Zeolitic imidazolate framework-67 derived Al-Co-S hierarchical sheets bridged by nitrogen-doped graphene: Incorporation of PANI derived carbon nanorods for solid-state asymmetric supercapacitors

Metal sulfides have been widely enticed as battery-type electrodes in supercapacitor devices because of their maximal theoretical capacitance. Nevertheless, their lower conductivity and ion transport kinetics can largely restrict their rate performance, hence the practical usage in fields of demanding high power devices. Therefore, the design of new electrodes with higher energy and power densities remains a highly challenging task. To the best of our knowledge, a novel hierarchical composite of Al-CoS2 on nitrogen-doped graphene (NG) is prepared based on a zeolite imidazole framework using a simple and scalable hydrothermal process. In this hybrid, ultrathin Al-CoS2 nanosheet arrays are vertically orientated on the NG framework to limit self-aggregation, hence increasing the electrical property and cycle stability of composite. It is investigated that the Al/Co feeding ratio plays a crucial role in controlling the obtained hierarchical structure of Al-Co-S sheets and their electrode performance. Also, Al3+ can influence remarkably the morphology and electrochemical property of the resultant graphene composite. An effective synergism is noticed between the redox Al-CoS2 and NG resulting in fast electron transfer and charging-discharging processes. Surprisingly, when the as-developed composite is utilized as a positive electrode at an applied current density of 1 A/g, a specific capacitance of 1915.8 F/g is attained with ultra-long cycle stability (96%, 10,000 cycles) and an excellent retention rate (∼89%). As a consequence, when a solid-state asymmetric supercapacitor (ASC) device is made by combining an Al-CoS2NG hybrid with a negative electrode made of polyaniline (PANI) derived carbon nanorods (PCNRs), it demonstrates remarkable specific capacitance (188 F/g), energy density (66.9 Wh/kg), and cyclic stability of 92% after 10,000 cycles. This may open the pathway for the application of the next-generation supercapacitors in the future. Ausführliche Beschreibung

Gespeichert in:

Autor*in:	Goda, Emad S. [verfasserIn] Pandit, Bidhan [verfasserIn] Hong, Sang Eun [verfasserIn] Singu, Bal Sydulu [verfasserIn] Kim, Seong K. [verfasserIn] Moustafa, Essam B. [verfasserIn] Yoon, Kuk Ro [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2022

Schlagwörter:	Hierarchical sheets MOFs Al-doped CoS Nitrogen-doped graphene Solid-state supercapacitor

Übergeordnetes Werk:	Enthalten in: Journal of Energy Chemistry - Amsterdam [u.a.] : Elsevier, 2013, 74, Seite 429-445
Übergeordnetes Werk:	volume:74 ; pages:429-445

DOI / URN:	10.1016/j.jechem.2022.07.033

Katalog-ID:	ELV008636826

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245	1	0	\|a Zeolitic imidazolate framework-67 derived Al-Co-S hierarchical sheets bridged by nitrogen-doped graphene: Incorporation of PANI derived carbon nanorods for solid-state asymmetric supercapacitors
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520			\|a Metal sulfides have been widely enticed as battery-type electrodes in supercapacitor devices because of their maximal theoretical capacitance. Nevertheless, their lower conductivity and ion transport kinetics can largely restrict their rate performance, hence the practical usage in fields of demanding high power devices. Therefore, the design of new electrodes with higher energy and power densities remains a highly challenging task. To the best of our knowledge, a novel hierarchical composite of Al-CoS2 on nitrogen-doped graphene (NG) is prepared based on a zeolite imidazole framework using a simple and scalable hydrothermal process. In this hybrid, ultrathin Al-CoS2 nanosheet arrays are vertically orientated on the NG framework to limit self-aggregation, hence increasing the electrical property and cycle stability of composite. It is investigated that the Al/Co feeding ratio plays a crucial role in controlling the obtained hierarchical structure of Al-Co-S sheets and their electrode performance. Also, Al3+ can influence remarkably the morphology and electrochemical property of the resultant graphene composite. An effective synergism is noticed between the redox Al-CoS2 and NG resulting in fast electron transfer and charging-discharging processes. Surprisingly, when the as-developed composite is utilized as a positive electrode at an applied current density of 1 A/g, a specific capacitance of 1915.8 F/g is attained with ultra-long cycle stability (96%, 10,000 cycles) and an excellent retention rate (∼89%). As a consequence, when a solid-state asymmetric supercapacitor (ASC) device is made by combining an Al-CoS2NG hybrid with a negative electrode made of polyaniline (PANI) derived carbon nanorods (PCNRs), it demonstrates remarkable specific capacitance (188 F/g), energy density (66.9 Wh/kg), and cyclic stability of 92% after 10,000 cycles. This may open the pathway for the application of the next-generation supercapacitors in the future.
