Effects of composition variation and hydrogenation on magnetocaloric properties of the (Gd
To identify promising magnetic refrigerant materials, we have studied the influence of composition variations and hydrogenation on the magnetocaloric effect (MCE) of the (Gd1-xTbx)Ni compounds. The end compositions of the series, Gd0.9Tb0.1Ni and Gd0.1Tb0.9Ni crystallize in orthorhombic CrB-type and...
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| Autor*in: |
Tereshina, I.S. [verfasserIn] Karpenkov, A.Yu. [verfasserIn] Kurganskaya, A.A. [verfasserIn] Chzhan, V.B. [verfasserIn] Lushnikov, S.A. [verfasserIn] Verbetsky, V.N. [verfasserIn] Kozlyakova, E.S. [verfasserIn] Vasiliev, A.N. [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2023 |
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| Schlagwörter: |
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| Übergeordnetes Werk: |
Enthalten in: Journal of magnetism and magnetic materials - Amsterdam : North-Holland Publ. Co., 1975, 574 |
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| Übergeordnetes Werk: |
volume:574 |
| DOI / URN: |
10.1016/j.jmmm.2023.170693 |
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ELV009564012 |
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| 520 | |a To identify promising magnetic refrigerant materials, we have studied the influence of composition variations and hydrogenation on the magnetocaloric effect (MCE) of the (Gd1-xTbx)Ni compounds. The end compositions of the series, Gd0.9Tb0.1Ni and Gd0.1Tb0.9Ni crystallize in orthorhombic CrB-type and monoclinic TbNi-type structures, respectively. Hydrogenation boosts the unit cell volume of (Gd,Tb)Ni by more than 20 % upon absorption of 4 at.H/f.u. Hydrogen absorption changes the structure type from TbNi to the CrB-type in Gd0.1Tb0.9Ni. Decrease of the Curie temperature in hydrides reaches ∼ 60 K. The magnetocaloric effect in (Gd,Tb)NiHy (y = 0 and 4) obtained by indirect method in the vicinity of TC revealed similar values of the maximum of specific isothermal entropy change -ΔST = 20.5 J kg−1 K−1 for Gd0.9Tb0.1Ni and its hydride Gd0.9Tb0.1NiH4 at μ0ΔH = 7 T. We show that the controlled synthesis of hydrides allows us to tailor the magnetocaloric effect in the multicomponent rare earth intermetallics and obtain materials with largely different TCs but with the same MCE values that are attractive for use in low-temperature magnetic cooling applications. | ||
| 650 | 4 | |a Rare earth compounds | |
| 650 | 4 | |a Substitutions | |
| 650 | 4 | |a Hydrogenation | |
| 650 | 4 | |a Magnetization | |
| 650 | 4 | |a Curie temperature | |
| 650 | 4 | |a Magnetocaloric effect | |
| 700 | 1 | |a Karpenkov, A.Yu. |e verfasserin |4 aut | |
| 700 | 1 | |a Kurganskaya, A.A. |e verfasserin |4 aut | |
| 700 | 1 | |a Chzhan, V.B. |e verfasserin |4 aut | |
| 700 | 1 | |a Lushnikov, S.A. |e verfasserin |4 aut | |
| 700 | 1 | |a Verbetsky, V.N. |e verfasserin |4 aut | |
| 700 | 1 | |a Kozlyakova, E.S. |e verfasserin |4 aut | |
| 700 | 1 | |a Vasiliev, A.N. |e verfasserin |4 aut | |
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10.1016/j.jmmm.2023.170693 doi (DE-627)ELV009564012 (ELSEVIER)S0304-8853(23)00342-6 DE-627 ger DE-627 rda eng 530 DE-600 33.16 bkl Tereshina, I.S. verfasserin aut Effects of composition variation and hydrogenation on magnetocaloric properties of the (Gd 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier To identify promising magnetic refrigerant materials, we have studied the influence of composition variations and hydrogenation on the magnetocaloric effect (MCE) of the (Gd1-xTbx)Ni compounds. The end compositions of the series, Gd0.9Tb0.1Ni and Gd0.1Tb0.9Ni crystallize in orthorhombic CrB-type and monoclinic TbNi-type structures, respectively. Hydrogenation boosts the unit cell volume of (Gd,Tb)Ni by more than 20 % upon absorption of 4 at.H/f.u. Hydrogen