Recent progress in heteroatom-doped carbon electrocatalysts for the two-electron oxygen reduction reaction
The electrochemical synthesis of hydrogen peroxide has received much attention due to its on-site production, absence of organic impurities during the synthesis, environmentally-friendly and low energy input with no need for further purification. This review focused on the metal-free heteroatom-dope...
Ausführliche Beschreibung
Autor*in: |
Byeon, Ayeong [verfasserIn] Yun, Won Chan [verfasserIn] Kim, Jong Min [verfasserIn] Lee, Jae W. [verfasserIn] |
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Format: |
E-Artikel |
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Sprache: |
Englisch |
Erschienen: |
2022 |
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Schlagwörter: |
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Übergeordnetes Werk: |
Enthalten in: The chemical engineering journal - Amsterdam : Elsevier, 1997, 456 |
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Übergeordnetes Werk: |
volume:456 |
DOI / URN: |
10.1016/j.cej.2022.141042 |
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Katalog-ID: |
ELV009088431 |
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520 | |a The electrochemical synthesis of hydrogen peroxide has received much attention due to its on-site production, absence of organic impurities during the synthesis, environmentally-friendly and low energy input with no need for further purification. This review focused on the metal-free heteroatom-doped carbon catalyst for the generation of hydrogen peroxide by the two-electron oxygen reduction reaction (2e- ORR). Depending on the type of heteroatoms, the electronic properties of the carbon can be changed, and they significantly affect the ORR catalytic activity. Even with the same heteroatoms, their specific chemical composition in a carbon frame has a large effect on the electrocatalytic activity. The location of the active catalytic sites within the carbon network is also investigated with a theoretical study, which is important for effective electrocatalysis of the 2e- ORR to occur. The physical and chemical properties of base carbon materials and the reaction environment for ORR such as the pH and additives of the electrolyte are discussed. This review provides fundamental insights into how the moiety of heteroatoms enhances the electrocatalytic activity of metal-free carbon materials for the 2e- ORR. | ||
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10.1016/j.cej.2022.141042 doi (DE-627)ELV009088431 (ELSEVIER)S1385-8947(22)06523-8 DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Byeon, Ayeong verfasserin aut Recent progress in heteroatom-doped carbon electrocatalysts for the two-electron oxygen reduction reaction 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The electrochemical synthesis of hydrogen peroxide has received much attention due to its on-site production, absence of organic impurities during the synthesis, environmentally-friendly and low energy input with no need for further purification. This review focused on the metal-free heteroatom-doped carbon catalyst for the generation of hydrogen peroxide by the two-electron oxygen reduction reaction (2e- ORR). Depending on the type of heteroatoms, the electronic properties of the carbon can be changed, and they significantly affect the ORR catalytic activity. Even with the same heteroatoms, their specific chemical composition in a carbon frame has a large effect on the electrocatalytic activity. The location of the active catalytic sites within the carbon network is also investigated with a theoretical study, which is important for effective electrocatalysis of the 2e- ORR to occur. The physical and chemical properties of base carbon materials and the reaction environment for ORR such as the pH and additives of the electrolyte are discussed. This review provides fundamental insights into how the moiety of heteroatoms enhances the electrocatalytic activity of metal-free carbon materials for the 2e- ORR. Two-electron oxygen reduction reaction H Electrocatalysts Heteroatom-doped carbon Yun, Won Chan verfasserin aut Kim, Jong Min verfasserin aut Lee, Jae W. verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 456 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:456 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 456 045F 660.05 |
spelling |
10.1016/j.cej.2022.141042 doi (DE-627)ELV009088431 (ELSEVIER)S1385-8947(22)06523-8 DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Byeon, Ayeong verfasserin aut Recent progress in heteroatom-doped carbon electrocatalysts for the two-electron oxygen reduction reaction 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The electrochemical synthesis of hydrogen peroxide has received much attention due to its on-site production, absence of organic impurities during the synthesis, environmentally-friendly and low energy input with no need for further purification. This review focused on the metal-free heteroatom-doped carbon catalyst for the generation of hydrogen peroxide by the two-electron oxygen reduction reaction (2e- ORR). Depending on the type of heteroatoms, the electronic properties of the carbon can be changed, and they significantly affect the ORR catalytic activity. Even with the same heteroatoms, their specific chemical composition in a carbon frame has a large effect on the electrocatalytic activity. The location of the active catalytic sites within the carbon network is also investigated with a theoretical study, which is important for effective electrocatalysis of the 2e- ORR to occur. The physical and chemical properties of base carbon materials and the reaction environment for ORR such as the pH and additives of the electrolyte are discussed. This review provides fundamental insights into how the moiety of heteroatoms enhances the electrocatalytic activity of metal-free carbon materials for the 2e- ORR. Two-electron oxygen reduction reaction H Electrocatalysts Heteroatom-doped carbon Yun, Won Chan verfasserin aut Kim, Jong Min verfasserin aut Lee, Jae W. verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 456 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:456 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 456 045F 660.05 |
