Metal-organic framework–derived NiCo

Ti3C2Tx MXene has become an excellent two-dimensional conductive substrate for electrode materials of supercapacitors (SCs) with prominent physicochemical properties. Whereas, due to the lower theoretical specific capacitance and its interlayer agglomerate, the practical application and electrochemical property of Ti3C2Tx have imposed serious restrictions. Herein, metal-organic framework (MOF) derived NiCo2S4 Co3S4 nanocages with superior yolk-shell structure are introduced to anchor on the surface of Ti3C2Tx via ion exchange reaction and electrostatic attraction, forming the distinctive hierarchical structure of NiCo2S4 @Co3S4/Ti3C2Tx composed of NiCo2S4 @Co3S4 yolk-shell nanocages (NiCo2S4 @Co3S4 YSNs) adsorbed on 2D Ti3C2Tx nanosheets. The NiCo2S4 @Co3S4 YSNs with a large void space, serving as a confined reactor, not only offer a buffer against the volume variation, but also supply abundant active sites and restrain the agglomeration of Ti3C2Tx nanosheets. Furthermore, the novel structure of NiCo2S4 @Co3S4/Ti3C2Tx composite as electrode material could accelerate the thermodynamic stability, suppress the textural instability, and moderate the unavoidable volume change of active substance. Benefited from the above merits, the NiCo2S4 @Co3S4/Ti3C2Tx electrode demonstrates a significant specific capacitance (1872 F g−1 at 2 mV s−1), remarkable rate capability in the high current density (such as, 1121.6 F g−1 at 20 A g−1, 1533 F g−1 at 0.5 A g−1) and displays an excellent life span with 92.2 % of the capacity retention after 12,000 cycles at 10 A g−1. More particularly, the asymmetric supercapacitors (ASCs) fabricated with NiCo2S4 @Co3S4/Ti3C2Tx represent a fascinating energy density of 241.9 Wh kg−1 at a power density of 1125 W kg−1, which can light up 10 LEDs simultaneously. The results further prove that this rational design method could provide a meaningful prospect for MXenes and MOF derivatives composites for high-performance ASCs. Ausführliche Beschreibung

Gespeichert in:

Autor*in:	Wu, Wenling [verfasserIn] Liu, Tiantian [verfasserIn] Diwu, Jiahao [verfasserIn] Li, Chenguang [verfasserIn] Zhu, Jianfeng [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2023

Schlagwörter:	MXenes Yolk-shell nanocages MOF Asymmetric supercapacitors

Übergeordnetes Werk:	Enthalten in: Journal of alloys and compounds - Lausanne : Elsevier, 1991, 954
Übergeordnetes Werk:	volume:954

DOI / URN:	10.1016/j.jallcom.2023.170213

Katalog-ID:	ELV00976075X

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520			\|a Ti3C2Tx MXene has become an excellent two-dimensional conductive substrate for electrode materials of supercapacitors (SCs) with prominent physicochemical properties. Whereas, due to the lower theoretical specific capacitance and its interlayer agglomerate, the practical application and electrochemical property of Ti3C2Tx have imposed serious restrictions. Herein, metal-organic framework (MOF) derived NiCo2S4 Co3S4 nanocages with superior yolk-shell structure are introduced to anchor on the surface of Ti3C2Tx via ion exchange reaction and electrostatic attraction, forming the distinctive hierarchical structure of NiCo2S4 @Co3S4/Ti3C2Tx composed of NiCo2S4 @Co3S4 yolk-shell nanocages (NiCo2S4 @Co3S4 YSNs) adsorbed on 2D Ti3C2Tx nanosheets. The NiCo2S4 @Co3S4 YSNs with a large void space, serving as a confined reactor, not only offer a buffer against the volume variation, but also supply abundant active sites and restrain the agglomeration of Ti3C2Tx nanosheets. Furthermore, the novel structure of NiCo2S4 @Co3S4/Ti3C2Tx composite as electrode material could accelerate the thermodynamic stability, suppress the textural instability, and moderate the unavoidable volume change of active substance. Benefited from the above merits, the NiCo2S4 @Co3S4/Ti3C2Tx electrode demonstrates a significant specific capacitance (1872 F g−1 at 2 mV s−1), remarkable rate capability in the high current density (such as, 1121.6 F g−1 at 20 A g−1, 1533 F g−1 at 0.5 A g−1) and displays an excellent life span with 92.2 % of the capacity retention after 12,000 cycles at 10 A g−1. More particularly, the asymmetric supercapacitors (ASCs) fabricated with NiCo2S4 @Co3S4/Ti3C2Tx represent a fascinating energy density of 241.9 Wh kg−1 at a power density of 1125 W kg−1, which can light up 10 LEDs simultaneously. The results further prove that this rational design method could provide a meaningful prospect for MXenes and MOF derivatives composites for high-performance ASCs.
