Ternary assembled MOF-derived composite: Anisotropic epitaxial growth and microwave absorption

In recent years, metal-organic framework (MOF)-derived absorbers have attracted much attention in the field of microwave absorption. It is interesting and difficult to construct multiple MOF-on-MOF heterostructures. Herein, we combine two unique anisotropic epitaxial growth strategies to build binar...
Ausführliche Beschreibung

Gespeichert in:

Autor*in:	Wu, Fei [verfasserIn] Wan, Lingyun [verfasserIn] Li, Qingyan [verfasserIn] Zhang, Qiuyu [verfasserIn] Zhang, Baoliang [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2022

Schlagwörter:	Anisotropic epitaxial growth MOF Porous materials Magnetic particles Microwave absorption

Übergeordnetes Werk:	Enthalten in: Composites / B - Amsterdam [u.a.] : Elsevier, 1996, 236
Übergeordnetes Werk:	volume:236

DOI / URN:	10.1016/j.compositesb.2022.109839

Katalog-ID:	ELV007808461

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245	1	0	\|a Ternary assembled MOF-derived composite: Anisotropic epitaxial growth and microwave absorption
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520			\|a In recent years, metal-organic framework (MOF)-derived absorbers have attracted much attention in the field of microwave absorption. It is interesting and difficult to construct multiple MOF-on-MOF heterostructures. Herein, we combine two unique anisotropic epitaxial growth strategies to build binary assemblies DUT-52MIL-88B (DM) and DUT-52@MIL-88C (DMC), and then the ternary assembly DUT-52@MIL-88B@MIL-88C (DMM). The formation mechanisms of the assembled structure are clarified. Besides, they are converted into magnetic porous carbon-based absorbers (DM-700 and DMM-700) through a facile carbonization process. The microwave absorption mechanisms are elucidated. The results indicate that the exquisite multi-element composite structure endows the absorber with suitable impedance matching characteristics, complementary loss mechanisms and excellent electromagnetic loss capabilities. It is worth noting that DM-700 exhibits a remarkable minimum reflection loss (RLmin) of −67.5 dB under a matching thickness of 3.6 mm, corresponding to an effective absorption bandwidth (EAB, RL < −10 dB) of 2.0 GHz and the filler loading of 55%. The optimized absorber DMM-700 successfully achieves the optimization of the above-mentioned microwave absorbing properties. While maintaining the desirable RLmin (−56.4 dB), the matching thickness is reduced (2.4 mm), and at the same time, EAB is doubled (4.0 GHz). This study might provide a new idea for the construction of sophisticated absorbers with multi-MOF-on-MOF structures.
650		4	\|a Anisotropic epitaxial growth
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936	b	k	\|a 51.75 \|j Verbundwerkstoffe \|j Schichtstoffe
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Indexfelder