650		4	\|a Hierarchical sheets
650		4	\|a MOFs
650		4	\|a Al-doped CoS
650		4	\|a Nitrogen-doped graphene
650		4	\|a Solid-state supercapacitor
700	1		\|a Pandit, Bidhan \|e verfasserin \|4 aut
700	1		\|a Hong, Sang Eun \|e verfasserin \|4 aut
700	1		\|a Singu, Bal Sydulu \|e verfasserin \|4 aut
700	1		\|a Kim, Seong K. \|e verfasserin \|4 aut
700	1		\|a Moustafa, Essam B. \|e verfasserin \|4 aut
700	1		\|a Yoon, Kuk Ro \|e verfasserin \|4 aut
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allfields	10.1016/j.jechem.2022.07.033 doi (DE-627)ELV008636826 (ELSEVIER)S2095-4956(22)00410-7 DE-627 ger DE-627 rda eng 540 DE-600 Goda, Emad S. verfasserin aut Zeolitic imidazolate framework-67 derived Al-Co-S hierarchical sheets bridged by nitrogen-doped graphene: Incorporation of PANI derived carbon nanorods for solid-state asymmetric supercapacitors 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Metal sulfides have been widely enticed as battery-type electrodes in supercapacitor devices because of their maximal theoretical capacitance. Nevertheless, their lower conductivity and ion transport kinetics can largely restrict their rate performance, hence the practical usage in fields of demanding high power devices. Therefore, the design of new electrodes with higher energy and power densities remains a highly challenging task. To the best of our knowledge, a novel hierarchical composite of Al-CoS2 on nitrogen-doped graphene (NG) is prepared based on a zeolite imidazole framework using a simple and scalable hydrothermal process. In this hybrid, ultrathin Al-CoS2 nanosheet arrays are vertically orientated on the NG framework to limit self-aggregation, hence increasing the electrical property and cycle stability of composite. It is investigated that the Al/Co feeding ratio plays a crucial role in controlling the obtained hierarchical structure of Al-Co-S sheets and their electrode performance. Also, Al3+ can influence remarkably the morphology and electrochemical property of the resultant graphene composite. An effective synergism is noticed between the redox Al-CoS2 and NG resulting in fast electron transfer and charging-discharging processes. Surprisingly, when the as-developed composite is utilized as a positive electrode at an applied current density of 1 A/g, a specific capacitance of 1915.8 F/g is attained with ultra-long cycle stability (96%, 10,000 cycles) and an excellent retention rate (∼89%). As a consequence, when a solid-state asymmetric supercapacitor (ASC) device is made by combining an Al-CoS2NG hybrid with a negative electrode made of polyaniline (PANI) derived carbon nanorods (PCNRs), it demonstrates remarkable specific capacitance (188 F/g), energy density (66.9 Wh/kg), and cyclic stability of 92% after 10,000 cycles. This may open the pathway for the application of the next-generation supercapacitors in the future. Hierarchical sheets MOFs Al-doped CoS Nitrogen-doped graphene Solid-state supercapacitor Pandit, Bidhan verfasserin aut Hong, Sang Eun verfasserin aut Singu, Bal Sydulu verfasserin aut Kim, Seong K. verfasserin aut Moustafa, Essam B. verfasserin aut Yoon, Kuk Ro verfasserin aut Enthalten in Journal of Energy Chemistry Amsterdam [u.a.] : Elsevier, 2013 74, Seite 429-445 Online-Ressource (DE-627)745616399 (DE-600)2714311-9 (DE-576)382032861 2096-885X nnns volume:74 pages:429-445 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 AR 74 429-445
