Inner-shell ionisation of Xe

The generation of collision-induced vacancies and their transfer within the electronic inner shells are the source of several unprecedented phenomena, which have been revealed in recent experimental studies conducted using state-of-the-art next-generation accelerators and detectors. Despite the multitude of studies conducted over the years, our understanding of the atomic vacancy transfer mechanisms remains exiguous. The detection and analysis of collision-induced X-rays is a widely-used powerful technique for analysing atomic-scale phenomena. However, both experimental and theoretical investigations on ion–atom collision-induced X-rays have remained mostly restricted to high-energy light-ion impact on heavy atoms. To date, only a few studies have been reported on the investigation of very-low-energy heavy-ion impact on heavy atoms using X-rays, especially M-shell X-rays of the heavy atom. This study was conducted to evaluate the inner-shell ionisation of Au (135 and 508 μ g / cm 2 ) and Pb (107, 157 and 390 μ g / cm 2 ) targets due to low-energy (2–5 MeV) 54Xe q + -ion impact. The collision-induced X-ray spectra of both the collision partners were examined, and the corresponding intensity ratios and cross-sections were compared with those calculated using two well-known ionisation theories, viz. PWBA and ECPSSR. The measured cross-sections were underestimated by these theories. Moreover, the cross-sections measured in this study were found to be several orders of magnitude higher than those obtained in other reported studies on low-energy lighter-ion-impact on Au and Pb. The significant discrepancies observed between the experimental and theoretical values have been explained qualitatively within the framework of quasi-molecular orbital formation using level correlations. The insights obtained from the results of this study can be applied to analyse the vacancy transfer mechanisms in very-heavy systems (combined atomic number > 100). Ausführliche Beschreibung

Gespeichert in:

Autor*in:	Ahmad, C.V. [verfasserIn] Gupta, R. [verfasserIn] Chakraborty, K. [verfasserIn] Swami, D.K. [verfasserIn] Verma, P. [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2022

Schlagwörter:	X-rays PWBA ECPSSR Heavy-ion impact Molecular orbital

Übergeordnetes Werk:	Enthalten in: Nuclear instruments & methods in physics research / B - Amsterdam [u.a.] : Elsevier, 1984, 531, Seite 9-23
Übergeordnetes Werk:	volume:531 ; pages:9-23

DOI / URN:	10.1016/j.nimb.2022.08.010

Katalog-ID:	ELV008694796

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520			\|a The generation of collision-induced vacancies and their transfer within the electronic inner shells are the source of several unprecedented phenomena, which have been revealed in recent experimental studies conducted using state-of-the-art next-generation accelerators and detectors. Despite the multitude of studies conducted over the years, our understanding of the atomic vacancy transfer mechanisms remains exiguous. The detection and analysis of collision-induced X-rays is a widely-used powerful technique for analysing atomic-scale phenomena. However, both experimental and theoretical investigations on ion–atom collision-induced X-rays have remained mostly restricted to high-energy light-ion impact on heavy atoms. To date, only a few studies have been reported on the investigation of very-low-energy heavy-ion impact on heavy atoms using X-rays, especially M-shell X-rays of the heavy atom. This study was conducted to evaluate the inner-shell ionisation of Au (135 and 508 μ g / cm 2 ) and Pb (107, 157 and 390 μ g / cm 2 ) targets due to low-energy (2–5 MeV) 54Xe q + -ion impact. The collision-induced X-ray spectra of both the collision partners were examined, and the corresponding intensity ratios and cross-sections were compared with those calculated using two well-known ionisation theories, viz. PWBA and ECPSSR. The measured cross-sections were underestimated by these theories. Moreover, the cross-sections measured in this study were found to be several orders of magnitude higher than those obtained in other reported studies on low-energy lighter-ion-impact on Au and Pb. The significant discrepancies observed between the experimental and theoretical values have been explained qualitatively within the framework of quasi-molecular orbital formation using level correlations. The insights obtained from the results of this study can be applied to analyse the vacancy transfer mechanisms in very-heavy systems (combined atomic number > 100).
