect of type-II and the Z-scheme charge transfer on the interfaces of m-Bi2O4, Bi2O4−x and BiOCl, which then lead to an accelerated separation and migration of photo-generated carriers. Meanwhile, the photoluminescence (PL) test and photoelectrochemistry (PEC) test provided strong evidence for the construction of the heterojunction. Moreover, the repeatability of m-Bi2O4/Bi2O4−x/BiOCl heterojunction photocatalyst was also investigated, and it still remained 90% photocatalytic activity after four successive cycles. This work proposed a possible photocatalytic pathway for m-Bi2O4/Bi2O4−x/BiOCl, which would open up a new avenue for water environment treatment utilizing ternary photocatalysts. Bi Ternary heterojunction Photocatalytic activity Organic pollutant Liu, Gang verfasserin aut Liu, Xinmei verfasserin aut Wang, Xiaoyi verfasserin aut Chen, YunLong verfasserin aut Yang, Wenlong verfasserin aut Gao, Chunpeng verfasserin aut Wang, Guanxiang verfasserin aut Teng, Zhengchun verfasserin aut Enthalten in Colloids and surfaces / A Amsterdam [u.a.] : Elsevier Science, 1993 643 Online-Ressource (DE-627)306659956 (DE-600)1500517-3 (DE-576)098614843 1873-4359 nnns volume:643 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2411 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.18 Kolloidchemie Grenzflächenchemie 33.68 Oberflächen Dünne Schichten Grenzflächen Physik 52.78 Oberflächentechnik Wärmebehandlung 58.20 Chemische Technologien: Allgemeines AR 643
allfields_unstemmed	10.1016/j.colsurfa.2022.128772 doi (DE-627)ELV00766236X (ELSEVIER)S0927-7757(22)00527-1 DE-627 ger DE-627 rda eng 540 DE-600 35.18 bkl 33.68 bkl 52.78 bkl 58.20 bkl Liu, Miaomiao verfasserin aut One-pot synthesis of m-Bi 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Developing efficient photocatalysts is critical for degradation of organic pollutants. Herein, a highly efficient heterojunction photocatalyst (m-Bi2O4/Bi2O4−x/BiOCl) was synthesized by a hydrothermal method. Through changing the added volume of concentrated HCl acid, the ternary composite based on BiOCl nanosheets matrix on which the m-Bi2O4 micro-rods and the Bi2O4−x nanospheres are firmly attached. The prepared m-Bi2O4/Bi2O4−x/BiOCl showed a favorable degradation rate and mineralization ability towards Bisphenol A (BPA) and Ciprofloxacin (CIP) under visible light irradiation, which degraded 98.3% of BPA in 30 min, 82.3% of CIP in 80 min, and the rate constants were around 30.16 and 2.82 times higher than that of pure BiOCl, respectively. This enhanced photocatalytic activity of m-Bi2O4/Bi2O4−x/BiOCl composite can be originated from the improved light adsorption range and the synergistic effect of type-II and the Z-scheme charge transfer on the interfaces of m-Bi2O4, Bi2O4−x and BiOCl, which then lead to an accelerated separation and migration of photo-generated carriers. Meanwhile, the photoluminescence (PL) test and photoelectrochemistry (PEC) test provided strong evidence for the construction of the heterojunction. Moreover, the repeatability of m-Bi2O4/Bi2O4−x/BiOCl heterojunction photocatalyst was also investigated, and it still remained 90% photocatalytic activity after four successive cycles. This work proposed a possible photocatalytic pathway for m-Bi2O4/Bi2O4−x/BiOCl, which would open up a new avenue for water environment treatment utilizing ternary photocatalysts. Bi Ternary heterojunction Photocatalytic activity Organic pollutant Liu, Gang verfasserin aut Liu, Xinmei verfasserin aut Wang, Xiaoyi verfasserin aut Chen, YunLong verfasserin aut Yang, Wenlong verfasserin aut Gao, Chunpeng verfasserin aut Wang, Guanxiang verfasserin aut Teng, Zhengchun verfasserin aut Enthalten in Colloids and surfaces / A Amsterdam [u.a.] : Elsevier Science, 1993 643 Online-Ressource (DE-627)306659956 (DE-600)1500517-3 (DE-576)098614843 1873-4359 nnns volume:643 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2411 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.18 Kolloidchemie Grenzflächenchemie 33.68 Oberflächen Dünne Schichten Grenzflächen Physik 52.78 Oberflächentechnik Wärmebehandlung 58.20 Chemische Technologien: Allgemeines AR 643
