Regulation of magnetism on Fe- and Ni-doped SnO
We investigated the ferromagnetism of Fe- and Ni-doped SnO2 (110) surfaces and the regulation of the ferromagnetism on doped surfaces by the oxygen vacancy and adsorbed O2 molecule. The introduction of Fe/Ni dopant can make the nonmagnetic SnO2 (110) surface have a magnetic moment of 3.45 µB/1.97 µB...
Ausführliche Beschreibung
Autor*in: |
Shi, Xiaojing [verfasserIn] Zhang, Yongjia [verfasserIn] Hao, Weidong [verfasserIn] Yang, Zhi [verfasserIn] |
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Format: |
E-Artikel |
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Sprache: |
Englisch |
Erschienen: |
2023 |
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Schlagwörter: |
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Übergeordnetes Werk: |
Enthalten in: Journal of magnetism and magnetic materials - Amsterdam : North-Holland Publ. Co., 1975, 567 |
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Übergeordnetes Werk: |
volume:567 |
DOI / URN: |
10.1016/j.jmmm.2023.170356 |
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Katalog-ID: |
ELV009097740 |
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520 | |a We investigated the ferromagnetism of Fe- and Ni-doped SnO2 (110) surfaces and the regulation of the ferromagnetism on doped surfaces by the oxygen vacancy and adsorbed O2 molecule. The introduction of Fe/Ni dopant can make the nonmagnetic SnO2 (110) surface have a magnetic moment of 3.45 µB/1.97 µB and exhibit stable ferromagnetic coupling. After forming oxygen vacancy under oxygen-deficient conditions, a fraction of the remaining electrons provided by vacancy is acquired by the doped atom, which reduces the number of unpaired electrons in the doped atom d shell, thereby reducing the surface magnetic moment by about 0.6 µB. The oxygen vacancy reduces the magnetization of the bound magnetopolaron, which leads to the weakening of the surface ferromagnetic coupling. The free O2 molecule can exothermically adsorb on the defect surface and fill the oxygen vacancy, forming a magnetic cluster with the doped atom. Although the magnetic moment of the spontaneously adsorbed O2 molecule decreases due to obtaining a small number of electrons from the surface, the magnetic moment of the O2-adsorbed surface increases about 1.0 µB. The magnetic coupling of the O2-adsorbed surface is determined by the competition mechanism of antimagnetic coupling between O2 molecules and ferromagnetic coupling between magnetopolarons. | ||
650 | 4 | |a Hybrid Function | |
650 | 4 | |a Ferromagnetism | |
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700 | 1 | |a Zhang, Yongjia |e verfasserin |4 aut | |
700 | 1 | |a Hao, Weidong |e verfasserin |4 aut | |
700 | 1 | |a Yang, Zhi |e verfasserin |4 aut | |
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10.1016/j.jmmm.2023.170356 doi (DE-627)ELV009097740 (ELSEVIER)S0304-8853(23)00005-7 DE-627 ger DE-627 rda eng 530 DE-600 33.16 bkl Shi, Xiaojing verfasserin aut Regulation of magnetism on Fe- and Ni-doped SnO 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier We investigated the ferromagnetism of Fe- and Ni-doped SnO2 (110) surfaces and the regulation of the ferromagnetism on doped surfaces by the oxygen vacancy and adsorbed O2 molecule. The introduction of Fe/Ni dopant can make the nonmagnetic SnO2 (110) surface have a magnetic moment of 3.45 µB/1.97 µB and exhibit stable ferromagnetic coupling. After forming oxygen vacancy under oxygen-deficient conditions, a fraction of the remaining electrons provided by vacancy is acquired by the doped atom, which reduces the number of unpaired electrons in the doped atom d shell, thereby reducing the surface magnetic moment by about 0.6 µB. The oxygen vacancy reduces the magnetization of the bound magnetopolaron, which leads to the weakening of the surface ferromagnetic coupling. The free O2 molecule can exothermically adsorb on the defect surface and fill the oxygen vacancy, forming a magnetic cluster with the doped atom. Although the magnetic moment of the spontaneously adsorbed O2 molecule decreases due to obtaining a small number of electrons from the surface, the magnetic moment of the O2-adsorbed surface increases about 1.0 µB. The magnetic coupling of the O2-adsorbed surface is determined by the competition mechanism of antimagnetic coupling between O2 molecules and ferromagnetic coupling between magnetopolarons. Hybrid Function Ferromagnetism Surface Vacancy Oxygen Adsorption Zhang, Yongjia verfasserin aut Hao, Weidong verfasserin aut Yang, Zhi verfasserin aut Enthalten in Journal of magnetism and magnetic materials Amsterdam : North-Holland Publ. Co., 1975 567 Online-Ressource (DE-627)271175958 (DE-600)1479000-2 (DE-576)078412331 0304-8853 nnns volume:567 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.16 Elektrizität Magnetismus AR 567 |