spelling	10.1016/j.jechem.2022.07.033 doi (DE-627)ELV008636826 (ELSEVIER)S2095-4956(22)00410-7 DE-627 ger DE-627 rda eng 540 DE-600 Goda, Emad S. verfasserin aut Zeolitic imidazolate framework-67 derived Al-Co-S hierarchical sheets bridged by nitrogen-doped graphene: Incorporation of PANI derived carbon nanorods for solid-state asymmetric supercapacitors 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Metal sulfides have been widely enticed as battery-type electrodes in supercapacitor devices because of their maximal theoretical capacitance. Nevertheless, their lower conductivity and ion transport kinetics can largely restrict their rate performance, hence the practical usage in fields of demanding high power devices. Therefore, the design of new electrodes with higher energy and power densities remains a highly challenging task. To the best of our knowledge, a novel hierarchical composite of Al-CoS2 on nitrogen-doped graphene (NG) is prepared based on a zeolite imidazole framework using a simple and scalable hydrothermal process. In this hybrid, ultrathin Al-CoS2 nanosheet arrays are vertically orientated on the NG framework to limit self-aggregation, hence increasing the electrical property and cycle stability of composite. It is investigated that the Al/Co feeding ratio plays a crucial role in controlling the obtained hierarchical structure of Al-Co-S sheets and their electrode performance. Also, Al3+ can influence remarkably the morphology and electrochemical property of the resultant graphene composite. An effective synergism is noticed between the redox Al-CoS2 and NG resulting in fast electron transfer and charging-discharging processes. Surprisingly, when the as-developed composite is utilized as a positive electrode at an applied current density of 1 A/g, a specific capacitance of 1915.8 F/g is attained with ultra-long cycle stability (96%, 10,000 cycles) and an excellent retention rate (∼89%). As a consequence, when a solid-state asymmetric supercapacitor (ASC) device is made by combining an Al-CoS2NG hybrid with a negative electrode made of polyaniline (PANI) derived carbon nanorods (PCNRs), it demonstrates remarkable specific capacitance (188 F/g), energy density (66.9 Wh/kg), and cyclic stability of 92% after 10,000 cycles. This may open the pathway for the application of the next-generation supercapacitors in the future. Hierarchical sheets MOFs Al-doped CoS Nitrogen-doped graphene Solid-state supercapacitor Pandit, Bidhan verfasserin aut Hong, Sang Eun verfasserin aut Singu, Bal Sydulu verfasserin aut Kim, Seong K. verfasserin aut Moustafa, Essam B. verfasserin aut Yoon, Kuk Ro verfasserin aut Enthalten in Journal of Energy Chemistry Amsterdam [u.a.] : Elsevier, 2013 74, Seite 429-445 Online-Ressource (DE-627)745616399 (DE-600)2714311-9 (DE-576)382032861 2096-885X nnns volume:74 pages:429-445 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 AR 74 429-445
allfields_unstemmed	10.1016/j.jechem.2022.07.033 doi (DE-627)ELV008636826 (ELSEVIER)S2095-4956(22)00410-7 DE-627 ger DE-627 rda eng 540 DE-600 Goda, Emad S. verfasserin aut Zeolitic imidazolate framework-67 derived Al-Co-S hierarchical sheets bridged by nitrogen-doped graphene: Incorporation of PANI derived carbon nanorods for solid-state asymmetric supercapacitors 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Metal sulfides have been widely enticed as battery-type electrodes in supercapacitor devices because of their maximal theoretical capacitance. Nevertheless, their lower conductivity and ion transport kinetics can largely restrict their rate performance, hence the practical usage in fields of demanding high power devices. Therefore, the design of new electrodes with higher energy and power densities remains a highly challenging task. To the best of our knowledge, a novel hierarchical composite of Al-CoS2 on nitrogen-doped graphene (NG) is prepared based on a zeolite imidazole framework using a simple and scalable hydrothermal process. In this hybrid, ultrathin Al-CoS2 nanosheet arrays are vertically orientated on the NG framework to limit self-aggregation, hence increasing the electrical property and cycle stability of composite. It is investigated that the Al/Co feeding ratio plays a crucial role in controlling the obtained hierarchical structure of Al-Co-S sheets and their electrode performance. Also, Al3+ can influence remarkably the morphology and electrochemical property of the resultant graphene composite. An effective synergism is noticed between the redox Al-CoS2 and NG resulting in fast electron transfer and