absorption changes the structure type from TbNi to the CrB-type in Gd0.1Tb0.9Ni. Decrease of the Curie temperature in hydrides reaches ∼ 60 K. The magnetocaloric effect in (Gd,Tb)NiHy (y = 0 and 4) obtained by indirect method in the vicinity of TC revealed similar values of the maximum of specific isothermal entropy change -ΔST = 20.5 J kg−1 K−1 for Gd0.9Tb0.1Ni and its hydride Gd0.9Tb0.1NiH4 at μ0ΔH = 7 T. We show that the controlled synthesis of hydrides allows us to tailor the magnetocaloric effect in the multicomponent rare earth intermetallics and obtain materials with largely different TCs but with the same MCE values that are attractive for use in low-temperature magnetic cooling applications. Rare earth compounds Substitutions Hydrogenation Magnetization Curie temperature Magnetocaloric effect Karpenkov, A.Yu. verfasserin aut Kurganskaya, A.A. verfasserin aut Chzhan, V.B. verfasserin aut Lushnikov, S.A. verfasserin aut Verbetsky, V.N. verfasserin aut Kozlyakova, E.S. verfasserin aut Vasiliev, A.N. verfasserin aut Enthalten in Journal of magnetism and magnetic materials Amsterdam : North-Holland Publ. Co., 1975 574 Online-Ressource (DE-627)271175958 (DE-600)1479000-2 (DE-576)078412331 0304-8853 nnns volume:574 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.16 Elektrizität Magnetismus AR 574 |
| spelling |
10.1016/j.jmmm.2023.170693 doi (DE-627)ELV009564012 (ELSEVIER)S0304-8853(23)00342-6 DE-627 ger DE-627 rda eng 530 DE-600 33.16 bkl Tereshina, I.S. verfasserin aut Effects of composition variation and hydrogenation on magnetocaloric properties of the (Gd 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier To identify promising magnetic refrigerant materials, we have studied the influence of composition variations and hydrogenation on the magnetocaloric effect (MCE) of the (Gd1-xTbx)Ni compounds. The end compositions of the series, Gd0.9Tb0.1Ni and Gd0.1Tb0.9Ni crystallize in orthorhombic CrB-type and monoclinic TbNi-type structures, respectively. Hydrogenation boosts the unit cell volume of (Gd,Tb)Ni by more than 20 % upon absorption of 4 at.H/f.u. Hydrogen absorption changes the structure type from TbNi to the CrB-type in Gd0.1Tb0.9Ni. Decrease of the Curie temperature in hydrides reaches ∼ 60 K. The magnetocaloric effect in (Gd,Tb)NiHy (y = 0 and 4) obtained by indirect method in the vicinity of TC revealed similar values of the maximum of specific isothermal entropy change -ΔST = 20.5 J kg−1 K−1 for Gd0.9Tb0.1Ni and its hydride Gd0.9Tb0.1NiH4 at μ0ΔH = 7 T. We show that the controlled synthesis of hydrides allows us to tailor the magnetocaloric effect in the multicomponent rare earth intermetallics and obtain materials with largely different TCs but with the same MCE values that are attractive for use in low-temperature magnetic cooling applications. Rare earth compounds Substitutions Hydrogenation Magnetization Curie temperature Magnetocaloric effect Karpenkov, A.Yu. verfasserin aut Kurganskaya, A.A. verfasserin aut Chzhan, V.B. verfasserin aut Lushnikov, S.A. verfasserin aut Verbetsky, V.N. verfasserin aut Kozlyakova, E.S. verfasserin aut Vasiliev, A.N. verfasserin aut Enthalten in Journal of magnetism and magnetic materials Amsterdam : North-Holland Publ. Co., 1975 574 Online-Ressource (DE-627)271175958 (DE-600)1479000-2 (DE-576)078412331 0304-8853 nnns volume:574 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.16 Elektrizität Magnetismus AR 574 |
| allfields_unstemmed |
