Interspersing CdS nanodots into iodine vacancy-rich BiOI sphere for photocatalytic lignin valorization
Flower-like BiOI was decorated by CdS nanodots and followed by the introduction of iodine vacancies (VI) for photocatalytic sodium lignosulfonate (SLS) valorization under visible light. The iodine vacancies could adjust the band configuration, strengthen the light absorption and act as electron trap...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Dai, Dingliang [verfasserIn] Qiu, Jianhao [verfasserIn] Xia, Guanglu [verfasserIn] Zhang, Lu [verfasserIn] Ma, Hong [verfasserIn] Yang, Luan [verfasserIn] Yao, Jianfeng [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2022 |
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| Schlagwörter: |
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| Übergeordnetes Werk: |
Enthalten in: International journal of biological macromolecules - New York, NY [u.a.] : Elsevier, 1979, 227, Seite 1317-1324 |
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| Übergeordnetes Werk: |
volume:227 ; pages:1317-1324 |
| DOI / URN: |
10.1016/j.ijbiomac.2022.12.007 |
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| 520 | |a Flower-like BiOI was decorated by CdS nanodots and followed by the introduction of iodine vacancies (VI) for photocatalytic sodium lignosulfonate (SLS) valorization under visible light. The iodine vacancies could adjust the band configuration, strengthen the light absorption and act as electron traps, while the intimate contact between BiOI and CdS nanodots provides a high-speed channel for charge transfer. As a consequence, the photocatalytic performance of SLS conversion into value-added vanillin was greatly improved over CdS/BiOI-VI compared with those of CdS, BiOI and CdS/BiOI. The highest yield of vanillin is 10.95 mg/gSLS over CdS/BiOI-VI, about 5, 8.7, 1.3 times those of CdS, BiOI, CdS/BiOI, respectively, and exceeding most related photocatalysts reported elsewhere. More significantly, as to the lignin from Masson pine and alkali lignin, the corresponding vanillin yield can reach 7.04 and 6.54 mg/glignin, respectively, under the same condition, which suggests the great potential and universality for photocatalytic lignin valorization over such CdS/BiOI-VI heterostructure. | ||
| 650 | 4 | |a Photocatalysis | |
| 650 | 4 | |a Lignin valorization | |
| 650 | 4 | |a Vanillin | |
| 700 | 1 | |a Qiu, Jianhao |e verfasserin |4 aut | |
| 700 | 1 | |a Xia, Guanglu |e verfasserin |4 aut | |
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| 700 | 1 | |a Ma, Hong |e verfasserin |4 aut | |
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| 700 | 1 | |a Yao, Jianfeng |e verfasserin |4 aut | |
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10.1016/j.ijbiomac.2022.12.007 doi (DE-627)ELV009056831 (ELSEVIER)S0141-8130(22)02898-7 DE-627 ger DE-627 rda eng 540 570 VZ BIODIV DE-30 fid 35.80 bkl 58.30 bkl Dai, Dingliang verfasserin aut Interspersing CdS nanodots into iodine vacancy-rich BiOI sphere for photocatalytic lignin valorization 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Flower-like BiOI was decorated by CdS nanodots and followed by the introduction of iodine vacancies (VI) for photocatalytic sodium lignosulfonate (SLS) valorization under visible light. The iodine vacancies could adjust the band configuration, strengthen the light absorption and act as electron traps, while the intimate contact between BiOI and CdS nanodots provides a high-speed channel for charge transfer. As a consequence, the photocatalytic performance of SLS conversion into value-added vanillin was greatly improved over CdS/BiOI-VI compared with those of CdS, BiOI and CdS/BiOI. The highest yield of vanillin is 10.95 mg/gSLS over CdS/BiOI-VI, about 5, 8.7, 1.3 times those of CdS, BiOI, CdS/BiOI, respectively, and exceeding most related photocatalysts reported elsewhere. More significantly, as to the lignin from Masson pine and alkali lignin, the corresponding vanillin yield can reach 7.04 and 6.54 mg/glignin, respectively, under the same condition, which suggests the great potential and universality for photocatalytic lignin valorization over such CdS/BiOI-VI heterostructure. Photocatalysis Lignin valorization Vanillin Qiu, Jianhao verfasserin aut Xia, Guanglu verfasserin aut Zhang, Lu verfasserin aut Ma, Hong verfasserin aut Yang, Luan verfasserin aut Yao, Jianfeng verfasserin aut Enthalten in International journal of biological macromolecules New York, NY [u.a.] : Elsevier, 1979 227, Seite 1317-1324 Online-Ressource (DE-627)30089502X (DE-600)1483284-7 (DE-576)259270814 1879-0003 nnns volume:227 pages:1317-1324 GBV_USEFLAG_U GBV_ELV SYSFLAG_U FID-BIODIV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.80 Makromolekulare Chemie VZ 58.30 Biotechnologie VZ AR 227 1317-1324 |