author_variant	f w fw l w lw q l ql q z qz b z bz
matchkey_str	article:18791069:2022----::enrasmldodrvdopstaiorpcptxagot
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publishDate	2022
allfields	10.1016/j.compositesb.2022.109839 doi (DE-627)ELV007808461 (ELSEVIER)S1359-8368(22)00220-7 DE-627 ger DE-627 rda eng 660 DE-600 51.75 bkl Wu, Fei verfasserin aut Ternary assembled MOF-derived composite: Anisotropic epitaxial growth and microwave absorption 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier In recent years, metal-organic framework (MOF)-derived absorbers have attracted much attention in the field of microwave absorption. It is interesting and difficult to construct multiple MOF-on-MOF heterostructures. Herein, we combine two unique anisotropic epitaxial growth strategies to build binary assemblies DUT-52MIL-88B (DM) and DUT-52@MIL-88C (DMC), and then the ternary assembly DUT-52@MIL-88B@MIL-88C (DMM). The formation mechanisms of the assembled structure are clarified. Besides, they are converted into magnetic porous carbon-based absorbers (DM-700 and DMM-700) through a facile carbonization process. The microwave absorption mechanisms are elucidated. The results indicate that the exquisite multi-element composite structure endows the absorber with suitable impedance matching characteristics, complementary loss mechanisms and excellent electromagnetic loss capabilities. It is worth noting that DM-700 exhibits a remarkable minimum reflection loss (RLmin) of −67.5 dB under a matching thickness of 3.6 mm, corresponding to an effective absorption bandwidth (EAB, RL < −10 dB) of 2.0 GHz and the filler loading of 55%. The optimized absorber DMM-700 successfully achieves the optimization of the above-mentioned microwave absorbing properties. While maintaining the desirable RLmin (−56.4 dB), the matching thickness is reduced (2.4 mm), and at the same time, EAB is doubled (4.0 GHz). This study might provide a new idea for the construction of sophisticated absorbers with multi-MOF-on-MOF structures. Anisotropic epitaxial growth MOF Porous materials Magnetic particles Microwave absorption Wan, Lingyun verfasserin aut Li, Qingyan verfasserin aut Zhang, Qiuyu verfasserin aut Zhang, Baoliang verfasserin (orcid)0000-0002-0290-4949 aut Enthalten in Composites / B Amsterdam [u.a.] : Elsevier, 1996 236 Online-Ressource (DE-627)32050235X (DE-600)2012385-1 (DE-576)094531420 1879-1069 nnns volume:236 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 51.75 Verbundwerkstoffe Schichtstoffe AR 236
spelling	10.1016/j.compositesb.2022.109839 doi (DE-627)ELV007808461 (ELSEVIER)S1359-8368(22)00220-7 DE-627 ger DE-627 rda eng 660 DE-600 51.75 bkl Wu, Fei verfasserin aut Ternary assembled MOF-derived composite: Anisotropic epitaxial growth and microwave absorption 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier In recent years, metal-organic framework (MOF)-derived absorbers have attracted much attention in the field of microwave absorption. It is interesting and difficult to construct multiple MOF-on-MOF heterostructures. Herein, we combine two unique anisotropic epitaxial growth strategies to build binary assemblies DUT-52MIL-88B (DM) and DUT-52@MIL-88C (DMC), and then the ternary assembly DUT-52@MIL-88B@MIL-88C (DMM). The formation mechanisms of the assembled structure are clarified. Besides, they are converted into magnetic porous carbon-based absorbers (DM-700 and DMM-700) through a facile carbonization process. The microwave absorption mechanisms are elucidated. The results indicate that the exquisite multi-element composite structure endows the absorber with suitable impedance matching characteristics, complementary loss mechanisms and excellent electromagnetic loss capabilities. It is worth noting that DM-700 exhibits a remarkable minimum reflection loss (RLmin) of −67.5 dB under a matching thickness of 3.6 mm, corresponding to an effective absorption bandwidth (EAB, RL < −10 dB) of 2.0 GHz and the filler loading of 55%. The optimized absorber DMM-700 successfully achieves the optimization of the above-mentioned microwave absorbing properties. While maintaining the desirable RLmin (−56.4 dB), the matching thickness is reduced (2.4 mm), and at the same time, EAB is doubled (4.0 GHz). This study might provide a new idea for the construction of sophisticated absorbers with multi-MOF-on-MOF structures. Anisotropic epitaxial growth MOF Porous materials Magnetic particles Microwave absorption Wan, Lingyun verfasserin aut Li, Qingyan verfasserin aut Zhang, Qiuyu verfasserin aut Zhang, Baoliang verfasserin (orcid)0000-0002-0290-4949 aut Enthalten in Composites / B Amsterdam [u.a.] : Elsevier, 1996 236 Online-Ressource (DE-627)32050235X (DE-600)2012385-1 (DE-576)094531420 1879-1069 nnns volume:236 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 51.75 Verbundwerkstoffe Schichtstoffe AR 236