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700	1		\|a Chakraborty, K. \|e verfasserin \|0 (orcid)0000-0003-0666-4572 \|4 aut
700	1		\|a Swami, D.K. \|e verfasserin \|4 aut
700	1		\|a Verma, P. \|e verfasserin \|0 (orcid)0000-0001-7686-6829 \|4 aut
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936	b	k	\|a 33.05 \|j Experimentalphysik
936	b	k	\|a 33.40 \|j Kernphysik
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allfields	10.1016/j.nimb.2022.08.010 doi (DE-627)ELV008694796 (ELSEVIER)S0168-583X(22)00214-2 DE-627 ger DE-627 rda eng 530 DE-600 33.05 bkl 33.40 bkl Ahmad, C.V. verfasserin (orcid)0000-0001-5130-6948 aut Inner-shell ionisation of Xe 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The generation of collision-induced vacancies and their transfer within the electronic inner shells are the source of several unprecedented phenomena, which have been revealed in recent experimental studies conducted using state-of-the-art next-generation accelerators and detectors. Despite the multitude of studies conducted over the years, our understanding of the atomic vacancy transfer mechanisms remains exiguous. The detection and analysis of collision-induced X-rays is a widely-used powerful technique for analysing atomic-scale phenomena. However, both experimental and theoretical investigations on ion–atom collision-induced X-rays have remained mostly restricted to high-energy light-ion impact on heavy atoms. To date, only a few studies have been reported on the investigation of very-low-energy heavy-ion impact on heavy atoms using X-rays, especially M-shell X-rays of the heavy atom. This study was conducted to evaluate the inner-shell ionisation of Au (135 and 508 μ g / cm 2 ) and Pb (107, 157 and 390 μ g / cm 2 ) targets due to low-energy (2–5 MeV) 54Xe q + -ion impact. The collision-induced X-ray spectra of both the collision partners were examined, and the corresponding intensity ratios and cross-sections were compared with those calculated using two well-known ionisation theories, viz. PWBA and ECPSSR. The measured cross-sections were underestimated by these theories. Moreover, the cross-sections measured in this study were found to be several orders of magnitude higher than those obtained in other reported studies on low-energy lighter-ion-impact on Au and Pb. The significant discrepancies observed between the experimental and theoretical values have been explained qualitatively within the framework of quasi-molecular orbital formation using level correlations. The insights obtained from the results of this study can be applied to analyse the vacancy transfer mechanisms in very-heavy systems (combined atomic number > 100). X-rays PWBA ECPSSR Heavy-ion impact Molecular orbital Gupta, R. verfasserin (orcid)0000-0001-9592-1299 aut Chakraborty, K. verfasserin (orcid)0000-0003-0666-4572 aut Swami, D.K. verfasserin aut Verma, P. verfasserin (orcid)0000-0001-7686-6829 aut Enthalten in Nuclear instruments & methods in physics research / B Amsterdam [u.a.] : Elsevier, 1984 531, Seite 9-23 Online-Ressource (DE-627)266014585 (DE-600)1466524-4 (DE-576)074959735 nnns volume:531 pages:9-23 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 33.05 Experimentalphysik 33.40 Kernphysik AR 531 9-23
spelling	10.1016/j.nimb.2022.08.010 doi (DE-627)ELV008694796 (ELSEVIER)S0168-583X(22)00214-2 DE-627 ger DE-627 rda eng 530 DE-600 33.05 bkl 33.40 bkl Ahmad, C.V. verfasserin (orcid)0000-0001-5130-6948 aut Inner-shell ionisation of Xe 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The generation of collision-induced vacancies and their transfer within the electronic inner shells are the source of several unprecedented phenomena, which have been revealed in recent experimental studies conducted using state-of-the-art next-generation accelerators and detectors. Despite the multitude of studies conducted over the years, our understanding of the atomic vacancy transfer mechanisms remains exiguous. The detection and analysis of collision-induced X-rays is a widely-used powerful technique for analysing atomic-scale phenomena. However, both experimental and theoretical investigations on ion–atom collision-induced X-rays have remained mostly restricted to high-energy light-ion impact on heavy atoms. To date, only a few studies have been reported on the investigation of very-low-energy heavy-ion impact on heavy atoms using X-rays, especially M-shell X-rays of the heavy atom. This study was conducted to evaluate the inner-shell