Low-power, fast response simplified electrochromic device based on functionalized gel electrolyte
Metallo-supramolecular polymer (MEPE)-based thin film electrochromic devices (ECDs) have been considered to be a promising platform for portable electronics as their low cost, excellent redox properties, high optical contrast, and rich colors. However, poor cycle stability and slow response speed ar...
Ausführliche Beschreibung
Autor*in: |
Xu, Lijuan [verfasserIn] Li, Yangyang [verfasserIn] Ji, Yuan [verfasserIn] Zhang, Jichi [verfasserIn] Shao, Lu [verfasserIn] Zhang, Dawei [verfasserIn] Ma, Lina [verfasserIn] Gao, Guolin [verfasserIn] Jiang, Zaixing [verfasserIn] |
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Format: |
E-Artikel |
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Sprache: |
Englisch |
Erschienen: |
2023 |
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Schlagwörter: |
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Übergeordnetes Werk: |
Enthalten in: The chemical engineering journal - Amsterdam : Elsevier, 1997, 467 |
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Übergeordnetes Werk: |
volume:467 |
DOI / URN: |
10.1016/j.cej.2023.143400 |
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Katalog-ID: |
ELV01014286X |
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245 | 1 | 0 | |a Low-power, fast response simplified electrochromic device based on functionalized gel electrolyte |
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520 | |a Metallo-supramolecular polymer (MEPE)-based thin film electrochromic devices (ECDs) have been considered to be a promising platform for portable electronics as their low cost, excellent redox properties, high optical contrast, and rich colors. However, poor cycle stability and slow response speed are serious bottlenecks for widespread commercial devices. Here, a gel electrolyte functionalized by the anodic active species p-benzoquinone (p-BQ) (GET-BQ) was reported. It has outstanding conductivity (∼4.62 mS cm−1) and transparency. Fe(Ⅱ)-MEPE-based ECDs incorporating the GET-BQ electrolyte (ECD-BQ) showed lower voltage operation (∼1.1 V), higher optical contrast (ca. ΔT ∼ 35.7%), faster response rate (tb ∼ 2.5 s, tc ∼ 0.3 s), and superb cycling durability (<1.7% ΔT loss after 1440 cycles) than those without p-BQ. Moreover, the charge transport kinetics of ECD-BQ were explored by the CV curve, in situ infrared spectroelectrochemical analysis, and electrochemical impedance spectroscopy. The charge transfer mechanism of electrochromic material and electrolytes in ECD-BQ offers a novel entry to design superior electrolytes for high-performance ECD. | ||
650 | 4 | |a Functionalized gel electrolyte | |
650 | 4 | |a Cathodic active species | |
650 | 4 | |a Charge-transport kinetic | |
650 | 4 | |a Electrochromic device | |
700 | 1 | |a Li, Yangyang |e verfasserin |4 aut | |
700 | 1 | |a Ji, Yuan |e verfasserin |4 aut | |
700 | 1 | |a Zhang, Jichi |e verfasserin |4 aut | |
700 | 1 | |a Shao, Lu |e verfasserin |4 aut | |
700 | 1 | |a Zhang, Dawei |e verfasserin |4 aut | |
700 | 1 | |a Ma, Lina |e verfasserin |4 aut | |
700 | 1 | |a Gao, Guolin |e verfasserin |0 (orcid)0000-0001-5177-9139 |4 aut | |
700 | 1 | |a Jiang, Zaixing |e verfasserin |4 aut | |
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10.1016/j.cej.2023.143400 doi (DE-627)ELV01014286X (ELSEVIER)S1385-8947(23)02131-9 DE-627 ger DE-627 rda eng 660 VZ 660 VZ 58.10 bkl Xu, Lijuan verfasserin aut Low-power, fast response simplified electrochromic device based on functionalized gel electrolyte 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Metallo-supramolecular polymer (MEPE)-based thin film electrochromic devices (ECDs) have been considered to be a promising platform for portable electronics as their low cost, excellent redox properties, high optical contrast, and rich colors. However, poor