Polyrotaxane in-situ copolymerization stretchable supramolecular hydrogels for photo-controlled cascade energy transfer

Amphiphilic polysorbate (Tween 80) encapsulated hydrophobic methyl acrylate (MA), spiropyran (SP), nitrobenzoxadiazole (NBDAE) and cyanine 5 (Cy5) was mixed to form micelles, which in-situ copolymerized with acrylamide (AM) and polyrotaxane (PR) containing polyethylene glycol (PEG) threaded into vin...
Ausführliche Beschreibung

Gespeichert in:

Autor*in:	Zhang, Hui [verfasserIn] Zhang, Yi [verfasserIn] Chen, Yong [verfasserIn] Wang, Shuai-Peng [verfasserIn] Zhang, Chang [verfasserIn] Liu, Yu [verfasserIn]

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2023

Schlagwörter:	Polyrotaxane Cascade energy transfer Hydrogel Copolymerization Photo-control

Übergeordnetes Werk:	Enthalten in: European polymer journal - New York, NY [u.a.] : Elsevier, 1965, 192
Übergeordnetes Werk:	volume:192

DOI / URN:	10.1016/j.eurpolymj.2023.112070

Katalog-ID:	ELV009903933

Internformat


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245	1	0	\|a Polyrotaxane in-situ copolymerization stretchable supramolecular hydrogels for photo-controlled cascade energy transfer
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520			\|a Amphiphilic polysorbate (Tween 80) encapsulated hydrophobic methyl acrylate (MA), spiropyran (SP), nitrobenzoxadiazole (NBDAE) and cyanine 5 (Cy5) was mixed to form micelles, which in-situ copolymerized with acrylamide (AM) and polyrotaxane (PR) containing polyethylene glycol (PEG) threaded into vinyl modified α-cyclodextrin (α-CD) with amantadine end-capping to form stretchable supramolecular hydrogel. Benefiting from the sliding cross-linking points of PR, the hydrogel exhibited excellent mechanical properties (1300 % breaking strain and 0.26 MPa breaking stress). Meanwhile, photoreactive achievement of reversible SP acted as primary energy acceptor tuned cascade energy transfer from energy donor NBDAE to secondary acceptor Cy5 (energy transfer efficiency = 80 % for primary transfer, 65 % for secondary transfer). Therefore, this stretchable supramolecular hydrogel material can achieve phototunable multi-color emission and be applied in the field of time-resolved information anti-counterfeiting.
650		4	\|a Polyrotaxane
650		4	\|a Cascade energy transfer
650		4	\|a Hydrogel
650		4	\|a Copolymerization
650		4	\|a Photo-control
700	1		\|a Zhang, Yi \|e verfasserin \|4 aut
700	1		\|a Chen, Yong \|e verfasserin \|4 aut
700	1		\|a Wang, Shuai-Peng \|e verfasserin \|4 aut
700	1		\|a Zhang, Chang \|e verfasserin \|4 aut
700	1		\|a Liu, Yu \|e verfasserin \|4 aut
773	0	8	\|i Enthalten in \|t European polymer journal \|d New York, NY [u.a.] : Elsevier, 1965 \|g 192 \|h Online-Ressource \|w (DE-627)300897375 \|w (DE-600)1483529-0 \|w (DE-576)259270830 \|7 nnns
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912			\|a GBV_ILN_100
912			\|a GBV_ILN_105
912			\|a GBV_ILN_110
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912			\|a GBV_ILN_2021
912			\|a GBV_ILN_2025
912			\|a GBV_ILN_2026
912			\|a GBV_ILN_2027
912			\|a GBV_ILN_2034
912			\|a GBV_ILN_2044
912			\|a GBV_ILN_2048
912			\|a GBV_ILN_2049
912			\|a GBV_ILN_2050
912			\|a GBV_ILN_2055
912			\|a GBV_ILN_2056
912			\|a GBV_ILN_2059
912			\|a GBV_ILN_2061
912			\|a GBV_ILN_2064
912			\|a GBV_ILN_2106
912			\|a GBV_ILN_2110
912			\|a GBV_ILN_2111
912			\|a GBV_ILN_2112
912			\|a GBV_ILN_2122
912			\|a GBV_ILN_2129
912			\|a GBV_ILN_2143
912			\|a GBV_ILN_2152
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912			\|a GBV_ILN_2190
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912			\|a GBV_ILN_2411
912			\|a GBV_ILN_2470
912			\|a GBV_ILN_2507
912			\|a GBV_ILN_4035
912			\|a GBV_ILN_4037
912			\|a GBV_ILN_4112
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912			\|a GBV_ILN_4306
912			\|a GBV_ILN_4307
912			\|a GBV_ILN_4313
912			\|a GBV_ILN_4322
912			\|a GBV_ILN_4323
912			\|a GBV_ILN_4324
912			\|a GBV_ILN_4326
912			\|a GBV_ILN_4333
912			\|a GBV_ILN_4334
912			\|a GBV_ILN_4338
912			\|a GBV_ILN_4393
912			\|a GBV_ILN_4700
936	b	k	\|a 35.80 \|j Makromolekulare Chemie \|q VZ
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Indexfelder