allfieldsGer	10.1016/j.colsurfa.2022.128772 doi (DE-627)ELV00766236X (ELSEVIER)S0927-7757(22)00527-1 DE-627 ger DE-627 rda eng 540 DE-600 35.18 bkl 33.68 bkl 52.78 bkl 58.20 bkl Liu, Miaomiao verfasserin aut One-pot synthesis of m-Bi 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Developing efficient photocatalysts is critical for degradation of organic pollutants. Herein, a highly efficient heterojunction photocatalyst (m-Bi2O4/Bi2O4−x/BiOCl) was synthesized by a hydrothermal method. Through changing the added volume of concentrated HCl acid, the ternary composite based on BiOCl nanosheets matrix on which the m-Bi2O4 micro-rods and the Bi2O4−x nanospheres are firmly attached. The prepared m-Bi2O4/Bi2O4−x/BiOCl showed a favorable degradation rate and mineralization ability towards Bisphenol A (BPA) and Ciprofloxacin (CIP) under visible light irradiation, which degraded 98.3% of BPA in 30 min, 82.3% of CIP in 80 min, and the rate constants were around 30.16 and 2.82 times higher than that of pure BiOCl, respectively. This enhanced photocatalytic activity of m-Bi2O4/Bi2O4−x/BiOCl composite can be originated from the improved light adsorption range and the synergistic effect of type-II and the Z-scheme charge transfer on the interfaces of m-Bi2O4, Bi2O4−x and BiOCl, which then lead to an accelerated separation and migration of photo-generated carriers. Meanwhile, the photoluminescence (PL) test and photoelectrochemistry (PEC) test provided strong evidence for the construction of the heterojunction. Moreover, the repeatability of m-Bi2O4/Bi2O4−x/BiOCl heterojunction photocatalyst was also investigated, and it still remained 90% photocatalytic activity after four successive cycles. This work proposed a possible photocatalytic pathway for m-Bi2O4/Bi2O4−x/BiOCl, which would open up a new avenue for water environment treatment utilizing ternary photocatalysts. Bi Ternary heterojunction Photocatalytic activity Organic pollutant Liu, Gang verfasserin aut Liu, Xinmei verfasserin aut Wang, Xiaoyi verfasserin aut Chen, YunLong verfasserin aut Yang, Wenlong verfasserin aut Gao, Chunpeng verfasserin aut Wang, Guanxiang verfasserin aut Teng, Zhengchun verfasserin aut Enthalten in Colloids and surfaces / A Amsterdam [u.a.] : Elsevier Science, 1993 643 Online-Ressource (DE-627)306659956 (DE-600)1500517-3 (DE-576)098614843 1873-4359 nnns volume:643 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2411 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.18 Kolloidchemie Grenzflächenchemie 33.68 Oberflächen Dünne Schichten Grenzflächen Physik 52.78 Oberflächentechnik Wärmebehandlung 58.20 Chemische Technologien: Allgemeines AR 643
allfieldsSound	10.1016/j.colsurfa.2022.128772 doi (DE-627)ELV00766236X (ELSEVIER)S0927-7757(22)00527-1 DE-627 ger DE-627 rda eng 540 DE-600 35.18 bkl 33.68 bkl 52.78 bkl 58.20 bkl Liu, Miaomiao verfasserin aut One-pot synthesis of m-Bi 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Developing efficient photocatalysts is critical for degradation of organic pollutants. Herein, a highly efficient heterojunction photocatalyst (m-Bi2O4/Bi2O4−x/BiOCl) was synthesized by a hydrothermal method. Through changing the added volume of concentrated HCl acid, the ternary composite based on BiOCl nanosheets matrix on which the m-Bi2O4 micro-rods and the Bi2O4−x nanospheres are firmly attached. The prepared m-Bi2O4/Bi2O4−x/BiOCl showed a favorable degradation rate and mineralization ability towards Bisphenol A (BPA) and Ciprofloxacin (CIP) under visible light irradiation, which degraded 98.3% of BPA in 30 min, 82.3% of CIP in 80 min, and the rate constants were around 30.16 and 2.82 times higher than that of pure BiOCl, respectively. This enhanced photocatalytic activity of m-Bi2O4/Bi2O4−x/BiOCl composite can be originated from the improved light adsorption range and the synergistic effect of type-II and the Z-scheme charge transfer on the interfaces of m-Bi2O4, Bi2O4−x and BiOCl, which then lead to an accelerated separation and migration of photo-generated carriers. Meanwhile, the photoluminescence (PL) test and photoelectrochemistry (PEC) test provided strong evidence for the construction of the heterojunction. Moreover, the repeatability of m-Bi2O4/Bi2O4−x/BiOCl heterojunction photocatalyst was also investigated, and it still remained 90% photocatalytic activity after four successive cycles. This work proposed a possible photocatalytic pathway for m-Bi2O4/Bi2O4−x/BiOCl, which