cycle stability and slow response speed are serious bottlenecks for widespread commercial devices. Here, a gel electrolyte functionalized by the anodic active species p-benzoquinone (p-BQ) (GET-BQ) was reported. It has outstanding conductivity (∼4.62 mS cm−1) and transparency. Fe(Ⅱ)-MEPE-based ECDs incorporating the GET-BQ electrolyte (ECD-BQ) showed lower voltage operation (∼1.1 V), higher optical contrast (ca. ΔT ∼ 35.7%), faster response rate (tb ∼ 2.5 s, tc ∼ 0.3 s), and superb cycling durability (<1.7% ΔT loss after 1440 cycles) than those without p-BQ. Moreover, the charge transport kinetics of ECD-BQ were explored by the CV curve, in situ infrared spectroelectrochemical analysis, and electrochemical impedance spectroscopy. The charge transfer mechanism of electrochromic material and electrolytes in ECD-BQ offers a novel entry to design superior electrolytes for high-performance ECD. Functionalized gel electrolyte Cathodic active species Charge-transport kinetic Electrochromic device Li, Yangyang verfasserin aut Ji, Yuan verfasserin aut Zhang, Jichi verfasserin aut Shao, Lu verfasserin aut Zhang, Dawei verfasserin aut Ma, Lina verfasserin aut Gao, Guolin verfasserin (orcid)0000-0001-5177-9139 aut Jiang, Zaixing verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 467 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:467 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.10 Verfahrenstechnik: Allgemeines VZ AR 467 |
spelling |
10.1016/j.cej.2023.143400 doi (DE-627)ELV01014286X (ELSEVIER)S1385-8947(23)02131-9 DE-627 ger DE-627 rda eng 660 VZ 660 VZ 58.10 bkl Xu, Lijuan verfasserin aut Low-power, fast response simplified electrochromic device based on functionalized gel electrolyte 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Metallo-supramolecular polymer (MEPE)-based thin film electrochromic devices (ECDs) have been considered to be a promising platform for portable electronics as their low cost, excellent redox properties, high optical contrast, and rich colors. However, poor cycle stability and slow response speed are serious bottlenecks for widespread commercial devices. Here, a gel electrolyte functionalized by the anodic active species p-benzoquinone (p-BQ) (GET-BQ) was reported. It has outstanding conductivity (∼4.62 mS cm−1) and transparency. Fe(Ⅱ)-MEPE-based ECDs incorporating the GET-BQ electrolyte (ECD-BQ) showed lower voltage operation (∼1.1 V), higher optical contrast (ca. ΔT ∼ 35.7%), faster response rate (tb ∼ 2.5 s, tc ∼ 0.3 s), and superb cycling durability (<1.7% ΔT loss after 1440 cycles) than those without p-BQ. Moreover, the charge transport kinetics of ECD-BQ were explored by the CV curve, in situ infrared spectroelectrochemical analysis, and electrochemical impedance spectroscopy. The charge transfer mechanism of electrochromic material and electrolytes in ECD-BQ offers a novel entry to design superior electrolytes for high-performance ECD. Functionalized gel electrolyte Cathodic active species Charge-transport kinetic Electrochromic device Li, Yangyang verfasserin aut Ji, Yuan verfasserin aut Zhang, Jichi verfasserin aut Shao, Lu verfasserin aut Zhang, Dawei verfasserin aut Ma, Lina verfasserin aut Gao, Guolin verfasserin (orcid)0000-0001-5177-9139 aut Jiang, Zaixing verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 467 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:467 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.10 Verfahrenstechnik: Allgemeines VZ AR 467 |
allfields_unstemmed |