author_variant	h z hz y z yz y c yc s p w spw c z cz y l yl
matchkey_str	zhanghuizhangyichenyongwangshuaipengzhan:2023----:oyoaaeniuooyeiaintecalspaoeuahdoesopooo
hierarchy_sort_str	2023
bklnumber	35.80
publishDate	2023
allfields	10.1016/j.eurpolymj.2023.112070 doi (DE-627)ELV009903933 (ELSEVIER)S0014-3057(23)00253-7 DE-627 ger DE-627 rda eng 670 VZ 35.80 bkl Zhang, Hui verfasserin aut Polyrotaxane in-situ copolymerization stretchable supramolecular hydrogels for photo-controlled cascade energy transfer 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Amphiphilic polysorbate (Tween 80) encapsulated hydrophobic methyl acrylate (MA), spiropyran (SP), nitrobenzoxadiazole (NBDAE) and cyanine 5 (Cy5) was mixed to form micelles, which in-situ copolymerized with acrylamide (AM) and polyrotaxane (PR) containing polyethylene glycol (PEG) threaded into vinyl modified α-cyclodextrin (α-CD) with amantadine end-capping to form stretchable supramolecular hydrogel. Benefiting from the sliding cross-linking points of PR, the hydrogel exhibited excellent mechanical properties (1300 % breaking strain and 0.26 MPa breaking stress). Meanwhile, photoreactive achievement of reversible SP acted as primary energy acceptor tuned cascade energy transfer from energy donor NBDAE to secondary acceptor Cy5 (energy transfer efficiency = 80 % for primary transfer, 65 % for secondary transfer). Therefore, this stretchable supramolecular hydrogel material can achieve phototunable multi-color emission and be applied in the field of time-resolved information anti-counterfeiting. Polyrotaxane Cascade energy transfer Hydrogel Copolymerization Photo-control Zhang, Yi verfasserin aut Chen, Yong verfasserin aut Wang, Shuai-Peng verfasserin aut Zhang, Chang verfasserin aut Liu, Yu verfasserin aut Enthalten in European polymer journal New York, NY [u.a.] : Elsevier, 1965 192 Online-Ressource (DE-627)300897375 (DE-600)1483529-0 (DE-576)259270830 nnns volume:192 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2411 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.80 Makromolekulare Chemie VZ AR 192
spelling	10.1016/j.eurpolymj.2023.112070 doi (DE-627)ELV009903933 (ELSEVIER)S0014-3057(23)00253-7 DE-627 ger DE-627 rda eng 670 VZ 35.80 bkl Zhang, Hui verfasserin aut Polyrotaxane in-situ copolymerization stretchable supramolecular hydrogels for photo-controlled cascade energy transfer 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Amphiphilic polysorbate (Tween 80) encapsulated hydrophobic methyl acrylate (MA), spiropyran (SP), nitrobenzoxadiazole (NBDAE) and cyanine 5 (Cy5) was mixed to form micelles, which in-situ copolymerized with acrylamide (AM) and polyrotaxane (PR) containing polyethylene glycol (PEG) threaded into vinyl modified α-cyclodextrin (α-CD) with amantadine end-capping to form stretchable supramolecular hydrogel. Benefiting from the sliding cross-linking points of PR, the hydrogel exhibited excellent mechanical properties (1300 % breaking strain and 0.26 MPa breaking stress). Meanwhile, photoreactive achievement of reversible SP acted as primary energy acceptor tuned cascade energy transfer from energy donor NBDAE to secondary acceptor Cy5 (energy transfer efficiency = 80 % for primary transfer, 65 % for secondary transfer). Therefore, this stretchable supramolecular hydrogel material can achieve phototunable multi-color emission and be applied in the field of time-resolved information anti-counterfeiting. Polyrotaxane Cascade energy transfer Hydrogel Copolymerization Photo-control Zhang, Yi verfasserin aut Chen, Yong verfasserin aut Wang, Shuai-Peng verfasserin aut Zhang, Chang verfasserin aut Liu, Yu verfasserin aut Enthalten in European polymer journal New York, NY [u.a.] : Elsevier, 1965 192 Online-Ressource (DE-627)300897375 (DE-600)1483529-0 (DE-576)259270830 nnns volume:192 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2411 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.80 Makromolekulare Chemie VZ AR 192
