Heterostructure design of 3D hydrangea-like Fe

In an era dominated by electronic equipment, the development of high-efficiency electromagnetic wave (EMW) absorbers is of great significance in solving the problem of electromagnetic (EM) pollution. Heterointerface engineering for optimizing EMW absorption performance depends on the design of vacan...
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Autor*in:	Wang, Yan [verfasserIn] Cheng, Runrun [verfasserIn] Cui, Wen-Gang [verfasserIn] Lu, Zhao [verfasserIn] Yang, Yaxiong [verfasserIn] Pan, Hongge [verfasserIn] Che, Renchao [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2023

Schlagwörter:	Electromagnetic absorption Hydrangea-like composite Sulfur doping Iron oxide Radar cross section (RCS)

Übergeordnetes Werk:	Enthalten in: Carbon - Amsterdam [u.a.] : Elsevier Science, 1963, 210
Übergeordnetes Werk:	volume:210

DOI / URN:	10.1016/j.carbon.2023.118043

Katalog-ID:	ELV009729712

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520			\|a In an era dominated by electronic equipment, the development of high-efficiency electromagnetic wave (EMW) absorbers is of great significance in solving the problem of electromagnetic (EM) pollution. Heterointerface engineering for optimizing EMW absorption performance depends on the design of vacancy, defect, and heterogeneous interface, which remains a considerable challenge in adjusting the micro and macro-interface effects. In this work, S atoms are incorporated into a dielectric-magnetic complementary system (Fe3O4/Fe7S8C) to arouse the polarization effect of vacancies, defects, and non-uniform interfaces, thus tremendously boosting the EM energy attenuation capacity. Besides, the carbon shell provides more propagation paths for the dissipation of EMWs, and dielectric-magnetic synergy improves impedance matching. Eventually, in comparison with Fe2O3 and Fe3O4@C composites, interface-engineered Fe3O4/Fe7S8@C acquires a much better EM wave absorption performance. Its minimum reflection loss value reaches as much as −56.2 dB with a thickness of only 1.6 mm, and the corresponding effective absorption bandwidth (EAB) is up to 4.5 GHz. This unique hydrangea-like layered structure provides space to facilitate non-uniform coupling between the layers and has strong anisotropy to enhance the magnetic response. The high density of magnetic flux in the nanosheets builds a three-dimensional magnetic coupling network, which is supported by off-axis electron holography. Besides, the radar cross section from HFSS simulation further confirms that S-doping can favor the best synergy between dielectric and magnetic losses, facilitating the composite to achieve a more optimal impedance matching and improve the absorption capacity. In conclusion, this work presents new ideas for the design of excellent absorbing materials.
650		4	\|a Electromagnetic absorption
650		4	\|a Hydrangea-like composite
650		4	\|a Sulfur doping
650		4	\|a Iron oxide
650		4	\|a Radar cross section (RCS)
700	1		\|a Cheng, Runrun \|e verfasserin \|4 aut
700	1		\|a Cui, Wen-Gang \|e verfasserin \|4 aut
700	1		\|a Lu, Zhao \|e verfasserin \|4 aut
700	1		\|a Yang, Yaxiong \|e verfasserin \|4 aut
700	1		\|a Pan, Hongge \|e verfasserin \|4 aut
700	1		\|a Che, Renchao \|e verfasserin \|4 aut
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allfields	10.1016/j.carbon.2023.118043 doi (DE-627)ELV009729712 (ELSEVIER)S0008-6223(23)00284-1 DE-627 ger DE-627 rda eng 540 VZ 51.79 bkl 35.48 bkl Wang, Yan verfasserin (orcid)0000-0001-5231-275X aut Heterostructure design of 3D hydrangea-like Fe 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier In an era dominated by electronic equipment, the development of high-efficiency electromagnetic wave (EMW) absorbers is of great significance in solving the problem of electromagnetic (EM) pollution. Heterointerface engineering for optimizing EMW absorption performance depends on the design of vacancy, defect, and heterogeneous interface, which remains a considerable challenge in adjusting the micro and macro-interface effects. In this work, S atoms are incorporated into a dielectric-magnetic complementary