10.1016/j.jmmm.2023.170693 doi (DE-627)ELV009564012 (ELSEVIER)S0304-8853(23)00342-6 DE-627 ger DE-627 rda eng 530 DE-600 33.16 bkl Tereshina, I.S. verfasserin aut Effects of composition variation and hydrogenation on magnetocaloric properties of the (Gd 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier To identify promising magnetic refrigerant materials, we have studied the influence of composition variations and hydrogenation on the magnetocaloric effect (MCE) of the (Gd1-xTbx)Ni compounds. The end compositions of the series, Gd0.9Tb0.1Ni and Gd0.1Tb0.9Ni crystallize in orthorhombic CrB-type and monoclinic TbNi-type structures, respectively. Hydrogenation boosts the unit cell volume of (Gd,Tb)Ni by more than 20 % upon absorption of 4 at.H/f.u. Hydrogen absorption changes the structure type from TbNi to the CrB-type in Gd0.1Tb0.9Ni. Decrease of the Curie temperature in hydrides reaches ∼ 60 K. The magnetocaloric effect in (Gd,Tb)NiHy (y = 0 and 4) obtained by indirect method in the vicinity of TC revealed similar values of the maximum of specific isothermal entropy change -ΔST = 20.5 J kg−1 K−1 for Gd0.9Tb0.1Ni and its hydride Gd0.9Tb0.1NiH4 at μ0ΔH = 7 T. We show that the controlled synthesis of hydrides allows us to tailor the magnetocaloric effect in the multicomponent rare earth intermetallics and obtain materials with largely different TCs but with the same MCE values that are attractive for use in low-temperature magnetic cooling applications. Rare earth compounds Substitutions Hydrogenation Magnetization Curie temperature Magnetocaloric effect Karpenkov, A.Yu. verfasserin aut Kurganskaya, A.A. verfasserin aut Chzhan, V.B. verfasserin aut Lushnikov, S.A. verfasserin aut Verbetsky, V.N. verfasserin aut Kozlyakova, E.S. verfasserin aut Vasiliev, A.N. verfasserin aut Enthalten in Journal of magnetism and magnetic materials Amsterdam : North-Holland Publ. Co., 1975 574 Online-Ressource (DE-627)271175958 (DE-600)1479000-2 (DE-576)078412331 0304-8853 nnns volume:574 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.16 Elektrizität Magnetismus AR 574 |
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10.1016/j.jmmm.2023.170693 doi (DE-627)ELV009564012 (ELSEVIER)S0304-8853(23)00342-6 DE-627 ger DE-627 rda eng 530 DE-600 33.16 bkl Tereshina, I.S. verfasserin aut Effects of composition variation and hydrogenation on magnetocaloric properties of the (Gd 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier To identify promising magnetic refrigerant materials, we have studied the influence of composition variations and hydrogenation on the magnetocaloric effect (MCE) of the (Gd1-xTbx)Ni compounds. The end compositions of the series, Gd0.9Tb0.1Ni and Gd0.1Tb0.9Ni crystallize in orthorhombic CrB-type and monoclinic TbNi-type structures, respectively. Hydrogenation boosts the unit cell volume of (Gd,Tb)Ni by more than 20 % upon absorption of 4 at.H/f.u. Hydrogen absorption changes the structure type from TbNi to the CrB-type in Gd0.1Tb0.9Ni. Decrease of the Curie temperature in hydrides reaches ∼ 60 K. The magnetocaloric effect in (Gd,Tb)NiHy (y = 0 and 4) obtained by indirect method in the vicinity of TC revealed similar values of the maximum of specific isothermal entropy change -ΔST = 20.5 J kg−1 K−1 for Gd0.9Tb0.1Ni and its hydride Gd0.9Tb0.1NiH4 at μ0ΔH = 7 T. We show that the controlled synthesis of hydrides allows us to tailor the magnetocaloric effect in the multicomponent rare earth intermetallics and obtain materials with largely different TCs but with the same MCE values that are attractive for use in low-temperature magnetic cooling applications. Rare earth compounds Substitutions Hydrogenation Magnetization Curie temperature Magnetocaloric effect Karpenkov, A.Yu. verfasserin aut Kurganskaya, A.A. verfasserin aut Chzhan, V.B. verfasserin aut Lushnikov, S.A. verfasserin aut Verbetsky, V.N. verfasserin aut Kozlyakova, E.S. verfasserin aut Vasiliev, A.N. verfasserin aut Enthalten in Journal of magnetism and magnetic materials Amsterdam : North-Holland Publ. Co., 1975 574 Online-Ressource (DE-627)271175958 (DE-600)1479000-2 (DE-576)078412331 0304-8853 nnns volume:574 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.16 Elektrizität Magnetismus AR 574 |