| spelling |
10.1016/j.ijbiomac.2022.12.007 doi (DE-627)ELV009056831 (ELSEVIER)S0141-8130(22)02898-7 DE-627 ger DE-627 rda eng 540 570 VZ BIODIV DE-30 fid 35.80 bkl 58.30 bkl Dai, Dingliang verfasserin aut Interspersing CdS nanodots into iodine vacancy-rich BiOI sphere for photocatalytic lignin valorization 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Flower-like BiOI was decorated by CdS nanodots and followed by the introduction of iodine vacancies (VI) for photocatalytic sodium lignosulfonate (SLS) valorization under visible light. The iodine vacancies could adjust the band configuration, strengthen the light absorption and act as electron traps, while the intimate contact between BiOI and CdS nanodots provides a high-speed channel for charge transfer. As a consequence, the photocatalytic performance of SLS conversion into value-added vanillin was greatly improved over CdS/BiOI-VI compared with those of CdS, BiOI and CdS/BiOI. The highest yield of vanillin is 10.95 mg/gSLS over CdS/BiOI-VI, about 5, 8.7, 1.3 times those of CdS, BiOI, CdS/BiOI, respectively, and exceeding most related photocatalysts reported elsewhere. More significantly, as to the lignin from Masson pine and alkali lignin, the corresponding vanillin yield can reach 7.04 and 6.54 mg/glignin, respectively, under the same condition, which suggests the great potential and universality for photocatalytic lignin valorization over such CdS/BiOI-VI heterostructure. Photocatalysis Lignin valorization Vanillin Qiu, Jianhao verfasserin aut Xia, Guanglu verfasserin aut Zhang, Lu verfasserin aut Ma, Hong verfasserin aut Yang, Luan verfasserin aut Yao, Jianfeng verfasserin aut Enthalten in International journal of biological macromolecules New York, NY [u.a.] : Elsevier, 1979 227, Seite 1317-1324 Online-Ressource (DE-627)30089502X (DE-600)1483284-7 (DE-576)259270814 1879-0003 nnns volume:227 pages:1317-1324 GBV_USEFLAG_U GBV_ELV SYSFLAG_U FID-BIODIV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.80 Makromolekulare Chemie VZ 58.30 Biotechnologie VZ AR 227 1317-1324 |
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10.1016/j.ijbiomac.2022.12.007 doi (DE-627)ELV009056831 (ELSEVIER)S0141-8130(22)02898-7 DE-627 ger DE-627 rda eng 540 570 VZ BIODIV DE-30 fid 35.80 bkl 58.30 bkl Dai, Dingliang verfasserin aut Interspersing CdS nanodots into iodine vacancy-rich BiOI sphere for photocatalytic lignin valorization 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Flower-like BiOI was decorated by CdS nanodots and followed by the introduction of iodine vacancies (VI) for photocatalytic sodium lignosulfonate (SLS) valorization under visible light. The iodine vacancies could adjust the band configuration, strengthen the light absorption and act as electron traps, while the intimate contact between BiOI and CdS nanodots provides a high-speed channel for charge transfer. As a consequence, the photocatalytic performance of SLS conversion into value-added vanillin was greatly improved over CdS/BiOI-VI compared with those of CdS, BiOI and CdS/BiOI. The highest yield of vanillin is 10.95 mg/gSLS over CdS/BiOI-VI, about 5, 8.7, 1.3 times those of CdS, BiOI, CdS/BiOI, respectively, and exceeding most related photocatalysts reported elsewhere. More significantly, as to the lignin from Masson pine and alkali lignin, the corresponding vanillin yield can reach 7.04 and 6.54 mg/glignin, respectively, under the same condition, which suggests the great potential and universality for photocatalytic lignin valorization over such CdS/BiOI-VI heterostructure. Photocatalysis Lignin valorization Vanillin Qiu, Jianhao verfasserin aut Xia, Guanglu verfasserin aut Zhang, Lu verfasserin aut Ma, Hong verfasserin aut Yang, Luan verfasserin aut Yao, Jianfeng verfasserin aut Enthalten in International journal of biological macromolecules New York, NY [u.a.] : Elsevier, 1979 227, Seite 1317-1324 Online-Ressource (DE-627)30089502X (DE-600)1483284-7 (DE-576)259270814 1879-0003 nnns volume:227 pages:1317-1324 GBV_USEFLAG_U GBV_ELV SYSFLAG_U FID-BIODIV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.80 Makromolekulare Chemie VZ 58.30 Biotechnologie VZ AR 227 1317-1324 |