allfields_unstemmed	10.1016/j.eurpolymj.2023.112070 doi (DE-627)ELV009903933 (ELSEVIER)S0014-3057(23)00253-7 DE-627 ger DE-627 rda eng 670 VZ 35.80 bkl Zhang, Hui verfasserin aut Polyrotaxane in-situ copolymerization stretchable supramolecular hydrogels for photo-controlled cascade energy transfer 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Amphiphilic polysorbate (Tween 80) encapsulated hydrophobic methyl acrylate (MA), spiropyran (SP), nitrobenzoxadiazole (NBDAE) and cyanine 5 (Cy5) was mixed to form micelles, which in-situ copolymerized with acrylamide (AM) and polyrotaxane (PR) containing polyethylene glycol (PEG) threaded into vinyl modified α-cyclodextrin (α-CD) with amantadine end-capping to form stretchable supramolecular hydrogel. Benefiting from the sliding cross-linking points of PR, the hydrogel exhibited excellent mechanical properties (1300 % breaking strain and 0.26 MPa breaking stress). Meanwhile, photoreactive achievement of reversible SP acted as primary energy acceptor tuned cascade energy transfer from energy donor NBDAE to secondary acceptor Cy5 (energy transfer efficiency = 80 % for primary transfer, 65 % for secondary transfer). Therefore, this stretchable supramolecular hydrogel material can achieve phototunable multi-color emission and be applied in the field of time-resolved information anti-counterfeiting. Polyrotaxane Cascade energy transfer Hydrogel Copolymerization Photo-control Zhang, Yi verfasserin aut Chen, Yong verfasserin aut Wang, Shuai-Peng verfasserin aut Zhang, Chang verfasserin aut Liu, Yu verfasserin aut Enthalten in European polymer journal New York, NY [u.a.] : Elsevier, 1965 192 Online-Ressource (DE-627)300897375 (DE-600)1483529-0 (DE-576)259270830 nnns volume:192 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2411 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.80 Makromolekulare Chemie VZ AR 192
allfieldsGer	10.1016/j.eurpolymj.2023.112070 doi (DE-627)ELV009903933 (ELSEVIER)S0014-3057(23)00253-7 DE-627 ger DE-627 rda eng 670 VZ 35.80 bkl Zhang, Hui verfasserin aut Polyrotaxane in-situ copolymerization stretchable supramolecular hydrogels for photo-controlled cascade energy transfer 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Amphiphilic polysorbate (Tween 80) encapsulated hydrophobic methyl acrylate (MA), spiropyran (SP), nitrobenzoxadiazole (NBDAE) and cyanine 5 (Cy5) was mixed to form micelles, which in-situ copolymerized with acrylamide (AM) and polyrotaxane (PR) containing polyethylene glycol (PEG) threaded into vinyl modified α-cyclodextrin (α-CD) with amantadine end-capping to form stretchable supramolecular hydrogel. Benefiting from the sliding cross-linking points of PR, the hydrogel exhibited excellent mechanical properties (1300 % breaking strain and 0.26 MPa breaking stress). Meanwhile, photoreactive achievement of reversible SP acted as primary energy acceptor tuned cascade energy transfer from energy donor NBDAE to secondary acceptor Cy5 (energy transfer efficiency = 80 % for primary transfer, 65 % for secondary transfer). Therefore, this stretchable supramolecular hydrogel material can achieve phototunable multi-color emission and be applied in the field of time-resolved information anti-counterfeiting. Polyrotaxane Cascade energy transfer Hydrogel Copolymerization Photo-control Zhang, Yi verfasserin aut Chen, Yong verfasserin aut Wang, Shuai-Peng verfasserin aut Zhang, Chang verfasserin aut Liu, Yu verfasserin aut Enthalten in European polymer journal New York, NY [u.a.] : Elsevier, 1965 192 Online-Ressource (DE-627)300897375 (DE-600)1483529-0 (DE-576)259270830 nnns volume:192 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2411 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.80 Makromolekulare Chemie VZ AR 192