ionisation of Au (135 and 508 μ g / cm 2 ) and Pb (107, 157 and 390 μ g / cm 2 ) targets due to low-energy (2–5 MeV) 54Xe q + -ion impact. The collision-induced X-ray spectra of both the collision partners were examined, and the corresponding intensity ratios and cross-sections were compared with those calculated using two well-known ionisation theories, viz. PWBA and ECPSSR. The measured cross-sections were underestimated by these theories. Moreover, the cross-sections measured in this study were found to be several orders of magnitude higher than those obtained in other reported studies on low-energy lighter-ion-impact on Au and Pb. The significant discrepancies observed between the experimental and theoretical values have been explained qualitatively within the framework of quasi-molecular orbital formation using level correlations. The insights obtained from the results of this study can be applied to analyse the vacancy transfer mechanisms in very-heavy systems (combined atomic number > 100). X-rays PWBA ECPSSR Heavy-ion impact Molecular orbital Gupta, R. verfasserin (orcid)0000-0001-9592-1299 aut Chakraborty, K. verfasserin (orcid)0000-0003-0666-4572 aut Swami, D.K. verfasserin aut Verma, P. verfasserin (orcid)0000-0001-7686-6829 aut Enthalten in Nuclear instruments & methods in physics research / B Amsterdam [u.a.] : Elsevier, 1984 531, Seite 9-23 Online-Ressource (DE-627)266014585 (DE-600)1466524-4 (DE-576)074959735 nnns volume:531 pages:9-23 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 33.05 Experimentalphysik 33.40 Kernphysik AR 531 9-23
allfields_unstemmed	10.1016/j.nimb.2022.08.010 doi (DE-627)ELV008694796 (ELSEVIER)S0168-583X(22)00214-2 DE-627 ger DE-627 rda eng 530 DE-600 33.05 bkl 33.40 bkl Ahmad, C.V. verfasserin (orcid)0000-0001-5130-6948 aut Inner-shell ionisation of Xe 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The generation of collision-induced vacancies and their transfer within the electronic inner shells are the source of several unprecedented phenomena, which have been revealed in recent experimental studies conducted using state-of-the-art next-generation accelerators and detectors. Despite the multitude of studies conducted over the years, our understanding of the atomic vacancy transfer mechanisms remains exiguous. The detection and analysis of collision-induced X-rays is a widely-used powerful technique for analysing atomic-scale phenomena. However, both experimental and theoretical investigations on ion–atom collision-induced X-rays have remained mostly restricted to high-energy light-ion impact on heavy atoms. To date, only a few studies have been reported on the investigation of very-low-energy heavy-ion impact on heavy atoms using X-rays, especially M-shell X-rays of the heavy atom. This study was conducted to evaluate the inner-shell ionisation of Au (135 and 508 μ g / cm 2 ) and Pb (107, 157 and 390 μ g / cm 2 ) targets due to low-energy (2–5 MeV) 54Xe q + -ion impact. The collision-induced X-ray spectra of both the collision partners were examined, and the corresponding intensity ratios and cross-sections were compared with those calculated using two well-known ionisation theories, viz. PWBA and ECPSSR. The measured cross-sections were underestimated by these theories. Moreover, the cross-sections measured in this study were found to be several orders of magnitude higher than those obtained in other reported studies on low-energy lighter-ion-impact on Au and Pb. The significant discrepancies observed between the experimental and theoretical values have been explained qualitatively within the framework of quasi-molecular orbital formation using level correlations. The insights obtained from the results of this study can be applied to analyse the vacancy transfer mechanisms in very-heavy systems (combined atomic number > 100). X-rays PWBA ECPSSR Heavy-ion impact Molecular orbital Gupta, R. verfasserin (orcid)0000-0001-9592-1299 aut Chakraborty, K. verfasserin (orcid)0000-0003-0666-4572 aut Swami, D.K. verfasserin aut Verma, P. verfasserin (orcid)0000-0001-7686-6829 aut Enthalten in Nuclear instruments & methods in physics research / B Amsterdam [u.a.] : Elsevier, 1984 531, Seite 9-23 Online-Ressource (DE-627)266014585 (DE-600)1466524-4 (DE-576)074959735 nnns volume:531 pages:9-23 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 33.05 Experimentalphysik 33.40 Kernphysik AR 531 9-23