10.1016/j.cej.2023.143400 doi (DE-627)ELV01014286X (ELSEVIER)S1385-8947(23)02131-9 DE-627 ger DE-627 rda eng 660 VZ 660 VZ 58.10 bkl Xu, Lijuan verfasserin aut Low-power, fast response simplified electrochromic device based on functionalized gel electrolyte 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Metallo-supramolecular polymer (MEPE)-based thin film electrochromic devices (ECDs) have been considered to be a promising platform for portable electronics as their low cost, excellent redox properties, high optical contrast, and rich colors. However, poor cycle stability and slow response speed are serious bottlenecks for widespread commercial devices. Here, a gel electrolyte functionalized by the anodic active species p-benzoquinone (p-BQ) (GET-BQ) was reported. It has outstanding conductivity (∼4.62 mS cm−1) and transparency. Fe(Ⅱ)-MEPE-based ECDs incorporating the GET-BQ electrolyte (ECD-BQ) showed lower voltage operation (∼1.1 V), higher optical contrast (ca. ΔT ∼ 35.7%), faster response rate (tb ∼ 2.5 s, tc ∼ 0.3 s), and superb cycling durability (<1.7% ΔT loss after 1440 cycles) than those without p-BQ. Moreover, the charge transport kinetics of ECD-BQ were explored by the CV curve, in situ infrared spectroelectrochemical analysis, and electrochemical impedance spectroscopy. The charge transfer mechanism of electrochromic material and electrolytes in ECD-BQ offers a novel entry to design superior electrolytes for high-performance ECD. Functionalized gel electrolyte Cathodic active species Charge-transport kinetic Electrochromic device Li, Yangyang verfasserin aut Ji, Yuan verfasserin aut Zhang, Jichi verfasserin aut Shao, Lu verfasserin aut Zhang, Dawei verfasserin aut Ma, Lina verfasserin aut Gao, Guolin verfasserin (orcid)0000-0001-5177-9139 aut Jiang, Zaixing verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 467 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:467 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.10 Verfahrenstechnik: Allgemeines VZ AR 467 |
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10.1016/j.cej.2023.143400 doi (DE-627)ELV01014286X (ELSEVIER)S1385-8947(23)02131-9 DE-627 ger DE-627 rda eng 660 VZ 660 VZ 58.10 bkl Xu, Lijuan verfasserin aut Low-power, fast response simplified electrochromic device based on functionalized gel electrolyte 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Metallo-supramolecular polymer (MEPE)-based thin film electrochromic devices (ECDs) have been considered to be a promising platform for portable electronics as their low cost, excellent redox properties, high optical contrast, and rich colors. However, poor cycle stability and slow response speed are serious bottlenecks for widespread commercial devices. Here, a gel electrolyte functionalized by the anodic active species p-benzoquinone (p-BQ) (GET-BQ) was reported. It has outstanding conductivity (∼4.62 mS cm−1) and transparency. Fe(Ⅱ)-MEPE-based ECDs incorporating the GET-BQ electrolyte (ECD-BQ) showed lower voltage operation (∼1.1 V), higher optical contrast (ca. ΔT ∼ 35.7%), faster response rate (tb ∼ 2.5 s, tc ∼ 0.3 s), and superb cycling durability (<1.7% ΔT loss after 1440 cycles) than those without p-BQ. Moreover, the charge transport kinetics of ECD-BQ were explored by the CV curve, in situ infrared spectroelectrochemical analysis, and electrochemical impedance spectroscopy. The charge transfer mechanism of electrochromic material and electrolytes in ECD-BQ offers a novel entry to design superior electrolytes for high-performance ECD. Functionalized gel electrolyte Cathodic active species Charge-transport kinetic Electrochromic device Li, Yangyang verfasserin aut Ji, Yuan verfasserin aut Zhang, Jichi verfasserin aut Shao, Lu verfasserin aut Zhang, Dawei verfasserin aut Ma, Lina verfasserin aut Gao, Guolin verfasserin (orcid)0000-0001-5177-9139 aut Jiang, Zaixing verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 467 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:467 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.10 Verfahrenstechnik: Allgemeines VZ AR 467 |
allfieldsSound |