allfieldsSound	10.1016/j.eurpolymj.2023.112070 doi (DE-627)ELV009903933 (ELSEVIER)S0014-3057(23)00253-7 DE-627 ger DE-627 rda eng 670 VZ 35.80 bkl Zhang, Hui verfasserin aut Polyrotaxane in-situ copolymerization stretchable supramolecular hydrogels for photo-controlled cascade energy transfer 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Amphiphilic polysorbate (Tween 80) encapsulated hydrophobic methyl acrylate (MA), spiropyran (SP), nitrobenzoxadiazole (NBDAE) and cyanine 5 (Cy5) was mixed to form micelles, which in-situ copolymerized with acrylamide (AM) and polyrotaxane (PR) containing polyethylene glycol (PEG) threaded into vinyl modified α-cyclodextrin (α-CD) with amantadine end-capping to form stretchable supramolecular hydrogel. Benefiting from the sliding cross-linking points of PR, the hydrogel exhibited excellent mechanical properties (1300 % breaking strain and 0.26 MPa breaking stress). Meanwhile, photoreactive achievement of reversible SP acted as primary energy acceptor tuned cascade energy transfer from energy donor NBDAE to secondary acceptor Cy5 (energy transfer efficiency = 80 % for primary transfer, 65 % for secondary transfer). Therefore, this stretchable supramolecular hydrogel material can achieve phototunable multi-color emission and be applied in the field of time-resolved information anti-counterfeiting. Polyrotaxane Cascade energy transfer Hydrogel Copolymerization Photo-control Zhang, Yi verfasserin aut Chen, Yong verfasserin aut Wang, Shuai-Peng verfasserin aut Zhang, Chang verfasserin aut Liu, Yu verfasserin aut Enthalten in European polymer journal New York, NY [u.a.] : Elsevier, 1965 192 Online-Ressource (DE-627)300897375 (DE-600)1483529-0 (DE-576)259270830 nnns volume:192 GBV_USEFLAG_U SYSFLAG_U GBV_ELV GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2411 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 35.80 Makromolekulare Chemie VZ AR 192
language	English
source	Enthalten in European polymer journal 192 volume:192
sourceStr	Enthalten in European polymer journal 192 volume:192
format_phy_str_mv	Article
bklname	Makromolekulare Chemie
institution	findex.gbv.de
topic_facet	Polyrotaxane Cascade energy transfer Hydrogel Copolymerization Photo-control
dewey-raw	670
isfreeaccess_bool	false
container_title	European polymer journal
authorswithroles_txt_mv	Zhang, Hui @@aut@@ Zhang, Yi @@aut@@ Chen, Yong @@aut@@ Wang, Shuai-Peng @@aut@@ Zhang, Chang @@aut@@ Liu, Yu @@aut@@
publishDateDaySort_date	2023-01-01T00:00:00Z
hierarchy_top_id	300897375
dewey-sort	3670
id	ELV009903933
language_de	englisch
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author	Zhang, Hui
spellingShingle	Zhang, Hui ddc 670 bkl 35.80 misc Polyrotaxane misc Cascade energy transfer misc Hydrogel misc Copolymerization misc Photo-control Polyrotaxane in-situ copolymerization stretchable supramolecular hydrogels for photo-controlled cascade energy transfer
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topic_title	670 VZ 35.80 bkl Polyrotaxane in-situ copolymerization stretchable supramolecular hydrogels for photo-controlled cascade energy transfer Polyrotaxane Cascade energy transfer Hydrogel Copolymerization Photo-control
topic	ddc 670 bkl 35.80 misc Polyrotaxane misc Cascade energy transfer misc Hydrogel misc Copolymerization misc Photo-control
topic_unstemmed	ddc 670 bkl 35.80 misc Polyrotaxane misc Cascade energy transfer misc Hydrogel misc Copolymerization misc Photo-control
topic_browse	ddc 670 bkl 35.80 misc Polyrotaxane misc Cascade energy transfer misc Hydrogel misc Copolymerization misc Photo-control
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title	Polyrotaxane in-situ copolymerization stretchable supramolecular hydrogels for photo-controlled cascade energy transfer
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title_full	Polyrotaxane in-situ copolymerization stretchable supramolecular hydrogels for photo-controlled cascade energy transfer
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author_browse	Zhang, Hui Zhang, Yi Chen, Yong Wang, Shuai-Peng Zhang, Chang Liu, Yu
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author-letter	Zhang, Hui
doi_str_mv	10.1016/j.eurpolymj.2023.112070
dewey-full	670