allfields_unstemmed	10.1016/j.compositesb.2022.109839 doi (DE-627)ELV007808461 (ELSEVIER)S1359-8368(22)00220-7 DE-627 ger DE-627 rda eng 660 DE-600 51.75 bkl Wu, Fei verfasserin aut Ternary assembled MOF-derived composite: Anisotropic epitaxial growth and microwave absorption 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier In recent years, metal-organic framework (MOF)-derived absorbers have attracted much attention in the field of microwave absorption. It is interesting and difficult to construct multiple MOF-on-MOF heterostructures. Herein, we combine two unique anisotropic epitaxial growth strategies to build binary assemblies DUT-52MIL-88B (DM) and DUT-52@MIL-88C (DMC), and then the ternary assembly DUT-52@MIL-88B@MIL-88C (DMM). The formation mechanisms of the assembled structure are clarified. Besides, they are converted into magnetic porous carbon-based absorbers (DM-700 and DMM-700) through a facile carbonization process. The microwave absorption mechanisms are elucidated. The results indicate that the exquisite multi-element composite structure endows the absorber with suitable impedance matching characteristics, complementary loss mechanisms and excellent electromagnetic loss capabilities. It is worth noting that DM-700 exhibits a remarkable minimum reflection loss (RLmin) of −67.5 dB under a matching thickness of 3.6 mm, corresponding to an effective absorption bandwidth (EAB, RL < −10 dB) of 2.0 GHz and the filler loading of 55%. The optimized absorber DMM-700 successfully achieves the optimization of the above-mentioned microwave absorbing properties. While maintaining the desirable RLmin (−56.4 dB), the matching thickness is reduced (2.4 mm), and at the same time, EAB is doubled (4.0 GHz). This study might provide a new idea for the construction of sophisticated absorbers with multi-MOF-on-MOF structures. Anisotropic epitaxial growth MOF Porous materials Magnetic particles Microwave absorption Wan, Lingyun verfasserin aut Li, Qingyan verfasserin aut Zhang, Qiuyu verfasserin aut Zhang, Baoliang verfasserin (orcid)0000-0002-0290-4949 aut Enthalten in Composites / B Amsterdam [u.a.] : Elsevier, 1996 236 Online-Ressource (DE-627)32050235X (DE-600)2012385-1 (DE-576)094531420 1879-1069 nnns volume:236 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 51.75 Verbundwerkstoffe Schichtstoffe AR 236
allfieldsGer	10.1016/j.compositesb.2022.109839 doi (DE-627)ELV007808461 (ELSEVIER)S1359-8368(22)00220-7 DE-627 ger DE-627 rda eng 660 DE-600 51.75 bkl Wu, Fei verfasserin aut Ternary assembled MOF-derived composite: Anisotropic epitaxial growth and microwave absorption 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier In recent years, metal-organic framework (MOF)-derived absorbers have attracted much attention in the field of microwave absorption. It is interesting and difficult to construct multiple MOF-on-MOF heterostructures. Herein, we combine two unique anisotropic epitaxial growth strategies to build binary assemblies DUT-52MIL-88B (DM) and DUT-52@MIL-88C (DMC), and then the ternary assembly DUT-52@MIL-88B@MIL-88C (DMM). The formation mechanisms of the assembled structure are clarified. Besides, they are converted into magnetic porous carbon-based absorbers (DM-700 and DMM-700) through a facile carbonization process. The microwave absorption mechanisms are elucidated. The results indicate that the exquisite multi-element composite structure endows the absorber with suitable impedance matching characteristics, complementary loss mechanisms and excellent electromagnetic loss capabilities. It is worth noting that DM-700 exhibits a remarkable minimum reflection loss (RLmin) of −67.5 dB under a matching thickness of 3.6 mm, corresponding to an effective absorption bandwidth (EAB, RL < −10 dB) of 2.0 GHz and the filler loading of 55%. The optimized absorber DMM-700 successfully achieves the optimization of the above-mentioned microwave absorbing properties. While maintaining the desirable RLmin (−56.4 dB), the matching thickness is reduced (2.4 mm), and at the same time, EAB is doubled (4.0 GHz). This study might provide a new idea for the construction of sophisticated absorbers with multi-MOF-on-MOF structures. Anisotropic epitaxial growth MOF Porous materials Magnetic particles Microwave absorption Wan, Lingyun verfasserin aut Li, Qingyan verfasserin aut Zhang, Qiuyu verfasserin aut Zhang, Baoliang verfasserin (orcid)0000-0002-0290-4949 aut Enthalten in Composites / B Amsterdam [u.a.] : Elsevier, 1996 236 Online-Ressource (DE-627)32050235X (DE-600)2012385-1 (DE-576)094531420 1879-1069 nnns volume:236 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 51.75 Verbundwerkstoffe Schichtstoffe AR 236