charging-discharging processes. Surprisingly, when the as-developed composite is utilized as a positive electrode at an applied current density of 1 A/g, a specific capacitance of 1915.8 F/g is attained with ultra-long cycle stability (96%, 10,000 cycles) and an excellent retention rate (∼89%). As a consequence, when a solid-state asymmetric supercapacitor (ASC) device is made by combining an Al-CoS2NG hybrid with a negative electrode made of polyaniline (PANI) derived carbon nanorods (PCNRs), it demonstrates remarkable specific capacitance (188 F/g), energy density (66.9 Wh/kg), and cyclic stability of 92% after 10,000 cycles. This may open the pathway for the application of the next-generation supercapacitors in the future. Hierarchical sheets MOFs Al-doped CoS Nitrogen-doped graphene Solid-state supercapacitor Pandit, Bidhan verfasserin aut Hong, Sang Eun verfasserin aut Singu, Bal Sydulu verfasserin aut Kim, Seong K. verfasserin aut Moustafa, Essam B. verfasserin aut Yoon, Kuk Ro verfasserin aut Enthalten in Journal of Energy Chemistry Amsterdam [u.a.] : Elsevier, 2013 74, Seite 429-445 Online-Ressource (DE-627)745616399 (DE-600)2714311-9 (DE-576)382032861 2096-885X nnns volume:74 pages:429-445 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 AR 74 429-445
allfieldsGer	10.1016/j.jechem.2022.07.033 doi (DE-627)ELV008636826 (ELSEVIER)S2095-4956(22)00410-7 DE-627 ger DE-627 rda eng 540 DE-600 Goda, Emad S. verfasserin aut Zeolitic imidazolate framework-67 derived Al-Co-S hierarchical sheets bridged by nitrogen-doped graphene: Incorporation of PANI derived carbon nanorods for solid-state asymmetric supercapacitors 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Metal sulfides have been widely enticed as battery-type electrodes in supercapacitor devices because of their maximal theoretical capacitance. Nevertheless, their lower conductivity and ion transport kinetics can largely restrict their rate performance, hence the practical usage in fields of demanding high power devices. Therefore, the design of new electrodes with higher energy and power densities remains a highly challenging task. To the best of our knowledge, a novel hierarchical composite of Al-CoS2 on nitrogen-doped graphene (NG) is prepared based on a zeolite imidazole framework using a simple and scalable hydrothermal process. In this hybrid, ultrathin Al-CoS2 nanosheet arrays are vertically orientated on the NG framework to limit self-aggregation, hence increasing the electrical property and cycle stability of composite. It is investigated that the Al/Co feeding ratio plays a crucial role in controlling the obtained hierarchical structure of Al-Co-S sheets and their electrode performance. Also, Al3+ can influence remarkably the morphology and electrochemical property of the resultant graphene composite. An effective synergism is noticed between the redox Al-CoS2 and NG resulting in fast electron transfer and charging-discharging processes. Surprisingly, when the as-developed composite is utilized as a positive electrode at an applied current density of 1 A/g, a specific capacitance of 1915.8 F/g is attained with ultra-long cycle stability (96%, 10,000 cycles) and an excellent retention rate (∼89%). As a consequence, when a solid-state asymmetric supercapacitor (ASC) device is made by combining an Al-CoS2NG hybrid with a negative electrode made of polyaniline (PANI) derived carbon nanorods (PCNRs), it demonstrates remarkable specific capacitance (188 F/g), energy density (66.9 Wh/kg), and cyclic stability of 92% after 10,000 cycles. This may open the pathway for the application of the next-generation supercapacitors in the future. Hierarchical sheets MOFs Al-doped CoS Nitrogen-doped graphene Solid-state supercapacitor Pandit, Bidhan verfasserin aut Hong, Sang Eun verfasserin aut Singu, Bal Sydulu verfasserin aut Kim, Seong K. verfasserin aut Moustafa, Essam B. verfasserin aut Yoon, Kuk Ro verfasserin aut Enthalten in Journal of Energy Chemistry Amsterdam [u.a.] : Elsevier, 2013 74, Seite 429-445 Online-Ressource (DE-627)745616399 (DE-600)2714311-9 (DE-576)382032861 2096-885X nnns volume:74 pages:429-445 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 AR 74 429-445