650		4	\|a MXenes
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700	1		\|a Liu, Tiantian \|e verfasserin \|4 aut
700	1		\|a Diwu, Jiahao \|e verfasserin \|4 aut
700	1		\|a Li, Chenguang \|e verfasserin \|4 aut
700	1		\|a Zhu, Jianfeng \|e verfasserin \|4 aut
773	0	8	\|i Enthalten in \|t Journal of alloys and compounds \|d Lausanne : Elsevier, 1991 \|g 954 \|h Online-Ressource \|w (DE-627)320504646 \|w (DE-600)2012675-X \|w (DE-576)098615009 \|7 nnns
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author_variant	w w ww t l tl j d jd c l cl j z jz
matchkey_str	wuwenlingliutiantiandiwujiahaolichenguan:2023----:eaogncrmwrdr
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allfields	10.1016/j.jallcom.2023.170213 doi (DE-627)ELV00976075X (ELSEVIER)S0925-8388(23)01516-5 DE-627 ger DE-627 rda eng 670 540 VZ 51.54 bkl 33.61 bkl 35.90 bkl Wu, Wenling verfasserin (orcid)0000-0002-7974-5544 aut Metal-organic framework–derived NiCo 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Ti3C2Tx MXene has become an excellent two-dimensional conductive substrate for electrode materials of supercapacitors (SCs) with prominent physicochemical properties. Whereas, due to the lower theoretical specific capacitance and its interlayer agglomerate, the practical application and electrochemical property of Ti3C2Tx have imposed serious restrictions. Herein, metal-organic framework (MOF) derived NiCo2S4 Co3S4 nanocages with superior yolk-shell structure are introduced to anchor on the surface of Ti3C2Tx via ion exchange reaction and electrostatic attraction, forming the distinctive hierarchical structure of NiCo2S4 @Co3S4/Ti3C2Tx composed of NiCo2S4 @Co3S4 yolk-shell nanocages (NiCo2S4 @Co3S4 YSNs) adsorbed on 2D Ti3C2Tx nanosheets. The NiCo2S4 @Co3S4 YSNs with a large void space, serving as a confined reactor, not only offer a buffer against the volume variation, but also supply abundant active sites and restrain the agglomeration of Ti3C2Tx nanosheets. Furthermore, the novel structure of NiCo2S4 @Co3S4/Ti3C2Tx composite as electrode material could accelerate the thermodynamic stability, suppress the textural instability, and moderate the unavoidable volume change of active substance. Benefited from the above merits, the NiCo2S4 @Co3S4/Ti3C2Tx electrode demonstrates a significant specific capacitance (1872 F g−1 at 2 mV s−1), remarkable rate capability in the high current density (such as, 1121.6 F g−1 at 20 A g−1, 1533 F g−1 at 0.5 A g−1) and displays an excellent life span with 92.2 % of the capacity retention after 12,000 cycles at 10 A g−1. More particularly, the asymmetric supercapacitors (ASCs) fabricated with NiCo2S4 @Co3S4/Ti3C2Tx represent a fascinating energy density of 241.9 Wh kg−1 at a power density of 1125 W kg−1, which can light up 10 LEDs simultaneously. The results further prove that this rational design method could provide a meaningful prospect for MXenes and MOF derivatives composites for high-performance ASCs. MXenes Yolk-shell nanocages MOF Asymmetric supercapacitors Liu, Tiantian verfasserin aut Diwu, Jiahao verfasserin aut Li, Chenguang verfasserin aut Zhu, Jianfeng verfasserin aut Enthalten in Journal of alloys and compounds Lausanne : Elsevier, 1991 954 Online-Ressource (DE-627)320504646 (DE-600)2012675-X (DE-576)098615009 nnns volume:954 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 51.54 Nichteisenmetalle und ihre Legierungen VZ 33.61 Festkörperphysik VZ 35.90 Festkörperchemie VZ AR 954
spelling	10.1016/j.jallcom.2023.170213 doi (DE-627)ELV00976075X (ELSEVIER)S0925-8388(23)01516-5 DE-627 ger DE-627 rda eng 670 540 VZ 51.54 bkl 33.61 bkl 35.90 bkl Wu, Wenling verfasserin (orcid)0000-0002-7974-5544 aut Metal-organic framework–derived NiCo 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Ti3C2Tx MXene has become an excellent two-dimensional conductive substrate for electrode materials of supercapacitors (SCs) with prominent physicochemical properties. Whereas, due to the lower theoretical specific capacitance and its interlayer agglomerate, the practical application and electrochemical property of Ti3C2Tx have imposed serious restrictions. Herein, metal-organic framework (MOF) derived NiCo2S4 Co3S4 nanocages with superior yolk-shell structure are introduced to anchor on the surface of Ti3C2Tx via ion exchange reaction and electrostatic attraction, forming the distinctive hierarchical structure of NiCo2S4 @Co3S4/Ti3C2Tx composed of NiCo2S4 @Co3S4 yolk-shell nanocages (NiCo2S4 @Co3S4 YSNs) adsorbed on 2D Ti3C2Tx nanosheets. The NiCo2S4 @Co3S4 YSNs with a large void space, serving as a