Effective removal of nitroimidazole antibiotics in aqueous solution by an aluminum-based metal-organic framework: Performance and mechanistic studies

The removal of antibiotics from wastewater has received extensive attention. An aluminum-based metal-organic framework (Al-TCPP) was synthesized as an adsorbent to remove ornidazole (ONZ) and metronidazole (MNZ). Al-TCPP has high adsorption capacities of 609.8 mg g−1 and 320.5 mg g−1 for ONZ and...
Ausführliche Beschreibung

Gespeichert in:

Autor*in:	Li, Gan [verfasserIn] Yan, Tongan [verfasserIn] Zhao, Huifang [verfasserIn] Liu, Dahuan [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2022

Schlagwörter:	Adsorption Metal-organic framework Hydrogen bond π−π interaction Theoretical calculation

Übergeordnetes Werk:	Enthalten in: Journal of solid state chemistry - Orlando, Fla. : Academic Press, 1969, 317
Übergeordnetes Werk:	volume:317

DOI / URN:	10.1016/j.jssc.2022.123659

Katalog-ID:	ELV00887168X

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520			\|a The removal of antibiotics from wastewater has received extensive attention. An aluminum-based metal-organic framework (Al-TCPP) was synthesized as an adsorbent to remove ornidazole (ONZ) and metronidazole (MNZ). Al-TCPP has high adsorption capacities of 609.8 mg g−1 and 320.5 mg g−1 for ONZ and MNZ, respectively, superior to the reported adsorbents. And the adsorption data can fit well with the Langmuir model and the pseudo-second-order model. Besides, the adsorbent exhibits excellent anti-interference to coexisting salts and pH, which indicates that it has good practical application value. Furthermore, the possible adsorption mechanisms were proposed by FT-IR, XPS, Zeta potential, theoretical calculation, as well as the control experiments. These results indicate that hydrogen bonding interaction dominates the adsorption process. Therefore, Al-TCPP may have broad application prospects in purifying wastewater containing nitroimidazole antibiotics. The proposal of the dominant force is beneficial to the development of new adsorbents for the removal of antibiotics from aqueous solution.
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allfields	10.1016/j.jssc.2022.123659 doi (DE-627)ELV00887168X (ELSEVIER)S0022-4596(22)00784-8 DE-627 ger DE-627 rda eng 540 DE-600 35.90 bkl Li, Gan verfasserin aut Effective removal of nitroimidazole antibiotics in aqueous solution by an aluminum-based metal-organic framework: Performance and mechanistic studies 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The removal of antibiotics from wastewater has received extensive attention. An aluminum-based metal-organic framework (Al-TCPP) was synthesized as an adsorbent to remove ornidazole (ONZ) and metronidazole (MNZ). Al-TCPP has high adsorption capacities of 609.8 mg g−1 and 320.5 mg g−1 for ONZ and MNZ, respectively, superior to the reported adsorbents. And the adsorption data can fit well with the Langmuir model and the pseudo-second-order model. Besides, the adsorbent exhibits excellent anti-interference to coexisting salts and pH, which indicates that it has good practical application value. Furthermore, the possible adsorption mechanisms were proposed by FT-IR, XPS, Zeta potential, theoretical calculation, as well as the control experiments. These results indicate that hydrogen bonding interaction dominates the adsorption process. Therefore, Al-TCPP may have broad application prospects in purifying wastewater containing nitroimidazole antibiotics. The proposal of the dominant force is beneficial to the development of new adsorbents for the removal of antibiotics from aqueous solution. Adsorption Metal-organic framework Hydrogen bond π−π interaction Theoretical calculation Yan, Tongan verfasserin aut Zhao, Huifang verfasserin aut Liu, Dahuan verfasserin aut Enthalten in Journal of solid state chemistry Orlando, Fla. : Academic Press, 1969 317 Online-Ressource (DE-627)267328451 (DE-600)1469806-7 (DE-576)10337325X nnns volume:317 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.90 Festkörperchemie AR 317
