Contamination characteristics of polycyclic aromatic compounds from coal sources in typical coal mining areas in Huaibei area, China
The Huaibei area is rich in coal resources and serves as the main energy production base in East China. However, serious environmental consequences are associated with coal mining and utilization. With increasing reports on distribution and risks by polycyclic aromatic compounds (PACs), the potentia...
Ausführliche Beschreibung
Autor*in: |
Xu, Zhenpeng [verfasserIn] Qian, Yahui [verfasserIn] Hong, Xiuping [verfasserIn] Luo, Zhonggeng [verfasserIn] Gao, Xiulong [verfasserIn] Liang, Handong [verfasserIn] |
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E-Artikel |
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Sprache: |
Englisch |
Erschienen: |
2023 |
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Übergeordnetes Werk: |
Enthalten in: The science of the total environment - Amsterdam [u.a.] : Elsevier Science, 1972, 873 |
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Übergeordnetes Werk: |
volume:873 |
DOI / URN: |
10.1016/j.scitotenv.2023.162311 |
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Katalog-ID: |
ELV01014014X |
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520 | |a The Huaibei area is rich in coal resources and serves as the main energy production base in East China. However, serious environmental consequences are associated with coal mining and utilization. With increasing reports on distribution and risks by polycyclic aromatic compounds (PACs), the potential pollution of coal sources must be addressed. Here, the PAC concentrations in the topsoil, coal, and coal gangue of a typical coal mining area in Huaibei were evaluated. The mean ΣPACs in topsoil, coal, and coal gangue were 1528.3, 274,815.8, and 10,908.3 μg·kg−1, respectively. Alkyl polycyclic aromatic hydrocarbons (aPAHs) were identified as primary contributors to PACs, and the concentrations of oxygenated PAHs (oPAHs) were significantly higher in coal and coal gangue than in topsoil. PAC pollution was mainly concentrated in the coal mine area and near the coal gangue landfill road. Not only sixteen high priority pollutant PAHs (16PAHs), but PAH derivatives also contributed to the organic pollution from coal sources. Principal components analysis, multiple linear regression, characteristic ratios, and positive matrix factor analysis were used to trace PAC sources. The characteristic ratios for organic pollution from coal and gangue particles involving 16PAHs, aPAHs, and oPAHs were proposed. Further, the high–ring 16PAH ratio was also found suitable for coal mining areas. The Monte–Carlo risk assessment showed that coal particles were highly carcinogenic, and despite the low carcinogenicity of coal gangue and topsoil, they might also serve as potential carcinogens. This study aimed to disseminate knowledge on PACs from coal and coal gangue, provide a useful background for efficient resource utilization of coal gangue, and a reference for tracing PAC sources in coal mine environment media. | ||
650 | 4 | |a Coal mine area | |
650 | 4 | |a Polycyclic aromatic compounds | |
650 | 4 | |a Topsoil | |
650 | 4 | |a Analysis of sources | |
650 | 4 | |a Monte–Carlo simulation | |
700 | 1 | |a Qian, Yahui |e verfasserin |4 aut | |
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700 | 1 | |a Liang, Handong |e verfasserin |4 aut | |
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10.1016/j.scitotenv.2023.162311 doi (DE-627)ELV01014014X (ELSEVIER)S0048-9697(23)00927-0 DE-627 ger DE-627 rda eng 333.7 610 VZ 43.12 bkl 43.13 bkl 44.13 bkl Xu, Zhenpeng verfasserin aut Contamination characteristics of polycyclic aromatic compounds from coal sources in typical coal mining areas in Huaibei area, China 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The Huaibei area is rich in coal resources and serves as the main energy production base in East China. However, serious environmental consequences are associated with coal mining and utilization. With increasing reports on distribution and risks by polycyclic aromatic compounds (PACs), the potential pollution of coal sources must be addressed. Here, the PAC concentrations in the topsoil, coal, and coal gangue of a typical coal mining area in Huaibei were evaluated. The mean ΣPACs in topsoil, coal, and coal gangue were 1528.3, 274,815.8, and 10,908.3 μg·kg−1, respectively. Alkyl polycyclic aromatic hydrocarbons (aPAHs) were identified as primary contributors to PACs, and the concentrations of oxygenated PAHs (oPAHs) were significantly higher in coal and coal gangue than in topsoil. PAC pollution was mainly concentrated in the coal mine area and near the coal gangue landfill road. Not only