allfieldsSound	10.1016/j.jechem.2022.07.033 doi (DE-627)ELV008636826 (ELSEVIER)S2095-4956(22)00410-7 DE-627 ger DE-627 rda eng 540 DE-600 Goda, Emad S. verfasserin aut Zeolitic imidazolate framework-67 derived Al-Co-S hierarchical sheets bridged by nitrogen-doped graphene: Incorporation of PANI derived carbon nanorods for solid-state asymmetric supercapacitors 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Metal sulfides have been widely enticed as battery-type electrodes in supercapacitor devices because of their maximal theoretical capacitance. Nevertheless, their lower conductivity and ion transport kinetics can largely restrict their rate performance, hence the practical usage in fields of demanding high power devices. Therefore, the design of new electrodes with higher energy and power densities remains a highly challenging task. To the best of our knowledge, a novel hierarchical composite of Al-CoS2 on nitrogen-doped graphene (NG) is prepared based on a zeolite imidazole framework using a simple and scalable hydrothermal process. In this hybrid, ultrathin Al-CoS2 nanosheet arrays are vertically orientated on the NG framework to limit self-aggregation, hence increasing the electrical property and cycle stability of composite. It is investigated that the Al/Co feeding ratio plays a crucial role in controlling the obtained hierarchical structure of Al-Co-S sheets and their electrode performance. Also, Al3+ can influence remarkably the morphology and electrochemical property of the resultant graphene composite. An effective synergism is noticed between the redox Al-CoS2 and NG resulting in fast electron transfer and charging-discharging processes. Surprisingly, when the as-developed composite is utilized as a positive electrode at an applied current density of 1 A/g, a specific capacitance of 1915.8 F/g is attained with ultra-long cycle stability (96%, 10,000 cycles) and an excellent retention rate (∼89%). As a consequence, when a solid-state asymmetric supercapacitor (ASC) device is made by combining an Al-CoS2NG hybrid with a negative electrode made of polyaniline (PANI) derived carbon nanorods (PCNRs), it demonstrates remarkable specific capacitance (188 F/g), energy density (66.9 Wh/kg), and cyclic stability of 92% after 10,000 cycles. This may open the pathway for the application of the next-generation supercapacitors in the future. Hierarchical sheets MOFs Al-doped CoS Nitrogen-doped graphene Solid-state supercapacitor Pandit, Bidhan verfasserin aut Hong, Sang Eun verfasserin aut Singu, Bal Sydulu verfasserin aut Kim, Seong K. verfasserin aut Moustafa, Essam B. verfasserin aut Yoon, Kuk Ro verfasserin aut Enthalten in Journal of Energy Chemistry Amsterdam [u.a.] : Elsevier, 2013 74, Seite 429-445 Online-Ressource (DE-627)745616399 (DE-600)2714311-9 (DE-576)382032861 2096-885X nnns volume:74 pages:429-445 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2008 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 AR 74 429-445
language	English
source	Enthalten in Journal of Energy Chemistry 74, Seite 429-445 volume:74 pages:429-445
sourceStr	Enthalten in Journal of Energy Chemistry 74, Seite 429-445 volume:74 pages:429-445
format_phy_str_mv	Article
institution	findex.gbv.de
topic_facet	Hierarchical sheets MOFs Al-doped CoS Nitrogen-doped graphene Solid-state supercapacitor
dewey-raw	540
isfreeaccess_bool	false
container_title	Journal of Energy Chemistry
authorswithroles_txt_mv	Goda, Emad S. @@aut@@ Pandit, Bidhan @@aut@@ Hong, Sang Eun @@aut@@ Singu, Bal Sydulu @@aut@@ Kim, Seong K. @@aut@@ Moustafa, Essam B. @@aut@@ Yoon, Kuk Ro @@aut@@
publishDateDaySort_date	2022-01-01T00:00:00Z
hierarchy_top_id	745616399
dewey-sort	3540
id	ELV008636826
language_de	englisch
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author	Goda, Emad S.