spelling	10.1016/j.jssc.2022.123659 doi (DE-627)ELV00887168X (ELSEVIER)S0022-4596(22)00784-8 DE-627 ger DE-627 rda eng 540 DE-600 35.90 bkl Li, Gan verfasserin aut Effective removal of nitroimidazole antibiotics in aqueous solution by an aluminum-based metal-organic framework: Performance and mechanistic studies 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The removal of antibiotics from wastewater has received extensive attention. An aluminum-based metal-organic framework (Al-TCPP) was synthesized as an adsorbent to remove ornidazole (ONZ) and metronidazole (MNZ). Al-TCPP has high adsorption capacities of 609.8 mg g−1 and 320.5 mg g−1 for ONZ and MNZ, respectively, superior to the reported adsorbents. And the adsorption data can fit well with the Langmuir model and the pseudo-second-order model. Besides, the adsorbent exhibits excellent anti-interference to coexisting salts and pH, which indicates that it has good practical application value. Furthermore, the possible adsorption mechanisms were proposed by FT-IR, XPS, Zeta potential, theoretical calculation, as well as the control experiments. These results indicate that hydrogen bonding interaction dominates the adsorption process. Therefore, Al-TCPP may have broad application prospects in purifying wastewater containing nitroimidazole antibiotics. The proposal of the dominant force is beneficial to the development of new adsorbents for the removal of antibiotics from aqueous solution. Adsorption Metal-organic framework Hydrogen bond π−π interaction Theoretical calculation Yan, Tongan verfasserin aut Zhao, Huifang verfasserin aut Liu, Dahuan verfasserin aut Enthalten in Journal of solid state chemistry Orlando, Fla. : Academic Press, 1969 317 Online-Ressource (DE-627)267328451 (DE-600)1469806-7 (DE-576)10337325X nnns volume:317 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.90 Festkörperchemie AR 317
allfields_unstemmed	10.1016/j.jssc.2022.123659 doi (DE-627)ELV00887168X (ELSEVIER)S0022-4596(22)00784-8 DE-627 ger DE-627 rda eng 540 DE-600 35.90 bkl Li, Gan verfasserin aut Effective removal of nitroimidazole antibiotics in aqueous solution by an aluminum-based metal-organic framework: Performance and mechanistic studies 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The removal of antibiotics from wastewater has received extensive attention. An aluminum-based metal-organic framework (Al-TCPP) was synthesized as an adsorbent to remove ornidazole (ONZ) and metronidazole (MNZ). Al-TCPP has high adsorption capacities of 609.8 mg g−1 and 320.5 mg g−1 for ONZ and MNZ, respectively, superior to the reported adsorbents. And the adsorption data can fit well with the Langmuir model and the pseudo-second-order model. Besides, the adsorbent exhibits excellent anti-interference to coexisting salts and pH, which indicates that it has good practical application value. Furthermore, the possible adsorption mechanisms were proposed by FT-IR, XPS, Zeta potential, theoretical calculation, as well as the control experiments. These results indicate that hydrogen bonding interaction dominates the adsorption process. Therefore, Al-TCPP may have broad application prospects in purifying wastewater containing nitroimidazole antibiotics. The proposal of the dominant force is beneficial to the development of new adsorbents for the removal of antibiotics from aqueous solution. Adsorption Metal-organic framework Hydrogen bond π−π interaction Theoretical calculation Yan, Tongan verfasserin aut Zhao, Huifang verfasserin aut Liu, Dahuan verfasserin aut Enthalten in Journal of solid state chemistry Orlando, Fla. : Academic Press, 1969 317 Online-Ressource (DE-627)267328451 (DE-600)1469806-7 (DE-576)10337325X nnns volume:317 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.90 Festkörperchemie AR 317
allfieldsGer	10.1016/j.jssc.2022.123659 doi (DE-627)ELV00887168X (ELSEVIER)S0022-4596(22)00784-8 DE-627 ger DE-627 rda eng 540 DE-600 35.90 bkl Li, Gan verfasserin aut Effective removal of nitroimidazole antibiotics in aqueous solution by an aluminum-based metal-organic framework: Performance and mechanistic studies 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The removal of antibiotics from wastewater has received extensive attention. An aluminum-based metal-organic framework (Al-TCPP) was synthesized as an adsorbent to remove ornidazole (ONZ) and metronidazole (MNZ). Al-TCPP has high adsorption capacities of 609.8 mg g−1 and 320.5 mg g−1 for ONZ and MNZ, respectively, superior to the reported adsorbents. And the adsorption data can fit well with the Langmuir model and the pseudo-second-order model. Besides, the adsorbent exhibits excellent anti-interference to coexisting salts and pH, which indicates that it has good practical application value. Furthermore, the possible adsorption mechanisms were proposed by FT-IR, XPS, Zeta potential, theoretical calculation, as well as the control experiments. These