system (Fe3O4/Fe7S8C) to arouse the polarization effect of vacancies, defects, and non-uniform interfaces, thus tremendously boosting the EM energy attenuation capacity. Besides, the carbon shell provides more propagation paths for the dissipation of EMWs, and dielectric-magnetic synergy improves impedance matching. Eventually, in comparison with Fe2O3 and Fe3O4@C composites, interface-engineered Fe3O4/Fe7S8@C acquires a much better EM wave absorption performance. Its minimum reflection loss value reaches as much as −56.2 dB with a thickness of only 1.6 mm, and the corresponding effective absorption bandwidth (EAB) is up to 4.5 GHz. This unique hydrangea-like layered structure provides space to facilitate non-uniform coupling between the layers and has strong anisotropy to enhance the magnetic response. The high density of magnetic flux in the nanosheets builds a three-dimensional magnetic coupling network, which is supported by off-axis electron holography. Besides, the radar cross section from HFSS simulation further confirms that S-doping can favor the best synergy between dielectric and magnetic losses, facilitating the composite to achieve a more optimal impedance matching and improve the absorption capacity. In conclusion, this work presents new ideas for the design of excellent absorbing materials. Electromagnetic absorption Hydrangea-like composite Sulfur doping Iron oxide Radar cross section (RCS) Cheng, Runrun verfasserin aut Cui, Wen-Gang verfasserin aut Lu, Zhao verfasserin aut Yang, Yaxiong verfasserin aut Pan, Hongge verfasserin aut Che, Renchao verfasserin aut Enthalten in Carbon Amsterdam [u.a.] : Elsevier Science, 1963 210 Online-Ressource (DE-627)320522164 (DE-600)2014715-6 (DE-576)103484280 0008-6223 nnns volume:210 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 51.79 Sonstige Werkstoffe VZ 35.48 Sonstige anorganische Elemente und ihre Verbindungen VZ AR 210
spelling	10.1016/j.carbon.2023.118043 doi (DE-627)ELV009729712 (ELSEVIER)S0008-6223(23)00284-1 DE-627 ger DE-627 rda eng 540 VZ 51.79 bkl 35.48 bkl Wang, Yan verfasserin (orcid)0000-0001-5231-275X aut Heterostructure design of 3D hydrangea-like Fe 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier In an era dominated by electronic equipment, the development of high-efficiency electromagnetic wave (EMW) absorbers is of great significance in solving the problem of electromagnetic (EM) pollution. Heterointerface engineering for optimizing EMW absorption performance depends on the design of vacancy, defect, and heterogeneous interface, which remains a considerable challenge in adjusting the micro and macro-interface effects. In this work, S atoms are incorporated into a dielectric-magnetic complementary system (Fe3O4/Fe7S8C) to arouse the polarization effect of vacancies, defects, and non-uniform interfaces, thus tremendously boosting the EM energy attenuation capacity. Besides, the carbon shell provides more propagation paths for the dissipation of EMWs, and dielectric-magnetic synergy improves impedance matching. Eventually, in comparison with Fe2O3 and Fe3O4@C composites, interface-engineered Fe3O4/Fe7S8@C acquires a much better EM wave absorption performance. Its minimum reflection loss value reaches as much as −56.2 dB with a thickness of only 1.6 mm, and the corresponding effective absorption bandwidth (EAB) is up to 4.5 GHz. This unique hydrangea-like layered structure provides space to facilitate non-uniform coupling between the layers and has strong anisotropy to enhance the magnetic response. The high density of magnetic flux in the nanosheets builds a three-dimensional magnetic coupling network, which is supported by off-axis electron holography. Besides, the radar cross section from HFSS simulation further confirms that S-doping can favor the best synergy between dielectric and magnetic losses, facilitating the composite to achieve a more optimal impedance matching and improve the absorption capacity. In conclusion, this work presents new ideas for the design of excellent absorbing materials. Electromagnetic absorption Hydrangea-like composite Sulfur doping Iron oxide Radar cross section (RCS) Cheng, Runrun verfasserin aut Cui, Wen-Gang verfasserin aut Lu, Zhao verfasserin aut Yang, Yaxiong verfasserin aut Pan, Hongge verfasserin aut Che, Renchao verfasserin aut Enthalten in Carbon Amsterdam [u.a.] : Elsevier Science, 1963 210 Online-Ressource (DE-627)320522164 (DE-600)2014715-6 (DE-576)103484280 0008-6223 nnns volume:210 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 51.79 Sonstige Werkstoffe VZ 35.48 Sonstige anorganische Elemente und ihre Verbindungen VZ AR 210