allfieldsSound	10.1016/j.compositesb.2022.109839 doi (DE-627)ELV007808461 (ELSEVIER)S1359-8368(22)00220-7 DE-627 ger DE-627 rda eng 660 DE-600 51.75 bkl Wu, Fei verfasserin aut Ternary assembled MOF-derived composite: Anisotropic epitaxial growth and microwave absorption 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier In recent years, metal-organic framework (MOF)-derived absorbers have attracted much attention in the field of microwave absorption. It is interesting and difficult to construct multiple MOF-on-MOF heterostructures. Herein, we combine two unique anisotropic epitaxial growth strategies to build binary assemblies DUT-52MIL-88B (DM) and DUT-52@MIL-88C (DMC), and then the ternary assembly DUT-52@MIL-88B@MIL-88C (DMM). The formation mechanisms of the assembled structure are clarified. Besides, they are converted into magnetic porous carbon-based absorbers (DM-700 and DMM-700) through a facile carbonization process. The microwave absorption mechanisms are elucidated. The results indicate that the exquisite multi-element composite structure endows the absorber with suitable impedance matching characteristics, complementary loss mechanisms and excellent electromagnetic loss capabilities. It is worth noting that DM-700 exhibits a remarkable minimum reflection loss (RLmin) of −67.5 dB under a matching thickness of 3.6 mm, corresponding to an effective absorption bandwidth (EAB, RL < −10 dB) of 2.0 GHz and the filler loading of 55%. The optimized absorber DMM-700 successfully achieves the optimization of the above-mentioned microwave absorbing properties. While maintaining the desirable RLmin (−56.4 dB), the matching thickness is reduced (2.4 mm), and at the same time, EAB is doubled (4.0 GHz). This study might provide a new idea for the construction of sophisticated absorbers with multi-MOF-on-MOF structures. Anisotropic epitaxial growth MOF Porous materials Magnetic particles Microwave absorption Wan, Lingyun verfasserin aut Li, Qingyan verfasserin aut Zhang, Qiuyu verfasserin aut Zhang, Baoliang verfasserin (orcid)0000-0002-0290-4949 aut Enthalten in Composites / B Amsterdam [u.a.] : Elsevier, 1996 236 Online-Ressource (DE-627)32050235X (DE-600)2012385-1 (DE-576)094531420 1879-1069 nnns volume:236 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2008 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 51.75 Verbundwerkstoffe Schichtstoffe AR 236
language	English
source	Enthalten in Composites / B 236 volume:236
sourceStr	Enthalten in Composites / B 236 volume:236
format_phy_str_mv	Article
bklname	Verbundwerkstoffe Schichtstoffe
institution	findex.gbv.de
topic_facet	Anisotropic epitaxial growth MOF Porous materials Magnetic particles Microwave absorption
dewey-raw	660
isfreeaccess_bool	false
container_title	Composites / B
authorswithroles_txt_mv	Wu, Fei @@aut@@ Wan, Lingyun @@aut@@ Li, Qingyan @@aut@@ Zhang, Qiuyu @@aut@@ Zhang, Baoliang @@aut@@
publishDateDaySort_date	2022-01-01T00:00:00Z
hierarchy_top_id	32050235X
dewey-sort	3660
id	ELV007808461
language_de	englisch
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author	Wu, Fei
spellingShingle	Wu, Fei ddc 660 bkl 51.75 misc Anisotropic epitaxial growth misc MOF misc Porous materials misc Magnetic particles misc Microwave absorption Ternary assembled MOF-derived composite: Anisotropic epitaxial growth and microwave absorption
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topic_title	660 DE-600 51.75 bkl Ternary assembled MOF-derived composite: Anisotropic epitaxial growth and microwave absorption Anisotropic epitaxial growth MOF Porous materials Magnetic particles Microwave absorption
topic	ddc 660 bkl 51.75 misc Anisotropic epitaxial growth misc MOF misc Porous materials misc Magnetic particles misc Microwave absorption
topic_unstemmed	ddc 660 bkl 51.75 misc Anisotropic epitaxial growth misc MOF misc Porous materials misc Magnetic particles misc Microwave absorption
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title	Ternary assembled MOF-derived composite: Anisotropic epitaxial growth and microwave absorption
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title_full	Ternary assembled MOF-derived composite: Anisotropic epitaxial growth and microwave absorption
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title_sort	ternary assembled mof-derived composite: anisotropic epitaxial growth and microwave absorption
title_auth	Ternary assembled MOF-derived composite: Anisotropic epitaxial growth and microwave absorption