results indicate that hydrogen bonding interaction dominates the adsorption process. Therefore, Al-TCPP may have broad application prospects in purifying wastewater containing nitroimidazole antibiotics. The proposal of the dominant force is beneficial to the development of new adsorbents for the removal of antibiotics from aqueous solution. Adsorption Metal-organic framework Hydrogen bond π−π interaction Theoretical calculation Yan, Tongan verfasserin aut Zhao, Huifang verfasserin aut Liu, Dahuan verfasserin aut Enthalten in Journal of solid state chemistry Orlando, Fla. : Academic Press, 1969 317 Online-Ressource (DE-627)267328451 (DE-600)1469806-7 (DE-576)10337325X nnns volume:317 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.90 Festkörperchemie AR 317
allfieldsSound	10.1016/j.jssc.2022.123659 doi (DE-627)ELV00887168X (ELSEVIER)S0022-4596(22)00784-8 DE-627 ger DE-627 rda eng 540 DE-600 35.90 bkl Li, Gan verfasserin aut Effective removal of nitroimidazole antibiotics in aqueous solution by an aluminum-based metal-organic framework: Performance and mechanistic studies 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The removal of antibiotics from wastewater has received extensive attention. An aluminum-based metal-organic framework (Al-TCPP) was synthesized as an adsorbent to remove ornidazole (ONZ) and metronidazole (MNZ). Al-TCPP has high adsorption capacities of 609.8 mg g−1 and 320.5 mg g−1 for ONZ and MNZ, respectively, superior to the reported adsorbents. And the adsorption data can fit well with the Langmuir model and the pseudo-second-order model. Besides, the adsorbent exhibits excellent anti-interference to coexisting salts and pH, which indicates that it has good practical application value. Furthermore, the possible adsorption mechanisms were proposed by FT-IR, XPS, Zeta potential, theoretical calculation, as well as the control experiments. These results indicate that hydrogen bonding interaction dominates the adsorption process. Therefore, Al-TCPP may have broad application prospects in purifying wastewater containing nitroimidazole antibiotics. The proposal of the dominant force is beneficial to the development of new adsorbents for the removal of antibiotics from aqueous solution. Adsorption Metal-organic framework Hydrogen bond π−π interaction Theoretical calculation Yan, Tongan verfasserin aut Zhao, Huifang verfasserin aut Liu, Dahuan verfasserin aut Enthalten in Journal of solid state chemistry Orlando, Fla. : Academic Press, 1969 317 Online-Ressource (DE-627)267328451 (DE-600)1469806-7 (DE-576)10337325X nnns volume:317 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.90 Festkörperchemie AR 317
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author	Li, Gan
spellingShingle	Li, Gan ddc 540 bkl 35.90 misc Adsorption misc Metal-organic framework misc Hydrogen bond misc π−π interaction misc Theoretical calculation Effective removal of nitroimidazole antibiotics in aqueous solution by an aluminum-based metal-organic framework: Performance and mechanistic studies
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topic_title	540 DE-600 35.90 bkl Effective removal of nitroimidazole antibiotics in aqueous solution by an aluminum-based metal-organic framework: Performance and mechanistic studies Adsorption Metal-organic framework Hydrogen bond π−π interaction Theoretical calculation
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title	Effective removal of nitroimidazole antibiotics in aqueous solution by an aluminum-based metal-organic framework: Performance and mechanistic studies
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title_full	Effective removal of nitroimidazole antibiotics in aqueous solution by an aluminum-based metal-organic framework: Performance and mechanistic studies
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title_sort	effective removal of nitroimidazole antibiotics in aqueous solution by an aluminum-based metal-organic framework: performance and mechanistic studies
title_auth	Effective removal of nitroimidazole antibiotics in aqueous solution by an aluminum-based metal-organic framework: Performance and mechanistic studies