allfields_unstemmed	10.1016/j.carbon.2023.118043 doi (DE-627)ELV009729712 (ELSEVIER)S0008-6223(23)00284-1 DE-627 ger DE-627 rda eng 540 VZ 51.79 bkl 35.48 bkl Wang, Yan verfasserin (orcid)0000-0001-5231-275X aut Heterostructure design of 3D hydrangea-like Fe 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier In an era dominated by electronic equipment, the development of high-efficiency electromagnetic wave (EMW) absorbers is of great significance in solving the problem of electromagnetic (EM) pollution. Heterointerface engineering for optimizing EMW absorption performance depends on the design of vacancy, defect, and heterogeneous interface, which remains a considerable challenge in adjusting the micro and macro-interface effects. In this work, S atoms are incorporated into a dielectric-magnetic complementary system (Fe3O4/Fe7S8C) to arouse the polarization effect of vacancies, defects, and non-uniform interfaces, thus tremendously boosting the EM energy attenuation capacity. Besides, the carbon shell provides more propagation paths for the dissipation of EMWs, and dielectric-magnetic synergy improves impedance matching. Eventually, in comparison with Fe2O3 and Fe3O4@C composites, interface-engineered Fe3O4/Fe7S8@C acquires a much better EM wave absorption performance. Its minimum reflection loss value reaches as much as −56.2 dB with a thickness of only 1.6 mm, and the corresponding effective absorption bandwidth (EAB) is up to 4.5 GHz. This unique hydrangea-like layered structure provides space to facilitate non-uniform coupling between the layers and has strong anisotropy to enhance the magnetic response. The high density of magnetic flux in the nanosheets builds a three-dimensional magnetic coupling network, which is supported by off-axis electron holography. Besides, the radar cross section from HFSS simulation further confirms that S-doping can favor the best synergy between dielectric and magnetic losses, facilitating the composite to achieve a more optimal impedance matching and improve the absorption capacity. In conclusion, this work presents new ideas for the design of excellent absorbing materials. Electromagnetic absorption Hydrangea-like composite Sulfur doping Iron oxide Radar cross section (RCS) Cheng, Runrun verfasserin aut Cui, Wen-Gang verfasserin aut Lu, Zhao verfasserin aut Yang, Yaxiong verfasserin aut Pan, Hongge verfasserin aut Che, Renchao verfasserin aut Enthalten in Carbon Amsterdam [u.a.] : Elsevier Science, 1963 210 Online-Ressource (DE-627)320522164 (DE-600)2014715-6 (DE-576)103484280 0008-6223 nnns volume:210 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 51.79 Sonstige Werkstoffe VZ 35.48 Sonstige anorganische Elemente und ihre Verbindungen VZ AR 210
allfieldsGer	10.1016/j.carbon.2023.118043 doi (DE-627)ELV009729712 (ELSEVIER)S0008-6223(23)00284-1 DE-627 ger DE-627 rda eng 540 VZ 51.79 bkl 35.48 bkl Wang, Yan verfasserin (orcid)0000-0001-5231-275X aut Heterostructure design of 3D hydrangea-like Fe 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier In an era dominated by electronic equipment, the development of high-efficiency electromagnetic wave (EMW) absorbers is of great significance in solving the problem of electromagnetic (EM) pollution. Heterointerface engineering for optimizing EMW absorption performance depends on the design of vacancy, defect, and heterogeneous interface, which remains a considerable challenge in adjusting the micro and macro-interface effects. In this work, S atoms are incorporated into a dielectric-magnetic complementary system (Fe3O4/Fe7S8C) to arouse the polarization effect of vacancies, defects, and non-uniform interfaces, thus tremendously