sixteen high priority pollutant PAHs (16PAHs), but PAH derivatives also contributed to the organic pollution from coal sources. Principal components analysis, multiple linear regression, characteristic ratios, and positive matrix factor analysis were used to trace PAC sources. The characteristic ratios for organic pollution from coal and gangue particles involving 16PAHs, aPAHs, and oPAHs were proposed. Further, the high–ring 16PAH ratio was also found suitable for coal mining areas. The Monte–Carlo risk assessment showed that coal particles were highly carcinogenic, and despite the low carcinogenicity of coal gangue and topsoil, they might also serve as potential carcinogens. This study aimed to disseminate knowledge on PACs from coal and coal gangue, provide a useful background for efficient resource utilization of coal gangue, and a reference for tracing PAC sources in coal mine environment media. Coal mine area Polycyclic aromatic compounds Topsoil Analysis of sources Monte–Carlo simulation Qian, Yahui verfasserin aut Hong, Xiuping verfasserin aut Luo, Zhonggeng verfasserin aut Gao, Xiulong verfasserin aut Liang, Handong verfasserin aut Enthalten in The science of the total environment Amsterdam [u.a.] : Elsevier Science, 1972 873 Online-Ressource (DE-627)306591456 (DE-600)1498726-0 (DE-576)081953178 1879-1026 nnns volume:873 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA SSG-OPC-GGO GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 43.12 Umweltchemie VZ 43.13 Umwelttoxikologie VZ 44.13 Medizinische Ökologie VZ AR 873 |
spelling |
10.1016/j.scitotenv.2023.162311 doi (DE-627)ELV01014014X (ELSEVIER)S0048-9697(23)00927-0 DE-627 ger DE-627 rda eng 333.7 610 VZ 43.12 bkl 43.13 bkl 44.13 bkl Xu, Zhenpeng verfasserin aut Contamination characteristics of polycyclic aromatic compounds from coal sources in typical coal mining areas in Huaibei area, China 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The Huaibei area is rich in coal resources and serves as the main energy production base in East China. However, serious environmental consequences are associated with coal mining and utilization. With increasing reports on distribution and risks by polycyclic aromatic compounds (PACs), the potential pollution of coal sources must be addressed. Here, the PAC concentrations in the topsoil, coal, and coal gangue of a typical coal mining area in Huaibei were evaluated. The mean ΣPACs in topsoil, coal, and coal gangue were 1528.3, 274,815.8, and 10,908.3 μg·kg−1, respectively. Alkyl polycyclic aromatic hydrocarbons (aPAHs) were identified as primary contributors to PACs, and the concentrations of oxygenated PAHs (oPAHs) were significantly higher in coal and coal gangue than in topsoil. PAC pollution was mainly concentrated in the coal mine area and near the coal gangue landfill road. Not only sixteen high priority pollutant PAHs (16PAHs), but PAH derivatives also contributed to the organic pollution from coal sources. Principal components analysis, multiple linear regression, characteristic ratios, and positive matrix factor analysis were used to trace PAC sources. The characteristic ratios for organic pollution from coal and gangue particles involving 16PAHs, aPAHs, and oPAHs were proposed. Further, the high–ring 16PAH ratio was also found suitable for coal mining areas. The Monte–Carlo risk assessment showed that coal particles were highly carcinogenic, and despite the low carcinogenicity of coal gangue and topsoil, they might also serve as potential carcinogens. This study aimed to disseminate knowledge on PACs from coal and coal gangue, provide a useful background for efficient resource utilization of coal gangue, and a reference for tracing PAC sources in coal mine environment media. Coal mine area Polycyclic aromatic compounds Topsoil Analysis of sources Monte–Carlo simulation Qian, Yahui verfasserin aut Hong, Xiuping verfasserin aut Luo, Zhonggeng verfasserin aut Gao, Xiulong verfasserin aut Liang, Handong verfasserin aut Enthalten in The science of the total environment Amsterdam [u.a.] : Elsevier Science, 1972 873 Online-Ressource (DE-627)306591456 (DE-600)1498726-0 (DE-576)081953178 1879-1026 nnns volume:873 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA SSG-OPC-GGO GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 43.12 Umweltchemie VZ 43.13 Umwelttoxikologie VZ 44.13 Medizinische Ökologie VZ AR 873 |
allfields_unstemmed |
