Comparison of the activation efficiency of peroxymonosulfate on carbon nanotubes modified by carbon nitride vs nitrogen-doping for nonradical degradation of p-hydroxybenzoic acid

The carbon nanotubes (CNT) were modified with graphitic carbon nitride (g-C3N4) for the first time to prepare new metal-free composites for peroxymonosulfate activation. The results showed that the modification of CNT with g-C3N4 significantly enhanced the catalytic performance in activating PMS for...
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Gespeichert in:

Autor*in:	Guo, Zongbao [verfasserIn] Han, Ruirui [verfasserIn] Hao, Zhengran [verfasserIn] Sun, Ping [verfasserIn] Zhai, Zhicai [verfasserIn] Fang, Yingsen [verfasserIn] Liu, Hui [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2022

Schlagwörter:	Metal-free catalysts Graphitic carbon nitride-modified carbon nanotubes Peroxymonosulfate Non-radical activation Singlet oxygen

Übergeordnetes Werk:	Enthalten in: No title available - 171
Übergeordnetes Werk:	volume:171

DOI / URN:	10.1016/j.catcom.2022.106506

Katalog-ID:	ELV008612099

Internformat


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024	7		\|a 10.1016/j.catcom.2022.106506 \|2 doi
035			\|a (DE-627)ELV008612099
035			\|a (ELSEVIER)S1566-7367(22)00111-X
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041			\|a eng
100	1		\|a Guo, Zongbao \|e verfasserin \|4 aut
245	1	0	\|a Comparison of the activation efficiency of peroxymonosulfate on carbon nanotubes modified by carbon nitride vs nitrogen-doping for nonradical degradation of p-hydroxybenzoic acid
264		1	\|c 2022
336			\|a nicht spezifiziert \|b zzz \|2 rdacontent
337			\|a Computermedien \|b c \|2 rdamedia
338			\|a Online-Ressource \|b cr \|2 rdacarrier
520			\|a The carbon nanotubes (CNT) were modified with graphitic carbon nitride (g-C3N4) for the first time to prepare new metal-free composites for peroxymonosulfate activation. The results showed that the modification of CNT with g-C3N4 significantly enhanced the catalytic performance in activating PMS for the degradation of p-hydroxybenzoic acid (HBA)than the traditional N doping. Moreover, the oxidation system was not affected by the water quality factors (e.g., Cl−, NO3 −, HCO3 −, and humic acid) as it had a high pollutant mineralization rate with the removal of total organic carbon (TOC) was ≈72%, and could effectively remove other pollutants (e.g., ferulic acid, methylparaben, phenol, and paracetamol). The singlet oxygen was the main active species involved in the reaction, indicating that HBA degradation mainly depended on non-free radical oxidation mechanisms.
650		4	\|a Metal-free catalysts
650		4	\|a Graphitic carbon nitride-modified carbon nanotubes
650		4	\|a Peroxymonosulfate