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10.1016/j.ijbiomac.2022.12.007 doi (DE-627)ELV009056831 (ELSEVIER)S0141-8130(22)02898-7 DE-627 ger DE-627 rda eng 540 570 VZ BIODIV DE-30 fid 35.80 bkl 58.30 bkl Dai, Dingliang verfasserin aut Interspersing CdS nanodots into iodine vacancy-rich BiOI sphere for photocatalytic lignin valorization 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Flower-like BiOI was decorated by CdS nanodots and followed by the introduction of iodine vacancies (VI) for photocatalytic sodium lignosulfonate (SLS) valorization under visible light. The iodine vacancies could adjust the band configuration, strengthen the light absorption and act as electron traps, while the intimate contact between BiOI and CdS nanodots provides a high-speed channel for charge transfer. As a consequence, the photocatalytic performance of SLS conversion into value-added vanillin was greatly improved over CdS/BiOI-VI compared with those of CdS, BiOI and CdS/BiOI. The highest yield of vanillin is 10.95 mg/gSLS over CdS/BiOI-VI, about 5, 8.7, 1.3 times those of CdS, BiOI, CdS/BiOI, respectively, and exceeding most related photocatalysts reported elsewhere. More significantly, as to the lignin from Masson pine and alkali lignin, the corresponding vanillin yield can reach 7.04 and 6.54 mg/glignin, respectively, under the same condition, which suggests the great potential and universality for photocatalytic lignin valorization over such CdS/BiOI-VI heterostructure. Photocatalysis Lignin valorization Vanillin Qiu, Jianhao verfasserin aut Xia, Guanglu verfasserin aut Zhang, Lu verfasserin aut Ma, Hong verfasserin aut Yang, Luan verfasserin aut Yao, Jianfeng verfasserin aut Enthalten in International journal of biological macromolecules New York, NY [u.a.] : Elsevier, 1979 227, Seite 1317-1324 Online-Ressource (DE-627)30089502X (DE-600)1483284-7 (DE-576)259270814 1879-0003 nnns volume:227 pages:1317-1324 GBV_USEFLAG_U GBV_ELV SYSFLAG_U FID-BIODIV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.80 Makromolekulare Chemie VZ 58.30 Biotechnologie VZ AR 227 1317-1324 |
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10.1016/j.ijbiomac.2022.12.007 doi (DE-627)ELV009056831 (ELSEVIER)S0141-8130(22)02898-7 DE-627 ger DE-627 rda eng 540 570 VZ BIODIV DE-30 fid 35.80 bkl 58.30 bkl Dai, Dingliang verfasserin aut Interspersing CdS nanodots into iodine vacancy-rich BiOI sphere for photocatalytic lignin valorization 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Flower-like BiOI was decorated by CdS nanodots and followed by the introduction of iodine vacancies (VI) for photocatalytic sodium lignosulfonate (SLS) valorization under visible light. The iodine vacancies could adjust the band configuration, strengthen the light absorption and act as electron traps, while the intimate contact between BiOI and CdS nanodots provides a high-speed channel for charge transfer. As a consequence, the photocatalytic performance of SLS conversion into value-added vanillin was greatly improved over CdS/BiOI-VI compared with those of CdS, BiOI and CdS/BiOI. The highest yield of vanillin is 10.95 mg/gSLS over CdS/BiOI-VI, about 5, 8.7, 1.3 times those of CdS, BiOI, CdS/BiOI, respectively, and exceeding most related photocatalysts reported elsewhere. More significantly, as to the lignin from Masson pine and alkali lignin, the corresponding vanillin yield can reach 7.04 and 6.54 mg/glignin, respectively, under the same condition, which suggests the great potential and universality for photocatalytic lignin valorization over such CdS/BiOI-VI heterostructure. Photocatalysis Lignin valorization Vanillin Qiu, Jianhao verfasserin aut Xia, Guanglu verfasserin aut Zhang, Lu verfasserin aut Ma, Hong verfasserin aut Yang, Luan verfasserin aut Yao, Jianfeng verfasserin aut Enthalten in International journal of biological macromolecules New York, NY [u.a.] : Elsevier, 1979 227, Seite 1317-1324 Online-Ressource (DE-627)30089502X (DE-600)1483284-7 (DE-576)259270814 1879-0003 nnns volume:227 pages:1317-1324 GBV_USEFLAG_U GBV_ELV SYSFLAG_U FID-BIODIV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 35.80 Makromolekulare Chemie VZ 58.30 Biotechnologie VZ AR 227 1317-1324 |