confined reactor, not only offer a buffer against the volume variation, but also supply abundant active sites and restrain the agglomeration of Ti3C2Tx nanosheets. Furthermore, the novel structure of NiCo2S4 @Co3S4/Ti3C2Tx composite as electrode material could accelerate the thermodynamic stability, suppress the textural instability, and moderate the unavoidable volume change of active substance. Benefited from the above merits, the NiCo2S4 @Co3S4/Ti3C2Tx electrode demonstrates a significant specific capacitance (1872 F g−1 at 2 mV s−1), remarkable rate capability in the high current density (such as, 1121.6 F g−1 at 20 A g−1, 1533 F g−1 at 0.5 A g−1) and displays an excellent life span with 92.2 % of the capacity retention after 12,000 cycles at 10 A g−1. More particularly, the asymmetric supercapacitors (ASCs) fabricated with NiCo2S4 @Co3S4/Ti3C2Tx represent a fascinating energy density of 241.9 Wh kg−1 at a power density of 1125 W kg−1, which can light up 10 LEDs simultaneously. The results further prove that this rational design method could provide a meaningful prospect for MXenes and MOF derivatives composites for high-performance ASCs. MXenes Yolk-shell nanocages MOF Asymmetric supercapacitors Liu, Tiantian verfasserin aut Diwu, Jiahao verfasserin aut Li, Chenguang verfasserin aut Zhu, Jianfeng verfasserin aut Enthalten in Journal of alloys and compounds Lausanne : Elsevier, 1991 954 Online-Ressource (DE-627)320504646 (DE-600)2012675-X (DE-576)098615009 nnns volume:954 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 51.54 Nichteisenmetalle und ihre Legierungen VZ 33.61 Festkörperphysik VZ 35.90 Festkörperchemie VZ AR 954
allfields_unstemmed	10.1016/j.jallcom.2023.170213 doi (DE-627)ELV00976075X (ELSEVIER)S0925-8388(23)01516-5 DE-627 ger DE-627 rda eng 670 540 VZ 51.54 bkl 33.61 bkl 35.90 bkl Wu, Wenling verfasserin (orcid)0000-0002-7974-5544 aut Metal-organic framework–derived NiCo 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Ti3C2Tx MXene has become an excellent two-dimensional conductive substrate for electrode materials of supercapacitors (SCs) with prominent physicochemical properties. Whereas, due to the lower theoretical specific capacitance and its interlayer agglomerate, the practical application and electrochemical property of Ti3C2Tx have imposed serious restrictions. Herein, metal-organic framework (MOF) derived NiCo2S4 Co3S4 nanocages with superior yolk-shell structure are introduced to anchor on the surface of Ti3C2Tx via ion exchange reaction and electrostatic attraction, forming the distinctive hierarchical structure of NiCo2S4 @Co3S4/Ti3C2Tx composed of NiCo2S4 @Co3S4 yolk-shell nanocages (NiCo2S4 @Co3S4 YSNs) adsorbed on 2D Ti3C2Tx nanosheets. The NiCo2S4 @Co3S4 YSNs with a large void space, serving as a confined reactor, not only offer a buffer against the volume variation, but also supply abundant active sites and restrain the agglomeration of Ti3C2Tx nanosheets. Furthermore, the novel structure of NiCo2S4 @Co3S4/Ti3C2Tx composite as electrode material could accelerate the thermodynamic stability, suppress the textural instability, and moderate the unavoidable volume change of active substance. Benefited from the above merits, the NiCo2S4 @Co3S4/Ti3C2Tx electrode demonstrates a significant specific capacitance (1872 F g−1 at 2 mV s−1), remarkable rate capability in the high current density (such as, 1121.6 F g−1 at 20 A g−1, 1533 F g−1 at 0.5 A g−1) and displays an excellent life span with 92.2 % of the capacity retention after 12,000 cycles at 10 A g−1. More particularly, the asymmetric supercapacitors (ASCs) fabricated with NiCo2S4 @Co3S4/Ti3C2Tx represent a fascinating energy density of 241.9 Wh kg−1 at a power density of 1125 W kg−1, which can light up 10 LEDs simultaneously. The results further prove that this rational design method could provide a meaningful prospect for MXenes and MOF derivatives composites for high-performance ASCs. MXenes Yolk-shell nanocages MOF Asymmetric supercapacitors Liu, Tiantian verfasserin aut Diwu, Jiahao verfasserin aut Li, Chenguang verfasserin aut Zhu, Jianfeng verfasserin aut Enthalten in Journal of alloys and compounds Lausanne : Elsevier, 1991 954 Online-Ressource (DE-627)320504646 (DE-600)2012675-X (DE-576)098615009 nnns volume:954 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 51.54 Nichteisenmetalle und ihre Legierungen VZ 33.61 Festkörperphysik VZ 35.90 Festkörperchemie VZ AR 954