10.1016/j.cej.2023.143400 doi (DE-627)ELV01014286X (ELSEVIER)S1385-8947(23)02131-9 DE-627 ger DE-627 rda eng 660 VZ 660 VZ 58.10 bkl Xu, Lijuan verfasserin aut Low-power, fast response simplified electrochromic device based on functionalized gel electrolyte 2023 nicht spezifiziert zzz rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier Metallo-supramolecular polymer (MEPE)-based thin film electrochromic devices (ECDs) have been considered to be a promising platform for portable electronics as their low cost, excellent redox properties, high optical contrast, and rich colors. However, poor cycle stability and slow response speed are serious bottlenecks for widespread commercial devices. Here, a gel electrolyte functionalized by the anodic active species p-benzoquinone (p-BQ) (GET-BQ) was reported. It has outstanding conductivity (∼4.62 mS cm−1) and transparency. Fe(Ⅱ)-MEPE-based ECDs incorporating the GET-BQ electrolyte (ECD-BQ) showed lower voltage operation (∼1.1 V), higher optical contrast (ca. ΔT ∼ 35.7%), faster response rate (tb ∼ 2.5 s, tc ∼ 0.3 s), and superb cycling durability (<1.7% ΔT loss after 1440 cycles) than those without p-BQ. Moreover, the charge transport kinetics of ECD-BQ were explored by the CV curve, in situ infrared spectroelectrochemical analysis, and electrochemical impedance spectroscopy. The charge transfer mechanism of electrochromic material and electrolytes in ECD-BQ offers a novel entry to design superior electrolytes for high-performance ECD. Functionalized gel electrolyte Cathodic active species Charge-transport kinetic Electrochromic device Li, Yangyang verfasserin aut Ji, Yuan verfasserin aut Zhang, Jichi verfasserin aut Shao, Lu verfasserin aut Zhang, Dawei verfasserin aut Ma, Lina verfasserin aut Gao, Guolin verfasserin (orcid)0000-0001-5177-9139 aut Jiang, Zaixing verfasserin aut Enthalten in The chemical engineering journal Amsterdam : Elsevier, 1997 467 Online-Ressource (DE-627)320500322 (DE-600)2012137-4 (DE-576)098330152 1873-3212 nnns volume:467 GBV_USEFLAG_U GBV_ELV SYSFLAG_U SSG-OLC-PHA GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_150 GBV_ILN_151 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2034 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2088 GBV_ILN_2106 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2470 GBV_ILN_2507 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4242 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 58.10 Verfahrenstechnik: Allgemeines VZ AR 467 |
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Xu, Lijuan @@aut@@ Li, Yangyang @@aut@@ Ji, Yuan @@aut@@ Zhang, Jichi @@aut@@ Shao, Lu @@aut@@ Zhang, Dawei @@aut@@ Ma, Lina @@aut@@ Gao, Guolin @@aut@@ Jiang, Zaixing @@aut@@ |
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Xu, Lijuan ddc 660 bkl 58.10 misc Functionalized gel electrolyte misc Cathodic active species misc Charge-transport kinetic misc Electrochromic device Low-power, fast response simplified electrochromic device based on functionalized gel electrolyte |
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660 VZ 58.10 bkl Low-power, fast response simplified electrochromic device based on functionalized gel electrolyte Functionalized gel electrolyte Cathodic active species Charge-transport kinetic Electrochromic device |
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ddc 660 bkl 58.10 misc Functionalized gel electrolyte misc Cathodic active species misc Charge-transport kinetic misc Electrochromic device |
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Low-power, fast response simplified electrochromic device based on functionalized gel electrolyte |
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Xu, Lijuan Li, Yangyang Ji, Yuan Zhang, Jichi Shao, Lu Zhang, Dawei Ma, Lina Gao, Guolin Jiang, Zaixing |
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low-power, fast response simplified electrochromic device based on functionalized gel electrolyte |
title_auth |
Low-power, fast response simplified electrochromic device based on functionalized gel electrolyte |
abstract |