allfieldsGer	10.1016/j.nimb.2022.08.010 doi (DE-627)ELV008694796 (ELSEVIER)S0168-583X(22)00214-2 DE-627 ger DE-627 rda eng 530 DE-600 33.05 bkl 33.40 bkl Ahmad, C.V. verfasserin (orcid)0000-0001-5130-6948 aut Inner-shell ionisation of Xe 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The generation of collision-induced vacancies and their transfer within the electronic inner shells are the source of several unprecedented phenomena, which have been revealed in recent experimental studies conducted using state-of-the-art next-generation accelerators and detectors. Despite the multitude of studies conducted over the years, our understanding of the atomic vacancy transfer mechanisms remains exiguous. The detection and analysis of collision-induced X-rays is a widely-used powerful technique for analysing atomic-scale phenomena. However, both experimental and theoretical investigations on ion–atom collision-induced X-rays have remained mostly restricted to high-energy light-ion impact on heavy atoms. To date, only a few studies have been reported on the investigation of very-low-energy heavy-ion impact on heavy atoms using X-rays, especially M-shell X-rays of the heavy atom. This study was conducted to evaluate the inner-shell ionisation of Au (135 and 508 μ g / cm 2 ) and Pb (107, 157 and 390 μ g / cm 2 ) targets due to low-energy (2–5 MeV) 54Xe q + -ion impact. The collision-induced X-ray spectra of both the collision partners were examined, and the corresponding intensity ratios and cross-sections were compared with those calculated using two well-known ionisation theories, viz. PWBA and ECPSSR. The measured cross-sections were underestimated by these theories. Moreover, the cross-sections measured in this study were found to be several orders of magnitude higher than those obtained in other reported studies on low-energy lighter-ion-impact on Au and Pb. The significant discrepancies observed between the experimental and theoretical values have been explained qualitatively within the framework of quasi-molecular orbital formation using level correlations. The insights obtained from the results of this study can be applied to analyse the vacancy transfer mechanisms in very-heavy systems (combined atomic number > 100). X-rays PWBA ECPSSR Heavy-ion impact Molecular orbital Gupta, R. verfasserin (orcid)0000-0001-9592-1299 aut Chakraborty, K. verfasserin (orcid)0000-0003-0666-4572 aut Swami, D.K. verfasserin aut Verma, P. verfasserin (orcid)0000-0001-7686-6829 aut Enthalten in Nuclear instruments & methods in physics research / B Amsterdam [u.a.] : Elsevier, 1984 531, Seite 9-23 Online-Ressource (DE-627)266014585 (DE-600)1466524-4 (DE-576)074959735 nnns volume:531 pages:9-23 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 33.05 Experimentalphysik 33.40 Kernphysik AR 531 9-23
allfieldsSound	10.1016/j.nimb.2022.08.010 doi (DE-627)ELV008694796 (ELSEVIER)S0168-583X(22)00214-2 DE-627 ger DE-627 rda eng 530 DE-600 33.05 bkl 33.40 bkl Ahmad, C.V. verfasserin (orcid)0000-0001-5130-6948 aut Inner-shell ionisation of Xe 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The generation of collision-induced vacancies and their transfer within the electronic inner shells are the source of several unprecedented phenomena, which have been revealed in recent experimental studies conducted using state-of-the-art next-generation accelerators and detectors. Despite the multitude of studies conducted over the years, our understanding of the atomic vacancy transfer mechanisms remains exiguous. The detection and analysis of collision-induced X-rays is a widely-used powerful technique for analysing atomic-scale phenomena. However, both experimental and theoretical investigations on ion–atom collision-induced X-rays have remained mostly restricted to high-energy light-ion impact on heavy atoms. To date, only a few studies have been reported on the investigation of very-low-energy heavy-ion impact on heavy atoms using X-rays, especially M-shell X-rays of the heavy atom. This study was conducted to evaluate the inner-shell ionisation of Au (135 and 508 μ g / cm 2 ) and Pb (107, 157 and 390 μ g / cm 2 ) targets due to low-energy (2–5 MeV) 54Xe q + -ion impact. The collision-induced X-ray spectra of both the collision partners were examined, and the corresponding intensity ratios and cross-sections were compared with those calculated using two well-known ionisation theories, viz. PWBA and ECPSSR. The measured cross-sections were underestimated by these theories. Moreover, the cross-sections measured in this study were found to be