allfieldsGer	10.1016/j.jallcom.2023.170213 doi (DE-627)ELV00976075X (ELSEVIER)S0925-8388(23)01516-5 DE-627 ger DE-627 rda eng 670 540 VZ 51.54 bkl 33.61 bkl 35.90 bkl Wu, Wenling verfasserin (orcid)0000-0002-7974-5544 aut Metal-organic framework–derived NiCo 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Ti3C2Tx MXene has become an excellent two-dimensional conductive substrate for electrode materials of supercapacitors (SCs) with prominent physicochemical properties. Whereas, due to the lower theoretical specific capacitance and its interlayer agglomerate, the practical application and electrochemical property of Ti3C2Tx have imposed serious restrictions. Herein, metal-organic framework (MOF) derived NiCo2S4 Co3S4 nanocages with superior yolk-shell structure are introduced to anchor on the surface of Ti3C2Tx via ion exchange reaction and electrostatic attraction, forming the distinctive hierarchical structure of NiCo2S4 @Co3S4/Ti3C2Tx composed of NiCo2S4 @Co3S4 yolk-shell nanocages (NiCo2S4 @Co3S4 YSNs) adsorbed on 2D Ti3C2Tx nanosheets. The NiCo2S4 @Co3S4 YSNs with a large void space, serving as a confined reactor, not only offer a buffer against the volume variation, but also supply abundant active sites and restrain the agglomeration of Ti3C2Tx nanosheets. Furthermore, the novel structure of NiCo2S4 @Co3S4/Ti3C2Tx composite as electrode material could accelerate the thermodynamic stability, suppress the textural instability, and moderate the unavoidable volume change of active substance. Benefited from the above merits, the NiCo2S4 @Co3S4/Ti3C2Tx electrode demonstrates a significant specific capacitance (1872 F g−1 at 2 mV s−1), remarkable rate capability in the high current density (such as, 1121.6 F g−1 at 20 A g−1, 1533 F g−1 at 0.5 A g−1) and displays an excellent life span with 92.2 % of the capacity retention after 12,000 cycles at 10 A g−1. More particularly, the asymmetric supercapacitors (ASCs) fabricated with NiCo2S4 @Co3S4/Ti3C2Tx represent a fascinating energy density of 241.9 Wh kg−1 at a power density of 1125 W kg−1, which can light up 10 LEDs simultaneously. The results further prove that this rational design method could provide a meaningful prospect for MXenes and MOF derivatives composites for high-performance ASCs. MXenes Yolk-shell nanocages MOF Asymmetric supercapacitors Liu, Tiantian verfasserin aut Diwu, Jiahao verfasserin aut Li, Chenguang verfasserin aut Zhu, Jianfeng verfasserin aut Enthalten in Journal of alloys and compounds Lausanne : Elsevier, 1991 954 Online-Ressource (DE-627)320504646 (DE-600)2012675-X (DE-576)098615009 nnns volume:954 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 51.54 Nichteisenmetalle und ihre Legierungen VZ 33.61 Festkörperphysik VZ 35.90 Festkörperchemie VZ AR 954
allfieldsSound	10.1016/j.jallcom.2023.170213 doi (DE-627)ELV00976075X (ELSEVIER)S0925-8388(23)01516-5 DE-627 ger DE-627 rda eng 670 540 VZ 51.54 bkl 33.61 bkl 35.90 bkl Wu, Wenling verfasserin (orcid)0000-0002-7974-5544 aut Metal-organic framework–derived NiCo 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Ti3C2Tx MXene has become an excellent two-dimensional conductive substrate for electrode materials of supercapacitors (SCs) with prominent physicochemical properties. Whereas, due to the lower theoretical specific capacitance and its interlayer agglomerate, the practical application and electrochemical property of Ti3C2Tx have imposed serious restrictions. Herein, metal-organic framework (MOF) derived NiCo2S4 Co3S4 nanocages with superior yolk-shell structure are introduced to anchor on the surface of Ti3C2Tx via ion exchange reaction and electrostatic attraction, forming the distinctive hierarchical structure of NiCo2S4 @Co3S4/Ti3C2Tx composed of NiCo2S4 @Co3S4 yolk-shell nanocages (NiCo2S4 @Co3S4 YSNs) adsorbed on 2D Ti3C2Tx nanosheets. The NiCo2S4 @Co3S4 YSNs with a large void space, serving as a confined reactor, not only offer a buffer against the volume variation, but also supply abundant active sites and restrain the agglomeration of Ti3C2Tx nanosheets. Furthermore, the novel structure of NiCo2S4 @Co3S4/Ti3C2Tx composite as electrode material could accelerate the thermodynamic stability, suppress the textural instability, and moderate the unavoidable volume change of active substance. Benefited from the above merits, the NiCo2S4 @Co3S4/Ti3C2Tx electrode demonstrates a significant specific capacitance (1872 F g−1 at 2 mV s−1), remarkable rate capability in the high current density (such as, 1121.6 F g−1 at 20 A g−1, 1533 F g−1 at 0.5 A g−1) and displays an excellent life span with 92.2 % of the capacity retention after 12,000 cycles at 10 A g−1. More particularly, the asymmetric supercapacitors (ASCs) fabricated with NiCo2S4 @Co3S4/Ti3C2Tx represent a fascinating energy density of 241.9 Wh kg−1 at a power density of 1125 W kg−1, which can light up 10 LEDs simultaneously. The results further prove that this rational design method could provide a meaningful prospect for MXenes and MOF derivatives composites for high-performance ASCs. MXenes Yolk-shell nanocages MOF Asymmetric supercapacitors Liu, Tiantian verfasserin aut Diwu, Jiahao verfasserin aut Li, Chenguang verfasserin aut Zhu, Jianfeng verfasserin aut Enthalten in Journal of alloys and compounds Lausanne : Elsevier, 1991 954 Online-Ressource (DE-627)320504646 (DE-600)2012675-X (DE-576)098615009 nnns volume:954 GBV_USEFLAG_U SYSFLAG_U GBV_ELV SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 51.54 Nichteisenmetalle und ihre Legierungen VZ 33.61 Festkörperphysik VZ 35.90 Festkörperchemie VZ AR 954
language	English
source	Enthalten in Journal of alloys and compounds 954 volume:954
sourceStr	Enthalten in Journal of alloys and compounds 954 volume:954
format_phy_str_mv	Article
bklname	Nichteisenmetalle und ihre Legierungen Festkörperphysik Festkörperchemie
institution	findex.gbv.de
topic_facet	MXenes Yolk-shell nanocages MOF Asymmetric supercapacitors
dewey-raw	670
isfreeaccess_bool	false
container_title	Journal of alloys and compounds
authorswithroles_txt_mv	Wu, Wenling @@aut@@ Liu, Tiantian @@aut@@ Diwu, Jiahao @@aut@@ Li, Chenguang @@aut@@ Zhu, Jianfeng @@aut@@
publishDateDaySort_date	2023-01-01T00:00:00Z
hierarchy_top_id	320504646
dewey-sort	3670
id	ELV00976075X
language_de	englisch
fullrecord	<?xml version="1.0" encoding="UTF-8"?><collection xmlns="http://www.loc.gov/MARC21/slim"><record><leader>01000naa a22002652 4500</leader><controlfield tag="001">ELV00976075X</controlfield><controlfield tag="003">DE-627</controlfield><controlfield tag="005">20230530150233.0</controlfield><controlfield tag="007">cr uuu---uuuuu</controlfield><controlfield tag="008">230530s2023 xx \|\|\|\|\|o 00\| \|\|eng c</controlfield><datafield tag="024" ind1="7" ind2=" "><subfield code="a">10.1016/j.jallcom.2023.170213</subfield><subfield code="2">doi</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(DE-627)ELV00976075X</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(ELSEVIER)S0925-8388(23)01516-5</subfield></datafield><datafield tag="040" ind1=" " ind2=" "><subfield code="a">DE-627</subfield><subfield code="b">ger</subfield><subfield code="c">DE-627</subfield><subfield code="e">rda</subfield></datafield><datafield tag="041" ind1=" " ind2=" "><subfield code="a">eng</subfield></datafield><datafield tag="082" ind1="0" ind2="4"><subfield code="a">670</subfield><subfield code="a">540</subfield><subfield code="q">VZ</subfield></datafield><datafield tag="084" ind1=" " ind2=" "><subfield code="a">51.54</subfield><subfield code="2">bkl</subfield></datafield><datafield tag="084" ind1=" " ind2=" "><subfield code="a">33.61</subfield><subfield code="2">bkl</subfield></datafield><datafield tag="084" ind1=" " ind2=" "><subfield code="a">35.90</subfield><subfield code="2">bkl</subfield></datafield><datafield tag="100" ind1="1" ind2=" "><subfield code="a">Wu, Wenling</subfield><subfield code="e">verfasserin</subfield><subfield code="0">(orcid)0000-0002-7974-5544</subfield><subfield code="4">aut</subfield></datafield><datafield tag="245" ind1="1" ind2="0"><subfield code="a">Metal-organic framework–derived NiCo</subfield></datafield><datafield tag="264" ind1=" " ind2="1"><subfield code="c">2023</subfield></datafield><datafield tag="336" ind1=" " ind2=" "><subfield code="a">nicht spezifiziert</subfield><subfield code="b">zzz</subfield><subfield code="2">rdacontent</subfield></datafield><datafield tag="337" ind1=" " ind2=" "><subfield code="a">Computermedien</subfield><subfield code="b">c</subfield><subfield code="2">rdamedia</subfield></datafield><datafield tag="338" ind1=" " ind2=" "><subfield code="a">Online-Ressource</subfield><subfield code="b">cr</subfield><subfield code="2">rdacarrier</subfield></datafield><datafield tag="520" ind1=" " ind2=" "><subfield code="a">Ti3C2Tx MXene has become an excellent two-dimensional conductive substrate for electrode materials of supercapacitors (SCs) with prominent physicochemical properties. Whereas, due to the lower theoretical specific capacitance and its interlayer agglomerate, the practical application and electrochemical property of Ti3C2Tx have imposed serious restrictions. Herein, metal-organic framework (MOF) derived NiCo2S4 Co3S4 nanocages with superior yolk-shell structure are introduced to anchor on the surface of Ti3C2Tx via