Synthesis of Zn-Al layered double oxides using eucalyptus leaf extract as template for efficient and ultrafast thorium(IV) removal

Efficient capture of Th(IV) from aqueous solution is of importance to both solve the radioactive pollution for environmental safety and provide clean energy for sustainable development. However, it still faces huge challenge. In this study, eucalyptus leaf extract was applied as template agent to fa...
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Autor*in:	Chen, Congcong [verfasserIn] Xie, Ying [verfasserIn] Jia, Lingyi [verfasserIn] Zhang, Yong [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2022

Schlagwörter:	Layered double oxides Eucalyptus leaf extract Th(IV) Removal

Übergeordnetes Werk:	Enthalten in: Journal of molecular liquids - New York, NY [u.a.] : Elsevier, 1983, 369
Übergeordnetes Werk:	volume:369

DOI / URN:	10.1016/j.molliq.2022.120973

Katalog-ID:	ELV00900792X

Internformat


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520			\|a Efficient capture of Th(IV) from aqueous solution is of importance to both solve the radioactive pollution for environmental safety and provide clean energy for sustainable development. However, it still faces huge challenge. In this study, eucalyptus leaf extract was applied as template agent to fabricate Zn/Al-bimetallic layered double oxides (ZnAlLDO), providing more active sites for Th(IV) removal. The removal process of Th(IV) onto ZnAlLDO could reach equilibrium within 5 min and the maximum removal capacity calculated from the Langmuir model was 1153.71 mg g−1 at pH = 4.0 and 298 K. Over 97 % Th(IV) could be removed by ZnAlLDO during the dynamic adsorption process and the removal efficiency still remained at a high level (85 %) after 5 cycles. The Th(IV) removal process on ZnAlLDO was ascribed to electrostatic attraction, complexation and ion exchange. It could be believed that the ZnAlLDO with large removal capacity (1155.5 mg g−1), fast equilibrium time (5 min) and easy desorption (91.76 %) with high recovery (85 %) might be a promising adsorbent for the separation of Th(IV).
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matchkey_str	article:18733166:2022----::yteiozalyrdobexdssneclpulaetatsepaeoefce
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allfields	10.1016/j.molliq.2022.120973 doi (DE-627)ELV00900792X (ELSEVIER)S0167-7322(22)02512-0 DE-627 ger DE-627 rda eng 540 DE-600 35.21 bkl Chen, Congcong verfasserin aut Synthesis of Zn-Al layered double oxides using eucalyptus leaf extract as template for efficient and ultrafast thorium(IV) removal 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Efficient capture of Th(IV) from aqueous solution is of importance to both solve the radioactive pollution for environmental safety and provide clean energy for sustainable development. However, it still faces huge challenge. In this study, eucalyptus leaf extract was applied as template agent to fabricate Zn/Al-bimetallic layered double oxides (ZnAlLDO), providing more active sites for Th(IV) removal. The removal process of Th(IV) onto ZnAlLDO could reach equilibrium within 5 min and the maximum removal capacity calculated from the Langmuir model was 1153.71 mg g−1 at pH = 4.0 and 298 K. Over 97 % Th(IV) could be removed by ZnAlLDO during the dynamic adsorption process and the removal efficiency still remained at a high level (85 %) after 5 cycles. The Th(IV) removal process on ZnAlLDO was ascribed to electrostatic attraction, complexation and ion exchange. It could be believed that the ZnAlLDO with large removal capacity (1155.5 mg g−1), fast equilibrium time (5 min) and easy desorption (91.76 %) with high recovery (85 %) might be a promising adsorbent for the separation of Th(IV). Layered double oxides Eucalyptus leaf extract Th(IV) Removal Xie, Ying verfasserin aut Jia, Lingyi verfasserin aut Zhang, Yong verfasserin aut Enthalten in Journal of molecular liquids New York, NY [u.a.] : Elsevier, 1983 369 Online-Ressource (DE-627)302469664 (DE-600)1491496-7 (DE-576)259483915 1873-3166 nnns volume:369 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_374 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2807 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.21 Lösungen Flüssigkeiten Physikalische Chemie AR 369