spelling |
10.1016/j.jmmm.2023.170356 doi (DE-627)ELV009097740 (ELSEVIER)S0304-8853(23)00005-7 DE-627 ger DE-627 rda eng 530 DE-600 33.16 bkl Shi, Xiaojing verfasserin aut Regulation of magnetism on Fe- and Ni-doped SnO 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier We investigated the ferromagnetism of Fe- and Ni-doped SnO2 (110) surfaces and the regulation of the ferromagnetism on doped surfaces by the oxygen vacancy and adsorbed O2 molecule. The introduction of Fe/Ni dopant can make the nonmagnetic SnO2 (110) surface have a magnetic moment of 3.45 µB/1.97 µB and exhibit stable ferromagnetic coupling. After forming oxygen vacancy under oxygen-deficient conditions, a fraction of the remaining electrons provided by vacancy is acquired by the doped atom, which reduces the number of unpaired electrons in the doped atom d shell, thereby reducing the surface magnetic moment by about 0.6 µB. The oxygen vacancy reduces the magnetization of the bound magnetopolaron, which leads to the weakening of the surface ferromagnetic coupling. The free O2 molecule can exothermically adsorb on the defect surface and fill the oxygen vacancy, forming a magnetic cluster with the doped atom. Although the magnetic moment of the spontaneously adsorbed O2 molecule decreases due to obtaining a small number of electrons from the surface, the magnetic moment of the O2-adsorbed surface increases about 1.0 µB. The magnetic coupling of the O2-adsorbed surface is determined by the competition mechanism of antimagnetic coupling between O2 molecules and ferromagnetic coupling between magnetopolarons. Hybrid Function Ferromagnetism Surface Vacancy Oxygen Adsorption Zhang, Yongjia verfasserin aut Hao, Weidong verfasserin aut Yang, Zhi verfasserin aut Enthalten in Journal of magnetism and magnetic materials Amsterdam : North-Holland Publ. Co., 1975 567 Online-Ressource (DE-627)271175958 (DE-600)1479000-2 (DE-576)078412331 0304-8853 nnns volume:567 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.16 Elektrizität Magnetismus AR 567 |
allfields_unstemmed |
10.1016/j.jmmm.2023.170356 doi (DE-627)ELV009097740 (ELSEVIER)S0304-8853(23)00005-7 DE-627 ger DE-627 rda eng 530 DE-600 33.16 bkl Shi, Xiaojing verfasserin aut Regulation of magnetism on Fe- and Ni-doped SnO 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier We investigated the ferromagnetism of Fe- and Ni-doped SnO2 (110) surfaces and the regulation of the ferromagnetism on doped surfaces by the oxygen vacancy and adsorbed O2 molecule. The introduction of Fe/Ni dopant can make the nonmagnetic SnO2 (110) surface have a magnetic moment of 3.45 µB/1.97 µB and exhibit stable ferromagnetic coupling. After forming oxygen vacancy under oxygen-deficient conditions, a fraction of the remaining electrons provided by vacancy is acquired by the doped atom, which reduces the number of unpaired electrons in the doped atom d shell, thereby reducing the surface magnetic moment by about 0.6 µB. The oxygen vacancy reduces the magnetization of the bound magnetopolaron, which leads to the weakening of the surface ferromagnetic coupling. The free O2 molecule can exothermically adsorb on the defect surface and fill the oxygen vacancy, forming a magnetic cluster with the doped atom. Although the magnetic moment of the spontaneously adsorbed O2 molecule decreases due to obtaining a small number of electrons from the surface, the magnetic moment of the O2-adsorbed surface increases about 1.0 µB. The magnetic coupling of the O2-adsorbed surface is determined by the competition mechanism of antimagnetic coupling between O2 molecules and ferromagnetic coupling between magnetopolarons. Hybrid Function Ferromagnetism Surface Vacancy Oxygen Adsorption Zhang, Yongjia verfasserin aut Hao, Weidong verfasserin aut Yang, Zhi verfasserin aut Enthalten in Journal of magnetism and magnetic materials Amsterdam : North-Holland Publ. Co., 1975 567 Online-Ressource (DE-627)271175958 (DE-600)1479000-2 (DE-576)078412331 0304-8853 nnns volume:567 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.16 Elektrizität Magnetismus AR 567 |
allfieldsGer |