boosting the EM energy attenuation capacity. Besides, the carbon shell provides more propagation paths for the dissipation of EMWs, and dielectric-magnetic synergy improves impedance matching. Eventually, in comparison with Fe2O3 and Fe3O4@C composites, interface-engineered Fe3O4/Fe7S8@C acquires a much better EM wave absorption performance. Its minimum reflection loss value reaches as much as −56.2 dB with a thickness of only 1.6 mm, and the corresponding effective absorption bandwidth (EAB) is up to 4.5 GHz. This unique hydrangea-like layered structure provides space to facilitate non-uniform coupling between the layers and has strong anisotropy to enhance the magnetic response. The high density of magnetic flux in the nanosheets builds a three-dimensional magnetic coupling network, which is supported by off-axis electron holography. Besides, the radar cross section from HFSS simulation further confirms that S-doping can favor the best synergy between dielectric and magnetic losses, facilitating the composite to achieve a more optimal impedance matching and improve the absorption capacity. In conclusion, this work presents new ideas for the design of excellent absorbing materials. Electromagnetic absorption Hydrangea-like composite Sulfur doping Iron oxide Radar cross section (RCS) Cheng, Runrun verfasserin aut Cui, Wen-Gang verfasserin aut Lu, Zhao verfasserin aut Yang, Yaxiong verfasserin aut Pan, Hongge verfasserin aut Che, Renchao verfasserin aut Enthalten in Carbon Amsterdam [u.a.] : Elsevier Science, 1963 210 Online-Ressource (DE-627)320522164 (DE-600)2014715-6 (DE-576)103484280 0008-6223 nnns volume:210 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 51.79 Sonstige Werkstoffe VZ 35.48 Sonstige anorganische Elemente und ihre Verbindungen VZ AR 210
allfieldsSound	10.1016/j.carbon.2023.118043 doi (DE-627)ELV009729712 (ELSEVIER)S0008-6223(23)00284-1 DE-627 ger DE-627 rda eng 540 VZ 51.79 bkl 35.48 bkl Wang, Yan verfasserin (orcid)0000-0001-5231-275X aut Heterostructure design of 3D hydrangea-like Fe 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier In an era dominated by electronic equipment, the development of high-efficiency electromagnetic wave (EMW) absorbers is of great significance in solving the problem of electromagnetic (EM) pollution. Heterointerface engineering for optimizing EMW absorption performance depends on the design of vacancy, defect, and heterogeneous interface, which remains a considerable challenge in adjusting the micro and macro-interface effects. In this work, S atoms are incorporated into a dielectric-magnetic complementary system (Fe3O4/Fe7S8C) to arouse the polarization effect of vacancies, defects, and non-uniform interfaces, thus tremendously boosting the EM energy attenuation capacity. Besides, the carbon shell provides more propagation paths for the dissipation of EMWs, and dielectric-magnetic synergy improves impedance matching. Eventually, in comparison with Fe2O3 and Fe3O4@C composites, interface-engineered Fe3O4/Fe7S8@C acquires a much better EM wave absorption performance. Its minimum reflection loss value reaches as much as −56.2 dB with a thickness of only 1.6 mm, and the corresponding effective absorption bandwidth (EAB) is up to 4.5 GHz. This unique hydrangea-like layered structure provides space to facilitate non-uniform coupling between the layers and has strong anisotropy to enhance the magnetic response. The high density of magnetic flux in the nanosheets builds a three-dimensional magnetic coupling network, which is supported by off-axis electron holography. Besides, the radar cross section from HFSS simulation further confirms that S-doping can favor the best synergy between dielectric and magnetic losses, facilitating the composite to achieve a more optimal impedance matching and improve the absorption capacity. In conclusion, this work presents new ideas for the design of excellent absorbing materials. Electromagnetic absorption Hydrangea-like composite Sulfur doping Iron oxide Radar cross section (RCS) Cheng, Runrun verfasserin aut Cui, Wen-Gang verfasserin aut Lu, Zhao verfasserin aut Yang, Yaxiong verfasserin aut Pan, Hongge verfasserin aut Che, Renchao verfasserin aut Enthalten in Carbon Amsterdam [u.a.] : Elsevier Science, 1963 210 Online-Ressource (DE-627)320522164 (DE-600)2014715-6 (DE-576)103484280 0008-6223 nnns volume:210 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 51.79 Sonstige Werkstoffe VZ 35.48 Sonstige anorganische Elemente und ihre Verbindungen VZ AR 210