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10.1016/j.jmmm.2023.170693 doi (DE-627)ELV009564012 (ELSEVIER)S0304-8853(23)00342-6 DE-627 ger DE-627 rda eng 530 DE-600 33.16 bkl Tereshina, I.S. verfasserin aut Effects of composition variation and hydrogenation on magnetocaloric properties of the (Gd 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier To identify promising magnetic refrigerant materials, we have studied the influence of composition variations and hydrogenation on the magnetocaloric effect (MCE) of the (Gd1-xTbx)Ni compounds. The end compositions of the series, Gd0.9Tb0.1Ni and Gd0.1Tb0.9Ni crystallize in orthorhombic CrB-type and monoclinic TbNi-type structures, respectively. Hydrogenation boosts the unit cell volume of (Gd,Tb)Ni by more than 20 % upon absorption of 4 at.H/f.u. Hydrogen absorption changes the structure type from TbNi to the CrB-type in Gd0.1Tb0.9Ni. Decrease of the Curie temperature in hydrides reaches ∼ 60 K. The magnetocaloric effect in (Gd,Tb)NiHy (y = 0 and 4) obtained by indirect method in the vicinity of TC revealed similar values of the maximum of specific isothermal entropy change -ΔST = 20.5 J kg−1 K−1 for Gd0.9Tb0.1Ni and its hydride Gd0.9Tb0.1NiH4 at μ0ΔH = 7 T. We show that the controlled synthesis of hydrides allows us to tailor the magnetocaloric effect in the multicomponent rare earth intermetallics and obtain materials with largely different TCs but with the same MCE values that are attractive for use in low-temperature magnetic cooling applications. Rare earth compounds Substitutions Hydrogenation Magnetization Curie temperature Magnetocaloric effect Karpenkov, A.Yu. verfasserin aut Kurganskaya, A.A. verfasserin aut Chzhan, V.B. verfasserin aut Lushnikov, S.A. verfasserin aut Verbetsky, V.N. verfasserin aut Kozlyakova, E.S. verfasserin aut Vasiliev, A.N. verfasserin aut Enthalten in Journal of magnetism and magnetic materials Amsterdam : North-Holland Publ. Co., 1975 574 Online-Ressource (DE-627)271175958 (DE-600)1479000-2 (DE-576)078412331 0304-8853 nnns volume:574 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.16 Elektrizität Magnetismus AR 574 |
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Rare earth compounds Substitutions Hydrogenation Magnetization Curie temperature Magnetocaloric effect |
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Tereshina, I.S. @@aut@@ Karpenkov, A.Yu. @@aut@@ Kurganskaya, A.A. @@aut@@ Chzhan, V.B. @@aut@@ Lushnikov, S.A. @@aut@@ Verbetsky, V.N. @@aut@@ Kozlyakova, E.S. @@aut@@ Vasiliev, A.N. @@aut@@ |
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2023-01-01T00:00:00Z |
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Tereshina, I.S. ddc 530 bkl 33.16 misc Rare earth compounds misc Substitutions misc Hydrogenation misc Magnetization misc Curie temperature misc Magnetocaloric effect Effects of composition variation and hydrogenation on magnetocaloric properties of the (Gd |
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530 DE-600 33.16 bkl Effects of composition variation and hydrogenation on magnetocaloric properties of the (Gd Rare earth compounds Substitutions Hydrogenation Magnetization Curie temperature Magnetocaloric effect |
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Effects of composition variation and hydrogenation on magnetocaloric properties of the (Gd |
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Effects of composition variation and hydrogenation on magnetocaloric properties of the (Gd |
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Tereshina, I.S. Karpenkov, A.Yu. Kurganskaya, A.A. Chzhan, V.B. Lushnikov, S.A. Verbetsky, V.N. Kozlyakova, E.S. Vasiliev, A.N. |
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effects of composition variation and hydrogenation on magnetocaloric properties of the (gd |
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Effects of composition variation and hydrogenation on magnetocaloric properties of the (Gd |