10.1016/j.jmmm.2023.170356 doi (DE-627)ELV009097740 (ELSEVIER)S0304-8853(23)00005-7 DE-627 ger DE-627 rda eng 530 DE-600 33.16 bkl Shi, Xiaojing verfasserin aut Regulation of magnetism on Fe- and Ni-doped SnO 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier We investigated the ferromagnetism of Fe- and Ni-doped SnO2 (110) surfaces and the regulation of the ferromagnetism on doped surfaces by the oxygen vacancy and adsorbed O2 molecule. The introduction of Fe/Ni dopant can make the nonmagnetic SnO2 (110) surface have a magnetic moment of 3.45 µB/1.97 µB and exhibit stable ferromagnetic coupling. After forming oxygen vacancy under oxygen-deficient conditions, a fraction of the remaining electrons provided by vacancy is acquired by the doped atom, which reduces the number of unpaired electrons in the doped atom d shell, thereby reducing the surface magnetic moment by about 0.6 µB. The oxygen vacancy reduces the magnetization of the bound magnetopolaron, which leads to the weakening of the surface ferromagnetic coupling. The free O2 molecule can exothermically adsorb on the defect surface and fill the oxygen vacancy, forming a magnetic cluster with the doped atom. Although the magnetic moment of the spontaneously adsorbed O2 molecule decreases due to obtaining a small number of electrons from the surface, the magnetic moment of the O2-adsorbed surface increases about 1.0 µB. The magnetic coupling of the O2-adsorbed surface is determined by the competition mechanism of antimagnetic coupling between O2 molecules and ferromagnetic coupling between magnetopolarons. Hybrid Function Ferromagnetism Surface Vacancy Oxygen Adsorption Zhang, Yongjia verfasserin aut Hao, Weidong verfasserin aut Yang, Zhi verfasserin aut Enthalten in Journal of magnetism and magnetic materials Amsterdam : North-Holland Publ. Co., 1975 567 Online-Ressource (DE-627)271175958 (DE-600)1479000-2 (DE-576)078412331 0304-8853 nnns volume:567 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.16 Elektrizität Magnetismus AR 567 |
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10.1016/j.jmmm.2023.170356 doi (DE-627)ELV009097740 (ELSEVIER)S0304-8853(23)00005-7 DE-627 ger DE-627 rda eng 530 DE-600 33.16 bkl Shi, Xiaojing verfasserin aut Regulation of magnetism on Fe- and Ni-doped SnO 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier We investigated the ferromagnetism of Fe- and Ni-doped SnO2 (110) surfaces and the regulation of the ferromagnetism on doped surfaces by the oxygen vacancy and adsorbed O2 molecule. The introduction of Fe/Ni dopant can make the nonmagnetic SnO2 (110) surface have a magnetic moment of 3.45 µB/1.97 µB and exhibit stable ferromagnetic coupling. After forming oxygen vacancy under oxygen-deficient conditions, a fraction of the remaining electrons provided by vacancy is acquired by the doped atom, which reduces the number of unpaired electrons in the doped atom d shell, thereby reducing the surface magnetic moment by about 0.6 µB. The oxygen vacancy reduces the magnetization of the bound magnetopolaron, which leads to the weakening of the surface ferromagnetic coupling. The free O2 molecule can exothermically adsorb on the defect surface and fill the oxygen vacancy, forming a magnetic cluster with the doped atom. Although the magnetic moment of the spontaneously adsorbed O2 molecule decreases due to obtaining a small number of electrons from the surface, the magnetic moment of the O2-adsorbed surface increases about 1.0 µB. The magnetic coupling of the O2-adsorbed surface is determined by the competition mechanism of antimagnetic coupling between O2 molecules and ferromagnetic coupling between magnetopolarons. Hybrid Function Ferromagnetism Surface Vacancy Oxygen Adsorption Zhang, Yongjia verfasserin aut Hao, Weidong verfasserin aut Yang, Zhi verfasserin aut Enthalten in Journal of magnetism and magnetic materials Amsterdam : North-Holland Publ. Co., 1975 567 Online-Ressource (DE-627)271175958 (DE-600)1479000-2 (DE-576)078412331 0304-8853 nnns volume:567 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.16 Elektrizität Magnetismus AR 567 |
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Regulation of magnetism on Fe- and Ni-doped SnO |
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Regulation of magnetism on Fe- and Ni-doped SnO |
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Shi, Xiaojing |
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Journal of magnetism and magnetic materials |
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Shi, Xiaojing Zhang, Yongjia Hao, Weidong Yang, Zhi |