650		4	\|a Non-radical activation
650		4	\|a Singlet oxygen
700	1		\|a Han, Ruirui \|e verfasserin \|4 aut
700	1		\|a Hao, Zhengran \|e verfasserin \|4 aut
700	1		\|a Sun, Ping \|e verfasserin \|4 aut
700	1		\|a Zhai, Zhicai \|e verfasserin \|4 aut
700	1		\|a Fang, Yingsen \|e verfasserin \|4 aut
700	1		\|a Liu, Hui \|e verfasserin \|4 aut
773	0	8	\|i Enthalten in \|t No title available \|g 171 \|w (DE-627)32578910X \|x 1566-7367 \|7 nnns
773	1	8	\|g volume:171
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912			\|a GBV_ILN_23
912			\|a GBV_ILN_24
912			\|a GBV_ILN_31
912			\|a GBV_ILN_39
912			\|a GBV_ILN_40
912			\|a GBV_ILN_60
912			\|a GBV_ILN_62
912			\|a GBV_ILN_63
912			\|a GBV_ILN_65
912			\|a GBV_ILN_69
912			\|a GBV_ILN_70
912			\|a GBV_ILN_73
912			\|a GBV_ILN_95
912			\|a GBV_ILN_105
912			\|a GBV_ILN_110
912			\|a GBV_ILN_151
912			\|a GBV_ILN_161
912			\|a GBV_ILN_170
912			\|a GBV_ILN_213
912			\|a GBV_ILN_224
912			\|a GBV_ILN_230
912			\|a GBV_ILN_285
912			\|a GBV_ILN_293
912			\|a GBV_ILN_602
912			\|a GBV_ILN_2001
912			\|a GBV_ILN_2003
912			\|a GBV_ILN_2004
912			\|a GBV_ILN_2005
912			\|a GBV_ILN_2007
912			\|a GBV_ILN_2008
912			\|a GBV_ILN_2009
912			\|a GBV_ILN_2010
912			\|a GBV_ILN_2011
912			\|a GBV_ILN_2014
912			\|a GBV_ILN_2015
912			\|a GBV_ILN_2020
912			\|a GBV_ILN_2021
912			\|a GBV_ILN_2025
912			\|a GBV_ILN_2026
912			\|a GBV_ILN_2027
912			\|a GBV_ILN_2031
912			\|a GBV_ILN_2034
912			\|a GBV_ILN_2038
912			\|a GBV_ILN_2044
912			\|a GBV_ILN_2048
912			\|a GBV_ILN_2049
912			\|a GBV_ILN_2050
912			\|a GBV_ILN_2055
912			\|a GBV_ILN_2056
912			\|a GBV_ILN_2059
912			\|a GBV_ILN_2061
912			\|a GBV_ILN_2064
912			\|a GBV_ILN_2065
912			\|a GBV_ILN_2068
912			\|a GBV_ILN_2088
912			\|a GBV_ILN_2106
912			\|a GBV_ILN_2110
912			\|a GBV_ILN_2111
912			\|a GBV_ILN_2112
912			\|a GBV_ILN_2118
912			\|a GBV_ILN_2122
912			\|a GBV_ILN_2129
912			\|a GBV_ILN_2143
912			\|a GBV_ILN_2147
912			\|a GBV_ILN_2148
912			\|a GBV_ILN_2152
912			\|a GBV_ILN_2153
912			\|a GBV_ILN_2190
912			\|a GBV_ILN_2232
912			\|a GBV_ILN_2336
912			\|a GBV_ILN_2470
912			\|a GBV_ILN_2507
912			\|a GBV_ILN_2548
912			\|a GBV_ILN_4012
912			\|a GBV_ILN_4035
912			\|a GBV_ILN_4037
912			\|a GBV_ILN_4046
912			\|a GBV_ILN_4112
912			\|a GBV_ILN_4125
912			\|a GBV_ILN_4126
912			\|a GBV_ILN_4242
912			\|a GBV_ILN_4249
912			\|a GBV_ILN_4251
912			\|a GBV_ILN_4305
912			\|a GBV_ILN_4306
912			\|a GBV_ILN_4307
912			\|a GBV_ILN_4313
912			\|a GBV_ILN_4322
912			\|a GBV_ILN_4323
912			\|a GBV_ILN_4324
912			\|a GBV_ILN_4325
912			\|a GBV_ILN_4326
912			\|a GBV_ILN_4333
912			\|a GBV_ILN_4334
912			\|a GBV_ILN_4338
912			\|a GBV_ILN_4367
912			\|a GBV_ILN_4393
912			\|a GBV_ILN_4700
951			\|a AR
952			\|d 171