spelling	10.1016/j.molliq.2022.120973 doi (DE-627)ELV00900792X (ELSEVIER)S0167-7322(22)02512-0 DE-627 ger DE-627 rda eng 540 DE-600 35.21 bkl Chen, Congcong verfasserin aut Synthesis of Zn-Al layered double oxides using eucalyptus leaf extract as template for efficient and ultrafast thorium(IV) removal 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Efficient capture of Th(IV) from aqueous solution is of importance to both solve the radioactive pollution for environmental safety and provide clean energy for sustainable development. However, it still faces huge challenge. In this study, eucalyptus leaf extract was applied as template agent to fabricate Zn/Al-bimetallic layered double oxides (ZnAlLDO), providing more active sites for Th(IV) removal. The removal process of Th(IV) onto ZnAlLDO could reach equilibrium within 5 min and the maximum removal capacity calculated from the Langmuir model was 1153.71 mg g−1 at pH = 4.0 and 298 K. Over 97 % Th(IV) could be removed by ZnAlLDO during the dynamic adsorption process and the removal efficiency still remained at a high level (85 %) after 5 cycles. The Th(IV) removal process on ZnAlLDO was ascribed to electrostatic attraction, complexation and ion exchange. It could be believed that the ZnAlLDO with large removal capacity (1155.5 mg g−1), fast equilibrium time (5 min) and easy desorption (91.76 %) with high recovery (85 %) might be a promising adsorbent for the separation of Th(IV). Layered double oxides Eucalyptus leaf extract Th(IV) Removal Xie, Ying verfasserin aut Jia, Lingyi verfasserin aut Zhang, Yong verfasserin aut Enthalten in Journal of molecular liquids New York, NY [u.a.] : Elsevier, 1983 369 Online-Ressource (DE-627)302469664 (DE-600)1491496-7 (DE-576)259483915 1873-3166 nnns volume:369 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_374 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2807 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.21 Lösungen Flüssigkeiten Physikalische Chemie AR 369
allfields_unstemmed	10.1016/j.molliq.2022.120973 doi (DE-627)ELV00900792X (ELSEVIER)S0167-7322(22)02512-0 DE-627 ger DE-627 rda eng 540 DE-600 35.21 bkl Chen, Congcong verfasserin aut Synthesis of Zn-Al layered double oxides using eucalyptus leaf extract as template for efficient and ultrafast thorium(IV) removal 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Efficient capture of Th(IV) from aqueous solution is of importance to both solve the radioactive pollution for environmental safety and provide clean energy for sustainable development. However, it still faces huge challenge. In this study, eucalyptus leaf extract was applied as template agent to fabricate Zn/Al-bimetallic layered double oxides (ZnAlLDO), providing more active sites for Th(IV) removal. The removal process of Th(IV) onto ZnAlLDO could reach equilibrium within 5 min and the maximum removal capacity calculated from the Langmuir model was 1153.71 mg g−1 at pH = 4.0 and 298 K. Over 97 % Th(IV) could be removed by ZnAlLDO during the dynamic adsorption process and the removal efficiency still remained at a high level (85 %) after 5 cycles. The Th(IV) removal process on ZnAlLDO was ascribed to electrostatic attraction, complexation and ion exchange. It could be believed that the ZnAlLDO with large removal capacity (1155.5 mg g−1), fast equilibrium time (5 min) and easy desorption (91.76 %) with high recovery (85 %) might be a promising adsorbent for the separation of Th(IV). Layered double oxides Eucalyptus leaf extract Th(IV) Removal Xie, Ying verfasserin aut Jia, Lingyi verfasserin aut Zhang, Yong verfasserin aut Enthalten in Journal of molecular liquids New York, NY [u.a.] : Elsevier, 1983 369 Online-Ressource (DE-627)302469664 (DE-600)1491496-7 (DE-576)259483915 1873-3166 nnns volume:369 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_374 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2807 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.21 Lösungen Flüssigkeiten Physikalische Chemie AR 369
allfieldsGer	10.1016/j.molliq.2022.120973 doi (DE-627)ELV00900792X (ELSEVIER)S0167-7322(22)02512-0 DE-627 ger DE-627 rda eng 540 DE-600 35.21 bkl Chen, Congcong verfasserin aut Synthesis of Zn-Al layered double oxides using eucalyptus leaf extract as template for efficient and ultrafast thorium(IV) removal 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Efficient capture of Th(IV) from aqueous solution is of importance to both solve the radioactive pollution for environmental safety and provide clean energy for sustainable development. However, it still faces huge challenge. In this study, eucalyptus leaf extract was applied as template agent to fabricate Zn/Al-bimetallic layered double oxides (ZnAlLDO), providing more active sites for Th(IV) removal. The removal process of Th(IV) onto ZnAlLDO could reach equilibrium within 5 min and the maximum removal capacity calculated from the Langmuir model was 