ion exchange reaction and electrostatic attraction, forming the distinctive hierarchical structure of NiCo2S4 @Co3S4/Ti3C2Tx composed of NiCo2S4 @Co3S4 yolk-shell nanocages (NiCo2S4 @Co3S4 YSNs) adsorbed on 2D Ti3C2Tx nanosheets. The NiCo2S4 @Co3S4 YSNs with a large void space, serving as a confined reactor, not only offer a buffer against the volume variation, but also supply abundant active sites and restrain the agglomeration of Ti3C2Tx nanosheets. Furthermore, the novel structure of NiCo2S4 @Co3S4/Ti3C2Tx composite as electrode material could accelerate the thermodynamic stability, suppress the textural instability, and moderate the unavoidable volume change of active substance. Benefited from the above merits, the NiCo2S4 @Co3S4/Ti3C2Tx electrode demonstrates a significant specific capacitance (1872 F g−1 at 2 mV s−1), remarkable rate capability in the high current density (such as, 1121.6 F g−1 at 20 A g−1, 1533 F g−1 at 0.5 A g−1) and displays an excellent life span with 92.2 % of the capacity retention after 12,000 cycles at 10 A g−1. More particularly, the asymmetric supercapacitors (ASCs) fabricated with NiCo2S4 @Co3S4/Ti3C2Tx represent a fascinating energy density of 241.9 Wh kg−1 at a power density of 1125 W kg−1, which can light up 10 LEDs simultaneously. 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author	Wu, Wenling
spellingShingle	Wu, Wenling ddc 670 bkl 51.54 bkl 33.61 bkl 35.90 misc MXenes misc Yolk-shell nanocages misc MOF misc Asymmetric supercapacitors Metal-organic framework–derived NiCo
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topic_title	670 540 VZ 51.54 bkl 33.61 bkl 35.90 bkl Metal-organic framework–derived NiCo MXenes Yolk-shell nanocages MOF Asymmetric supercapacitors
topic	ddc 670 bkl 51.54 bkl 33.61 bkl 35.90 misc MXenes misc Yolk-shell nanocages misc MOF misc Asymmetric supercapacitors
topic_unstemmed	ddc 670 bkl 51.54 bkl 33.61 bkl 35.90 misc MXenes misc Yolk-shell nanocages misc MOF misc Asymmetric supercapacitors
topic_browse	ddc 670 bkl 51.54 bkl 33.61 bkl 35.90 misc MXenes misc Yolk-shell nanocages misc MOF misc Asymmetric supercapacitors
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title	Metal-organic framework–derived NiCo
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title_full	Metal-organic framework–derived NiCo
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author_browse	Wu, Wenling Liu, Tiantian Diwu, Jiahao Li, Chenguang Zhu, Jianfeng
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title_sort	metal-organic framework–derived nico
title_auth	Metal-organic framework–derived NiCo
abstract	Ti3C2Tx MXene has become an excellent two-dimensional conductive substrate for electrode materials of supercapacitors (SCs) with prominent physicochemical properties. Whereas, due to the lower theoretical specific capacitance and its interlayer agglomerate, the practical application and electrochemical property of Ti3C2Tx have imposed serious restrictions. Herein, metal-organic framework (MOF) derived NiCo2S4 Co3S4 nanocages with superior yolk-shell structure are introduced to anchor on the surface of Ti3C2Tx via ion exchange reaction and electrostatic attraction, forming the distinctive hierarchical structure of NiCo2S4 @Co3S4/Ti3C2Tx composed of NiCo2S4 @Co3S4 yolk-shell nanocages (NiCo2S4 @Co3S4 YSNs) adsorbed on 2D Ti3C2Tx nanosheets. The NiCo2S4 @Co3S4 YSNs with a large void space, serving as a confined reactor, not only offer a buffer against the volume variation, but also supply abundant active sites and restrain the agglomeration of Ti3C2Tx nanosheets. Furthermore, the novel structure of NiCo2S4 @Co3S4/Ti3C2Tx composite as electrode material could accelerate the thermodynamic stability, suppress the textural instability, and moderate the unavoidable volume change of active substance. Benefited from the above merits, the NiCo2S4 @Co3S4/Ti3C2Tx electrode demonstrates a significant specific capacitance (1872 F g−1 at 2 mV s−1), remarkable rate capability in the high current density (such as, 1121.6 F g−1 at 20 A g−1, 1533 F g−1 at 0.5 A g−1) and displays an excellent life span with 92.2 % of the capacity retention after 12,000 cycles at 10 A g−1. More particularly, the asymmetric supercapacitors (ASCs) fabricated with NiCo2S4 @Co3S4/Ti3C2Tx represent a fascinating energy density of 241.9 Wh kg−1 at a power density of 1125 W kg−1, which can light up 10 LEDs simultaneously. The results further prove that this rational design method could provide a meaningful prospect for MXenes and MOF derivatives composites for high-performance ASCs.