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publishDate	2022
allfields	10.1016/j.catcom.2022.106506 doi (DE-627)ELV008612099 (ELSEVIER)S1566-7367(22)00111-X DE-627 ger DE-627 rda eng Guo, Zongbao verfasserin aut Comparison of the activation efficiency of peroxymonosulfate on carbon nanotubes modified by carbon nitride vs nitrogen-doping for nonradical degradation of p-hydroxybenzoic acid 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The carbon nanotubes (CNT) were modified with graphitic carbon nitride (g-C3N4) for the first time to prepare new metal-free composites for peroxymonosulfate activation. The results showed that the modification of CNT with g-C3N4 significantly enhanced the catalytic performance in activating PMS for the degradation of p-hydroxybenzoic acid (HBA)than the traditional N doping. Moreover, the oxidation system was not affected by the water quality factors (e.g., Cl−, NO3 −, HCO3 −, and humic acid) as it had a high pollutant mineralization rate with the removal of total organic carbon (TOC) was ≈72%, and could effectively remove other pollutants (e.g., ferulic acid, methylparaben, phenol, and paracetamol). The singlet oxygen was the main active species involved in the reaction, indicating that HBA degradation mainly depended on non-free radical oxidation mechanisms. Metal-free catalysts Graphitic carbon nitride-modified carbon nanotubes Peroxymonosulfate Non-radical activation Singlet oxygen Han, Ruirui verfasserin aut Hao, Zhengran verfasserin aut Sun, Ping verfasserin aut Zhai, Zhicai verfasserin aut Fang, Yingsen verfasserin aut Liu, Hui verfasserin aut Enthalten in No title available 171 (DE-627)32578910X 1566-7367 nnns volume:171 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_602 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 171
spelling	10.1016/j.catcom.2022.106506 doi (DE-627)ELV008612099 (ELSEVIER)S1566-7367(22)00111-X DE-627 ger DE-627 rda eng Guo, Zongbao verfasserin aut Comparison of the activation efficiency of peroxymonosulfate on carbon nanotubes modified by carbon nitride vs nitrogen-doping for nonradical degradation of p-hydroxybenzoic acid 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The carbon nanotubes (CNT) were modified with graphitic carbon nitride (g-C3N4) for the first time to prepare new metal-free composites for peroxymonosulfate activation. The results showed that the modification of CNT with g-C3N4 significantly enhanced the catalytic performance in activating PMS for the degradation of p-hydroxybenzoic acid (HBA)than the traditional N doping. Moreover, the oxidation system was not affected by the water quality factors (e.g., Cl−, NO3 −, HCO3 −, and humic acid) as it had a high pollutant mineralization rate with the removal of total organic carbon (TOC) was ≈72%, and could effectively remove other pollutants (e.g., ferulic acid, methylparaben, phenol, and paracetamol). The singlet oxygen was the main active species involved in the reaction, indicating that HBA degradation mainly depended on non-free radical oxidation mechanisms. Metal-free catalysts Graphitic carbon nitride-modified carbon nanotubes Peroxymonosulfate Non-radical activation Singlet oxygen Han, Ruirui verfasserin aut Hao, Zhengran verfasserin aut Sun, Ping verfasserin aut Zhai, Zhicai verfasserin aut Fang, Yingsen verfasserin aut Liu, Hui verfasserin aut Enthalten in No title available 171 (DE-627)32578910X 1566-7367 nnns volume:171 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_602 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 171
allfields_unstemmed	10.1016/j.catcom.2022.106506 doi (DE-627)ELV008612099 (ELSEVIER)S1566-7367(22)00111-X DE-627 ger DE-627 rda eng Guo, Zongbao verfasserin aut Comparison of the activation efficiency of peroxymonosulfate on carbon nanotubes modified by carbon nitride vs nitrogen-doping for nonradical degradation of p-hydroxybenzoic acid 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The carbon nanotubes (CNT) were modified with graphitic carbon nitride (g-C3N4) for the first time to prepare new metal-free composites for peroxymonosulfate activation. The results showed that the modification of CNT with g-C3N4 significantly enhanced the catalytic performance in activating PMS for the degradation of p-hydroxybenzoic acid (HBA)than the traditional N doping. Moreover, the oxidation system was not affected by the water quality factors (e.g., Cl−, NO3 −, HCO3 −, and humic acid) as it had a high pollutant mineralization rate with the removal of total organic carbon (TOC) was ≈72%, and could effectively remove other pollutants (e.g., ferulic acid, methylparaben, phenol, and paracetamol). The singlet oxygen was the main active species involved in the reaction, indicating that HBA degradation mainly depended on non-free radical oxidation mechanisms. Metal-free catalysts Graphitic carbon nitride-modified carbon nanotubes Peroxymonosulfate Non-radical activation Singlet oxygen Han, Ruirui verfasserin aut Hao, Zhengran verfasserin aut Sun, Ping verfasserin aut Zhai, Zhicai verfasserin aut Fang, Yingsen verfasserin aut Liu, Hui verfasserin aut Enthalten in No title available 171 (DE-627)32578910X 1566-7367 nnns volume:171 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_602 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 171