language	English
source	Enthalten in Carbon 210 volume:210
sourceStr	Enthalten in Carbon 210 volume:210
format_phy_str_mv	Article
bklname	Sonstige Werkstoffe Sonstige anorganische Elemente und ihre Verbindungen
institution	findex.gbv.de
topic_facet	Electromagnetic absorption Hydrangea-like composite Sulfur doping Iron oxide Radar cross section (RCS)
dewey-raw	540
isfreeaccess_bool	false
container_title	Carbon
authorswithroles_txt_mv	Wang, Yan @@aut@@ Cheng, Runrun @@aut@@ Cui, Wen-Gang @@aut@@ Lu, Zhao @@aut@@ Yang, Yaxiong @@aut@@ Pan, Hongge @@aut@@ Che, Renchao @@aut@@
publishDateDaySort_date	2023-01-01T00:00:00Z
hierarchy_top_id	320522164
dewey-sort	3540
id	ELV009729712
language_de	englisch
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author	Wang, Yan
spellingShingle	Wang, Yan ddc 540 bkl 51.79 bkl 35.48 misc Electromagnetic absorption misc Hydrangea-like composite misc Sulfur doping misc Iron oxide misc Radar cross section (RCS) Heterostructure design of 3D hydrangea-like Fe
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topic_title	540 VZ 51.79 bkl 35.48 bkl Heterostructure design of 3D hydrangea-like Fe Electromagnetic absorption Hydrangea-like composite Sulfur doping Iron oxide Radar cross section (RCS)
topic	ddc 540 bkl 51.79 bkl 35.48 misc Electromagnetic absorption misc Hydrangea-like composite misc Sulfur doping misc Iron oxide misc Radar cross section (RCS)
topic_unstemmed	ddc 540 bkl 51.79 bkl 35.48 misc Electromagnetic absorption misc Hydrangea-like composite misc Sulfur doping misc Iron oxide misc Radar cross section (RCS)
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title	Heterostructure design of 3D hydrangea-like Fe
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title_full	Heterostructure design of 3D hydrangea-like Fe
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title_sort	heterostructure design of 3d hydrangea-like fe
title_auth	Heterostructure design of 3D hydrangea-like Fe
abstract	In an era dominated by electronic equipment, the development of high-efficiency electromagnetic wave (EMW) absorbers is of great significance in solving the problem of electromagnetic (EM) pollution. Heterointerface engineering for optimizing EMW absorption performance depends on the design of vacancy, defect, and heterogeneous interface, which remains a considerable challenge in adjusting the micro and macro-interface effects. In this work, S atoms are incorporated into a dielectric-magnetic complementary system (Fe3O4/Fe7S8C) to arouse the polarization effect of vacancies, defects, and non-uniform interfaces, thus tremendously boosting the EM energy attenuation capacity. Besides, the carbon shell provides more propagation paths for the dissipation of EMWs, and dielectric-magnetic synergy improves impedance matching. Eventually, in comparison with Fe2O3 and Fe3O4@C composites, interface-engineered Fe3O4/Fe7S8@C acquires a much better EM wave absorption performance. Its minimum reflection loss value reaches as much as −56.2 dB with a thickness of only 1.6 mm, and the corresponding effective absorption bandwidth (EAB) is up to 4.5 GHz. This unique hydrangea-like layered structure provides space to facilitate non-uniform coupling between the layers and has strong anisotropy to enhance the magnetic response. The high density of magnetic flux in the nanosheets builds a three-dimensional magnetic coupling network, which is supported by off-axis electron holography. Besides, the radar cross section from HFSS simulation further confirms that S-doping can favor the best synergy between dielectric and magnetic losses, facilitating the composite to achieve a more optimal impedance matching and improve the absorption capacity. In conclusion, this work presents new ideas for the design of excellent absorbing materials.