abstract	The removal of antibiotics from wastewater has received extensive attention. An aluminum-based metal-organic framework (Al-TCPP) was synthesized as an adsorbent to remove ornidazole (ONZ) and metronidazole (MNZ). Al-TCPP has high adsorption capacities of 609.8 mg g−1 and 320.5 mg g−1 for ONZ and MNZ, respectively, superior to the reported adsorbents. And the adsorption data can fit well with the Langmuir model and the pseudo-second-order model. Besides, the adsorbent exhibits excellent anti-interference to coexisting salts and pH, which indicates that it has good practical application value. Furthermore, the possible adsorption mechanisms were proposed by FT-IR, XPS, Zeta potential, theoretical calculation, as well as the control experiments. These results indicate that hydrogen bonding interaction dominates the adsorption process. Therefore, Al-TCPP may have broad application prospects in purifying wastewater containing nitroimidazole antibiotics. The proposal of the dominant force is beneficial to the development of new adsorbents for the removal of antibiotics from aqueous solution.
abstractGer	The removal of antibiotics from wastewater has received extensive attention. An aluminum-based metal-organic framework (Al-TCPP) was synthesized as an adsorbent to remove ornidazole (ONZ) and metronidazole (MNZ). Al-TCPP has high adsorption capacities of 609.8 mg g−1 and 320.5 mg g−1 for ONZ and MNZ, respectively, superior to the reported adsorbents. And the adsorption data can fit well with the Langmuir model and the pseudo-second-order model. Besides, the adsorbent exhibits excellent anti-interference to coexisting salts and pH, which indicates that it has good practical application value. Furthermore, the possible adsorption mechanisms were proposed by FT-IR, XPS, Zeta potential, theoretical calculation, as well as the control experiments. These results indicate that hydrogen bonding interaction dominates the adsorption process. Therefore, Al-TCPP may have broad application prospects in purifying wastewater containing nitroimidazole antibiotics. The proposal of the dominant force is beneficial to the development of new adsorbents for the removal of antibiotics from aqueous solution.
abstract_unstemmed	The removal of antibiotics from wastewater has received extensive attention. An aluminum-based metal-organic framework (Al-TCPP) was synthesized as an adsorbent to remove ornidazole (ONZ) and metronidazole (MNZ). Al-TCPP has high adsorption capacities of 609.8 mg g−1 and 320.5 mg g−1 for ONZ and MNZ, respectively, superior to the reported adsorbents. And the adsorption data can fit well with the Langmuir model and the pseudo-second-order model. Besides, the adsorbent exhibits excellent anti-interference to coexisting salts and pH, which indicates that it has good practical application value. Furthermore, the possible adsorption mechanisms were proposed by FT-IR, XPS, Zeta potential, theoretical calculation, as well as the control experiments. These results indicate that hydrogen bonding interaction dominates the adsorption process. Therefore, Al-TCPP may have broad application prospects in purifying wastewater containing nitroimidazole antibiotics. The proposal of the dominant force is beneficial to the development of new adsorbents for the removal of antibiotics from aqueous solution.
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title_short	Effective removal of nitroimidazole antibiotics in aqueous solution by an aluminum-based metal-organic framework: Performance and mechanistic studies
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up_date	2024-07-06T21:11:38.749Z
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An aluminum-based metal-organic framework (Al-TCPP) was synthesized as an adsorbent to remove ornidazole (ONZ) and metronidazole (MNZ). Al-TCPP has high adsorption capacities of 609.8 mg g−1 and 320.5 mg g−1 for ONZ and MNZ, respectively, superior to the reported adsorbents. And the adsorption data can fit well with the Langmuir model and the pseudo-second-order model. Besides, the adsorbent exhibits excellent anti-interference to coexisting salts and pH, which indicates that it has good practical application value. Furthermore, the possible adsorption mechanisms were proposed by FT-IR, XPS, Zeta potential, theoretical calculation, as well as the control experiments. These results indicate that hydrogen bonding interaction dominates the adsorption process. Therefore, Al-TCPP may have broad application prospects in purifying wastewater containing nitroimidazole antibiotics. 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Effective removal of nitroimidazole antibiotics in aqueous solution by an aluminum-based metal-organic framework: Performance and mechanistic studies

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