allfieldsGer	10.1016/j.catcom.2022.106506 doi (DE-627)ELV008612099 (ELSEVIER)S1566-7367(22)00111-X DE-627 ger DE-627 rda eng Guo, Zongbao verfasserin aut Comparison of the activation efficiency of peroxymonosulfate on carbon nanotubes modified by carbon nitride vs nitrogen-doping for nonradical degradation of p-hydroxybenzoic acid 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The carbon nanotubes (CNT) were modified with graphitic carbon nitride (g-C3N4) for the first time to prepare new metal-free composites for peroxymonosulfate activation. The results showed that the modification of CNT with g-C3N4 significantly enhanced the catalytic performance in activating PMS for the degradation of p-hydroxybenzoic acid (HBA)than the traditional N doping. Moreover, the oxidation system was not affected by the water quality factors (e.g., Cl−, NO3 −, HCO3 −, and humic acid) as it had a high pollutant mineralization rate with the removal of total organic carbon (TOC) was ≈72%, and could effectively remove other pollutants (e.g., ferulic acid, methylparaben, phenol, and paracetamol). The singlet oxygen was the main active species involved in the reaction, indicating that HBA degradation mainly depended on non-free radical oxidation mechanisms. Metal-free catalysts Graphitic carbon nitride-modified carbon nanotubes Peroxymonosulfate Non-radical activation Singlet oxygen Han, Ruirui verfasserin aut Hao, Zhengran verfasserin aut Sun, Ping verfasserin aut Zhai, Zhicai verfasserin aut Fang, Yingsen verfasserin aut Liu, Hui verfasserin aut Enthalten in No title available 171 (DE-627)32578910X 1566-7367 nnns volume:171 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_602 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 171
allfieldsSound	10.1016/j.catcom.2022.106506 doi (DE-627)ELV008612099 (ELSEVIER)S1566-7367(22)00111-X DE-627 ger DE-627 rda eng Guo, Zongbao verfasserin aut Comparison of the activation efficiency of peroxymonosulfate on carbon nanotubes modified by carbon nitride vs nitrogen-doping for nonradical degradation of p-hydroxybenzoic acid 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The carbon nanotubes (CNT) were modified with graphitic carbon nitride (g-C3N4) for the first time to prepare new metal-free composites for peroxymonosulfate activation. The results showed that the modification of CNT with g-C3N4 significantly enhanced the catalytic performance in activating PMS for the degradation of p-hydroxybenzoic acid (HBA)than the traditional N doping. Moreover, the oxidation system was not affected by the water quality factors (e.g., Cl−, NO3 −, HCO3 −, and humic acid) as it had a high pollutant mineralization rate with the removal of total organic carbon (TOC) was ≈72%, and could effectively remove other pollutants (e.g., ferulic acid, methylparaben, phenol, and paracetamol). The singlet oxygen was the main active species involved in the reaction, indicating that HBA degradation mainly depended on non-free radical oxidation mechanisms. Metal-free catalysts Graphitic carbon nitride-modified carbon nanotubes Peroxymonosulfate Non-radical activation Singlet oxygen Han, Ruirui verfasserin aut Hao, Zhengran verfasserin aut Sun, Ping verfasserin aut Zhai, Zhicai verfasserin aut Fang, Yingsen verfasserin aut Liu, Hui verfasserin aut Enthalten in No title available 171 (DE-627)32578910X 1566-7367 nnns volume:171 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_170 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_602 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2548 GBV_ILN_4012 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4393 GBV_ILN_4700 AR 171
language	English
source	Enthalten in No title available 171 volume:171
sourceStr	Enthalten in No title available 171 volume:171
format_phy_str_mv	Article
institution	findex.gbv.de
topic_facet	Metal-free catalysts Graphitic carbon nitride-modified carbon nanotubes Peroxymonosulfate Non-radical activation Singlet oxygen
isfreeaccess_bool	false
container_title	No title available
authorswithroles_txt_mv	Guo, Zongbao @@aut@@ Han, Ruirui @@aut@@ Hao, Zhengran @@aut@@ Sun, Ping @@aut@@ Zhai, Zhicai @@aut@@ Fang, Yingsen @@aut@@ Liu, Hui @@aut@@
publishDateDaySort_date	2022-01-01T00:00:00Z
hierarchy_top_id	32578910X
id	ELV008612099
language_de	englisch
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author	Guo, Zongbao
spellingShingle	Guo, Zongbao misc Metal-free catalysts misc Graphitic carbon nitride-modified carbon nanotubes misc Peroxymonosulfate misc Non-radical activation misc Singlet oxygen Comparison of the activation efficiency of peroxymonosulfate on carbon nanotubes modified by carbon nitride vs nitrogen-doping for nonradical degradation of p-hydroxybenzoic acid
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topic_title	Comparison of the activation efficiency of peroxymonosulfate on carbon nanotubes modified by carbon nitride vs nitrogen-doping for nonradical degradation of p-hydroxybenzoic acid Metal-free catalysts Graphitic carbon nitride-modified carbon nanotubes Peroxymonosulfate Non-radical activation Singlet oxygen