would open up a new avenue for water environment treatment utilizing ternary photocatalysts. Bi Ternary heterojunction Photocatalytic activity Organic pollutant Liu, Gang verfasserin aut Liu, Xinmei verfasserin aut Wang, Xiaoyi verfasserin aut Chen, YunLong verfasserin aut Yang, Wenlong verfasserin aut Gao, Chunpeng verfasserin aut Wang, Guanxiang verfasserin aut Teng, Zhengchun verfasserin aut Enthalten in Colloids and surfaces / A Amsterdam [u.a.] : Elsevier Science, 1993 643 Online-Ressource (DE-627)306659956 (DE-600)1500517-3 (DE-576)098614843 1873-4359 nnns volume:643 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2411 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.18 Kolloidchemie Grenzflächenchemie 33.68 Oberflächen Dünne Schichten Grenzflächen Physik 52.78 Oberflächentechnik Wärmebehandlung 58.20 Chemische Technologien: Allgemeines AR 643
language	English
source	Enthalten in Colloids and surfaces / A 643 volume:643
sourceStr	Enthalten in Colloids and surfaces / A 643 volume:643
format_phy_str_mv	Article
bklname	Kolloidchemie Grenzflächenchemie Oberflächen Dünne Schichten Grenzflächen Oberflächentechnik Wärmebehandlung Chemische Technologien: Allgemeines
institution	findex.gbv.de
topic_facet	Bi Ternary heterojunction Photocatalytic activity Organic pollutant
dewey-raw	540
isfreeaccess_bool	false
container_title	Colloids and surfaces / A
authorswithroles_txt_mv	Liu, Miaomiao @@aut@@ Liu, Gang @@aut@@ Liu, Xinmei @@aut@@ Wang, Xiaoyi @@aut@@ Chen, YunLong @@aut@@ Yang, Wenlong @@aut@@ Gao, Chunpeng @@aut@@ Wang, Guanxiang @@aut@@ Teng, Zhengchun @@aut@@
publishDateDaySort_date	2022-01-01T00:00:00Z
hierarchy_top_id	306659956
dewey-sort	3540
id	ELV00766236X
language_de	englisch
fullrecord	<?xml version="1.0" encoding="UTF-8"?><collection xmlns="http://www.loc.gov/MARC21/slim"><record><leader>01000caa a22002652 4500</leader><controlfield tag="001">ELV00766236X</controlfield><controlfield tag="003">DE-627</controlfield><controlfield tag="005">20230524152138.0</controlfield><controlfield tag="007">cr uuu---uuuuu</controlfield><controlfield tag="008">230507s2022 xx \|\|\|\|\|o 00\| \|\|eng c</controlfield><datafield tag="024" ind1="7" ind2=" "><subfield code="a">10.1016/j.colsurfa.2022.128772</subfield><subfield code="2">doi</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(DE-627)ELV00766236X</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(ELSEVIER)S0927-7757(22)00527-1</subfield></datafield><datafield tag="040" ind1=" " ind2=" "><subfield code="a">DE-627</subfield><subfield code="b">ger</subfield><subfield code="c">DE-627</subfield><subfield code="e">rda</subfield></datafield><datafield tag="041" ind1=" " ind2=" "><subfield code="a">eng</subfield></datafield><datafield tag="082" ind1="0" ind2="4"><subfield code="a">540</subfield><subfield code="q">DE-600</subfield></datafield><datafield tag="084" ind1=" " ind2=" "><subfield code="a">35.18</subfield><subfield code="2">bkl</subfield></datafield><datafield tag="084" ind1=" " ind2=" "><subfield code="a">33.68</subfield><subfield code="2">bkl</subfield></datafield><datafield tag="084" ind1=" " ind2=" "><subfield code="a">52.78</subfield><subfield code="2">bkl</subfield></datafield><datafield tag="084" ind1=" " ind2=" "><subfield code="a">58.20</subfield><subfield code="2">bkl</subfield></datafield><datafield tag="100" ind1="1" ind2=" "><subfield code="a">Liu, Miaomiao</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="245" ind1="1" ind2="0"><subfield code="a">One-pot synthesis of m-Bi</subfield></datafield><datafield tag="264" ind1=" " ind2="1"><subfield code="c">2022</subfield></datafield><datafield tag="336" ind1=" " ind2=" "><subfield code="a">nicht spezifiziert</subfield><subfield code="b">zzz</subfield><subfield code="2">rdacontent</subfield></datafield><datafield tag="337" ind1=" " ind2=" "><subfield code="a">Computermedien</subfield><subfield code="b">c</subfield><subfield code="2">rdamedia</subfield></datafield><datafield tag="338" ind1=" " ind2=" "><subfield code="a">Online-Ressource</subfield><subfield code="b">cr</subfield><subfield code="2">rdacarrier</subfield></datafield><datafield tag="520" ind1=" " ind2=" "><subfield code="a">Developing efficient photocatalysts is critical for degradation of organic pollutants. Herein, a highly efficient