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title_sort	polyrotaxane in-situ copolymerization stretchable supramolecular hydrogels for photo-controlled cascade energy transfer
title_auth	Polyrotaxane in-situ copolymerization stretchable supramolecular hydrogels for photo-controlled cascade energy transfer
abstract	Amphiphilic polysorbate (Tween 80) encapsulated hydrophobic methyl acrylate (MA), spiropyran (SP), nitrobenzoxadiazole (NBDAE) and cyanine 5 (Cy5) was mixed to form micelles, which in-situ copolymerized with acrylamide (AM) and polyrotaxane (PR) containing polyethylene glycol (PEG) threaded into vinyl modified α-cyclodextrin (α-CD) with amantadine end-capping to form stretchable supramolecular hydrogel. Benefiting from the sliding cross-linking points of PR, the hydrogel exhibited excellent mechanical properties (1300 % breaking strain and 0.26 MPa breaking stress). Meanwhile, photoreactive achievement of reversible SP acted as primary energy acceptor tuned cascade energy transfer from energy donor NBDAE to secondary acceptor Cy5 (energy transfer efficiency = 80 % for primary transfer, 65 % for secondary transfer). Therefore, this stretchable supramolecular hydrogel material can achieve phototunable multi-color emission and be applied in the field of time-resolved information anti-counterfeiting.
abstractGer	Amphiphilic polysorbate (Tween 80) encapsulated hydrophobic methyl acrylate (MA), spiropyran (SP), nitrobenzoxadiazole (NBDAE) and cyanine 5 (Cy5) was mixed to form micelles, which in-situ copolymerized with acrylamide (AM) and polyrotaxane (PR) containing polyethylene glycol (PEG) threaded into vinyl modified α-cyclodextrin (α-CD) with amantadine end-capping to form stretchable supramolecular hydrogel. Benefiting from the sliding cross-linking points of PR, the hydrogel exhibited excellent mechanical properties (1300 % breaking strain and 0.26 MPa breaking stress). Meanwhile, photoreactive achievement of reversible SP acted as primary energy acceptor tuned cascade energy transfer from energy donor NBDAE to secondary acceptor Cy5 (energy transfer efficiency = 80 % for primary transfer, 65 % for secondary transfer). Therefore, this stretchable supramolecular hydrogel material can achieve phototunable multi-color emission and be applied in the field of time-resolved information anti-counterfeiting.
abstract_unstemmed	Amphiphilic polysorbate (Tween 80) encapsulated hydrophobic methyl acrylate (MA), spiropyran (SP), nitrobenzoxadiazole (NBDAE) and cyanine 5 (Cy5) was mixed to form micelles, which in-situ copolymerized with acrylamide (AM) and polyrotaxane (PR) containing polyethylene glycol (PEG) threaded into vinyl modified α-cyclodextrin (α-CD) with amantadine end-capping to form stretchable supramolecular hydrogel. Benefiting from the sliding cross-linking points of PR, the hydrogel exhibited excellent mechanical properties (1300 % breaking strain and 0.26 MPa breaking stress). Meanwhile, photoreactive achievement of reversible SP acted as primary energy acceptor tuned cascade energy transfer from energy donor NBDAE to secondary acceptor Cy5 (energy transfer efficiency = 80 % for primary transfer, 65 % for secondary transfer). Therefore, this stretchable supramolecular hydrogel material can achieve phototunable multi-color emission and be applied in the field of time-resolved information anti-counterfeiting.
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title_short	Polyrotaxane in-situ copolymerization stretchable supramolecular hydrogels for photo-controlled cascade energy transfer
remote_bool	true
author2	Zhang, Yi Chen, Yong Wang, Shuai-Peng Zhang, Chang Liu, Yu
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doi_str	10.1016/j.eurpolymj.2023.112070
up_date	2024-07-07T00:45:24.724Z
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Polyrotaxane in-situ copolymerization stretchable supramolecular hydrogels for photo-controlled cascade energy transfer

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