spellingShingle	Goda, Emad S. ddc 540 misc Hierarchical sheets misc MOFs misc Al-doped CoS misc Nitrogen-doped graphene misc Solid-state supercapacitor Zeolitic imidazolate framework-67 derived Al-Co-S hierarchical sheets bridged by nitrogen-doped graphene: Incorporation of PANI derived carbon nanorods for solid-state asymmetric supercapacitors
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topic_title	540 DE-600 Zeolitic imidazolate framework-67 derived Al-Co-S hierarchical sheets bridged by nitrogen-doped graphene: Incorporation of PANI derived carbon nanorods for solid-state asymmetric supercapacitors Hierarchical sheets MOFs Al-doped CoS Nitrogen-doped graphene Solid-state supercapacitor
topic	ddc 540 misc Hierarchical sheets misc MOFs misc Al-doped CoS misc Nitrogen-doped graphene misc Solid-state supercapacitor
topic_unstemmed	ddc 540 misc Hierarchical sheets misc MOFs misc Al-doped CoS misc Nitrogen-doped graphene misc Solid-state supercapacitor
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title	Zeolitic imidazolate framework-67 derived Al-Co-S hierarchical sheets bridged by nitrogen-doped graphene: Incorporation of PANI derived carbon nanorods for solid-state asymmetric supercapacitors
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title_full	Zeolitic imidazolate framework-67 derived Al-Co-S hierarchical sheets bridged by nitrogen-doped graphene: Incorporation of PANI derived carbon nanorods for solid-state asymmetric supercapacitors
author_sort	Goda, Emad S.
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author_browse	Goda, Emad S. Pandit, Bidhan Hong, Sang Eun Singu, Bal Sydulu Kim, Seong K. Moustafa, Essam B. Yoon, Kuk Ro
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title_sort	zeolitic imidazolate framework-67 derived al-co-s hierarchical sheets bridged by nitrogen-doped graphene: incorporation of pani derived carbon nanorods for solid-state asymmetric supercapacitors
title_auth	Zeolitic imidazolate framework-67 derived Al-Co-S hierarchical sheets bridged by nitrogen-doped graphene: Incorporation of PANI derived carbon nanorods for solid-state asymmetric supercapacitors
abstract	Metal sulfides have been widely enticed as battery-type electrodes in supercapacitor devices because of their maximal theoretical capacitance. Nevertheless, their lower conductivity and ion transport kinetics can largely restrict their rate performance, hence the practical usage in fields of demanding high power devices. Therefore, the design of new electrodes with higher energy and power densities remains a highly challenging task. To the best of our knowledge, a novel hierarchical composite of Al-CoS2 on nitrogen-doped graphene (NG) is prepared based on a zeolite imidazole framework using a simple and scalable hydrothermal process. In this hybrid, ultrathin Al-CoS2 nanosheet arrays are vertically orientated on the NG framework to limit self-aggregation, hence increasing the electrical property and cycle stability of composite. It is investigated that the Al/Co feeding ratio plays a crucial role in controlling the obtained hierarchical structure of Al-Co-S sheets and their electrode performance. Also, Al3+ can influence remarkably the morphology and electrochemical property of the resultant graphene composite. An effective synergism is noticed between the redox Al-CoS2 and NG resulting in fast electron transfer and charging-discharging processes. Surprisingly, when the as-developed composite is utilized as a positive electrode at an applied current density of 1 A/g, a specific capacitance of 1915.8 F/g is attained with ultra-long cycle stability (96%, 10,000 cycles) and an excellent retention rate (∼89%). As a consequence, when a solid-state asymmetric supercapacitor (ASC) device is made by combining an Al-CoS2NG hybrid with a negative electrode made of polyaniline (PANI) derived carbon nanorods (PCNRs), it demonstrates remarkable specific capacitance (188 F/g), energy density (66.9 Wh/kg), and cyclic stability of 92% after 10,000 cycles. This may open the pathway for the application of the next-generation supercapacitors in the future.