abstract	In recent years, metal-organic framework (MOF)-derived absorbers have attracted much attention in the field of microwave absorption. It is interesting and difficult to construct multiple MOF-on-MOF heterostructures. Herein, we combine two unique anisotropic epitaxial growth strategies to build binary assemblies DUT-52MIL-88B (DM) and DUT-52@MIL-88C (DMC), and then the ternary assembly DUT-52@MIL-88B@MIL-88C (DMM). The formation mechanisms of the assembled structure are clarified. Besides, they are converted into magnetic porous carbon-based absorbers (DM-700 and DMM-700) through a facile carbonization process. The microwave absorption mechanisms are elucidated. The results indicate that the exquisite multi-element composite structure endows the absorber with suitable impedance matching characteristics, complementary loss mechanisms and excellent electromagnetic loss capabilities. It is worth noting that DM-700 exhibits a remarkable minimum reflection loss (RLmin) of −67.5 dB under a matching thickness of 3.6 mm, corresponding to an effective absorption bandwidth (EAB, RL < −10 dB) of 2.0 GHz and the filler loading of 55%. The optimized absorber DMM-700 successfully achieves the optimization of the above-mentioned microwave absorbing properties. While maintaining the desirable RLmin (−56.4 dB), the matching thickness is reduced (2.4 mm), and at the same time, EAB is doubled (4.0 GHz). This study might provide a new idea for the construction of sophisticated absorbers with multi-MOF-on-MOF structures.
abstractGer	In recent years, metal-organic framework (MOF)-derived absorbers have attracted much attention in the field of microwave absorption. It is interesting and difficult to construct multiple MOF-on-MOF heterostructures. Herein, we combine two unique anisotropic epitaxial growth strategies to build binary assemblies DUT-52MIL-88B (DM) and DUT-52@MIL-88C (DMC), and then the ternary assembly DUT-52@MIL-88B@MIL-88C (DMM). The formation mechanisms of the assembled structure are clarified. Besides, they are converted into magnetic porous carbon-based absorbers (DM-700 and DMM-700) through a facile carbonization process. The microwave absorption mechanisms are elucidated. The results indicate that the exquisite multi-element composite structure endows the absorber with suitable impedance matching characteristics, complementary loss mechanisms and excellent electromagnetic loss capabilities. It is worth noting that DM-700 exhibits a remarkable minimum reflection loss (RLmin) of −67.5 dB under a matching thickness of 3.6 mm, corresponding to an effective absorption bandwidth (EAB, RL < −10 dB) of 2.0 GHz and the filler loading of 55%. The optimized absorber DMM-700 successfully achieves the optimization of the above-mentioned microwave absorbing properties. While maintaining the desirable RLmin (−56.4 dB), the matching thickness is reduced (2.4 mm), and at the same time, EAB is doubled (4.0 GHz). This study might provide a new idea for the construction of sophisticated absorbers with multi-MOF-on-MOF structures.
abstract_unstemmed	In recent years, metal-organic framework (MOF)-derived absorbers have attracted much attention in the field of microwave absorption. It is interesting and difficult to construct multiple MOF-on-MOF heterostructures. Herein, we combine two unique anisotropic epitaxial growth strategies to build binary assemblies DUT-52MIL-88B (DM) and DUT-52@MIL-88C (DMC), and then the ternary assembly DUT-52@MIL-88B@MIL-88C (DMM). The formation mechanisms of the assembled structure are clarified. Besides, they are converted into magnetic porous carbon-based absorbers (DM-700 and DMM-700) through a facile carbonization process. The microwave absorption mechanisms are elucidated. The results indicate that the exquisite multi-element composite structure endows the absorber with suitable impedance matching characteristics, complementary loss mechanisms and excellent electromagnetic loss capabilities. It is worth noting that DM-700 exhibits a remarkable minimum reflection loss (RLmin) of −67.5 dB under a matching thickness of 3.6 mm, corresponding to an effective absorption bandwidth (EAB, RL < −10 dB) of 2.0 GHz and the filler loading of 55%. The optimized absorber DMM-700 successfully achieves the optimization of the above-mentioned microwave absorbing properties. While maintaining the desirable RLmin (−56.4 dB), the matching thickness is reduced (2.4 mm), and at the same time, EAB is doubled (4.0 GHz). This study might provide a new idea for the construction of sophisticated absorbers with multi-MOF-on-MOF structures.
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title_short	Ternary assembled MOF-derived composite: Anisotropic epitaxial growth and microwave absorption
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doi_str	10.1016/j.compositesb.2022.109839
up_date	2024-07-06T17:32:11.361Z
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Ternary assembled MOF-derived composite: Anisotropic epitaxial growth and microwave absorption

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