allfields_unstemmed |
10.1016/j.cej.2022.141042 doi (DE-627)ELV009088431 (ELSEVIER)S1385-8947(22)06523-8 DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Byeon, Ayeong verfasserin aut Recent progress in heteroatom-doped carbon electrocatalysts for the two-electron oxygen reduction reaction 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The electrochemical synthesis of hydrogen peroxide has received much attention due to its on-site production, absence of organic impurities during the synthesis, environmentally-friendly and low energy input with no need for further purification. This review focused on the metal-free heteroatom-doped carbon catalyst for the generation of hydrogen peroxide by the two-electron oxygen reduction reaction (2e- ORR). Depending on the type of heteroatoms, the electronic properties of the carbon can be changed, and they significantly affect the ORR catalytic activity. Even with the same heteroatoms, their specific chemical composition in a carbon frame has a large effect on the electrocatalytic activity. The location of the active catalytic sites within the carbon network is also investigated with a theoretical study, which is important for effective electrocatalysis of the 2e- ORR to occur. The physical and chemical properties of base carbon materials and the reaction environment for ORR such as the pH and additives of the electrolyte are discussed. This review provides fundamental insights into how the moiety of heteroatoms enhances the electrocatalytic activity of metal-free carbon materials for the 2e- ORR. Two-electron oxygen reduction reaction H Electrocatalysts Heteroatom-doped carbon Yun, Won Chan verfasserin aut Kim, Jong Min verfasserin aut Lee, Jae W. verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 456 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:456 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 456 045F 660.05 |
allfieldsGer |
10.1016/j.cej.2022.141042 doi (DE-627)ELV009088431 (ELSEVIER)S1385-8947(22)06523-8 DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Byeon, Ayeong verfasserin aut Recent progress in heteroatom-doped carbon electrocatalysts for the two-electron oxygen reduction reaction 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The electrochemical synthesis of hydrogen peroxide has received much attention due to its on-site production, absence of organic impurities during the synthesis, environmentally-friendly and low energy input with no need for further purification. This review focused on the metal-free heteroatom-doped carbon catalyst for the generation of hydrogen peroxide by the two-electron oxygen reduction reaction (2e- ORR). Depending on the type of heteroatoms, the electronic properties of the carbon can be changed, and they significantly affect the ORR catalytic activity. Even with the same heteroatoms, their specific chemical composition in a carbon frame has a large effect on the electrocatalytic activity. The location of the active catalytic sites within the carbon network is also investigated with a theoretical study, which is important for effective electrocatalysis of the 2e- ORR to occur. The physical and chemical properties of base carbon materials and the reaction environment for ORR such as the pH and additives of the electrolyte are discussed. This review provides fundamental insights into how the moiety of heteroatoms enhances the electrocatalytic activity of metal-free carbon materials for the 2e- ORR. Two-electron oxygen reduction reaction H Electrocatalysts Heteroatom-doped carbon Yun, Won Chan verfasserin aut Kim, Jong Min verfasserin aut Lee, Jae W. verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 456 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:456 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 456 045F 660.05 |
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10.1016/j.cej.2022.141042 doi (DE-627)ELV009088431 (ELSEVIER)S1385-8947(22)06523-8 DE-627 ger DE-627 rda eng 660.05 DE-101 660 DE-101 660 DE-600 58.10 bkl Byeon, Ayeong verfasserin aut Recent progress in heteroatom-doped carbon electrocatalysts for the two-electron oxygen reduction reaction 2022 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The electrochemical synthesis of hydrogen peroxide has received much attention due to its on-site production, absence of organic impurities during the synthesis, environmentally-friendly and low energy input with no need for further purification. This review focused on the metal-free heteroatom-doped carbon catalyst for the generation of hydrogen peroxide by the two-electron oxygen reduction reaction (2e- ORR). Depending on the type of heteroatoms, the electronic properties of the carbon can be changed, and they significantly affect the ORR catalytic activity. Even with the same heteroatoms, their specific chemical composition in a carbon frame has