abstractGer	Metal sulfides have been widely enticed as battery-type electrodes in supercapacitor devices because of their maximal theoretical capacitance. Nevertheless, their lower conductivity and ion transport kinetics can largely restrict their rate performance, hence the practical usage in fields of demanding high power devices. Therefore, the design of new electrodes with higher energy and power densities remains a highly challenging task. To the best of our knowledge, a novel hierarchical composite of Al-CoS2 on nitrogen-doped graphene (NG) is prepared based on a zeolite imidazole framework using a simple and scalable hydrothermal process. In this hybrid, ultrathin Al-CoS2 nanosheet arrays are vertically orientated on the NG framework to limit self-aggregation, hence increasing the electrical property and cycle stability of composite. It is investigated that the Al/Co feeding ratio plays a crucial role in controlling the obtained hierarchical structure of Al-Co-S sheets and their electrode performance. Also, Al3+ can influence remarkably the morphology and electrochemical property of the resultant graphene composite. An effective synergism is noticed between the redox Al-CoS2 and NG resulting in fast electron transfer and charging-discharging processes. Surprisingly, when the as-developed composite is utilized as a positive electrode at an applied current density of 1 A/g, a specific capacitance of 1915.8 F/g is attained with ultra-long cycle stability (96%, 10,000 cycles) and an excellent retention rate (∼89%). As a consequence, when a solid-state asymmetric supercapacitor (ASC) device is made by combining an Al-CoS2NG hybrid with a negative electrode made of polyaniline (PANI) derived carbon nanorods (PCNRs), it demonstrates remarkable specific capacitance (188 F/g), energy density (66.9 Wh/kg), and cyclic stability of 92% after 10,000 cycles. This may open the pathway for the application of the next-generation supercapacitors in the future.
abstract_unstemmed	Metal sulfides have been widely enticed as battery-type electrodes in supercapacitor devices because of their maximal theoretical capacitance. Nevertheless, their lower conductivity and ion transport kinetics can largely restrict their rate performance, hence the practical usage in fields of demanding high power devices. Therefore, the design of new electrodes with higher energy and power densities remains a highly challenging task. To the best of our knowledge, a novel hierarchical composite of Al-CoS2 on nitrogen-doped graphene (NG) is prepared based on a zeolite imidazole framework using a simple and scalable hydrothermal process. In this hybrid, ultrathin Al-CoS2 nanosheet arrays are vertically orientated on the NG framework to limit self-aggregation, hence increasing the electrical property and cycle stability of composite. It is investigated that the Al/Co feeding ratio plays a crucial role in controlling the obtained hierarchical structure of Al-Co-S sheets and their electrode performance. Also, Al3+ can influence remarkably the morphology and electrochemical property of the resultant graphene composite. An effective synergism is noticed between the redox Al-CoS2 and NG resulting in fast electron transfer and charging-discharging processes. Surprisingly, when the as-developed composite is utilized as a positive electrode at an applied current density of 1 A/g, a specific capacitance of 1915.8 F/g is attained with ultra-long cycle stability (96%, 10,000 cycles) and an excellent retention rate (∼89%). As a consequence, when a solid-state asymmetric supercapacitor (ASC) device is made by combining an Al-CoS2NG hybrid with a negative electrode made of polyaniline (PANI) derived carbon nanorods (PCNRs), it demonstrates remarkable specific capacitance (188 F/g), energy density (66.9 Wh/kg), and cyclic stability of 92% after 10,000 cycles. This may open the pathway for the application of the next-generation supercapacitors in the future.