heterojunction photocatalyst (m-Bi2O4/Bi2O4−x/BiOCl) was synthesized by a hydrothermal method. Through changing the added volume of concentrated HCl acid, the ternary composite based on BiOCl nanosheets matrix on which the m-Bi2O4 micro-rods and the Bi2O4−x nanospheres are firmly attached. The prepared m-Bi2O4/Bi2O4−x/BiOCl showed a favorable degradation rate and mineralization ability towards Bisphenol A (BPA) and Ciprofloxacin (CIP) under visible light irradiation, which degraded 98.3% of BPA in 30 min, 82.3% of CIP in 80 min, and the rate constants were around 30.16 and 2.82 times higher than that of pure BiOCl, respectively. This enhanced photocatalytic activity of m-Bi2O4/Bi2O4−x/BiOCl composite can be originated from the improved light adsorption range and the synergistic effect of type-II and the Z-scheme charge transfer on the interfaces of m-Bi2O4, Bi2O4−x and BiOCl, which then lead to an accelerated separation and migration of photo-generated carriers. Meanwhile, the photoluminescence (PL) test and photoelectrochemistry (PEC) test provided strong evidence for the construction of the heterojunction. Moreover, the repeatability of m-Bi2O4/Bi2O4−x/BiOCl heterojunction photocatalyst was also investigated, and it still remained 90% photocatalytic activity after four successive cycles. 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author	Liu, Miaomiao
spellingShingle	Liu, Miaomiao ddc 540 bkl 35.18 bkl 33.68 bkl 52.78 bkl 58.20 misc Bi misc Ternary heterojunction misc Photocatalytic activity misc Organic pollutant One-pot synthesis of m-Bi
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topic_title	540 DE-600 35.18 bkl 33.68 bkl 52.78 bkl 58.20 bkl One-pot synthesis of m-Bi Bi Ternary heterojunction Photocatalytic activity Organic pollutant
topic	ddc 540 bkl 35.18 bkl 33.68 bkl 52.78 bkl 58.20 misc Bi misc Ternary heterojunction misc Photocatalytic activity misc Organic pollutant
topic_unstemmed	ddc 540 bkl 35.18 bkl 33.68 bkl 52.78 bkl 58.20 misc Bi misc Ternary heterojunction misc Photocatalytic activity misc Organic pollutant
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title	One-pot synthesis of m-Bi
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title_full	One-pot synthesis of m-Bi
author_sort	Liu, Miaomiao
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author_browse	Liu, Miaomiao Liu, Gang Liu, Xinmei Wang, Xiaoyi Chen, YunLong Yang, Wenlong Gao, Chunpeng Wang, Guanxiang Teng, Zhengchun
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doi_str_mv	10.1016/j.colsurfa.2022.128772
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title_sort	one-pot synthesis of m-bi
title_auth	One-pot synthesis of m-Bi
abstract	Developing efficient photocatalysts is critical for degradation of organic pollutants. Herein, a highly efficient heterojunction photocatalyst (m-Bi2O4/Bi2O4−x/BiOCl) was synthesized by a hydrothermal method. Through changing the added volume of concentrated HCl acid, the ternary composite based on BiOCl nanosheets matrix on which the m-Bi2O4 micro-rods and the Bi2O4−x nanospheres are firmly attached. The prepared m-Bi2O4/Bi2O4−x/BiOCl showed a favorable degradation rate and mineralization ability towards Bisphenol A (BPA) and Ciprofloxacin (CIP) under visible light irradiation, which degraded 98.3% of BPA in 30 min, 82.3% of CIP in 80 min, and the rate constants were around 30.16 and 2.82 times higher than that of pure BiOCl, respectively. This enhanced photocatalytic activity of m-Bi2O4/Bi2O4−x/BiOCl composite can be originated from the improved light adsorption range and the synergistic effect of type-II and the Z-scheme charge transfer on the interfaces of m-Bi2O4, Bi2O4−x and BiOCl, which then lead to an accelerated separation and migration of photo-generated carriers. Meanwhile, the photoluminescence (PL) test and photoelectrochemistry (PEC) test provided strong evidence for the construction of the heterojunction. Moreover, the repeatability of m-Bi2O4/Bi2O4−x/BiOCl heterojunction photocatalyst was also investigated, and it still remained 90% photocatalytic activity after four successive cycles. This work proposed a possible photocatalytic pathway for m-Bi2O4/Bi2O4−x/BiOCl, which would open up a new avenue for water environment treatment utilizing ternary photocatalysts.