topic	misc Metal-free catalysts misc Graphitic carbon nitride-modified carbon nanotubes misc Peroxymonosulfate misc Non-radical activation misc Singlet oxygen
topic_unstemmed	misc Metal-free catalysts misc Graphitic carbon nitride-modified carbon nanotubes misc Peroxymonosulfate misc Non-radical activation misc Singlet oxygen
topic_browse	misc Metal-free catalysts misc Graphitic carbon nitride-modified carbon nanotubes misc Peroxymonosulfate misc Non-radical activation misc Singlet oxygen
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title	Comparison of the activation efficiency of peroxymonosulfate on carbon nanotubes modified by carbon nitride vs nitrogen-doping for nonradical degradation of p-hydroxybenzoic acid
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title_full	Comparison of the activation efficiency of peroxymonosulfate on carbon nanotubes modified by carbon nitride vs nitrogen-doping for nonradical degradation of p-hydroxybenzoic acid
author_sort	Guo, Zongbao
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author_browse	Guo, Zongbao Han, Ruirui Hao, Zhengran Sun, Ping Zhai, Zhicai Fang, Yingsen Liu, Hui
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author-letter	Guo, Zongbao
doi_str_mv	10.1016/j.catcom.2022.106506
author2-role	verfasserin
title_sort	comparison of the activation efficiency of peroxymonosulfate on carbon nanotubes modified by carbon nitride vs nitrogen-doping for nonradical degradation of p-hydroxybenzoic acid
title_auth	Comparison of the activation efficiency of peroxymonosulfate on carbon nanotubes modified by carbon nitride vs nitrogen-doping for nonradical degradation of p-hydroxybenzoic acid
abstract	The carbon nanotubes (CNT) were modified with graphitic carbon nitride (g-C3N4) for the first time to prepare new metal-free composites for peroxymonosulfate activation. The results showed that the modification of CNT with g-C3N4 significantly enhanced the catalytic performance in activating PMS for the degradation of p-hydroxybenzoic acid (HBA)than the traditional N doping. Moreover, the oxidation system was not affected by the water quality factors (e.g., Cl−, NO3 −, HCO3 −, and humic acid) as it had a high pollutant mineralization rate with the removal of total organic carbon (TOC) was ≈72%, and could effectively remove other pollutants (e.g., ferulic acid, methylparaben, phenol, and paracetamol). The singlet oxygen was the main active species involved in the reaction, indicating that HBA degradation mainly depended on non-free radical oxidation mechanisms.
abstractGer	The carbon nanotubes (CNT) were modified with graphitic carbon nitride (g-C3N4) for the first time to prepare new metal-free composites for peroxymonosulfate activation. The results showed that the modification of CNT with g-C3N4 significantly enhanced the catalytic performance in activating PMS for the degradation of p-hydroxybenzoic acid (HBA)than the traditional N doping. Moreover, the oxidation system was not affected by the water quality factors (e.g., Cl−, NO3 −, HCO3 −, and humic acid) as it had a high pollutant mineralization rate with the removal of total organic carbon (TOC) was ≈72%, and could effectively remove other pollutants (e.g., ferulic acid, methylparaben, phenol, and paracetamol). The singlet oxygen was the main active species involved in the reaction, indicating that HBA degradation mainly depended on non-free radical oxidation mechanisms.
abstract_unstemmed	The carbon nanotubes (CNT) were modified with graphitic carbon nitride (g-C3N4) for the first time to prepare new metal-free composites for peroxymonosulfate activation. The results showed that the modification of CNT with g-C3N4 significantly enhanced the catalytic performance in activating PMS for the degradation of p-hydroxybenzoic acid (HBA)than the traditional N doping. Moreover, the oxidation system was not affected by the water quality factors (e.g., Cl−, NO3 −, HCO3 −, and humic acid) as it had a high pollutant mineralization rate with the removal of total organic carbon (TOC) was ≈72%, and could effectively remove other pollutants (e.g., ferulic acid, methylparaben, phenol, and paracetamol). The singlet oxygen was the main active species involved in the reaction, indicating that HBA degradation mainly depended on non-free radical oxidation mechanisms.
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title_short	Comparison of the activation efficiency of peroxymonosulfate on carbon nanotubes modified by carbon nitride vs nitrogen-doping for nonradical degradation of p-hydroxybenzoic acid
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author2	Han, Ruirui Hao, Zhengran Sun, Ping Zhai, Zhicai Fang, Yingsen Liu, Hui
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doi_str	10.1016/j.catcom.2022.106506
up_date	2024-07-06T20:18:03.925Z
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Comparison of the activation efficiency of peroxymonosulfate on carbon nanotubes modified by carbon nitride vs nitrogen-doping for nonradical degradation of p-hydroxybenzoic acid

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