10.1016/j.scitotenv.2023.162311 doi (DE-627)ELV01014014X (ELSEVIER)S0048-9697(23)00927-0 DE-627 ger DE-627 rda eng 333.7 610 VZ 43.12 bkl 43.13 bkl 44.13 bkl Xu, Zhenpeng verfasserin aut Contamination characteristics of polycyclic aromatic compounds from coal sources in typical coal mining areas in Huaibei area, China 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The Huaibei area is rich in coal resources and serves as the main energy production base in East China. However, serious environmental consequences are associated with coal mining and utilization. With increasing reports on distribution and risks by polycyclic aromatic compounds (PACs), the potential pollution of coal sources must be addressed. Here, the PAC concentrations in the topsoil, coal, and coal gangue of a typical coal mining area in Huaibei were evaluated. The mean ΣPACs in topsoil, coal, and coal gangue were 1528.3, 274,815.8, and 10,908.3 μg·kg−1, respectively. Alkyl polycyclic aromatic hydrocarbons (aPAHs) were identified as primary contributors to PACs, and the concentrations of oxygenated PAHs (oPAHs) were significantly higher in coal and coal gangue than in topsoil. PAC pollution was mainly concentrated in the coal mine area and near the coal gangue landfill road. Not only sixteen high priority pollutant PAHs (16PAHs), but PAH derivatives also contributed to the organic pollution from coal sources. Principal components analysis, multiple linear regression, characteristic ratios, and positive matrix factor analysis were used to trace PAC sources. The characteristic ratios for organic pollution from coal and gangue particles involving 16PAHs, aPAHs, and oPAHs were proposed. Further, the high–ring 16PAH ratio was also found suitable for coal mining areas. The Monte–Carlo risk assessment showed that coal particles were highly carcinogenic, and despite the low carcinogenicity of coal gangue and topsoil, they might also serve as potential carcinogens. This study aimed to disseminate knowledge on PACs from coal and coal gangue, provide a useful background for efficient resource utilization of coal gangue, and a reference for tracing PAC sources in coal mine environment media. Coal mine area Polycyclic aromatic compounds Topsoil Analysis of sources Monte–Carlo simulation Qian, Yahui verfasserin aut Hong, Xiuping verfasserin aut Luo, Zhonggeng verfasserin aut Gao, Xiulong verfasserin aut Liang, Handong verfasserin aut Enthalten in The science of the total environment Amsterdam [u.a.] : Elsevier Science, 1972 873 Online-Ressource (DE-627)306591456 (DE-600)1498726-0 (DE-576)081953178 1879-1026 nnns volume:873 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA SSG-OPC-GGO GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 43.12 Umweltchemie VZ 43.13 Umwelttoxikologie VZ 44.13 Medizinische Ökologie VZ AR 873 |
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10.1016/j.scitotenv.2023.162311 doi (DE-627)ELV01014014X (ELSEVIER)S0048-9697(23)00927-0 DE-627 ger DE-627 rda eng 333.7 610 VZ 43.12 bkl 43.13 bkl 44.13 bkl Xu, Zhenpeng verfasserin aut Contamination characteristics of polycyclic aromatic compounds from coal sources in typical coal mining areas in Huaibei area, China 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The Huaibei area is rich in coal resources and serves as the main energy production base in East China. However, serious environmental consequences are associated with coal mining and utilization. With increasing reports on distribution and risks by polycyclic aromatic compounds (PACs), the potential pollution of coal sources must be addressed. Here, the PAC concentrations in the topsoil, coal, and coal gangue of a typical coal mining area in Huaibei were evaluated. The mean ΣPACs in topsoil, coal, and coal gangue were 1528.3, 274,815.8, and 10,908.3 μg·kg−1, respectively. Alkyl polycyclic aromatic hydrocarbons (aPAHs) were identified as primary contributors to PACs, and the concentrations of oxygenated PAHs (oPAHs) were significantly higher in coal and coal gangue than in topsoil. PAC pollution was mainly concentrated in the coal mine area and near the coal gangue landfill road. Not only sixteen high priority pollutant PAHs (16PAHs), but PAH derivatives also contributed to the organic pollution from coal sources. Principal components analysis, multiple linear regression, characteristic ratios, and positive matrix factor analysis were used to trace PAC sources. The characteristic ratios for organic pollution from coal and gangue particles involving 16PAHs, aPAHs, and oPAHs were proposed. Further, the high–ring 16PAH ratio was also found suitable for coal mining areas. The Monte–Carlo risk assessment showed that coal particles were highly carcinogenic, and despite the low carcinogenicity of coal gangue and topsoil, they might also serve as potential carcinogens. This study aimed to disseminate knowledge on PACs from coal and coal gangue, provide a useful background for efficient resource utilization of coal gangue, and a reference for tracing PAC sources in coal mine environment media. Coal mine area Polycyclic aromatic compounds Topsoil Analysis of sources Monte–Carlo simulation Qian, Yahui verfasserin aut Hong, Xiuping verfasserin aut Luo, Zhonggeng verfasserin aut Gao, Xiulong verfasserin aut Liang, Handong verfasserin aut Enthalten in The science of the total environment Amsterdam [u.a.] : Elsevier Science, 1972 873 Online-Ressource (DE-627)306591456 (DE-600)1498726-0 (DE-576)081953178 1879-1026 nnns volume:873 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA SSG-OPC-GGO GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 43.12 Umweltchemie VZ 43.13 Umwelttoxikologie VZ 44.13 Medizinische Ökologie VZ AR 873 |