abstractGer	Ti3C2Tx MXene has become an excellent two-dimensional conductive substrate for electrode materials of supercapacitors (SCs) with prominent physicochemical properties. Whereas, due to the lower theoretical specific capacitance and its interlayer agglomerate, the practical application and electrochemical property of Ti3C2Tx have imposed serious restrictions. Herein, metal-organic framework (MOF) derived NiCo2S4 Co3S4 nanocages with superior yolk-shell structure are introduced to anchor on the surface of Ti3C2Tx via ion exchange reaction and electrostatic attraction, forming the distinctive hierarchical structure of NiCo2S4 @Co3S4/Ti3C2Tx composed of NiCo2S4 @Co3S4 yolk-shell nanocages (NiCo2S4 @Co3S4 YSNs) adsorbed on 2D Ti3C2Tx nanosheets. The NiCo2S4 @Co3S4 YSNs with a large void space, serving as a confined reactor, not only offer a buffer against the volume variation, but also supply abundant active sites and restrain the agglomeration of Ti3C2Tx nanosheets. Furthermore, the novel structure of NiCo2S4 @Co3S4/Ti3C2Tx composite as electrode material could accelerate the thermodynamic stability, suppress the textural instability, and moderate the unavoidable volume change of active substance. Benefited from the above merits, the NiCo2S4 @Co3S4/Ti3C2Tx electrode demonstrates a significant specific capacitance (1872 F g−1 at 2 mV s−1), remarkable rate capability in the high current density (such as, 1121.6 F g−1 at 20 A g−1, 1533 F g−1 at 0.5 A g−1) and displays an excellent life span with 92.2 % of the capacity retention after 12,000 cycles at 10 A g−1. More particularly, the asymmetric supercapacitors (ASCs) fabricated with NiCo2S4 @Co3S4/Ti3C2Tx represent a fascinating energy density of 241.9 Wh kg−1 at a power density of 1125 W kg−1, which can light up 10 LEDs simultaneously. The results further prove that this rational design method could provide a meaningful prospect for MXenes and MOF derivatives composites for high-performance ASCs.
abstract_unstemmed	Ti3C2Tx MXene has become an excellent two-dimensional conductive substrate for electrode materials of supercapacitors (SCs) with prominent physicochemical properties. Whereas, due to the lower theoretical specific capacitance and its interlayer agglomerate, the practical application and electrochemical property of Ti3C2Tx have imposed serious restrictions. Herein, metal-organic framework (MOF) derived NiCo2S4 Co3S4 nanocages with superior yolk-shell structure are introduced to anchor on the surface of Ti3C2Tx via ion exchange reaction and electrostatic attraction, forming the distinctive hierarchical structure of NiCo2S4 @Co3S4/Ti3C2Tx composed of NiCo2S4 @Co3S4 yolk-shell nanocages (NiCo2S4 @Co3S4 YSNs) adsorbed on 2D Ti3C2Tx nanosheets. The NiCo2S4 @Co3S4 YSNs with a large void space, serving as a confined reactor, not only offer a buffer against the volume variation, but also supply abundant active sites and restrain the agglomeration of Ti3C2Tx nanosheets. Furthermore, the novel structure of NiCo2S4 @Co3S4/Ti3C2Tx composite as electrode material could accelerate the thermodynamic stability, suppress the textural instability, and moderate the unavoidable volume change of active substance. Benefited from the above merits, the NiCo2S4 @Co3S4/Ti3C2Tx electrode demonstrates a significant specific capacitance (1872 F g−1 at 2 mV s−1), remarkable rate capability in the high current density (such as, 1121.6 F g−1 at 20 A g−1, 1533 F g−1 at 0.5 A g−1) and displays an excellent life span with 92.2 % of the capacity retention after 12,000 cycles at 10 A g−1. More particularly, the asymmetric supercapacitors (ASCs) fabricated with NiCo2S4 @Co3S4/Ti3C2Tx represent a fascinating energy density of 241.9 Wh kg−1 at a power density of 1125 W kg−1, which can light up 10 LEDs simultaneously. The results further prove that this rational design method could provide a meaningful prospect for MXenes and MOF derivatives composites for high-performance ASCs.