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To identify promising magnetic refrigerant materials, we have studied the influence of composition variations and hydrogenation on the magnetocaloric effect (MCE) of the (Gd1-xTbx)Ni compounds. The end compositions of the series, Gd0.9Tb0.1Ni and Gd0.1Tb0.9Ni crystallize in orthorhombic CrB-type and monoclinic TbNi-type structures, respectively. Hydrogenation boosts the unit cell volume of (Gd,Tb)Ni by more than 20 % upon absorption of 4 at.H/f.u. Hydrogen absorption changes the structure type from TbNi to the CrB-type in Gd0.1Tb0.9Ni. Decrease of the Curie temperature in hydrides reaches ∼ 60 K. The magnetocaloric effect in (Gd,Tb)NiHy (y = 0 and 4) obtained by indirect method in the vicinity of TC revealed similar values of the maximum of specific isothermal entropy change -ΔST = 20.5 J kg−1 K−1 for Gd0.9Tb0.1Ni and its hydride Gd0.9Tb0.1NiH4 at μ0ΔH = 7 T. We show that the controlled synthesis of hydrides allows us to tailor the magnetocaloric effect in the multicomponent rare earth intermetallics and obtain materials with largely different TCs but with the same MCE values that are attractive for use in low-temperature magnetic cooling applications. |
| abstractGer |
To identify promising magnetic refrigerant materials, we have studied the influence of composition variations and hydrogenation on the magnetocaloric effect (MCE) of the (Gd1-xTbx)Ni compounds. The end compositions of the series, Gd0.9Tb0.1Ni and Gd0.1Tb0.9Ni crystallize in orthorhombic CrB-type and monoclinic TbNi-type structures, respectively. Hydrogenation boosts the unit cell volume of (Gd,Tb)Ni by more than 20 % upon absorption of 4 at.H/f.u. Hydrogen absorption changes the structure type from TbNi to the CrB-type in Gd0.1Tb0.9Ni. Decrease of the Curie temperature in hydrides reaches ∼ 60 K. The magnetocaloric effect in (Gd,Tb)NiHy (y = 0 and 4) obtained by indirect method in the vicinity of TC revealed similar values of the maximum of specific isothermal entropy change -ΔST = 20.5 J kg−1 K−1 for Gd0.9Tb0.1Ni and its hydride Gd0.9Tb0.1NiH4 at μ0ΔH = 7 T. We show that the controlled synthesis of hydrides allows us to tailor the magnetocaloric effect in the multicomponent rare earth intermetallics and obtain materials with largely different TCs but with the same MCE values that are attractive for use in low-temperature magnetic cooling applications. |
| abstract_unstemmed |
To identify promising magnetic refrigerant materials, we have studied the influence of composition variations and hydrogenation on the magnetocaloric effect (MCE) of the (Gd1-xTbx)Ni compounds. The end compositions of the series, Gd0.9Tb0.1Ni and Gd0.1Tb0.9Ni crystallize in orthorhombic CrB-type and monoclinic TbNi-type structures, respectively. Hydrogenation boosts the unit cell volume of (Gd,Tb)Ni by more than 20 % upon absorption of 4 at.H/f.u. Hydrogen absorption changes the structure type from TbNi to the CrB-type in Gd0.1Tb0.9Ni. Decrease of the Curie temperature in hydrides reaches ∼ 60 K. The magnetocaloric effect in (Gd,Tb)NiHy (y = 0 and 4) obtained by indirect method in the vicinity of TC revealed similar values of the maximum of specific isothermal entropy change -ΔST = 20.5 J kg−1 K−1 for Gd0.9Tb0.1Ni and its hydride Gd0.9Tb0.1NiH4 at μ0ΔH = 7 T. We show that the controlled synthesis of hydrides allows us to tailor the magnetocaloric effect in the multicomponent rare earth intermetallics and obtain materials with largely different TCs but with the same MCE values that are attractive for use in low-temperature magnetic cooling applications. |
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Effects of composition variation and hydrogenation on magnetocaloric properties of the (Gd |
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| score |
7.397773 |