1153.71 mg g−1 at pH = 4.0 and 298 K. Over 97 % Th(IV) could be removed by ZnAlLDO during the dynamic adsorption process and the removal efficiency still remained at a high level (85 %) after 5 cycles. The Th(IV) removal process on ZnAlLDO was ascribed to electrostatic attraction, complexation and ion exchange. It could be believed that the ZnAlLDO with large removal capacity (1155.5 mg g−1), fast equilibrium time (5 min) and easy desorption (91.76 %) with high recovery (85 %) might be a promising adsorbent for the separation of Th(IV). Layered double oxides Eucalyptus leaf extract Th(IV) Removal Xie, Ying verfasserin aut Jia, Lingyi verfasserin aut Zhang, Yong verfasserin aut Enthalten in Journal of molecular liquids New York, NY [u.a.] : Elsevier, 1983 369 Online-Ressource (DE-627)302469664 (DE-600)1491496-7 (DE-576)259483915 1873-3166 nnns volume:369 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_374 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2807 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.21 Lösungen Flüssigkeiten Physikalische Chemie AR 369
allfieldsSound	10.1016/j.molliq.2022.120973 doi (DE-627)ELV00900792X (ELSEVIER)S0167-7322(22)02512-0 DE-627 ger DE-627 rda eng 540 DE-600 35.21 bkl Chen, Congcong verfasserin aut Synthesis of Zn-Al layered double oxides using eucalyptus leaf extract as template for efficient and ultrafast thorium(IV) removal 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Efficient capture of Th(IV) from aqueous solution is of importance to both solve the radioactive pollution for environmental safety and provide clean energy for sustainable development. However, it still faces huge challenge. In this study, eucalyptus leaf extract was applied as template agent to fabricate Zn/Al-bimetallic layered double oxides (ZnAlLDO), providing more active sites for Th(IV) removal. The removal process of Th(IV) onto ZnAlLDO could reach equilibrium within 5 min and the maximum removal capacity calculated from the Langmuir model was 1153.71 mg g−1 at pH = 4.0 and 298 K. Over 97 % Th(IV) could be removed by ZnAlLDO during the dynamic adsorption process and the removal efficiency still remained at a high level (85 %) after 5 cycles. The Th(IV) removal process on ZnAlLDO was ascribed to electrostatic attraction, complexation and ion exchange. It could be believed that the ZnAlLDO with large removal capacity (1155.5 mg g−1), fast equilibrium time (5 min) and easy desorption (91.76 %) with high recovery (85 %) might be a promising adsorbent for the separation of Th(IV). Layered double oxides Eucalyptus leaf extract Th(IV) Removal Xie, Ying verfasserin aut Jia, Lingyi verfasserin aut Zhang, Yong verfasserin aut Enthalten in Journal of molecular liquids New York, NY [u.a.] : Elsevier, 1983 369 Online-Ressource (DE-627)302469664 (DE-600)1491496-7 (DE-576)259483915 1873-3166 nnns volume:369 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_374 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2807 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.21 Lösungen Flüssigkeiten Physikalische Chemie AR 369
language	English
source	Enthalten in Journal of molecular liquids 369 volume:369
sourceStr	Enthalten in Journal of molecular liquids 369 volume:369
format_phy_str_mv	Article
bklname	Lösungen Flüssigkeiten
institution	findex.gbv.de
topic_facet	Layered double oxides Eucalyptus leaf extract Th(IV) Removal
dewey-raw	540
isfreeaccess_bool	false
container_title	Journal of molecular liquids
authorswithroles_txt_mv	Chen, Congcong @@aut@@ Xie, Ying @@aut@@ Jia, Lingyi @@aut@@ Zhang, Yong @@aut@@
publishDateDaySort_date	2022-01-01T00:00:00Z
hierarchy_top_id	302469664
dewey-sort	3540
id	ELV00900792X
language_de	englisch
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author	Chen, Congcong
spellingShingle	Chen, Congcong ddc 540 bkl 35.21 misc Layered double oxides misc Eucalyptus leaf extract misc Th(IV) misc Removal Synthesis of Zn-Al layered double oxides using eucalyptus leaf extract as template for efficient and ultrafast thorium(IV) removal
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topic_title	540 DE-600 35.21 bkl Synthesis of Zn-Al layered double oxides using eucalyptus leaf extract as template for efficient and ultrafast thorium(IV) removal Layered double oxides Eucalyptus leaf extract Th(IV) Removal
topic	ddc 540 bkl 35.21 misc Layered double oxides misc Eucalyptus leaf extract misc Th(IV) misc Removal
topic_unstemmed	ddc 540 bkl 35.21 misc Layered double oxides misc Eucalyptus leaf extract misc Th(IV) misc Removal