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10.1016/j.scitotenv.2023.162311 doi (DE-627)ELV01014014X (ELSEVIER)S0048-9697(23)00927-0 DE-627 ger DE-627 rda eng 333.7 610 VZ 43.12 bkl 43.13 bkl 44.13 bkl Xu, Zhenpeng verfasserin aut Contamination characteristics of polycyclic aromatic compounds from coal sources in typical coal mining areas in Huaibei area, China 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier The Huaibei area is rich in coal resources and serves as the main energy production base in East China. However, serious environmental consequences are associated with coal mining and utilization. With increasing reports on distribution and risks by polycyclic aromatic compounds (PACs), the potential pollution of coal sources must be addressed. Here, the PAC concentrations in the topsoil, coal, and coal gangue of a typical coal mining area in Huaibei were evaluated. The mean ΣPACs in topsoil, coal, and coal gangue were 1528.3, 274,815.8, and 10,908.3 μg·kg−1, respectively. Alkyl polycyclic aromatic hydrocarbons (aPAHs) were identified as primary contributors to PACs, and the concentrations of oxygenated PAHs (oPAHs) were significantly higher in coal and coal gangue than in topsoil. PAC pollution was mainly concentrated in the coal mine area and near the coal gangue landfill road. Not only sixteen high priority pollutant PAHs (16PAHs), but PAH derivatives also contributed to the organic pollution from coal sources. Principal components analysis, multiple linear regression, characteristic ratios, and positive matrix factor analysis were used to trace PAC sources. The characteristic ratios for organic pollution from coal and gangue particles involving 16PAHs, aPAHs, and oPAHs were proposed. Further, the high–ring 16PAH ratio was also found suitable for coal mining areas. The Monte–Carlo risk assessment showed that coal particles were highly carcinogenic, and despite the low carcinogenicity of coal gangue and topsoil, they might also serve as potential carcinogens. This study aimed to disseminate knowledge on PACs from coal and coal gangue, provide a useful background for efficient resource utilization of coal gangue, and a reference for tracing PAC sources in coal mine environment media. Coal mine area Polycyclic aromatic compounds Topsoil Analysis of sources Monte–Carlo simulation Qian, Yahui verfasserin aut Hong, Xiuping verfasserin aut Luo, Zhonggeng verfasserin aut Gao, Xiulong verfasserin aut Liang, Handong verfasserin aut Enthalten in The science of the total environment Amsterdam [u.a.] : Elsevier Science, 1972 873 Online-Ressource (DE-627)306591456 (DE-600)1498726-0 (DE-576)081953178 1879-1026 nnns volume:873 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA SSG-OPC-GGO GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 43.12 Umweltchemie VZ 43.13 Umwelttoxikologie VZ 44.13 Medizinische Ökologie VZ AR 873 |
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contamination characteristics of polycyclic aromatic compounds from coal sources in typical coal mining areas in huaibei area, china |
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Contamination characteristics of polycyclic aromatic compounds from coal sources in typical coal mining areas in Huaibei area, China |
abstract |
The Huaibei area is rich in coal resources and serves as the main energy production base in East China. However, serious environmental consequences are associated with coal mining and utilization. With increasing reports on distribution and risks by polycyclic aromatic compounds (PACs), the potential pollution of coal sources must be addressed. Here, the PAC concentrations in the topsoil, coal, and coal gangue of a typical coal mining area in Huaibei were evaluated. The mean ΣPACs in topsoil, coal, and coal gangue were 1528.3, 274,815.8, and 10,908.3 μg·kg−1, respectively. Alkyl polycyclic aromatic hydrocarbons (aPAHs) were identified as primary contributors to PACs, and the concentrations of oxygenated PAHs (oPAHs) were significantly higher in coal and coal gangue than in topsoil. PAC pollution was