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540 570 VZ BIODIV DE-30 fid 35.80 bkl 58.30 bkl Interspersing CdS nanodots into iodine vacancy-rich BiOI sphere for photocatalytic lignin valorization Photocatalysis Lignin valorization Vanillin |
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Interspersing CdS nanodots into iodine vacancy-rich BiOI sphere for photocatalytic lignin valorization |
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Dai, Dingliang Qiu, Jianhao Xia, Guanglu Zhang, Lu Ma, Hong Yang, Luan Yao, Jianfeng |
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interspersing cds nanodots into iodine vacancy-rich bioi sphere for photocatalytic lignin valorization |
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Interspersing CdS nanodots into iodine vacancy-rich BiOI sphere for photocatalytic lignin valorization |
| abstract |
Flower-like BiOI was decorated by CdS nanodots and followed by the introduction of iodine vacancies (VI) for photocatalytic sodium lignosulfonate (SLS) valorization under visible light. The iodine vacancies could adjust the band configuration, strengthen the light absorption and act as electron traps, while the intimate contact between BiOI and CdS nanodots provides a high-speed channel for charge transfer. As a consequence, the photocatalytic performance of SLS conversion into value-added vanillin was greatly improved over CdS/BiOI-VI compared with those of CdS, BiOI and CdS/BiOI. The highest yield of vanillin is 10.95 mg/gSLS over CdS/BiOI-VI, about 5, 8.7, 1.3 times those of CdS, BiOI, CdS/BiOI, respectively, and exceeding most related photocatalysts reported elsewhere. More significantly, as to the lignin from Masson pine and alkali lignin, the corresponding vanillin yield can reach 7.04 and 6.54 mg/glignin, respectively, under the same condition, which suggests the great potential and universality for photocatalytic lignin valorization over such CdS/BiOI-VI heterostructure. |
| abstractGer |
Flower-like BiOI was decorated by CdS nanodots and followed by the introduction of iodine vacancies (VI) for photocatalytic sodium lignosulfonate (SLS) valorization under visible light. The iodine vacancies could adjust the band configuration, strengthen the light absorption and act as electron traps, while the intimate contact between BiOI and CdS nanodots provides a high-speed channel for charge transfer. As a consequence, the photocatalytic performance of SLS conversion into value-added vanillin was greatly improved over CdS/BiOI-VI compared with those of CdS, BiOI and CdS/BiOI. The highest yield of vanillin is 10.95 mg/gSLS over CdS/BiOI-VI, about 5, 8.7, 1.3 times those of CdS, BiOI, CdS/BiOI, respectively, and exceeding most related photocatalysts reported elsewhere. More significantly, as to the lignin from Masson pine and alkali lignin, the corresponding vanillin yield can reach 7.04 and 6.54 mg/glignin, respectively, under the same condition, which suggests the great potential and universality for photocatalytic lignin valorization over such CdS/BiOI-VI heterostructure. |
| abstract_unstemmed |
Flower-like BiOI was decorated by CdS nanodots and followed by the introduction of iodine vacancies (VI) for photocatalytic sodium lignosulfonate (SLS) valorization under visible light. The iodine vacancies could adjust the band configuration, strengthen the light absorption and act as electron traps, while the intimate contact between BiOI and CdS nanodots provides a high-speed channel for charge transfer. As a consequence, the photocatalytic performance of SLS conversion into value-added vanillin was greatly improved over CdS/BiOI-VI compared with those of CdS, BiOI and CdS/BiOI. The highest yield of vanillin is 10.95 mg/gSLS over CdS/BiOI-VI, about 5, 8.7, 1.3 times those of CdS, BiOI, CdS/BiOI, respectively, and exceeding most related photocatalysts reported elsewhere. More significantly, as to the lignin from Masson pine and alkali lignin, the corresponding vanillin yield can reach 7.04 and 6.54 mg/glignin, respectively, under the same condition, which suggests the great potential and universality for photocatalytic lignin valorization over such CdS/BiOI-VI heterostructure. |
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