several orders of magnitude higher than those obtained in other reported studies on low-energy lighter-ion-impact on Au and Pb. The significant discrepancies observed between the experimental and theoretical values have been explained qualitatively within the framework of quasi-molecular orbital formation using level correlations. The insights obtained from the results of this study can be applied to analyse the vacancy transfer mechanisms in very-heavy systems (combined atomic number > 100). X-rays PWBA ECPSSR Heavy-ion impact Molecular orbital Gupta, R. verfasserin (orcid)0000-0001-9592-1299 aut Chakraborty, K. verfasserin (orcid)0000-0003-0666-4572 aut Swami, D.K. verfasserin aut Verma, P. verfasserin (orcid)0000-0001-7686-6829 aut Enthalten in Nuclear instruments & methods in physics research / B Amsterdam [u.a.] : Elsevier, 1984 531, Seite 9-23 Online-Ressource (DE-627)266014585 (DE-600)1466524-4 (DE-576)074959735 nnns volume:531 pages:9-23 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 33.05 Experimentalphysik 33.40 Kernphysik AR 531 9-23
language	English
source	Enthalten in Nuclear instruments & methods in physics research / B 531, Seite 9-23 volume:531 pages:9-23
sourceStr	Enthalten in Nuclear instruments & methods in physics research / B 531, Seite 9-23 volume:531 pages:9-23
format_phy_str_mv	Article
bklname	Experimentalphysik Kernphysik
institution	findex.gbv.de
topic_facet	X-rays PWBA ECPSSR Heavy-ion impact Molecular orbital
dewey-raw	530
isfreeaccess_bool	false
container_title	Nuclear instruments & methods in physics research / B
authorswithroles_txt_mv	Ahmad, C.V. @@aut@@ Gupta, R. @@aut@@ Chakraborty, K. @@aut@@ Swami, D.K. @@aut@@ Verma, P. @@aut@@
publishDateDaySort_date	2022-01-01T00:00:00Z
hierarchy_top_id	266014585
dewey-sort	3530
id	ELV008694796
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author	Ahmad, C.V.
spellingShingle	Ahmad, C.V. ddc 530 bkl 33.05 bkl 33.40 misc X-rays misc PWBA misc ECPSSR misc Heavy-ion impact misc Molecular orbital Inner-shell ionisation of Xe
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topic_title	530 DE-600 33.05 bkl 33.40 bkl Inner-shell ionisation of Xe X-rays PWBA ECPSSR Heavy-ion impact Molecular orbital
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title	Inner-shell ionisation of Xe
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title_full	Inner-shell ionisation of Xe
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title_sort	inner-shell ionisation of xe
title_auth	Inner-shell ionisation of Xe
abstract	The generation of collision-induced vacancies and their transfer within the electronic inner shells are the source of several unprecedented phenomena, which have been revealed in recent experimental studies conducted using state-of-the-art next-generation accelerators and detectors. Despite the multitude of studies conducted over the years, our understanding of the atomic vacancy transfer mechanisms remains exiguous. The detection and analysis of collision-induced X-rays is a widely-used powerful technique for analysing atomic-scale phenomena. However, both experimental and theoretical investigations on ion–atom collision-induced X-rays have remained mostly restricted to high-energy light-ion impact on heavy atoms. To date, only a few studies have been reported on the investigation of very-low-energy heavy-ion impact on heavy atoms using X-rays, especially M-shell X-rays of the heavy atom. This study was conducted to evaluate the inner-shell ionisation of Au (135 and 508 μ g / cm 2 ) and Pb (107, 157 and 390 μ g / cm 2 ) targets due to low-energy (2–5 MeV) 54Xe q + -ion impact. The collision-induced X-ray spectra of both the collision partners were examined, and the corresponding intensity ratios and cross-sections were compared with those calculated using two well-known ionisation theories, viz. PWBA and ECPSSR. The measured cross-sections were underestimated by these theories. Moreover, the cross-sections measured in this study were found to be several orders of magnitude higher than those obtained in other reported studies on low-energy lighter-ion-impact on Au and Pb. The significant discrepancies observed between the experimental and theoretical values have been explained qualitatively within the framework of quasi-molecular orbital formation using level correlations. The insights obtained from the results of this study can be applied to analyse the vacancy transfer mechanisms in very-heavy systems (combined atomic number > 100).