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title_short	Zeolitic imidazolate framework-67 derived Al-Co-S hierarchical sheets bridged by nitrogen-doped graphene: Incorporation of PANI derived carbon nanorods for solid-state asymmetric supercapacitors
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author2	Pandit, Bidhan Hong, Sang Eun Singu, Bal Sydulu Kim, Seong K. Moustafa, Essam B. Yoon, Kuk Ro
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doi_str	10.1016/j.jechem.2022.07.033
up_date	2024-07-06T20:23:17.165Z
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fullrecord_marcxml	<?xml version="1.0" encoding="UTF-8"?><collection xmlns="http://www.loc.gov/MARC21/slim"><record><leader>01000caa a22002652 4500</leader><controlfield tag="001">ELV008636826</controlfield><controlfield tag="003">DE-627</controlfield><controlfield tag="005">20230524122626.0</controlfield><controlfield tag="007">cr uuu---uuuuu</controlfield><controlfield tag="008">230509s2022 xx \|\|\|\|\|o 00\| \|\|eng c</controlfield><datafield tag="024" ind1="7" ind2=" "><subfield code="a">10.1016/j.jechem.2022.07.033</subfield><subfield code="2">doi</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(DE-627)ELV008636826</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(ELSEVIER)S2095-4956(22)00410-7</subfield></datafield><datafield tag="040" ind1=" " ind2=" "><subfield code="a">DE-627</subfield><subfield code="b">ger</subfield><subfield code="c">DE-627</subfield><subfield code="e">rda</subfield></datafield><datafield tag="041" ind1=" " ind2=" "><subfield code="a">eng</subfield></datafield><datafield tag="082" ind1="0" ind2="4"><subfield code="a">540</subfield><subfield code="q">DE-600</subfield></datafield><datafield tag="100" ind1="1" ind2=" "><subfield code="a">Goda, Emad S.</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="245" ind1="1" ind2="0"><subfield code="a">Zeolitic imidazolate framework-67 derived Al-Co-S hierarchical sheets bridged by nitrogen-doped graphene: Incorporation of PANI derived carbon nanorods for solid-state asymmetric supercapacitors</subfield></datafield><datafield tag="264" ind1=" " ind2="1"><subfield code="c">2022</subfield></datafield><datafield tag="336" ind1=" " ind2=" "><subfield code="a">nicht spezifiziert</subfield><subfield code="b">zzz</subfield><subfield code="2">rdacontent</subfield></datafield><datafield tag="337" ind1=" " ind2=" "><subfield code="a">Computermedien</subfield><subfield code="b">c</subfield><subfield code="2">rdamedia</subfield></datafield><datafield tag="338" ind1=" " ind2=" "><subfield code="a">Online-Ressource</subfield><subfield code="b">cr</subfield><subfield code="2">rdacarrier</subfield></datafield><datafield tag="520" ind1=" " ind2=" "><subfield code="a">Metal sulfides have been widely enticed as battery-type electrodes in supercapacitor devices because of their maximal theoretical capacitance. Nevertheless, their lower conductivity and ion transport kinetics can largely restrict their rate performance, hence the practical usage in fields of demanding high power devices. Therefore, the design of new electrodes with higher energy and power densities remains a highly challenging task. To the best of our knowledge, a novel hierarchical composite of Al-CoS2 on nitrogen-doped graphene (NG) is prepared based on a zeolite imidazole framework using a simple and scalable hydrothermal process. In this hybrid, ultrathin Al-CoS2 nanosheet arrays are vertically orientated on the NG framework to limit self-aggregation, hence increasing the electrical property and cycle stability of composite. It is investigated that the Al/Co feeding ratio plays a crucial role in controlling the obtained hierarchical structure of Al-Co-S sheets and their electrode performance. Also, Al3+ can influence remarkably the morphology and electrochemical property of the resultant graphene composite. An effective synergism is noticed between the redox Al-CoS2 and NG resulting in fast electron transfer and charging-discharging processes. Surprisingly, when the as-developed composite is utilized as a positive electrode at an applied current density of 1 A/g, a specific capacitance of 1915.8 F/g is attained with ultra-long cycle stability (96%, 10,000 cycles) and an excellent retention rate (∼89%). As a consequence, when a solid-state asymmetric supercapacitor (ASC) device is made by combining an Al-CoS2NG hybrid with a negative electrode made of polyaniline (PANI) derived carbon nanorods (PCNRs), it demonstrates remarkable specific capacitance (188 F/g), energy density (66.9 Wh/kg), and cyclic stability of 92% after 10,000 cycles. 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Zeolitic imidazolate framework-67 derived Al-Co-S hierarchical sheets bridged by nitrogen-doped graphene: Incorporation of PANI derived carbon nanorods for solid-state asymmetric supercapacitors

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