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Shi, Xiaojing |
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regulation of magnetism on fe- and ni-doped sno |
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Regulation of magnetism on Fe- and Ni-doped SnO |
abstract |
We investigated the ferromagnetism of Fe- and Ni-doped SnO2 (110) surfaces and the regulation of the ferromagnetism on doped surfaces by the oxygen vacancy and adsorbed O2 molecule. The introduction of Fe/Ni dopant can make the nonmagnetic SnO2 (110) surface have a magnetic moment of 3.45 µB/1.97 µB and exhibit stable ferromagnetic coupling. After forming oxygen vacancy under oxygen-deficient conditions, a fraction of the remaining electrons provided by vacancy is acquired by the doped atom, which reduces the number of unpaired electrons in the doped atom d shell, thereby reducing the surface magnetic moment by about 0.6 µB. The oxygen vacancy reduces the magnetization of the bound magnetopolaron, which leads to the weakening of the surface ferromagnetic coupling. The free O2 molecule can exothermically adsorb on the defect surface and fill the oxygen vacancy, forming a magnetic cluster with the doped atom. Although the magnetic moment of the spontaneously adsorbed O2 molecule decreases due to obtaining a small number of electrons from the surface, the magnetic moment of the O2-adsorbed surface increases about 1.0 µB. The magnetic coupling of the O2-adsorbed surface is determined by the competition mechanism of antimagnetic coupling between O2 molecules and ferromagnetic coupling between magnetopolarons. |
abstractGer |
We investigated the ferromagnetism of Fe- and Ni-doped SnO2 (110) surfaces and the regulation of the ferromagnetism on doped surfaces by the oxygen vacancy and adsorbed O2 molecule. The introduction of Fe/Ni dopant can make the nonmagnetic SnO2 (110) surface have a magnetic moment of 3.45 µB/1.97 µB and exhibit stable ferromagnetic coupling. After forming oxygen vacancy under oxygen-deficient conditions, a fraction of the remaining electrons provided by vacancy is acquired by the doped atom, which reduces the number of unpaired electrons in the doped atom d shell, thereby reducing the surface magnetic moment by about 0.6 µB. The oxygen vacancy reduces the magnetization of the bound magnetopolaron, which leads to the weakening of the surface ferromagnetic coupling. The free O2 molecule can exothermically adsorb on the defect surface and fill the oxygen vacancy, forming a magnetic cluster with the doped atom. Although the magnetic moment of the spontaneously adsorbed O2 molecule decreases due to obtaining a small number of electrons from the surface, the magnetic moment of the O2-adsorbed surface increases about 1.0 µB. The magnetic coupling of the O2-adsorbed surface is determined by the competition mechanism of antimagnetic coupling between O2 molecules and ferromagnetic coupling between magnetopolarons. |
abstract_unstemmed |
We investigated the ferromagnetism of Fe- and Ni-doped SnO2 (110) surfaces and the regulation of the ferromagnetism on doped surfaces by the oxygen vacancy and adsorbed O2 molecule. The introduction of Fe/Ni dopant can make the nonmagnetic SnO2 (110) surface have a magnetic moment of 3.45 µB/1.97 µB and exhibit stable ferromagnetic coupling. After forming oxygen vacancy under oxygen-deficient conditions, a fraction of the remaining electrons provided by vacancy is acquired by the doped atom, which reduces the number of unpaired electrons in the doped atom d shell, thereby reducing the surface magnetic moment by about 0.6 µB. The oxygen vacancy reduces the magnetization of the bound magnetopolaron, which leads to the weakening of the surface ferromagnetic coupling. The free O2 molecule can exothermically adsorb on the defect surface and fill the oxygen vacancy, forming a magnetic cluster with the doped atom. Although the magnetic moment of the spontaneously adsorbed O2 molecule decreases due to obtaining a small number of electrons from the surface, the magnetic moment of the O2-adsorbed surface increases about 1.0 µB. The magnetic coupling of the O2-adsorbed surface is determined by the competition mechanism of antimagnetic coupling between O2 molecules and ferromagnetic coupling between magnetopolarons. |
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title_short |
Regulation of magnetism on Fe- and Ni-doped SnO |
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Zhang, Yongjia Hao, Weidong Yang, Zhi |
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