abstractGer	The generation of collision-induced vacancies and their transfer within the electronic inner shells are the source of several unprecedented phenomena, which have been revealed in recent experimental studies conducted using state-of-the-art next-generation accelerators and detectors. Despite the multitude of studies conducted over the years, our understanding of the atomic vacancy transfer mechanisms remains exiguous. The detection and analysis of collision-induced X-rays is a widely-used powerful technique for analysing atomic-scale phenomena. However, both experimental and theoretical investigations on ion–atom collision-induced X-rays have remained mostly restricted to high-energy light-ion impact on heavy atoms. To date, only a few studies have been reported on the investigation of very-low-energy heavy-ion impact on heavy atoms using X-rays, especially M-shell X-rays of the heavy atom. This study was conducted to evaluate the inner-shell ionisation of Au (135 and 508 μ g / cm 2 ) and Pb (107, 157 and 390 μ g / cm 2 ) targets due to low-energy (2–5 MeV) 54Xe q + -ion impact. The collision-induced X-ray spectra of both the collision partners were examined, and the corresponding intensity ratios and cross-sections were compared with those calculated using two well-known ionisation theories, viz. PWBA and ECPSSR. The measured cross-sections were underestimated by these theories. Moreover, the cross-sections measured in this study were found to be several orders of magnitude higher than those obtained in other reported studies on low-energy lighter-ion-impact on Au and Pb. The significant discrepancies observed between the experimental and theoretical values have been explained qualitatively within the framework of quasi-molecular orbital formation using level correlations. The insights obtained from the results of this study can be applied to analyse the vacancy transfer mechanisms in very-heavy systems (combined atomic number > 100).
abstract_unstemmed	The generation of collision-induced vacancies and their transfer within the electronic inner shells are the source of several unprecedented phenomena, which have been revealed in recent experimental studies conducted using state-of-the-art next-generation accelerators and detectors. Despite the multitude of studies conducted over the years, our understanding of the atomic vacancy transfer mechanisms remains exiguous. The detection and analysis of collision-induced X-rays is a widely-used powerful technique for analysing atomic-scale phenomena. However, both experimental and theoretical investigations on ion–atom collision-induced X-rays have remained mostly restricted to high-energy light-ion impact on heavy atoms. To date, only a few studies have been reported on the investigation of very-low-energy heavy-ion impact on heavy atoms using X-rays, especially M-shell X-rays of the heavy atom. This study was conducted to evaluate the inner-shell ionisation of Au (135 and 508 μ g / cm 2 ) and Pb (107, 157 and 390 μ g / cm 2 ) targets due to low-energy (2–5 MeV) 54Xe q + -ion impact. The collision-induced X-ray spectra of both the collision partners were examined, and the corresponding intensity ratios and cross-sections were compared with those calculated using two well-known ionisation theories, viz. PWBA and ECPSSR. The measured cross-sections were underestimated by these theories. Moreover, the cross-sections measured in this study were found to be several orders of magnitude higher than those obtained in other reported studies on low-energy lighter-ion-impact on Au and Pb. The significant discrepancies observed between the experimental and theoretical values have been explained qualitatively within the framework of quasi-molecular orbital formation using level correlations. The insights obtained from the results of this study can be applied to analyse the vacancy transfer mechanisms in very-heavy systems (combined atomic number > 100).
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title_short	Inner-shell ionisation of Xe
remote_bool	true
author2	Gupta, R. Chakraborty, K. Swami, D.K. Verma, P.
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doi_str	10.1016/j.nimb.2022.08.010
up_date	2024-07-06T20:35:05.403Z
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The collision-induced X-ray spectra of both the collision partners were examined, and the corresponding intensity ratios and cross-sections were compared with those calculated using two well-known ionisation theories, viz. PWBA and ECPSSR. The measured cross-sections were underestimated by these theories. Moreover, the cross-sections measured in this study were found to be several orders of magnitude higher than those obtained in other reported studies on low-energy lighter-ion-impact on Au and Pb. The significant discrepancies observed between the experimental and theoretical values have been explained qualitatively within the framework of quasi-molecular orbital formation using level correlations. 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code="0">(orcid)0000-0003-0666-4572</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Swami, D.K.</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Verma, P.</subfield><subfield code="e">verfasserin</subfield><subfield code="0">(orcid)0000-0001-7686-6829</subfield><subfield code="4">aut</subfield></datafield><datafield tag="773" ind1="0" ind2="8"><subfield code="i">Enthalten in</subfield><subfield code="t">Nuclear instruments & methods in physics research / B</subfield><subfield code="d">Amsterdam [u.a.] : Elsevier, 1984</subfield><subfield code="g">531, Seite 9-23</subfield><subfield code="h">Online-Ressource</subfield><subfield code="w">(DE-627)266014585</subfield><subfield code="w">(DE-600)1466524-4</subfield><subfield code="w">(DE-576)074959735</subfield><subfield code="7">nnns</subfield></datafield><datafield 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