abstractGer	Developing efficient photocatalysts is critical for degradation of organic pollutants. Herein, a highly efficient heterojunction photocatalyst (m-Bi2O4/Bi2O4−x/BiOCl) was synthesized by a hydrothermal method. Through changing the added volume of concentrated HCl acid, the ternary composite based on BiOCl nanosheets matrix on which the m-Bi2O4 micro-rods and the Bi2O4−x nanospheres are firmly attached. The prepared m-Bi2O4/Bi2O4−x/BiOCl showed a favorable degradation rate and mineralization ability towards Bisphenol A (BPA) and Ciprofloxacin (CIP) under visible light irradiation, which degraded 98.3% of BPA in 30 min, 82.3% of CIP in 80 min, and the rate constants were around 30.16 and 2.82 times higher than that of pure BiOCl, respectively. This enhanced photocatalytic activity of m-Bi2O4/Bi2O4−x/BiOCl composite can be originated from the improved light adsorption range and the synergistic effect of type-II and the Z-scheme charge transfer on the interfaces of m-Bi2O4, Bi2O4−x and BiOCl, which then lead to an accelerated separation and migration of photo-generated carriers. Meanwhile, the photoluminescence (PL) test and photoelectrochemistry (PEC) test provided strong evidence for the construction of the heterojunction. Moreover, the repeatability of m-Bi2O4/Bi2O4−x/BiOCl heterojunction photocatalyst was also investigated, and it still remained 90% photocatalytic activity after four successive cycles. This work proposed a possible photocatalytic pathway for m-Bi2O4/Bi2O4−x/BiOCl, which would open up a new avenue for water environment treatment utilizing ternary photocatalysts.
abstract_unstemmed	Developing efficient photocatalysts is critical for degradation of organic pollutants. Herein, a highly efficient heterojunction photocatalyst (m-Bi2O4/Bi2O4−x/BiOCl) was synthesized by a hydrothermal method. Through changing the added volume of concentrated HCl acid, the ternary composite based on BiOCl nanosheets matrix on which the m-Bi2O4 micro-rods and the Bi2O4−x nanospheres are firmly attached. The prepared m-Bi2O4/Bi2O4−x/BiOCl showed a favorable degradation rate and mineralization ability towards Bisphenol A (BPA) and Ciprofloxacin (CIP) under visible light irradiation, which degraded 98.3% of BPA in 30 min, 82.3% of CIP in 80 min, and the rate constants were around 30.16 and 2.82 times higher than that of pure BiOCl, respectively. This enhanced photocatalytic activity of m-Bi2O4/Bi2O4−x/BiOCl composite can be originated from the improved light adsorption range and the synergistic effect of type-II and the Z-scheme charge transfer on the interfaces of m-Bi2O4, Bi2O4−x and BiOCl, which then lead to an accelerated separation and migration of photo-generated carriers. Meanwhile, the photoluminescence (PL) test and photoelectrochemistry (PEC) test provided strong evidence for the construction of the heterojunction. Moreover, the repeatability of m-Bi2O4/Bi2O4−x/BiOCl heterojunction photocatalyst was also investigated, and it still remained 90% photocatalytic activity after four successive cycles. This work proposed a possible photocatalytic pathway for m-Bi2O4/Bi2O4−x/BiOCl, which would open up a new avenue for water environment treatment utilizing ternary photocatalysts.