a large effect on the electrocatalytic activity. The location of the active catalytic sites within the carbon network is also investigated with a theoretical study, which is important for effective electrocatalysis of the 2e- ORR to occur. The physical and chemical properties of base carbon materials and the reaction environment for ORR such as the pH and additives of the electrolyte are discussed. This review provides fundamental insights into how the moiety of heteroatoms enhances the electrocatalytic activity of metal-free carbon materials for the 2e- ORR. Two-electron oxygen reduction reaction H Electrocatalysts Heteroatom-doped carbon Yun, Won Chan verfasserin aut Kim, Jong Min verfasserin aut Lee, Jae W. verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 456 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:456 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_224 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2038 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2336 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4313 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4393 58.10 Verfahrenstechnik: Allgemeines AR 456 045F 660.05 |
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Byeon, Ayeong Yun, Won Chan Kim, Jong Min Lee, Jae W. |
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Byeon, Ayeong |
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recent progress in heteroatom-doped carbon electrocatalysts for the two-electron oxygen reduction reaction |
title_auth |
Recent progress in heteroatom-doped carbon electrocatalysts for the two-electron oxygen reduction reaction |
abstract |
The electrochemical synthesis of hydrogen peroxide has received much attention due to its on-site production, absence of organic impurities during the synthesis, environmentally-friendly and low energy input with no need for further purification. This review focused on the metal-free heteroatom-doped carbon catalyst for the generation of hydrogen peroxide by the two-electron oxygen reduction reaction (2e- ORR). Depending on the type of heteroatoms, the electronic properties of the carbon can be changed, and they significantly affect the ORR catalytic activity. Even with the same heteroatoms, their specific chemical composition in a carbon frame has a large effect on the electrocatalytic activity. The location of the active catalytic sites within the carbon network is also investigated with a theoretical study, which is important for effective electrocatalysis of the 2e- ORR to occur. The physical and chemical properties of base carbon materials and the reaction environment for ORR such as the pH and additives of the electrolyte are discussed. This review provides fundamental insights into how the moiety of heteroatoms enhances the electrocatalytic activity of metal-free carbon materials for the 2e- ORR. |
abstractGer |
The electrochemical synthesis of hydrogen peroxide has received much attention due to its on-site production, absence of organic impurities during the synthesis, environmentally-friendly and low energy input with no need for further purification. This review focused on the metal-free heteroatom-doped carbon catalyst for the generation of hydrogen peroxide by the two-electron oxygen reduction reaction (2e- ORR). Depending on the type of heteroatoms, the electronic properties of the carbon can be changed, and they significantly affect the ORR catalytic activity. Even with the same heteroatoms, their specific chemical composition in a carbon frame has a large effect on the electrocatalytic activity. The location of the active catalytic sites within the carbon network is also investigated with a theoretical study, which is important for effective electrocatalysis of the 2e- ORR to occur. The physical and chemical properties of base carbon materials and the reaction environment for ORR such as the pH and additives of the electrolyte are discussed. This review provides fundamental insights into how the moiety of heteroatoms enhances the electrocatalytic activity of metal-free carbon materials for the 2e- ORR. |
abstract_unstemmed |
The electrochemical synthesis of hydrogen peroxide has received much attention due to its on-site production, absence of organic impurities during the synthesis, environmentally-friendly and low energy input with no need for further purification. This review focused on the metal-free heteroatom-doped carbon catalyst for the generation of hydrogen peroxide by the two-electron oxygen reduction reaction (2e- ORR). Depending on the type of heteroatoms, the electronic properties of the carbon can be changed, and they significantly affect the ORR catalytic activity. Even with the same heteroatoms, their specific chemical composition in a carbon frame has a large effect on the electrocatalytic activity. The location of the active catalytic sites within the carbon network is also investigated with a theoretical study, which is important for effective electrocatalysis of the 2e- ORR to occur. The physical and chemical properties of base carbon materials and the reaction environment for ORR such as the pH and additives of the electrolyte are discussed. This review provides fundamental insights into how the moiety of heteroatoms enhances the electrocatalytic activity of metal-free carbon materials for the 2e- ORR. |
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title_short |
Recent progress in heteroatom-doped carbon electrocatalysts for the two-electron oxygen reduction reaction |
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