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title	Synthesis of Zn-Al layered double oxides using eucalyptus leaf extract as template for efficient and ultrafast thorium(IV) removal
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title_full	Synthesis of Zn-Al layered double oxides using eucalyptus leaf extract as template for efficient and ultrafast thorium(IV) removal
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author_browse	Chen, Congcong Xie, Ying Jia, Lingyi Zhang, Yong
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title_sort	synthesis of zn-al layered double oxides using eucalyptus leaf extract as template for efficient and ultrafast thorium(iv) removal
title_auth	Synthesis of Zn-Al layered double oxides using eucalyptus leaf extract as template for efficient and ultrafast thorium(IV) removal
abstract	Efficient capture of Th(IV) from aqueous solution is of importance to both solve the radioactive pollution for environmental safety and provide clean energy for sustainable development. However, it still faces huge challenge. In this study, eucalyptus leaf extract was applied as template agent to fabricate Zn/Al-bimetallic layered double oxides (ZnAlLDO), providing more active sites for Th(IV) removal. The removal process of Th(IV) onto ZnAlLDO could reach equilibrium within 5 min and the maximum removal capacity calculated from the Langmuir model was 1153.71 mg g−1 at pH = 4.0 and 298 K. Over 97 % Th(IV) could be removed by ZnAlLDO during the dynamic adsorption process and the removal efficiency still remained at a high level (85 %) after 5 cycles. The Th(IV) removal process on ZnAlLDO was ascribed to electrostatic attraction, complexation and ion exchange. It could be believed that the ZnAlLDO with large removal capacity (1155.5 mg g−1), fast equilibrium time (5 min) and easy desorption (91.76 %) with high recovery (85 %) might be a promising adsorbent for the separation of Th(IV).
abstractGer	Efficient capture of Th(IV) from aqueous solution is of importance to both solve the radioactive pollution for environmental safety and provide clean energy for sustainable development. However, it still faces huge challenge. In this study, eucalyptus leaf extract was applied as template agent to fabricate Zn/Al-bimetallic layered double oxides (ZnAlLDO), providing more active sites for Th(IV) removal. The removal process of Th(IV) onto ZnAlLDO could reach equilibrium within 5 min and the maximum removal capacity calculated from the Langmuir model was 1153.71 mg g−1 at pH = 4.0 and 298 K. Over 97 % Th(IV) could be removed by ZnAlLDO during the dynamic adsorption process and the removal efficiency still remained at a high level (85 %) after 5 cycles. The Th(IV) removal process on ZnAlLDO was ascribed to electrostatic attraction, complexation and ion exchange. It could be believed that the ZnAlLDO with large removal capacity (1155.5 mg g−1), fast equilibrium time (5 min) and easy desorption (91.76 %) with high recovery (85 %) might be a promising adsorbent for the separation of Th(IV).
abstract_unstemmed	Efficient capture of Th(IV) from aqueous solution is of importance to both solve the radioactive pollution for environmental safety and provide clean energy for sustainable development. However, it still faces huge challenge. In this study, eucalyptus leaf extract was applied as template agent to fabricate Zn/Al-bimetallic layered double oxides (ZnAlLDO), providing more active sites for Th(IV) removal. The removal process of Th(IV) onto ZnAlLDO could reach equilibrium within 5 min and the maximum removal capacity calculated from the Langmuir model was 1153.71 mg g−1 at pH = 4.0 and 298 K. Over 97 % Th(IV) could be removed by ZnAlLDO during the dynamic adsorption process and the removal efficiency still remained at a high level (85 %) after 5 cycles. The Th(IV) removal process on ZnAlLDO was ascribed to electrostatic attraction, complexation and ion exchange. It could be believed that the ZnAlLDO with large removal capacity (1155.5 mg g−1), fast equilibrium time (5 min) and easy desorption (91.76 %) with high recovery (85 %) might be a promising adsorbent for the separation of Th(IV).
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title_short	Synthesis of Zn-Al layered double oxides using eucalyptus leaf extract as template for efficient and ultrafast thorium(IV) removal
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up_date	2024-07-06T21:39:58.110Z
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Synthesis of Zn-Al layered double oxides using eucalyptus leaf extract as template for efficient and ultrafast thorium(IV) removal

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