mainly concentrated in the coal mine area and near the coal gangue landfill road. Not only sixteen high priority pollutant PAHs (16PAHs), but PAH derivatives also contributed to the organic pollution from coal sources. Principal components analysis, multiple linear regression, characteristic ratios, and positive matrix factor analysis were used to trace PAC sources. The characteristic ratios for organic pollution from coal and gangue particles involving 16PAHs, aPAHs, and oPAHs were proposed. Further, the high–ring 16PAH ratio was also found suitable for coal mining areas. The Monte–Carlo risk assessment showed that coal particles were highly carcinogenic, and despite the low carcinogenicity of coal gangue and topsoil, they might also serve as potential carcinogens. This study aimed to disseminate knowledge on PACs from coal and coal gangue, provide a useful background for efficient resource utilization of coal gangue, and a reference for tracing PAC sources in coal mine environment media. |
abstractGer |
The Huaibei area is rich in coal resources and serves as the main energy production base in East China. However, serious environmental consequences are associated with coal mining and utilization. With increasing reports on distribution and risks by polycyclic aromatic compounds (PACs), the potential pollution of coal sources must be addressed. Here, the PAC concentrations in the topsoil, coal, and coal gangue of a typical coal mining area in Huaibei were evaluated. The mean ΣPACs in topsoil, coal, and coal gangue were 1528.3, 274,815.8, and 10,908.3 μg·kg−1, respectively. Alkyl polycyclic aromatic hydrocarbons (aPAHs) were identified as primary contributors to PACs, and the concentrations of oxygenated PAHs (oPAHs) were significantly higher in coal and coal gangue than in topsoil. PAC pollution was mainly concentrated in the coal mine area and near the coal gangue landfill road. Not only sixteen high priority pollutant PAHs (16PAHs), but PAH derivatives also contributed to the organic pollution from coal sources. Principal components analysis, multiple linear regression, characteristic ratios, and positive matrix factor analysis were used to trace PAC sources. The characteristic ratios for organic pollution from coal and gangue particles involving 16PAHs, aPAHs, and oPAHs were proposed. Further, the high–ring 16PAH ratio was also found suitable for coal mining areas. The Monte–Carlo risk assessment showed that coal particles were highly carcinogenic, and despite the low carcinogenicity of coal gangue and topsoil, they might also serve as potential carcinogens. This study aimed to disseminate knowledge on PACs from coal and coal gangue, provide a useful background for efficient resource utilization of coal gangue, and a reference for tracing PAC sources in coal mine environment media. |
abstract_unstemmed |
The Huaibei area is rich in coal resources and serves as the main energy production base in East China. However, serious environmental consequences are associated with coal mining and utilization. With increasing reports on distribution and risks by polycyclic aromatic compounds (PACs), the potential pollution of coal sources must be addressed. Here, the PAC concentrations in the topsoil, coal, and coal gangue of a typical coal mining area in Huaibei were evaluated. The mean ΣPACs in topsoil, coal, and coal gangue were 1528.3, 274,815.8, and 10,908.3 μg·kg−1, respectively. Alkyl polycyclic aromatic hydrocarbons (aPAHs) were identified as primary contributors to PACs, and the concentrations of oxygenated PAHs (oPAHs) were significantly higher in coal and coal gangue than in topsoil. PAC pollution was mainly concentrated in the coal mine area and near the coal gangue landfill road. Not only sixteen high priority pollutant PAHs (16PAHs), but PAH derivatives also contributed to the organic pollution from coal sources. Principal components analysis, multiple linear regression, characteristic ratios, and positive matrix factor analysis were used to trace PAC sources. The characteristic ratios for organic pollution from coal and gangue particles involving 16PAHs, aPAHs, and oPAHs were proposed. Further, the high–ring 16PAH ratio was also found suitable for coal mining areas. The Monte–Carlo risk assessment showed that coal particles were highly carcinogenic, and despite the low carcinogenicity of coal gangue and topsoil, they might also serve as potential carcinogens. This study aimed to disseminate knowledge on PACs from coal and coal gangue, provide a useful background for efficient resource utilization of coal gangue, and a reference for tracing PAC sources in coal mine environment media. |
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score |
7.4031916 |