abstractGer	In an era dominated by electronic equipment, the development of high-efficiency electromagnetic wave (EMW) absorbers is of great significance in solving the problem of electromagnetic (EM) pollution. Heterointerface engineering for optimizing EMW absorption performance depends on the design of vacancy, defect, and heterogeneous interface, which remains a considerable challenge in adjusting the micro and macro-interface effects. In this work, S atoms are incorporated into a dielectric-magnetic complementary system (Fe3O4/Fe7S8C) to arouse the polarization effect of vacancies, defects, and non-uniform interfaces, thus tremendously boosting the EM energy attenuation capacity. Besides, the carbon shell provides more propagation paths for the dissipation of EMWs, and dielectric-magnetic synergy improves impedance matching. Eventually, in comparison with Fe2O3 and Fe3O4@C composites, interface-engineered Fe3O4/Fe7S8@C acquires a much better EM wave absorption performance. Its minimum reflection loss value reaches as much as −56.2 dB with a thickness of only 1.6 mm, and the corresponding effective absorption bandwidth (EAB) is up to 4.5 GHz. This unique hydrangea-like layered structure provides space to facilitate non-uniform coupling between the layers and has strong anisotropy to enhance the magnetic response. The high density of magnetic flux in the nanosheets builds a three-dimensional magnetic coupling network, which is supported by off-axis electron holography. Besides, the radar cross section from HFSS simulation further confirms that S-doping can favor the best synergy between dielectric and magnetic losses, facilitating the composite to achieve a more optimal impedance matching and improve the absorption capacity. In conclusion, this work presents new ideas for the design of excellent absorbing materials.
abstract_unstemmed	In an era dominated by electronic equipment, the development of high-efficiency electromagnetic wave (EMW) absorbers is of great significance in solving the problem of electromagnetic (EM) pollution. Heterointerface engineering for optimizing EMW absorption performance depends on the design of vacancy, defect, and heterogeneous interface, which remains a considerable challenge in adjusting the micro and macro-interface effects. In this work, S atoms are incorporated into a dielectric-magnetic complementary system (Fe3O4/Fe7S8C) to arouse the polarization effect of vacancies, defects, and non-uniform interfaces, thus tremendously boosting the EM energy attenuation capacity. Besides, the carbon shell provides more propagation paths for the dissipation of EMWs, and dielectric-magnetic synergy improves impedance matching. Eventually, in comparison with Fe2O3 and Fe3O4@C composites, interface-engineered Fe3O4/Fe7S8@C acquires a much better EM wave absorption performance. Its minimum reflection loss value reaches as much as −56.2 dB with a thickness of only 1.6 mm, and the corresponding effective absorption bandwidth (EAB) is up to 4.5 GHz. This unique hydrangea-like layered structure provides space to facilitate non-uniform coupling between the layers and has strong anisotropy to enhance the magnetic response. The high density of magnetic flux in the nanosheets builds a three-dimensional magnetic coupling network, which is supported by off-axis electron holography. Besides, the radar cross section from HFSS simulation further confirms that S-doping can favor the best synergy between dielectric and magnetic losses, facilitating the composite to achieve a more optimal impedance matching and improve the absorption capacity. In conclusion, this work presents new ideas for the design of excellent absorbing materials.
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title_short	Heterostructure design of 3D hydrangea-like Fe
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author2	Cheng, Runrun Cui, Wen-Gang Lu, Zhao Yang, Yaxiong Pan, Hongge Che, Renchao
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Heterointerface engineering for optimizing EMW absorption performance depends on the design of vacancy, defect, and heterogeneous interface, which remains a considerable challenge in adjusting the micro and macro-interface effects. In this work, S atoms are incorporated into a dielectric-magnetic complementary system (Fe3O4/Fe7S8C) to arouse the polarization effect of vacancies, defects, and non-uniform interfaces, thus tremendously boosting the EM energy attenuation capacity. Besides, the carbon shell provides more propagation paths for the dissipation of EMWs, and dielectric-magnetic synergy improves impedance matching. Eventually, in comparison with Fe2O3 and Fe3O4@C composites, interface-engineered Fe3O4/Fe7S8@C acquires a much better EM wave absorption performance. Its minimum reflection loss value reaches as much as −56.2 dB with a thickness of only 1.6 mm, and the corresponding effective absorption bandwidth (EAB) is up to 4.5 GHz. This unique hydrangea-like layered structure provides space to facilitate non-uniform coupling between the layers and has strong anisotropy to enhance the magnetic response. The high density of magnetic flux in the nanosheets builds a three-dimensional magnetic coupling network, which is supported by off-axis electron holography. Besides, the radar cross section from HFSS simulation further confirms that S-doping can favor the best synergy between dielectric and magnetic losses, facilitating the composite to achieve a more optimal impedance matching and improve the absorption capacity. 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Heterostructure design of 3D hydrangea-like Fe

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