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title_short	Metal-organic framework–derived NiCo
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author2	Liu, Tiantian Diwu, Jiahao Li, Chenguang Zhu, Jianfeng
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doi_str	10.1016/j.jallcom.2023.170213
up_date	2024-07-07T00:15:38.976Z
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fullrecord_marcxml	<?xml version="1.0" encoding="UTF-8"?><collection xmlns="http://www.loc.gov/MARC21/slim"><record><leader>01000naa a22002652 4500</leader><controlfield tag="001">ELV00976075X</controlfield><controlfield tag="003">DE-627</controlfield><controlfield tag="005">20230530150233.0</controlfield><controlfield tag="007">cr uuu---uuuuu</controlfield><controlfield tag="008">230530s2023 xx \|\|\|\|\|o 00\| \|\|eng c</controlfield><datafield tag="024" ind1="7" ind2=" "><subfield code="a">10.1016/j.jallcom.2023.170213</subfield><subfield code="2">doi</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(DE-627)ELV00976075X</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(ELSEVIER)S0925-8388(23)01516-5</subfield></datafield><datafield tag="040" ind1=" " ind2=" "><subfield code="a">DE-627</subfield><subfield code="b">ger</subfield><subfield code="c">DE-627</subfield><subfield code="e">rda</subfield></datafield><datafield tag="041" ind1=" " ind2=" "><subfield code="a">eng</subfield></datafield><datafield tag="082" ind1="0" ind2="4"><subfield code="a">670</subfield><subfield code="a">540</subfield><subfield code="q">VZ</subfield></datafield><datafield tag="084" ind1=" " ind2=" "><subfield code="a">51.54</subfield><subfield code="2">bkl</subfield></datafield><datafield tag="084" ind1=" " ind2=" "><subfield code="a">33.61</subfield><subfield code="2">bkl</subfield></datafield><datafield tag="084" ind1=" " ind2=" "><subfield code="a">35.90</subfield><subfield code="2">bkl</subfield></datafield><datafield tag="100" ind1="1" ind2=" "><subfield code="a">Wu, Wenling</subfield><subfield code="e">verfasserin</subfield><subfield code="0">(orcid)0000-0002-7974-5544</subfield><subfield code="4">aut</subfield></datafield><datafield tag="245" ind1="1" ind2="0"><subfield code="a">Metal-organic framework–derived NiCo</subfield></datafield><datafield tag="264" ind1=" " ind2="1"><subfield code="c">2023</subfield></datafield><datafield tag="336" ind1=" " ind2=" "><subfield code="a">nicht spezifiziert</subfield><subfield code="b">zzz</subfield><subfield code="2">rdacontent</subfield></datafield><datafield tag="337" ind1=" " ind2=" "><subfield code="a">Computermedien</subfield><subfield code="b">c</subfield><subfield code="2">rdamedia</subfield></datafield><datafield tag="338" ind1=" " ind2=" "><subfield code="a">Online-Ressource</subfield><subfield code="b">cr</subfield><subfield code="2">rdacarrier</subfield></datafield><datafield tag="520" ind1=" " ind2=" "><subfield code="a">Ti3C2Tx MXene has become an excellent two-dimensional conductive substrate for electrode materials of supercapacitors (SCs) with prominent physicochemical properties. Whereas, due to the lower theoretical specific capacitance and its interlayer agglomerate, the practical application and electrochemical property of Ti3C2Tx have imposed serious restrictions. Herein, metal-organic framework (MOF) derived NiCo2S4 Co3S4 nanocages with superior yolk-shell structure are introduced to anchor on the surface of Ti3C2Tx via ion exchange reaction and electrostatic attraction, forming the distinctive hierarchical structure of NiCo2S4 @Co3S4/Ti3C2Tx composed of NiCo2S4 @Co3S4 yolk-shell nanocages (NiCo2S4 @Co3S4 YSNs) adsorbed on 2D Ti3C2Tx nanosheets. The NiCo2S4 @Co3S4 YSNs with a large void space, serving as a confined reactor, not only offer a buffer against the volume variation, but also supply abundant active sites and restrain the agglomeration of Ti3C2Tx nanosheets. Furthermore, the novel structure of NiCo2S4 @Co3S4/Ti3C2Tx composite as electrode material could accelerate the thermodynamic stability, suppress the textural instability, and moderate the unavoidable volume change of active substance. Benefited from the above merits, the NiCo2S4 @Co3S4/Ti3C2Tx electrode demonstrates a significant specific capacitance (1872 F g−1 at 2 mV s−1), remarkable rate capability in the high current density (such as, 1121.6 F g−1 at 20 A g−1, 1533 F g−1 at 0.5 A g−1) and displays an excellent life span with 92.2 % of the capacity retention after 12,000 cycles at 10 A g−1. More particularly, the asymmetric supercapacitors (ASCs) fabricated with NiCo2S4 @Co3S4/Ti3C2Tx represent a fascinating energy density of 241.9 Wh kg−1 at a power density of 1125 W kg−1, which can light up 10 LEDs simultaneously. The results further prove that this rational design method could provide a meaningful prospect for MXenes and MOF derivatives composites for high-performance ASCs.</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">MXenes</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Yolk-shell nanocages</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">MOF</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Asymmetric supercapacitors</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Liu, Tiantian</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Diwu, Jiahao</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Li, Chenguang</subfield><subfield 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Metal-organic framework–derived NiCo

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