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title_short	One-pot synthesis of m-Bi
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author2	Liu, Gang Liu, Xinmei Wang, Xiaoyi Chen, YunLong Yang, Wenlong Gao, Chunpeng Wang, Guanxiang Teng, Zhengchun
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doi_str	10.1016/j.colsurfa.2022.128772
up_date	2024-07-06T17:02:22.977Z
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fullrecord_marcxml	<?xml version="1.0" encoding="UTF-8"?><collection xmlns="http://www.loc.gov/MARC21/slim"><record><leader>01000caa a22002652 4500</leader><controlfield tag="001">ELV00766236X</controlfield><controlfield tag="003">DE-627</controlfield><controlfield tag="005">20230524152138.0</controlfield><controlfield tag="007">cr uuu---uuuuu</controlfield><controlfield tag="008">230507s2022 xx \|\|\|\|\|o 00\| \|\|eng c</controlfield><datafield tag="024" ind1="7" ind2=" "><subfield code="a">10.1016/j.colsurfa.2022.128772</subfield><subfield code="2">doi</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(DE-627)ELV00766236X</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(ELSEVIER)S0927-7757(22)00527-1</subfield></datafield><datafield tag="040" ind1=" " ind2=" "><subfield code="a">DE-627</subfield><subfield code="b">ger</subfield><subfield code="c">DE-627</subfield><subfield code="e">rda</subfield></datafield><datafield tag="041" ind1=" " ind2=" "><subfield code="a">eng</subfield></datafield><datafield tag="082" ind1="0" ind2="4"><subfield code="a">540</subfield><subfield code="q">DE-600</subfield></datafield><datafield tag="084" ind1=" " ind2=" "><subfield code="a">35.18</subfield><subfield code="2">bkl</subfield></datafield><datafield tag="084" ind1=" " ind2=" "><subfield code="a">33.68</subfield><subfield code="2">bkl</subfield></datafield><datafield tag="084" ind1=" " ind2=" "><subfield code="a">52.78</subfield><subfield code="2">bkl</subfield></datafield><datafield tag="084" ind1=" " ind2=" "><subfield code="a">58.20</subfield><subfield code="2">bkl</subfield></datafield><datafield tag="100" ind1="1" ind2=" "><subfield code="a">Liu, Miaomiao</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="245" ind1="1" ind2="0"><subfield code="a">One-pot synthesis of m-Bi</subfield></datafield><datafield tag="264" ind1=" " ind2="1"><subfield code="c">2022</subfield></datafield><datafield tag="336" ind1=" " ind2=" "><subfield code="a">nicht spezifiziert</subfield><subfield code="b">zzz</subfield><subfield code="2">rdacontent</subfield></datafield><datafield tag="337" ind1=" " ind2=" "><subfield code="a">Computermedien</subfield><subfield code="b">c</subfield><subfield code="2">rdamedia</subfield></datafield><datafield tag="338" ind1=" " ind2=" "><subfield code="a">Online-Ressource</subfield><subfield code="b">cr</subfield><subfield code="2">rdacarrier</subfield></datafield><datafield tag="520" ind1=" " ind2=" "><subfield code="a">Developing efficient photocatalysts is critical for degradation of organic pollutants. Herein, a highly efficient heterojunction photocatalyst (m-Bi2O4/Bi2O4−x/BiOCl) was synthesized by a hydrothermal method. Through changing the added volume of concentrated HCl acid, the ternary composite based on BiOCl nanosheets matrix on which the m-Bi2O4 micro-rods and the Bi2O4−x nanospheres are firmly attached. The prepared m-Bi2O4/Bi2O4−x/BiOCl showed a favorable degradation rate and mineralization ability towards Bisphenol A (BPA) and Ciprofloxacin (CIP) under visible light irradiation, which degraded 98.3% of BPA in 30 min, 82.3% of CIP in 80 min, and the rate constants were around 30.16 and 2.82 times higher than that of pure BiOCl, respectively. This enhanced photocatalytic activity of m-Bi2O4/Bi2O4−x/BiOCl composite can be originated from the improved light adsorption range and the synergistic effect of type-II and the Z-scheme charge transfer on the interfaces of m-Bi2O4, Bi2O4−x and BiOCl, which then lead to an accelerated separation and migration of photo-generated carriers. Meanwhile, the photoluminescence (PL) test and photoelectrochemistry (PEC) test provided strong evidence for the construction of the heterojunction. Moreover, the repeatability of m-Bi2O4/Bi2O4−x/BiOCl heterojunction photocatalyst was also investigated, and it still remained 90% photocatalytic activity after four successive cycles. 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One-pot synthesis of m-Bi

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