Metallo-supramolecular polymer (MEPE)-based thin film electrochromic devices (ECDs) have been considered to be a promising platform for portable electronics as their low cost, excellent redox properties, high optical contrast, and rich colors. However, poor cycle stability and slow response speed are serious bottlenecks for widespread commercial devices. Here, a gel electrolyte functionalized by the anodic active species p-benzoquinone (p-BQ) (GET-BQ) was reported. It has outstanding conductivity (∼4.62 mS cm−1) and transparency. Fe(Ⅱ)-MEPE-based ECDs incorporating the GET-BQ electrolyte (ECD-BQ) showed lower voltage operation (∼1.1 V), higher optical contrast (ca. ΔT ∼ 35.7%), faster response rate (tb ∼ 2.5 s, tc ∼ 0.3 s), and superb cycling durability (<1.7% ΔT loss after 1440 cycles) than those without p-BQ. Moreover, the charge transport kinetics of ECD-BQ were explored by the CV curve, in situ infrared spectroelectrochemical analysis, and electrochemical impedance spectroscopy. The charge transfer mechanism of electrochromic material and electrolytes in ECD-BQ offers a novel entry to design superior electrolytes for high-performance ECD. |
abstractGer |
Metallo-supramolecular polymer (MEPE)-based thin film electrochromic devices (ECDs) have been considered to be a promising platform for portable electronics as their low cost, excellent redox properties, high optical contrast, and rich colors. However, poor cycle stability and slow response speed are serious bottlenecks for widespread commercial devices. Here, a gel electrolyte functionalized by the anodic active species p-benzoquinone (p-BQ) (GET-BQ) was reported. It has outstanding conductivity (∼4.62 mS cm−1) and transparency. Fe(Ⅱ)-MEPE-based ECDs incorporating the GET-BQ electrolyte (ECD-BQ) showed lower voltage operation (∼1.1 V), higher optical contrast (ca. ΔT ∼ 35.7%), faster response rate (tb ∼ 2.5 s, tc ∼ 0.3 s), and superb cycling durability (<1.7% ΔT loss after 1440 cycles) than those without p-BQ. Moreover, the charge transport kinetics of ECD-BQ were explored by the CV curve, in situ infrared spectroelectrochemical analysis, and electrochemical impedance spectroscopy. The charge transfer mechanism of electrochromic material and electrolytes in ECD-BQ offers a novel entry to design superior electrolytes for high-performance ECD. |
abstract_unstemmed |
Metallo-supramolecular polymer (MEPE)-based thin film electrochromic devices (ECDs) have been considered to be a promising platform for portable electronics as their low cost, excellent redox properties, high optical contrast, and rich colors. However, poor cycle stability and slow response speed are serious bottlenecks for widespread commercial devices. Here, a gel electrolyte functionalized by the anodic active species p-benzoquinone (p-BQ) (GET-BQ) was reported. It has outstanding conductivity (∼4.62 mS cm−1) and transparency. Fe(Ⅱ)-MEPE-based ECDs incorporating the GET-BQ electrolyte (ECD-BQ) showed lower voltage operation (∼1.1 V), higher optical contrast (ca. ΔT ∼ 35.7%), faster response rate (tb ∼ 2.5 s, tc ∼ 0.3 s), and superb cycling durability (<1.7% ΔT loss after 1440 cycles) than those without p-BQ. Moreover, the charge transport kinetics of ECD-BQ were explored by the CV curve, in situ infrared spectroelectrochemical analysis, and electrochemical impedance spectroscopy. The charge transfer mechanism of electrochromic material and electrolytes in ECD-BQ offers a novel entry to design superior electrolytes for high-performance ECD. |
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title_short |
Low-power, fast response simplified electrochromic device based on functionalized gel electrolyte |
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Li, Yangyang Ji, Yuan Zhang, Jichi Shao, Lu Zhang, Dawei Ma, Lina Gao, Guolin Jiang, Zaixing |
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|
score |
7.400275 |